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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys. Discuss.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name></publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-2020-380</article-id>
<title-group>
<article-title>Transport model diagnosis of the mean age of air derived from stratospheric samples in the tropics</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Nguyen</surname>
<given-names>Hanh T.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ishijima</surname>
<given-names>Kentaro</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Sugawara</surname>
<given-names>Satoshi</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hasebe</surname>
<given-names>Fumio</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Graduate School of Environmental Science, Hokkaido University, Sapporo 060-0810, Japan</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Japan Agency for Marine-Earth Science and Technology, Yokohama 236-0001, Japan</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Miyagi University of Education, Sendai 980-0845, Japan</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Faculty of Environmental Earth Science, Hokkaido University, Sapporo 060-0810, Japan</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>present address: Meteorological Research Institute, Tsukuba 305-0052, Japan</addr-line>
</aff>
<pub-date pub-type="epub">
<day>07</day>
<month>05</month>
<year>2020</year>
</pub-date>
<volume>2020</volume>
<fpage>1</fpage>
<lpage>32</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2020 Hanh T. Nguyen et al.</copyright-statement>
<copyright-year>2020</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/preprints/acp-2020-380/">This article is available from https://acp.copernicus.org/preprints/acp-2020-380/</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/preprints/acp-2020-380/acp-2020-380.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/preprints/acp-2020-380/acp-2020-380.pdf</self-uri>
<abstract>
<p>&lt;p&gt;Stratospheric profiles of the mean age of air estimated from cryogenic air samples acquired during the CUBE/Biak field campaign over Indonesia are investigated with the aid of an atmospheric chemistry transport model nudged to ERA-Interim meteorological fields. Application of the boundary impulse response (BIR) method and Lagrangian backward trajectories to the transport field simulated by a single model prove useful in interpreting the observational results, which include discrepancies between CO&lt;sub&gt;2&lt;/sub&gt;- and SF&lt;sub&gt;6&lt;/sub&gt;-derived mean ages. This may be because the BIR method takes unresolved diffusive processes into account while the Lagrangian method distinguishes the pathways the air parcels have taken before reaching the sample site. The capability to estimate the vertical profiles of the clock tracer concentrations and the water vapor “tape recorder” is another advantage of the Lagrangian method, confirming the reality of the trajectory calculations. The profile of CO&lt;sub&gt;2&lt;/sub&gt;-mean age is reproduced reasonably well by trajectory-derived mean age, while BIR-derived mean age is much greater than CO&lt;sub&gt;2&lt;/sub&gt; age at 28 and 29&amp;thinsp;km, possibly due to high diffusivity in the transport model. On the other hand, SF&lt;sub&gt;6&lt;/sub&gt; age is reproducible only in the lower stratosphere, but far exceeds the trajectory-derived mean age above 25&amp;thinsp;km. As air parcels of mesospheric origin are missing in the Lagrangian age estimation, this discrepancy, together with the fact that the observed SF&lt;sub&gt;6&lt;/sub&gt; concentrations are much lower than the trajectory-derived values in this height region, is consistent with the idea that the stratospheric air samples are mixed with SF&lt;sub&gt;6&lt;/sub&gt;-depleted mesospheric air, leading to overestimation of the mean age.&lt;/p&gt;</p>
</abstract>
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<award-id>26220101</award-id>
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