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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-23-3517-2023</article-id><title-group><article-title>Characterisations of Europe's integrated water vapour and assessments of atmospheric reanalyses using more than 2 decades of ground-based GPS</article-title><alt-title>Europe's GPS water vapour and assessments of atmospheric reanalyses</alt-title>
      </title-group><?xmltex \runningtitle{Europe's GPS water vapour and assessments of atmospheric reanalyses}?><?xmltex \runningauthor{P. Yuan et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>Yuan</surname><given-names>Peng</given-names></name>
          <email>peng.yuan@kit.edu</email>
        <ext-link>https://orcid.org/0000-0002-1717-8425</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Van Malderen</surname><given-names>Roeland</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1369-8853</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3">
          <name><surname>Yin</surname><given-names>Xungang</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4">
          <name><surname>Vogelmann</surname><given-names>Hannes</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff5">
          <name><surname>Jiang</surname><given-names>Weiping</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff6">
          <name><surname>Awange</surname><given-names>Joseph</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Heck</surname><given-names>Bernhard</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Kutterer</surname><given-names>Hansjörg</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>Geodetic Institute, Karlsruhe Institute of Technology, Karlsruhe 76131, Germany</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>KMI-IRM, Royal Meteorological Institute of Belgium, Brussels 1180, Belgium</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>NOAA National Centers for Environmental Information, Asheville, NC 28801, USA</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>IMK-IFU, Karlsruhe Institute of Technology, Garmisch-Partenkirchen 82467, Germany</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>GNSS Research Center, Wuhan University, Wuhan 430079, China</institution>
        </aff>
        <aff id="aff6"><label>6</label><institution>School of Earth and Planetary Sciences, Curtin University, Perth, WA 6845, Australia</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Peng Yuan (peng.yuan@kit.edu)</corresp></author-notes><pub-date><day>21</day><month>March</month><year>2023</year></pub-date>
      
      <volume>23</volume>
      <issue>6</issue>
      <fpage>3517</fpage><lpage>3541</lpage>
      <history>
        <date date-type="received"><day>21</day><month>September</month><year>2021</year></date>
           <date date-type="rev-request"><day>26</day><month>October</month><year>2021</year></date>
           <date date-type="rev-recd"><day>9</day><month>January</month><year>2023</year></date>
           <date date-type="accepted"><day>1</day><month>March</month><year>2023</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2023 </copyright-statement>
        <copyright-year>2023</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/.html">This article is available from https://acp.copernicus.org/articles/.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d1e181">The ground-based Global Positioning System (GPS) has been
used extensively   to retrieve integrated water vapour (IWV) and has been
adopted as a unique tool for the assessments of atmospheric reanalyses. In
this study, we investigated the multi-temporal-scale variabilities and
trends of IWV over Europe by using IWV time series from 108 GPS stations for more than 2 decades (1994–2018). We then adopted the GPS IWV as a
reference to assess six commonly used atmospheric reanalyses, namely the Climate Forecast System
Reanalysis (CFSR); ERA5; ERA-Interim; the Japanese 55-year Reanalysis
(JRA-55); the Modern-Era Retrospective
Analysis for Research and Applications, version 2 (MERRA-2); and NCEP-DOE AMIP-II Reanalysis (NCEP-2). The GPS results show that the
peaks of the diurnal harmonics are within 15:00–21:00 in local solar time at 90 % of the stations. The diurnal amplitudes are 0–1.2 kg m<inline-formula><mml:math id="M1" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (0 %–8 % of the daily mean IWV), and they are found to be related to seasons and locations with different mechanisms, such as solar heating, land–sea breeze, and orographic circulation. However, mismatches in the diurnal cycle of ERA5 IWV between 09:00 and 10:00 UTC as well as between 21:00 and 22:00 UTC were found and evaluated for the first time, and they can be attributed to the edge effect in each ERA5 assimilation cycle. The average ERA5 IWV shifts are <inline-formula><mml:math id="M2" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula> and 0.19 kg m<inline-formula><mml:math id="M3" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> at the two epochs, and they were found
to be more significant in summer and in the Alps and in Eastern and central
Europe in some cases. Nevertheless, ERA5 outperforms the other reanalyses in
reproducing diurnal IWV anomalies at all the 1-, 3-, and 6-hourly temporal
resolutions. ERA5 is also superior to the others in modelling the annual
cycle and linear trend of IWV. For instance, the IWV trend differences
between ERA5 and GPS are quite small, with a mean value and a standard
deviation of 0.01 % per decade and 0.97 % per decade,
respectively. However, due to significant discrepancies with respect to GPS,
CFSR and NCEP-2 are not recommended for the analysis of IWV trends over
southern Europe and the whole of Europe, respectively.</p>
  </abstract>
    
<funding-group>
<award-group id="gs1">
<funding-source>Deutsche Forschungsgemeinschaft</funding-source>
<award-id>321886779</award-id>
</award-group>
</funding-group>
</article-meta>
  </front>
<body>
      

<?pagebreak page3518?><sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e227">Water vapour is the most important component of the Earth's atmosphere regarding the transport of energy by latent heat and radiative forcing. It is the most important gaseous source of infrared opacity in the atmosphere and thus the largest contributor to the natural greenhouse effect (Kiehl and Trenberth, 1997; Harries, 1997). It plays a key role in water and energy cycles (e.g. Trenberth and Fasullo, 2013), climate change (e.g. Schneider et
al., 2010), and various weather and climate processes (e.g. Vonder Haar et al., 2012) and is crucial for the understanding of many extreme meteorological
phenomena, such as atmospheric rivers (e.g. Zhu and Newell, 1994),
hurricanes (e.g. Ejigu et al., 2021), floods (e.g. Turato et al., 2004), and
droughts and monsoons (e.g. Jiang et al., 2017; Fadnavis et al., 2021).
However, due to its large spatiotemporal variability, its high-accuracy
quantification remains a challenge.</p>
      <p id="d1e230">Characterising the multiple spatiotemporal-scale variabilities and long-term
trends of water vapour is of great importance for Europe, which is like a
peninsula of the Eurasian landmass mainly surrounded by the Arctic Ocean,
Atlantic Ocean, and Mediterranean Sea to the north, west, and south,
respectively. Owing to the moisture from the oceans carried by the
prevailing westerlies, most of western Europe has an oceanic climate with
mild, wet, and turbulent weather in winter. In contrast, southern Europe is
characterised by a well-known dry summer Mediterranean climate. Europe is
generally vulnerable to the extreme events associated with abnormal water
vapour transport and is very sensitive to climate change (Field et al., 2014; Lavers et al., 2016) and has been the fastest warming continent in
recent decades (e.g. Copernicus, 2019). Since a 1 K rise in temperature leads
to a 7 % increase in the water-vapour-holding capacity of the atmosphere
as implied by the Clausius–Clapeyron equation (Trenberth et al., 2003),
Europe's water vapour amount is noticeably increasing (Yuan et al., 2021).
The increasing water vapour content fortifies the radiative forcing, leading
to a higher temperature, which becomes the most powerful if additional water
vapour enters the upper troposphere and lower stratosphere (Solomon et al., 2010). The warmer and moister climate impacts all weather events and
aggravates the risks of extreme events (Trenberth, 2012).</p>
      <p id="d1e233">Atmospheric water vapour content can be expressed by using integrated water
vapour (IWV), which is defined as the total amount of water vapour present
in a vertical atmospheric column from the Earth's surface to the top of the
atmosphere in units of kilogram per square metre (Jones et al., 2020). The IWV is also
known as the total column water vapour (TCWV) or precipitable water vapour
(PWV). At present, numerous techniques have been developed to measure water
vapour, such as balloon-borne radiosondes (e.g. Durre et al., 2018; Kunz et
al., 2013; Müller et al., 2016), aircraft measurements (e.g. Tilmes et
al., 2010; Kunz et al., 2014; Krämer et al., 2020), satellite
observations (e.g. Grossi et al., 2015; Beirle et al., 2018), and
ground-based methods (e.g. Kämpfer, 2013; Vogelmann and Trickl, 2008).
A global navigation satellite system (GNSS), represented by the USA's
Global Positioning System (GPS), has been exploited for water vapour
retrieval by using its ground-based measurements (e.g. Bevis et al., 1992)
or space-based radio occultation (e.g. Kursinski et al., 1995) since the
1990s. Although accurate vertical distribution of water vapour in the upper
troposphere can be obtained by the GPS radio occultation (e.g. Randel and
Wu, 2005; Randel et al., 2007), its accuracy is limited in the lower
troposphere (e.g. Ao et al., 2003; Awange 2018) where the water vapour is
most abundant. On the contrary, the ground-based GPS has proven to be an
effective technique for IWV retrieval with advantages of high accuracy, high
temporal resolution, and all-weather-condition availability (Jones et al., 2020). The ground-based GPS has been utilised for IWV measurement in
numerous global (e.g. Wang and Zhang, 2009; Vey et al., 2010; Chen and Liu,
2016) as well as regional (e.g. Bernet et al., 2020; Ejigu et al., 2021;
Huang et al., 2021) studies. In addition, there have been nearly 3 decades of continuous GPS measurements with increasingly densified networks
in Europe, such as the European Reference Frame (EUREF) Permanent Global
Navigation Satellite System (GNSS) Network (EPN; Bruyninx et al., 2012).
Given these benefits, ground-based GPS offers a unique tool to investigate
the multiple spatiotemporal-scale variabilities of IWV over Europe. The
homogeneously reprocessed long-term time series of GPS IWV is also quite
beneficial to climate change studies (e.g. Van Malderen et al., 2020). GPS
has increasingly been adopted in many studies to investigate various temporal features of
Europe's IWV, such as diurnal cycle (e.g. Diedrich et al., 2016; Steinke et al., 2019), annual cycle (e.g.
Parracho et al., 2018; Van Malderen et al., 2022), and trends (e.g. Nilsson
and Elgered, 2008; Ning et al., 2016; Wang et al., 2016). However, the
multi-temporal-scale variabilities and trends of Europe's IWV have rarely
been comprehensively studied using GPS.</p>
      <p id="d1e236">Atmospheric reanalyses have been extensively adopted as the data source of
IWV acquisition for the last several decades, owing to the benefits of
regional or global coverage, consistent spatiotemporal resolution, and the
availability of many other meteorological variables. However, their products
may still be subject to large uncertainty. On the one hand, this is due to
the fact that the reanalyses from different providers and different versions
are inconsistent in the input data and assimilation schemes, besides using
different physical schemes and representations. For example, the newly
released fifth generation global reanalysis from ECMWF (ERA5; Hersbach et
al., 2020) has assimilated more datasets and instruments, which were not
ingested in its predecessor ERA-Interim (ERAI; Dee et al., 2011). The
assimilation system of ERA5 is also more advanced. On the other hand,
systematic and random errors in the input data are unavoidable. For
instance, the Integrated Global Radiosonde Archive<?pagebreak page3519?> (IGR; Durre et al., 2018) provides a long record of relative humidity observations for the
assimilation of reanalysis, but long-term radiosonde humidity measurements
are very sensitive to changes in instrumentation and measuring practice
(McCarthy et al., 2009; Dai et al., 2011). Therefore, assessments of the
reanalyses' water vapour products are indispensable for the accurate
understanding and interpretation of Europe's weather and climate processes.
The performances of various reanalyses' IWV products in Europe have been
assessed by many regional or global studies using ground-based GPS data, as the
GPS observations are not operationally assimilated by reanalyses (Hagemann
et al., 2003; Bock et al., 2005; Heise et al., 2009; Vey et al., 2010;
Alshawaf et al., 2018; Parracho et al., 2018; Wang et al., 2020; Yuan et
al., 2021). However, it is still quite hard to draw consistent conclusions
on the performances of different reanalyses from these studies, as they are
different in many aspects, such as the numbers and locations of the GPS
stations, period of observations, data processing strategies, and
performance metrics. A consistent assessment of various reanalyses, by using
homogeneously reprocessed long-term time series of GPS IWV as reference in
Europe, is still lacking. In addition, few studies have focused on the
performance of the latest ERA5 in reproducing the temporal features of
Europe's IWV so far.</p>
      <p id="d1e240">In this paper, we focus on characterising the multi-temporal-scale
variabilities and trends of Europe's IWV by using more than 2 decades of
GPS IWV, and then we assess the performances of six reanalyses' IWV products
over Europe. The paper is organised as follows: in Sect. 2, we describe
the GPS and reanalyses datasets, IWV calculation methods, and consistency
evaluation metrics. Section 3 assesses the consistency of daily time series
and representativeness differences, while the diurnal variations and
associated diurnal cycle, annual cycle, and long-term trends of Europe's IWV
are investigated using GPS in Sects. 4, 5, and 6, respectively. The
performances of the reanalyses are also assessed accordingly, and the main
findings are summarised in Sect. 7.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Data and methods</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>GPS data</title>
      <p id="d1e258">To characterise the IWV over Europe and to assess the reanalyses, 1-hourly GPS
IWV retrievals obtained from 108 stations are used (Fig. 1). Most GPS
stations are from the EPN network (Bruyninx et al., 2001). The GPS
observations are from January 1994 to December 2018 with an average time
length of 21 years and an average integration rate of 92 % (Table S1 in the Supplement). The integration rate is the ratio between the number of available daily IWV data points and the theoretical number of all possible observations in the time range. The IWV retrievals were estimated with GPS zenith total delay (ZTD) provided by the Nevada Geodetic Laboratory (NGL; Blewitt et al., 2018). The GPS ZTD products from NGL were used because it covers a long time period of 25 years so that it allows for better evaluations of the diurnal and annual climatological averages and long-term trends. In comparison, another ZTD dataset from EPN-Repro2 (Pacione et al., 2017) only has about 19 years of data, ending in 2014.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><?xmltex \currentcnt{1}?><?xmltex \def\figurename{Figure}?><label>Figure 1</label><caption><p id="d1e263">Geographical distribution of the 108 GPS stations (red
dots). An enlarged version of this figure with station names is provided in
Fig. S1. The coordinates of the stations and their time lengths are provided in Table S1.</p></caption>
          <?xmltex \igopts{width=207.705118pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f01.png"/>

        </fig>

      <p id="d1e272">The NGL processes the GPS data using the newly improved GipsyX v1.0 software
in precise point positioning (PPP) mode (Bertiger et al., 2020). Reprocessed
orbits and clocks from the Jet Propulsion Laboratory (JPL) Repro 3 were used
together with the 2014 International GNSS Service (IGS) reference frame
(IGS14; Rebischung and Schmid, 2016). The observations were weighted based
on an elevation (<inline-formula><mml:math id="M4" display="inline"><mml:mi>e</mml:mi></mml:math></inline-formula>)-dependent function of <inline-formula><mml:math id="M5" display="inline"><mml:mrow><mml:mi>sin⁡</mml:mi><mml:mi>e</mml:mi></mml:mrow></mml:math></inline-formula>. The cutoff elevation
angle was set to 7<inline-formula><mml:math id="M6" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>. The first-order effect of the ionosphere was
removed by employing ionosphere-free combinations of the GPS observations.
The second-order effect was corrected with the International Geomagnetic
Reference Field 12 (IGRF-12; Thébault et al., 2015) and JPL's ionosphere
maps. As for the modelling of tropospheric delay, the Vienna Mapping
Function 1 (VMF1; Boehm et al., 2006) and its associated a priori zenith hydrostatic delay (ZHD) were adopted.</p>
</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Reanalysis data</title>
      <?pagebreak page3520?><p id="d1e309">The IWV derived from six commonly used global atmospheric reanalyses,
namely the newly released fifth generation global reanalysis (ERA5) and its
predecessor ERA-Interim (ERAI) from ECMWF; the Japanese 55-year Reanalysis
(JRA-55) from the Japan Meteorological Agency (JMA); the Modern-Era Retrospective
Analysis for Research and Applications, version 2 (MERRA-2), from NASA's Global
Modeling and Assimilation Office (GMAO); and the Climate Forecast System
Reanalysis (CFSR) and NCEP-DOE AMIP-II Reanalysis (NCEP-2) from the National
Centers for Environmental Prediction (NCEP), is analysed. The features of
the reanalyses are summarised in Table 1. It is worth noting that JRA-55 only
provides humidity information at 27 pressure levels from 1000 to 100 hPa,
though it has 37 levels in total. These six reanalyses are selected as their
IWV products have covered the period of the ground-based GPS data available since
1994. Despite ERAI having been decommissioned and superseded by ERA5 in
August 2019, we still include it for the purpose of evaluating the progress
of its successor ERA5. We therefore restricted the time range of all data
records to a common period from 1994 to 2018.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e315">Six atmospheric reanalyses used in this study and their
characteristics.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="7">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:colspec colnum="5" colname="col5" align="left"/>
     <oasis:colspec colnum="6" colname="col6" align="left"/>
     <oasis:colspec colnum="7" colname="col7" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Reanalysis</oasis:entry>
         <oasis:entry colname="col2">CFSR</oasis:entry>
         <oasis:entry colname="col3">ERA5</oasis:entry>
         <oasis:entry colname="col4">ERAI</oasis:entry>
         <oasis:entry colname="col5">JRA-55</oasis:entry>
         <oasis:entry colname="col6">MERRA-2</oasis:entry>
         <oasis:entry colname="col7">NCEP-2</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Source</oasis:entry>
         <oasis:entry colname="col2">NCEP</oasis:entry>
         <oasis:entry colname="col3">ECMWF</oasis:entry>
         <oasis:entry colname="col4">ECMWF</oasis:entry>
         <oasis:entry colname="col5">JMA</oasis:entry>
         <oasis:entry colname="col6">GMAO</oasis:entry>
         <oasis:entry colname="col7">NCEP</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Assimilation</oasis:entry>
         <oasis:entry colname="col2">3DVAR</oasis:entry>
         <oasis:entry colname="col3">4DVAR</oasis:entry>
         <oasis:entry colname="col4">4DVAR</oasis:entry>
         <oasis:entry colname="col5">4DVAR</oasis:entry>
         <oasis:entry colname="col6">3DVAR</oasis:entry>
         <oasis:entry colname="col7">3DVAR</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Time range</oasis:entry>
         <oasis:entry colname="col2">1979–present</oasis:entry>
         <oasis:entry colname="col3">1940–present</oasis:entry>
         <oasis:entry colname="col4">1979–August 2019</oasis:entry>
         <oasis:entry colname="col5">1958–present</oasis:entry>
         <oasis:entry colname="col6">1980–present</oasis:entry>
         <oasis:entry colname="col7">1979–present</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Temporal res. (hour)</oasis:entry>
         <oasis:entry colname="col2">6</oasis:entry>
         <oasis:entry colname="col3">1</oasis:entry>
         <oasis:entry colname="col4">6</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">3</oasis:entry>
         <oasis:entry colname="col7">6</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Horizontal res. (lat <inline-formula><mml:math id="M7" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> long)</oasis:entry>
         <oasis:entry colname="col2">0.5<inline-formula><mml:math id="M8" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M9" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.5<inline-formula><mml:math id="M10" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">0.25<inline-formula><mml:math id="M11" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M12" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.25<inline-formula><mml:math id="M13" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">0.75<inline-formula><mml:math id="M14" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M15" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.75<inline-formula><mml:math id="M16" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">1.25<inline-formula><mml:math id="M17" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M18" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.25<inline-formula><mml:math id="M19" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">0.5<inline-formula><mml:math id="M20" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M21" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.625<inline-formula><mml:math id="M22" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">2.5<inline-formula><mml:math id="M23" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M24" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.5<inline-formula><mml:math id="M25" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Pressure levels</oasis:entry>
         <oasis:entry colname="col2">37</oasis:entry>
         <oasis:entry colname="col3">37</oasis:entry>
         <oasis:entry colname="col4">37</oasis:entry>
         <oasis:entry colname="col5">37</oasis:entry>
         <oasis:entry colname="col6">42</oasis:entry>
         <oasis:entry colname="col7">17</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">References</oasis:entry>
         <oasis:entry colname="col2">Saha et al.</oasis:entry>
         <oasis:entry colname="col3">Hersbach et</oasis:entry>
         <oasis:entry colname="col4">Dee et al. (2011)</oasis:entry>
         <oasis:entry colname="col5">Kobayashi et</oasis:entry>
         <oasis:entry colname="col6">Gelaro et</oasis:entry>
         <oasis:entry colname="col7">Kanamitsu et</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(2010, 2014)</oasis:entry>
         <oasis:entry colname="col3">al. (2020)</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5">al. (2015)</oasis:entry>
         <oasis:entry colname="col6">al. (2017)</oasis:entry>
         <oasis:entry colname="col7">al. (2002)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><title>IWV retrievals</title>
      <p id="d1e727">The zenith total delay (ZTD) estimates derived from GPS data processing can
be converted into IWV, the total amount of water vapour present in a vertical atmospheric column from the Earth's surface to the top of the atmosphere in units of kilogram per square metre, using the following equation (Bevis et al., 1992):
            <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M26" display="block"><mml:mrow><mml:mtext>IWV</mml:mtext><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi>V</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mfenced close="]" open="["><mml:mrow><mml:msubsup><mml:mi>k</mml:mi><mml:mn mathvariant="normal">2</mml:mn><mml:mo>′</mml:mo></mml:msubsup><mml:mo>+</mml:mo><mml:msub><mml:mi>k</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mfenced open="(" close=")"><mml:mrow><mml:mtext>ZTD</mml:mtext><mml:mo>-</mml:mo><mml:mtext>ZHD</mml:mtext></mml:mrow></mml:mfenced><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi>V</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> denotes the gas constant for water vapour, <inline-formula><mml:math id="M28" display="inline"><mml:mrow><mml:msubsup><mml:mi>k</mml:mi><mml:mn mathvariant="normal">2</mml:mn><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M29" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> are atmospheric refractivity constants (Bevis et al., 1994), and <inline-formula><mml:math id="M30" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> denotes the weighted mean temperature:
            <disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M31" display="block"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mo>∫</mml:mo><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">top</mml:mi></mml:msub></mml:mrow></mml:msubsup><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi>e</mml:mi><mml:mi>T</mml:mi></mml:mfrac></mml:mstyle><mml:mi mathvariant="normal">d</mml:mi><mml:mi>p</mml:mi></mml:mrow><mml:mrow><mml:msub><mml:mo>∫</mml:mo><mml:mrow><mml:msubsup><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi><mml:mi mathvariant="normal">top</mml:mi></mml:msubsup></mml:mrow></mml:msub><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mi>e</mml:mi><mml:mrow><mml:msup><mml:mi>T</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mi mathvariant="normal">d</mml:mi><mml:mi>p</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M32" display="inline"><mml:mi>e</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M33" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> are water vapour pressure and temperature profiles of the
geopotential heights of the GPS station (<inline-formula><mml:math id="M34" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) to the top level of
reanalysis (<inline-formula><mml:math id="M35" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">top</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), respectively.</p>
      <p id="d1e943">The ZHD was modelled as follows (Saastamoinen, 1972; Davis et al., 1985):
            <disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M36" display="block"><mml:mrow><?xmltex \hack{\hbox\bgroup\fontsize{9.1}{9.1}\selectfont$\displaystyle}?><mml:mtext mathvariant="normal">ZHD</mml:mtext><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2.2768</mml:mn><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>p</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2.66</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:mi>cos⁡</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2.8</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">7</mml:mn></mml:mrow></mml:msup><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo><?xmltex \hack{$\egroup}?></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:msub><mml:mi>p</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> denotes the pressure at the GPS station with a latitude of <inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and a height of <inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The <inline-formula><mml:math id="M40" display="inline"><mml:mrow><mml:msub><mml:mi>p</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M41" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are computed by using the ERA5 pressure-level product (see Yuan et al., 2021, and references therein). ERA5 is selected as it can provide a 1-hourly product without temporal interpolation.</p>
      <p id="d1e1076">IWV values at the GPS stations are also calculated from the six reanalyses.
In this calculation, the pressure-level products of the reanalyses are used
rather than their surface-level IWV products, though it requires a heavier
workload. This is because the GPS station and its nearby reanalysis surface
grids are usually related to different heights. Vertical IWV adjustment is
therefore usually required for the intercomparison between the IWV estimates
from GPS and reanalyses. Compared to the reanalyses' surface-level products,
their pressure-level products allow for a better characterisation of the
vertical distribution of water vapour and tends to minimise the errors of
the vertical adjustment (Parracho et al., 2018).</p>
      <p id="d1e1079">The scheme of the calculation is illustrated in Fig. 2. We assume a GPS station
with a geopotential height of <inline-formula><mml:math id="M42" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is located between two adjacent
reanalysis pressure levels (<inline-formula><mml:math id="M43" display="inline"><mml:mrow><mml:msub><mml:mi>p</mml:mi><mml:mi>j</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M44" display="inline"><mml:mrow><mml:msub><mml:mi>p</mml:mi><mml:mrow><mml:mi>j</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>). We first determine its eight surrounding reanalysis grid nodes at these pressure levels (<inline-formula><mml:math id="M45" display="inline"><mml:mrow><mml:msubsup><mml:mi>N</mml:mi><mml:mi>i</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:msubsup><mml:mi>N</mml:mi><mml:mi>i</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M47" display="inline"><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:math></inline-formula>, and 4) and four auxiliary points (<inline-formula><mml:math id="M48" display="inline"><mml:mrow><mml:msub><mml:mi>A</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).
The auxiliary points are located at the GPS station height, whereas their
horizontal locations are identical to the associated reanalysis nodes. We
then calculate the related meteorological variables at each auxiliary point.
Exponential and linear interpolations are employed for the vertical
corrections of pressure and temperature, respectively. If the auxiliary
point is lower than the lowest pressure level (e.g. 1000 hPa), an
extrapolation of these variables is conducted. For details of the vertical
adjustment, readers are referred to Schüler (2001) and Wang et al. (2005). Next, we calculate the IWV at each auxiliary point by using a
vertical integration:
            <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M49" display="block"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi>i</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msubsup><mml:mo>∫</mml:mo><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">top</mml:mi></mml:msub></mml:mrow></mml:msubsup><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi>q</mml:mi><mml:mi>g</mml:mi></mml:mfrac></mml:mstyle><mml:mi mathvariant="normal">d</mml:mi><mml:mi>p</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M50" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M51" display="inline"><mml:mi>g</mml:mi></mml:math></inline-formula> are specific humidity and gravitational acceleration
profiles from <inline-formula><mml:math id="M52" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to the reanalysis top level, respectively.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><?xmltex \currentcnt{2}?><?xmltex \def\figurename{Figure}?><label>Figure 2</label><caption><p id="d1e1260">Schematic plot of the vertical and horizontal interpolation of the reanalysis pressure-level products. The IWV at each auxiliary point (<inline-formula><mml:math id="M53" display="inline"><mml:mrow><mml:msub><mml:mi>A</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; orange dots) is calculated with vertical interpolation or extrapolation of the adjacent reanalysis nodes (<inline-formula><mml:math id="M54" display="inline"><mml:mrow><mml:msubsup><mml:mi>N</mml:mi><mml:mi>i</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M55" display="inline"><mml:mrow><mml:msubsup><mml:mi>N</mml:mi><mml:mi>i</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mi>j</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula>; green dots). The IWV at the GPS station (red dot) is then estimated with horizontal interpolation of the auxiliary points.</p></caption>
          <?xmltex \igopts{width=184.942913pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f02.png"/>

        </fig>

      <?pagebreak page3521?><p id="d1e1320">It is noteworthy that a geopotential height system is employed in the
reanalyses. Accordingly, the geopotential heights (<inline-formula><mml:math id="M56" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">gp</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) of the GPS stations rather than their ellipsoidal (<inline-formula><mml:math id="M57" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">el</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) or orthometric heights (<inline-formula><mml:math id="M58" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">or</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are used in the above calculations. The conversion of height systems is carried out as follows (Dirksen et al., 2014; Wang et al., 2016; World Meteorological Organization, 2018):
            <disp-formula id="Ch1.Ex1"><mml:math id="M59" display="block"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">or</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">el</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:mi>N</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M60" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E5"><mml:mtd><mml:mtext>5</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">gp</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="italic">γ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow><mml:mn mathvariant="normal">9.80665</mml:mn></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi>R</mml:mi><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>⋅</mml:mo><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">or</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mi>R</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>+</mml:mo><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">or</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E6"><mml:mtd><mml:mtext>6</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:msub><mml:mi mathvariant="italic">γ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mn mathvariant="normal">9.780325</mml:mn><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1.93185</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mi>sin⁡</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mn mathvariant="normal">6.69435</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:msup><mml:mi>sin⁡</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E7"><mml:mtd><mml:mtext>7</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi>R</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">6.378137</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1.006803</mml:mn><mml:mo>-</mml:mo><mml:mn mathvariant="normal">6.706</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>⋅</mml:mo><mml:mi>sin⁡</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            where <inline-formula><mml:math id="M61" display="inline"><mml:mi>N</mml:mi></mml:math></inline-formula> is the geoid heights in metre from the Earth Gravitational
Model 2008 (EGM2008; Pavlis et al., 2012).</p>
      <p id="d1e1637">In the end, we estimate the IWV at the GPS station using a horizontal
interpolation with an inverse distance weighting algorithm (Jade and
Vijayan, 2008).</p>
      <p id="d1e1640">Representativeness differences arise in the comparison of the IWV derived by
the ground-based GPS and reanalyses (Bock and Parracho, 2019). This is
because local variations of IWV measured by the GPS might fail to be
resolved by the reanalyses due to their coarse horizontal resolution. The
representativeness differences can be evaluated statistically as proposed by
Bock and Parracho (2019):
            <disp-formula id="Ch1.E8" content-type="numbered"><label>8</label><mml:math id="M62" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub><mml:mo>=</mml:mo><mml:mo movablelimits="false">max⁡</mml:mo><mml:mfenced open="(" close=")"><mml:mfenced open="|" close="|"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi>i</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi>k</mml:mi></mml:msub></mml:mrow></mml:mfenced></mml:mfenced><mml:mo>,</mml:mo><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi>i</mml:mi><mml:mi>k</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">3</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">4</mml:mn><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi>i</mml:mi><mml:mo>≠</mml:mo><mml:mi>k</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M64" display="inline"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi>k</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are the IWV values of
the horizontal auxiliary points <inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msub><mml:mi>A</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M66" display="inline"><mml:mrow><mml:msub><mml:mi>A</mml:mi><mml:mi>k</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, respectively (Fig. 2). Bock and Parracho (2019) found that the measure <inline-formula><mml:math id="M67" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula> was correlated with the standard deviation of the IWV differences between GPS and ERAI (<inline-formula><mml:math id="M68" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and thus concluded that the representativeness differences between the IWV from GPS and ERAI contributed to their discrepancies. Here, we extend their work by estimating and comparing the representativeness statistics of the six reanalyses with various spatial resolutions (Table 1).</p>
</sec>
<sec id="Ch1.S2.SS4">
  <label>2.4</label><title>Pre-processing</title>
      <p id="d1e1786">The 1-, 3-, and 6-hourly IWV time series are screened by using a robust
outlier detection method as follows (Yuan et al., 2021). For each data
point, the data within a 30 d window centred at this point are extracted.
The 25th percentile (Q1), 75th percentile (Q3), and interquartile range
(IQR) of the subsequent time series are then calculated. Finally, the data
point is identified as an outlier if it is outside the range of
<inline-formula><mml:math id="M69" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mtext>Q1</mml:mtext><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.5</mml:mn><mml:mo>×</mml:mo><mml:mtext>IQR</mml:mtext><mml:mo>,</mml:mo><mml:mtext>Q3</mml:mtext><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1.5</mml:mn><mml:mo>×</mml:mo><mml:mtext>IQR</mml:mtext><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. The IQR
threshold and the 30 d sliding window are adopted, as they allow for a good
robustness and a proper accommodation for the natural variability of IWV. On
average, about 1 % of data were filtered out by the data screening.</p>
      <p id="d1e1822">In this study, the performances of reanalysis IWV products in daily time
series, diurnal cycle and variations, monthly annual cycles, and long-term
linear trends are evaluated. As the temporal resolutions of the datasets are
different, temporal interpolation and aggregation are conducted. To obtain
daily mean IWV values, the 1-, 3-, and 6-hourly IWV time series are
aggregated if they have at least 12, 4, and 2 data points in a day,
respectively. The daily mean IWV time series at each station is further
aggregated into monthly mean IWV series if there are at least 15 data points
available in a month.</p>
</sec>
<sec id="Ch1.S2.SS5">
  <label>2.5</label><title>Homogenisation</title>
      <p id="d1e1834">The GPS IWV time series can be inhomogeneous due to changes in GPS data
processing strategies and station-related changes like hardware changes or
changes in the electromagnetic environment (Van Malderen et al., 2020;
Nguyen et al., 2021, and references therein). We employed a homogenisation
approach as described in Appendix A with step-by-step details and examples
at two stations (HERS and ERLA).</p>
      <p id="d1e1837">Here, we only provide a brief introduction to the approach. We first avoided
inhomogeneities due to changes in GPS data processing strategy by using the
homogeneously reprocessed GPS ZTD product. We then homogenised the GPS IWV
time series by using the RHtestsV4 software (Wang and Feng,<?pagebreak page3522?> 2013). This
software is especially developed for the detection and adjustment of
changepoints in climatic time series, and it has been used in the
homogenisation of IWV time series in previous studies (Ning et al., 2016;
Schröder et al., 2016; Van Malderen et al., 2020).</p>
      <p id="d1e1840">We took the IWV time series from all six reanalyses as references for
the GPS IWV homogenisation and used a strategy to avoid the impacts of
possible changepoints in individual reanalyses. However, we did not
homogenise the reanalyses IWV time series because they represent the native
quality of the reanalyses that we would like to assess. In addition to
matching the detected changepoints with inspecting GPS metadata information
(GPS station log files and IGS mail archives (IGSMAIL)), we also allowed for possible
undocumented changepoints in the GPS IWV time series.</p>
</sec>
<sec id="Ch1.S2.SS6">
  <label>2.6</label><title>Metrics for consistency evaluation</title>
      <p id="d1e1851">To evaluate the performances of the reanalyses in reproducing IWV,
the Kling–Gupta efficiency (KGE) is employed as a metric. The KGE is a composite
index introduced by Gupta et al. (2009) and modified by Kling et al. (2012).
It takes bias, variability, and correlation into account in the equation
below:
            <disp-formula id="Ch1.E9" content-type="numbered"><label>9</label><mml:math id="M70" display="block"><mml:mrow><mml:mtext>KGE</mml:mtext><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msqrt><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="italic">β</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:mo>(</mml:mo><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:msqrt><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          with

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M71" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E10"><mml:mtd><mml:mtext>10</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi mathvariant="italic">β</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E11"><mml:mtd><mml:mtext>11</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mtext>CV</mml:mtext><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mtext>CV</mml:mtext><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            where <inline-formula><mml:math id="M72" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M73" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M74" display="inline"><mml:mrow><mml:msub><mml:mtext>CV</mml:mtext><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are the mean value, standard deviation, and coefficient of variation of the reanalysis IWV time series, respectively. <inline-formula><mml:math id="M75" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M76" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:msub><mml:mtext>CV</mml:mtext><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are the corresponding parameters for GPS. <inline-formula><mml:math id="M78" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M79" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula> indicate the consistencies in the mean and variability, respectively. In the case of <inline-formula><mml:math id="M80" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M81" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">μ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> being equal to zero, such as for the diurnal anomalies
in Sect. 4.3, <inline-formula><mml:math id="M82" display="inline"><mml:mrow><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:math></inline-formula>. <inline-formula><mml:math id="M83" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula>
indicates the Pearson correlation coefficient between the GPS and reanalyses
time series. With perfect consistencies in mean, variability, and
correlation, the values of <inline-formula><mml:math id="M84" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M85" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M86" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> are identical to 1,
respectively. From Eq. (9), it follows that a larger KGE score indicates a
better consistency. Ideally, the KGE metric reaches its maximum of 1.</p>
      <p id="d1e2162">In addition, to be comparable to some previous studies, we also used the
root mean square estimation of the IWV differences between the reanalyses
and GPS:
            <disp-formula id="Ch1.E12" content-type="numbered"><label>12</label><mml:math id="M87" display="block"><mml:mrow><mml:msub><mml:mtext>rms</mml:mtext><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msqrt><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mo>∑</mml:mo><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mi>n</mml:mi></mml:msubsup><mml:msup><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi mathvariant="normal">R</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow><mml:mi>n</mml:mi></mml:mfrac></mml:mstyle></mml:msqrt><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M88" display="inline"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi mathvariant="normal">R</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M89" display="inline"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi mathvariant="normal">G</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are the IWV time series at a specific station from reanalysis and GPS, respectively, and <inline-formula><mml:math id="M90" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula> is number of data points in the IWV time series.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Assessments of daily time series</title>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>Representativeness differences</title>
      <p id="d1e2260">Figure 3 compares the standard deviations of daily IWV difference (<inline-formula><mml:math id="M91" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and the representativeness statistic (<inline-formula><mml:math id="M92" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula>) for the six reanalyses. The first point to
note is that <inline-formula><mml:math id="M93" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M94" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula> are strongly correlated for all the reanalyses, with <inline-formula><mml:math id="M95" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> values from 0.76 for NCEP-2 to 0.90 for ERA5. The result is in line with Bock and Parracho (2019), who compared ERAI to a global GPS network. Figure 3 indicates that
the representativeness differences contribute to the discrepancies between
the reanalyses and GPS. The larger <inline-formula><mml:math id="M96" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M97" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula> values are found at stations close to mountains or seas, such
as BZRG (Bolzano, Italy; 46.50<inline-formula><mml:math id="M98" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 11.34<inline-formula><mml:math id="M99" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) and
TORI (Turin, Italy; 45.06<inline-formula><mml:math id="M100" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 7.66<inline-formula><mml:math id="M101" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) at the foothills of
the Alps and ALME (Almería, Spain; 36.85<inline-formula><mml:math id="M102" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 2.46<inline-formula><mml:math id="M103" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> W) near the west coast of the Mediterranean Sea. On the whole, ERA5
is characterised by the lowest <inline-formula><mml:math id="M104" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M105" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula>, with values of 0.5–1.6 and 0.2–2.1 kg m<inline-formula><mml:math id="M106" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, respectively. In contrast, NCEP-2 has the largest <inline-formula><mml:math id="M107" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula>, with values of 1.1–3.0 and 1.8–5.2 kg m<inline-formula><mml:math id="M109" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, respectively. The difference could be due to the fact that the spatiotemporal resolution of ERA5 is much higher than of NCEP-2 as indicated in Table 1. This result indicates that ERA5, with improved spatiotemporal
resolution and data assimilation, is capable of reducing the discrepancy and
representativeness difference with respect to GPS.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F3" specific-use="star"><?xmltex \currentcnt{3}?><?xmltex \def\figurename{Figure}?><label>Figure 3</label><caption><p id="d1e2463">Scatterplots showing the relationships between the standard deviations of daily IWV difference (<inline-formula><mml:math id="M110" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and the representativeness error statistic (<inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>max⁡</mml:mo></mml:msub></mml:mrow></mml:math></inline-formula>) for the 108 GPS stations.</p></caption>
          <?xmltex \igopts{width=441.017717pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f03.png"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Assessments using KGE</title>
      <p id="d1e2502">Figure 4 shows the geographical distributions of the ratio of mean <inline-formula><mml:math id="M112" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>,
the ratio of coefficient of variation <inline-formula><mml:math id="M113" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, the correlation <inline-formula><mml:math id="M114" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula>, and
the synthetic KGE metric for the six reanalyses by using the daily GPS IWV
time series as references. Moreover, the statistics of these scores are
displayed in Fig. 5 with box-and-whisker plots. From the first column of
Figs. 4 and 5a we can see that <inline-formula><mml:math id="M115" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula> scores are slightly larger than 1
for all the reanalyses except JRA-55, indicating a general wet bias with
respect to the GPS IWV. For example, MERRA-2 has the largest median <inline-formula><mml:math id="M116" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>
with a value of 1.04, indicating a general wet bias of 4 %. Only JRA-55
scores a median <inline-formula><mml:math id="M117" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula> smaller than 1 (0.99, Fig. 5a), indicating a slight
dry bias of 1 %. The wet and dry biases in the reanalyses have  partly been reported by several previous studies. For instance, Schröder et al. (2018) concluded that CFSR, ERAI, and MERRA-2 are too moist over Europe
compared to the ensemble mean of various satellite and reanalysis IWV
records, whereas JRA-55 has negligible bias there. The wet bias in ERAI over
Europe was also noted by Parracho et al. (2018). Analysing the reasons of
the biases is of potential interest; however, it would go beyond the scope
of this paper.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F4" specific-use="star"><?xmltex \currentcnt{4}?><?xmltex \def\figurename{Figure}?><label>Figure 4</label><caption><p id="d1e2550">Plots of the KGE parameters for the daily IWV time series
of the 108 GPS stations. <inline-formula><mml:math id="M118" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M119" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula> indicate the
consistencies in the mean and variability, respectively. <inline-formula><mml:math id="M120" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> indicates
the Pearson correlation coefficient between the GPS and reanalyses time
series. With perfect consistencies in mean, variability, and correlation,
<inline-formula><mml:math id="M121" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M122" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M123" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> are identical to 1, respectively. When
<inline-formula><mml:math id="M124" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M125" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M126" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> are identical to 1, the KGE score will reach
its maximum value of 1.</p></caption>
          <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f04.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5" specific-use="star"><?xmltex \currentcnt{5}?><?xmltex \def\figurename{Figure}?><label>Figure 5</label><caption><p id="d1e2625">Box–whisker plots of the KGE parameters for the daily time series <bold>(a–d)</bold> and monthly annual cycle of IWV <bold>(e–h)</bold> from the reanalyses compared to GPS for the 108 stations.</p></caption>
          <?xmltex \igopts{width=441.017717pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f05.png"/>

        </fig>

      <?pagebreak page3524?><p id="d1e2641">Regarding the consistency in variability, most of the <inline-formula><mml:math id="M127" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula> scores are
less than 1, with the associated median values ranging between 0.96 and 0.98
(Fig. 5b). The results indicate a good reproduction of daily IWV variability
by the reanalyses, albeit with a slight underestimation. The correlations
are also pretty good with median values larger than 0.97 (Fig. 5c). However,
the scores in variability and correlation are lower for the coastal
stations, as shown in the second and third columns of Fig. 4, respectively.
In particular, <inline-formula><mml:math id="M128" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M129" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> of NCEP-2 are less than 0.96 for some
coastal stations located in western and southern Europe. This could be
explained by the representativeness differences that impact the consistency
of the IWV from reanalyses and GPS in their variabilities. For a coastal GPS
station with an on-site measurement of IWV, part of its associated four
reanalysis grid nodes may be located over the sea whereas others over land.
As a consequence, the representativeness difference for such a coastal site
is more severe than inland stations surrounded with flat terrain due to
land–sea thermal contrast (Drobinski et al., 2018).</p>
      <p id="d1e2665">Figure 5d compares the overall consistency in daily IWV evaluated using KGE.
It can be seen that ERA5 is characterised by the largest median KGE (0.97).
The result reveals the superiority of ERA5 over the other reanalyses.
Moreover, comparing <inline-formula><mml:math id="M130" display="inline"><mml:mi mathvariant="italic">β</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M131" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M132" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> (Fig. 5a–c) shows that
<inline-formula><mml:math id="M133" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> tends to contribute the least to the overall inconsistency, indicating
that improving the consistencies in both mean values and variabilities is more
important for the daily IWV time series.</p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Assessments of diurnal variations</title>
      <p id="d1e2705">Despite the atmospheric water vapour being quite unstable, it is
characterised by a diurnal cycle. The diurnal IWV cycle can be driven by
different mechanisms, such as evapotranspiration and condensation related to
temperature, solar heating, and underlying surface conditions, as well as
advection of air at different spatial scales (Dai et al., 2002; Diedrich et
al., 2016; Koji et al., 2022).</p>
      <p id="d1e2708">In this section, the diurnal variations of IWV are investigated in two
regards: diurnal cycle and diurnal anomaly. The diurnal anomalies
(<inline-formula><mml:math id="M134" display="inline"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi mathvariant="normal">DA</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are calculated as follows (Diedrich et al., 2016;
Steinke et al., 2019):
          <disp-formula id="Ch1.E13" content-type="numbered"><label>13</label><mml:math id="M135" display="block"><mml:mrow><mml:msub><mml:mtext>IWV</mml:mtext><mml:mi mathvariant="normal">DA</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mtext>IWV</mml:mtext><mml:mo>-</mml:mo><mml:mover accent="true"><mml:mtext>IWV</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where IWV is the 1-hourly IWV time series in 1 d, and <inline-formula><mml:math id="M136" display="inline"><mml:mover accent="true"><mml:mtext>IWV</mml:mtext><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> is the associated daily mean.</p>
      <p id="d1e2756">Each station's diurnal cycle is computed by averaging its diurnal anomalies
for each season separately and for the entire time span. Diurnal and
semidiurnal harmonics are calculated with least squares estimation (LSE)
based on the seasonal-averaged and all-time-averaged diurnal anomalies:
          <disp-formula id="Ch1.E14" content-type="numbered"><label>14</label><mml:math id="M137" display="block"><mml:mrow><mml:mtext>IWV</mml:mtext><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msubsup><mml:mo>∑</mml:mo><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup><mml:msub><mml:mi>A</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mi>sin⁡</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">π</mml:mi></mml:mrow><mml:mn mathvariant="normal">24</mml:mn></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mi>t</mml:mi><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where <inline-formula><mml:math id="M138" display="inline"><mml:mi>t</mml:mi></mml:math></inline-formula> is local solar time (LST) in hours, and <inline-formula><mml:math id="M139" display="inline"><mml:mrow><mml:msub><mml:mi>A</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M140" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are
the amplitudes and phases of the diurnal (<inline-formula><mml:math id="M141" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) and semidiurnal (<inline-formula><mml:math id="M142" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>)
cycles, respectively. The phases are then adjusted to the peaks of the
associated harmonics, with <inline-formula><mml:math id="M143" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub><mml:mo>∈</mml:mo><mml:mo>[</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">24</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M144" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">φ</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>∈</mml:mo><mml:mo>[</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mo>,</mml:mo><mml:mn mathvariant="normal">12</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> LST in hours.</p>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Diurnal GPS IWV cycle</title>
      <p id="d1e2923">Starting with the all-time-averaged amplitudes of the diurnal GPS IWV
harmonic shown in Fig. 6e, two remarkable values can first be noted at
stations NICO (Nicosia, Cyprus; 33.14<inline-formula><mml:math id="M145" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 33.40<inline-formula><mml:math id="M146" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E;
161.9 m) and ZECK (Zelenchukskaya, Russia; 43.79<inline-formula><mml:math id="M147" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 41.57<inline-formula><mml:math id="M148" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E; 1143.4 m), with values of 1.2 and 1.0 kg m<inline-formula><mml:math id="M149" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
respectively. Moreover, the diurnal harmonics at the Mediterranean Coast are
generally stronger than at the other regions in Europe (0.5–0.8 kg m<inline-formula><mml:math id="M150" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> versus 0–0.5 kg m<inline-formula><mml:math id="M151" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Obvious seasonal differences can also be seen in their diurnal harmonics, with significantly larger amplitudes<?pagebreak page3525?> in summer (June, July, and August; JJA) than in the other seasons due to the stronger solar
heating effect with minimal cloud coverage in Mediterranean summers
(Enriquez-Alonso et al., 2016). However, the semidiurnal harmonics are much
weaker, and their seasonal variations are less significant (Fig. 6f–j).
The all-time-averaged semidiurnal amplitudes are lower than 0.22 kg m<inline-formula><mml:math id="M152" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, except for the two stations NICO and ZECK with values of 0.4 and 0.3 kg m<inline-formula><mml:math id="M153" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, respectively. The ratios between the all-time-averaged
semidiurnal and diurnal amplitudes are lower than 30 % at 88 % of the
stations (95 out of 108). As for the phases, the diurnal and semidiurnal terms are
generally consistent over seasons (Fig. 6k–t), and their all-time-averaged
peaks are within 15:00–21:00 and 01:00–06:00 LST at 90 % of the stations
(97 out of 108), respectively.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><?xmltex \currentcnt{6}?><?xmltex \def\figurename{Figure}?><label>Figure 6</label><caption><p id="d1e3025">Plots of the amplitudes <bold>(a, f)</bold> and phases <bold>(k, p)</bold> for the first (<inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) and second (<inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) harmonics of the diurnal GPS IWV cycle averaged in March, April, and May (MAM; spring) at each station, respectively. The other subplots are for JJA (summer); September, October, and November (SON; autumn); December, January, and February (DJF; winter); and annual, from left to right, respectively. The phases are in local solar time (LST) at the peak of associated harmonics.</p></caption>
          <?xmltex \igopts{width=441.017717pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f06.png"/>

        </fig>

      <p id="d1e3062">In order to compare the characteristics of diurnal IWV amplitudes at
different stations, we calculated each station's relative amplitude as the
ratio between their respective (semi) diurnal amplitudes and mean IWV as
displayed in Fig. 7a and d. We classified the GPS stations into three types
according to their geographical characteristics (Fig. 7a) and analysed their
relationships with each station's altitude and distance to sea (SeaDist).
Firstly, we divided the stations with a limit of 20 km on their SeaDist. We
further separated the stations located at the Mediterranean Coast (MedCoast;
SeaDist <inline-formula><mml:math id="M156" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> km; 32<inline-formula><mml:math id="M157" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N <inline-formula><mml:math id="M158" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> lat <inline-formula><mml:math id="M159" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">46</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M160" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 5<inline-formula><mml:math id="M161" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> W <inline-formula><mml:math id="M162" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> long <inline-formula><mml:math id="M163" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 45<inline-formula><mml:math id="M164" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) from the other coastal (OtherCoast) stations because their characteristics are quite different as can be seen from Fig. 7a. Consequently, the 108 stations are classified into 62 Inland stations, 12 MedCoast stations, and 34 OtherCoast stations.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><?xmltex \def\figurename{Figure}?><label>Figure 7</label><caption><p id="d1e3145"><bold>(a)</bold> Relative amplitudes of the first harmonic (<inline-formula><mml:math id="M165" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) of the diurnal GPS IWV cycle. Panels <bold>(b)</bold> and <bold>(c)</bold> are the variations of the relative <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> amplitudes with respect to station altitude and distance to sea, respectively. Panels <bold>(d)</bold>–<bold>(f)</bold> are the same as panels <bold>(a)</bold>–<bold>(c)</bold> but for the second harmonic (<inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>). The stations are classified into three types, namely Inland, MedCoast, and OtherCoast. The type of Inland includes 62 stations with their distance to sea (SeaDist) no shorter than 20 km. The type of MedCoast contains 12 stations located at the coastal region of the Mediterranean (SeaDist <inline-formula><mml:math id="M168" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> km; 32<inline-formula><mml:math id="M169" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N <inline-formula><mml:math id="M170" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> lat <inline-formula><mml:math id="M171" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 46<inline-formula><mml:math id="M172" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 45<inline-formula><mml:math id="M173" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E <inline-formula><mml:math id="M174" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> long <inline-formula><mml:math id="M175" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 5<inline-formula><mml:math id="M176" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> W). The rest of the 34 stations are classified as OtherCoast.</p></caption>
          <?xmltex \igopts{width=441.017717pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f07.png"/>

        </fig>

      <p id="d1e3284">As can be seen from Fig. 7a–c, all OtherCoast stations are lower than
300 m, and their relative diurnal IWV amplitudes are the weakest, with a
range from 0.3 % to 1.9 % and a median of 1.1 %. Within the altitude limit of 300 m, the Inland stations are characterised by moderately larger diurnal amplitudes (1.5 %–2.5 %). The results indicate the effect of land–sea breeze circulation on mitigating the intensity of the diurnal IWV cycle at the Atlantic coasts of Europe with respect to inland Europe. However, the land–sea breeze effect can be less significant for the MedCoast stations because their diurnal amplitudes are significantly larger (1.1 %–4.2 %) than the OtherCoast stations'. The stronger diurnal IWV cycles at the MedCoast stations can be explained by the stronger solar heating effect at the Mediterranean Coast than at the other European coasts, especially during summer daytime under stable and clear-sky weather conditions. In addition, it can be seen from Fig. 7b and e that the relative diurnal and semidiurnal IWV amplitudes are well correlated with altitudes, with correlation coefficients of 0.66 and 0.67, respectively. This
relationship indicates the effect of orographic circulation, which can
enhance the diurnal range of temperature at higher altitudes (Diedrich et
al., 2016).</p>
      <p id="d1e3287">In addition, we selected six stations with various altitudes, SeaDist, and
climates to illustrate the diversity of diurnal IWV cycles in Europe as
shown in Fig. 8. The climate zones of the GPS stations are classified
according to the Köppen climate classification system (Beck et al., 2018), and the
properties of the stations are listed in Table S2.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><?xmltex \def\figurename{Figure}?><label>Figure 8</label><caption><p id="d1e3292">Diurnal IWV cycles at selected six stations obtained from
1-hourly GPS (green dots) and ERA5 (red squares). The stations are selected
with the consideration of different altitudes, distance to sea (SeaDist),
and climate zones classified according to the Köppen climate classification system (Beck et al., 2018). The data points are fitted with diurnal (<inline-formula><mml:math id="M177" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) and semidiurnal (<inline-formula><mml:math id="M178" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) harmonics (dashed blue curve for GPS and orange curve for ERA5). The amplitudes and phases of the <inline-formula><mml:math id="M179" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M180" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> harmonics are also given. The phases are shown as the local solar time (LST) at the peak of associated harmonics. For instance, the <inline-formula><mml:math id="M181" display="inline"><mml:mrow><mml:msub><mml:mi>D</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> amplitude and phase of GPS IWV at station NICO are 1.2 kg m<inline-formula><mml:math id="M182" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and 15.8 LST, respectively. By comparison, the values of its ERA5 IWV are 0.8 kg m<inline-formula><mml:math id="M183" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and 15.2 LST, respectively. The
vertical dotted black lines at 09:00 and 12:00 UTC indicate the time of possible mismatches in the ERA5 IWV cycle.</p></caption>
          <?xmltex \igopts{width=384.112205pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f08.png"/>

        </fig>

      <p id="d1e3381">Station NICO is located in Cyprus with hot semi-arid climate (BSh).
Despite being only 21.5 km away from the coastline, NICO has the largest diurnal
IWV amplitude with a value of 1.2 kg m<inline-formula><mml:math id="M184" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, equivalent to a relative
amplitude of 6.7 %. This is mainly due to the large diurnal temperature
range in Cyprus, especially in summer (Price et al., 1999).</p>
      <p id="d1e3397">Both the MedCoast station VALE (Valencia, Spain; 39.48<inline-formula><mml:math id="M185" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 0.34<inline-formula><mml:math id="M186" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> W; 27.0 m) and the OtherCoast station NEWL (Newlyn, UK; 50.10<inline-formula><mml:math id="M187" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 5.54<inline-formula><mml:math id="M188" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> W; 11.0 m) are very close to the coastline, with SeaDist values of 1.2 and 0.5 km, respectively. However, their diurnal
amplitudes are quite different (absolutely 0.8 kg m<inline-formula><mml:math id="M189" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> versus 0.1 kg m<inline-formula><mml:math id="M190" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, relatively 3.9 % versus 0.7 %). As explained earlier for the difference between the two station types, their weather conditions are different. VALE is located at the Mediterranean Coast with cold semi-arid (BSk) climate. Its strong diurnal cycle, especially in summer with an amplitude of 1.4 kg m<inline-formula><mml:math id="M191" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (4.6 %), is attributed to intense solar heating under minimal-cloud-coverage weather conditions. In contrast, NEWL is located at the coast of the English Channel with temperate oceanic (Cfb) climate, and its smaller diurnal amplitude can be due to the weaker solar heating effect under unstable and cloudy weather conditions, in addition to the land–sea breeze effect on mitigating diurnal temperature range.</p>
      <p id="d1e3473">Station ZECK is in the Greater Caucasus with humid continental (Dfb)
climate. Its diurnal amplitude is much stronger than PENC's (Penc, Hungary;
47.79<inline-formula><mml:math id="M192" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 19.28<inline-formula><mml:math id="M193" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E; 248.3 m) with the same climate
(1.0 kg m<inline-formula><mml:math id="M194" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and 7.9 % versus 0.2 kg m<inline-formula><mml:math id="M195" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and 1.5 %). As ZECK is much higher than PENC, their difference in amplitude is consistent with the
pattern for most Inland stations, which can be explained by the effect of
orographic circulation (Diedrich et al., 2016). In addition, KIR0 (Kiruna,
Sweden; 67.88<inline-formula><mml:math id="M196" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 21.06<inline-formula><mml:math id="M197" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E; 469.3 m) is typical for
many stations in northern Europe. Although its diurnal cycle is quite weak with
an amplitude of only 0.1 kg m<inline-formula><mml:math id="M198" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (1.7 %), it is well fitted by the
sinusoidal harmonic curve fitting.</p>
</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Mismatches in diurnal ERA5 IWV cycle</title>
      <p id="d1e3558">Only the diurnal IWV cycle from the 1-hourly ERA5 time series was evaluated
with respect to GPS, as the temporal resolutions of the other reanalyses are
too coarse to characterise the diurnal cycle. However, we found significant
shifts in the diurnal IWV anomalies between 09:00 and 10:00 (10:00–09:00) UTC as well as
between 21:00 and 22:00 (22:00–21:00) UTC at part of the stations, such as NEWL and PENC displayed in Fig. 8. The ERA5 developers have noticed such mismatches in the
diurnal cycles of individual meteorological variables, such as its near-surface wind, temperature, and humidity products (see Known Issues 8 and 9
in <uri>https://confluence.ecmwf.int/display/CKB/ERA5:+data+documentation#ERA5:datadocumentation-Knownissues</uri>,<?pagebreak page3526?> last access: 8 January 2023),
and the problem is attributed to the edge effect in each ERA5 assimilation
cycle (from 10:00 to 21:00 UTC and from 22:00 to 09:00 UTC<inline-formula><mml:math id="M199" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1 d). However, according to our knowledge, the magnitude of the mismatch in the diurnal cycle of ERA5 IWV and its spatiotemporal characterisations have not been investigated yet. Therefore, we will quantify and analyse the mismatch in the ERA5 IWV over Europe in this section.</p>
      <p id="d1e3571">Figure 9 compares the diurnal IWV cycle of ERA5 and GPS for each season at
station PENC. From this figure, we can derive that there are no mismatches
in the diurnal GPS IWV cycle, although the GPS IWV (slightly) relies on
<inline-formula><mml:math id="M200" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (hence humidity and temperature) from ERA5 for the ZTD to IWV
conversion, as shown in Eq. (2). GPS IWV estimates are therefore regarded as
reference data to evaluate the mismatches in the diurnal cycle of ERA5 IWV.
At station PENC, the mismatches in ERA5 are seasonal dependent, which are
strongest in summer (JJA) but weakest in winter (DJF).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9" specific-use="star"><?xmltex \currentcnt{9}?><?xmltex \def\figurename{Figure}?><label>Figure 9</label><caption><p id="d1e3587">Similar to Fig. 8 but for the seasonal-averaged and all-time-averaged diurnal IWV cycles at station PENC. The green and red numbers are the IWV shifts from ERA5 and GPS, respectively. The numbers on the left and right are the IWV shifts from 09:00  to 10:00 UTC and from 21:00 to 22:00 UTC,
respectively.</p></caption>
          <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f09.png"/>

        </fig>

      <p id="d1e3597">Figure 10 compares the shifts at 10:00–09:00 UTC and 22:00–21:00 UTC from ERA5 and GPS at all the stations, respectively. The shifts in the GPS IWV cycle are regarded as reference, representing the natural IWV changes at the two epochs. As can be seen from Fig. 10a–e and k–o, the ERA5 IWV series generally drop from 09:00 to 10:00 UTC and then jump from 21:00 to 22:00 UTC. The ERA5 artificial shifts at the two epochs are most significant in summer, with average values of <inline-formula><mml:math id="M201" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.23</mml:mn></mml:mrow></mml:math></inline-formula> and 0.35 kg m<inline-formula><mml:math id="M202" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. In contrast, the
average natural shifts in summer estimated from GPS IWV are only 0.11 and
<inline-formula><mml:math id="M203" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula> kg m<inline-formula><mml:math id="M204" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Moreover, the all-time-averaged natural
shifts in GPS IWV are only 0.05 and <inline-formula><mml:math id="M205" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula> kg m<inline-formula><mml:math id="M206" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.
However, the artificial shifts in ERA5 IWV are <inline-formula><mml:math id="M207" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula> and 0.19. As can be seen from the geographic distributions of the shifts shown in Fig. 10e and o, the ERA5 shifts at 10:00–09:00 UTC are most significant at the Alps and in Eastern Europe, whereas the shifts at 22:00–21:00 UTC are more widespread in central Europe. The reasons for their geographical patterns are unknown and needs further investigation. Since the average diurnal amplitude of the reference GPS IWV is only 0.32 kg m<inline-formula><mml:math id="M208" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, the artificial shifts in ERA5 IWV cannot be ignored when analysing the diurnal IWV cycle in these regions.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F10" specific-use="star"><?xmltex \currentcnt{10}?><?xmltex \def\figurename{Figure}?><label>Figure 10</label><caption><p id="d1e3691">Seasonal-averaged and all-time-averaged IWV shifts in the GPS and
ERA5 diurnal cycles from 09:00 to 10:00 UTC and from 21:00 to 22:00 UTC.</p></caption>
          <?xmltex \igopts{width=441.017717pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f10.png"/>

        </fig>

</sec>
<?pagebreak page3528?><sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Diurnal anomalies</title>
      <p id="d1e3708">Diurnal anomaly represents high-frequency variations of IWV associated with
weather phenomena like heavy rainfall. Therefore, evaluations of the
consistencies between the IWV diurnal anomalies from reanalyses with respect
to GPS are conducive to a better understanding of their performances in
extreme weather, especially for ERA5 with a significantly enhanced temporal
resolution of 1 h.</p>
      <p id="d1e3711">We first evaluated all the reanalyses with respect to GPS at 1 h temporal
resolution. For the reanalyses with coarser resolutions (3 and 6 h),
we interpolated their time series to 1 h by using cubic spline, which is
slightly superior to linear interpolation. Statistics of the evaluation
results are listed in Table 2. At the temporal resolution of 1 h, ERA5
scores the highest average <inline-formula><mml:math id="M209" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M210" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula>, and KGE with values of 0.98,
0.89, and 0.88, respectively. The results indicate that the 1-hourly ERA5
diurnal anomalies have the best agreement with GPS in variability and
correlation. However, NCEP-2 performs the worst, as it scores the lowest
<inline-formula><mml:math id="M211" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M212" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula>, and KGE with values of 0.75, 0.69, and 0.60, respectively.
To be comparable to many other studies, we also evaluated the consistencies
by using the more commonly used indicator – rms of IWV difference
(<inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:msub><mml:mtext>rms</mml:mtext><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) as shown in Eq. (12). Results show that ERA5 and NCEP-2 score the lowest and largest average <inline-formula><mml:math id="M214" display="inline"><mml:mrow><mml:msub><mml:mtext>rms</mml:mtext><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
values of 0.97 and 1.57 kg m<inline-formula><mml:math id="M215" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, respectively. Therefore, we drew the
same conclusion as from the KGE scores. The evaluations confirm the
superiority of the 1-hourly ERA5 over the other reanalyses, most likely
because of its enhanced spatiotemporal resolutions and other improvements in
data assimilation.</p>

<?xmltex \floatpos{p}?><table-wrap id="Ch1.T2" specific-use="star"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e3780">Statistics of the consistencies in diurnal IWV anomalies
from reanalyses compared to GPS.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="8">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="center"/>
     <oasis:colspec colnum="3" colname="col3" align="center"/>
     <oasis:colspec colnum="4" colname="col4" align="center"/>
     <oasis:colspec colnum="5" colname="col5" align="center"/>
     <oasis:colspec colnum="6" colname="col6" align="center"/>
     <oasis:colspec colnum="7" colname="col7" align="center"/>
     <oasis:colspec colnum="8" colname="col8" align="center"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Temporal</oasis:entry>
         <oasis:entry colname="col3">CFSR</oasis:entry>
         <oasis:entry colname="col4">ERA5</oasis:entry>
         <oasis:entry colname="col5">ERAI</oasis:entry>
         <oasis:entry colname="col6">JRA-55</oasis:entry>
         <oasis:entry colname="col7">MERRA-2</oasis:entry>
         <oasis:entry colname="col8">NCEP-2</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">resolution</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M216" display="inline"><mml:mi mathvariant="italic">γ</mml:mi></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">1 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M217" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.98</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M218" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.98</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.03</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M219" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.91</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M220" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.86</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M221" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.02</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M222" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.75</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">3 h</oasis:entry>
         <oasis:entry colname="col3">–</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M223" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.97</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.03</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">–</oasis:entry>
         <oasis:entry colname="col6">–</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M224" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.02</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">6 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M225" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.99</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.03</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M226" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.96</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.03</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M227" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.92</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M228" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.87</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">–</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M229" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.76</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.0</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M230" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">1 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M231" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.85</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M232" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.89</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M233" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.85</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M234" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.83</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M235" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.86</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M236" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.69</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">3 h</oasis:entry>
         <oasis:entry colname="col3">–</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M237" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.89</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">–</oasis:entry>
         <oasis:entry colname="col6">–</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M238" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.86</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">6 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.87</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M240" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.90</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M241" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.86</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.07</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.84</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.07</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">–</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.69</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">KGE</oasis:entry>
         <oasis:entry colname="col2">1 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M244" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.85</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M245" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.88</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M246" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.82</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.07</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M247" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.78</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.07</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M248" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.85</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M249" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.60</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.09</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">3 h</oasis:entry>
         <oasis:entry colname="col3">–</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M250" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.89</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">–</oasis:entry>
         <oasis:entry colname="col6">–</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M251" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.86</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">6 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M252" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.86</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M253" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.89</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M254" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.83</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.07</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M255" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.79</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.07</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">–</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M256" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.60</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">rms<inline-formula><mml:math id="M257" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">1 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M258" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.14</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.19</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M259" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.97</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.21</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M260" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.14</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.22</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M261" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.20</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.21</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M262" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.14</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.22</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M263" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.57</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.24</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">(kg m<inline-formula><mml:math id="M264" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">3 h</oasis:entry>
         <oasis:entry colname="col3">–</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M265" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.97</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.21</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">–</oasis:entry>
         <oasis:entry colname="col6">–</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M266" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.15</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.22</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">6 h</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.09</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.21</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M268" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.94</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.21</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M269" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.09</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.24</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M270" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.16</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.22</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">–</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M271" display="inline"><mml:mrow><mml:mn mathvariant="normal">1.59</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.24</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d1e4741">For a fairer intercomparison, we also evaluated ERA5 and the other
reanalyses at their respective native resolutions. Accordingly, we extracted
the ERA5 IWV every 3 and 6 h. The comparison with MERRA-2 at its native
resolution of 3 h shows that ERA5 achieves larger KGE (0.89 versus 0.86)
and smaller <inline-formula><mml:math id="M272" display="inline"><mml:mrow><mml:msub><mml:mtext>rms</mml:mtext><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (0.97 kg m<inline-formula><mml:math id="M273" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> versus 1.15 kg m<inline-formula><mml:math id="M274" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Moreover, the average KGE value of the 6-hourly ERA5 IWV is 0.89, which is higher than those of CFSR, ERAI, JRA-55, and NCEP-2, with values of 0.86, 0.83, 0.79, and 0.60, respectively. The results indicate that ERA5 is still superior to the other reanalyses at the coarser temporal resolutions.</p>
</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Assessments of annual cycle</title>
      <p id="d1e4789">We analysed the annual cycles of the homogenised monthly GPS IWV time series
as shown in Fig. 11a with increasing latitude from the bottom to the top. Most of the
annual IWV cycles reach their maxima in July and August, with peak values
from 17.1 to 32.2 kg m<inline-formula><mml:math id="M275" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. In contrast, the minima of the annual cycles
are typically in January and February, with values from 4.2 to 17.1 kg m<inline-formula><mml:math id="M276" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The maximum and minimum values of the annual cycles are generally increasing with decreasing latitude (Fig. 10a) and decreasing altitude (not shown).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11" specific-use="star"><?xmltex \currentcnt{11}?><?xmltex \def\figurename{Figure}?><label>Figure 11</label><caption><p id="d1e4818"><bold>(a)</bold> Monthly annual cycle of GPS IWV in kilogram per square metre for
the 108 GPS stations with increasing latitude from the bottom to the top. <bold>(b–g)</bold> The differences between the annual cycles of the various reanalyses compared to the GPS.</p></caption>
        <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f11.png"/>

      </fig>

      <p id="d1e4832">Figure 11b–g present the differences between the annual cycle of IWV
estimated by the reanalyses with respect to GPS. It can be seen that ERA5
has the least differences. Indeed, the quantitative evaluation shows that
ERA5 obtains the highest median KGE score having a value of 0.97 (Fig. 5h),
indicating that it outperforms the other reanalyses. CFSR ranks last (median
KGE <inline-formula><mml:math id="M277" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.94</mml:mn></mml:mrow></mml:math></inline-formula>) due to its overestimation of mean values (median <inline-formula><mml:math id="M278" display="inline"><mml:mrow><mml:mi mathvariant="italic">β</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1.04</mml:mn></mml:mrow></mml:math></inline-formula>) and underestimation of variability (median <inline-formula><mml:math id="M279" display="inline"><mml:mrow><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.96</mml:mn></mml:mrow></mml:math></inline-formula>).
Moreover, although the consistencies between the annual IWV signals from
reanalyses and GPS are generally rather good, there could be significant
discrepancies in specific seasons and regions. For example, JRA-55 has an
average dry bias of 0.5 kg m<inline-formula><mml:math id="M280" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> with respect to the GPS IWV from May to
September at the stations in the south (32–48<inline-formula><mml:math id="M281" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N;
Fig. 11e), whereas NCEP has obvious wet biases (0.7–2.4 kg m<inline-formula><mml:math id="M282" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) in
the annual average of IWV with respect to the GPS results at low latitudes
(32–40<inline-formula><mml:math id="M283" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N; Fig. 11g). In addition, significant biases (1.2–5.9 kg m<inline-formula><mml:math id="M284" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) from March to September can be seen at station BZRG in the evaluations of CFSR, ERAI, and MERRA-2. The discrepancies are most likely related to the remarkable representativeness differences between the reanalyses and GPS at BZRG (Fig. 3), which is located in the Alps.</p>
</sec>
<sec id="Ch1.S6">
  <label>6</label><title>Assessments of linear trends</title>
      <?pagebreak page3530?><p id="d1e4932">We carried out a homogenisation of the GPS IWV time series by using the
RHtestsV4 software (Wang and Feng, 2013) before the analysis. The software
is dedicated to the homogenisation of climatic time series. In addition, we
adopted a homogenisation strategy which allows for changepoints with and
without support from metadata. We took all six reanalyses as references
and attempted to avoid the impacts of possible changepoints in specific
reanalyses. However, we did not homogenise the reanalyses IWV time series
because they represent the native quality of the reanalyses that we would
like to assess. The homogenisation approach is detailed in Appendix A.</p>
      <p id="d1e4935">We then estimated the linear IWV trends from all six reanalyses and the
homogenised GPS IWV time series after the removal of the annual cycle. In order
to obtain realistic uncertainties of the trend estimates, we analysed the
time series by using Hector software version 1.7.2 (Bos et al., 2012). We
tested four commonly used noise models, namely white noise (WN), first-order
autoregressive (AR(1)), autoregressive moving average (ARMA(1,1)), and power-law
noise (PL). We then selected the optimal model of each time series by using the
Bayesian information criterion (BIC; Schwarz, 1978). Readers are referred to
Yuan et al. (2021) for more details. The IWV trend estimates, associated
uncertainties, and specific optimal noise models are listed in Table S3.</p>
      <p id="d1e4938">Figure 12a shows the GPS IWV trends after the homogenisation. The IWV trends
generally increase from the Atlantic coasts towards the southeast. The average
trends of the OtherCoast, Inland, and MedCoast stations are 0.2, 0.5, and
0.9 kg m<inline-formula><mml:math id="M285" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade, respectively. The corresponding relative IWV
trends are 1.7 %, 3.1 %, and 5.0 % per decade (Fig. 12d),
respectively. The largest trend is found at station TUBI (Gebze, Turkey; 40.8<inline-formula><mml:math id="M286" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 29.5<inline-formula><mml:math id="M287" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) with a value of 1.6 kg m<inline-formula><mml:math id="M288" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade (8.7 % per decade). As can be seen from Fig. 12b, AR(1) is
the optimal noise model at 58 % of the stations (63 out of 108), which are mostly located close to sea or in northern Europe. Most parts of central
Europe are characterised by WN, whereas Belgium and central Germany are best
modelled by ARMA(1,1). In addition, PL is superior to the other models at four
stations. The optimal noise models for the monthly IWV time series of the
six reanalyses show similar geographical patterns as the GPS IWV. The
geographical patterns of the optimal noise models obtained in this study are
different from Yuan et al. (2021), although the geographical patterns of the
IWV trends are consistent to previous studies (Parracho et al., 2018; Nguyen
et al., 2021; Yuan et al., 2021). It is most likely due to the difference
that monthly IWV time series are used here, whereas daily IWV series were
used in their work.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F12" specific-use="star"><?xmltex \currentcnt{12}?><?xmltex \def\figurename{Figure}?><label>Figure 12</label><caption><p id="d1e4986"><bold>(a)</bold> Map of the absolute trends of the homogenised monthly GPS IWV anomaly time series. The squares and circles indicate the trend estimates being significant and insignificant at 95 % confidence level, respectively. The trend uncertainties are estimated based on optimal noise models <bold>(b)</bold>. The relative trends <bold>(d)</bold> are calculated as the absolute trends <bold>(a)</bold> divided by the associated average IWV <bold>(c)</bold>.</p></caption>
        <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f12.png"/>

      </fig>

      <p id="d1e5009">We evaluated the IWV trends derived from the six reanalyses by taking the
trends from the homogenised GPS IWV time series as reference. We compared
the difference in the relative IWV trend rather than the absolute trend because
the relative trend is not affected by the IWV bias in individual reanalysis.
As can be seen in Fig. 13, ERA5 shows the best agreement in IWV trends with
respect to GPS, with a mean value and a standard deviation of 0.01 % per
decade and 0.97 % per decade in their trend differences, respectively, indicating an improvement compared to its predecessor ERAI (<inline-formula><mml:math id="M289" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.04</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">1.15</mml:mn></mml:mrow></mml:math></inline-formula> % per decade). JRA-55 also only has an average trend difference of as low as 0.01 % per decade but with a slightly larger
standard deviation (1.12 % per decade) than ERA5. Compared to the GPS
IWV trends, MERRA-2 has an underestimation of 0.22 % per decade on
average (Fig. 13e), whereas CFSR resulted in an overestimation of 0.22 % per decade (Fig. 13a). The standard deviation of the CFSR GPS IWV trend
differences is as large as 1.73 % per decade, which is mainly caused by the significant differences from <inline-formula><mml:math id="M290" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">5.1</mml:mn></mml:mrow></mml:math></inline-formula> % per decade to 4.9 % per
decade in southern Europe (Fig. 13a). The results suggest that the CFSR
IWV trends are less accurate in southern Europe and should be carefully
validated before climate change analysis.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F13" specific-use="star"><?xmltex \currentcnt{13}?><?xmltex \def\figurename{Figure}?><label>Figure 13</label><caption><p id="d1e5038">Comparison of the relative IWV trend differences (percent per decade) for various reanalyses with respect to GPS. The numbers in each subplot indicate the mean value and standard deviation of the associated relative IWV trend differences.</p></caption>
        <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f13.png"/>

      </fig>

      <?pagebreak page3532?><p id="d1e5047">In addition, Fig. 13f shows that the mean value and standard deviation of
NCEP-2 GPS IWV trend differences are 1.61 % per decade and 1.86 % per decade, respectively, indicating a general overestimation of IWV trends from NCEP-2 with respect to GPS. In particular, the average NCEP-2 GPS
IWV trend differences is as large as 2.9 % per decade at 31 stations
located in southern Europe (32<inline-formula><mml:math id="M291" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N <inline-formula><mml:math id="M292" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> lat <inline-formula><mml:math id="M293" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 46<inline-formula><mml:math id="M294" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 10<inline-formula><mml:math id="M295" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> W <inline-formula><mml:math id="M296" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> long <inline-formula><mml:math id="M297" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 25<inline-formula><mml:math id="M298" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E). However, NCEP-2 underestimates the trends  at two stations in the eastern Mediterranean, with an average difference of <inline-formula><mml:math id="M299" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3.1</mml:mn></mml:mrow></mml:math></inline-formula> % per decade compared to GPS IWV. Therefore, we concluded that the NCEP-2 IWV trends are not qualified for climate change analysis in Europe.</p>
</sec>
<sec id="Ch1.S7" sec-type="conclusions">
  <label>7</label><title>Conclusions</title>
      <p id="d1e5133">In this study, integrated water vapour (IWV) time series for the period 1994–2018 were retrieved from continuous GPS observations at 108
ground-based GPS stations in Europe, with an average period of 21 years for
those time series. The temporal features of Europe's IWV, such as its
diurnal cycle and variation, annual cycle, and linear trend, were then
investigated. Moreover, the performances of six frequently used global
atmospheric reanalyses in Europe were assessed for the first time, namely
CFSR, ERA5, ERA-Interim (ERAI), JRA-55, MERRA-2, and NCEP-2. The main findings
are summarised below:
<list list-type="custom"><list-item><label>i.</label>
      <p id="d1e5138">The agreement between the daily GPS IWV time series and the six reanalyses is found to be the best for ERA5 and the worst for NCEP-2, with standard deviations of IWV differences of 0.5–1.6 and 1.1–3.0 kg m<inline-formula><mml:math id="M300" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, respectively. The standard deviations of IWV differences are well correlated with representativeness statistics of the six reanalyses, indicating that the representativeness differences contribute to the discrepancies between the reanalyses and GPS.</p></list-item><list-item><label>ii.</label>
      <p id="d1e5154">The diurnal amplitudes are 0–1.2 kg m<inline-formula><mml:math id="M301" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, accounting for 0 %–8 % of the associated daily mean IWV. The semidiurnal amplitudes are weaker, with values lower than 30 % of the diurnal amplitudes at 88 % of the stations. The peaks of the diurnal and semidiurnal harmonics are within 15:00–21:00 and 01:00–06:00 LST at 90 % of the stations, respectively. The diurnal amplitudes are larger at the Mediterranean Coast (1.1 %–4.2 %), which is most likely because of a stronger solar heating effect. In comparison, the diurnal amplitudes at other coastal regions in Europe are lower (0.3 %–1.9 %), which can be due to a land–sea breeze and a weaker solar heating effect. In addition, the relative diurnal and semidiurnal IWV amplitudes are correlated with altitudes with correlation coefficients of 0.66 and 0.67, respectively, which can be related to orographic circulation.</p></list-item><list-item><label>iii.</label>
      <p id="d1e5170">Mismatches in the diurnal cycle of the ERA5 IWV product were found and evaluated between 09:00 and 10:00 UTC as well as between 21:00 and 22:00 UTC. The problem can be attributed to the edge effect in each ERA5 assimilation cycle, and it has been noticed in some other meteorological variables provided by ERA5. The average artificial shifts in ERA5 IWV are <inline-formula><mml:math id="M302" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.08</mml:mn></mml:mrow></mml:math></inline-formula> and 0.19 kg m<inline-formula><mml:math id="M303" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> at the two epochs. In contrast, the natural shifts in GPS IWV are 0.05 and <inline-formula><mml:math id="M304" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.05</mml:mn></mml:mrow></mml:math></inline-formula> kg m<inline-formula><mml:math id="M305" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The ERA5 shifts are dependent on seasons and locations. The ERA5 shifts are more significant in summer than in winter. Moreover, the ERA5 shifts from 09:00 to 10:00 UTC are most significant at the Alps and Eastern Europe, whereas the shifts from 21:00 to 22:00 UTC are more widespread in central Europe. As the average diurnal IWV amplitude obtained from GPS is only 0.32 kg m<inline-formula><mml:math id="M306" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, the artificial shifts in ERA5 IWV cannot be ignored in the diurnal IWV cycle analysis in these regions.</p></list-item><list-item><label>iv.</label>
      <p id="d1e5230">Regarding diurnal IWV anomalies, ERA5 shows the best consistency with GPS at a temporal resolution of 1 h, with an average rms of the IWV difference (<inline-formula><mml:math id="M307" display="inline"><mml:mrow><mml:msub><mml:mtext>rms</mml:mtext><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) of 0.97 kg m<inline-formula><mml:math id="M308" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, whereas the average <inline-formula><mml:math id="M309" display="inline"><mml:mrow><mml:msub><mml:mtext>rms</mml:mtext><mml:mi mathvariant="normal">Δ</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is 1.14–1.57 kg m<inline-formula><mml:math id="M310" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the other five reanalyses. ERA5 also outperforms the other reanalyses at their respective resolutions (3 and 6 h), indicating the benefits of its enhanced spatial resolutions and other improvements in data assimilation, in addition to its higher temporal resolution.</p></list-item><list-item><label>v.</label>
      <p id="d1e5280">All the monthly IWV time series are modulated with apparent annual cycles, with minima in January and February (4–17 kg m<inline-formula><mml:math id="M311" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and maxima in July and August (17–32 kg m<inline-formula><mml:math id="M312" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). The maxima and minima of the annual cycles show consistent geographical patterns, with larger values towards the Equator and at lower-altitude sites. ERA5 ranks first in modelling the annual cycles of IWV (median KGE <inline-formula><mml:math id="M313" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.97</mml:mn></mml:mrow></mml:math></inline-formula>) with respect to GPS IWV; CFSR ranks last (median KGE <inline-formula><mml:math id="M314" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.94</mml:mn></mml:mrow></mml:math></inline-formula>) due to its overestimation of mean values (median <inline-formula><mml:math id="M315" display="inline"><mml:mrow><mml:mi mathvariant="italic">β</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1.04</mml:mn></mml:mrow></mml:math></inline-formula>) and underestimation of variability (median <inline-formula><mml:math id="M316" display="inline"><mml:mrow><mml:mi mathvariant="italic">γ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.96</mml:mn></mml:mrow></mml:math></inline-formula>).</p></list-item><list-item><label>vi.</label>
      <p id="d1e5353">Europe's IWV is increasing as observed from more than 2 decades of continuous GPS observations. The trends generally increase from the Atlantic Coast towards the southeast. The average trends of the Atlantic coasts, inland Europe, and Mediterranean coasts are 0.2, 0.5, and 0.9 kg m<inline-formula><mml:math id="M317" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade, which are equivalent to relative values of 1.7 % per decade, 3.1 % per decade, and 5.0 % per decade, respectively. The monthly IWV time series are best modelled by first-order autoregressive (AR(1)) noise at most stations located close to the sea and northern Europe, whereas autoregressive moving average (ARMA(1,1)), white noise (WN), and ARMA(1,1) models are preferred at the rest of the stations. Power-law noise (PL) is found to be optimal at only four stations. As for the performances of the reanalyses in reproducing IWV trends, ERA5 achieves the best consistency with GPS IWV trends, with a mean value and a standard deviation of 0.01 % per decade and 0.97 % per decade in their trend differences, respectively. However, CFSR is not qualified for the analysis of IWV trends in southern Europe due to its significant discrepancies with respect to GPS. The NCEP-2 IWV trends over the<?pagebreak page3533?> whole of Europe are also not recommend for the same reason.</p></list-item></list></p>
      <p id="d1e5368">Overall, it can be concluded that the reanalyses successfully reproduce the
spatiotemporal IWV variability over Europe, as assessed by using the GPS IWV
dataset, with ERA5 slightly outperforming the other reanalyses at most
temporal scales. It is noteworthy that the pressure and weighted mean
temperature obtained from ERA5 were used in the conversion of GPS ZTD to IWV
due to a lack of long-term accurate and complete in situ  meteorological observations at the GPS stations. This could partly contribute to the superior agreement between the IWV from ERA5 and GPS. Future studies could validate the IWV products of reanalyses using ground-based GPS when independent, quality-assured, and complete meteorological observations at the GPS stations are available. IWV measurements from other techniques could also be helpful.</p>
</sec>

      
      </body>
    <back><app-group>

<app id="App1.Ch1.S1">
  <?xmltex \currentcnt{A}?><label>Appendix A</label><title>Homogenisation of GNSS IWV time series</title>
      <p id="d1e5382">Long-term IWV time series often suffer from inhomogeneities due to changes
in instrumentation, data processing methods, and local environmental
conditions (Van Malderen et al., 2020; Nguyen et al., 2021, and references
therein). These inhomogeneities can manifest themselves as changes in the
mean of the time series (“biases”) at specific epochs, i.e. breaks or
changepoints. If such changepoints are not properly corrected, they can
significantly modify the estimations of long-term linear trends and
multi-temporal-scale variabilities (e.g. Ning et al., 2016; Van Malderen et
al., 2020; Yuan et al., 2021). Therefore, the homogenisation of the IWV time
series is essential for a sound understanding and proper interpretation of
IWV variability under climate change.</p>
      <p id="d1e5385">In this work, we examined the homogeneity of the monthly GPS IWV time series
by using the RHtestsV4 software (Wang and Feng, 2013). This software is
developed especially for the detection and adjustment of changepoints in
climatic time series, and it has been used in the homogenisation of IWV time
series in previous studies (Ning et al., 2016; Schröder et al., 2016;
Van Malderen et al., 2020). The software is based on a penalised maximal <italic>t</italic>
test with the consideration of linear trend, annual cycle, and AR(1) noise
in the time series (Wang et al., 2007; Wang 2008).</p>
      <p id="d1e5391">We took all six reanalyses as references for the homogenisation of the
GNSS IWV time series, meaning that we inspected the monthly IWV difference
time series between the GNSS and each of the reanalysis IWV. It is
noteworthy that the reanalyses may also contain changepoints (e.g. Ning et
al., 2016; Schröder et al., 2016). However, we did not homogenise the
reanalyses IWV time series because they represent the native quality of the
reanalyses that we would like to assess in this work. Also, by taking all
six reanalyses as references, we are confident that we can minimise the impact of
inhomogeneities in either reanalysis of the homogenisation process of the
GNSS IWV time series. Practically, we used the following strategy to avoid
the impacts of changepoints in specific reanalyses on the homogenisation of
the GPS IWV time series:
<list list-type="order"><list-item>
      <p id="d1e5396">We examined the GPS IWV and metadata (station log file and IGSMAIL) carefully. If there was an instrumentation change within the first (or the last) year, we removed the several months before (or after) the epoch of change. Moreover, we also inspected the station up-coordinate time series and excluded periods with quality problems, as it is well known that they are strongly correlated with the GPS tropospheric delay estimates (Tregoning and Herring, 2006). An example is given in Fig. A1 and will be described later in this Appendix.</p></list-item><list-item>
      <p id="d1e5400">We used the <italic>FindU.wRef</italic> command of the RHtestsV4 software to identify all possible changepoints in each GPS-reanalysis IWV monthly mean difference time series, which can be significant at a confidence level of 99 %, no matter if they are documented in metadata or not.</p></list-item><list-item>
      <p id="d1e5407">If a changepoint was within 3 months before or after a documented change in instrumentation, we adjusted its epoch according to the metadata and set it as Type 0. The rest of the changepoints were set as Type 1.</p></list-item><list-item>
      <p id="d1e5411">If identical Type-1 changepoints were reported within 6 months in at least four GPS-reanalysis IWV differences, but not supported by metadata, we recognised them as a single Type-1 changepoint at the median of the epochs.</p></list-item><list-item>
      <p id="d1e5415">We estimated the amplitudes of the Type-0 and Type-1 changepoints and tested their amplitude significances at a confidence level of 99 % with the <italic>StepSize.wRef</italic> command of the RHtestsV4 software.</p></list-item><list-item>
      <p id="d1e5422">We calculated the amplitude of each changepoint as the average of all the significant amplitude estimates from the six GPS-reanalysis IWV differences.</p></list-item><list-item>
      <p id="d1e5426">We removed a changepoint if its amplitude was only significant in less than four GPS-reanalysis comparisons or if its amplitude was less than 3 times its standard deviation. Then, we repeated the steps of (5) and (6) until the rest of the changepoints were significant.</p></list-item></list></p>
      <p id="d1e5429">The changepoint identification is finished after one or two iterations for
most stations. In the end, we identified 44 Type-0 and 9 Type-1 changepoints
as listed in Table A1. The total number of 53 changepoints is consistent with
a previous global GPS IWV homogenisation study carried out by Ning et al. (2016), which identified 45 changepoints in total at 101 stations.</p><?xmltex \hack{\clearpage}?><?xmltex \floatpos{h!}?><fig id="App1.Ch1.S1.F14"><?xmltex \currentcnt{A1}?><?xmltex \def\figurename{Figure}?><label>Figure A1</label><caption><p id="d1e5435">Monthly GPS-reanalysis IWV difference <bold>(a–f)</bold>, monthly GPS IWV <bold>(g)</bold>, and daily up-coordinate time series at station HERS. The GPS data before 3 September 2001 were deleted due to a problem in station antenna (see IGSMAIL-3503). The IWV time series before and after the homogenisation are labelled as blue dots and red crosses in panels <bold>(a)</bold>–<bold>(g)</bold>. The types of instrumentation changes are listed in Table A2. The Type-0 changepoint on 19 August 2010 is significant at a confidence level of 99 % (green downward-pointing triangle), and its value was calculated as the average of the values estimated in each GPS-reanalysis comparison as shown in panels <bold>(a)</bold>–<bold>(f)</bold>.</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f14.png"/>

      </fig>

<?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T3" specific-use="star"><?xmltex \currentcnt{A1}?><label>Table A1</label><caption><p id="d1e5468">The identified changepoints in GPS IWV time series. The Type 0 and Type 1 are changepoints with and without changes in
instrumentation as documented in GPS station log files, respectively. The
full names of the Type-0 changepoint events are shown in Table A2, and the
Type-1 changepoints are labelled as Unknown. G-C, G-E, G-I, G-J, G-M,
and G-N indicate the GPS IWV changepoints in kilogram per square metre estimated by
comparing it to  CFSR, ERA5, ERAI, JRA-55, MERRA-2, and NCEP-2, respectively. The
NaN indicates that the changepoint in the specific GPS-reanalysis comparison
is insignificant at a confidence level of 99 %. The mean and SD are the
mean value and standard deviation of each changepoint.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.80}[.80]?><oasis:tgroup cols="12">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="center"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="center"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:colspec colnum="9" colname="col9" align="right"/>
     <oasis:colspec colnum="10" colname="col10" align="right"/>
     <oasis:colspec colnum="11" colname="col11" align="right"/>
     <oasis:colspec colnum="12" colname="col12" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Station</oasis:entry>
         <oasis:entry colname="col2">Type</oasis:entry>
         <oasis:entry colname="col3">Date</oasis:entry>
         <oasis:entry colname="col4">Mean</oasis:entry>
         <oasis:entry colname="col5">SD</oasis:entry>
         <oasis:entry colname="col6">G-C</oasis:entry>
         <oasis:entry colname="col7">G-E</oasis:entry>
         <oasis:entry colname="col8">G-I</oasis:entry>
         <oasis:entry colname="col9">G-J</oasis:entry>
         <oasis:entry colname="col10">G-M</oasis:entry>
         <oasis:entry colname="col11">G-N</oasis:entry>
         <oasis:entry colname="col12">Events</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">APEL</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 September 2006</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M318" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.31</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.10</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M319" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.26</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M320" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M321" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.32</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M322" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.22</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M323" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.26</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M324" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.50</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">APEL</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">19 June 2013</oasis:entry>
         <oasis:entry colname="col4">0.36</oasis:entry>
         <oasis:entry colname="col5">0.10</oasis:entry>
         <oasis:entry colname="col6">0.36</oasis:entry>
         <oasis:entry colname="col7">0.32</oasis:entry>
         <oasis:entry colname="col8">0.40</oasis:entry>
         <oasis:entry colname="col9">0.44</oasis:entry>
         <oasis:entry colname="col10">0.47</oasis:entry>
         <oasis:entry colname="col11">0.20</oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">APEL</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 April 2016</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M325" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.33</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.04</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M326" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.37</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M327" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.29</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8">NaN</oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M328" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.32</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M329" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.33</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BELL</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">26 January 2012</oasis:entry>
         <oasis:entry colname="col4">1.22</oasis:entry>
         <oasis:entry colname="col5">0.30</oasis:entry>
         <oasis:entry colname="col6">0.67</oasis:entry>
         <oasis:entry colname="col7">1.43</oasis:entry>
         <oasis:entry colname="col8">1.30</oasis:entry>
         <oasis:entry colname="col9">1.34</oasis:entry>
         <oasis:entry colname="col10">1.47</oasis:entry>
         <oasis:entry colname="col11">1.11</oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BELL</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">22 September 2014</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M330" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.47</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.13</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M331" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.36</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M332" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.49</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M333" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.49</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M334" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.32</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M335" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.46</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M336" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.69</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BELL</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">12 May 2016</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M337" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.61</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.05</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M338" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.56</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M339" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.57</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M340" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.59</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M341" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.71</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M342" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.63</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M343" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.63</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">AntCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BRST</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">26 October 2011</oasis:entry>
         <oasis:entry colname="col4">0.36</oasis:entry>
         <oasis:entry colname="col5">0.08</oasis:entry>
         <oasis:entry colname="col6">0.45</oasis:entry>
         <oasis:entry colname="col7">0.28</oasis:entry>
         <oasis:entry colname="col8">0.39</oasis:entry>
         <oasis:entry colname="col9">0.41</oasis:entry>
         <oasis:entry colname="col10">0.37</oasis:entry>
         <oasis:entry colname="col11">0.25</oasis:entry>
         <oasis:entry colname="col12">AntCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CREU</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">17 May 2016</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M344" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.03</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.17</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M345" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.81</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M346" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.11</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M347" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.08</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M348" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.04</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M349" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.87</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M350" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.28</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">AntCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">DELF</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">23 July 2000</oasis:entry>
         <oasis:entry colname="col4">0.23</oasis:entry>
         <oasis:entry colname="col5">0.05</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7">0.26</oasis:entry>
         <oasis:entry colname="col8">0.27</oasis:entry>
         <oasis:entry colname="col9">0.20</oasis:entry>
         <oasis:entry colname="col10">0.18</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">DOUR</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">2 March 2015</oasis:entry>
         <oasis:entry colname="col4">0.37</oasis:entry>
         <oasis:entry colname="col5">0.03</oasis:entry>
         <oasis:entry colname="col6">0.40</oasis:entry>
         <oasis:entry colname="col7">0.35</oasis:entry>
         <oasis:entry colname="col8">0.35</oasis:entry>
         <oasis:entry colname="col9">0.34</oasis:entry>
         <oasis:entry colname="col10">0.39</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EIJS</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">28 April2000</oasis:entry>
         <oasis:entry colname="col4">0.22</oasis:entry>
         <oasis:entry colname="col5">0.07</oasis:entry>
         <oasis:entry colname="col6">0.33</oasis:entry>
         <oasis:entry colname="col7">0.25</oasis:entry>
         <oasis:entry colname="col8">0.19</oasis:entry>
         <oasis:entry colname="col9">0.18</oasis:entry>
         <oasis:entry colname="col10">0.15</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ERLA</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 July 2005</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M351" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.64</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.15</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M352" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.50</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M353" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.48</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M354" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.62</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M355" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.68</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M356" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.68</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M357" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.90</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ERLA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">18 August 2010</oasis:entry>
         <oasis:entry colname="col4">0.23</oasis:entry>
         <oasis:entry colname="col5">0.05</oasis:entry>
         <oasis:entry colname="col6">0.16</oasis:entry>
         <oasis:entry colname="col7">0.22</oasis:entry>
         <oasis:entry colname="col8">0.28</oasis:entry>
         <oasis:entry colname="col9">0.31</oasis:entry>
         <oasis:entry colname="col10">0.21</oasis:entry>
         <oasis:entry colname="col11">0.22</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EUSK</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">9 May 2001</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M358" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.74</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.13</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M359" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.56</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M360" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.74</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M361" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.76</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M362" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.73</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M363" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.71</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M364" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.97</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GOPE</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">4 November 1999</oasis:entry>
         <oasis:entry colname="col4">0.27</oasis:entry>
         <oasis:entry colname="col5">0.03</oasis:entry>
         <oasis:entry colname="col6">0.25</oasis:entry>
         <oasis:entry colname="col7">0.24</oasis:entry>
         <oasis:entry colname="col8">NaN</oasis:entry>
         <oasis:entry colname="col9">NaN</oasis:entry>
         <oasis:entry colname="col10">0.31</oasis:entry>
         <oasis:entry colname="col11">0.28</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GOPE</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">24 July 2000</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M365" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.96</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.07</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M366" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.06</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M367" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.86</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M368" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.97</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M369" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.00</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M370" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.98</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M371" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.92</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GOPE</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 September 2001</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M372" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.51</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.10</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M373" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.52</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M374" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.57</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M375" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.34</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M376" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.51</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M377" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.65</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M378" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.49</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GOPE</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">14 July 2006</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M379" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.39</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.09</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M380" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.39</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M381" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M382" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.32</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M383" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.33</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M384" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.47</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M385" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.52</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GOPE</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">14 December 2009</oasis:entry>
         <oasis:entry colname="col4">0.35</oasis:entry>
         <oasis:entry colname="col5">0.10</oasis:entry>
         <oasis:entry colname="col6">0.17</oasis:entry>
         <oasis:entry colname="col7">0.33</oasis:entry>
         <oasis:entry colname="col8">0.40</oasis:entry>
         <oasis:entry colname="col9">0.43</oasis:entry>
         <oasis:entry colname="col10">0.33</oasis:entry>
         <oasis:entry colname="col11">0.42</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GOPE</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 May 2016</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M386" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.36</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M387" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.29</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M388" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.36</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M389" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.33</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M390" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.35</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M391" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.46</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HELG</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">2 September 2008</oasis:entry>
         <oasis:entry colname="col4">0.19</oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6">0.23</oasis:entry>
         <oasis:entry colname="col7">0.15</oasis:entry>
         <oasis:entry colname="col8">0.11</oasis:entry>
         <oasis:entry colname="col9">0.19</oasis:entry>
         <oasis:entry colname="col10">0.27</oasis:entry>
         <oasis:entry colname="col11">0.18</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HELG</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">9 September 2014</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M392" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.14</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.04</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M393" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.19</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M394" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.10</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M395" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.11</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10">NaN</oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M396" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.17</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HERS</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">19 August 2010</oasis:entry>
         <oasis:entry colname="col4">0.51</oasis:entry>
         <oasis:entry colname="col5">0.16</oasis:entry>
         <oasis:entry colname="col6">0.66</oasis:entry>
         <oasis:entry colname="col7">0.41</oasis:entry>
         <oasis:entry colname="col8">0.52</oasis:entry>
         <oasis:entry colname="col9">0.50</oasis:entry>
         <oasis:entry colname="col10">0.71</oasis:entry>
         <oasis:entry colname="col11">0.27</oasis:entry>
         <oasis:entry colname="col12">AntCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HOBU</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">28 February 2007</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M397" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.31</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.08</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M398" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.23</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M399" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.24</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M400" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.33</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M401" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.40</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M402" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.24</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M403" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.40</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HOBU</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">22 November 2010</oasis:entry>
         <oasis:entry colname="col4">0.40</oasis:entry>
         <oasis:entry colname="col5">0.08</oasis:entry>
         <oasis:entry colname="col6">0.34</oasis:entry>
         <oasis:entry colname="col7">0.28</oasis:entry>
         <oasis:entry colname="col8">0.44</oasis:entry>
         <oasis:entry colname="col9">0.50</oasis:entry>
         <oasis:entry colname="col10">0.40</oasis:entry>
         <oasis:entry colname="col11">0.45</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HOBU</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">27 May 2015</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M404" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.22</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M405" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.27</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M406" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.19</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M407" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.20</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M408" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.13</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M409" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.21</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M410" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HOFN</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">21 September 2001</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M411" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.95</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.09</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M412" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.11</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M413" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.91</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M414" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.92</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M415" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.85</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M416" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.98</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M417" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.91</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">KARL</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">10 May 2001</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M418" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.64</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.14</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M419" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.64</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M420" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.47</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M421" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.54</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M422" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.65</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M423" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.68</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M424" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.89</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">KLOP</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">8 May  2001</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M425" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.60</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.11</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M426" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.40</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M427" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.55</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M428" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.65</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M429" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.67</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M430" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.62</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M431" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.72</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LAMP</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 March 2013</oasis:entry>
         <oasis:entry colname="col4">0.99</oasis:entry>
         <oasis:entry colname="col5">0.17</oasis:entry>
         <oasis:entry colname="col6">1.05</oasis:entry>
         <oasis:entry colname="col7">0.70</oasis:entry>
         <oasis:entry colname="col8">NaN</oasis:entry>
         <oasis:entry colname="col9">1.00</oasis:entry>
         <oasis:entry colname="col10">1.10</oasis:entry>
         <oasis:entry colname="col11">1.10</oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LAMP</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">11 April 2014</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M432" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.75</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.18</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M433" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.53</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M434" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.60</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M435" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.94</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M436" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.82</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M437" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.66</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M438" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.95</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">AntCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LAMP</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">26 September 2017</oasis:entry>
         <oasis:entry colname="col4">0.52</oasis:entry>
         <oasis:entry colname="col5">0.13</oasis:entry>
         <oasis:entry colname="col6">0.48</oasis:entry>
         <oasis:entry colname="col7">0.36</oasis:entry>
         <oasis:entry colname="col8">0.69</oasis:entry>
         <oasis:entry colname="col9">0.47</oasis:entry>
         <oasis:entry colname="col10">0.59</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LEED</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">11 November 2008</oasis:entry>
         <oasis:entry colname="col4">0.38</oasis:entry>
         <oasis:entry colname="col5">0.11</oasis:entry>
         <oasis:entry colname="col6">0.24</oasis:entry>
         <oasis:entry colname="col7">0.38</oasis:entry>
         <oasis:entry colname="col8">0.39</oasis:entry>
         <oasis:entry colname="col9">0.46</oasis:entry>
         <oasis:entry colname="col10">0.53</oasis:entry>
         <oasis:entry colname="col11">0.29</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LEIJ</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">1 July 2010</oasis:entry>
         <oasis:entry colname="col4">0.25</oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7">0.23</oasis:entry>
         <oasis:entry colname="col8">0.31</oasis:entry>
         <oasis:entry colname="col9">0.29</oasis:entry>
         <oasis:entry colname="col10">NaN</oasis:entry>
         <oasis:entry colname="col11">0.17</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MAN2</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">23 January 2008</oasis:entry>
         <oasis:entry colname="col4">0.29</oasis:entry>
         <oasis:entry colname="col5">0.04</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7">0.24</oasis:entry>
         <oasis:entry colname="col8">0.32</oasis:entry>
         <oasis:entry colname="col9">0.32</oasis:entry>
         <oasis:entry colname="col10">0.28</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">AntCod and RecMod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MODA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">12 July 2007</oasis:entry>
         <oasis:entry colname="col4">1.54</oasis:entry>
         <oasis:entry colname="col5">0.08</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7">1.45</oasis:entry>
         <oasis:entry colname="col8">1.64</oasis:entry>
         <oasis:entry colname="col9">1.60</oasis:entry>
         <oasis:entry colname="col10">1.56</oasis:entry>
         <oasis:entry colname="col11">1.47</oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MODA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">8 January 2008</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M439" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.60</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.28</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M440" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.11</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M441" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.53</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M442" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.69</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M443" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.68</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M444" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.92</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M445" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.70</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MOPI</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 August 2004</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M446" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.53</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.09</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M447" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.43</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M448" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.54</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M449" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.51</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M450" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.44</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M451" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.65</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M452" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.62</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">OSNA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">22 April 2004</oasis:entry>
         <oasis:entry colname="col4">0.38</oasis:entry>
         <oasis:entry colname="col5">0.07</oasis:entry>
         <oasis:entry colname="col6">0.47</oasis:entry>
         <oasis:entry colname="col7">0.41</oasis:entry>
         <oasis:entry colname="col8">0.32</oasis:entry>
         <oasis:entry colname="col9">0.31</oasis:entry>
         <oasis:entry colname="col10">0.37</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">OSNA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">23 April 2007</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M453" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.61</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M454" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.60</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M455" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.57</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M456" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.62</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M457" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.59</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M458" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.57</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M459" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.73</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">OSNA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">5 April 2011</oasis:entry>
         <oasis:entry colname="col4">0.23</oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6">0.18</oasis:entry>
         <oasis:entry colname="col7">0.14</oasis:entry>
         <oasis:entry colname="col8">0.28</oasis:entry>
         <oasis:entry colname="col9">0.29</oasis:entry>
         <oasis:entry colname="col10">0.24</oasis:entry>
         <oasis:entry colname="col11">0.26</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">OSNA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">11 June 2015</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M460" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.18</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M461" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.17</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M462" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.20</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M463" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.12</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M464" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.16</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M465" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.18</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M466" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.28</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PENC</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">22 May 2003</oasis:entry>
         <oasis:entry colname="col4">0.55</oasis:entry>
         <oasis:entry colname="col5">0.10</oasis:entry>
         <oasis:entry colname="col6">0.54</oasis:entry>
         <oasis:entry colname="col7">0.57</oasis:entry>
         <oasis:entry colname="col8">0.56</oasis:entry>
         <oasis:entry colname="col9">0.59</oasis:entry>
         <oasis:entry colname="col10">0.37</oasis:entry>
         <oasis:entry colname="col11">0.68</oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PENC</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">26 June 2007</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M467" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.32</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M468" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.29</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M469" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M470" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.29</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M471" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.29</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M472" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.34</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M473" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.43</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PTBB</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 June 2014</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M474" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.50</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.11</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M475" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.57</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M476" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.49</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M477" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.39</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M478" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.36</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M479" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.53</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M480" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.65</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">REYK</oasis:entry>
         <oasis:entry colname="col2">1</oasis:entry>
         <oasis:entry colname="col3">15 March 2003</oasis:entry>
         <oasis:entry colname="col4">0.31</oasis:entry>
         <oasis:entry colname="col5">0.03</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7">0.35</oasis:entry>
         <oasis:entry colname="col8">0.34</oasis:entry>
         <oasis:entry colname="col9">0.28</oasis:entry>
         <oasis:entry colname="col10">0.29</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">Unknown</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">REYK</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">13 March 2008</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M481" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.30</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.08</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M482" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.19</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M483" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.28</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M484" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.36</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M485" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.31</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M486" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.25</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M487" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.42</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">REYK</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">2 May 2013</oasis:entry>
         <oasis:entry colname="col4">0.27</oasis:entry>
         <oasis:entry colname="col5">0.09</oasis:entry>
         <oasis:entry colname="col6">0.24</oasis:entry>
         <oasis:entry colname="col7">0.13</oasis:entry>
         <oasis:entry colname="col8">0.34</oasis:entry>
         <oasis:entry colname="col9">0.33</oasis:entry>
         <oasis:entry colname="col10">0.28</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod and RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">SULD</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">14 June 2005</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M488" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.53</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.11</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M489" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.54</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M490" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.52</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M491" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.56</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M492" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.55</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M493" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.32</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M494" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.67</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">AntCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">TERS</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">16 September 2008</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M495" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.20</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M496" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.29</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M497" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.18</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M498" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.20</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M499" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.14</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M500" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.13</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M501" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.26</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">TERS</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">29 August 2013</oasis:entry>
         <oasis:entry colname="col4">0.35</oasis:entry>
         <oasis:entry colname="col5">0.05</oasis:entry>
         <oasis:entry colname="col6">0.30</oasis:entry>
         <oasis:entry colname="col7">0.37</oasis:entry>
         <oasis:entry colname="col8">0.39</oasis:entry>
         <oasis:entry colname="col9">0.36</oasis:entry>
         <oasis:entry colname="col10">0.41</oasis:entry>
         <oasis:entry colname="col11">0.28</oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">TRDS</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">7 May 2007</oasis:entry>
         <oasis:entry colname="col4">0.25</oasis:entry>
         <oasis:entry colname="col5">0.06</oasis:entry>
         <oasis:entry colname="col6">0.27</oasis:entry>
         <oasis:entry colname="col7">0.20</oasis:entry>
         <oasis:entry colname="col8">0.27</oasis:entry>
         <oasis:entry colname="col9">0.18</oasis:entry>
         <oasis:entry colname="col10">0.32</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">A&amp;RCod</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">WSRA</oasis:entry>
         <oasis:entry colname="col2">0</oasis:entry>
         <oasis:entry colname="col3">6 January 2000</oasis:entry>
         <oasis:entry colname="col4">0.14</oasis:entry>
         <oasis:entry colname="col5">0.02</oasis:entry>
         <oasis:entry colname="col6">NaN</oasis:entry>
         <oasis:entry colname="col7">0.15</oasis:entry>
         <oasis:entry colname="col8">0.16</oasis:entry>
         <oasis:entry colname="col9">0.11</oasis:entry>
         <oasis:entry colname="col10">0.13</oasis:entry>
         <oasis:entry colname="col11">NaN</oasis:entry>
         <oasis:entry colname="col12">RecM&amp;M</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

      <p id="d1e9202">As the changepoint detection was carried out on a monthly level, the specific
dates of the Type-0 changepoint are fixed as documented. However, for the
Type-1 changepoints without support from metadata, their time of
occurrence is fixed to the 15th day of the associated month. We adjusted the
GPS IWV time series by adding the amplitude of each changepoint to the GPS
IWV data points before its time of occurrence. Note that five out of the
nine Type-1 changepoints are significant in all  six GPS-reanalyses
comparisons. Although we tried to minimise the impacts of changepoints in
specific reanalyses on the results here, we cannot completely rule out that
identical changepoints appear in all  six reanalyses by ingesting the
same observational datasets through data assimilation.</p><?xmltex \hack{\newpage}?>
      <p id="d1e9206"><?xmltex \hack{\vspace*{161mm}}?>Figures A1 and A2 show the homogenisation results at two stations. Station
HERS (Herstmonceux, UK; 50.87<inline-formula><mml:math id="M502" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 0.34<inline-formula><mml:math id="M503" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) is
characterised by abnormal variations in its up-coordinate time series
before the changes of the antenna and receiver on 18 February 1998 as shown in Fig. A1h, indicating low-quality observations related to the instrumentation. In addition, obvious abnormal variations can be seen in all the GPS-reanalysis comparisons before  September of 2001. We checked IGSMAIL-3503 (<uri>https://lists.igs.org/pipermail/igsmail/2001/004876.html</uri>, last access: 8 January 2023), which reported a repair of antenna at station HERS until 3 September 2001. Therefore, we excluded the GPS IWV data before the date of repair. Then, we used the RHtestsV4 software to identify the changepoints in the rest of the GPS IWV time series and found <?pagebreak page3535?>one on 19 August 2010, which is significant at a confidence level of 99 %. It is a Type-0 changepoint due to antenna and receiver changes as recorded in the station log file. After the homogenisation, the linear trend of the GPS IWV time series at station HERS has been reduced from 0.71 to 0.27 kg m<inline-formula><mml:math id="M504" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade, which generally agrees better with the trend estimates from reanalyses, which are 0.15, 0.43, 0.33, 0.37, 0.10, and 0.59 kg m<inline-formula><mml:math id="M505" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade for CFSR, ERA5, ERAI, JRA-55, MERRA-2, and NCEP-2, respectively.</p>

      <?xmltex \floatpos{h!}?><fig id="App1.Ch1.S1.F15"><?xmltex \currentcnt{A2}?><?xmltex \def\figurename{Figure}?><label>Figure A2</label><caption><p id="d1e9258">The same as Fig. A1 but for station ERLA. A Type-0
changepoint is significant on 18 August 2010 (green triangle) due to changes in the
antenna and radome at the station. A Type-1 changepoint in  July of 2005 (green
vertical line and upward-pointing triangle) is significant but without
support from metadata, and hence its date was fixed to 15 July 2005.</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://acp.copernicus.org/articles/23/3517/2023/acp-23-3517-2023-f15.png"/>

      </fig>

      <p id="d1e9269">Station ERLA (Erlangen, Germany; 49.59<inline-formula><mml:math id="M506" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 11.01<inline-formula><mml:math id="M507" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E)
has a Type-1 changepoint in July of 2015 for unknown reasons, in addition to a
Type 0 one due to antenna and radome<?pagebreak page3536?> changes on 18 August 2010 (Fig. A2). The
date of the Type-1 changepoint was fixed to 15 July 2005. With the homogenisation, the linear trend of the GPS IWV time series at station ERLA
has been increased from 0.14 to 0.40 kg m<inline-formula><mml:math id="M508" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade, which is
closer to the trend estimates from reanalyses, which are 0.43, 0.36, 0.41,
0.43, 0.52, and 0.68 kg m<inline-formula><mml:math id="M509" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade for CFSR, ERA5, ERAI, JRA-55,
MERRA-2, and NCEP-2, respectively. Moreover, we compared the GPS IWV trend to
three nearby stations (KARL, KLOP, and WTZR) with values of 0.56, 0.32, and
0.66 kg m<inline-formula><mml:math id="M510" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade and their distances to ERLA of 198.6, 177.5,
and 144.4 km, respectively. The results indicate an improved spatial
consistency in the GPS IWV trends from the homogenised time series.
Therefore, the homogenisation at station ERLA is considered to be
reasonable.</p><?xmltex \hack{\newpage}?><?xmltex \hack{\vspace*{162mm}}?><?xmltex \floatpos{h!}?><table-wrap id="App1.Ch1.S1.T4"><?xmltex \currentcnt{A2}?><label>Table A2</label><caption><p id="d1e9330">Types of changes in GPS instrumentation.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Abbreviation</oasis:entry>
         <oasis:entry colname="col3">Type of change</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">1</oasis:entry>
         <oasis:entry colname="col2">AntCod</oasis:entry>
         <oasis:entry colname="col3">Antenna code</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2</oasis:entry>
         <oasis:entry colname="col2">RadCod</oasis:entry>
         <oasis:entry colname="col3">Radome code</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">3</oasis:entry>
         <oasis:entry colname="col2">A&amp;RCod</oasis:entry>
         <oasis:entry colname="col3">Antenna and radome code</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">4</oasis:entry>
         <oasis:entry colname="col2">RecMod</oasis:entry>
         <oasis:entry colname="col3">Receiver model</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">5</oasis:entry>
         <oasis:entry colname="col2">RecM&amp;M</oasis:entry>
         <oasis:entry colname="col3">Receiver make and model</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?>
</app>
  </app-group><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e9427">The GPS ZTD data were provided by NGL (<uri>http://geodesy.unr.edu/gps_timeseries/trop</uri>, Blewitt et al., 2023). The ERA5 and ERAI data were downloaded from the Climate Data Store (CDS; <ext-link xlink:href="https://doi.org/10.24381/cds.bd0915c6" ext-link-type="DOI">10.24381/cds.bd0915c6</ext-link>, Hersbach et al., 2023) and ECWMF (<uri>https://apps.ecmwf.int/datasets/data/interim-full-daily/levtype=pl</uri>, last access: 8 January 2023), respectively. The CFSR (<ext-link xlink:href="https://doi.org/10.5065/D61C1TXF" ext-link-type="DOI">10.5065/D61C1TXF</ext-link>; Saha et al., 2011) and JRA55 (<ext-link xlink:href="https://doi.org/10.5065/D6HH6H41" ext-link-type="DOI">10.5065/D6HH6H41</ext-link>; Japan Meteorological Agency, 2013) data are available in the research data archive of NCAR. MERRA2 data were derived from NASA Goddard Earth Sciences Data and Information Services Center (<ext-link xlink:href="https://doi.org/10.5067/QBZ6MG944HW0" ext-link-type="DOI">10.5067/QBZ6MG944HW0</ext-link>; Global Modeling and Assimilation Office, 2015). NCEP2 data were obtained from NOAA Physical Sciences Laboratory (NOAA PSL; <uri>https://psl.noaa.gov/data/gridded/data.ncep.reanalysis2.html</uri>, last access: 8 January 2023). The GNSS IWV time series are available from the corresponding author upon reasonable request.</p>
  </notes><app-group>
        <supplementary-material position="anchor"><p id="d1e9452">The supplement related to this article is available online at: <inline-supplementary-material xlink:href="https://doi.org/10.5194/acp-23-3517-2023-supplement" xlink:title="zip">https://doi.org/10.5194/acp-23-3517-2023-supplement</inline-supplementary-material>.</p></supplementary-material>
        </app-group><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e9461">PY: conceptualisation, methodology, formal analysis, investigation, writing (original draft), and visualisation. RV, XY, HV, WJ, JA, and BH: investigation and reviewing. HK: investigation, reviewing, supervision, project administration, and funding acquisition.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e9467">The contact author has declared that none of the authors has any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d1e9474">Publisher’s note: Copernicus Publications remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.</p>
  </notes><notes notes-type="sistatement"><title>Special issue statement</title>

      <p id="d1e9480">This article is part of the special issue “Analysis of atmospheric water vapour observations and their uncertainties for climate applications (ACP/AMT/ESSD/HESS inter-journal SI)”. It is not associated with a conference.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e9486">We are grateful to NGL for providing the GPS ZTD products and many
institutions for sharing the continuous GPS observations. We thank ECMWF,
JMA, NASA GAMO, and NCEP for providing the reanalyses products. We would like to thank the German Research Foundation and the Program for Hubei Provincial Science and Technology Innovation Talents of China for financial support.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e9491">This research has been supported by the Deutsche Forschungsgemeinschaft (grant no. 321886779). Weiping Jiang is funded by the Program for Hubei Provincial Science and Technology Innovation Talents of China (grant no. 2022EJD010).<?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>The article processing charges for this open-access <?xmltex \notforhtml{\newline}?>publication were covered by the Karlsruhe Institute<?xmltex \notforhtml{\newline}?> of Technology (KIT).</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e9504">This paper was edited by Rolf Müller and reviewed by two anonymous referees.</p>
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