Articles | Volume 11, issue 21
Atmos. Chem. Phys., 11, 10791–10801, 2011
Atmos. Chem. Phys., 11, 10791–10801, 2011

Research article 02 Nov 2011

Research article | 02 Nov 2011

The first estimates of global nucleation mode aerosol concentrations based on satellite measurements

M. Kulmala1, A. Arola2, T. Nieminen1, L. Riuttanen1, L. Sogacheva3, G. de Leeuw1,3, V.-M. Kerminen1,3, and K. E. J. Lehtinen2,4 M. Kulmala et al.
  • 1Department of Physics, University of Helsinki, P.O. Box 64, 00014 University of Helsinki, Finland
  • 2Finnish Meteorological Institute, Kuopio Unit, P.O. Box 1627, 70211 Kuopio, Finland
  • 3Finnish Meteorological Institute, Climate Change Unit, P.O. Box 503, 00101 Helsinki, Finland
  • 4Department of Applied Physics, University of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland

Abstract. Atmospheric aerosols play a key role in the Earth's climate system by scattering and absorbing solar radiation and by acting as cloud condensation nuclei. Satellites are increasingly used to obtain information on properties of aerosol particles with a diameter larger than about 100 nm. However, new aerosol particles formed by nucleation are initially much smaller and grow into the optically active size range on time scales of many hours. In this paper we derive proxies, based on process understanding and ground-based observations, to determine the concentrations of these new particles and their spatial distribution using satellite data. The results are applied to provide seasonal variation of nucleation mode concentration. The proxies describe the concentration of nucleation mode particles over continents. The source rates are related to both regional nucleation and nucleation associated with more restricted sources. The global pattern of nucleation mode particle number concentration predicted by satellite data using our proxies is compared qualitatively against both observations and global model simulations.

Final-revised paper