Articles | Volume 12, issue 15
Atmos. Chem. Phys., 12, 7165–7185, 2012

Special issue: The Pan European Gas-Aerosols Climate Interaction Study...

Atmos. Chem. Phys., 12, 7165–7185, 2012

Research article 07 Aug 2012

Research article | 07 Aug 2012

The direct effect of aerosols on solar radiation over the broader Mediterranean basin

C. D. Papadimas1, N. Hatzianastassiou1, C. Matsoukas2, M. Kanakidou3,4, N. Mihalopoulos3,4, and I. Vardavas5 C. D. Papadimas et al.
  • 1Laboratory of Meteorology, Department of Physics, University of Ioannina, 45110 Ioannina, Greece
  • 2Department of Environment, University of the Aegean, 81100 Mytilene, Greece
  • 3Environmental Chemical Processes Laboratory, Department of Chemistry, University of Crete, P.O. Box 2208, 71003 Heraklion, Crete, Greece
  • 4Institute of Chemical Engineering and High Temperature Chemical Processes (ICE-HT), Foundation for Research and Technology Hellas (FORTH), Patras, 26504, Greece
  • 5Department of Physics, University of Crete, 71110 Heraklion, Crete, Greece

Abstract. For the first time, the direct radiative effect (DRE) of aerosols on solar radiation is computed over the entire Mediterranean basin, one of the most climatically sensitive world regions, using a deterministic spectral radiation transfer model (RTM). The DRE effects on the outgoing shortwave radiation at the top of atmosphere (TOA), DRETOA, on the absorption of solar radiation in the atmospheric column, DREatm, and on the downward and absorbed surface solar radiation (SSR), DREsurf and DREnetsurf, respectively, are computed separately. The model uses input data for the period 2000–2007 for various surface and atmospheric parameters, taken from satellite (International Satellite Cloud Climatology Project, ISCCP-D2), Global Reanalysis projects (National Centers for Environmental Prediction – National Center for Atmospheric Research, NCEP/NCAR), and other global databases. The spectral aerosol optical properties (aerosol optical depth, AOD, asymmetry parameter, gaer and single scattering albedo, ωaer), are taken from the MODerate resolution Imaging Spectroradiometer (MODIS) of NASA (National Aeronautics and Space Administration) and they are supplemented by the Global Aerosol Data Set (GADS). The model SSR fluxes have been successfully validated against measurements from 80 surface stations of the Global Energy Balance Archive (GEBA) covering the period 2000–2007.

A planetary cooling is found above the Mediterranean on an annual basis (regional mean DRETOA = −2.4 W m−2). Although a planetary cooling is found over most of the region, of up to −7 W m−2, large positive DRETOA values (up to +25 W m−2) are found over North Africa, indicating a strong planetary warming, and a weaker warming over the Alps (+0.5 W m−2). Aerosols are found to increase the absorption of solar radiation in the atmospheric column over the region (DREatm = +11.1 W m−2) and to decrease SSR (DREsurf = −16.5 W m−2 and DREnetsurf−13.5 W m−2) inducing thus significant atmospheric warming and surface radiative cooling. The calculated seasonal and monthly DREs are even larger, reaching −25.4 W m−2 (for DREsurf). Within the range of observed natural or anthropogenic variability of aerosol optical properties, AOD seems to be the main responsible parameter for modifications of regional aerosol radiative effects, which are found to be quasi-linearly dependent on AOD, ωaer and gaer.

Final-revised paper