Preprints
https://doi.org/10.5194/acp-2021-1032
https://doi.org/10.5194/acp-2021-1032

  04 Jan 2022

04 Jan 2022

Review status: this preprint is currently under review for the journal ACP.

Assessing the consequences of including aerosol absorption in potential Stratospheric Aerosol Injection Climate Intervention Strategies

Jim Haywood1,2, Andy Jones2, Ben Johnson2, and William McFarlane Smith1,a Jim Haywood et al.
  • 1College of Engineering, Mathematics and Physical Science, University of Exeter, Exeter, EX4 4QE, UK
  • 2Met Office Hadley Centre, Exeter, EX1 3PB, UK
  • anow at: Downing College, Cambridge, CB2 1DQ, UK

Abstract. Theoretical Stratospheric Aerosol Intervention (SAI) strategies model the deliberate injection of aerosols or their precursors into the stratosphere thereby reflecting incident sunlight back to space and counterbalancing a fraction of the warming due to increased concentrations of greenhouse gases. This cooling mechanism is known to be relatively robust through analogues from explosive volcanic eruptions which have been documented to cool the climate of the Earth. However, a practical difficulty of SAI strategies is how to deliver the injection high enough to ensure dispersal of the aerosol within the stratosphere on a global scale. Recently, it has been suggested that including a small amount of absorbing material in a dedicated 10-day intensive deployment might enable aerosols or precursor gases to be injected at significantly lower, more technologically-feasible altitudes. The material then absorbs sunlight causing a localised heating and ‘lofting’ of the particles, enabling them to penetrate into the stratosphere. Such self-lofting has recently been observed following the intensive wildfires in 2019–2020 in south east Australia, where the resulting absorbing aerosol penetrated into the stratosphere and was monitored by satellite instrumentation for many months subsequent to emission. This study uses the fully coupled UKESM1 climate model simulations performed for the Geoengineering Model Intercomparison Project (GeoMIP) and new simulations where the aerosol optical properties have been adjusted to include a moderate degree of absorption. The results indicate that partially absorbing aerosols i) reduce the cooling efficiency per unit mass of aerosol injected, ii) increase deficits in global precipitation iii) delay the recovery of the stratospheric ozone hole, iv) disrupt the Quasi Biennial Oscillation when global mean temperatures are reduced by as little as 0.1 K, v) enhance the positive phase of the wintertime North Atlantic Oscillation which is associated with floods in Northern Europe and droughts in Southern Europe. While these results are dependent upon the exact details of the injection strategies and our simulations use ten times the ratio of black carbon to sulfate that is considered in the recent intensive deployment studies, they demonstrate some of the potential pitfalls of injecting an absorbing aerosol into the stratosphere to combat the global warming problem.

Jim Haywood et al.

Status: open (until 15 Feb 2022)

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse

Jim Haywood et al.

Jim Haywood et al.

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Short summary
Simulations are presented investigating the influence of moderately absorbing aerosol in the stratosphere to combat the impacts of climate change. A number of detrimental impacts are noted compared to sulfate aerosol, including i) reduced the cooling efficiency, ii) increases deficits in global precipitation, iii) delays in the recovery of the stratospheric ozone hole, iv) disruption of the stratospheric circulation and the wintertime storm-tracks that impact European precipitation.
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