Articles | Volume 12, issue 14
https://doi.org/10.5194/acp-12-6323-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-12-6323-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Identification and characterization of aging products in the glyoxal/ammonium sulfate system – implications for light-absorbing material in atmospheric aerosols
C. J. Kampf
Institute for Inorganic and Analytical Chemistry, Johannes Gutenberg-University Mainz, 55128 Mainz, Germany
R. Jakob
Institute for Inorganic and Analytical Chemistry, Johannes Gutenberg-University Mainz, 55128 Mainz, Germany
T. Hoffmann
Institute for Inorganic and Analytical Chemistry, Johannes Gutenberg-University Mainz, 55128 Mainz, Germany
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Cited
146 citations as recorded by crossref.
- High Pressure Inside Nanometer-Sized Particles Influences the Rate and Products of Chemical Reactions M. Riva et al.
- Enhancement in Particulate Organic Nitrogen and Light Absorption of Humic-Like Substances over Tibetan Plateau Due to Long-Range Transported Biomass Burning Emissions Y. Wang et al.
- Quantification of Imidazole Compounds in Ambient Aerosols at Suburban and Forest Sites in Western Japan Y. Takao et al.
- Relative Humidity Modulates the Physicochemical Processing of Secondary Brown Carbon Formation from Nighttime Oxidation of Furan and Pyrrole K. Chen et al.
- Photoinduced Transformation in Glyoxal- and Methylglyoxal-Ammonium Solutions: Role of Photolysis and Photosensitization J. Gu et al.
- Effective Henry’s Law Partitioning and the Salting Constant of Glyoxal in Aerosols Containing Sulfate C. Kampf et al.
- Global modeling study of soluble organic nitrogen from open biomass burning A. Ito et al.
- Brown Carbon Formation by Aqueous-Phase Reactions of Glycolaldehyde and Methylamine C. Carthy et al.
- Online and offline mass spectrometric study of the impact of oxidation and ageing on glyoxal chemistry and uptake onto ammonium sulfate aerosols J. Hamilton et al.
- Separation and detection of aqueous atmospheric aerosol mimics using supercritical fluid chromatography–mass spectrometry D. Grace et al.
- Spectroscopic and Photochemical Properties of Secondary Brown Carbon from Aqueous Reactions of Methylglyoxal A. Harrison et al.
- Reaction of Glyoxal and Ammonium as a Potential Contributor to Protein-like Fluorescence in Atmospheric Measurements A. Harrison et al.
- Response of imidazole-containing particles to emission reduction policies in China: Insights from observations in a megacity in the Sichuan Basin C. Chen et al.
- pH Dependence of the Imidazole-2-carboxaldehyde Hydration Equilibrium: Implications for Atmospheric Light Absorbance J. Ackendorf et al.
- Theoretical analysis of glyoxal condensation with ammonia in aqueous solution V. Tuguldurova et al.
- Characterization of Imidazole Compounds in Aqueous Secondary Organic Aerosol Generated from Evaporation of Droplets Containing Pyruvaldehyde and Inorganic Ammonium X. Lin et al.
- Contribution of Carbonyl Chromophores in Secondary Brown Carbon from Nighttime Oxidation of Unsaturated Heterocyclic Volatile Organic Compounds K. Chen et al.
- Aqueous Reaction of Dicarbonyls with Ammonia as a Potential Source of Organic Nitrogen in Airborne Nanoparticles C. Stangl & M. Johnston
- Photochemical processing of aqueous atmospheric brown carbon R. Zhao et al.
- A smog chamber study coupling a photoionization aerosol electron/ion spectrometer to VUV synchrotron radiation: organic and inorganic-organic mixed aerosol analysis M. Baeza-Romero et al.
- Seasonal variations in the production of singlet oxygen and organic triplet excited states in aqueous PM2.5 in Hong Kong SAR, South China Y. Lyu et al.
- Evidence for the Formation of Imidazole from Carbonyls and Reduced Nitrogen Species at the Individual Particle Level in the Ambient Atmosphere X. Lian et al.
- Online Speciation of Glyoxal Multiphase Reactions on Deliquesced Ammonium Sulfate Particles N. Brun et al.
- Formation mechanisms and yields of small imidazoles from reactions of glyoxal with NH4+ in water at neutral pH A. Maxut et al.
- A new method for the determination of imidazole-like brown carbons using gas chromatography-mass spectrometry P. Chen et al.
- Reprint of "How do components of real cloud water affect aqueous pyruvate oxidation?" A. Boris et al.
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- Substantial organic impurities at the surface of synthetic ammonium sulfate particles J. Wu et al.
- Comparison of aqueous secondary organic aerosol (aqSOA) product distributions from guaiacol oxidation by non-phenolic and phenolic methoxybenzaldehydes as photosensitizers in the absence and presence of ammonium nitrate B. Go et al.
- Seasonal variations of imidazoles in urban areas of Beijing and Guangzhou, China by single particle mass spectrometry X. Lian et al.
- Influence of NH3 on secondary organic aerosols from the ozonolysis and photooxidation of α-pinene in a flow reactor Z. Babar et al.
- Effect of Solar Radiation on the Optical Properties and Molecular Composition of Laboratory Proxies of Atmospheric Brown Carbon H. Lee et al.
- Optical properties and aging of light-absorbing secondary organic aerosol J. Liu et al.
- Seasonal variability of nitroaromatic compounds in ambient aerosols: Mass size distribution, possible sources and contribution to water-soluble brown carbon light absorption S. Frka et al.
- Characterization of Chromophoric Water-Soluble Organic Matter in Urban, Forest, and Marine Aerosols by HR-ToF-AMS Analysis and Excitation–Emission Matrix Spectroscopy Q. Chen et al.
- Aqueous-Phase Production of Secondary Organic Aerosols from Oxidation of Dibenzothiophene (DBT) Y. Liu et al.
- Revisiting the reaction of dicarbonyls in aerosol proxy solutions containing ammonia: the case of butenedial J. Hensley et al.
- Catalysis of Ferric Ions and Ferrous Ions on the Reaction of Methylglyoxal and Ammonium Sulfate J. Yang et al.
- Glyoxal as a Potential Source of Highly Viscous Aerosol Particles J. Peters et al.
- Surface Formation Pathway of Nitrogen- and Sulfur-Containing Organic Compounds on Ammonium Sulfate J. Chen et al.
- Atmospheric Processing of Particulate Imidazole Compounds Driven by Photochemistry X. Hu et al.
- Optical properties investigation of the reactions between methylglyoxal and glycine/ammonium sulfate Y. Gao & Y. Zhang
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al.
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa
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- Reactive Uptake of Glyoxal by Ammonium-Containing Salt Particles as a Function of Relative Humidity M. Gen et al.
- Experimental study on the imidazoles of aqueous secondary organic aerosol formed from reaction of methylglyoxal and ammonium sulphate M. Zhu et al.
- The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges B. Nozière et al.
- Effects of inorganic seed aerosols on the particulate products of aged 1,3,5-trimethylbenzene secondary organic aerosol M. Huang et al.
- How do components of real cloud water affect aqueous pyruvate oxidation? A. Boris et al.
- A time-resolved study of the multiphase chemistry of excited carbonyls: Imidazole-2-carboxaldehyde and halides L. Tinel et al.
- Light-Absorbing Oligomer Formation in Secondary Organic Aerosol from Reactive Uptake of Isoprene Epoxydiols Y. Lin et al.
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- Surfactant Effects in Irradiated, Hanging-Droplet, Aqueous-Phase Glyoxal/Ammonium Sulfate Aerosol Mimic Systems D. Fertil et al.
- OH-Initiated Oxidation of Imidazoles in Tropospheric Aqueous-Phase Chemistry T. Felber et al.
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- Tropospheric Aqueous-Phase Chemistry: Kinetics, Mechanisms, and Its Coupling to a Changing Gas Phase H. Herrmann et al.
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- Maillard Chemistry in Clouds and Aqueous Aerosol As a Source of Atmospheric Humic-Like Substances L. Hawkins et al.
- Radical-Initiated Brown Carbon Formation in Sunlit Carbonyl–Amine–Ammonium Sulfate Mixtures and Aqueous Aerosol Particles N. Jimenez et al.
- Hydration, Orientation, and Conformation of Methylglyoxal at the Air–Water Interface S. Wren et al.
- No evidence for brown carbon formation in ambient particles undergoing atmospherically relevant drying V. Pratap et al.
- First Quantification of Imidazoles in Ambient Aerosol Particles: Potential Photosensitizers, Brown Carbon Constituents, and Hazardous Components M. Teich et al.
- Comprehensive spectral analysis of reaction of three aldehydes with ammonium sulfate and glycine Y. Gao et al.
- Diol it up: The influence of NaCl on methylglyoxal surface adsorption and hydration state at the air–water interface B. Gordon et al.
- UV/Vis and IRMPD Spectroscopic Analysis of the Absorption Properties of Methylglyoxal Brown Carbon L. Vo et al.
- Contributions of nitrated aromatic compounds to the light absorption of water-soluble and particulate brown carbon in different atmospheric environments in Germany and China M. Teich et al.
- Measurement report: Brown carbon aerosol in polluted urban air of the North China Plain – day–night differences in the chromophores and optical properties Y. Gong et al.
- Mass spectrometric study of aged benzene secondary organic aerosol in the presence of dry ammonium sulfate M. Huang et al.
- Glyoxal Induced Atmospheric Photosensitized Chemistry Leading to Organic Aerosol Growth S. Rossignol et al.
- Seasonal Variations of Imidazoles in Urban Areas of Beijing and Guangzhou, China by Single Particle Mass Spectrometry X. Lian et al.
- Brown Carbon Formation by Aqueous-Phase Carbonyl Compound Reactions with Amines and Ammonium Sulfate M. Powelson et al.
- In Situ Surface Tension Measurements of Hanging Droplet Methylglyoxal/Ammonium Sulfate Aerosol Mimics under Photooxidative Conditions T. Beier et al.
- High-Resolution Fluorescence Spectra of Airborne Biogenic Secondary Organic Aerosols: Comparisons to Primary Biological Aerosol Particles and Implications for Single-Particle Measurements M. Zhang et al.
- Photochemical Reactions of Glyoxal during Particulate Ammonium Nitrate Photolysis: Brown Carbon Formation, Enhanced Glyoxal Decay, and Organic Phase Formation R. Zhang et al.
- Formation of Light Absorbing Organo-Nitrogen Species from Evaporation of Droplets Containing Glyoxal and Ammonium Sulfate A. Lee et al.
- Chemical Composition and Reaction Mechanisms for Aged p‐Xylene Secondary Organic Aerosol in the Presence of Ammonia J. Xu et al.
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- Revealing Brown Carbon Chromophores Produced in Reactions of Methylglyoxal with Ammonium Sulfate P. Lin et al.
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- Organic matrix effects on the formation of light-absorbing compounds from α-dicarbonyls in aqueous salt solution G. Drozd & V. McNeill
- pH-Dependent Kinetics of Imidazole Production in Aqueous Glyoxal/Ammonium Sulfate Microdroplets M. Marracci & C. Murray
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- Chemical analysis of particulate products of aged 1,3,5-trimethylbenzene secondary organic aerosol in the presence of ammonia M. Huang et al.
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146 citations as recorded by crossref.
- High Pressure Inside Nanometer-Sized Particles Influences the Rate and Products of Chemical Reactions M. Riva et al.
- Enhancement in Particulate Organic Nitrogen and Light Absorption of Humic-Like Substances over Tibetan Plateau Due to Long-Range Transported Biomass Burning Emissions Y. Wang et al.
- Quantification of Imidazole Compounds in Ambient Aerosols at Suburban and Forest Sites in Western Japan Y. Takao et al.
- Relative Humidity Modulates the Physicochemical Processing of Secondary Brown Carbon Formation from Nighttime Oxidation of Furan and Pyrrole K. Chen et al.
- Photoinduced Transformation in Glyoxal- and Methylglyoxal-Ammonium Solutions: Role of Photolysis and Photosensitization J. Gu et al.
- Effective Henry’s Law Partitioning and the Salting Constant of Glyoxal in Aerosols Containing Sulfate C. Kampf et al.
- Global modeling study of soluble organic nitrogen from open biomass burning A. Ito et al.
- Brown Carbon Formation by Aqueous-Phase Reactions of Glycolaldehyde and Methylamine C. Carthy et al.
- Online and offline mass spectrometric study of the impact of oxidation and ageing on glyoxal chemistry and uptake onto ammonium sulfate aerosols J. Hamilton et al.
- Separation and detection of aqueous atmospheric aerosol mimics using supercritical fluid chromatography–mass spectrometry D. Grace et al.
- Spectroscopic and Photochemical Properties of Secondary Brown Carbon from Aqueous Reactions of Methylglyoxal A. Harrison et al.
- Reaction of Glyoxal and Ammonium as a Potential Contributor to Protein-like Fluorescence in Atmospheric Measurements A. Harrison et al.
- Response of imidazole-containing particles to emission reduction policies in China: Insights from observations in a megacity in the Sichuan Basin C. Chen et al.
- pH Dependence of the Imidazole-2-carboxaldehyde Hydration Equilibrium: Implications for Atmospheric Light Absorbance J. Ackendorf et al.
- Theoretical analysis of glyoxal condensation with ammonia in aqueous solution V. Tuguldurova et al.
- Characterization of Imidazole Compounds in Aqueous Secondary Organic Aerosol Generated from Evaporation of Droplets Containing Pyruvaldehyde and Inorganic Ammonium X. Lin et al.
- Contribution of Carbonyl Chromophores in Secondary Brown Carbon from Nighttime Oxidation of Unsaturated Heterocyclic Volatile Organic Compounds K. Chen et al.
- Aqueous Reaction of Dicarbonyls with Ammonia as a Potential Source of Organic Nitrogen in Airborne Nanoparticles C. Stangl & M. Johnston
- Photochemical processing of aqueous atmospheric brown carbon R. Zhao et al.
- A smog chamber study coupling a photoionization aerosol electron/ion spectrometer to VUV synchrotron radiation: organic and inorganic-organic mixed aerosol analysis M. Baeza-Romero et al.
- Seasonal variations in the production of singlet oxygen and organic triplet excited states in aqueous PM2.5 in Hong Kong SAR, South China Y. Lyu et al.
- Evidence for the Formation of Imidazole from Carbonyls and Reduced Nitrogen Species at the Individual Particle Level in the Ambient Atmosphere X. Lian et al.
- Online Speciation of Glyoxal Multiphase Reactions on Deliquesced Ammonium Sulfate Particles N. Brun et al.
- Formation mechanisms and yields of small imidazoles from reactions of glyoxal with NH4+ in water at neutral pH A. Maxut et al.
- A new method for the determination of imidazole-like brown carbons using gas chromatography-mass spectrometry P. Chen et al.
- Reprint of "How do components of real cloud water affect aqueous pyruvate oxidation?" A. Boris et al.
- Formation of aqueous-phase secondary organic aerosols from glycolaldehyde and ammonium sulfate/amines: A kinetic and mechanistic study Y. Yi et al.
- Secondary brown carbon formation via the dicarbonyl imine pathway: nitrogen heterocycle formation and synergistic effects C. Kampf et al.
- Insights into high concentrations of particle-bound imidazoles in the background atmosphere of southern China: Potential sources and influencing factors C. He et al.
- Substantial organic impurities at the surface of synthetic ammonium sulfate particles J. Wu et al.
- Comparison of aqueous secondary organic aerosol (aqSOA) product distributions from guaiacol oxidation by non-phenolic and phenolic methoxybenzaldehydes as photosensitizers in the absence and presence of ammonium nitrate B. Go et al.
- Seasonal variations of imidazoles in urban areas of Beijing and Guangzhou, China by single particle mass spectrometry X. Lian et al.
- Influence of NH3 on secondary organic aerosols from the ozonolysis and photooxidation of α-pinene in a flow reactor Z. Babar et al.
- Effect of Solar Radiation on the Optical Properties and Molecular Composition of Laboratory Proxies of Atmospheric Brown Carbon H. Lee et al.
- Optical properties and aging of light-absorbing secondary organic aerosol J. Liu et al.
- Seasonal variability of nitroaromatic compounds in ambient aerosols: Mass size distribution, possible sources and contribution to water-soluble brown carbon light absorption S. Frka et al.
- Characterization of Chromophoric Water-Soluble Organic Matter in Urban, Forest, and Marine Aerosols by HR-ToF-AMS Analysis and Excitation–Emission Matrix Spectroscopy Q. Chen et al.
- Aqueous-Phase Production of Secondary Organic Aerosols from Oxidation of Dibenzothiophene (DBT) Y. Liu et al.
- Revisiting the reaction of dicarbonyls in aerosol proxy solutions containing ammonia: the case of butenedial J. Hensley et al.
- Catalysis of Ferric Ions and Ferrous Ions on the Reaction of Methylglyoxal and Ammonium Sulfate J. Yang et al.
- Glyoxal as a Potential Source of Highly Viscous Aerosol Particles J. Peters et al.
- Surface Formation Pathway of Nitrogen- and Sulfur-Containing Organic Compounds on Ammonium Sulfate J. Chen et al.
- Atmospheric Processing of Particulate Imidazole Compounds Driven by Photochemistry X. Hu et al.
- Optical properties investigation of the reactions between methylglyoxal and glycine/ammonium sulfate Y. Gao & Y. Zhang
- Aging of Atmospheric Brown Carbon Aerosol R. Hems et al.
- Multiphase Chemistry at the Atmosphere–Biosphere Interface Influencing Climate and Public Health in the Anthropocene U. Pöschl & M. Shiraiwa
- A comparative study on the formation of nitrogen-containing organic compounds in cloud droplets and aerosol particles G. Zhang et al.
- Speciation of Nitrogen-Bearing Species Using Negative and Positive Secondary Ion Spectra with Nano Secondary Ion Mass Spectrometry K. Li et al.
- Reactive Uptake of Glyoxal by Ammonium-Containing Salt Particles as a Function of Relative Humidity M. Gen et al.
- Experimental study on the imidazoles of aqueous secondary organic aerosol formed from reaction of methylglyoxal and ammonium sulphate M. Zhu et al.
- The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges B. Nozière et al.
- Effects of inorganic seed aerosols on the particulate products of aged 1,3,5-trimethylbenzene secondary organic aerosol M. Huang et al.
- How do components of real cloud water affect aqueous pyruvate oxidation? A. Boris et al.
- A time-resolved study of the multiphase chemistry of excited carbonyls: Imidazole-2-carboxaldehyde and halides L. Tinel et al.
- Light-Absorbing Oligomer Formation in Secondary Organic Aerosol from Reactive Uptake of Isoprene Epoxydiols Y. Lin et al.
- Separation and quantification of imidazoles in atmospheric particles using LC–Orbitrap‐MS M. Teich et al.
- Chemistry of Atmospheric Brown Carbon A. Laskin et al.
- Surfactant Effects in Irradiated, Hanging-Droplet, Aqueous-Phase Glyoxal/Ammonium Sulfate Aerosol Mimic Systems D. Fertil et al.
- OH-Initiated Oxidation of Imidazoles in Tropospheric Aqueous-Phase Chemistry T. Felber et al.
- Aqueous-Phase Photoreactions of Mixed Aromatic Carbonyl Photosensitizers Yield More Oxygenated, Oxidized, and less Light-Absorbing Secondary Organic Aerosol (SOA) than Single Systems B. Go et al.
- Research progress on secondary formation, photosensitive reaction mechanism and human health effects of chromophoric brown carbon B. Chen et al.
- Airborne Microbial Aerosol Detection by Combining Single Particle Mass Spectrometry and a Fluorescent Aerosol Particle Sizer H. Lu et al.
- Halogen activation and radical cycling initiated by imidazole-2-carboxaldehyde photochemistry P. Corral Arroyo et al.
- Acidity and the multiphase chemistry of atmospheric aqueous particles and clouds A. Tilgner et al.
- Kinetics, Products, and Brown Carbon Formation by Aqueous-Phase Reactions of Glycolaldehyde with Atmospheric Amines and Ammonium Sulfate A. Rodriguez et al.
- Tropospheric Aqueous-Phase Chemistry: Kinetics, Mechanisms, and Its Coupling to a Changing Gas Phase H. Herrmann et al.
- Aqueous-phase formation of N-containing secondary organic compounds affected by the ionic strength Y. Gan et al.
- Maillard Chemistry in Clouds and Aqueous Aerosol As a Source of Atmospheric Humic-Like Substances L. Hawkins et al.
- Radical-Initiated Brown Carbon Formation in Sunlit Carbonyl–Amine–Ammonium Sulfate Mixtures and Aqueous Aerosol Particles N. Jimenez et al.
- Hydration, Orientation, and Conformation of Methylglyoxal at the Air–Water Interface S. Wren et al.
- No evidence for brown carbon formation in ambient particles undergoing atmospherically relevant drying V. Pratap et al.
- First Quantification of Imidazoles in Ambient Aerosol Particles: Potential Photosensitizers, Brown Carbon Constituents, and Hazardous Components M. Teich et al.
- Comprehensive spectral analysis of reaction of three aldehydes with ammonium sulfate and glycine Y. Gao et al.
- Diol it up: The influence of NaCl on methylglyoxal surface adsorption and hydration state at the air–water interface B. Gordon et al.
- UV/Vis and IRMPD Spectroscopic Analysis of the Absorption Properties of Methylglyoxal Brown Carbon L. Vo et al.
- Contributions of nitrated aromatic compounds to the light absorption of water-soluble and particulate brown carbon in different atmospheric environments in Germany and China M. Teich et al.
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