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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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https://doi.org/10.5194/acp-2020-1096
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-2020-1096
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

  12 Nov 2020

12 Nov 2020

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This preprint is currently under review for the journal ACP.

Contrasting ice formation in Arctic clouds: surface coupled vs decoupled clouds

Hannes J. Griesche, Kevin Ohneiser, Patric Seifert, Albert Ansmann, and Ronny Engelmann Hannes J. Griesche et al.
  • Leibniz Institute for Tropospheric Research (TROPOS), Leipzig, Germany

Abstract. In the Arctic summer of 2017 (June, 1st to July, 16th) measurements with the multiwavelength polarization lidar PollyXT-OCEANET, 35-GHz cloud radar of the OCEANET platform, and radiosonde measurements were conducted during cruise PS106 of the research vessel Polarstern around Svalbard. In the scope of the presented study, the influence of cloud height and surface coupling on the probability of clouds to contain and form ice is investigated. The analyzed data set shows a significant impact of the surface-coupling state on the probability of ice formation. Surface-coupled clouds, identified by a quasi-constant potential temperature profile from the surface up to liquid layer base, in the same cloud-top temperature range contain ice more frequent than decoupled clouds by a factor of up to 5 for cloud-top intervals between −7.5 and −5 °C (169 vs. 31 profiles). These findings provide evidence that heterogeneous ice formation in Arctic mixed-phase clouds occurs by a factor of 2–5 more likely when the cloud layer is coupled to the surface. In turn, for cloud-top temperatures below −15 °C, the frequency of ice-containing cloud profiles for coupled and decoupled conditions approached the respective curve for the Central-European site of Leipzig, Germany (51° N, 12° E). This provides further evidence that the free-tropospheric ice nucleating particles (INP) reservoir over the Arctic is controlled by continental aerosol. One possible explanation for the observation is that turbulent mixing of the air below surface-coupled clouds allows ice particles, acting as seeds for ice multiplication, or marine aerosols, acting as INP, to be transported into the cloud layer more efficiently than in the case of decoupled conditions. This hypothesis is corroborated by recent in-situ measurements of INP in the Arctic, of which much higher concentrations were found in the surface-coupled atmosphere in close vicinity to the ice shore. Using lidar measurements we also found evidence for enhanced INP number concentrations (INPC) within surface-coupled cloud-free air masses. The INPC have been estimated based on particle backscatter profiles, published freezing spectra of biogenic INP and existing parameterizations.

Hannes J. Griesche et al.

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Hannes J. Griesche et al.

Data sets

OCEANET-ATMOSPHERE PollyXT measurements during POLARSTERN cruise PS106 Griesche, Hannes, Seifert, Patric, Engelmann, Ronny, Radenz, Martin, and Bühl, Johannes https://doi.org/10.1594/PANGAEA.899458

OCEANET-ATMOSPHERE Cloud radar Mira-35 during PS106 Griesche, Hannes, Seifert, Patric, Engelmann, Ronny, Radenz, Martin, and Bühl, Johannes https://doi.org/10.1594/PANGAEA.919556

Upper air soundings during POLARSTERN cruise PS106/1 (ARK-XXXI/1.1) Schmithüsen, Holger https://doi.org/10.1594/PANGAEA.882736

Upper air soundings during POLARSTERN cruise PS106/2 (ARK-XXXI/1.2) Schmithüsen, Holger https://doi.org/10.1594/PANGAEA.882843

Hannes J. Griesche et al.

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Short summary
Heterogeneous ice formation in arctic mixed-phase clouds under consideration of their surface-coupling state is investigated. Cloud phase and macrophysical properties were determined by means of lidar and cloud radar measurements, the coupling state and cloud-top temperature (CTT) by radiosonde profiles. Above −15 °C CTT surface-coupled clouds contain ice more likely by a factor of 2–5. By means of recent in-situ studies and in-depth lidar analysis different causes of this effect are discussed.
Heterogeneous ice formation in arctic mixed-phase clouds under consideration of their...
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