Articles | Volume 13, issue 14
https://doi.org/10.5194/acp-13-6663-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-13-6663-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
15 Jul 2013
Research article |
| 15 Jul 2013
Kinetic regimes and limiting cases of gas uptake and heterogeneous reactions in atmospheric aerosols and clouds: a general classification scheme
T. Berkemeier
Faculty of Chemistry, Bielefeld University, Bielefeld, Germany
Institute for Atmospheric and Climate Science, ETH Zürich, Zürich, Switzerland
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
A. J. Huisman
Institute for Atmospheric and Climate Science, ETH Zürich, Zürich, Switzerland
now at: Department of Chemistry, Union College, Schenectady, NY, USA
M. Ammann
Laboratory of Radiochemistry and Environmental Chemistry, Paul Scherrer Institute, Villigen, Switzerland
M. Shiraiwa
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, California, USA
Faculty of Chemistry, Bielefeld University, Bielefeld, Germany
U. Pöschl
Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, Germany
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Cited
54 citations as recorded by crossref.
- Predicting Aerosol Reactivity Across Scales: from the Laboratory to the Atmosphere F. Houle et al. 10.1021/acs.est.8b04688
- Plasma–liquid interactions: a review and roadmap P. Bruggeman et al. 10.1088/0963-0252/25/5/053002
- The persistence of a proxy for cooking emissions in megacities: a kinetic study of the ozonolysis of self-assembled films by simultaneous small and wide angle X-ray scattering (SAXS/WAXS) and Raman microscopy A. Milsom et al. 10.1039/D0FD00088D
- Sustainability of Transient Kinetic Regimes and Origins of Death D. Zubarev & L. Pachón 10.1038/srep20562
- Technical note: Monte Carlo genetic algorithm (MCGA) for model analysis of multiphase chemical kinetics to determine transport and reaction rate coefficients using multiple experimental data sets T. Berkemeier et al. 10.5194/acp-17-8021-2017
- Importance of Unimolecular HO2 Elimination in the Heterogeneous OH Reaction of Highly Oxygenated Tartaric Acid Aerosol C. Cheng et al. 10.1021/acs.jpca.6b05289
- Quantifying the Role of the Relative Humidity-Dependent Physical State of Organic Particulate Matter in the Uptake of Semivolatile Organic Molecules Y. Han et al. 10.1021/acs.est.9b05354
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa 10.1021/cr500487s
- Heterogeneous reactions of mineral dust aerosol: implications for tropospheric oxidation capacity M. Tang et al. 10.5194/acp-17-11727-2017
- Oxidation of a model alkane aerosol by OH radical: the emergent nature of reactive uptake F. Houle et al. 10.1039/C4CP05093B
- Modelling non-equilibrium secondary organic aerosol formation and evaporation with the aerosol dynamics, gas- and particle-phase chemistry kinetic multilayer model ADCHAM P. Roldin et al. 10.5194/acp-14-7953-2014
- Shikimic acid ozonolysis kinetics of the transition from liquid aqueous solution to highly viscous glass S. Steimer et al. 10.1039/C5CP04544D
- Glass Formation Processes in Mixed Inorganic/Organic Aerosol Particles H. Dette & T. Koop 10.1021/jp5106967
- Understanding interactions of organic nitrates with the surface and bulk of organic films: implications for particle growth in the atmosphere A. Vander Wall et al. 10.1039/C8EM00348C
- Ozonolysis of Oleic Acid Aerosol Revisited: Multiphase Chemical Kinetics and Reaction Mechanisms T. Berkemeier et al. 10.1021/acsearthspacechem.1c00232
- Multiphase Chemical Kinetics of OH Radical Uptake by Molecular Organic Markers of Biomass Burning Aerosols: Humidity and Temperature Dependence, Surface Reaction, and Bulk Diffusion A. Arangio et al. 10.1021/jp510489z
- Kinetic modeling of formation and evaporation of secondary organic aerosol from NO<sub>3</sub> oxidation of pure and mixed monoterpenes T. Berkemeier et al. 10.5194/acp-20-15513-2020
- Reaction Mechanism of Ozone with Methane Flame Soot: Langmuir–Hinshelwood or Unimolecular Decomposition? V. Zelenov & E. Aparina 10.1134/S1990793121030143
- Influence of particle viscosity on mass transfer and heterogeneous ozonolysis kinetics in aqueous–sucrose–maleic acid aerosol F. Marshall et al. 10.1039/C8CP01666F
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. 10.1039/C6CP00634E
- Evidence for a kinetically controlled burying mechanism for growth of high viscosity secondary organic aerosol A. Vander Wall et al. 10.1039/C9EM00379G
- Modeling kinetic partitioning of secondary organic aerosol and size distribution dynamics: representing effects of volatility, phase state, and particle-phase reaction R. Zaveri et al. 10.5194/acp-14-5153-2014
- Enhanced Gas Uptake during α-Pinene Ozonolysis Points to a Burying Mechanism A. Vander Wall et al. 10.1021/acsearthspacechem.0c00163
- Uptake of Gas Phase Nitrous Acid onto Boundary Layer Soil Surfaces M. Donaldson et al. 10.1021/es404156a
- Glyoxal as a Potential Source of Highly Viscous Aerosol Particles J. Peters et al. 10.1021/acsearthspacechem.1c00245
- Comprehensive modeling study of ozonolysis of oleic acid aerosol based on real-time, online measurements of aerosol composition P. Gallimore et al. 10.1002/2016JD026221
- Plasma-driven solution electrolysis P. Bruggeman et al. 10.1063/5.0044261
- An efficient approach for treating composition-dependent diffusion within organic particles S. O'Meara et al. 10.5194/acp-17-10477-2017
- Glass-Forming Properties of 3-Methylbutane-1,2,3-tricarboxylic Acid and Its Mixtures with Water and Pinonic Acid H. Dette et al. 10.1021/jp505910w
- Interactions of Water with Mineral Dust Aerosol: Water Adsorption, Hygroscopicity, Cloud Condensation, and Ice Nucleation M. Tang et al. 10.1021/acs.chemrev.5b00529
- Physical state of 2-methylbutane-1,2,3,4-tetraol in pure and internally mixed aerosols J. Lessmeier et al. 10.5194/acp-18-15841-2018
- Compilation and evaluation of gas phase diffusion coefficients of reactive trace gases in the atmosphere: Volume 2. Diffusivities of organic compounds, pressure-normalised mean free paths, and average Knudsen numbers for gas uptake calculations M. Tang et al. 10.5194/acp-15-5585-2015
- Kinetics, mechanisms and ionic liquids in the uptake of n-butylamine onto low molecular weight dicarboxylic acids M. Fairhurst et al. 10.1039/C6CP08663B
- Size-dependent chemical ageing of oleic acid aerosol under dry and humidified conditions S. Al-Kindi et al. 10.5194/acp-16-15561-2016
- Visualizing reaction and diffusion in xanthan gum aerosol particles exposed to ozone P. Alpert et al. 10.1039/C9CP03731D
- Effects of Phase State and Phase Separation on Dimethylamine Uptake of Ammonium Sulfate and Ammonium Sulfate–Sucrose Mixed Particles W. DeRieux et al. 10.1021/acsearthspacechem.9b00142
- Influence of the coating level on the heterogeneous ozonolysis kinetics and product yields of chlorpyrifos ethyl adsorbed on sand particles A. El Masri et al. 10.1016/j.chemosphere.2016.09.036
- Condensation Kinetics of Water on Amorphous Aerosol Particles N. Rothfuss et al. 10.1021/acs.jpclett.8b01365
- Solid, Semisolid, and Liquid Phase States of Individual Submicrometer Particles Directly Probed Using Atomic Force Microscopy H. Lee et al. 10.1021/acs.analchem.7b02755
- The effect of viscosity and diffusion on the HO<sub>2</sub> uptake by sucrose and secondary organic aerosol particles P. Lakey et al. 10.5194/acp-16-13035-2016
- Molecular corridors and kinetic regimes in the multiphase chemical evolution of secondary organic aerosol M. Shiraiwa et al. 10.5194/acp-14-8323-2014
- The influence of physical state on shikimic acid ozonolysis: a case for in situ microspectroscopy S. Steimer et al. 10.5194/acp-14-10761-2014
- Reactive oxygen species formed in aqueous mixtures of secondary organic aerosols and mineral dust influencing cloud chemistry and public health in the Anthropocene H. Tong et al. 10.1039/C7FD00023E
- Heterogeneous OH Oxidation, Shielding Effects, and Implications for the Atmospheric Fate of Terbuthylazine and Other Pesticides J. Socorro et al. 10.1021/acs.est.7b04307
- Changes in Reactivity as Chemistry Becomes Confined to an Interface. The Case of Free Radical Oxidation of C30H62 Alkane by OH F. Houle et al. 10.1021/acs.jpclett.8b00172
- Effects of Relative Humidity and Particle Phase Water on the Heterogeneous OH Oxidation of 2-Methylglutaric Acid Aqueous Droplets M. Chim et al. 10.1021/acs.jpca.6b11606
- Multiphase Kinetic Multilayer Model Interfaces for Simulating Surface and Bulk Chemistry for Environmental and Atmospheric Chemistry Teaching A. Hua et al. 10.1021/acs.jchemed.1c00931
- Chemical Reactivity and Liquid/Nonliquid States of Secondary Organic Material Y. Li et al. 10.1021/acs.est.5b03392
- Protein Cross-Linking and Oligomerization through Dityrosine Formation upon Exposure to Ozone C. Kampf et al. 10.1021/acs.est.5b02902
- Introductory lecture: atmospheric chemistry in the Anthropocene B. Finlayson-Pitts 10.1039/C7FD00161D
- Hydroxyl radicals from secondary organic aerosol decomposition in water H. Tong et al. 10.5194/acp-16-1761-2016
- Organic Nitrate Contribution to New Particle Formation and Growth in Secondary Organic Aerosols from α-Pinene Ozonolysis T. Berkemeier et al. 10.1021/acs.est.6b00961
- Chemical kinetics of multiphase reactions between ozone and human skin lipids: Implications for indoor air quality and health effects P. Lakey et al. 10.1111/ina.12360
- Compositional evolution of particle-phase reaction products and water in the heterogeneous OH oxidation of model aqueous organic aerosols M. Chim et al. 10.5194/acp-17-14415-2017
54 citations as recorded by crossref.
- Predicting Aerosol Reactivity Across Scales: from the Laboratory to the Atmosphere F. Houle et al. 10.1021/acs.est.8b04688
- Plasma–liquid interactions: a review and roadmap P. Bruggeman et al. 10.1088/0963-0252/25/5/053002
- The persistence of a proxy for cooking emissions in megacities: a kinetic study of the ozonolysis of self-assembled films by simultaneous small and wide angle X-ray scattering (SAXS/WAXS) and Raman microscopy A. Milsom et al. 10.1039/D0FD00088D
- Sustainability of Transient Kinetic Regimes and Origins of Death D. Zubarev & L. Pachón 10.1038/srep20562
- Technical note: Monte Carlo genetic algorithm (MCGA) for model analysis of multiphase chemical kinetics to determine transport and reaction rate coefficients using multiple experimental data sets T. Berkemeier et al. 10.5194/acp-17-8021-2017
- Importance of Unimolecular HO2 Elimination in the Heterogeneous OH Reaction of Highly Oxygenated Tartaric Acid Aerosol C. Cheng et al. 10.1021/acs.jpca.6b05289
- Quantifying the Role of the Relative Humidity-Dependent Physical State of Organic Particulate Matter in the Uptake of Semivolatile Organic Molecules Y. Han et al. 10.1021/acs.est.9b05354
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa 10.1021/cr500487s
- Heterogeneous reactions of mineral dust aerosol: implications for tropospheric oxidation capacity M. Tang et al. 10.5194/acp-17-11727-2017
- Oxidation of a model alkane aerosol by OH radical: the emergent nature of reactive uptake F. Houle et al. 10.1039/C4CP05093B
- Modelling non-equilibrium secondary organic aerosol formation and evaporation with the aerosol dynamics, gas- and particle-phase chemistry kinetic multilayer model ADCHAM P. Roldin et al. 10.5194/acp-14-7953-2014
- Shikimic acid ozonolysis kinetics of the transition from liquid aqueous solution to highly viscous glass S. Steimer et al. 10.1039/C5CP04544D
- Glass Formation Processes in Mixed Inorganic/Organic Aerosol Particles H. Dette & T. Koop 10.1021/jp5106967
- Understanding interactions of organic nitrates with the surface and bulk of organic films: implications for particle growth in the atmosphere A. Vander Wall et al. 10.1039/C8EM00348C
- Ozonolysis of Oleic Acid Aerosol Revisited: Multiphase Chemical Kinetics and Reaction Mechanisms T. Berkemeier et al. 10.1021/acsearthspacechem.1c00232
- Multiphase Chemical Kinetics of OH Radical Uptake by Molecular Organic Markers of Biomass Burning Aerosols: Humidity and Temperature Dependence, Surface Reaction, and Bulk Diffusion A. Arangio et al. 10.1021/jp510489z
- Kinetic modeling of formation and evaporation of secondary organic aerosol from NO<sub>3</sub> oxidation of pure and mixed monoterpenes T. Berkemeier et al. 10.5194/acp-20-15513-2020
- Reaction Mechanism of Ozone with Methane Flame Soot: Langmuir–Hinshelwood or Unimolecular Decomposition? V. Zelenov & E. Aparina 10.1134/S1990793121030143
- Influence of particle viscosity on mass transfer and heterogeneous ozonolysis kinetics in aqueous–sucrose–maleic acid aerosol F. Marshall et al. 10.1039/C8CP01666F
- Ozone uptake on glassy, semi-solid and liquid organic matter and the role of reactive oxygen intermediates in atmospheric aerosol chemistry T. Berkemeier et al. 10.1039/C6CP00634E
- Evidence for a kinetically controlled burying mechanism for growth of high viscosity secondary organic aerosol A. Vander Wall et al. 10.1039/C9EM00379G
- Modeling kinetic partitioning of secondary organic aerosol and size distribution dynamics: representing effects of volatility, phase state, and particle-phase reaction R. Zaveri et al. 10.5194/acp-14-5153-2014
- Enhanced Gas Uptake during α-Pinene Ozonolysis Points to a Burying Mechanism A. Vander Wall et al. 10.1021/acsearthspacechem.0c00163
- Uptake of Gas Phase Nitrous Acid onto Boundary Layer Soil Surfaces M. Donaldson et al. 10.1021/es404156a
- Glyoxal as a Potential Source of Highly Viscous Aerosol Particles J. Peters et al. 10.1021/acsearthspacechem.1c00245
- Comprehensive modeling study of ozonolysis of oleic acid aerosol based on real-time, online measurements of aerosol composition P. Gallimore et al. 10.1002/2016JD026221
- Plasma-driven solution electrolysis P. Bruggeman et al. 10.1063/5.0044261
- An efficient approach for treating composition-dependent diffusion within organic particles S. O'Meara et al. 10.5194/acp-17-10477-2017
- Glass-Forming Properties of 3-Methylbutane-1,2,3-tricarboxylic Acid and Its Mixtures with Water and Pinonic Acid H. Dette et al. 10.1021/jp505910w
- Interactions of Water with Mineral Dust Aerosol: Water Adsorption, Hygroscopicity, Cloud Condensation, and Ice Nucleation M. Tang et al. 10.1021/acs.chemrev.5b00529
- Physical state of 2-methylbutane-1,2,3,4-tetraol in pure and internally mixed aerosols J. Lessmeier et al. 10.5194/acp-18-15841-2018
- Compilation and evaluation of gas phase diffusion coefficients of reactive trace gases in the atmosphere: Volume 2. Diffusivities of organic compounds, pressure-normalised mean free paths, and average Knudsen numbers for gas uptake calculations M. Tang et al. 10.5194/acp-15-5585-2015
- Kinetics, mechanisms and ionic liquids in the uptake of n-butylamine onto low molecular weight dicarboxylic acids M. Fairhurst et al. 10.1039/C6CP08663B
- Size-dependent chemical ageing of oleic acid aerosol under dry and humidified conditions S. Al-Kindi et al. 10.5194/acp-16-15561-2016
- Visualizing reaction and diffusion in xanthan gum aerosol particles exposed to ozone P. Alpert et al. 10.1039/C9CP03731D
- Effects of Phase State and Phase Separation on Dimethylamine Uptake of Ammonium Sulfate and Ammonium Sulfate–Sucrose Mixed Particles W. DeRieux et al. 10.1021/acsearthspacechem.9b00142
- Influence of the coating level on the heterogeneous ozonolysis kinetics and product yields of chlorpyrifos ethyl adsorbed on sand particles A. El Masri et al. 10.1016/j.chemosphere.2016.09.036
- Condensation Kinetics of Water on Amorphous Aerosol Particles N. Rothfuss et al. 10.1021/acs.jpclett.8b01365
- Solid, Semisolid, and Liquid Phase States of Individual Submicrometer Particles Directly Probed Using Atomic Force Microscopy H. Lee et al. 10.1021/acs.analchem.7b02755
- The effect of viscosity and diffusion on the HO<sub>2</sub> uptake by sucrose and secondary organic aerosol particles P. Lakey et al. 10.5194/acp-16-13035-2016
- Molecular corridors and kinetic regimes in the multiphase chemical evolution of secondary organic aerosol M. Shiraiwa et al. 10.5194/acp-14-8323-2014
- The influence of physical state on shikimic acid ozonolysis: a case for in situ microspectroscopy S. Steimer et al. 10.5194/acp-14-10761-2014
- Reactive oxygen species formed in aqueous mixtures of secondary organic aerosols and mineral dust influencing cloud chemistry and public health in the Anthropocene H. Tong et al. 10.1039/C7FD00023E
- Heterogeneous OH Oxidation, Shielding Effects, and Implications for the Atmospheric Fate of Terbuthylazine and Other Pesticides J. Socorro et al. 10.1021/acs.est.7b04307
- Changes in Reactivity as Chemistry Becomes Confined to an Interface. The Case of Free Radical Oxidation of C30H62 Alkane by OH F. Houle et al. 10.1021/acs.jpclett.8b00172
- Effects of Relative Humidity and Particle Phase Water on the Heterogeneous OH Oxidation of 2-Methylglutaric Acid Aqueous Droplets M. Chim et al. 10.1021/acs.jpca.6b11606
- Multiphase Kinetic Multilayer Model Interfaces for Simulating Surface and Bulk Chemistry for Environmental and Atmospheric Chemistry Teaching A. Hua et al. 10.1021/acs.jchemed.1c00931
- Chemical Reactivity and Liquid/Nonliquid States of Secondary Organic Material Y. Li et al. 10.1021/acs.est.5b03392
- Protein Cross-Linking and Oligomerization through Dityrosine Formation upon Exposure to Ozone C. Kampf et al. 10.1021/acs.est.5b02902
- Introductory lecture: atmospheric chemistry in the Anthropocene B. Finlayson-Pitts 10.1039/C7FD00161D
- Hydroxyl radicals from secondary organic aerosol decomposition in water H. Tong et al. 10.5194/acp-16-1761-2016
- Organic Nitrate Contribution to New Particle Formation and Growth in Secondary Organic Aerosols from α-Pinene Ozonolysis T. Berkemeier et al. 10.1021/acs.est.6b00961
- Chemical kinetics of multiphase reactions between ozone and human skin lipids: Implications for indoor air quality and health effects P. Lakey et al. 10.1111/ina.12360
- Compositional evolution of particle-phase reaction products and water in the heterogeneous OH oxidation of model aqueous organic aerosols M. Chim et al. 10.5194/acp-17-14415-2017
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