<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "https://jats.nlm.nih.gov/nlm-dtd/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" specific-use="SMUR" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys. Discuss.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name></publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-8-16027-2008</article-id>
<title-group>
<article-title>Global error maps of aerosol optical properties: an error propagation analysis</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Tsigaridis</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Balkanski</surname>
<given-names>Y.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Schulz</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Benedetti</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Lab. des Sciences du Climat et de l&apos;Environnement (LSCE), 91191 Gif-sur-Yvette, France</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>European Center for Medium Range Weather Forecasts (ECMWF), Reading, UK</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>now at: NASA Goddard Institute for Space Studies (GISS), 2880 Broadway, NY 10025, USA</addr-line>
</aff>
<pub-date pub-type="epub">
<day>22</day>
<month>08</month>
<year>2008</year>
</pub-date>
<volume>8</volume>
<issue>4</issue>
<fpage>16027</fpage>
<lpage>16059</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2008 K. Tsigaridis et al.</copyright-statement>
<copyright-year>2008</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 3.0 Unported License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/3.0/">https://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/preprints/8/16027/2008/acpd-8-16027-2008.html">This article is available from https://acp.copernicus.org/preprints/8/16027/2008/acpd-8-16027-2008.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/preprints/8/16027/2008/acpd-8-16027-2008.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/preprints/8/16027/2008/acpd-8-16027-2008.pdf</self-uri>
<abstract>
<p>Among the numerous atmospheric constituents, aerosols play a unique role on
climate, due to their scattering and absorbing capabilities, visibility
degradation and their effect on incoming and outgoing radiation. The most
important optical properties are the aerosol optical depth (AOD), the
asymmetry parameter (&lt;I&gt;g&lt;/I&gt;) and the single scattering albedo (SSA). Uncertainties
in aerosol microphysics in global models, which in turn affect their optical
properties, propagate to uncertainties on the effect of aerosols on climate.
This study aims to estimate the uncertainty of AOD, &lt;I&gt;g&lt;/I&gt; and SSA attributable to
the aerosol representation in models, namely mixing state, aerosol size and
aerosol associated water. As a reference, the monthly mean output of the
general circulation model LMDz-INCA from the international comparison
exercise AEROCOM B was used. For the optical properties calculations,
aerosols were considered either externally mixed, homogeneously internally
mixed or coated spheres. The radius was allowed to vary by &amp;plusmn;20%
(with 2% intervals) and the aerosol water content by &amp;plusmn;50% (with
5% intervals) with respect to the reference model output. All of these
possible combinations were assumed to be equally likely and the optical
properties were calculated for each one of them. A probability density
function (PDF) was constructed at each model grid point for AOD, &lt;I&gt;g&lt;/I&gt; and SSA.
From this PDF, the 1σ and 2σ uncertainties of the AOD, &lt;I&gt;g&lt;/I&gt; and SSA were
calculated and are available as global maps for each month. For the range of
the cases studied, we derive a maximum 2σ uncertainty range in AOD of 70%,
while for &lt;I&gt;g&lt;/I&gt; and SSA the maxima reach 18% and 28% respectively. The
mixing state was calculated to be important, with the aerosol absorption and
SSA being the most affected properties when absorbing aerosols are present.</p>
</abstract>
<counts><page-count count="33"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Bohren, C. F. and Huffman, D. R.: Absorption and scattering of light by small particles, John Wiley and Sons, New York, USA, 1983. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Bond, T. C., Habib, G., and Bergstrom, R. W.: Limitations in the enhancement of visible light absorption due to mixing state, J. Geophys. Res., 111, D20211, https://doi.org/10.1029/2006JD007315, 2006. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Bond, T. C. and Bergstrom, R. W.: Light absorption by carbonaceous particles: an investigative review, Aerosol Sci. Tech., 40, 27–67, 2006. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> d&apos;Almeida, G. A., Koepke, P., and Shettle, E. P.: Atmospheric aerosols: global climatology and radiative characteristics, A. Deepak, Hampton, VA, USA, 1991. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Fuller, K. A.: Scattering and absorption cross sections of compounded spheres – 3: Spheres containing arbitrarily located spherical inhomogeneities, J. Opt. Soc. Am. A, 12, 893–904, 1995. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Fuller, K. A., Malm, W. C., and Kreidenweis, S. M.: Effects of mixing on extinction by carbonaceous particles, J. Geophys. Res., 104, 15 941–15 954, 1999. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Hale, G. M. and Querry, M. R.: Optical constants of water in the 200 nm to 200 mm wavelength region, Appl. Optics, 12, 555–563, 1973. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Hauglustaine, D. A., Hourdin, F., Jourdain, L., Filiberti, M.-A., Walters, S., Lamarque, J.-F., and Holland, E. A.: Interactive chemistry in the Laboratoire de Météorologie Dynamique general circulation model: description and background tropospheric chemistry evaluation, J. Geophys. Res., 109, D04314, https://doi.org/10.1029/2003JD003957, 2004. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Hourdin, F. and Armengaud, A.: The use of finite-volume methods for atmospheric advection of trace species – Part 1: test of various formulations in a general circulation model, Mon. Weather. Rev., 127, 822–837, 1999. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Jacobson, M. Z., Kaufman, Y. J., and Rudich, Y.: Examining feedbacks of aerosols to urban climate with a model that treats 3-D clouds with aerosol inclusions, J. Geophys. Res., 112, https://doi.org/10.1029/2007JD008922, 2007. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Kinne, S., Schulz, M., Textor, C., Guibert, S., Balkanski, Y., Bauer, S. E., Berntsen, T., Berglen, T. F., Boucher, O., Chin, M., Collins, W., Dentener, F., Diehl, T., Easter, R., Feichter, J., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Herzog, M., Horowitz, L., Isaksen, I., Iversen, T., Kirkev&amp;aring;g, A., Kloster, S., Koch, D., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Lesins, G., Liu, X., Lohmann, U., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, O., Stier, P., Takemura, T., and Tie, X.: An AeroCom initial assessment – optical properties in aerosol component modules of global models, Atmos. Chem. Phys., 6, 1815–1834, 2006. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Lesins, G., Chylek, P., and Lohmann, U.: A study of internal and external mixing scenarios and its effect on aerosol optical properties and direct radiative forcing, J. Geophys. Res., 107, 4094, https://doi.org/10.1029/2001JD000973, 2002. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Liu, X., Penner, J. E., Das, B., Bergmann, D., Rodriguez, J. M., Strahan, S., Wang, M., and Feng, Y.: Uncertainties in global aerosol simulations: Assessment using three meteorological data sets, J. Geophys. Res., 112, D11212, https://doi.org/10.1029/2006JD008216, 2007. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> McMurry, P. H.: A review of atmospheric aerosol measurements, Atmos. Environ., 34, 1959–1999, 2000. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Moteki, N., Kondo, Y., Miyazaki, Y., Takegawa, N., Komazaki, Y., Kurata, G., Shirai, T., Blake, D. R., Miyakawa, T., and Koike, M.: Evolution of mixing state of black carbon particles: Aircraft measurements over the western Pacific in March 2004, Geophys. Res. Lett., 34, L11803, https://doi.org/10.1029/2006GL028943, 2007. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Reddy, M. S., Boucher, O., Balkanski, Y., and Schulz, M.: Aerosol optical depths and direct radiative perturbations by species and source type, Geophys. Res. Lett., 32, L12803, https://doi.org/10.1029/2004GL021743, 2005. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Reid, J. S., Eck, T. F., Christopher, S. A., Koppmann, R., Dubovik, O., Eleuterio, D. P., Holben, B. N., Reid, E. A., and Zhang, J.: A review of biomass burning emissions – Part 3: Intensive optical properties of biomass burning particles, Atmos. Chem. Phys., 5, 827–849, 2005a. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Reid, J. S., Koppmann, R., Eck, T. F., and Eleuterio, D. P.: A review of biomass burning emissions – Part 2: intensive physical properties of biomass burning particles, Atmos. Chem. Phys., 5, 799–825, 2005b. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Shettle, E. P. and Fenn, R. W.: Models of the aerosols of the lower atmosphere and the effects of humidity variations on their optical properties, Project 7670, Air Force Geoph. Lab., Massachusetts, USA, 1979. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Song, C. H. and Carmichael, G. R.: The aging process of naturally emitted aerosol (sea-salt and mineral aerosol) during long range transport, Atmos. Environ., 33, 2203–2218, 1999. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Song, C. H., Maxwell-Meier, K., Weber, R. J., Kapustin, V., and Clarke, A.: Dust composition and mixing state inferred from airborne composition measurements during ACE-Asia C130 Flight #6, Atmos. Environ, 39, 359–369, 2005. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125–1156, 2005. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Textor, C., Schulz, M., Kinne, S., et al.: Analysis and quantification of the diversities of aerosol life cycles within AeroCom, Atmos. Chem. Phys., 6, 1777–1813, 2006. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Toon, O. B., Pollack, J. B., and Khare, B. N.: The optical constants of several atmospheric aerosol species: ammonium sulfate, aluminium oxide, and sodium chloride, J. Geophys. Res., 81, 5733–5748, 1976. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Toon, O. B. and Ackerman, T. P.: Algorithms for the calculation of scattering by stratified spheres, Appl. Optics, 20, 3657–3660, 1981. </mixed-citation>
</ref>
</ref-list>
</back>
</article>