Preprints
https://doi.org/10.5194/acp-2021-355
https://doi.org/10.5194/acp-2021-355

  03 Jun 2021

03 Jun 2021

Review status: this preprint is currently under review for the journal ACP.

The regional impact of urban emissions on air quality in Europe: the role of the urban canopy effects

Peter Huszar1, Jan Karlický1,3, Jana Marková1,2, Tereza Nováková1, Marina Liaskoni1, and Lukáš Bartík1 Peter Huszar et al.
  • 1Department of Atmospheric Physics, Faculty of Mathematics and Physics, Charles University, Prague, V Holešovičkách 2, 18000, Prague 8, Czech Republic
  • 2Czech Hydrometeorological Institute (CHMI), Na Šabatce 17, 14306, Prague 4, Czech Republic
  • 3Institute of Meteorology and Climatology, Department of Water, Atmosphere and Environment, University of Natural Resources and Life Sciences, Vienna, Gregor-Mendel-Straße 33, 1180 Vienna, Austria

Abstract. Urban areas are hot-spots of intense emissions and they influence air-quality not only locally but on regional or even global scales. The impact of urban emissions over different scales depends on the dilution and chemical transformation of the urban plumes which are governed by the local and regional scale meteorological conditions. These are influenced by the presence of urbanized land-surface via the so called urban canopy meteorological forcing (UCMF). In this study, we investigate for selected central European cities (Berlin, Budapest, Munich, Prague, Vienna and Warsaw), how the urban emission impact (UEI) is modulated by the UCMF for present day climate conditions (2015–2016) using three regional climate-chemistry models: the regional climate models RegCM and WRF-Chem (its meteorological part), the chemistry transport model CAMx coupled to either RegCM and WRF and the “chemical” component of WRF-Chem. The UCMF was calculated by replacing the urbanized surface by rural one while the UEI was estimated by removing all anthropogenic emissions from the selected cities.

We analyzed the urban emissions induced changes of near surface concentrations of NO2, O3 and PM2.5. We found increases of NO2 and PM2.5 concentrations over cities by 4–6 ppbv, and 4–6 μgm−3, respectively meaning that about 40–60 % and 20–40 % of urban concentrations of NO2 and PM2.5 are caused by local emissions and the rest is the result of emissions from surrounding rural areas. We showed that if UCMF is included, the UEI of these pollutants is about 40–60 % smaller, or in other words, the urban emission impact is overestimated if urban canopy effects are not taken into account. In case of ozone, models due to UEI usually predict decreases around −2 to −4 ppbv (about 10–20 %), which is again smaller if UCMF is considered (by about 60 %). We further showed that the impact on extreme (95th percentile) air-pollution is much stronger, as well as the modulation of UEI is larger for such situations. Finally, we evaluated the contribution of the urbanization induced modifications of vertical eddy-diffusion to the modulation of UEI, and found that it alone is able to explain the modelled decrease of the urban emission impact if the effects of UCMF are considered. In summary, our results showed that the meteorological changes resulting from urbanization have to be included in regional model studies if they intend to quantify the regional fingerprint of urban emissions. Ignoring these meteorological changes can lead to strong overestimation of UEI.

Peter Huszar et al.

Status: open (until 15 Jul 2021)

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Peter Huszar et al.

Peter Huszar et al.

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Short summary
Urban areas are strong hotspots of emissions influencing local and regional air-quality. Cities furthermore influence the meteorological conditions due to their characteristic surface properties and geometry. We found that if these later effects are not included in the quantification of the impact of urban emissions on regional air-quality, this impact will be overestimated and this overestimation is mainly due to the enhanced turbulence that is present in cities compared to rural areas.
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