Articles | Volume 18, issue 1
Atmos. Chem. Phys., 18, 227–246, 2018

Special issue: Quadrennial Ozone Symposium 2016 – Status and trends...

Atmos. Chem. Phys., 18, 227–246, 2018

Research article 09 Jan 2018

Research article | 09 Jan 2018

Ultraviolet radiation modelling from ground-based and satellite measurements on Reunion Island, southern tropics

Kévin Lamy1, Thierry Portafaix1, Colette Brogniez2, Sophie Godin-Beekmann3, Hassan Bencherif1,4, Béatrice Morel5, Andrea Pazmino3, Jean Marc Metzger6, Frédérique Auriol2, Christine Deroo2, Valentin Duflot1, Philippe Goloub2, and Charles N. Long7 Kévin Lamy et al.
  • 1LACy, Laboratoire de l'Atmosphère et des Cyclones (UMR 8105 CNRS, Université de La Réunion, Météo-France), Saint-Denis, Reunion Island, France
  • 2Laboratoire d'Optique Atmosphérique (LOA), Université Lille 1 Sciences et Technologies, Villeneuve d'Ascq, France
  • 3Laboratoire Atmosphères, Milieux, Observations Spatiales, Service d'Aéronomie (LATMOS), CNRS, Institut Pierre Simon Laplace, Pierre et Marie Curie University, Paris, France
  • 4School of Chemistry and Physics, University of KwaZulu Natal, Durban, South Africa
  • 5Laboratoire d'Energétique, d'Electronique et Procédés (LE2P), Université de la Réunion, Saint-Denis, Reunion Island, France
  • 6Observatoire des Sciences de l'Univers Réunion (OSU-R), UMS 3365, Université de la Réunion, Saint-Denis, Reunion Island, France
  • 7National Oceanographic and Atmospheric Administration, Earth System Research Laboratory, Boulder, Colorado, USA

Abstract. Surface ultraviolet radiation (SUR) is not an increasing concern after the implementation of the Montreal Protocol and the recovery of the ozone layer (Morgenstern et al., 2008). However, large uncertainties remain in the prediction of future changes of SUR (Bais et al., 2015). Several studies pointed out that UV-B impacts the biosphere (Erickson et al., 2015), especially the aquatic system, which plays a central part in the biogeochemical cycle (Hader et al., 2007). It can affect phytoplankton productivity (Smith and Cullen, 1995). This influence can result in either positive or negative feedback on climate (Zepp et al., 2007).

Global circulation model simulations predict an acceleration of the Brewer-Dobson circulation over the next century (Butchart, 2014), which would lead to a decrease in ozone levels in the tropics and an enhancement at higher latitudes (Hegglin and Shepherd, 2009). Reunion Island is located in the tropics (21° S, 55° E), in a part of the world where the amount of ozone in the ozone column is naturally low. In addition, this island is mountainous and the marine atmosphere is often clean with low aerosol concentrations. Thus, measurements show much higher SUR than at other sites at the same latitude or at midlatitudes. Ground-based measurements of SUR have been taken on Reunion Island by a Bentham DTMc300 spectroradiometer since 2009. This instrument is affiliated with the Network for the Detection of Atmospheric Composition Change (NDACC). In order to quantify the future evolution of SUR in the tropics, it is necessary to validate a model against present observations. This study is designed to be a preliminary parametric and sensitivity study of SUR modelling in the tropics.

We developed a local parameterisation using the Tropospheric Ultraviolet and Visible Model (TUV; Madronich, 1993) and compared the output of TUV to multiple years of Bentham spectral measurements. This comparison started in early 2009 and continued until 2016.

Only clear-sky SUR was modelled, so we needed to sort out the clear-sky measurements. We used two methods to detect cloudy conditions: the first was based on an observer's hourly report on the sky cover, while the second was based on applying Long and Ackerman (2000)'s algorithm to broadband pyranometer data to obtain the cloud fraction and then discriminating clear-sky windows on SUR measurements. Long et al. (2006)'s algorithm, with the co-located pyranometer data, gave better results for clear-sky filtering than the observer's report.

Multiple model inputs were tested to evaluate the model sensitivity to different parameters such as total ozone column, aerosol optical properties, extraterrestrial spectrum or ozone cross section. For total column ozone, we used ground-based measurements from the SAOZ (Système d'Analyse par Observation Zénithale) spectrometer and satellite measurements from the OMI and SBUV instruments, while ozone profiles were derived from radio-soundings and the MLS ozone product. Aerosol optical properties came from a local aerosol climatology established using a Cimel photometer. Since the mean difference between various inputs of total ozone column was small, the corresponding response on UVI modelling was also quite small, at about 1 %. The radiative amplification factor of total ozone column on UVI was also compared for observations and the model. Finally, we were able to estimate UVI on Reunion Island with, at best, a mean relative difference of about 0.5 %, compared to clear-sky observations.

Short summary
This work focuses on solar radiation in the tropics, more specifically on ultraviolet radiation. From ground-based and satellite observations of the chemical state of the atmosphere, we were able to model the ultraviolet measurements measured in the southern tropics with a very small error. This is a first step to modelling and predicting future ultraviolet levels in the tropics from chemistry-climate projections.
Final-revised paper