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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-26-13983-2026</article-id><title-group><article-title>Impacts of mesoscale atmospheric subsidence on cloud glaciation and decoupling in Arctic marine cold air outbreaks</article-title><alt-title>Mesoscale subsidence in Arctic marine cold air outbreak clouds</alt-title>
      </title-group>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>Paulus</surname><given-names>Fiona</given-names></name>
          <email>fpaulus@uni-koeln.de</email>
        <ext-link>https://orcid.org/0000-0002-2701-1178</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Müller</surname><given-names>Joshua J.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-6584-2581</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2 aff3">
          <name><surname>Kirbus</surname><given-names>Benjamin</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-8824-2244</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4 aff5">
          <name><surname>Sodemann</surname><given-names>Harald</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-8167-0860</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>van Gelder</surname><given-names>Lars</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-6751-387X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Walbröl</surname><given-names>Andreas</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-2603-2724</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Wendisch</surname><given-names>Manfred</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-4652-5561</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Neggers</surname><given-names>Roel A. J.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-9182-3050</ext-link></contrib>
        <aff id="aff1"><label>1</label><institution>Institute for Geophysics and Meteorology, University of Cologne, Cologne, Germany</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Leipzig Institute for Meteorology, Leipzig University, Leipzig, Germany</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Fraunhofer Institute for Energy Economics and Energy System Technology, Kassel, Germany</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>Geophysical Institute, University of Bergen, Bergen, Norway</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>Bjerknes Center for Climate Research, Bergen, Norway</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Fiona Paulus (fpaulus@uni-koeln.de)</corresp></author-notes><pub-date><day>6</day><month>October</month><year>2026</year></pub-date>
      
      <volume>26</volume>
      <issue>19</issue>
      <fpage>13983</fpage><lpage>14014</lpage>
      <history>
        <date date-type="received"><day>29</day><month>January</month><year>2026</year></date>
           <date date-type="rev-request"><day>11</day><month>February</month><year>2026</year></date>
           <date date-type="rev-recd"><day>28</day><month>July</month><year>2026</year></date>
           <date date-type="accepted"><day>17</day><month>August</month><year>2026</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2026 Fiona Paulus et al.</copyright-statement>
        <copyright-year>2026</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026.html">This article is available from https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d2e174">The impact of mesoscale vertical atmospheric motion on the thermodynamic, microphysical, and convective transformations of air masses during marine cold air outbreaks (MCAOs) is largely unknown, partly due to scarcity of suitable observations in Arctic regions. To help close this gap, this study investigates the effects of mesoscale subsidence on the evolution of atmospheric boundary-layer (ABL) properties, cloud phase, and precipitation characteristics for a case study of a shallow MCAO observed in the Fram Strait  during the HALO–(<inline-formula><mml:math id="M1" display="inline"><mml:mrow><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi></mml:mrow></mml:math></inline-formula>)<sup>3</sup> campaign in March 2022. Quasi-Lagrangian Large-Eddy Simulations (LES) are conducted with observational initialisation and larger-scale forcing, based on airborne in-situ and remote-sensing measurements. The LES control simulation accurately reproduces the measured thermodynamic ABL structure and the temporal evolution of the observed air mass moving over the Arctic sea ice onto the open ocean. Specifically, the measured ABL height, integrated water vapour, and cloud water paths are well represented by the LES control run. Sensitivity experiments using the LES assuming prescribed subsidence reveal that weaker subsidence substantially deepens the ABL and causes an earlier onset of cloud glaciation. Decoupling of the cloud layer occurs sooner under weaker mesoscale subsidence, triggering convective graupel formation. This link between glaciation and decoupling explains the typical evolution of the cloud liquid water path observed in many MCAOs.</p>
  </abstract>
    
<funding-group>
<award-group id="gs1">
<funding-source>Deutsche Forschungsgemeinschaft</funding-source>
<award-id>268020496</award-id>
<award-id>442649391</award-id>
<award-id>316646266</award-id>
</award-group>
<award-group id="gs2">
<funding-source>European Research Council</funding-source>
<award-id>773245</award-id>
</award-group>
</funding-group>
</article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d2e205">During marine cold air outbreaks (MCAOs), cold and dry polar air masses are advected over cold sea ice surfaces towards the warmer open ocean, where they heat up and pick up humidity from below. MCAOs are an essential phenomenon in the Arctic climate system that frequently occurs over extended marine regions at northern high latitudes <xref ref-type="bibr" rid="bib1.bibx21" id="paren.1"/>. Additionally, as these air masses cross the sea ice edge and move over open ocean, the strong near-surface air temperature contrast between the warmer open ocean surface and the overlaying colder air generates intense turbulent and convective mixing, producing large sensible vertical heat fluxes <xref ref-type="bibr" rid="bib1.bibx82 bib1.bibx73 bib1.bibx63 bib1.bibx38" id="paren.2"/>. This vertical turbulent exchange rapidly transforms the air mass and deepens the Atmospheric Boundary Layer (ABL). As a result, spatially organised cloud structures evolve in the ABL that initially appear as cloud streets <xref ref-type="bibr" rid="bib1.bibx4 bib1.bibx43 bib1.bibx20 bib1.bibx39 bib1.bibx40" id="paren.3"/>. As the air mass continues to respond to the warm open ocean surface, low-level warming and moistening, together with persistent vertical surface energy flows, precipitation, and cloud microphysical processes such as riming and secondary ice production promotes a transition from cloud streets to deeper, broken cloud fields <xref ref-type="bibr" rid="bib1.bibx100 bib1.bibx58 bib1.bibx78" id="paren.4"/>. These evolving cloud and ABL characteristics modulate cloud-radiative interactions, determine precipitation formation, and increase surface winds <xref ref-type="bibr" rid="bib1.bibx41 bib1.bibx98 bib1.bibx47" id="paren.5"/>. Through this ocean–atmosphere coupling, MCAOs influence atmospheric and oceanic circulations <xref ref-type="bibr" rid="bib1.bibx70 bib1.bibx35 bib1.bibx62 bib1.bibx46" id="paren.6"/>, which are linked to feedback mechanisms of Arctic amplification <xref ref-type="bibr" rid="bib1.bibx110" id="paren.7"/>. The air mass transports during MCAOs and the corresponding transformation processes also contribute to heat and moisture exchange between the Arctic and mid-latitudes <xref ref-type="bibr" rid="bib1.bibx68" id="paren.8"/>.</p>
      <p id="d2e233">Despite extensive prior studies, key aspects of MCAO evolution remain poorly understood, particularly the onset of ABL decoupling in the sub-cloud layer, which accelerates stratocumulus breakup and promotes transitions between cloud regimes <xref ref-type="bibr" rid="bib1.bibx8 bib1.bibx48 bib1.bibx45 bib1.bibx117" id="paren.9"/>. Furthermore, precipitation formation and cloud microphysical developments that are influenced by riming and secondary ice production, reducing vertical mixing and altering ABL energy budgets, are not well represented in models <xref ref-type="bibr" rid="bib1.bibx1 bib1.bibx37 bib1.bibx114" id="paren.10"/>. Persistent observational gaps, particularly in remote upstream regions of MCAO pathways, continue to limit our understanding of these processes and their role in organising MCAO transitions. Consequently, major questions remain regarding how dynamical and microphysical processes support the transition to open-cell convection and how these should be represented in numerical models <xref ref-type="bibr" rid="bib1.bibx99 bib1.bibx15" id="paren.11"/>.</p>
      <p id="d2e245">The role of mesoscale vertical motion in MCAO evolution, and mixed-phase clouds in particular, is complex and not yet fully understood. Previous studies have shown that subsidence in surface-coupled convective layers can counteract mixed-layer growth by reducing the effective contributions of cloud-top entrainment. Increased liquid water paths inside the mixed-layer can enhance cloud-top radiative cooling and, together with precipitation-related diabatic processes, promote convective overturning and precipitation production. In turn, enhanced cloud-top radiative cooling and convective overturning under stronger subsidence can increase precipitation production in both rain and snow. Under surface-warming conditions, stronger subsidence can also suppress cloud-top ascent and help maintain a stable stratiform cloud layer <xref ref-type="bibr" rid="bib1.bibx116" id="paren.12"/>.</p>
      <p id="d2e251">In contrast, <xref ref-type="bibr" rid="bib1.bibx61" id="text.13"/> found that strong subsidence can cause mixed-phase cloud layers over the central Arctic sea ice to collapse, shifting thermal-infrared radiative cooling to the surface and hindering cloud reformation. These findings highlight that mesoscale subsidence can strongly modulate mixed-phase cloud layers, although it remains unknown how this modulation depends on the ABL structure. The involved interactions span a wide range of spatial scales, from mesoscale to synoptic subsidence. It covers processes such as turbulent entrainment, microphysical interactions, and aerosol particle evolution <xref ref-type="bibr" rid="bib1.bibx100 bib1.bibx101" id="paren.14"/>. A prime cause for our lack of insight into the impact of mesoscale subsidence on mixed-phase clouds is the distinct observational data gap on this variable at high latitudes. Measuring large-scale vertical motion or horizontal divergence remains difficult, as small errors in horizontal wind gradients lead to large uncertainties when using mass conservation. A more robust method applies regression to dropsonde data released in mesoscale patterns by fast aircraft, pioneered during two aircraft campaigns in the subtropical trades <xref ref-type="bibr" rid="bib1.bibx6 bib1.bibx96 bib1.bibx24" id="paren.15"/>. The application of this method to the coherent flow of an Arctic MCAO, as realized in this paper, helps to narrow this data gap and to enhance our understanding of the impacts of subsidence on the development of mixed-phase clouds in growing atmospheric boundary layers.</p>
      <p id="d2e264">The Fram Strait in the North Atlantic Ocean is a hotspot for MCAOs. It is relatively easy to access, making it a frequent target area for atmospheric observational and modelling studies. Although many recent Fram Strait studies are model-based, several field campaigns have filled key data gaps of MCAO processes. For example, the Cold air Outbreaks in the Marine Boundary Layer Experiment (COMBLE) in 2019 and 2020 observed several MCAOs with two permanent observational sites that provided continuous measurements of downstream conditions at Bear Island and Andenes <xref ref-type="bibr" rid="bib1.bibx23" id="paren.16"/>, and the Springtime Atmospheric Boundary Layer Experiment (STABLE) campaign in March 2013 and the Cold Air Outbreak Experiment in the Sub-Arctic Region (CAESAR), who provided airborne observations with research aircraft in the Fram Strait <xref ref-type="bibr" rid="bib1.bibx54 bib1.bibx118" id="paren.17"/>. The HALO–<inline-formula><mml:math id="M3" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign in 2022 sampled numerous MCAOs with multiple co-located aircraft, probing upstream and downstream regions <xref ref-type="bibr" rid="bib1.bibx106 bib1.bibx111 bib1.bibx112 bib1.bibx18" id="paren.18"/>. During HALO–<inline-formula><mml:math id="M4" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>, the mesoscale dropsonde pattern technique was applied to sample mesoscale atmospheric subsidence at multiple points along a MCAO trajectory for two consecutive days, producing the first robust high-latitude subsidence dataset of its kind <xref ref-type="bibr" rid="bib1.bibx66" id="paren.19"/>. This unique dataset creates new opportunities for investigating the role of subsidence in MCAO evolution.</p>
      <p id="d2e314">The main objective of this study is to use quasi-Lagrangian Large-Eddy Simulations (LES), driven by HALO–<inline-formula><mml:math id="M5" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> observational data, to gain insight into the impacts of mesoscale subsidence on MCAOs. For a particular case study, the LES follows an observed MCAO along its 2 d southbound trajectory, initialised with in-situ dropsonde profiles from the High Altitude and Long Range Aircraft (HALO) in the far north. The simulated air mass evolves freely, with large-scale forcings, including vertical motion, geostrophic wind, and advection tendencies, derived from circular dropsonde pattern observations and prescribed along the trajectory <xref ref-type="bibr" rid="bib1.bibx66" id="paren.20"/>. The simulated ABL and cloud properties are compared against independent downstream aircraft observations.</p>
      <p id="d2e337">Given this observationally constrained model setup, we ask how well the Lagrangian LES reproduces the independently observed cloud development. After evaluating the model performance, we conduct perturbation experiments on the mesoscale subsidence to assess the sensitivity of the MCAO, focusing on the evolution of the ABL structure, cloud mass, thermodynamic phase, and surface precipitation. This study aims to discuss how microphysical and dynamical properties and processes interact in their response to perturbed larger-scale subsidence forcing within the simulated MCAO system.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Observations</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>The HALO–<inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign</title>
      <p id="d2e373">The HALO–<inline-formula><mml:math id="M7" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> field campaign took place in the Norwegian/Greenland Seas and the Fram Strait from March to April 2022. The main objective of this airborne campaign was to understand the transformation of air masses between the Arctic and the mid-latitudes and to investigate the influence of these interactions on ABL processes and cloud formation. To this end, a quasi-Lagrangian sampling strategy was applied during the campaign, in which the transformation of individual air parcels of an air mass was tracked along their trajectories using three research aircraft flying at different altitudes (HALO, Polar 5, and Polar 6) <xref ref-type="bibr" rid="bib1.bibx111" id="paren.21"/>. An overview of the synoptic situation during the HALO–<inline-formula><mml:math id="M8" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign is provided by <xref ref-type="bibr" rid="bib1.bibx106" id="text.22"/>.</p>
      <p id="d2e416">This study focuses on a case study analysing two HALO Research Flights 10 and 11 (RF10 and RF11) conducted on 29 and 30 March 2022 (Fig. <xref ref-type="fig" rid="F1"/>). On these 2 d, a weak MCAO with an MCAO index of four was investigated <xref ref-type="bibr" rid="bib1.bibx62 bib1.bibx106" id="paren.23"/> (Appendix <xref ref-type="sec" rid="App1.Ch1.S2"/>). Both days were characterised by a persistent northerly wind of about 3 to 10 m<inline-formula><mml:math id="M9" display="inline"><mml:mspace width="0.125em" linebreak="nobreak"/></mml:math></inline-formula>s<sup>−1</sup> measured at 10 m altitude by dropsonde observations. These characteristics indicate a weak MCAO event compared with climatological values from the Fram Strait <xref ref-type="bibr" rid="bib1.bibx84" id="paren.24"/>. The slowly moving air mass was probed by HALO during these 2 d. The observed MCAO case embedded within a prolonged period of extensive MCAO activity from 21 March to 12 April 2022, between two intervals of particularly strong conditions on 21–26 March and 1–2 April 2022 <xref ref-type="bibr" rid="bib1.bibx106" id="paren.25"/>.</p>
      <p id="d2e451">The synoptic situation in the Fram Strait was characterised by a high-pressure system centred at the east coast of Greenland and a low-pressure area in the Barents Sea (Fig. <xref ref-type="fig" rid="FA1"/>). The cloud field was dominated by shallow convective mixed-phase clouds, with obvious street features near the sea ice edge. These cloud streets broke up further downstream in the area of C03 (Fig. <xref ref-type="fig" rid="F1"/>). A notable cloud-free area was located on the west coast of Svalbard (Fig. <xref ref-type="fig" rid="F2"/>), which can be attributed to the Foehn effect during easterly flow over Svalbard, similarly observed during other field campaigns <xref ref-type="bibr" rid="bib1.bibx83" id="paren.26"><named-content content-type="pre">e.g.,</named-content></xref>.</p>
      <p id="d2e466">The HALO flight plans on these 2 d aimed at tracking the location of an air mass sampled on the first day at a location in the high north above sea ice using trajectory estimates based on forecast data. At four locations along the trajectory, the air mass was sampled using a circular mesoscale dropsonde pattern, with a diameter of 150 km. This technique is inspired by <xref ref-type="bibr" rid="bib1.bibx44" id="text.27"/> and has been applied in the North Atlantic and subtropical region by <xref ref-type="bibr" rid="bib1.bibx95 bib1.bibx96" id="text.28"/> to measure mesoscale divergence and subsidence profiles. The centre of the initial circle (IC) (Fig. <xref ref-type="fig" rid="F1"/>) on the first day at 14:00 UTC was located at (84.4° N, 13.6° E) and featured only five dropsondes, a number limited by airspace restrictions. On the second day, three further circular patterns were flown along the predicted southern trajectory of the air mass. The circles sampled during the two subsequent days featured eight evenly distributed dropsondes, with two additional dropsondes launched in their inner areas. Only one of the day-two circles, (C02) at (78.6° N, 4.0° E, at 11:30 UTC), was located at the exact predicted location of the air mass as sampled on the previous day at the IC location. As shown in Fig. <xref ref-type="fig" rid="F1"/>, this circle was situated over open ocean. Two further circles were flown on day two, one (C01) further upstream over sea ice (80.8° N, 10.7° E, at 10:30 UTC), and another (C03) was flown at a downstream location at a similar distance (76.3° N, 3.3° E, at 12:30 UTC). The Polar 5 (P5) aircraft took additional measurements in the C02 area, shortly after the departure of the HALO aircraft from this area (at 12:00 UTC), using a rectangular flight pattern with three cross-flow legs. Additional measurements were conducted by a controlled meteorological balloon (CMET) launched from Ny-Ålesund, as part of the ISLAS2022 field experiment <xref ref-type="bibr" rid="bib1.bibx85" id="paren.29"/>, which took place at the same time as the HALO–<inline-formula><mml:math id="M11" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign.</p>

      <fig id="F1"><label>Figure 1</label><caption><p id="d2e502">Map of the simulation trajectory for the Lagrangian LES (bold line) initiated in the centre of the circular flight leg on 29 March 2022 of the HALO–<inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign, together with the flight paths of the HALO and P5 aircraft on 30 March 2022 and the trajectory of the CMET. Locations where dropsondes were released in IC on 29 March 2022 and in C01, C02 and C03 of 30 March 2022 from HALO are indicated by <inline-formula><mml:math id="M13" display="inline"><mml:mo>▾</mml:mo></mml:math></inline-formula>. The sea ice concentration retrieved from satellite observations <xref ref-type="bibr" rid="bib1.bibx90" id="paren.30"/> is indicated in grey and white, and the colour bar denotes the time (UTC) along the trajectory and flight paths.</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f01.png"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Data</title>
      <p id="d2e546">A combination of in-situ and remote sensing observations from the HALO–<inline-formula><mml:math id="M14" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign were used to constrain the LES experiments and evaluate the model performance. A comprehensive overview of the measurements collected during HALO–<inline-formula><mml:math id="M15" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> is described by <xref ref-type="bibr" rid="bib1.bibx18" id="text.31"/>, and a summary of the datasets used is presented in Table <xref ref-type="table" rid="T1"/>, including the variable names, associated instruments, and references to more detailed technical and scientific descriptions.</p>
      <p id="d2e588">The deployed Vaisala RD-41 dropsondes provide vertical profile measurements of the thermodynamic state, including air temperature at a resolution of 0.01 K, relative humidity at a resolution of 0.1 % and air pressure at a resolution of 0.01 h Pa at frequencies between 2 and 4 Hz and descend at speeds between 10 and 20 m s<sup>−1</sup> <xref ref-type="bibr" rid="bib1.bibx103" id="paren.32"/>. The measured profiles are interpolated to a uniform vertical grid of 5 m spacing. The horizontal wind speed profiles were determined from GPS data with an estimated accuracy of 0.1 m s<sup>−1</sup> <xref ref-type="bibr" rid="bib1.bibx31 bib1.bibx109" id="paren.33"/>. These observations were used to derive vertical profiles of subsidence (Fig. <xref ref-type="fig" rid="F3"/>), geostrophic wind, and advective tendencies of temperature, humidity, and wind through a regression algorithm applied to the dropsondes deployed in each circle. A comprehensive description of the calculation technique is provided by <xref ref-type="bibr" rid="bib1.bibx66" id="text.34"/>.</p>
      <p id="d2e627">To constrain the surface skin temperature <inline-formula><mml:math id="M18" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, airborne measurements of the thermal-infrared imager on board HALO VELOX <xref ref-type="bibr" rid="bib1.bibx76" id="paren.35"><named-content content-type="pre">Video airbornE Longwave Observations within siX channels;</named-content></xref> were used, which records 2-D fields (<inline-formula><mml:math id="M19" display="inline"><mml:mrow><mml:mn mathvariant="normal">640</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">512</mml:mn></mml:mrow></mml:math></inline-formula> px) of the thermal infrared brightness temperature. At typical HALO flight altitudes, this corresponds to a horizontal resolution of 10 m with a temporal resolution of 1 Hz for a field-of-view of <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:mn mathvariant="normal">6.4</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">5.1</mml:mn></mml:mrow></mml:math></inline-formula> km. From these brightness temperature images, the skin temperature <inline-formula><mml:math id="M21" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and sea-ice concentration were derived along the circular flight legs of HALO with estimated measurement uncertainties of 1.2 K and 5 %, respectively <xref ref-type="bibr" rid="bib1.bibx56" id="paren.36"/>. For partly cloudy open-ocean segments in C02 and C03, we apply a cloud mask and classify pixels whose retrieved values of <inline-formula><mml:math id="M22" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> exceed <inline-formula><mml:math id="M23" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.8 °C above the surrounding (cloudy) background as open ocean. The final surface skin temperature is the horizontal mean of each masked 2D-field at a 1 Hz time resolution.</p>
      <p id="d2e703">The datasets collected during the HALO–<inline-formula><mml:math id="M24" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign provide all atmospheric state variables required to run Lagrangian LES experiments following the air mass as it moves south. A small number of surface parameters, such as the surface albedo, the aerodynamic roughness length for momentum, and the thermal roughness length for heat, could not be measured, but are needed to prescribe the (latitude-dependent) surface boundary condition in the LES experiments. Therefore, these data were retrieved from the European Centre for Medium-Range Weather Forecasts (ECMWF) reanalysis product version 5 <xref ref-type="bibr" rid="bib1.bibx29" id="paren.37"><named-content content-type="pre">ERA5;</named-content></xref>. By combining the dropsonde and VELOX observations with the surface values from ERA5, a complete set of forcing fields for the Lagrangian LES has been compiled.</p>
      <p id="d2e729">For model validation, independent datasets obtained from the HALO–<inline-formula><mml:math id="M25" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign are used. The Airborne Mobile Aerosol Lidar (AMALi) on the P5 aircraft provides measurements of cloud top height, which are compared to the simulated cloud top heights <xref ref-type="bibr" rid="bib1.bibx92" id="paren.38"/>. The liquid water and ice water paths are derived from the Microwave Radar/Radiometer for Arctic Clouds (MiRAC) on board P5 <xref ref-type="bibr" rid="bib1.bibx51" id="paren.39"/>. The ice water path is derived from the 94 GHz-radar reflectivity using the Ze–IWC relationship of <xref ref-type="bibr" rid="bib1.bibx32" id="text.40"/>. We additionally include integrated water vapour (IWV) and liquid water path (LWP) data retrieved from the HALO Microwave Package (HAMP) over open ocean (not available over sea ice) <xref ref-type="bibr" rid="bib1.bibx50" id="paren.41"/>. These data allow a direct comparison with the quantities computed by the LES.</p>
      <p id="d2e761">Further thermodynamic observations were performed using Lagrangian CMET soundings <xref ref-type="bibr" rid="bib1.bibx105" id="paren.42"/>. The balloon was equipped with an air temperature sensor that operates over a range of <inline-formula><mml:math id="M26" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>40 to 105 °C with an interchangeability of <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> °C and measured relative humidity with respect to water with an accuracy of 1.5 %. Due to the cold, dry conditions, and the absence of active ventilation of the sensor package on the CMET, actual measurement errors would be substantially larger than the sensor interchangability, in particular during daytime when the balloon was drifting horizontally, creating an overall warm and dry bias.  This particular CMET-04 was launched in Ny-Ålesund on 30 March 2022 at 14:00 UTC following a trajectory parallel to the simulated trajectory (Fig. <xref ref-type="fig" rid="F1"/>), complementing the dropsonde observations and providing additional in-situ validation data within the lower ABL.</p>

<table-wrap id="T1" specific-use="star"><label>Table 1</label><caption><p id="d2e789">Variables used in the LES for initialisation (<inline-formula><mml:math id="M28" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula>), evaluation (<inline-formula><mml:math id="M29" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>), boundary condition (BC) and larger scale forcing (<inline-formula><mml:math id="M30" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula>).</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="7">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:colspec colnum="5" colname="col5" align="left"/>
     <oasis:colspec colnum="6" colname="col6" align="left"/>
     <oasis:colspec colnum="7" colname="col7" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">Variable</oasis:entry>

         <oasis:entry colname="col2">Unit</oasis:entry>

         <oasis:entry colname="col3">Description</oasis:entry>

         <oasis:entry colname="col4">Instrument</oasis:entry>

         <oasis:entry colname="col5">Platform</oasis:entry>

         <oasis:entry colname="col6">Reference</oasis:entry>

         <oasis:entry colname="col7">Usage</oasis:entry>

       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M31" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">K</oasis:entry>

         <oasis:entry colname="col3">Air temperature</oasis:entry>

         <oasis:entry rowsep="1" colname="col4" morerows="1">Dropsonde, CMET</oasis:entry>

         <oasis:entry rowsep="1" colname="col5" morerows="1">HALO, CMET</oasis:entry>

         <oasis:entry colname="col6"><xref ref-type="bibr" rid="bib1.bibx103" id="text.43"/>,</oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M32" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M33" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"><inline-formula><mml:math id="M34" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">kg kg<sup>−1</sup></oasis:entry>

         <oasis:entry colname="col3">Specific humidity</oasis:entry>

         <oasis:entry colname="col6">
                      <xref ref-type="bibr" rid="bib1.bibx105" id="text.44"/>
                    </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M36" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M37" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M38" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">h Pa</oasis:entry>

         <oasis:entry colname="col3">Pressure</oasis:entry>

         <oasis:entry rowsep="1" colname="col4" morerows="1">Dropsonde</oasis:entry>

         <oasis:entry rowsep="1" colname="col5" morerows="1">HALO</oasis:entry>

         <oasis:entry rowsep="1" colname="col6" morerows="1">
                        <xref ref-type="bibr" rid="bib1.bibx103" id="text.45"/>
                      </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M39" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M40" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"><inline-formula><mml:math id="M41" display="inline"><mml:mrow><mml:mi>u</mml:mi><mml:mo>,</mml:mo><mml:mi>v</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">m s<sup>−1</sup></oasis:entry>

         <oasis:entry colname="col3">Horizontal wind components</oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M43" display="inline"><mml:mi>I</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M44" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi>v</mml:mi><mml:mi>h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>T</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">K<inline-formula><mml:math id="M45" display="inline"><mml:mspace width="0.125em" linebreak="nobreak"/></mml:math></inline-formula>s<sup>−1</sup></oasis:entry>

         <oasis:entry colname="col3">Advection of air temperature</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col5" morerows="4">HALO</oasis:entry>

         <oasis:entry colname="col6" morerows="4">
                        <xref ref-type="bibr" rid="bib1.bibx66" id="text.46"/>
                      </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M47" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M48" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>q</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">kg kg<sup>−1</sup> s<sup>−1</sup></oasis:entry>

         <oasis:entry colname="col3">Advection of specific humidity</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M51" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M52" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>u</mml:mi></mml:mrow></mml:math></inline-formula>,</oasis:entry>

         <oasis:entry colname="col2">m s<sup>−2</sup></oasis:entry>

         <oasis:entry colname="col3">Advection of meridional/zonal wind</oasis:entry>

         <oasis:entry colname="col4">Regression from</oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M54" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M55" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>v</mml:mi></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2"/>

         <oasis:entry colname="col3"/>

         <oasis:entry colname="col4">Dropsondes</oasis:entry>

         <oasis:entry colname="col7"/>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M56" display="inline"><mml:mrow><mml:msub><mml:mi>u</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M57" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">m s<sup>−1</sup></oasis:entry>

         <oasis:entry colname="col3">Geostrophic wind</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M59" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"><inline-formula><mml:math id="M60" display="inline"><mml:mi>w</mml:mi></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">m s<sup>−1</sup></oasis:entry>

         <oasis:entry colname="col3">Subsidence</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col5"/>

         <oasis:entry colname="col6"/>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M62" display="inline"><mml:mi>F</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">K</oasis:entry>

         <oasis:entry colname="col3">Surface skin temperature</oasis:entry>

         <oasis:entry rowsep="1" colname="col4" morerows="1">VELOX</oasis:entry>

         <oasis:entry rowsep="1" colname="col5" morerows="1">HALO</oasis:entry>

         <oasis:entry rowsep="1" colname="col6" morerows="1">
                        <xref ref-type="bibr" rid="bib1.bibx56" id="text.47"/>
                      </oasis:entry>

         <oasis:entry colname="col7">BC</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">sic</oasis:entry>

         <oasis:entry colname="col2">%</oasis:entry>

         <oasis:entry colname="col3">Sea ice fraction</oasis:entry>

         <oasis:entry colname="col7">BC</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M64" display="inline"><mml:mi mathvariant="italic">α</mml:mi></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2"/>

         <oasis:entry colname="col3">Surface albedo</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry rowsep="1" colname="col5" morerows="2">ERA5</oasis:entry>

         <oasis:entry rowsep="1" colname="col6" morerows="2">
                        <xref ref-type="bibr" rid="bib1.bibx29" id="text.48"/>
                      </oasis:entry>

         <oasis:entry colname="col7">BC</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">m</oasis:entry>

         <oasis:entry colname="col3">Roughness length for momentum</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col7">BC</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"><inline-formula><mml:math id="M66" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mrow><mml:mn mathvariant="normal">0</mml:mn><mml:mo>,</mml:mo><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">m</oasis:entry>

         <oasis:entry colname="col3">Roughness length for heat</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col7">BC</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1"><inline-formula><mml:math id="M67" display="inline"><mml:mrow><mml:msubsup><mml:mi>z</mml:mi><mml:mi mathvariant="normal">c</mml:mi><mml:mi>t</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col2">m</oasis:entry>

         <oasis:entry colname="col3">Cloud top height</oasis:entry>

         <oasis:entry colname="col4">AMALi</oasis:entry>

         <oasis:entry colname="col5">P5</oasis:entry>

         <oasis:entry colname="col6">
                      <xref ref-type="bibr" rid="bib1.bibx92" id="text.49"/>
                    </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M68" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">IWV</oasis:entry>

         <oasis:entry colname="col2">kg m<sup>−2</sup></oasis:entry>

         <oasis:entry colname="col3">Integrated water vapour</oasis:entry>

         <oasis:entry colname="col4">HAMP</oasis:entry>

         <oasis:entry colname="col5">HALO</oasis:entry>

         <oasis:entry colname="col6">
                      <xref ref-type="bibr" rid="bib1.bibx50" id="text.50"/>
                    </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M70" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">LWP</oasis:entry>

         <oasis:entry colname="col2">g m<sup>−2</sup></oasis:entry>

         <oasis:entry colname="col3">Liquid water path</oasis:entry>

         <oasis:entry colname="col4">HAMP, MiRAC</oasis:entry>

         <oasis:entry colname="col5">HALO, P5</oasis:entry>

         <oasis:entry colname="col6">
                      <xref ref-type="bibr" rid="bib1.bibx50 bib1.bibx51" id="text.51"/>
                    </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M72" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">IWP</oasis:entry>

         <oasis:entry colname="col2">g m<sup>−2</sup></oasis:entry>

         <oasis:entry colname="col3">Ice water path</oasis:entry>

         <oasis:entry colname="col4">MiRAC</oasis:entry>

         <oasis:entry colname="col5">P5</oasis:entry>

         <oasis:entry colname="col6">
                      <xref ref-type="bibr" rid="bib1.bibx51" id="text.52"/>
                    </oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M74" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula></oasis:entry>

       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Model configuration</title>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>The Dutch Atmospheric Large-Eddy Simulation Model (DALES)</title>
      <p id="d2e1686">The simulations were performed using the Dutch Atmospheric Large-Eddy Simulation (DALES) <xref ref-type="bibr" rid="bib1.bibx30" id="paren.53"/>, which is an open-source model available at <uri>https://github.com/dalesteam/dales</uri> (last access: 2 October 2026). DALES has been tested and applied extensively in previous studies of ABL turbulence and clouds in various regions of the Earth <xref ref-type="bibr" rid="bib1.bibx104 bib1.bibx12 bib1.bibx74 bib1.bibx42 bib1.bibx71" id="paren.54"/>, including the Arctic <xref ref-type="bibr" rid="bib1.bibx61 bib1.bibx15 bib1.bibx17 bib1.bibx11 bib1.bibx79" id="paren.55"/>.</p>
      <p id="d2e1701">To represent Arctic mixed-phase clouds, the DALES code was equipped with the double-moment microphysics scheme of <xref ref-type="bibr" rid="bib1.bibx81" id="text.56"/>, which is predictive of both the mass and number concentrations of five hydrometeor classes (cloud water, cloud ice, rain, snow, and graupel) <xref ref-type="bibr" rid="bib1.bibx61 bib1.bibx11" id="paren.57"/>. The number concentration of cloud condensation nuclei (CCN) is prognostic, initialised with a constant vertical profile of 100 cm<sup>−3</sup> within the range observed during the HALO–<inline-formula><mml:math id="M76" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign in the Fram Strait <xref ref-type="bibr" rid="bib1.bibx111" id="paren.58"/> and in the high Arctic during MOSAiC <xref ref-type="bibr" rid="bib1.bibx2" id="paren.59"/>. The available INP number concentration is prescribed with an upper limit of <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> cm<sup>−3</sup>, following the setup of <xref ref-type="bibr" rid="bib1.bibx11" id="text.60"/> and <xref ref-type="bibr" rid="bib1.bibx28" id="text.61"/>, while the activated fraction depends on temperature and ice supersaturation through the <xref ref-type="bibr" rid="bib1.bibx72" id="text.62"/> parametrisation. Heterogeneous freezing processes are limited to temperatures below <inline-formula><mml:math id="M79" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>15 °C, and the maximum number of ice particles resulting from deposition nucleation is restricted to 200 L<sup>−1</sup>, while homogeneous freezing and secondary ice formation via the Hallett-Mossop process remain unchanged as represented in the <xref ref-type="bibr" rid="bib1.bibx81" id="text.63"/> model. This microphysical model setup was thoroughly tested by <xref ref-type="bibr" rid="bib1.bibx79" id="text.64"/> against a year of in-situ measurements of Arctic clouds in the central Arctic during the MOSAiC expedition.</p>
      <p id="d2e1811">Further model settings follow the setup described by <xref ref-type="bibr" rid="bib1.bibx79" id="text.65"/>. They include a radiative transfer scheme interactive with liquid and ice hydrometeors applying a four-stream radiative transfer solver in combination with Monte Carlo spectral integration <xref ref-type="bibr" rid="bib1.bibx67" id="paren.66"/>. The optical properties of ice particles are based on the physical properties of the ice crystals derived from the microphysics scheme <xref ref-type="bibr" rid="bib1.bibx49 bib1.bibx22 bib1.bibx5 bib1.bibx79" id="paren.67"/>. Resolved advection is calculated using a fifth-order central difference numerical scheme for momentum and a <inline-formula><mml:math id="M81" display="inline"><mml:mi mathvariant="italic">κ</mml:mi></mml:math></inline-formula>-limiter scheme for the other prognostic scalar variables. Subgrid-scale transport uses a prognostic turbulent kinetic energy (SFS-TKE) scheme <xref ref-type="bibr" rid="bib1.bibx14 bib1.bibx33" id="paren.68"/>. A sponge layer is applied in the upper 25 % of the range to dampen disruptive gravity waves. The surface fluxes of heat, moisture, and momentum are calculated based on Monin-Obukhov theory using Arctic stability functions derived by <xref ref-type="bibr" rid="bib1.bibx26" id="text.69"/>. Horizontally periodic boundary conditions are applied, while large-scale forcings are prescribed as time-dependent tendency profiles to account for advection, subsidence, and horizontal pressure gradients (geostrophic wind vector <inline-formula><mml:math id="M82" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).</p>
</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Trajectory calculation</title>
      <p id="d2e1856">To set up a Lagrangian LES experiment, the trajectories (pathways) of the air parcels forming the air mass need to be estimated. Trajectories for the low-level air parcels were calculated during flight planning using the Lagrangian Analysis Tool (LAGRANTO) <xref ref-type="bibr" rid="bib1.bibx91" id="paren.70"/> and based on IFS forecast winds. For this study, this was repeated using 3-D wind fields of the ERA5 reanalysis. Air parcels were identified, and their trajectories were calculated starting every 3 km lat/lon within the IC on 29 March 2022 and passed through the circle locations on 30 March 2022 <xref ref-type="bibr" rid="bib1.bibx39" id="paren.71"/>. The best match of the trajectories was found at 870 hPa in the initiation region. For the simulations, a mean trajectory was calculated by averaging all trajectories initiated within the first circle at 870 hPa. Each trajectory is included for every circle region it intersects, but is excluded from further analysis once it exits a circle region without entering the subsequent one. This procedure is illustrated in Fig. <xref ref-type="fig" rid="FC1"/>.</p>
</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>Observational forcing and boundary conditions</title>
      <p id="d2e1875">The lower boundary conditions are prescribed as time-varying fields along the Lagrangian simulation trajectory with hourly resolution. Surface skin temperature <inline-formula><mml:math id="M83" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and sea-ice concentration “sic” are derived from VELOX observations (Sect. <xref ref-type="sec" rid="Ch1.S2.SS2"/>), longitudinally averaged along the circular flight legs, and interpolated along the simulation trajectory. As the simulated air mass moves from sea ice through the marginal ice zone to the open ocean, this interpolation provides a temporally evolving surface boundary condition. The lower-boundary specific humidity is calculated following <xref ref-type="bibr" rid="bib1.bibx79" id="text.72"/> from the saturation specific humidity at the prescribed surface skin temperature and weighted by the local sea-ice fraction.</p>

      <fig id="F2"><label>Figure 2</label><caption><p id="d2e1896">VELOX observations of surface skin temperature (<inline-formula><mml:math id="M84" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) and sea ice concentration “sic” on the circular flight legs of the HALO flights on 29 March and 30 March 2022 during HALO–<inline-formula><mml:math id="M85" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> (circles), together with interpolated <inline-formula><mml:math id="M86" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and “sic” along the LES trajectory used as surface boundary conditions (bold line).</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f02.png"/>

        </fig>

      <p id="d2e1944">The prescribed large-scale forcing profiles are time-dependent and they are obtained by interpolation along the trajectory between the sonde data at the four circle locations. A regression algorithm is used to estimate horizontal gradients within each circle area, following the method of <xref ref-type="bibr" rid="bib1.bibx6" id="text.73"/>. The horizontal wind divergence and the associated subsidence <inline-formula><mml:math id="M87" display="inline"><mml:mi mathvariant="italic">ω</mml:mi></mml:math></inline-formula> are calculated as described by <xref ref-type="bibr" rid="bib1.bibx66" id="text.74"/>. At high latitudes, Cartesian latitude–longitude coordinates distort horizontal distances. To address this issue, <xref ref-type="bibr" rid="bib1.bibx66" id="text.75"/> introduced a regression method in spherical coordinates <inline-formula><mml:math id="M88" display="inline"><mml:mrow><mml:mfenced open="[" close="]"><mml:mrow><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="italic">φ</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfenced></mml:mrow></mml:math></inline-formula>. Assuming linear fluctuations of any variable <inline-formula><mml:math id="M89" display="inline"><mml:mrow><mml:mi mathvariant="italic">ξ</mml:mi><mml:mo>∈</mml:mo><mml:mfenced close="]" open="["><mml:mrow><mml:mi>u</mml:mi><mml:mo>,</mml:mo><mml:mi>v</mml:mi><mml:mo>,</mml:mo><mml:mi>q</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>,</mml:mo><mml:mi>p</mml:mi></mml:mrow></mml:mfenced></mml:mrow></mml:math></inline-formula> within the dropsonde area, <inline-formula><mml:math id="M90" display="inline"><mml:mi mathvariant="italic">ξ</mml:mi></mml:math></inline-formula> at the centre of the pattern can then be approximated at every vertical level by a first-order Taylor expansion:

            <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M91" display="block"><mml:mrow><mml:mi mathvariant="italic">ξ</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">ξ</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ξ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="italic">θ</mml:mi><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ξ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">φ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="italic">φ</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

          Here, <inline-formula><mml:math id="M92" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ξ</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> denotes the mean of all dropsonde measurements, and <inline-formula><mml:math id="M93" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M94" display="inline"><mml:mi mathvariant="italic">φ</mml:mi></mml:math></inline-formula> are the polar and azimuth angles, respectively. This approach is applied in this study to estimate divergence:

            <disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M95" display="block"><mml:mrow><mml:mi>D</mml:mi><mml:mo>=</mml:mo><mml:mi mathvariant="bold">∇</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>v</mml:mi><mml:mi>h</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mi>r</mml:mi><mml:mo>⋅</mml:mo><mml:mi>sin⁡</mml:mi><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mfenced close="]" open="["><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>u</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">φ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>sin⁡</mml:mi><mml:mi mathvariant="italic">θ</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi>v</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mfenced><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

          This allows for the estimation of the associated subsidence at height <inline-formula><mml:math id="M96" display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> by vertical integration from the surface:

            <disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M97" display="block"><mml:mrow><mml:mi mathvariant="italic">ω</mml:mi><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mi>g</mml:mi><mml:mo>⋅</mml:mo><mml:mi mathvariant="italic">ϱ</mml:mi><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi>z</mml:mi></mml:munderover><mml:mi>D</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">d</mml:mi><mml:mi>z</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>
      <p id="d2e2215">Figure <xref ref-type="fig" rid="F3"/> shows the resulting subsidence profiles in the four circles, provided in pressure and height units for reference, with key characteristics summarised in Table <xref ref-type="table" rid="TC1"/>. In IC and C02, subsidence dominates the lowest 3 km, with mean downward motions of <inline-formula><mml:math id="M98" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.74 and <inline-formula><mml:math id="M99" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.60 cm s<sup>−1</sup>, respectively, while C03 exhibits weaker subsidence throughout the profile. In contrast, C01 shows a mean upward motion over the 8 km profile. Uncertainties associated with the regression-based divergence estimate were calculated following <xref ref-type="bibr" rid="bib1.bibx66" id="text.76"/> and reach up to 0.025 cm s<sup>−1</sup> (0.002 Pa s<sup>−1</sup>) below 3 km across all circles, which cannot be resolved in the figure and are therefore not shown. These estimates reflect uncertainties propagated from the regression analysis and do not represent a complete uncertainty budget, as they exclude potential representativeness errors associated with temporal evolution during the sequential dropsonde releases and deformation of the sampling pattern due to horizontal sonde drift. The method assumes approximate stationarity over the sampling period; sensitivity tests by <xref ref-type="bibr" rid="bib1.bibx66" id="text.77"/> indicate that accounting for pattern deformation changes the derived divergence and pressure velocity by less than 1 % and 10 %, respectively. The subsidence magnitudes are consistent with reanalysis-based estimates of Arctic MCAOs <xref ref-type="bibr" rid="bib1.bibx66 bib1.bibx101" id="paren.78"/>, but are approximately an order of magnitude lower than those reported for the tropical Atlantic, possibly due to the specific weather conditions of the sampled case <xref ref-type="bibr" rid="bib1.bibx6 bib1.bibx24" id="paren.79"/>.</p>

      <fig id="F3" specific-use="star"><label>Figure 3</label><caption><p id="d2e2287">Subsidence profiles obtained through regression from a dropsonde pattern in pressure (<inline-formula><mml:math id="M103" display="inline"><mml:mi mathvariant="italic">ω</mml:mi></mml:math></inline-formula>, solid line) and height (<inline-formula><mml:math id="M104" display="inline"><mml:mi>w</mml:mi></mml:math></inline-formula>, dashed line) coordinate for all dropsonde patterns on 29 March  and 30 March 2022 of the HALO–<inline-formula><mml:math id="M105" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign. Associated uncertainty estimates cannot be resolved in the figure and are discussed in the main text.</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f03.png"/>

        </fig>

      <p id="d2e2327">The same regression approach using spherical coordinates can be applied to calculate the horizontal advective tendencies in the circular areas,

            <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M106" display="block"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="bold">∇</mml:mi><mml:mi mathvariant="italic">ξ</mml:mi><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mfenced open="[" close="]"><mml:mrow><mml:mi>u</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mi>r</mml:mi></mml:mfrac></mml:mstyle><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ξ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mi>r</mml:mi><mml:mo>⋅</mml:mo><mml:mi>sin⁡</mml:mi><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">ξ</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">φ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mfenced><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          and similarly, the horizontal pressure gradient force, here expressed as the geostrophic wind vector <inline-formula><mml:math id="M107" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,

            <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M108" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mi mathvariant="italic">ϱ</mml:mi><mml:mo>⋅</mml:mo><mml:mi>f</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mfenced close=")" open="("><mml:mtable class="array" columnalign="center"><mml:mtr><mml:mtd><mml:mstyle displaystyle="false"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>p</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">φ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mstyle></mml:mtd></mml:mtr><mml:mtr><mml:mtd><mml:mrow><mml:mstyle displaystyle="false"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mi>cos⁡</mml:mi><mml:mi mathvariant="italic">φ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mstyle><mml:mstyle displaystyle="false"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>p</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi mathvariant="italic">θ</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mstyle></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mfenced><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

          These profiles, which extend up to HALO's flight altitude at about 8 km, are linearly interpolated between the four circles and kept constant south of the last circle along the simulation trajectory (Fig. <xref ref-type="fig" rid="F4"/>). What stands out in the interpolated mesoscale vertical pressure velocity field <inline-formula><mml:math id="M109" display="inline"><mml:mrow><mml:mi mathvariant="italic">ω</mml:mi><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is the distinct maximum at C02 below 4 km, which indicates a relatively strong signal in the prescribed subsidence that will play a crucial role in this study. Concerning the advective tendencies, the temperature advection <inline-formula><mml:math id="M110" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="bold">∇</mml:mi><mml:mi>T</mml:mi></mml:mrow></mml:math></inline-formula> is dominated by cooling at low altitudes, below 1 km. The specific humidity exhibits low-level drying before the sea ice edge, transitioning to moistening south of C02. The horizontal wind components show low signals, except for a slight positive tendency of the meridional wind in the deepening ABL south of C01. These likely reflect Ekman-layer effects of Reynolds stresses, inducing a deviation of the wind from the geostrophic wind direction. The geostrophic wind (<inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:mo>|</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub><mml:mo>|</mml:mo></mml:mrow></mml:math></inline-formula>) expresses an eastward zonal pressure gradient force throughout the lower levels, consistent with the general synoptic situation during the 2 d. It should be noted that at a trajectory height of 870 h Pa corresponding to heights between 1.34 and 1.38 km, advective tendencies are, by definition, zero, as the air mass speed is subtracted from the wind in the Lagrangian forcing method.</p>
      <p id="d2e2545">Above 8 km altitude, which is well above the simulated ABL height (max 2 km), the sonde data are extended by ERA5 fields. The main objective of this procedure is to allow radiative flux density (irradiance) calculations above the model domain in which turbulence is resolved, which has a ceiling far below HALO's flight altitude (described in Sect. <xref ref-type="sec" rid="Ch1.S3.SS4"/>). As a result, it is concluded that the use of ERA5 fields above this height has no discernible impact on the model results.</p>

      <fig id="F4" specific-use="star"><label>Figure 4</label><caption><p id="d2e2552">Simulation forcing of subsidence <inline-formula><mml:math id="M112" display="inline"><mml:mi mathvariant="italic">ω</mml:mi></mml:math></inline-formula> (Ctrl) <bold>(a)</bold>, horizontal temperature advection <inline-formula><mml:math id="M113" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>T</mml:mi></mml:mrow></mml:math></inline-formula> <bold>(b)</bold>, horizontal humidity advection <inline-formula><mml:math id="M114" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>q</mml:mi></mml:mrow></mml:math></inline-formula> <bold>(c)</bold>, horizontal advection of the zonal and meridional wind components <inline-formula><mml:math id="M115" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>u</mml:mi></mml:mrow></mml:math></inline-formula> <bold>(d)</bold>, <inline-formula><mml:math id="M116" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">h</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">∇</mml:mi><mml:mi>v</mml:mi></mml:mrow></mml:math></inline-formula> <bold>(e)</bold>, and the geostrophic wind magnitude <inline-formula><mml:math id="M117" display="inline"><mml:mrow><mml:mo>|</mml:mo><mml:msub><mml:mi mathvariant="bold-italic">v</mml:mi><mml:mi mathvariant="normal">g</mml:mi></mml:msub><mml:mo>|</mml:mo></mml:mrow></mml:math></inline-formula> <bold>(f)</bold>. All fields are interpolated between dropsonde observation locations IC, C01, C02 and C03 (dashed blue lines). The surface cover is indicated at the bottom of each subfigure as sea ice (sic <inline-formula><mml:math id="M118" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, light blue), marginal sea-ice zone (<inline-formula><mml:math id="M119" display="inline"><mml:mrow><mml:mtext>0</mml:mtext><mml:msub><mml:mo>&lt;</mml:mo><mml:mi mathvariant="normal">sic</mml:mi></mml:msub><mml:mo>≤</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, hatched), and open ocean (sic <inline-formula><mml:math id="M120" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mtext>0</mml:mtext></mml:mrow></mml:math></inline-formula>, dark blue).</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f04.png"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS4">
  <label>3.4</label><title>Experimental setup</title>
      <p id="d2e2724">Apart from the control setup, four additional LES experiments are conducted using DALES to investigate the sensitivity of ABL evolution to the mesoscale subsidence forcing. The experimental setup includes (i) the control simulation (Ctrl) that employs the observed subsidence (Sect. <xref ref-type="sec" rid="Ch1.S3.SS3"/>), (ii) a simulation without subsidence (NoSub) to isolate the effects of entrainment on ABL development, and (iii) further experiments in which observed subsidence was scaled by 10 % (Sub10), 50 % (Sub50) and 200 % (Sub200). These scaling factors correspond to a range of subsidence rates covering weaker values (<inline-formula><mml:math id="M121" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.12 cm s<sup>−1</sup>) comparable to those used in LES studies of mixed-phase Arctic clouds <xref ref-type="bibr" rid="bib1.bibx88 bib1.bibx116" id="paren.80"/>, up to stronger rates of approximately <inline-formula><mml:math id="M123" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.3 cm s<sup>−1</sup>, and consistent with observations during the EUREC<sup>4</sup>. A campaign in the tropics <xref ref-type="bibr" rid="bib1.bibx69" id="paren.81"/>. In all sensitivity experiments, the temporal and vertical structure of the observed subsidence was retained, while only its magnitude was modified.</p>
      <p id="d2e2783">The model domain spans 12.8 km <inline-formula><mml:math id="M126" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 12.8 km with 50 m horizontal resolution and 191 vertical levels, starting at 10 m with 20 m spacing up to 2.1 km and increasing resolution aloft to a ceiling height of 6.8 km with maximum grid spacing of 177 m. Periodic horizontal boundaries are applied, and large-scale forcings are horizontally homogeneous but variable in time and height along the trajectory. The prescribed subsidence acts on the evolving model profile. Continuous Newtonian nudging towards the observed profiles of <inline-formula><mml:math id="M127" display="inline"><mml:mrow><mml:mo mathvariant="italic">{</mml:mo><mml:mi>T</mml:mi><mml:mo>,</mml:mo><mml:mi>q</mml:mi><mml:mo>,</mml:mo><mml:mi>u</mml:mi><mml:mo>,</mml:mo><mml:mi>v</mml:mi><mml:mo mathvariant="italic">}</mml:mo></mml:mrow></mml:math></inline-formula> is applied above the ABL, determined by the strongest inversion in liquid water potential temperature, with a buffer layer of 100 m where the nudging time scale increases linearly up to 3 h. Nudging increases in the upper quarter of the domain to suppress gravity waves, while below the ABL, the flow evolved freely. Each experiment is 45 h long, reaching the marginal sea ice zone approximately 15 h after initialisation.</p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Results I: Evaluation of the control simulation</title>
      <p id="d2e2826">In this section, we evaluate the performance of the control (Ctrl) LES in reproducing key characteristics of the MCAO observed on 29 March and 30 March 2022 during the HALO–<inline-formula><mml:math id="M128" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> campaign. We analyse the evolution of cloud liquid and ice water contents and paths, the vertical structure and evolution of the ABL height, air temperature and humidity profiles along the simulation trajectory, and the associated turbulent heat energy fluxes. As outlined in Sect. <xref ref-type="sec" rid="Ch1.S2"/>, observations from dropsondes, lidars, and radiometers are used to assess the model's ability to capture the spatial and temporal variability of the atmosphere, and the representation of turbulent and thermodynamic processes.</p>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Atmospheric boundary layer and cloud evolution</title>
      <p id="d2e2855">First, we examine the evolution of the ABL and clouds, focusing on the temporal development of cloud liquid and ice water contents as well as the deepening of the ABL along the simulation trajectory of the MCAO, expressed as a function of latitude in Fig. <xref ref-type="fig" rid="F5"/>. The initial atmospheric column at circle IC includes a shallow ABL of 65 m, which remains low over the sea ice in the simulation. The ABL begins to deepen once it reaches the marginal sea ice zone (MIZ) where warmer surface conditions trigger enhanced vertical latent and sensible heat fluxes. Convective updrafts form a thin mixed-phase cloud between C01 and C02, with ice reaching to the surface and a shallow liquid layer existing near the cloud top during the initial phase of the growing ABL. As the air mass moves over the open ocean, the ABL continues to deepen, reaching values of liquid water content <inline-formula><mml:math id="M129" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> up to 0.35 g kg<sup>−1</sup>. At the end of the 45 h simulation, the ABL has grown to approximately 1.5 km.</p>
      <p id="d2e2883">To evaluate the Ctrl simulation with respect to the ABL structure, several independent measurements of ABL height are compared with the simulation output. The ABL height was determined from dropsonde profiles using the Bulk Richardson number <inline-formula><mml:math id="M131" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:msub><mml:mi>i</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, which quantifies the balance between buoyancy and shear <xref ref-type="bibr" rid="bib1.bibx97" id="paren.82"/>. A critical threshold <inline-formula><mml:math id="M132" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:msubsup><mml:mi>i</mml:mi><mml:mi mathvariant="normal">b</mml:mi><mml:mtext>crit</mml:mtext></mml:msubsup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.25</mml:mn></mml:mrow></mml:math></inline-formula> was used to define the height of the ABL <inline-formula><mml:math id="M133" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, consistent with the diagnostics of the IFS CY43R1 model and the ERA5 reanalysis <xref ref-type="bibr" rid="bib1.bibx16 bib1.bibx80" id="paren.83"/>. Lidar measurements from the P5 aircraft (AMALi) provide cloud top height (<inline-formula><mml:math id="M134" display="inline"><mml:mrow><mml:msubsup><mml:mi>z</mml:mi><mml:mi mathvariant="normal">c</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula>), which is comparable to the ABL height in MCAO cases due to the strong coupling of ABL growth to cloud development. Finally, the simulation diagnoses the height of the ABL from the minimum flux of total liquid water potential temperature <xref ref-type="bibr" rid="bib1.bibx94" id="paren.84"/>, <inline-formula><mml:math id="M135" display="inline"><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>, within the lowest 3 km of the domain. AMALi measured a mean cloud top height of 0.63<inline-formula><mml:math id="M136" display="inline"><mml:mrow><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>±</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/></mml:mrow></mml:math></inline-formula>0.11 km at location C02, yielding an RMSE of 0.12 km compared to the simulation ABL height. The ABL height derived from the dropsondes was 0.07 km at C01, 0.43 km at C02, and 1.04 km at C03, resulting in an overall root mean square error (RMSE) of 0.14 km compared to the simulation. The conclusion from this evaluation against the three datasets is that the model reproduces the observed ABL height within 150 m throughout the simulation. The temporarily reduced deepening rate between C02 and C03 in the simulation is supported by the measured data, which is an interesting feature that could be related to the low-level maximum in subsidence during that period (Fig. <xref ref-type="fig" rid="F4"/>a).</p>

      <fig id="F5" specific-use="star"><label>Figure 5</label><caption><p id="d2e2987">Latitudinal evolution of cloud liquid (grey contour lines) and ice (red filled contours) along the MCAO trajectory. Results from the 45 h semi-Lagrangian DALES simulation Ctrl are shown, including model ABL height (red dashed), compared to dropsonde ABL heights (<inline-formula><mml:math id="M137" display="inline"><mml:mo lspace="0mm">▾</mml:mo></mml:math></inline-formula>) and cloud-top heights from AMALi lidar aboard the P5 aircraft (light blue boxplot, outliers not shown for better visibility). Dashed vertical lines indicate dropsonde circle locations.</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f05.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Temperature and humidity profiles</title>
      <p id="d2e3011">The vertical structure of virtual potential temperature (<inline-formula><mml:math id="M138" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and specific humidity (<inline-formula><mml:math id="M139" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>) in the Ctrl experiment is evaluated against in-situ observations from HALO dropsondes, closest to the simulation trajectory; the variability of all soundings in each circle is indicated as blue shading in Fig. <xref ref-type="fig" rid="F6"/>. This comparison reveals possible systematic biases in the thermodynamic state. Figure <xref ref-type="fig" rid="F6"/> focuses on the lowest 3 km of the atmosphere to highlight the ABL properties. Above 3 km altitude, the simulation closely follows the observed vertical structure of <inline-formula><mml:math id="M140" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> at all three locations. Larger differences occur for <inline-formula><mml:math id="M141" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>, primarily due to observed humidity layers not being captured in the smoother simulated humidity structure.</p>
      <p id="d2e3055">In the region of C01 (Fig. <xref ref-type="fig" rid="F6"/>a and d), located above sea ice near its edge, an inversion in <inline-formula><mml:math id="M142" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is detected near the surface at 30 m in the simulation, and at 20 m in the dropsonde profiles, with a thermodynamic wind profile above it. The simulated near surface <inline-formula><mml:math id="M143" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M144" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>25.6 °C differs by 1.4 K from the dropsonde observations of <inline-formula><mml:math id="M145" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>24.2 °C and lies within the observed variability. The humidity profiles show greater variability among the dropsondes, with several observed humid layers not captured by the smoother simulated profile; nevertheless, the simulation closely follows the vertical structure of the observed profiles. The near-surface value of <inline-formula><mml:math id="M146" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> at C01 was 0.5 g<inline-formula><mml:math id="M147" display="inline"><mml:mspace width="0.125em" linebreak="nobreak"/></mml:math></inline-formula>km<sup>−1</sup> in the simulation and 0.54 g<inline-formula><mml:math id="M149" display="inline"><mml:mspace width="0.125em" linebreak="nobreak"/></mml:math></inline-formula>kg<sup>−1</sup> in the observations. The close correspondence at C01 reflects the continuous nudging that is active above the ABL top, which is still very low at this stage.</p>
      <p id="d2e3141">As the air mass moved over the marginal sea ice zone (MIZ) and the open ocean to the location of C02 (Fig. <xref ref-type="fig" rid="F6"/>b and e), surface warming caused an increase in the near surface air temperature <inline-formula><mml:math id="M151" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mrow><mml:mi mathvariant="normal">v</mml:mi><mml:mo>,</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> in the simulation of <inline-formula><mml:math id="M152" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>14.5 K to <inline-formula><mml:math id="M153" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>11.1 °C, while observed warming was even stronger with a measured increase in <inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mrow><mml:mi mathvariant="normal">v</mml:mi><mml:mo>,</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M155" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>15.6 K to <inline-formula><mml:math id="M156" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>8.6 °C. The inversion height was approximately 590 m in both profiles, but the simulated inversion was less steep. Below the inversion, the model shows a cold deviation of 3.3 K, while reproducing the observed mixed-layer structure and inversion height. The increase in evaporation over the open ocean led to an increase in humidity, with surface moisture <inline-formula><mml:math id="M157" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> of 1.5 g kg<sup>−1</sup> in the simulation and 1.6 g kg<sup>−1</sup> in the observations. Both show a pronounced drop in humidity near 590 m, with the observed jump being stronger and sharper than the simulation, induced by the prescribed advection of <inline-formula><mml:math id="M160" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (shown in Fig. <xref ref-type="fig" rid="F4"/>c). Within the mixed layer, where temperature and humidity are uniform with height, the model underestimates the humidity by an average of 0.2 g g<sup>−1</sup>. Above the temperature inversion, additional differences result from observed moisture layers that are not captured in the simulation.</p>
      <p id="d2e3268">Further south, over the open ocean at C03 (Fig. <xref ref-type="fig" rid="F6"/>c and f), the ABL has deepened further and <inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> has continued to increase, with a simulated surface value of <inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mrow><mml:mi mathvariant="normal">v</mml:mi><mml:mo>,</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M164" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.5 °C and an observed value of <inline-formula><mml:math id="M165" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>4.6 °C representing an underestimation of near-surface warming by 2.9 K. The modelled inversion base is at 830 m, compared to 1000 m in the observations, with the simulated inversion being less steep. Below the temperature inversion, the model underestimates <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> by approximately 2 K. Therefore, there is a consistent cold bias of <inline-formula><mml:math id="M167" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2 to <inline-formula><mml:math id="M168" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>3 K across all circles, a tendency also found by <xref ref-type="bibr" rid="bib1.bibx112" id="text.85"/> in the limited-area configuration of the ICON model for all observed MCAO cases of HALO–<inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> and may reflect uncertainties in the prescribed surface skin temperature and limitations of the bulk surface-flux parametrisation. The humidity in the boundary layer at C03 has also increased further, reaching 1.7 g kg<sup>−1</sup> in the simulation and 2 g kg<sup>−1</sup> in the observations, with the model underestimating the surface layer of high humidity directly above the ocean. The simulated humidity jump is also weaker than observed. Below the temperature inversion, the model underestimates <inline-formula><mml:math id="M172" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> by 0.2 g kg<sup>−1</sup>.</p>
      <p id="d2e3405">Additional measurements taken with the CMET sonde drifting south along a similar trajectory further support these results. At the same latitude as C01, the CMET flew at an altitude of 340 m at a distance of 225 km to the simulated trajectory. The CMET reached the latitude of interest about 2.5 h later than the simulated air parcel. Here, <inline-formula><mml:math id="M174" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mtext>8.8</mml:mtext></mml:mrow></mml:math></inline-formula> °C and <inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mtext>0.52</mml:mtext></mml:mrow></mml:math></inline-formula> g kg<sup>−1</sup> were measured, which largely corresponds to the simulation in terms of humidity (difference of only 0.02 g kg<sup>−1</sup>), but with <inline-formula><mml:math id="M178" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> being 5.7 K warmer, which may be due to the proximity to Svalbard and the associated local warming effects. As the trajectory of CMET was closer to Svalbard and travelled through the cloud-free region associated with lee-effects, likely causing a warming of the lower layers. The CMET reached the latitude of C02 7.5 h later at a distance of 132 km from the simulated trajectory. The CMET measured at 902 m above sea level a temperature of <inline-formula><mml:math id="M179" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mtext>1.8</mml:mtext></mml:mrow></mml:math></inline-formula> °C and <inline-formula><mml:math id="M180" display="inline"><mml:mrow><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mtext>0.25</mml:mtext></mml:mrow></mml:math></inline-formula> g kg<sup>−1</sup>, which is 3.7 K warmer and 0.2 g kg<sup>−1</sup> drier than the simulation. At C03, the CMET was 2 h later and 149 km away from the simulation at an altitude of 1780 m. A virtual potential temperature <inline-formula><mml:math id="M183" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of 2.7 °C was measured, 1.8 K warmer than in the model and <inline-formula><mml:math id="M184" display="inline"><mml:mrow><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mtext>0.78</mml:mtext></mml:mrow></mml:math></inline-formula> g kg<sup>−1</sup>, only 0.06 g kg<sup>−1</sup> more humid. As the CMET moved south and the influence of Svalbard diminished, the measured air mass increasingly resembled that observed by the dropsondes, with the humidity in all three circles corresponding very closely to the simulated <inline-formula><mml:math id="M187" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> values measured by the dropsondes.</p>
      <p id="d2e3581">The overall conclusion from these results is that the LES model reproduces the observed evolution in the vertical thermodynamic structure after C01 to a reasonable degree. This is not trivial, as the nudging takes place above the temperature inversion only, and below it, the simulated ABL is free to evolve. A slight cold and dry bias is evident within the ABL, and the inversions at its top height appear less pronounced than observed. These differences may arise from (i) uncertainties in the surface boundary condition <inline-formula><mml:math id="M188" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>skin</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, and (ii) shortcomings in the bulk flux parametrisation at the surface. Nevertheless, the overall correspondence between simulation and observation indicates that the model adequately reproduces the thermodynamic structure of the observed MCAO, providing a robust basis for further analysis.</p>

      <fig id="F6" specific-use="star"><label>Figure 6</label><caption><p id="d2e3597">Vertical profiles of virtual potential temperature (<inline-formula><mml:math id="M189" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and specific humidity (<inline-formula><mml:math id="M190" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>). Dropsonde profile (blue) of the dropsonde closest to the simulation trajectory and spread between values measured by 10 sondes per circle (shading); simulation profiles are shown in red. CMET measurements are indicated as blue dots.</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f06.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Integrated water paths</title>
      <p id="d2e3632">The model performance in representing various column-integrated quantities is assessed next. In Fig. <xref ref-type="fig" rid="F7"/>a, the simulated integrated water vapour (IWV) is evaluated against observations from two sources. The first source are the data from the HAMP radiometer on board HALO which measured along the flight trajectory, and the second is the IWV determined from the dropsonde humidity profiles, averaged over the ten sondes in each circular pattern. The simulation accurately replicated the observed IWV at C01 of 1.9 kg m<sup>−2</sup> with a small difference of 0.1 kg m<sup>−2</sup>. At C02, the dropsondes measured 2.7 kg m<sup>−2</sup> IWV, reproduced with <inline-formula><mml:math id="M194" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.04 kg m<sup>−1</sup> in the simulation. At C03, the observed IWV was 4.4 kg m<sup>−2</sup>, which the simulation slightly overestimated by <inline-formula><mml:math id="M197" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.3 kg m<sup>−2</sup>. This temporal evolution of IWV closely follows the HAMP observations, with an RMSE of 0.2 kg m<sup>−2</sup> compared to the simulation. These results suggest that the net input of humidity into the deepening ABL is well captured by the model.</p>
      <p id="d2e3736">Figure <xref ref-type="fig" rid="F7"/>b compares the simulated LWP against two measurements. The LWP retrieved from HAMP onboard HALO exhibits a much higher short-term variability than in the simulation, resulting in an RMSE of 30 g m<sup>−2</sup>. Despite this, the overall temporal evolution aligns with the simulated LWP, with liquid water strongly increasing after the MIZ. The MiRAC instrument on P5 showed even higher variability due to its high spatial resolution and low flight altitude above the clouds. When averaged, MiRAC observations yield a mean LWP of 0.01 g m<sup>−2</sup>, which appears much lower than the simulated LWP of 12 g m<sup>−2</sup>, but the simulation value lies within the spread of the LWP observed by MiRAC. These results suggest that, while the observed LWP fluctuates more strongly due to higher resolution, capturing individual cloud streets, than the smoother, domain-average model output, the simulation captures the general trend and magnitude of the evolution of liquid water throughout the event.</p>
      <p id="d2e3777">The simulated ice water path of all frozen hydrometeors IWP shown in Fig. <xref ref-type="fig" rid="F7"/>c is only compared to MiRAC measurements aboard P5. The IWP retrievals by HALO were excluded due to large uncertainties for this case. The average observed IWP from MiRAC was 0.6 g m<sup>−2</sup>, but similar to the LWP observations, the variability due to the high resolution of individual clouds is large and values range up to 6.2 g m<sup>−2</sup>. This high variability may also result from the substantial uncertainties associated with IWP retrievals. The Ze–IWC relationship of <xref ref-type="bibr" rid="bib1.bibx32" id="text.86"/> exhibits uncertainties around a factor of 2, caused by the strong temperature dependence of ice particle size distributions and densities. At warmer temperatures, the ice water content IWC tends to be overestimated, whereas at colder temperatures it is generally underestimated. This temperature sensitivity is particularly relevant for 94 GHz radar, where Mie-scattering further increases the retrieval uncertainty. Compared to the simulated IWP in the location of the P5 measurements of 2.58 g m<sup>−2</sup>, an RMSE of 73.34 g m<sup>−2</sup> is found. It should also be noted that the P5 observations do not coincide with the air mass trajectory but were collected at a later time, limiting the comparability of the data (Fig. <xref ref-type="fig" rid="F1"/>). A notable feature of the latitudinal evolution of the simulated IWP is the local maximum reached in the simulation just before C02; the realism cannot be verified due to the absence of reliable IWP measurements along the whole trajectory.</p>
</sec>
<sec id="Ch1.S4.SS4">
  <label>4.4</label><title>Surface heat fluxes</title>
      <p id="d2e3845">The surface heat fluxes are key drivers of ABL evolution in MCAOs. To evaluate the simulated sensible (<inline-formula><mml:math id="M207" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula>) and latent (<inline-formula><mml:math id="M208" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>) heat fluxes, we estimate these data from dropsonde observations following the thermodynamic method suggested by <xref ref-type="bibr" rid="bib1.bibx27" id="text.87"/>. This method assumes steady-state conditions, negligible radiative divergence and cross-flow advection, and minimal entrainment above the mixed layer. Here, following <xref ref-type="bibr" rid="bib1.bibx27" id="text.88"/>, the steady-state assumption allows thermodynamic differences between successive downstream profiles to be interpreted as along-flow advective changes and linked to the vertically integrated surface heat and moisture input. Then, the sensible and latent heat energy fluxes can be calculated as

            <disp-formula id="Ch1.E6" content-type="numbered"><label>6</label><mml:math id="M209" display="block"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">DS</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="italic">ϱ</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>c</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:msub><mml:mi>u</mml:mi><mml:mi mathvariant="normal">ML</mml:mi></mml:msub><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">0</mml:mn></mml:munderover><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="italic">ϑ</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">d</mml:mi><mml:mi>z</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi>H</mml:mi><mml:mtext>C</mml:mtext></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula></p>
      <p id="d2e3936">
            <disp-formula id="Ch1.E7" content-type="numbered"><label>7</label><mml:math id="M210" display="block"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">DS</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="italic">ϱ</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:msub><mml:mi>u</mml:mi><mml:mi mathvariant="normal">ML</mml:mi></mml:msub><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow><mml:mn mathvariant="normal">0</mml:mn></mml:munderover><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">d</mml:mi><mml:mi>z</mml:mi><mml:mo>+</mml:mo><mml:msub><mml:mi>H</mml:mi><mml:mtext>C</mml:mtext></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M211" display="inline"><mml:mi mathvariant="italic">ϱ</mml:mi></mml:math></inline-formula> represents the air density, <inline-formula><mml:math id="M212" display="inline"><mml:mrow><mml:msub><mml:mi>c</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the specific heat capacity, <inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the latent heat of evaporation, <inline-formula><mml:math id="M214" display="inline"><mml:mrow><mml:msub><mml:mi>u</mml:mi><mml:mi mathvariant="normal">ML</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the mean horizontal wind speed within the mixed layer and <inline-formula><mml:math id="M215" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> the height of the ABL. <inline-formula><mml:math id="M216" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:math></inline-formula> is the horizontal distance between two profiles. The contribution of condensational heating within the cloud layer is represented by the following formulas:</p>
      <p id="d2e4071">
            <disp-formula id="Ch1.E8" content-type="numbered"><label>8</label><mml:math id="M217" display="block"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="italic">ϱ</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:msub><mml:mi>u</mml:mi><mml:mi mathvariant="normal">ML</mml:mi></mml:msub><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:munderover><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>l</mml:mi></mml:mrow><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>y</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">d</mml:mi><mml:mi>z</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M218" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represents the height of the cloud base, defined as the lowest altitude at which the relative humidity reaches saturation with respect to the ice or liquid. Meanwhile, <inline-formula><mml:math id="M219" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>l</mml:mi></mml:mrow></mml:math></inline-formula> refers to the difference in <inline-formula><mml:math id="M220" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> between the profiles, which is approximated as the upper limit of <inline-formula><mml:math id="M221" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> within the cloud layer. This is estimated as the difference of <inline-formula><mml:math id="M222" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> within the cloud and the average <inline-formula><mml:math id="M223" display="inline"><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mtext>t,BC</mml:mtext></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> below the cloud layer, following <xref ref-type="bibr" rid="bib1.bibx27" id="text.89"/>. In the model, the surface heat fluxes can be sampled continuously as</p>
      <p id="d2e4213">

                <disp-formula specific-use="align" content-type="numbered"><mml:math id="M224" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E9"><mml:mtd><mml:mtext>9</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi>H</mml:mi><mml:mtext>Ctrl</mml:mtext></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mo>=</mml:mo><mml:mi mathvariant="italic">ϱ</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>c</mml:mi><mml:mi mathvariant="normal">p</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E10"><mml:mtd><mml:mtext>10</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msub><mml:mi>E</mml:mi><mml:mtext>Ctrl</mml:mtext></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mo>=</mml:mo><mml:mi mathvariant="italic">ϱ</mml:mi><mml:mo>⋅</mml:mo><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mi>q</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            with <inline-formula><mml:math id="M225" display="inline"><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M226" display="inline"><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mi>q</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> representing the turbulent kinematic fluxes of temperature and moisture at the surface.</p>
      <p id="d2e4354">The simulation produced <inline-formula><mml:math id="M227" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mtext>Ctrl</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> values up to 830 W m<sup>−2</sup> and <inline-formula><mml:math id="M229" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mtext>Ctrl</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> values up to 102 W m<sup>−2</sup> over the open ocean. In particular, the sensible heat flux is substantially higher than the climatological mean sensible flux of about 200 W m<sup>−2</sup> during MCAOs, while the latent heat flux is comparable to the climatological mean latent heat flux of 100 W m<sup>−2</sup> reported by <xref ref-type="bibr" rid="bib1.bibx62" id="text.90"/> for MCAOs in the region west of Svalbard. The difference in potential temperature between the near-surface atmosphere and the ocean surface causes a direct response in the sensible heat flux, while the latent heat flux is limited by the saturation specific humidity at the sea surface temperature <xref ref-type="bibr" rid="bib1.bibx63 bib1.bibx62" id="paren.91"/>. In the observed region, <inline-formula><mml:math id="M233" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> was generally more efficient than <inline-formula><mml:math id="M234" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> in extracting energy from the ocean surface, but the relative importance of <inline-formula><mml:math id="M235" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula> increased as the air is mass advected away from the sea-ice edge over warmer waters. South of 75° N, the mean values of <inline-formula><mml:math id="M236" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mtext>Ctrl</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M237" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mtext>Ctrl</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> were 69 and 17 W m<sup>−2</sup>, respectively, consistent with the findings of <xref ref-type="bibr" rid="bib1.bibx10" id="text.92"/>.</p>
      <p id="d2e4493">Dropsonde-derived <inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">DS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> values considerably underestimate simulated surface sensible heat fluxes by 564 W m<sup>−2</sup> between C01 and C02 and 306 W m<sup>−2</sup> between C02 and C03. We speculate that this offset is mostly due to numerous assumptions in the method of deriving fluxes from observed profiles. To improve comparability between model and measurements and gain further insight, the same diagnostic technique is applied to the simulated profiles (Fig. <xref ref-type="fig" rid="F6"/>), yielding much better agreement. The associated RMSE between <inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mtext>DS</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mtext>Ctrl, Prof</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is 95 W m<sup>−2</sup>. Between C02 and C03, the thermodynamic method yields a simulated value of only <inline-formula><mml:math id="M245" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mtext>Ctrl, Prof</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mtext>21</mml:mtext></mml:mrow></mml:math></inline-formula> W m<sup>−2</sup>, compared to <inline-formula><mml:math id="M247" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mtext>DS</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mtext>170</mml:mtext></mml:mrow></mml:math></inline-formula> W m<sup>−2</sup>, largely underestimating the surface sensible heat flux. Note that the dropsonde-derived <inline-formula><mml:math id="M249" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">DS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in the marginal ice zone (C01–C02) is very small (2.6 W m<sup>−2</sup>) compared to the simulated fluxes that exceeded 100 W m<sup>−2</sup>, but increased to 16 W m<sup>−2</sup> between C02 and C03, closer to the simulated values. The RMSE of 8.9 W m<sup>−2</sup> between <inline-formula><mml:math id="M254" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">DS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M255" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mtext>Ctrl, Prof</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> indicates that although the observational profile-based method struggles to fully capture the true flux magnitudes in the early MCAO phase, it reproduces their relative variability well when applied consistently.</p>

      <fig id="F7" specific-use="star"><label>Figure 7</label><caption><p id="d2e4707">Latitudinal evolution of various bulk properties of the simulated MCAO in the Ctrl experiment. <bold>(a)</bold> Integrated water vapour IWV simulation (red line) compared to longitudinally averaged observations from HALO (blue line) and estimates based on dropsonde data (<inline-formula><mml:math id="M256" display="inline"><mml:mo lspace="0mm">▾</mml:mo></mml:math></inline-formula>). <bold>(b)</bold> Simulated liquid water path LWP and <bold>(c)</bold> ice water path IWP (red lines) compared to HALO (dark blue line) and P5 (light blue boxplot, outliers not shown for better visibility) observations. <bold>(d)</bold> Simulated surface latent (<inline-formula><mml:math id="M257" display="inline"><mml:mi>E</mml:mi></mml:math></inline-formula>, red line) and sensible (<inline-formula><mml:math id="M258" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula>, yellow line) heat fluxes compared to estimates based on dropsonde data following the method of <xref ref-type="bibr" rid="bib1.bibx27" id="text.93"/> (<inline-formula><mml:math id="M259" display="inline"><mml:mo lspace="0mm">▾</mml:mo></mml:math></inline-formula>). The same method applied to model profiles is also shown, for reference (<inline-formula><mml:math id="M260" display="inline"><mml:mo lspace="0mm">×</mml:mo></mml:math></inline-formula>). In all figures, the vertical dashed lines mark the location of the dropsonde circles. The coloured bar at the bottom indicates sea ice (sic <inline-formula><mml:math id="M261" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, light blue), marginal sea-ice (<inline-formula><mml:math id="M262" display="inline"><mml:mrow><mml:mtext>0</mml:mtext><mml:mo>&lt;</mml:mo><mml:mi mathvariant="normal">sic</mml:mi><mml:mo>≤</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, hatched), and open ocean (sic <inline-formula><mml:math id="M263" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mtext>0</mml:mtext></mml:mrow></mml:math></inline-formula>, dark blue).</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f07.png"/>

        </fig>

</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Results II: Subsidence impacts</title>
      <p id="d2e4814">The results discussed so far indicate that the Ctrl simulation reproduces the temporal evolution of the ABL well, including various water paths and surface energy fluxes. Therefore, the Ctrl experiment represents a robust and realistic foundation for subsequent Lagrangian LES sensitivity experiments, as applied in this section to investigate the impact of mesoscale subsidence on the ABL and cloud evolution. In total, five experiments with differing mesoscale subsidence are performed and analysed. As described in Sect. <xref ref-type="sec" rid="Ch1.S3.SS4"/>, four additional experiments were conducted with the Ctrl subsidence field multiplied by a factor <inline-formula><mml:math id="M264" display="inline"><mml:mrow><mml:mo mathvariant="italic">{</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mn mathvariant="normal">0.1</mml:mn><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mn mathvariant="normal">0.5</mml:mn><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mn mathvariant="normal">2.0</mml:mn><mml:mo mathvariant="italic">}</mml:mo></mml:mrow></mml:math></inline-formula>, respectively.</p>
<sec id="Ch1.S5.SS1">
  <label>5.1</label><title>Sensitivity analysis</title>
      <p id="d2e4854">Figure <xref ref-type="fig" rid="F8"/> shows the evolution of <inline-formula><mml:math id="M265" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M266" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> along the MCAO trajectory. In the no-subsidence (NoSub)  setup, the cloudy ABL deepens the fastest, approaching the parabolic deepening rate (<inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:msup><mml:mi>t</mml:mi><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) after the air mass moves over the open ocean <xref ref-type="bibr" rid="bib1.bibx93" id="paren.94"/>. In this setup, the cloud mass is the largest, both in liquid and frozen form. The higher the prescribed subsidence forcing, the more the ABL deepening driven by turbulent/convective entrainment is suppressed by subsidence. This in particular applies during the time period between C02 and C03, where the observed low-level subsidence has its maximum (Fig. <xref ref-type="fig" rid="F4"/>a). This leads to the development of thinner clouds and less <inline-formula><mml:math id="M268" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M269" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. In the Sub200 case, only a very thin, shallow mixed-phase cloud is observed.</p>

      <fig id="F8"><label>Figure 8</label><caption><p id="d2e4929">Latitudinal evolution of cloud liquid (grey)  and ice (red) along the MCAO trajectory for all sensitivity experiments. Dashed horizontal lines indicate dropsonde circle locations. Boundary layer height <inline-formula><mml:math id="M270" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud base <inline-formula><mml:math id="M271" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are indicated by grey dashed and dot-dashed lines, respectively. The markers <inline-formula><mml:math id="M272" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> and <inline-formula><mml:math id="M273" display="inline"><mml:mo>▴</mml:mo></mml:math></inline-formula> indicate decoupling points and heights with respect to <inline-formula><mml:math id="M274" display="inline"><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> and <inline-formula><mml:math id="M275" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M276" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> respectively (Sect. <xref ref-type="sec" rid="Ch1.S5.SS2"/> for definition). The coloured bar at the bottom indicates sea ice (sic <inline-formula><mml:math id="M277" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, light blue), marginal sea-ice (<inline-formula><mml:math id="M278" display="inline"><mml:mrow><mml:mtext>0</mml:mtext><mml:mo>&lt;</mml:mo><mml:mi mathvariant="normal">sic</mml:mi><mml:mo>≤</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, hatched), and open ocean (sic <inline-formula><mml:math id="M279" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mtext>0</mml:mtext></mml:mrow></mml:math></inline-formula>, dark blue).</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f08.png"/>

        </fig>

      <p id="d2e5060">To gain more insight into the spatial structure of the cloud field, Fig. <xref ref-type="fig" rid="F9"/> presents horizontal cross-sections of <inline-formula><mml:math id="M280" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M281" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> through the centre of the simulated domain for all five simulations. These locations are sampled at regular intervals along the trajectory, beginning at C01 near the sea-ice edge and extending southward to 73.25° N at the end of the simulation period. The grey shading highlights regions in which the cloud layer is decoupled from the surface, following the criterion of <xref ref-type="bibr" rid="bib1.bibx36" id="text.95"/>. This diagnostic is defined by the thresholds <inline-formula><mml:math id="M282" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mover accent="true"><mml:mi>q</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mrow><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mtext>bot</mml:mtext></mml:mrow></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mover accent="true"><mml:mi>q</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mrow><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mtext>top</mml:mtext></mml:mrow></mml:msub><mml:mo>&gt;</mml:mo><mml:mtext>0.5</mml:mtext></mml:mrow></mml:math></inline-formula> g kg<sup>−1</sup>, based on the layer-mean total-water mixing ratio in the upper and lower 25 % of the boundary layer, and <inline-formula><mml:math id="M284" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mtext>l,top</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mtext>l,bot</mml:mtext></mml:msub><mml:mo>&gt;</mml:mo><mml:mtext>0.5</mml:mtext></mml:mrow></mml:math></inline-formula> K, calculated analogously for the layer-mean liquid-water potential temperature. These metrics have been associated with the onset of boundary-layer decoupling and the subsequent transition from roll convection to open-cell structures in MCAOs <xref ref-type="bibr" rid="bib1.bibx37 bib1.bibx1" id="paren.96"/>. What stands out during the decoupled phase is the presence of liquid-phase shallow cumulus clouds, rising into the capping mixed-phase cloud layer.</p>
      <p id="d2e5191">Across the simulations, the onset of decoupling exhibits a systematic dependence on the prescribed subsidence: in cases with reduced subsidence, the decoupling occurs closer to the sea-ice edge and is accompanied by overall larger maxima in both liquid and ice water content. While all simulations show the initial formation of a thin ice cloud at C01, substantial differences arise beginning at C02, most notably in cloud-top height and the vertical distribution of liquid and ice. The Sub200 simulation produces only a shallow ice cloud capped by a thin liquid layer, with little variation in cloud-top altitude throughout the trajectory. In contrast, the simulations with weaker subsidence develop considerably deeper clouds, characterised by more complex internal structure and enhanced condensate mass.</p>

      <fig id="F9" specific-use="star"><label>Figure 9</label><caption><p id="d2e5196">Horizontal cross-sections of cloud liquid water (<inline-formula><mml:math id="M285" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and cloud ice (<inline-formula><mml:math id="M286" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) at the domain centre (<inline-formula><mml:math id="M287" display="inline"><mml:mrow><mml:mi>y</mml:mi><mml:mo>=</mml:mo><mml:mtext>6.4</mml:mtext></mml:mrow></mml:math></inline-formula> km), at different locations along the trajectory and for different subsidence experiments. Cross-sections of decoupled clouds (<inline-formula><mml:math id="M288" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> g kg<sup>−1</sup> and <inline-formula><mml:math id="M290" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub><mml:mo>&gt;</mml:mo><mml:mtext>0.5</mml:mtext></mml:mrow></mml:math></inline-formula> K) are highlighted in grey.</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f09.png"/>

        </fig>

      <p id="d2e5286">The impact of subsidence on the developing ABL is characterised by various bulk quantities, as shown in Fig. <xref ref-type="fig" rid="F10"/>. The integrated water vapour IWV (Fig. <xref ref-type="fig" rid="F10"/>a) is similar in all simulations, but the boundary layer (Fig. <xref ref-type="fig" rid="F10"/>d) in the NoSub case reaches substantially greater depths (2 km), following a parabolic deepening rate due to unimpeded entrainment at the ABL top. All simulations exhibit a similar strong initial boundary layer growth within the MIZ and immediately downstream of the sea ice edge (up to C02), driven primarily by intense surface heat fluxes in this region (Fig. <xref ref-type="fig" rid="F7"/>). However, after this initial phase, the Sub200 simulation boundary layer actually becomes shallower, with the strong subsidence keeping <inline-formula><mml:math id="M291" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> below 1 km. In contrast, the Ctrl, Sub50, and Sub10 simulations all maintain continued ABL deepening, though <inline-formula><mml:math id="M292" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> remains below the parabolic limit visible in NoSub.</p>
      <p id="d2e5320">The liquid water path LWP (Fig. <xref ref-type="fig" rid="F10"/>c) exhibits an initial peak near the sea ice in all simulations, coinciding with the region of strong boundary layer growth at approximately 80° N on average. The RMSE in the location of the peak between the simulations is 0.01° N, and the strength of the peak decreases with increasing subsidence by 18 g m<sup>−2</sup>, with an overall RMSE of 4.9 g m<sup>−2</sup>. A second, more pronounced  LWP  maximum occurs later at 76.3° N in NoSub, with a maximum value of 173 g m<sup>−2</sup>. For Sub50 and Ctrl, this secondary peak shifts to lower latitudes and reduced magnitudes, occurring at 76° N (167 g m<sup>−2</sup>) and 74.4° N (133 g m<sup>−2</sup>), respectively. In Sub200, the liquid water path does not recover after the initial maximum and shows only a gradual increase later in the simulation, beyond 74° N.</p>
      <p id="d2e5386">The ice water path IWP (Fig. <xref ref-type="fig" rid="F10"/>e), including all frozen hydrometeors, displays a similar spatial evolution, with an initial peak forming in the MIZ around 79.4° N, consistent in all simulations. Subsequently, IWP increases over the open ocean following the sea ice edge. Compared to LWP the ice growth begins slightly earlier (also visible in Fig. <xref ref-type="fig" rid="F9"/>), which is consistent with previous studies of Arctic MCAOs <xref ref-type="bibr" rid="bib1.bibx57 bib1.bibx34" id="paren.97"/>. The peak IWP in NoSub occurs at 75.7° N with 48 g m<sup>−2</sup>, whereas for Sub50 and Ctrl it shifts to 75.7 and 73.8° N respectively with reduced magnitudes of 41 and 31 g m<sup>−2</sup> respectively. The Sub200 simulation exhibits no such shift or comparable peak values, indicating a systematic suppression of ice growth under stronger subsidence.</p>
      <p id="d2e5421">The ratio of ice to liquid water, <inline-formula><mml:math id="M300" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi mathvariant="normal">IWP</mml:mi><mml:mi mathvariant="normal">LWP</mml:mi></mml:mfrac></mml:mstyle></mml:math></inline-formula>, calculated only for regions with a significant liquid content (<inline-formula><mml:math id="M301" display="inline"><mml:mrow><mml:mi mathvariant="normal">LWP</mml:mi><mml:mo>&gt;</mml:mo></mml:mrow></mml:math></inline-formula> 1 g m<sup>−2</sup>), highlights these differences more clearly (Fig. <xref ref-type="fig" rid="F10"/>b). The initial shallow cloud developing above the MIZ shows a similar structure among NoSub, Sub10, Sub50, and Ctrl, while Sub200 displays a slightly larger ice fraction in the initial cloud. However, because of the overall thinness of both liquid and ice layers, this difference cannot be regarded statistically significant. In later stages, LWP in Sub200 falls below 1 g m<sup>−2</sup>, producing a discontinuity in the <inline-formula><mml:math id="M304" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi mathvariant="normal">IWP</mml:mi><mml:mi mathvariant="normal">LWP</mml:mi></mml:mfrac></mml:mstyle></mml:math></inline-formula> ratio, while in the remaining cases a clear shift towards later growth of IWP is evident.</p>
      <p id="d2e5483">Finally, the impact of subsidence on the total surface precipitation rate (<inline-formula><mml:math id="M305" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mtext>tot</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) (Fig. <xref ref-type="fig" rid="F10"/>f) is broadly similar to the IWP. The NoSub simulation reaches precipitation rates up to 60 mm h<sup>−1</sup> towards the end of the simulation, compared with 25 mm h<sup>−1</sup> at the peak near 74° N for Ctrl. In Sub200, precipitation remains confined to the initial shallow cloud phase, with maximum rates of only 2.1 mm h<sup>−1</sup>.</p>

      <fig id="F10" specific-use="star"><label>Figure 10</label><caption><p id="d2e5537">Integrated water vapour IWV <bold>(a)</bold>, liquid water path LWP <bold>(c)</bold>, ice water path IWP <bold>(e)</bold>, including all frozen hydrometeors, together with its ratio <inline-formula><mml:math id="M309" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi mathvariant="normal">IWP</mml:mi><mml:mi mathvariant="normal">LWP</mml:mi></mml:mfrac></mml:mstyle></mml:math></inline-formula> <bold>(b)</bold>, the boundary layer height <inline-formula><mml:math id="M310" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <bold>(d)</bold> and the total precipitation rate <inline-formula><mml:math id="M311" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mtext>tot</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> <bold>(e)</bold> for Lagrangian LES with different subsidence forcings. The locations of the dropsonde circles are shown as vertical dashed lines, and the surface cover is indicated as sea ice (sic <inline-formula><mml:math id="M312" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0.9</mml:mn></mml:mrow></mml:math></inline-formula>, light blue), marginal sea-ice zone (<inline-formula><mml:math id="M313" display="inline"><mml:mrow><mml:mn mathvariant="normal">0</mml:mn><mml:mo>&lt;</mml:mo><mml:mi mathvariant="normal">sic</mml:mi><mml:mi mathvariant="normal">≤</mml:mi><mml:mn mathvariant="normal">0.9</mml:mn></mml:mrow></mml:math></inline-formula>, hatched), and open ocean (sic <inline-formula><mml:math id="M314" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>, dark blue).</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f10.png"/>

        </fig>

</sec>
<sec id="Ch1.S5.SS2">
  <label>5.2</label><title>Glaciation and decoupling</title>
      <p id="d2e5643">The results so far indicate that the behaviour of the cloud ice phase is particularly affected by the strength of subsidence. To gain further insight, the relative contributions by the three frozen hydrometeor classes in the LES microphysical scheme are investigated. The integrated column water paths of cloud ice (CIWP), snow (SIWP), and graupel (GIWP) are shown in Fig. <xref ref-type="fig" rid="F11"/>. The behaviour of CIWP (Fig. <xref ref-type="fig" rid="F11"/>a) closely follows that of the total ice water path (IWP), reflecting its dominant contribution to the total ice mass. The maximum values of CIWP reach 38 g m<sup>−2</sup> at 73.4° N for NoSub and 32 g m<sup>−2</sup> at 73.7° N for Ctrl, with a systematic decrease in amplitude under stronger subsidence. The SIWP (Fig. <xref ref-type="fig" rid="F11"/>c) distribution exhibits a similar latitudinal progression, with peak values occurring later and at reduced magnitudes as subsidence increases. However, unlike CIWP, SIWP does not sharply decline after the peak but plateaus afterwards, reaching 9.6 g m<sup>−2</sup> at 73.3° N for NoSub and 5.5 g m<sup>−2</sup> at 73.4° N for Ctrl. The graupel path GIWP (Fig. <xref ref-type="fig" rid="F11"/>b) exhibits the most distinct and localised peak. In NoSub the peak occurs at 76° N with a magnitude of 8.4 g m<sup>−2</sup>, generally shifting southward with increasing subsidence to 74° N for Ctrl, weakening in amplitude to 2.7 g m<sup>−2</sup>. The Sub200 experiment does not develop graupel. In this southward progression, the width of the graupel peak remains similar.</p>

      <fig id="F11"><label>Figure 11</label><caption><p id="d2e5729">Integrated cloud ice water path CIWP <bold>(a)</bold>, integrated snow water path SIWP <bold>(c)</bold> and integrated graupel water path GIWP <bold>(b)</bold>.  The locations of the dropsonde circles are shown as vertical dashed lines, and the surface cover is indicated as sea ice (sic <inline-formula><mml:math id="M321" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, light blue), marginal sea-ice zone (<inline-formula><mml:math id="M322" display="inline"><mml:mrow><mml:mtext>0</mml:mtext><mml:mo>&lt;</mml:mo><mml:mi mathvariant="normal">sic</mml:mi><mml:mo>≤</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, hatched), and open ocean (sic <inline-formula><mml:math id="M323" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mtext>0</mml:mtext></mml:mrow></mml:math></inline-formula>, dark blue).</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f11.png"/>

        </fig>

      <p id="d2e5784">Graupel is typically formed in convective updrafts, as it requires substantial vertical velocities. Accordingly, the southward shift and progressive weakening of the peak in GIWP with increasing subsidence probably reflects a similar shift in convective dynamics. This motivates a deeper investigation of the behaviour of boundary-layer internal decoupling. Previous MCAOs studies have established that such decoupling plays a central role in the transition from organised roll convection to open-cellular convection. Enhanced precipitation, often driven by secondary ice production and riming, has been shown to promote evaporation and sublimation below the cloud, thereby cooling and moistening the sub-cloud layer. This preconditioning in water vapour at lower levels accelerates the breakup of stratocumulus decks and favours the onset of cellular convection. As a result, the surface supply of moisture and heat to the cloud layer is reduced, weakening roll structures and promoting the development of cellular patterns <xref ref-type="bibr" rid="bib1.bibx1 bib1.bibx100 bib1.bibx37 bib1.bibx114" id="paren.98"/>. A slightly different form of decoupling that does not involve precipitation has been proposed earlier by <xref ref-type="bibr" rid="bib1.bibx8" id="text.99"/>, showing that during deepening marine subtropical stratocumulus-topped ABLs a layer of negative buoyancy flux <inline-formula><mml:math id="M324" display="inline"><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> can form below cloud base, as a result of top-down and bottom-up driven mixing becoming too far separated in the vertical. This negative buoyancy flux layer then disrupts the ABL-deep circulation, inducing decoupling. The latitudinal development of the buoyancy flux is shown in Fig. <xref ref-type="fig" rid="FD1"/>.</p>
      <p id="d2e5817">Both mechanisms of decoupling and the link to graupel formation are investigated next. The buoyancy-based decoupling mechanism is assessed by defining a decoupling point <inline-formula><mml:math id="M325" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:msub></mml:mrow></mml:math></inline-formula> as the time point at which <inline-formula><mml:math id="M326" display="inline"><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> becomes negative below cloud base for the first time, and remains so until the end of the simulation (indicated as <inline-formula><mml:math id="M327" display="inline"><mml:mo>▾</mml:mo></mml:math></inline-formula> in Fig. <xref ref-type="fig" rid="F8"/>). The humidity-based decoupling mechanism involving precipitation evaporation is assessed by defining a second decoupling point, this time inferred from <inline-formula><mml:math id="M328" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M329" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>  denoted <inline-formula><mml:math id="M330" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, as discussed above (Sect. <xref ref-type="sec" rid="Ch1.S5.SS1"/>). Comparing these two definitions gives insight into how exactly decoupling works in MCAOs and how it affects the shifts in ice phase hydrometeors.</p>
      <p id="d2e5926">Figure <xref ref-type="fig" rid="F12"/> compares the locations of the largest peaks in liquid water path (LWP<sub>max</sub>), graupel water path (GIWP<sub>max</sub>), and surface precipitation rate (<inline-formula><mml:math id="M333" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mtext>tot, max</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>) with the two decoupling points <inline-formula><mml:math id="M334" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M335" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:msub></mml:mrow></mml:math></inline-formula>, for all simulations except Sub200 (in which no graupel appears). A key result that stands out is that buoyancy-based decoupling (vertical axis) structurally happens first, in all simulations (also indicated in Fig. <xref ref-type="fig" rid="F8"/>). This is followed by the peak in LWP, then integrated graupel, then surface precipitation, and finally the precipitation-based decoupling point. This sequence of events typically covers 1° of latitude in this MCAO case, and shifts southward with increasing prescribed mesoscale subsidence. The order of appearance of the various maxima is consistent with the idea that (i) internal buoyancy-decoupling initiates events and causes stronger surface-driven convection, (ii) driving stronger precipitation formation (mainly in graupel form) that efficiently depletes cloud liquid water mass <xref ref-type="bibr" rid="bib1.bibx1" id="paren.100"><named-content content-type="pre">as discussed by</named-content></xref>, (iii) forming intense graupel for a while, (iv) associated with enhanced surface precipitation which then (v) further stabilises the lower boundary layer through evaporation below cloud base, suppressing vertical mixing and further enhancing decoupling <xref ref-type="bibr" rid="bib1.bibx114" id="paren.101"/>. The last step is also suggested by the slight lowering of liquid cloud base height visible in Fig. <xref ref-type="fig" rid="F8"/>. This sequence of events ultimately yields a fully decoupled structure with respect to  <inline-formula><mml:math id="M336" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M337" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> at <inline-formula><mml:math id="M338" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>.</p>

      <fig id="F12"><label>Figure 12</label><caption><p id="d2e6071">Location of the largest peak in liquid water path LWP<sub>max</sub>, graupel water path GIWP<sub>max</sub> and precipitation <inline-formula><mml:math id="M341" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mtext>tot, max</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and the location of decoupling with respect to the <inline-formula><mml:math id="M342" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M343" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> profiles <inline-formula><mml:math id="M344" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub><mml:mo>,</mml:mo><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> (following <xref ref-type="bibr" rid="bib1.bibx36" id="altparen.102"/>) in relation to the location of decoupling with respect to the buoyancy flux <inline-formula><mml:math id="M345" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:msub></mml:mrow></mml:math></inline-formula> (following <xref ref-type="bibr" rid="bib1.bibx8" id="altparen.103"/>). The colours represent the different simulation experiments as in Fig. <xref ref-type="fig" rid="F11"/>.</p></caption>
          <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f12.png"/>

        </fig>


</sec>
</sec>
<sec id="Ch1.S6">
  <label>6</label><title>Discussion</title>
      <p id="d2e6198">The sensitivity experiments suggest that the influence of subsidence extends beyond a simple control on boundary layer height. Previous observational and modelling studies have demonstrated that large-scale subsidence influences the evolution of Arctic marine cold air outbreaks by modifying inversion strength, cloud-top height, and the thermodynamic structure of the boundary layer <xref ref-type="bibr" rid="bib1.bibx10 bib1.bibx48 bib1.bibx116 bib1.bibx78" id="paren.104"/>. However, the exact causal connection between these features and processes including cloud glaciation and boundary layer decoupling has remained less clear. The results obtained in this study provide further insight, suggesting that larger-scale subsidence can act as a strong control on the entire transition of the atmospheric boundary layer and clouds. While the boundary layer evolution under such imposed subsidence involves various small-scale processes that could be described individually, we find that it makes much more sense to interpret them in combination, as they act as a sequence of strongly connected processes. This sequence was consistently diagnosed in all simulations carried out in this study.</p>
      <p id="d2e6204">Figure <xref ref-type="fig" rid="F13"/> conceptually summarizes the sequence of processes. Initially, the boundary layer is fully coupled to the ocean surface. Strong sensible heat fluxes maintain turbulent mixing throughout the boundary layer, resulting in nearly vertically homogeneous profiles of liquid water potential temperature and total water mixing ratio. Such coupled boundary layers are characteristic of the early stages of marine cold air outbreaks, where large surface-atmosphere temperature contrasts generate vigorous turbulence and rapid boundary layer growth <xref ref-type="bibr" rid="bib1.bibx10 bib1.bibx21 bib1.bibx13" id="paren.105"/>. During this stage, cloud evolution is primarily governed by the interaction between surface fluxes, entrainment-deepening and cloud-top radiative cooling, processes that have long been recognised as essential for maintaining Arctic mixed-phase stratocumulus <xref ref-type="bibr" rid="bib1.bibx55 bib1.bibx61" id="paren.106"><named-content content-type="pre">e.g.</named-content></xref>. During this phase, subsidence primarily controls the rate at which the boundary layer can deepen by opposing entrainment at the inversion.</p>

      <fig id="F13" specific-use="star"><label>Figure 13</label><caption><p id="d2e6219">Conceptual evolution of the atmospheric boundary layer during the modelled Arctic marine cold air outbreak. Black and grey profiles of liquid water potential temperature <inline-formula><mml:math id="M346" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, total humidity <inline-formula><mml:math id="M347" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and buoyancy flux <inline-formula><mml:math id="M348" display="inline"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> indicate a coupled boundary layer, whereas the orange profiles illustrate decoupling with respect to buoyancy-based (<inline-formula><mml:math id="M349" display="inline"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>) and thermodynamic (<inline-formula><mml:math id="M350" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M351" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). The top of the boundary layer is indicated as a dashed line.</p></caption>
        <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f13.png"/>

      </fig>

      <p id="d2e6310">Sustained entrainment deepening, driven by superimposed bottom-up (surface buoyancy flux) and top-down (cloud-top radiative cooling) processes <xref ref-type="bibr" rid="bib1.bibx115" id="paren.107"/>, at some point leads to boundary-layer internal decoupling. We find that this internal decoupling is first visible in the negative buoyancy flux that develops below cloud base, with liquid water potential temperature and total humidity still remaining relatively well mixed at this stage. This buoyancy-driven decoupling therefore represents the earliest stage of the transition, acting as a precursor to thermodynamic separation of the cloud and sub-cloud layer that is known to develop at a later stage <xref ref-type="bibr" rid="bib1.bibx1" id="paren.108"/>. To our knowledge, such buoyancy flux decoupling has not been previously been identified during Arctic marine cold air outbreaks.</p>
      <p id="d2e6319">At this point it is instructive to draw some parallels with warm  stratocumulus-to-cumulus transitions in the marine subtropics, which have been intensely studied for decades <xref ref-type="bibr" rid="bib1.bibx7 bib1.bibx9 bib1.bibx113 bib1.bibx104 bib1.bibx60" id="paren.109"/>. As outlined in the key study by <xref ref-type="bibr" rid="bib1.bibx8" id="text.110"/>, internal decoupling in the buoyancy flux profile in a deepening well-mixed boundary layer can initiate as a result of the top-down and bottom-up driven turbulent circulations failing to fully overlap. We find that the same happens in MCAOs, triggering the formation of cumulus clouds with their base at the decoupling level (visible in Fig. <xref ref-type="fig" rid="F9"/>). However, rather than resulting in a warm shallow-cumulus regime and eventual stratocumulus breakup, the transition proceeds towards a decoupled system that includes mixed-phase clouds. Ice microphysical processes such as ice growth, riming, graupel formation, and sub-cloud sublimation then become central to the subsequent cloud transition. These aspects represent defining differences with the warm subtropics.</p>
      <p id="d2e6330">Following this initial decoupling, the cloud layer continues to deepen while the upper and lower parts of the boundary layer become increasingly isolated from each other. During this stage the simulations exhibit a maximum in liquid water path before ice production and graupel formation become effective. This evolution is consistent with the established understanding of mixed-phase cloud microphysics, in which increasing liquid water availability promotes depositional ice growth through the Wegener–Bergeron–Findeisen process before riming becomes increasingly important and eventually produces graupel <xref ref-type="bibr" rid="bib1.bibx55 bib1.bibx116 bib1.bibx19" id="paren.111"/>. Enhanced graupel formation subsequently increases precipitation, removing condensate from the cloud layer and reducing cloud liquid water through collection and sedimentation. At the same time, sublimation below cloud base cools and moistens the sub-cloud layer, while reduced turbulent exchange strengthens the vertical gradients in liquid water potential temperature and moisture. Together these processes ultimately produce a fully thermodynamically decoupled boundary layer.</p>
      <p id="d2e6336">This particular sequence of processes, starting with buoyancy decoupling and defined by the set of markers as shown in Fig. <xref ref-type="fig" rid="F12"/>, occurred in every experiment conducted in this study. However, the imposed subsidence strength strongly affects its timing. Reduced subsidence allows more rapid boundary layer deepening, resulting in earlier buoyancy-driven decoupling, larger liquid water paths, enhanced convective overturning and stronger graupel formation. Conversely, stronger subsidence suppresses boundary layer deepening, delays the onset of decoupling and substantially reduces cloud glaciation. These results are in principle consistent with previous idealised and high-resolution simulations of Arctic cloud systems <xref ref-type="bibr" rid="bib1.bibx116 bib1.bibx61" id="paren.112"/>. This study provides more insight into these responses. A key outcome is that processes such as cloud glaciation and boundary layer decoupling do not act independently, but strongly interact and are part of the ongoing adjustment of the newly formed marine boundary layer to the changed external conditions after leaving the sea ice edge. Subsidence does not directly determine the microphysical evolution of the cloud, but modifies the boundary layer structure in which these processes occur. By controlling boundary layer deepening and decoupling, subsidence indirectly regulates the timing of cloud deepening, mixed-phase cloud development, precipitation formation and the transition towards a thermodynamically decoupled boundary layer.</p>
      <p id="d2e6344">The precise timing of cloud transitions during MCAOs thus depends on the environmental conditions encountered by the air mass. Factors such as the surface-air temperature difference, aerosol conditions and the effective strength of radiative cooling can all affect the exact onset of decoupling and subsequent cloud glaciation <xref ref-type="bibr" rid="bib1.bibx19 bib1.bibx100 bib1.bibx11" id="paren.113"/>. Additional sensitivity experiments using the same model setup indicate that the ice-phase pathway is sensitive to CCN concentrations, with higher CCN concentrations shifting ice precipitation from graupel toward snow (not shown). This suggests that the timing and partitioning of precipitating ice depend on the microphysical representation, including processes that control droplet size and riming, as well as on prescribed aerosol concentrations. A more systematic investigation of these sensitivities would be required to assess their impact on the processes identified in this study. In addition, local variations in the larger-scale subsidence field may similarly influence precipitation timing, including through lee-side effects associated with local orography. But the conceptual model shown in Fig. <xref ref-type="fig" rid="F13"/> does include all key processes found in this study to govern the cloud evolution during Arctic MCAOs. It might thus be useful as a physically consistent framework of reference for interpreting cloud transitions during both observed and modelled MCAO events.</p>
</sec>
<sec id="Ch1.S7" sec-type="conclusions">
  <label>7</label><title>Conclusions</title>
      <p id="d2e6360">This study investigates the sensitivity of Arctic mixed-phase cloud evolution in marine cold air outbreaks with respect to mesoscale subsidence. A Lagrangian Large-Eddy Simulation framework constrained by observations obtained during the airborne HALO–<inline-formula><mml:math id="M352" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>. The control simulation was evaluated against the extensive and independent set of airborne in-situ and remote-sensing and meteorological balloon measurements. In the control run, the model reproduced the vertical thermodynamic structure of the observed marine cold air outbreak within the range given by the measurement uncertainties, capturing the evolution of air temperature, humidity, and ABL height along the Lagrangian trajectory. Compared to dropsonde, radiometer, and lidar data, the control simulation accurately represented the integrated water vapour and liquid water path, with a slight cold and dry bias at lower levels. The general agreement between control run results and the corresponding measurements demonstrates that the applied forcing and initialisation derived from the HALO–<inline-formula><mml:math id="M353" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> measurements provide a robust foundation for reproducing the dynamics and properties of the Arctic atmospheric boundary layer, and underscores the importance of constraining simulations with detailed observations.</p>
      <p id="d2e6397">Sensitivity experiments with the tested large-eddy simulation model revealed that subsidence exerts a strong control on the depth of the atmospheric boundary layer, the height of the cloud top, and the partitioning between the liquid and ice phases in clouds. Weak or absent subsidence enables deeper growth of the atmospheric boundary layer, allowing it to approach the theoretical parabolic deepening rate implied by standard bulk mixed-layer modelling. Reduced subsidence also enhances convective overturning, promoting stronger mixed-phase cloud formation and an earlier onset of stronger graupel formation. In contrast, strong subsidence (Sub200) suppresses vertical development and convective activity, leading to thinner and shorter-lived clouds. The earlier and more pronounced graupel peak in the weak-subsidence cases, and an apparent time-correlation with the formation of a decoupled vertical structure in the cloud field (Fig. <xref ref-type="fig" rid="F9"/>) indicates that graupel formation is tightly linked to the onset of significant surface-driven convection featuring moist updrafts.</p>
      <p id="d2e6402">A deeper analysis of the decoupling process provides an additional perspective on these dynamical–microphysical interactions. Two expressions of decoupling are investigated: (i) one based on the buoyancy flux profile, and (ii) the other reflecting the internal vertical thermodynamic structure of the atmospheric boundary layer. A systematic dependence of the onset of decoupling on the prescribed subsidence is identified, indicating an earlier convective transition in cases with reduced subsidence. Buoyancy-based decoupling always happens first, closely followed by (i) a distinct maximum in the cloud liquid water path, (ii) a peak in the graupel path, (iii) a peak in surface precipitation, and (iv) complete thermodynamic decoupling. This robust order of events and its southward shift with increasing subsidence highlight the role of subsidence in the transformation of air masses during marine cold air outbreaks. Its impact on the atmospheric boundary layer depth plays a crucial role, promoting buoyancy decoupling below cloud base, which subsequently induces precipitation-driven stabilisation at low levels by accelerating the depletion of the cloud liquid water through graupel formation. This sequence of events eventually drives a transition towards a fully decoupled structure and to open cellular convection later on. These results underscore that subsidence not only constrains the atmospheric boundary layer and cloud depth but also controls the mixed-phase partitioning and the timing of falling hydrometeor formation during marine cold air outbreaks.</p>
      <p id="d2e6405">The results described above are based on a single case study. Their applicability across different Arctic conditions, particularly during stronger marine cold air outbreaks, has not yet been assessed. Furthermore, the prescribed aerosol particle number concentrations are held constant during  the sensitivity experiments, thereby excluding potential aerosol–cloud–precipitation feedbacks. Variations in cloud condensation nuclei (CCN) concentrations can modify cloud droplet number and size, with consequences for precipitation formation and the transition from closed- to open-cellular convection <xref ref-type="bibr" rid="bib1.bibx1" id="paren.114"><named-content content-type="pre">e.g.</named-content></xref>. Changes in aerosol concentrations may, therefore, alter the timing or strength of the precipitation and decoupling responses identified here, and potentially modulate their sensitivity to subsidence. Similarly, secondary ice production is limited to the Hallett–Mossop process, while other mechanisms, such as ice–ice collisional breakup and freezing fragmentation, are not represented in the model. These mechanisms may enhance ice particle concentrations and thereby modify ice growth, graupel formation, precipitation, and the timing of boundary-layer decoupling <xref ref-type="bibr" rid="bib1.bibx37 bib1.bibx89 bib1.bibx75" id="paren.115"><named-content content-type="pre">e.g.</named-content></xref>. Accordingly, future work should extend this analysis to additional cases and explore how the sensitivity to subsidence compares to variations in other factors, including CCN and ice-nucleating particle (INP) concentrations. Such investigations will help to disentangle the relative importance of dynamical versus microphysical controls across scales on mixed-phase cloud evolution in the convective atmospheric boundary layer at high latitudes.</p>
</sec>

      
      </body>
    <back><app-group>

<app id="App1.Ch1.S1">
  <label>Appendix A</label><title>Synoptic situation</title>
      <p id="d2e6430">For additional context on the large-scale atmospheric circulation during the case study, Fig. <xref ref-type="fig" rid="FA1"/> shows the ERA5 mean sea-level pressure and horizontal wind field over the study region.</p>

      <fig id="FA1"><label>Figure A1</label><caption><p id="d2e6437">Maps of geopotential height at 500 hPa (shading) and mean sea level pressure (black contour lines; <bold>a</bold>) and wind speed at 10 m (shading) and wind direction (arrows) on 30 March 2022 at 12:00 UTC during HALO–<inline-formula><mml:math id="M354" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> from ERA5 <bold>(b)</bold>. Flight paths of HALO flights RF10 (29 March 2022) and RF11 (30 March 2022) and P5 on 30 March 2022, together with CMET, Dropsonde (DS) locations (<inline-formula><mml:math id="M355" display="inline"><mml:mo lspace="0mm">▾</mml:mo></mml:math></inline-formula>) and the sea-ice concentration retrieved from satellite observations <xref ref-type="bibr" rid="bib1.bibx90" id="paren.116"/> indicated in grey and white <bold>(c)</bold>.</p></caption>
        
        <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f14.png"/>

      </fig>


</app>

<app id="App1.Ch1.S2">
  <label>Appendix B</label><title>Cold air outbreak and stability indices</title>
      <p id="d2e6495">Following <xref ref-type="bibr" rid="bib1.bibx62" id="text.117"/> and <xref ref-type="bibr" rid="bib1.bibx13" id="text.118"/>, the MCAO Index <inline-formula><mml:math id="M356" display="inline"><mml:mi>M</mml:mi></mml:math></inline-formula> is defined as the difference between the sea surface potential temperature <inline-formula><mml:math id="M357" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mtext>SKT</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and the potential temperature at 850 hPa <inline-formula><mml:math id="M358" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mrow><mml:mtext>850</mml:mtext><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mtext>hPa</mml:mtext></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>:

          <disp-formula id="App1.Ch1.S2.E11" content-type="numbered"><label>B1</label><mml:math id="M359" display="block"><mml:mrow><mml:mi>M</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mtext>SKT</mml:mtext></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mrow><mml:mtext>850</mml:mtext><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mtext>hPa</mml:mtext></mml:mrow></mml:msub></mml:mrow></mml:math></disp-formula>

        Positive values indicate enhanced instability, favouring convection and cloud formation, while negative values point to a more stable boundary layer. <xref ref-type="bibr" rid="bib1.bibx62" id="text.119"/> identify MCAO conditions if <inline-formula><mml:math id="M360" display="inline"><mml:mrow><mml:mi>M</mml:mi><mml:mo>&gt;</mml:mo><mml:mtext>0</mml:mtext></mml:mrow></mml:math></inline-formula> K and classify MCAOs as weak (0 K <inline-formula><mml:math id="M361" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mi>M</mml:mi><mml:mo>≤</mml:mo><mml:mtext>4</mml:mtext></mml:mrow></mml:math></inline-formula> K), moderate (4 K <inline-formula><mml:math id="M362" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mi>M</mml:mi><mml:mo>≤</mml:mo><mml:mtext>8</mml:mtext></mml:mrow></mml:math></inline-formula> K), strong (8 K <inline-formula><mml:math id="M363" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mi>M</mml:mi><mml:mo>≤</mml:mo><mml:mtext>12</mml:mtext></mml:mrow></mml:math></inline-formula> K) and very strong (<inline-formula><mml:math id="M364" display="inline"><mml:mrow><mml:mi>M</mml:mi><mml:mo>&gt;</mml:mo><mml:mtext>12</mml:mtext></mml:mrow></mml:math></inline-formula> K). In Fig. <xref ref-type="fig" rid="FB1"/> we present <inline-formula><mml:math id="M365" display="inline"><mml:mi>M</mml:mi></mml:math></inline-formula> as a function of latitude following the Lagrangian trajectory of the modelled air mass for the Ctrl simulation calculated from the model output, together with an estimation of <inline-formula><mml:math id="M366" display="inline"><mml:mi>M</mml:mi></mml:math></inline-formula> from the surface and dropsonde observations, using temperature and pressure profiles averaged over all sondes in one circle at the height level closest to 850 hPa for comparison.</p>
      <p id="d2e6650">The Stability Index is expressed as the ratio <inline-formula><mml:math id="M367" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow><mml:mi>L</mml:mi></mml:mfrac></mml:mstyle></mml:math></inline-formula>, diagnosed from the model as the minimum local gradient of virtual potential temperature, and calculated from the averaged dropsonde profiles as the level that reaches a critical value of the bulk Richardson number <inline-formula><mml:math id="M368" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:msub><mml:mi>i</mml:mi><mml:mtext>b,crit</mml:mtext></mml:msub><mml:mo>&gt;</mml:mo><mml:mtext>0.25</mml:mtext></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx16 bib1.bibx102" id="paren.120"/>. The Obukhov length <inline-formula><mml:math id="M369" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> characterises the role of buoyancy in turbulent flows:

          <disp-formula id="App1.Ch1.S2.E12" content-type="numbered"><label>B2</label><mml:math id="M370" display="block"><mml:mrow><mml:mi>L</mml:mi><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mi>u</mml:mi><mml:mo>*</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msubsup><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mrow><mml:mrow><mml:mi mathvariant="italic">κ</mml:mi><mml:mi>g</mml:mi><mml:mo>(</mml:mo><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:msub><mml:mo>)</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></disp-formula>

        with frictional velocity <inline-formula><mml:math id="M371" display="inline"><mml:mrow><mml:msub><mml:mi>u</mml:mi><mml:mo>*</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula>, mean virtual potential temperature <inline-formula><mml:math id="M372" display="inline"><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula>, surface virtual potential temperature flux <inline-formula><mml:math id="M373" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:msub><mml:mo>)</mml:mo><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and Kármán constant <inline-formula><mml:math id="M374" display="inline"><mml:mi mathvariant="italic">κ</mml:mi></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx97" id="paren.121"/>. <inline-formula><mml:math id="M375" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> is included in the model output and can be estimated from observations using a similar method by applying Monin–Obukhov similarity theory and iteratively solving the stability functions for <inline-formula><mml:math id="M376" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> using <inline-formula><mml:math id="M377" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:msub><mml:mi>i</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> as an initial guess <xref ref-type="bibr" rid="bib1.bibx30" id="paren.122"/>.</p><fig id="FB1"><label>Figure B1</label><caption><p id="d2e6852">MCAO Index from Ctrl model output (red line) and from surface observations using VELOX and dropsonde profiles (red triangles). Stability index <inline-formula><mml:math id="M378" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow><mml:mi>L</mml:mi></mml:mfrac></mml:mstyle></mml:mrow></mml:math></inline-formula> from Ctrl model output (yellow line) and from observations (yellow triangles) along the simulation trajectory.</p></caption>
        <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f15.png"/>

      </fig>


</app>

<app id="App1.Ch1.S3">
  <label>Appendix C</label><title>Trajectory calculation</title>

      <fig id="FC1"><label>Figure C1</label><caption><p id="d2e6891">Lagrangian trajectories initiated inside IC at 870 hPa that were recaptured in C01, C02 and C03 (orange). Trajectories that were not resampled in the subsequent circle were discarded (grey) from the calculation of the mean trajectory used for the simulation (red). Dropsonde locations are marked with <inline-formula><mml:math id="M379" display="inline"><mml:mo>▾</mml:mo></mml:math></inline-formula>. Satellite image at the time of RF11 29 March 2022 from Terra MODIS (<xref ref-type="bibr" rid="bib1.bibx59" id="text.123"/>, Worldview Snapshots) in the background.</p></caption>
        <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f16.png"/>

      </fig>

<table-wrap id="TC1"><label>Table C1</label><caption><p id="d2e6914">Summary of subsidence statistics derived from dropsonde observations for each circle. Mean values are computed over the full 8 km profile, while ranges and uncertainty estimates refer to the lowest 3 km.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="left" colsep="1"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right" colsep="1"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right" colsep="1"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right" colsep="1"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:colspec colnum="9" colname="col9" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Circle</oasis:entry>
         <oasis:entry namest="col2" nameend="col3" align="center" colsep="1">Mean (8 km) </oasis:entry>
         <oasis:entry namest="col4" nameend="col5" align="center" colsep="1">Range (3 km) </oasis:entry>
         <oasis:entry namest="col6" nameend="col7" align="center" colsep="1">Mean error (3 km) </oasis:entry>
         <oasis:entry namest="col8" nameend="col9" align="center">Error range (3 km) </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M380" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>Pa s<inline-formula><mml:math id="M381" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M382" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>cm s<inline-formula><mml:math id="M383" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M384" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>Pa s<inline-formula><mml:math id="M385" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M386" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>cm s<inline-formula><mml:math id="M387" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M388" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>Pa s<inline-formula><mml:math id="M389" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M390" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>cm s<inline-formula><mml:math id="M391" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M392" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>Pa s<inline-formula><mml:math id="M393" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M394" display="inline"><mml:mo>[</mml:mo></mml:math></inline-formula>cm s<inline-formula><mml:math id="M395" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">IC</oasis:entry>
         <oasis:entry colname="col2">0.08</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M396" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.74</oasis:entry>
         <oasis:entry colname="col4">0 to 0.11</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M397" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.17 to 0</oasis:entry>
         <oasis:entry colname="col6">0.002</oasis:entry>
         <oasis:entry colname="col7">0.018</oasis:entry>
         <oasis:entry colname="col8">0 to 0.002</oasis:entry>
         <oasis:entry colname="col9">0 to 0.025</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">C01</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M398" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.01</oasis:entry>
         <oasis:entry colname="col3">0.12</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M399" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.08 to 0.01</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M400" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.07 to 0.82</oasis:entry>
         <oasis:entry colname="col6">0.001</oasis:entry>
         <oasis:entry colname="col7">0.008</oasis:entry>
         <oasis:entry colname="col8">0 to 0.001</oasis:entry>
         <oasis:entry colname="col9">0 to 0.012</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">C02</oasis:entry>
         <oasis:entry colname="col2">0.07</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M401" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.60</oasis:entry>
         <oasis:entry colname="col4">0 to 0.13</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M402" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.16 to 0</oasis:entry>
         <oasis:entry colname="col6">0.001</oasis:entry>
         <oasis:entry colname="col7">0.006</oasis:entry>
         <oasis:entry colname="col8">0 to 0.001</oasis:entry>
         <oasis:entry colname="col9">0.001 to 0.009</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">C03</oasis:entry>
         <oasis:entry colname="col2">0.03</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M403" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.26</oasis:entry>
         <oasis:entry colname="col4">0 to 0.08</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M404" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.71 to 0</oasis:entry>
         <oasis:entry colname="col6">0.001</oasis:entry>
         <oasis:entry colname="col7">0.005</oasis:entry>
         <oasis:entry colname="col8">0 to 0.001</oasis:entry>
         <oasis:entry colname="col9">0 to 0.008</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>


</app>

<app id="App1.Ch1.S4">
  <label>Appendix D</label><title>Buoyancy flux evolution</title>
      <p id="d2e7344">The evolution of the Buoyancy Flux profile along the MCAO trajectory is shown in Fig. <xref ref-type="fig" rid="FD1"/>.</p>

      <fig id="FD1"><label>Figure D1</label><caption><p id="d2e7351">Latitudinal evolution of buoyancy flux along the MCAO trajectory for all sensitivity experiments. Dashed horizontal lines indicate dropsonde circle  locations. Boundary layer height <inline-formula><mml:math id="M405" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud base <inline-formula><mml:math id="M406" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">b</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are indicated by grey dashed and dot-dashed lines, respectively. The markers <inline-formula><mml:math id="M407" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> and <inline-formula><mml:math id="M408" display="inline"><mml:mo>▴</mml:mo></mml:math></inline-formula> indicate decoupling points and heights with respect to <inline-formula><mml:math id="M409" display="inline"><mml:mrow><mml:mi>w</mml:mi><mml:mi mathvariant="normal">′</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mi mathvariant="normal">′</mml:mi></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M410" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>q</mml:mi><mml:mi mathvariant="normal">t</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M411" display="inline"><mml:mrow><mml:mi mathvariant="italic">δ</mml:mi><mml:msub><mml:mi mathvariant="italic">ϑ</mml:mi><mml:mi mathvariant="normal">l</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> respectively. The coloured bar at the bottom indicates sea ice (sic <inline-formula><mml:math id="M412" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, light blue), marginal sea-ice (<inline-formula><mml:math id="M413" display="inline"><mml:mrow><mml:mtext>0</mml:mtext><mml:mo>&lt;</mml:mo><mml:mi mathvariant="normal">sic</mml:mi><mml:mo>≤</mml:mo><mml:mtext>0.9</mml:mtext></mml:mrow></mml:math></inline-formula>, hatched), and open ocean (sic <inline-formula><mml:math id="M414" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mtext>0</mml:mtext></mml:mrow></mml:math></inline-formula>, dark blue).</p></caption>
        <graphic xlink:href="https://acp.copernicus.org/articles/26/13983/2026/acp-26-13983-2026-f17.png"/>

      </fig>

</app>
  </app-group><notes notes-type="codedataavailability"><title>Code and data availability</title>

      <p id="d2e7480">The pre-processed dropsondes data are available from <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.968891" ext-link-type="DOI">10.1594/PANGAEA.968891</ext-link> <xref ref-type="bibr" rid="bib1.bibx25" id="paren.124"/>, and the regression processing followed <xref ref-type="bibr" rid="bib1.bibx66" id="text.125"/> (<ext-link xlink:href="https://doi.org/10.1175/JAS-D-24-0034.1" ext-link-type="DOI">10.1175/JAS-D-24-0034.1</ext-link>) and <xref ref-type="bibr" rid="bib1.bibx65" id="text.126"/> (<ext-link xlink:href="https://doi.org/10.5281/zenodo.10402061" ext-link-type="DOI">10.5281/zenodo.10402061</ext-link>). The integrated water vapour and liquid water path retrieved from HAMP observations are available at <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.992898" ext-link-type="DOI">10.1594/PANGAEA.992898</ext-link> <xref ref-type="bibr" rid="bib1.bibx107" id="paren.127"/> and  <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.992918" ext-link-type="DOI">10.1594/PANGAEA.992918</ext-link> <xref ref-type="bibr" rid="bib1.bibx108" id="paren.128"/>, respectively. Radar reflectivities from MiRAC used for the retrieval of ice water path are available from <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.964977" ext-link-type="DOI">10.1594/PANGAEA.964977</ext-link> <xref ref-type="bibr" rid="bib1.bibx53" id="paren.129"/> and can be accessed via the ac3airborne tool (<ext-link xlink:href="https://doi.org/10.5281/zenodo.7305585" ext-link-type="DOI">10.5281/zenodo.7305585</ext-link>, <xref ref-type="bibr" rid="bib1.bibx52" id="altparen.130"/>). VELOX 2-D cloud-top and surface brightness temperatures with 1 Hz temporal resolution, derived at flight altitude, are available from <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.963401" ext-link-type="DOI">10.1594/PANGAEA.963401</ext-link> <xref ref-type="bibr" rid="bib1.bibx77" id="paren.131"/>. The CMET data is published at <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.997054" ext-link-type="DOI">10.1594/PANGAEA.997054</ext-link> <xref ref-type="bibr" rid="bib1.bibx87" id="paren.132"/> and the entire dataset from the ISLAS2022 campaign can be found here <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.997052" ext-link-type="DOI">10.1594/PANGAEA.997052</ext-link> <xref ref-type="bibr" rid="bib1.bibx86" id="paren.133"/>. The model code, input and configuration files, generated forcing files, and selected model output are provided by <ext-link xlink:href="https://doi.org/10.5281/zenodo.18232592" ext-link-type="DOI">10.5281/zenodo.18232592</ext-link> <xref ref-type="bibr" rid="bib1.bibx64" id="paren.134"/>. The forcing files are compatible with typical single-column model (SCM) forcings, as DALES is run with horizontally homogeneous initial and boundary conditions. The DALES version used in this study is 4.3 with an extension for mixed-phase microphysics; the specific version applied here is included in <ext-link xlink:href="https://doi.org/10.5281/zenodo.18232592" ext-link-type="DOI">10.5281/zenodo.18232592</ext-link> <xref ref-type="bibr" rid="bib1.bibx64" id="paren.135"/>, while the official DALES repository is available from <ext-link xlink:href="https://doi.org/10.5281/zenodo.4604726" ext-link-type="DOI">10.5281/zenodo.4604726</ext-link> <xref ref-type="bibr" rid="bib1.bibx3" id="paren.136"/>. ERA5 datasets were retrieved from the Copernicus Climate Change Service (C3S) Climate Data Store (CDS) at <uri>https://cds.climate.copernicus.eu/</uri> (last access: 6 March 2026).</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d2e7571">The authors made distinct contributions to the project. FP ran and evaluated the simulations and prepared the manuscript. JM determined the surface temperature from VELOX; BK calculated the Lagrangian trajectories; LvG and AW calculated the integrated water vapour from HAMP and the ice water path from MiRAC, respectively; and HS contributed the CMET observations, and MW and RN revised various intermediate versions of the manuscript.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d2e7577">The contact author has declared that none of the authors has any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d2e7583">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims made in the text, published maps, institutional affiliations, or any other geographical representation in this paper. The authors bear the ultimate responsibility for providing appropriate place names. Views expressed in the text are those of the authors and do not necessarily reflect the views of the publisher.</p>
  </notes><notes notes-type="sistatement"><title>Special issue statement</title>

      <p id="d2e7590">This article is part of the special issue “HALO–(<inline-formula><mml:math id="M415" display="inline"><mml:mrow><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi></mml:mrow></mml:math></inline-formula>)<sup>3</sup> – an airborne campaign to study air mass transformations during warm-air intrusions and cold-air outbreaks”. It is not associated with a conference.</p>
  </notes><ack><title>Acknowledgements</title><p id="d2e7615">We gratefully acknowledge the Gauss Centre for Supercomputing e.V. (<uri>https://www.gauss-centre.eu/</uri>, last access: 2 October 2026) for providing computing time on the GCS Supercomputer JUWELS at the Jülich Supercomputing Centre (JSC) under projects RCONGM and HR-AFC. We appreciate the financial contributions of the Alfred Wegener Institute (AWI, Bremerhaven), the German Aerospace Centre (DLR, Oberpfaffenhofen), and the Max Planck Institute for Meteorology (MPI-M, Hamburg). We acknowledge the use of imagery from the Worldview Snapshots application (<uri>https://wvs.earthdata.nasa.gov</uri>, last access: 22 December 2025), part of the Earth Observing System Data and Information System (EOSDIS). ChatGPT-4o has been used to help create the first versions of this manuscript. Thank you to Niklas Schnierstein and Jan Chylik for developing the DALESCGN model with representation of Arctic mixed-phase clouds. At last, we want to acknowledge and thank everyone involved in the HALO–<inline-formula><mml:math id="M417" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="script">A</mml:mi><mml:mi mathvariant="script">C</mml:mi><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> and ISLAS2022 campaigns, especially Mario Mech, who kindly provided the liquid water path data fromMiRAC for this study.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d2e7643">This research has been supported by the Deutsche Forschungsgemeinschaft (grant nos. 268020496, 316646266, and 442649391) and European Research Council (grant no. 773245).This open-access publication  was funded by Universität zu Köln.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d2e7654">This paper was edited by Ivy Tan and reviewed by two anonymous referees.</p>
  </notes><ref-list>
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