Preprints
https://doi.org/10.5194/acp-2022-683
https://doi.org/10.5194/acp-2022-683
 
01 Nov 2022
01 Nov 2022
Status: this preprint is currently under review for the journal ACP.

The export of African mineral dust across the Atlantic and its impact over the Amazon Basin

Xurong Wang1,2,a,, Qiaoqiao Wang1,2,, Maria Prass3, Christopher Pöhlker3, Daniel Moran-Zuloaga3, Paulo Artaxo4, Jianwei Gu5, Ning Yang1,2, Xiajie Yang1,2, Jiangchuan Tao1,2, Juan Hong1,2, Nan Ma1,2, Yafang Cheng3, Hang Su3, and Meinrat O. Andreae3,6 Xurong Wang et al.
  • 1Institute for Environmental and Climate Research, Jinan University, Guangzhou, 511443, China
  • 2Guangdong-Hongkong-Macau Joint Laboratory of Collaborative Innovation for Environmental Quality, Guangzhou, 511443, China
  • 3Multiphase Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, Germany
  • 4Institute of Physics, University of São Paulo, São Paulo, 05508-900, Brazil
  • 5Institute of Environmental Health and Pollution Control, School of Environmental Science and Engineering, Guangdong University of Technology, Guangzhou, 510006, China
  • 6Scripps Institution of Oceanography, University of California, San Diego, CA 92093-0230, USA
  • anow at: Atmospheric Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, Germany
  • These authors contribute equally to this article.

Abstract. The Amazon Basin is frequently influenced by the trans-Atlantic transport of African dust plumes during its wet season (January–April), which not only interrupts the near-pristine atmospheric condition in that season, but also provides nutrient inputs into the Amazon rainforest associated with dust deposition. The factors controlling the long-range transport (LRT) of African dust towards the Amazon Basin and consequently the overall impact of African dust over the Amazon Basin are not yet well understood. In this study, we use the chemical transport model GEOS-Chem to investigate the impact of the export of African mineral dust upon the Amazon Basin during the period of 2013–2017, constrained by multiple datasets obtained from AERONET, MODIS, as well as Cayenne site and the Amazon Tall Tower Observatory (ATTO) site in the Amazon Basin. With optimized particle mass size distribution (PMSD), the model well captures observed AOD regarding both the mean value as well as the decline rate of the logarithm of AOD over the Atlantic Ocean along the transport path (AOaTP), implying the consistence with observed export efficiency of African dust along the trans-Atlantic transport. With an annual emission of 0.73 ± 0.12 Pg a-1, African dust entering the Amazon Basin has surface concentrations of 5.7 ± 1.3 µg m-3 (up to 15 µg m-3 in the northeast corner) during the wet season, accounting for 47 % ± 5.0 % (up to 70 %) of mass concentrations of total aerosols. The frequency of dust events in the Amazon Basin (defined as when surface dust concentrations reach the threshold of 9 µg m-3 on daily basis) in the wet season is around 18 % averaged over the basin, with maxima over 60 % at the northeast coast. During the dust events, AOD over most of the Amazon Basin is dominated by dust. Observed dust peaks over the Amazon Basin are generally associated with relatively higher African dust emissions (including Sahara and Sahel) and longer lifetime of dust along the trans-Atlantic transport, namely higher export efficiency of African dust across the Atlantic Ocean. Associated with dust deposition, we further estimate annual inputs of 52 ± 8.7, 0.97 ± 0.16 and 21 ± 3.6 mg m-2 a-1 for iron, phosphorus and magnesium deposited into the Amazon rainforest, respectively, which may well compensate the hydrologic losses of nutrients in the forest ecosystem.

Xurong Wang et al.

Status: open (until 19 Dec 2022)

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Xurong Wang et al.

Xurong Wang et al.

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Short summary
In this work, with optimized particle mass size distribution, we well captured observed AOD and coarse aerosol concentrations over source and/or receptor regions, demonstrating the well performance in simulating the export of African dust towards the Amazon Basin. In addition to the factors controlling the trans-Atlantic transport of African dust, the study also investigated the impact of African dust over the Amazon Basin including the nutrient inputs associated with dust deposition.
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