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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Preprints
https://doi.org/10.5194/acp-2019-996
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-2019-996
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.

  17 Dec 2019

17 Dec 2019

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A revised version of this preprint is currently under review for the journal ACP.

Spatial distribution of enhanced BrO and its relation to meteorological parameters in Arctic and Antarctic sea ice regions

Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows Sora Seo et al.
  • Institute of Environmental Physics, University of Bremen, Bremen, Germany

Abstract. Satellite observations have shown large areas of elevated BrO covering several thousand km2 over the Arctic and Antarctic sea ice region in polar spring. These enhancements of total BrO columns result from increases in stratospheric or tropospheric bromine amounts or both, and their occurrence may be related to local meteorological conditions. In this study, the spatial distribution of the occurrence of total BrO column enhancements and the associated changes in meteorological parameters are investigated in both the Arctic and Antarctic regions using 10 years of GOME-2 measurements in combination with meteorological model data. Statistical analysis of the data presents clear differences in the meteorological conditions between the 10 year mean and episodes of enhanced total BrO columns in both polar sea ice regions. These differences show pronounced spatial patterns. In general, atmospheric low pressure, cold surface air temperature, high surface-level wind speed and low tropopause heights were found during periods of enhanced total BrO columns. In addition, spatial patterns of prevailing wind directions related to the BrO enhancements are identified in both the Arctic and Antarctic sea ice region. The relevance of the different meteorological parameters for the total BrO column is evaluated based on a Spearman rank correlation analysis, finding that tropopause height and surface air temperature have the largest correlations with the total BrO vertical column density. Our results demonstrate that specific meteorological parameters can have a major impact on the BrO enhancement in some areas, but in general, multiple meteorological parameters interact with each other in their influence on BrO columns.

Sora Seo et al.

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Sora Seo et al.

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Short summary
In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
In this study, we present spatial distributions of occurrence frequency of enhanced total BrO...
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