Preprints
https://doi.org/10.5194/acp-2020-945
https://doi.org/10.5194/acp-2020-945

  25 Nov 2020

25 Nov 2020

Review status: this preprint is currently under review for the journal ACP.

Changes in biomass burning, wetland extent, or agriculture drive atmospheric NH3 trends in several African regions

Jonathan E. Hickman1, Niels Andela2, Enrico Dammers3, Lieven Clarisse4, Pierre-François Coheur4, Martin Van Damme4, Courtney Di Vittorio5, Money Ossohou6, Corrine Galy-Lacaux7, Kostas Tsigaridis1,8, and Susanne Bauer1 Jonathan E. Hickman et al.
  • 1NASA Goddard Institute for Space Studies, New York, USA
  • 2NASA Goddard Space Flight Center, Beltsville, USA
  • 3Air Quality Research Division, Environment and Climate Change Canada, Toronto, Canada
  • 4Université libre de Bruxelles (ULB), Service de Chimie Quantique et Photophysique, Atmospheric Spectroscopy, Brussels, Belgium
  • 5Wake Forest University, Winston-Salem, USA
  • 6Laboratoire de Physique de l'Atmosphère et de Mécanique des Fluides, Université Félix Houphouët-Boigny, Abidjan, Côte d’Ivoire
  • 7Laboratoire d'Aérologie, Université Toulouse III Paul Sabatier/CNRS, France
  • 8Columbia University, New York, USA

Abstract. Atmospheric ammonia (NH3) is a precursor to fine particulate matter and a source of nitrogen (N) deposition that can adversely affect ecosystem health. The main sources of NH3 – agriculture and biomass burning – are undergoing or expected to undergo substantial changes in Africa. Although evidence of increasing NH3 over parts of Africa has been observed, the mechanisms behind these trends are not well understood. Here we use observations of atmospheric NH3 vertical column densities (VCDs) from the Infrared Atmospheric Sounding Interferometer (IASI) along with other satellite observations of the land surface and atmosphere to evaluate how NH3 concentrations have changed over Africa from 2008 through 2017, and what has caused those changes. We find that NH3 VCDs have increased over several regions, including much of West Africa and parts of the Lake Victoria Basin. In West Africa NH3 VCDs are observed to increase during the late dry season, with increases of over 6 % yr−1 in Nigeria during February and March. These positive trends are associated with increasing burned area and CO trends during these months, likely related to agricultural preparation. Increases are also observed in the Lake Victoria Basin, where they are associated with expanding agricultural area. In contrast, South Sudan NH3 VCDs declined by over 2 % yr−1 during the February through May period, with the largest rates of change over the Sudd wetlands. Annual maxima in NH3 VCDs in South Sudan occur during February through May and are associated with drying of temporarily flooded wetland soils, which favor emissions of NH3. The change in mean NH3 VCDs over the Sudd and all of South Sudan during February through May is strongly correlated with variation in wetland extent in the Sudd: in years when more area remained flooded during the dry season, NH3 concentrations were higher (r = 0.69, p = 0.03). Relationships between agriculture and NH3 can be observed when evaluating national-scale statistics: countries with the largest declines in NH3 VCDs concentrations over time tended to have the smallest growth rates in crop productivity and livestock numbers as well as smaller negative changes in burned area than other countries. Fertilizer use in Africa is currently low but growing; implementing practices that can limit NH3 losses from fertilizer as agriculture is intensified may help mitigate impacts on health and ecosystems.

Jonathan E. Hickman et al.

 
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Jonathan E. Hickman et al.

Jonathan E. Hickman et al.

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Short summary
Ammonia (NH3) gas emitted from soils and biomass burning and contributes to particulate air pollution. We used satellite observations of the atmosphere over Africa to show that declines in NH3 concentrations over South Sudan's Sudd wetland in 2008–2017 are related to variation in wetland extent. We also find NH3 concentrations increased in West Africa as a result of biomass burning, and increased in the Lake Victoria Region, likely due to agricultural expansion and intensification.
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