Preprints
https://doi.org/10.5194/acp-2020-1271
https://doi.org/10.5194/acp-2020-1271

  29 Dec 2020

29 Dec 2020

Review status: this preprint is currently under review for the journal ACP.

UTLS wildfire smoke over the North Pole region, Arctic haze, and aerosol-cloud interaction during MOSAiC 2019/20: An introductory

Ronny Engelmann1, Albert Ansmann1, Kevin Ohneiser1, Hannes Griesche1, Martin Radenz1, Julian Hofer1, Dietrich Althausen1, Sandro Dahlke2, Marion Maturilli2, Igor Veselovskii3, Cristofer Jimenez1, Robert Wiesen1, Holger Baars1, Johannes Bühl1, Henriette Gebauer1, Moritz Haarig1, Patric Seifert1, Ulla Wandinger1, and Andreas Macke1 Ronny Engelmann et al.
  • 1Leibniz Institute for Tropospheric Research, Leipzig, Germany
  • 2Alfred Wegener Institute, Helmholtz Centre for Polar and Marine Research, Potsdam, Germany
  • 3Prokhorov General Physics Institute of the Russian Academy of Sciences, Moscow, Russia

Abstract. An advanced multiwavelength polarization Raman lidar was operated aboard the icebreaker Polarstern during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition, lasting from September 2019 to October 2020, to contiuously monitor aerosol and cloud layers in the Central Arctic up to 30 km height at latitudes mostly between 85° N and 88.5° N. The lidar was integrated in a complex remote sensing infrastructure aboard Polarstern. Modern aerosol lidar methods and new lidar techniques and concepts to explore aerosol-cloud interaction were applied for the first time in the Central Arctic. Aim of the introductory article is to provide an overview of the observational spectrum of the lidar products for representative measurement cases. Highlight of the lidar measurements was the detection of a 10 km deep wildfire smoke layer over the North Pole area from, on average, 7 km to 17 km height with an aerosol optical thickness (AOT) at 532 nm around 0.1 (in October–November 2019) and 0.05 from December to mid of March 2020. The wildfire smoke was trapped within the extraordinarily strong polar vortex and remained detectable until the beginning of May 2020. Arctic haze was also monitored and characterized in terms of backscatter, extinction, and extinction-to-backscatter ratio at 355 and 532 nm. High lidar ratios from 60–100 sr in lofted mixed haze and smoke plumes are indicative for the presence of strongly light-absorbing fine-mode particles. The AOT at 532 nm was of the order of 0.025 for the tropospheric haze layers. In addition, so-called cloud closure experiments were applied to Arctic mixed-phase cloud and cirrus observations. The good match between cloud condensation nucleus concentration (CCNC) and cloud droplet number concentration (CDNC) and, on the other hand, between ice-nucleating particle concentration (INPC) and ice crystal number concentration (ICNC) indicated a clear influence of aerosol particles on the evolution of the cloud systems. CDNC was mostly between 20 and 100 cm−3 in the liquid-water dominated cloud top layer. ICNC was of the order of 0.1–1 L−1. The study of the impact of wildfire smoke particles on cirrus formation revealed that heterogeneous ice formation with smoke particles (organic aerosol particles) as INPs may have prevailed. ICNC values of 10–40 L−1 were clearly below ICNC levels that would indicate homogeneous freezing.

Ronny Engelmann et al.

 
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Ronny Engelmann et al.

Ronny Engelmann et al.

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Short summary
A Raman lidar was operated aboard the icebreaker Polarstern during the MOSAiC and monitored aerosol and cloud layers in the Central Arctic up to 30 km height. The article provides an overview of the spectrum of aerosol profiling observations and shows aerosol-cloud interaction studies for liquid-water and ice clouds. A highlight was the detection of a 10 km deep wildfire smoke layer over the North Pole up to 17 km height from the fire season of 2019, which persisted over the whole winter period.
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