Preprints
https://doi.org/10.5194/acp-2022-124
https://doi.org/10.5194/acp-2022-124
 
18 Mar 2022
18 Mar 2022
Status: this preprint is currently under review for the journal ACP.

Comparisons between the distributions of dust and combustion aerosols in MERRA-2, FLEXPART and CALIPSO and implications for deposition freezing over wintertime Siberia

Lauren M. Zamora1,2, Ralph A. Kahn2, Nikolaos Evangeliou3, and Christine D. Groot Zwaaftink3 Lauren M. Zamora et al.
  • 1Earth System Science Interdisciplinary Center, University of Maryland, College Park, College Park, Maryland, U.S.A.
  • 2NASA Goddard Space Flight Center, Greenbelt, Maryland, U.S.A.
  • 3Norwegian Institute for Air Research (NILU), Kjeller, Norway

Abstract. Aerosol distributions have a potentially large influence on climate-relevant cloud properties but can be difficult to observe over the Arctic given pervasive cloudiness, long polar nights, data paucity over remote regions, and periodic diamond dust events that satellites can misclassify as aerosol. We compared Arctic 2008–2015 mineral dust and combustion aerosol distributions from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite, the Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2) reanalysis products, and the FLEX-ible PARTicle (FLEXPART) model. Based on Atmospheric Infrared Sounder (AIRS) satellite meteorological data, diamond dust may occur up to 60 % of the time in winter, but it hardly ever occurs in summer. In its absence, MERRA-2 and FLEXPART each predict the vertical distribution of combustion aerosols with relatively high confidence, as does FLEXPART for mineral dust. Comparisons to ground and satellite data suggest that MERRA-2 Arctic dust concentrations can be improved by the addition of local dust sources. Apparent false negative rates compared to lidar were substantially higher in conditions favouring diamond dust formation for both MERRA-2 and FLEXPART, as would be expected if CALIPSO were misclassifying diamond dust as mineral dust aerosols. All three products predicted that wintertime dust and combustion aerosols occur most frequently over the same Siberian regions where diamond dust is most common in the winter. This suggests that aerosol impacts on ice phase processes may be particularly high over Siberia, although further wintertime model validation with non-CALIPSO observations is needed. This assessment paves the way for applying the model-based aerosol simulations to a range of regional-scale Arctic aerosol-cloud interaction studies.

Lauren M. Zamora et al.

Status: final response (author comments only)

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Lauren M. Zamora et al.

Lauren M. Zamora et al.

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Short summary
Arctic dust, smoke and pollution particles can affect clouds and Arctic warming. The distributions of these particles were estimated in three different satellite and/or model products. These products showed good agreement overall, but indicate that it is important to include local dust in models. We hypothesize that dust effects on ice processes in the Arctic atmosphere might be highest over Siberia, where it is cold, moist, and subject to relatively high dust levels.
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