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Volume 16, issue 11
Atmos. Chem. Phys., 16, 7357–7371, 2016
https://doi.org/10.5194/acp-16-7357-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 7357–7371, 2016
https://doi.org/10.5194/acp-16-7357-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 14 Jun 2016

Research article | 14 Jun 2016

Characteristics of aerosol pollution during heavy haze events in Suzhou, China

Mi Tian1, Huanbo Wang1, Yang Chen1, Fumo Yang1,2,3, Xiaohua Zhang4, Qiang Zou4, Renquan Zhang4, Yongliang Ma5, and Kebin He5 Mi Tian et al.
  • 1Key Laboratory of Reservoir Aquatic Environment of CAS, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714, China
  • 2Center for Excellence in Urban Atmospheric Environment, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
  • 3Changjiang Normal University, Chongqing 408100, China
  • 4Suzhou Environmental Monitoring Center, Suzhou 215004, China
  • 5School of Environment, Tsinghua University, Beijing 100012, China

Abstract. Extremely severe haze weather events occurred in many cities in China, especially in the east part of the country, in January 2013. Comprehensive measurements including hourly concentrations of PM2.5 and its major chemical components (water-soluble inorganic ions, organic carbon (OC), and elemental carbon (EC)) and related gas-phase precursors were conducted via an online monitoring system in Suzhou, a medium-sized city in Jiangsu province, just east of Shanghai. PM2.5 (particulate matter with an aerodynamic diameter of 2.5 µm or less) frequently exceeded 150 µg m−3 on hazy days, with the maximum reaching 324 µg m−3 on 14 January 2013. Unfavorable weather conditions (high relative humidity (RH), and low rainfall, wind speed, and atmospheric pressure) were conducive to haze formation. High concentrations of secondary aerosol species (including SO42−, NO3, NH4+, and SOC) and gaseous precursors were observed during the first two haze events, while elevated primary carbonaceous species emissions were found during the third haze period, pointing to different haze formation mechanisms. Organic matter (OM), (NH4)2SO4, and NH4NO3 were found to be the major contributors to visibility impairment. High concentrations of sulfate and nitrate might be explained by homogeneous gas-phase reactions under low RH conditions and by heterogeneous processes under relatively high RH conditions. Analysis of air mass trajectory clustering and potential source contribution function showed that aerosol pollution in the studied areas was mainly caused by local activities and surrounding sources transported from nearby cities.

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The discussion was based on high time resolution data which could provide detailed insight into short haze periods. The dominant species in PM2.5 and which were responsible for the visibility reduction were identified in Suzhou. The formation mechanisms of sulfate and nitrate were explored as high secondary aerosol contributions to particulate pollution during haze events. The impact of local and transport sources on the origin of aerosol pollution in Suzhou was discussed.
The discussion was based on high time resolution data which could provide detailed insight into...
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