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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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https://doi.org/10.5194/acp-2017-308
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-2017-308
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

  05 May 2017

05 May 2017

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This preprint was under review for the journal ACP. A revision for further review has not been submitted.

Analyzing trace gas filaments in the Ex-UTLS by 4D-variational assimilation of airborne tomographic retrievals

Annika Vogel1,2, Jörn Ungermann3, and Hendrik Elbern1,2 Annika Vogel et al.
  • 1Rhenish Institute for Environmental Research at the University of Cologne, Germany
  • 2Institute for Energy and Climate Research - Troposphere (IEK-8), Forschungszentrum Jülich, Germany
  • 3Institute for Energy and Climate Research - Stratosphere (IEK-7), Forschungszentrum Jülich, German

Abstract. This case study explores the potential for chemical state analysis at extratropical upper tropospheric – lower stratospheric (Ex-UTLS) height levels with airborne limb-images, assimilated into an advanced spatio-temporal system. The investigation is motivated by the limited capability of both, nadir- and limb-viewing satellite sensors to resolve highly filamented structures, delineated by sharp trace gas gradients on small horizontal and vertical scales. The EURAD-IM (EURopean Air pollution Dispersion – Inverse Model) is applied as assimilation system and designed to extend the flight path confined retrievals from GLORIA (Gimballed Limb Observer for Radiance Imaging of the Atmosphere) to both, larger areas and detailed vertical structures by a tomographic flight pattern. Related potential and limitations of the method are studied with the following features applied: (i) airborne limb-imaging observations of the Ex-UTLS, (ii) spatio-temporal extension by 4-dimensional variational data assimilation, (iii) correlation between ozone and potential vorticity (PV) as an indicator of airmasses and (iv) anisotropic and inhomogeneous horizontal background error correlations in the Ex-UTLS, spreading information towards unobserved regions along PV isopleths. This setup demonstrated substantial improvements to basic approaches in exploring new data on the spatial extend and alignment of airmasses down to small-scale filaments in the Ex-UTLS. Tomographic observations provide detailed insight for reconstructing filamentary foldings along airmass boundaries above the tropopause during this case study.

Annika Vogel et al.

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Status: closed (peer review stopped)
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Annika Vogel et al.

Annika Vogel et al.

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Short summary
The potential for chemical state analysis at tropopause heights was investigated by combining airborne tomographic observations with a chemical data-assimilation system in form of a case study. Related developments include the use of potential vorticity for ozone initialization and flow-dependent horizontal correlations. This setup demonstrated substantial improvements in terms of spatial extend and alignment of atmospheric structures down to filamentary foldings along airmass boundaries.
The potential for chemical state analysis at tropopause heights was investigated by combining...
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