<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing with OASIS Tables v3.0 20080202//EN" "journalpub-oasis3.dtd">
<article xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:oasis="http://docs.oasis-open.org/ns/oasis-exchange/table" xml:lang="en" dtd-version="3.0" article-type="research-article"><?xmltex \bartext{Research article}?>
  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-22-419-2022</article-id><title-group><article-title>Observed slump of sea land breeze in Brisbane under the effect of aerosols
from remote transport during<?xmltex \hack{\break}?> 2019 Australian mega fire events</article-title><alt-title>Slump of sea land breeze by aerosols</alt-title>
      </title-group><?xmltex \runningtitle{Slump of sea land breeze by aerosols}?><?xmltex \runningauthor{L. Shen et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Shen</surname><given-names>Lixing</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="yes">
          <name><surname>Zhao</surname><given-names>Chuanfeng</given-names></name>
          <email>czhao@bnu.edu.cn</email>
        <ext-link>https://orcid.org/0000-0002-5196-3996</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Yang</surname><given-names>Xingchuan</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Yang</surname><given-names>Yikun</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-7427-6876</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Zhou</surname><given-names>Ping</given-names></name>
          
        </contrib>
        <aff id="aff1"><institution>College of Global Change and Earth System Science, and State Key
Laboratory of Earth Surface Processes and Resource Ecology, Beijing Normal
University, Beijing 100875, China
</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Chuanfeng Zhao (czhao@bnu.edu.cn)</corresp></author-notes><pub-date><day>12</day><month>January</month><year>2022</year></pub-date>
      
      <volume>22</volume>
      <issue>1</issue>
      <fpage>419</fpage><lpage>439</lpage>
      <history>
        <date date-type="received"><day>1</day><month>October</month><year>2021</year></date>
           <date date-type="rev-request"><day>4</day><month>October</month><year>2021</year></date>
           <date date-type="rev-recd"><day>16</day><month>November</month><year>2021</year></date>
           <date date-type="accepted"><day>6</day><month>December</month><year>2021</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2022 </copyright-statement>
        <copyright-year>2022</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/.html">This article is available from https://acp.copernicus.org/articles/.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d1e118">The 2019 Australian mega fires were unprecedented
considering their intensity and consistency. There has been much research
on the environmental and ecological effects of these mega fires, most of
which focused on the effect of huge aerosol loadings and the ecological
devastation. Sea land breeze (SLB) is a regional thermodynamic circulation
closely related to coastal pollution dispersion, yet few have looked into how
it is influenced by different types of aerosols transported from either
nearby or remote areas. Mega fires provide an optimal scenario of large
aerosol emissions. Near the coastal site of Brisbane Archerfield during
January 2020, when mega fires were the strongest, reanalysis data from
Modern-Era Retrospective analysis for Research and Applications version 2
(MERRA-2) showed that mega fires did release huge amounts of aerosols,
making aerosol optical depth (AOD) of total aerosols, black carbon (BC) and
organic carbon (OC) approximately 240 %, 425 % and 630 % of the averages
in other non-fire years. Using 20 years' wind observations of hourly time
resolution from a global observation network managed by the National Oceanic and
Atmospheric Administration (NOAA), we found that the SLB day number during
that month was only 4, accounting for 33.3 % of the multi-years'
average. The land wind (LW) speed and sea wind (SW) speed also decreased by
22.3 % and 14.8 % compared with their averages respectively.
Surprisingly, fire spot and fire radiative power (FRP) analysis showed that
heating effects and aerosol emission of the nearby fire spots were not the main
causes of the local SLB anomaly, while the remote transport of aerosols from the
fire centre was mainly responsible for the decrease of SW, which was
partially offset by the heating effect of nearby fire spots and the warming
effect of long-range transported BC and CO<inline-formula><mml:math id="M1" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>. The large-scale cooling
effect of aerosols on sea surface temperature (SST) and the burst of BC
contributed to the slump of LW. The remote transport of total aerosols was
mainly caused by free diffusion, while the large-scale wind field played a
secondary role at 500 m. The large-scale wind field played a more important role
in aerosol transport at 3 km than at 500 m, especially for the gathered
smoke, but free diffusion remained the major contributor. The decrease of
SLB speed boosted the local accumulation of aerosols, thus making SLB
speed decrease further, forming a positive feedback mechanism.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<?pagebreak page420?><sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e139">Aerosols play an important role in balancing the Earth's radiation budget,
through their direct or indirect effects (Albrecht, 1989; Garrett and Zhao,
2006; IPCC, 2013; McCoy and Hartmann, 2015). There are different types of
aerosols from various sources which have different climatological forcing
effects (Charlson et al., 1992; Yang et al., 2016). Aerosols differ in radiative
forcing effects as their physical and chemical properties vary, some of
which may affect the earth–atmosphere system by bringing changes to the
lifespan of clouds (Albrecht, 1989; Zhao and Garrett, 2015).</p>
      <p id="d1e142">Carbonaceous aerosol contains black carbon (BC) and organic carbon (OC) and
serves as a major radiation-influencing aerosol which mainly originates from
biomass burning (Vermote et al., 2009; Yang et al., 2021). There have been
studies addressing the importance of BC on atmospheric warming and that of
OC on weakening in situ downwelling solar radiation (Jacobson, 2001; Ramana et al.,
2010). There are also some studies that try to quantify the average radiative
forcing effects of BC and OC, while they also emphasize the potential
uncertainties with respect to the specific values (Zhang et al., 2017). At a
planetary scale, the change of aerosols brings many uncertainties to
the radiation balance, thus further influencing the magnitude of atmospheric
circulation (Wang et al., 2015; Zhao et al., 2020). At a synoptic scale,
aerosols can affect tropical cyclones by enlarging their rainfall area, which
is also related to their radiative properties (Zhao et al., 2018). At a
regional scale, Han et al. (2020) discussed in detail the radiative forcing
effect of aerosols on the speed of the urban heat island (UHI) in different
seasons.</p>
      <p id="d1e145">As mentioned above, biomass burning is an important source of aerosols,
especially for carbonaceous aerosols. Adequate amounts of fire-emitted
aerosols would bring perturbations to the balanced Earth's climate system
through both direct and indirect effects (Jacobson, 2014). There has been
much research discussing the characteristics of wild fire aerosols and
their effect around the world (Grandey et al., 2016; Mitchell et al., 2006).
For example, Portin et al. (2012) investigated the characterization of
burning aerosols in eastern Finland during Russian wild fires in the summer
of 2010. Kloss et al. (2019) pointed out that wild fires could bring plumes
of smoke that ascend very high and pollute remote areas with the help of
a monsoon. Grandey et al. (2016) quantified the radiative effect of the total
fire-induced aerosols over the globe, which was estimated to be <inline-formula><mml:math id="M2" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.0 W/m<inline-formula><mml:math id="M3" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> on average. The fire-induced aerosols could have more significant
radiative effects with clouds than under clear-sky conditions through
cloud–aerosol interaction, whose global forcing effect could reach <inline-formula><mml:math id="M4" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.16 W/m<inline-formula><mml:math id="M5" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> (Chuang et al., 2002).</p>
      <p id="d1e180">Australia is one of the areas where wild fires occur frequently (Yang et
al., 2021). An area of nearly 550 000 km<inline-formula><mml:math id="M6" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> of tropical and arid savanna
is burnt each year in Australia, contributing to about 6 %–8 % of global
carbon emissions from biomass burning (van der Werf et al., 2006; Meyer et
al., 2008). Particularly, there have been many studies concentrating on wild
fires' association with enhancing aerosol loadings and air pollution events
in Australia, some of which included the discussion on the combined effect
from background meteorological conditions (Mitchell et al., 2006; Luhar et
al., 2008; Meyer et al., 2008; Mitchell et al., 2013; Mallet et al., 2017).
The 2019 Australian wild fires from December 2019 to February 2020 were
unprecedented in recent decades in terms of the magnitude and consistency, so
they have attracted the attention of the world in a short time. Since
their outbreak, numerous studies have been carried out to investigate them
from different aspects. For example, Yang et al. (2021) examined the
statistical properties of aerosol properties associated with the 2019 Australian
mega fire events in both horizontal and vertical directions. Torres et al. (2020) investigated the aerosol emissions during the mega fires happening in
New South Wales, Australia, and found a great amount of carbonaceous aerosols
in the stratosphere. Ohneiser et al. (2020) traced wildfire smoke in one of
the most severely burnt areas in southeastern Australia and found that smoke
could even travel across the Pacific, which was detected by an observation
site at Punta Arenas in South America.</p>
      <p id="d1e193">Sea land breeze (SLB) is a common circulation over coastal areas whose
direct cause is the regional temperature difference between land and sea
(TDLS). Many studies have investigated this regional circulation. On the one
hand, the complicated influencing factors of SLB have been studied from
different perspectives (Miller et al., 2013). Our previous studies pointed
out that the change of TDLS is highly related to the change of in situ downwelling
solar radiation (Shen et al., 2021a, b; Shen and Zhao, 2020). We also found
that the continuous increase of surface roughness in cities can reduce the
SLB speed in the long term (Shen et al., 2019). The long-term significance and
trends of SLBs over the globe are driven by climate regimes which are
related to climatological differences in both in situ downwelling solar radiation
and background wind fields. There are also many other studies on the
influencing factors of SLB in short periods. For example, based on the case
analysis, Sarker et al. (1998) found that the UHI magnitude has a great impact
on the encroachment range of sea wind (SW) frontal surface. Using regional
model simulation, Ma et al. (2013) found that the UHI effect can greatly enhance
TDLS, which would result in strengthened SLB circulation in a great
metropolis. Miller et al. (2013) reviewed the studies on SLB and pointed out
that local topography such as the shape of the coastline is another
important influencing factor of SLB. On the other hand, SLB's effect has
also been extensively investigated. For example, SLB has been reported as a
direct controller of air pollutants which transports air pollutants inland
or to the vast ocean with the help of the background meteorological field (Nai
et al., 2018; Shen and Zhao, 2020). SLB is also essential to the
modification of the meteorological conditions and<?pagebreak page421?> local climate (Rajib and
Heekwa, 2010). Moreover, SLB is a determinant factor of the diurnal
variation of the precipitation on the island since its direction and
magnitude can affect the location and magnitude of convective systems (Zhu
et al., 2017).</p>
      <p id="d1e196">Over the years, the cause and effect of aerosols, wild fires in typical
areas and SLBs have been learned in detail. The relationship
between aerosols and other small-scale circulations such as UHI circulation
has also been investigated from many aspects (Han et al., 2020). However, few
studies have investigated the effects of different types of aerosols on SLBs
or looked into how local and remote aerosol emissions during mega fires
would affect local SLB with the help of the meteorological background field or
other potential mechanisms. There was an updated and important study calling
for attention of the record-breaking aerosol emissions during the 2019 Australian
mega fires which led to a significant cooling effect on ocean temperature
(Hirsch and Koren, 2021). Since in situ downwelling solar radiation and sea surface temperature (SST), which
are both important influential factors of SLB, are deeply affected by
different types of aerosols due to their different radiative properties, it
is interesting to examine in detail how the record-breaking mega fires would
influence SLB by releasing large amounts of aerosols.</p>
      <p id="d1e199">The paper is organized as follows. Section 2 describes the observation site,
data and analysis methods. Section 3 illustrates the characteristics of SLB,
the variation of SLB days, the distribution and fire radiative power (FRP)
of wild fire spots, the anomaly of observed SW speed, land wind (LW) speed
and air temperature, the effects of different aerosols on SLB's variation,
the analysis on background wind field and the comparison between local fire
spots' and the remote fire centre's contributions. Section 4 summarizes and
discusses the findings of the study and proposes a mechanism of aerosol–SLB
interaction during the peak of the 2019 Australian mega fires.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Data and methods</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>Site</title>
      <p id="d1e217">The 2019 Australian mega fires occurred mainly in the eastern and
southeastern coastal areas of Australian continent (Yang et al., 2021). The
southeastern parts, including the state of Victoria and the southeastern part of
the state of New South Wales, belong to a marine climate, where obvious
existence of SLB (OE-SLB) is not clearly verified because of the influence
of strong westerlies and water vapour accompanied with westerlies from the
ocean (Shen et al., 2021). Note that OE-SLB means that SLB is significant
from a climatological perspective. In other words, the SLB can be found
during most time of the year. Details of the definition of OE-SLB can be
found in Shen et al. (2021) and are not repeated here. Meanwhile, the wild
fire events there were the most severe with a great density according to
numerous reports, which could possibly have caused fire-induced complex flows and
circulation in the form of fire–atmosphere interactions in the vicinity of a
fire (Sun et al., 2019). Based on previous observation during mega fire
events, the concentrated fire spots changed the local air pressure field and
added a regional temperature-pressure field, bringing uncertainties to local
wind speed and wind direction (Jia et al., 1987; Li et al., 2016). On the one
hand, this could further interrupt the formation of SLB since it might make
the background wind field more complicated. On the other hand, the detected
SLB might not be accurate since it is likely to contain other wind
disturbances at a small regional scale.</p>
      <p id="d1e220">As shown in Fig. 1, we selected an urban site in Brisbane along the eastern
coast of Australia as the study site, which was due to several
considerations. First, alongside the eastern coastal areas of Australia
which belong to monsoon climate, including Brisbane and areas to its south
but to the north of the fire centre, the Australian monsoon system is not
strong, so the OE-SLB can be verified from a climatological perspective,
which also means integrated SLB circulation can be found during all seasons.
Second, compared to rural sites, there are longer periods of high-time-resolution observation data at urban sites, which is necessary for the
extraction of SLB signals. Third, the urban area of Brisbane is relatively
small and is not very far from vast areas of forests which provide stable
combustion environment, ensuring the persistent effect of wild fires.
Fourth, the UHI effect, which could possibly interrupt SLB and bring errors
when calculating SLB magnitude, should be small for the study region
considering the small scale of urban areas. Also, the wild fires near
suburban areas could further eliminate the UHI effect, even if it could exist
through their heating impact on these areas. In contrast, the forest site is
surrounded by or within great amounts of flora where the majority of solar
radiation is absorbed and scattered by leaves, prohibiting the surface
heating by solar radiation and then the formation and detection of SLB.
Actually, due to the existence of photosynthesis, the endothermic process of
leaves from solar radiation and the temperature rise of the “leaf surface” are
different from those of Earth's surface. As a result, the traditional
mechanism of SLB formation is not necessarily applicable when the site is in
the forest or quite close to clusters of flora. Coastal sites to the north
of Brisbane are too far from the fire centre, and they are mostly rural
sites covered with flora as well. Considering all of this, we chose the
site of Brisbane Archerfield located on the eastern coast of the state of Queensland
(Fig. 1) as the study site.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><?xmltex \currentcnt{1}?><?xmltex \def\figurename{Figure}?><label>Figure 1</label><caption><p id="d1e225">The map of eastern Australia with land-cover types. The
observation site is marked by a black dot.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f01.png"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Data</title>
      <p id="d1e242">Several types of data have been used in this study, including land-cover-type data, Modern-Era Retrospective analysis for Research and
Applications version 2 (MERRA-2) data, Moderate Resolution Imaging
Spectroradiometer (MODIS) data, ground site observation data, the Fifth
Version of European<?pagebreak page422?> Centre for Medium-Range Weather Forecasts (ECMWF)
ReAnalysis (ERA5) data, fire spot and FRP data and Global Data
Assimilation System (GDAS) data. The detailed data information is described
below one by one.</p>
      <p id="d1e245"><italic>Land-cover-type data</italic>. The land-cover-type data of Australia are from the Dynamic
Land Cover Dataset (DLCD) with Version 2.1 provided by Geoscience Australia.
In this study, the DLCD land-cover-type data were used to reveal the
surrounding landscape of Brisbane Archerfield. The spatial resolution of the
data is 0.002<inline-formula><mml:math id="M7" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M8" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.002<inline-formula><mml:math id="M9" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, which is based on
the annual mean of satellite observations from 2014 to 2015.</p>
      <p id="d1e275"><italic>MERRA-2 data</italic>. MERRA-2 belongs to the global atmospheric reanalysis product
managed by the National Aeronautics and Space Administration (NASA). It is
produced by the Global Modeling and Assimilation Office (GMAO), and the
assimilation system of Goddard Earth Observing System (GEOS-5) is used to
ensure the quality of this dataset. At major ground sites over Australia,
Yang et al. (2021) compared the monthly aerosol optical depth (AOD) product
with Aerosol Robotic Network (AERONET) observations and found their root mean square errors (RMSEs)
were all smaller than 0.05. Thus, MERRA-2 should be reliable to be used for
the analysis of the large-scale spatial distribution of AOD in Australia.
Yang et al. (2021) also denoted that the 2019 Australian mega fires were the
strongest in January 2020. Correspondingly, we used the monthly AOD in
January at 550 nm from 2002 to 2020 to check the AOD difference between the
mega fire year and years with no mega fires. The spatial resolution of
MERRA-2 AOD data is 0.625<inline-formula><mml:math id="M10" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M11" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M12" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>.</p>
      <p id="d1e305"><italic>MODIS data</italic>. The MODIS instrument is performed on Aqua and Terra platforms.
In this study, we used the MODIS cloud product which belongs to the dataset
of MCD06COSP_M3_MODIS. The cloud information
includes cloud optical depth (COD) and cloud fraction for all January months
during the period from 2003 to 2020 with a monthly time resolution. The
Brisbane Archerfield site is located at 153.008<inline-formula><mml:math id="M13" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E,
27.57<inline-formula><mml:math id="M14" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S. So we used COD and cloud fraction data whose space
range and resolution are 152.5–153.5<inline-formula><mml:math id="M15" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E <inline-formula><mml:math id="M16" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 28.5–26.5<inline-formula><mml:math id="M17" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and 1<inline-formula><mml:math id="M18" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M19" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M20" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> respectively. This spatial range covers the whole Brisbane area
and the normal encroaching distance of SLB, which is about tens of
kilometres (Rajib and Heekwa, 2010; Shen et al., 2019). In this study, their
spatial averages were calculated to represent the local COD and
cloud fraction every January from 2003 to 2020. Also, we used the MODIS
monthly AOD product for comparison with that of MERRA-2, which belongs to the
dataset of MOD08_M3. The spatial resolution of MODIS AOD data
is 1<inline-formula><mml:math id="M21" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M22" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M23" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, and the time range is the same as
that of MERRA-2.</p>
      <p id="d1e405"><italic>Ground site observation data</italic>. The wind and air temperature observation data
are from National Oceanic and Atmospheric Administration (NOAA) global
observation network at the site of Brisbane Archerfield (153.008<inline-formula><mml:math id="M24" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E, 27.57<inline-formula><mml:math id="M25" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S). We used data in January from 2001 to 2020 in this
study. The time resolution is every 3 h at 02:00, 05:00, 08:00, 11:00, 14:00,
17:00, 20:00 and 23:00 UTC on most days. The continuity of the observation data is
ensured; there are observations on each day in January throughout the whole
study period, with only one missing observation data on each day of a small
fraction time (approximately 3.5 %). The wind information includes wind
speed and wind direction. The air temperature is measured in Fahrenheit, and
we have converted it into Celsius. The observation data were the main data
used in this study to show the variations of both SLB and air temperature
during the fire.</p>
      <p id="d1e428"><italic>ERA5 data</italic>. The monthly mean U wind (zonal) speed and V wind (meridional) speed
in January 2020 from the ERA5 were used in this study to reveal the
background meteorological field so as to assess its effect on aerosol
transport. The spatial resolution is 0.250<inline-formula><mml:math id="M26" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M27" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.250<inline-formula><mml:math id="M28" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> at pressure levels of 1000, 975, 950, 925, 900, 875, 850, 825, 800, 775, 750 and 700 hPa.</p>
      <p id="d1e458"><italic>Fire spot and FRP data</italic>. Fire spot and FRP data are from the MODIS product (MCD14).
This product can catch and locate the active fire hotspots based on thermal anomalies
of 1 km pixel resolution (Giglio et al., 2016). The time resolution is daily,
and we used the monthly averages for January from 2002 to 2020 to look into
the fire situations over the years in detail.</p>
      <p id="d1e463"><italic>GDAS data</italic>. The GDAS data were used to perform the back-trajectory analysis
from the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT).
The spatial resolution of GDAS data is 1<inline-formula><mml:math id="M29" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M30" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M31" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> with daily time resolution.<?pagebreak page423?> The levels of GDAS data chosen in this study
to help to perform HYSPLIT analysis were 500 m and 3 km respectively. The
time range set in this study was the whole of January 2020.</p>
</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><title>Methods</title>
<sec id="Ch1.S2.SS3.SSS1">
  <label>2.3.1</label><title>Extracting SLB signal</title>
      <p id="d1e508">The verification of OE-SLB and extraction of SLB signals from original wind
observation over monsoon areas were carried out through the method of the
separation of the regional wind field (SRWF). The definition of OE-SLB, the
details of SRWF method and the criterion for verification were detailed in our
previous studies and are not repeated here (Shen et al., 2019; Shen and Zhao,
2020; Shen et al., 2021). Briefly speaking, SRWF calculates the vector
difference between observed wind vector and daily average wind vector for
each observation time. Then, the vector difference is considered to be the
local wind. The criterion of OE-SLB requires that there are intersection
sets among the range of SW, the range of LW and the range of hourly average
of wind angle in a diurnal period (HAWADP). Also, the intersection set
between the range of SW (LW) and the range of HAWADP only exists during
daytime (night-time). Then the local wind can be thought as the SLB signal as
long as the OE-SLB is verified at that site. Based on HAWADP and specific
sea–land distribution, we further defined the prevailing time of sea wind
(PTS) and prevailing time of land wind (PTL). Briefly speaking, during PTS
(PTL) the local wind keeps blowing from sea (land), and the wind angle keeps
rotating towards the direction of vast sea (inland). The HAWADP at Brisbane
Archerfield is shown in Fig. 2. As shown, the HAWADP of local wind was close
to sinusoid, which conformed to previous findings in other monsoon areas
(Shen et al., 2021; Yan and Anthes, 1987). According to the sea–land
distribution shown in Fig. 1, we first defined the ranges of SW and LW, and
then the OE-SLB of Brisbane Archerfield was verified using these criteria.
We further selected the PTS (PTL) based on the rules above.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><?xmltex \currentcnt{2}?><?xmltex \def\figurename{Figure}?><label>Figure 2</label><caption><p id="d1e513">Hourly average of wind angle in a diurnal period (HAWADP) of the
local wind.</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f02.png"/>

          </fig>

      <p id="d1e522">To make it clear, we summarize the range of SW, LW, PTS and PTL in Table 1.
The ranges of SW and LW refer to specific sea–land distribution. Notably,
there are few mountains within the ranges of SW and LW based on the accurate
site location and detailed landscape nearby, which helps to exclude
potential interruption from other small-scale circulations like
mountain–valley wind. Note that the actual PTS (PTL) may be longer than what
we defined here because the time resolution is 3 h instead of hourly in
this study. As a result, we cannot know the exact threshold of time when the
wind angle meets the criteria mentioned above. For instance, it is possible
that the wind angle is within the range of SW before 05:00 UTC. However, it
is still certain that the SW (LW) develops vigorously during 05:00–08:00 UTC
(14:00–20:00 UTC) based on Fig. 2, which means that 05:00–08:00 UTC and
14:00–20:00 UTC are within the real PTS and PTL respectively, even if they
are not the exact PTS or PTL. Thus, the PTS (PTL) defined in this study is
reliable. The aim of defining PTS (PTL) is to find the time period when SW
(LW) develops most vigorously so as to ensure further exclusion of winds
from synoptic scales when trying to extract real SLB signals after applying
the SRWF method (Shen and Zhao, 2020; Shen et al., 2021; Cuxart et al.,
2014).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e529">Summary of information for the verification of OE-SLB at Brisbane
Archerfield.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.9}[.9]?><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">The range of SW</oasis:entry>
         <oasis:entry colname="col2">The range of LW</oasis:entry>
         <oasis:entry colname="col3">PTS (UTC)</oasis:entry>
         <oasis:entry colname="col4">PTL (UTC)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">[20<inline-formula><mml:math id="M32" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> 135<inline-formula><mml:math id="M33" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> ]</oasis:entry>
         <oasis:entry colname="col2">[200<inline-formula><mml:math id="M34" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> 315<inline-formula><mml:math id="M35" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> ]</oasis:entry>
         <oasis:entry colname="col3">[05:00 08:00]</oasis:entry>
         <oasis:entry colname="col4">[14:00 20:00]</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S2.SS3.SSS2">
  <label>2.3.2</label><title>Definition of the SLB day</title>
      <?pagebreak page424?><p id="d1e626">The SLB day is the day when SLB circulation is most significant (Xue et al.,
1995). To some extent, the number of SLB days reveals the activity level of
SLB. Different criteria have been adopted when defining the SLB day. Here we
referred to our previous study (Shen et al., 2019) to adopt the criteria
based on the minimum times of successful detection of winds coming from the
range of SW (LW) during PTS (PTL). Since the time interval between two
adjacent observations is 3 h, which makes the number of total
observation times less than the total hours during prevailing time, we
modified the criteria slightly as follows: when the offshore land winds
occur in the period of 14:00–20:00 UTC with a total occurrence time of no fewer than
three times, and the onshore sea winds occur in the period of 05:00–08:00 UTC with a total
occurrence time of no fewer than two times, the day is counted as a SLB day.
<?xmltex \hack{\newpage}?></p>
</sec>
<sec id="Ch1.S2.SS3.SSS3">
  <label>2.3.3</label><title>The calculation of monthly SW and LW speeds</title>
      <p id="d1e638">After defining PTS, PTL and SLB day, we could finally calculate the monthly
SW and LW speeds. First, we picked up SLB days in every January from 2001 to
2020. Second, we picked up local wind speed during PTS (PTL) on SLB days and
calculated the monthly average of SW (LW) speed in every January from 2001
to 2020.</p>
      <p id="d1e641">Based on GDAS data throughout the whole of January 2020, the back
trajectories of the lower atmosphere at Brisbane Archerfield were simulated
using the HYSPLIT model, which could help analyse the effect of background
wind fields on aerosol transport at this site. The simulated levels at the
site were 500 m and 3 km since the lower level of the atmosphere (500 m) was
closer to fire spots, and there was also accumulated smoke at 3 km in the
southeastern parts of Australia during the exact same month (Yang et al.,
2021). The TrajStat module of Meteoinfo version 2.4.1 was also used to
cluster the back trajectories based on the Euclidean distance method, whose
details and source code can be found on its official website
(<uri>http://meteothink.org/docs/trajstat/index.html</uri>, last access: 31 January
2021).</p>
</sec>
<sec id="Ch1.S2.SS3.SSS4">
  <label>2.3.4</label><title>The calculation of monthly temperature during daytime and night-time</title>
      <p id="d1e655">After defining the SLB day, PTS and PTL, we calculated the monthly mean
temperature during daytime and night-time using the similar method as SW and
LW speeds. First we selected the temperature on SLB days. Second, we
calculated the monthly average of temperature during PTS (PTL) to represent
monthly average temperature during daytime (night-time) in January. Actually,
temperature during daytime (night-time) represents land temperature when SW
(LW) prevails. In order to make it clear and concise, we call it temperature
during PTS (PTL) or land temperature during daytime (night-time) in this
study.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Results</title>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>The variation of SLB day number</title>
      <p id="d1e675">Figure 3 shows the SLB day number in January from 2001 to 2020. As shown,
the SLB day number in January was normally larger than 10. Among these 20 years, there were 25 % of the years whose SLB days in January accounted
for more than half of the month. Note that it does not necessarily mean that
there is no SLB on days that are not SLB days. It is obvious that there was
a slump in the number of SLB days in 2020. The total SLB day number dropped
to only 4 during mega fires, accounting for only 33.33 % of the average
SLB day number during the past 20 years. Also, the year 2012 witnessed a low
SLB day number (6 d) in January. There are a lot of potential influencing
factors for SLB frequency, such as the background wind field (Miller et al.,
2013) and the interruption of other small-scale circulations (Kusaka et al.,
2000). Among all the influencing factors, cloud is one of the most important
because it has a significant effect on in situ solar radiation, which is the direct
cause of TDLS. We will discuss this in the following sections.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3"><?xmltex \currentcnt{3}?><?xmltex \def\figurename{Figure}?><label>Figure 3</label><caption><p id="d1e680">Number of SLB days in January from 2001 to 2020.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f03.png"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>The trends in SW and LW speeds and local air temperature</title>
      <p id="d1e697">The monthly mean SW and LW speeds in January from 2001 to 2020 are shown in
Fig. 4a. As can be seen, there were fluctuations in the trends of both SW
and LW speeds. The SW speed was higher than LW speed, which conformed to
many previous findings (Miller et al., 2013; Zhu et al., 2017). The averages
were calculated as 3.70 m/s for SW speed and 2.86 m/s for LW speed,
respectively. Figure 4b and c show the anomalies of both SW and LW speeds.
In general, LW speed fluctuated more significantly than SW speed did. This
is due to its lower level of kinetic energy which can make it more sensitive
to any potential interruptions from the background meteorological field
(Shen and Zhao, 2020). The negative anomalies of LW speed happened in 2001,
2004, 2008, 2010, 2011, 2015, 2016, 2017, 2018 and 2020. Different from
other years, it is obvious that the negative anomaly in 2020 was higher than
0.6 m/s, which was beyond the multi-years' oscillation range. The anomaly
accounted for 22.3 % of the multi-years' average LW speed. The negative
anomalies of SW speed happened in 2004, 2008, 2009, 2010, 2011, 2013, 2014,
2015, 2017 and 2020 (Fig. 4c). For SW speed, the negative anomaly in 2020
was also obvious, but its value was still within the multi-year oscillation
range. It was higher than 0.5 m/s, accounting for 14.8 % of the
multi-years' average. It is interesting to find that there were obvious
positive anomalies of both SW and LW speeds in 2003, whereas their absolute
values were not the highest. Also, the SLB day number in 2003 was near the
average. We will discuss this further, along with the aerosol emissions
during that year, in the following sections.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><?xmltex \currentcnt{4}?><?xmltex \def\figurename{Figure}?><label>Figure 4</label><caption><p id="d1e702">The trends of SW and LW speeds <bold>(a)</bold>, the LW speed anomaly and land
temperature during night-time <bold>(b)</bold> and the SW speed anomaly and land temperature
during daytime <bold>(c)</bold> based on their monthly average during January from
2001 to 2020.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f04.png"/>

        </fig>

      <?pagebreak page425?><p id="d1e720">It can be seen in Fig. 4b that there were also significant fluctuations in
night-time land temperature over the years. There was a soar in land
temperature during night-time in 2020 which approached nearly 24 <inline-formula><mml:math id="M36" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C. It was nearly 3 <inline-formula><mml:math id="M37" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C higher than the multi-years' average,
exceeding the range of multi-years' oscillation. The fluctuation in land
temperature during daytime was less significant than that during night-time.
There was an obvious positive anomaly in 2020, indicating that the daytime land
temperature was higher than that in normal years. Meanwhile, it was still
within the range of multi-years' oscillation, though the positive anomaly was
obvious. Fire spots have a heating effect on the nearby environment through
either shortwave radiation of light from fires or heat conduction caused by
a temperature gradient. It can be inferred that the mega wild fires in January 2020 contributed to the positive temperature anomalies during PTS (PTL)
through the heating effect of fires, though they might not be the only cause.
The heating effect during mega fires was more significant during night-time
than during daytime, which is probably due to a colder background temperature
field during night-time.</p>
      <p id="d1e742">Basically, the decreased SW (LW) speed revealed that the TDLS during PTS
(PTL) decreased. To be more specific, the temperature difference between the
small regions where the upward stream and downward stream of SLB circulation
lie became smaller during January 2020. Based on Fig. 4b
and c, temperature during PTL seems to be generally negatively related to LW
speed anomaly, while it is obvious that temperature during PTS does not show
any corresponding relationship with SW anomaly.</p>
      <p id="d1e745">In order to be more accurate, we carried out linear regression between
temperature during PTL and LW anomaly and found that they had a negative
linear relationship (<inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:mi>p</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>.02) with each other (Fig. 5). As the
temperature increased by 10 <inline-formula><mml:math id="M39" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C, the LW speed anomaly decreased by
1.52 m/s. The correlation coefficient <inline-formula><mml:math id="M40" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> was 0.52, which was at the medium
level. However, considering the significance level as well as low level of
sample number, it can be concluded that the LW speed is generally negatively
correlated with night-time land temperature. Moreover, their <inline-formula><mml:math id="M41" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> and
significance level could be 0.69 and 0.0012 respectively if we excluded the
only one abnormal point in 2019, which might be caused by some potential
disturbances on coastal SST where the vertical stream of SLB lies.
Considering all these, it can be concluded that the LW speed anomaly is
generally negatively correlated with night-time land temperature. During
night-time, the land is colder than the sea. As the land temperature
increases, the TDLS decreases if the SST of the area where the upward stream
of SLB lies remains relatively stable; the LW speed does too. Briefly, the
good linear relationship reveals that the variation of temperature during
PTL (night-time land temperature) could generally represent the variation of
TDLS during PTL, while the daytime land temperature variation could not
represent the TDLS variation during PTS. In our previous study, we also
found through observation that the daily lowest temperature (DLT) was clearly
negatively related to LW speed, while the SW speed was more related to in situ
downwelling solar radiation rather than merely land temperature (Shen et
al., 2021), which was similar to the findings here. It could be inferred
that although the land temperature during daytime increased during mega fire
events, TDLS was still narrowed during fire events. If we only consider the
land temperature, the SW speed should have increased during fire events
because SW circulation is formed due to warmer land and colder sea.
Consequently, there should be other factors which could cause decreased TDLS
during PTS, which is the direct cause of decreased SW speed. We would
investigate this in the following sections.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5"><?xmltex \currentcnt{5}?><?xmltex \def\figurename{Figure}?><label>Figure 5</label><caption><p id="d1e785">The relationship between LW anomaly and temperature during PTL
based on their monthly average during January from 2001 to 2020.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f05.png"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>The distribution and FRP of fire spots</title>
      <p id="d1e802">Since the heating effect depends largely on the distance between the area
heated and the heat centre, it is necessary to examine the distribution of
fire spots in January over the years, which is shown in Fig. 6. It can be
seen that fire spots are scattered all over the eastern part of Australia in
January over the years. January is the middle of Australian summer, which is
the season when wild fires happen most frequently (Yang et al., 2021). Apart
from 2020, other years also witnessed considerable scattered fire spots all
over the coastal and inland regions. It is obvious that there was an extreme
fire centre in the southeastern corner of Australia with a great density of
fire spots in January 2020. This was exactly the region where the 2019 Australian mega fires mainly happened. To be specific, it was the eastern
corner of the state of<?pagebreak page426?> Victoria and the southeastern corner of the state of New South Wales, which is in agreement with many reports in the media. There was also a great
fire centre in the southeastern corner in 2003, although the scale was
smaller than that in 2020. Considering the distribution of fire spots near
the site, the density of fire spots nearby was not higher than in other
years. Instead, there seems to be more fire spots nearby the site in 2003,
2005, 2006, 2010 and 2013 in the figure. If we restrained the nearby region
to areas of smaller scales, the year 2003 and 2013 rather than 2020 would have the most
nearby fire spots.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6"><?xmltex \currentcnt{6}?><?xmltex \def\figurename{Figure}?><label>Figure 6</label><caption><p id="d1e807">The fire spot distribution in eastern Australia during January
from 2002 to 2020.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f06.png"/>

        </fig>

      <p id="d1e816">There is another possibility that although the fire spots nearby the
site were not more concentrated with great density in 2020 than in other
years, the FRP of fire spots in 2020 was higher. This means that the fire
was greater regardless of the ordinary density of spots, which could also
result in more fire-induced aerosol emissions. So we further examined the
FRP of fire spots in 2020 and those in other years. In order to make it
comparable and verifiable, the time period of data chosen here was the same
as that in Fig. 6. As shown in Fig. 7a, both the nearby and local fire
spots in 2020 were mostly within the lowest FRP range, which was less than
235 MW. There were some sparse fire spots with greater FRP (235–863 MW)
scattered all over the eastern part of Australia. The FRP of the fire centre was higher than the FRP of other fire spots; there were many fire spots
with greater FRP which belonged to the range of 235–863 MW or 863–2194 MW. Figure 7b shows the FRP of all fire spots from 2002–2019. The FRP of
nearby or local fire spots also had the lowest values. As the number
of years increased, the density of fire spots with higher FRP (235–863 MW)
increased significantly, most of which were located in inland areas of
the Australian continent. This indicates that scattered wild fires with low or
medium FRP are common in Australia, but concentrated mega fires are not so
common. There were also some fire spots which belonged to the range of
235–863 MW or 863–2194 MW in 2003, yet the number was less, and the
distribution areas were smaller. Based on Fig. 7, one important point we
found is that there was no discrepancy between FRP of nearby or local fire
spots in 2020 and that of nearby or local fire spots in other years. So the
possibility mentioned above was discarded.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7"><?xmltex \currentcnt{7}?><?xmltex \def\figurename{Figure}?><label>Figure 7</label><caption><p id="d1e822">The fire radiative power (FRP) of total fire spots in eastern
Australia during January 2020 <bold>(a)</bold> and January from 2002 to 2019 <bold>(b)</bold>.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f07.png"/>

        </fig>

      <p id="d1e837">Based on the analysis above, the nearby fire spot density and FRP in 2020
were both at the same level as in other years for local regions near the
site. This implies that the heating<?pagebreak page427?> effect of nearby fire spots did exist in
2020, contributing to the increase of land temperature to some extent
(especially night-time land temperature), but it was not likely the major
cause of the land temperature anomaly. Fluctuation in land temperature might be
caused by combined mechanisms, including some other potential factors. In
other words, the heating effect of fire spots does not necessarily
correspond to the observed air temperature increase. For example, Fig. 4b
and c show that there were negative land temperature anomalies in 2003, but
actually this year witnessed a greater density of nearby or local fire spots.
In a real situation, the scale of SLB is quite small. The fire spots might be
quite a long distance away from the area where the vertical stream of SLB lies,
as a result of which the heating effect is weak.</p>
</sec>
<sec id="Ch1.S3.SS4">
  <label>3.4</label><title>The spatial distribution of aerosols</title>
      <p id="d1e848">Large fires have great aerosol emissions which affect the in situ solar
radiation and then the radiation budget. Based on the basic physical
mechanism of SLB formation, the observed decreased SW and LW speeds
demonstrated the decreased TDLS. As mentioned above, the heating effect of
nearby fire spots was weak and did not become more significant in 2020. So
the more important factors bringing about the decrease of SW and LW speeds
should be more closely related to TDLS rather than the land temperature only. The
TDLS during SLB formation is highly related to the in situ downwelling solar
radiation. As the shortwave radiation increases, the TDLS becomes larger due
to the different heat capacities between land and sea. SW forms and prevails
when TDLS is enough to drive this thermodynamic circulation. During
night-time, the land–sea system is a “heater” for the upper atmosphere as the land and sea both give out heat and undergo energy loss in the form of longwave
radiation. As the outgoing longwave radiation increases, the TDLS also
becomes larger due to the different heat capacities between the land and sea.
Then the LW forms in a similar way to SW.</p>
      <p id="d1e851">Based on discussions above, in situ downwelling solar radiation is a crucial
influencing factor of SW speed. Considering that aerosol is an important
factor affecting in situ downwelling solar radiation, it is necessary for us to
check the temporal and spatial variations of aerosols over the years. Figures 8 and 9 show the spatial distribution of AOD of total aerosols
(TA-AOD) over the years using MERRA-2 and MODIS aerosol products,
respectively. It shows that except for a little overestimation of AOD in the
fire centre in 2020, the overall distribution and value of AOD revealed by
MERRA-2 agreed well with those revealed by MODIS. Both MERRA-2 and MODIS
show that there was a burst of aerosols in the fire centre during January 2003 and 2020, and the latter was much more severe. Especially for the site
learned in this study, the difference of AODs between MERRA-2 (approximately
0.26) and MODIS (approximately 0.29) was very small. Thus, MERRA-2 agreed
well with both MODIS and AERONET in terms of AOD during mega fires, and it
has higher spatial resolution than MODIS. Considering all these aspects and
the focus of the study, we used the MERRA-2 product in the analysis on local
aerosol variations in the following sections. Figure 8 shows that the
background level of TA-AOD was generally low in Australia over the years,
implying that Australia was less polluted as a result of human activities. The TA-AOD
in 2020 increased significantly compared with the average level. It can be
seen that there was a maximum value centre in the southeast corner, which
overlapped the region of the fire spots' centre (Fig. 6). The peripheral area
of the maximum value centre was covered with isopleths, showing the
characteristics of free diffusion of aerosols in the air. There was also a
maximum value centre in 2003 whose scale was smaller, overlapping the
smaller region of the fire centre in 2003. Based on findings from these three
aspects, it can be concluded that the mega fire centre was the main source
of the large amounts of aerosols around the site location. In general, the
TA-AOD was about 240 % of the multi-years' average level at the site,
while the TA-AOD in the fire centre was at a more astonishing level,
accounting for more than 420 % of that at the local site of Brisbane.
Aerosol could significantly affect the in situ downwelling solar radiation through
direct radiative forcing. Turnock et al. (2015) calculated the relationship
between AOD and surface solar radiation (SSR) and found that when the
background value is low over the years, the SSR increases by 10 % as AOD
varies from 0.32 to 0.16. In this study, the TA-AOD increased even more
significantly (240 %), considering the low background value. Normally, when
we talk about the radiative forcing of aerosols in the form of SSR
difference, it means the instantaneous radiative forcing. However, the
formation of SLB is the result of different levels of radiation
accumulations between the land and sea. So the effect of aerosols on the total
in situ downwelling solar radiation can further accumulate in the process of SLB
formation and results in even more significant impacts on the change of
surface temperature.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><?xmltex \def\figurename{Figure}?><label>Figure 8</label><caption><p id="d1e856">The spatial distribution of aerosol optical depth (AOD) of total
aerosols in eastern Australia during January from 2002 to 2020 using the Modern-Era Retrospective analysis for Research and Applications version 2
(MERRA-2) AOD product.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f08.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9" specific-use="star"><?xmltex \currentcnt{9}?><?xmltex \def\figurename{Figure}?><label>Figure 9</label><caption><p id="d1e868">The spatial distribution of aerosol optical depth (AOD) of total
aerosols in eastern Australia during January from 2002 to 2020 using
the Moderate Resolution Imaging Spectroradiometer (MODIS) AOD product.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f09.png"/>

        </fig>

      <?xmltex \floatpos{p}?><fig id="Ch1.F10"><?xmltex \currentcnt{10}?><?xmltex \def\figurename{Figure}?><label>Figure 10</label><caption><p id="d1e879">The monthly cloud optical depth (COD) anomaly and cloud fraction
anomaly at Brisbane Archerfield during January from 2003 to 2020.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f10.png"/>

        </fig>

      <p id="d1e888">Apart from aerosols, clouds could play an even more important role in the
radiation budget. The COD and cloud fraction anomaly at this site are shown
in Fig. 10. The time range was from 2003 to 2020 due to data availability.
It can be seen that both the cloud fraction and COD in 2003 were at an
obvious low level, while both the cloud fraction and COD in 2020 showed a
tiny negative anomaly. Based on the spatial distribution of TA-AOD, both
2003 and 2020 witnessed a soar in TA-AOD at the site, while TA-AOD increased
more significantly in 2020. Figure 3 shows that there was a slump in SLB
number in 2020 but not in 2003, while Fig. 4 shows that there were
positive anomalies of both SW and LW speeds in 2003. Many previous studies
on SLB have pointed out that a high level of in situ downwelling solar radiation is
favourable for SLB formation and SLB speed increase (Shen and Zhao, 2020;
Shen et al., 2021b; Miller et al., 2013). Our previous study in a monsoon
climate region also showed that there was a positive linear relationship
between in situ<?pagebreak page428?> downwelling solar radiation and SW speed (Shen and Zhao, 2020). As we know, the in situ downwelling solar radiation is determined by both cloud and
aerosols through their combined “umbrella effect”. The finding shown in
Figs. 3 and 4 could be explained by the radiative cooling effects of
aerosols and clouds. Although there was a positive anomaly of TA-AOD in 2003,
the COD and cloud fraction were less than the average, offsetting the
aerosols' negative radiative forcing effect. In situ downwelling solar radiation of
the regional sea–land system was still ensured so that the SLB happened with
a normal frequency (Fig. 3) and with an even larger speed (Fig. 4). The
in situ downwelling solar radiation in January 2020 should be lower than the
average, considering the tiny negative anomaly in both COD and cloud
fraction and the significant increase in TA-AOD. The increased radiative
forcing effect of TA-AOD was accumulated during the formation of SW. In
conclusion, during daytime, the negative radiative forcing effect of total
aerosols was the determinant factor to weaken the in situ downwelling solar
radiation, resulting in lower level of TDLS and then decreased SW speed.</p>
      <p id="d1e891">Mega fire events are significant in the way that they emit large amounts of carbonaceous
aerosols, which include OC and BC. The OC is a very good scatter to solar
radiation. Thus, among all the aerosols, OC could be an important
contributor to the weakened TDLS during SW formation. Figure 11 shows the
spatial distribution of OC over the years. The spatial distribution of OC
was also similar to the fire spot distribution, which further confirmed that
the source of great aerosol emissions was the mega fire centre. There were
extreme value centres in the fire centre in both 2003 and 2020. The same as what
we found earlier, it can be seen that the large values spread further in 2020 than 2003, indicating that the fire events were more severe in
2020 than in 2003. Similarly, the background value of OC at the site was low
on average. The specific value of organic carbon AOD (OC-AOD) at the Brisbane site in 2020 was about
630 % of the multi-years' average, which was even higher than that of
total aerosol. This is easy to understand because the fire centre is also
covered with plants and trees, and their combustion can result in
significant amounts of carbonaceous aerosols. Zhang et al. (2017) estimated
the radiative forcing of OC globally using the BCC_AGCM2.0_CUACE/Aero model, which showed that Brisbane was
within the large value area, with high levels of negative radiative forcing
at the top of<?pagebreak page429?> atmosphere. They also attributed this to biomass combustion. Thus,
both total aerosol and OC made great contributions to the SW speed decrease by
decreasing in situ downwelling solar radiation in January 2020.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11" specific-use="star"><?xmltex \currentcnt{11}?><?xmltex \def\figurename{Figure}?><label>Figure 11</label><caption><p id="d1e896">The spatial distribution of aerosol optical depth (AOD) of
organic carbon (OC) in eastern Australia during January from 2002 to 2020.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f11.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F12" specific-use="star"><?xmltex \currentcnt{12}?><?xmltex \def\figurename{Figure}?><label>Figure 12</label><caption><p id="d1e908">The spatial distribution of aerosol optical depth (AOD) of black
carbon (BC) in eastern Australia during January from 2002 to 2020.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f12.png"/>

        </fig>

      <p id="d1e917">The result above is analysed based on the impacts of aerosols on solar
radiation. However there is almost no shortwave radiation during night-time.
Then one question pops up: why was the slump of LW speed more significant?
This indicated that the TDLS was significantly weakened at night in January
2020. While the heating effect of fire spots on night-time land
temperature did exist, which was more significant than that during daytime,
it was not likely the main cause of weakened TDLS based on FRP and fire spot
distribution analysis. We next investigated the spatial distribution of BC
over the years in Fig. 12. It shows that the black carbon AOD (BC-AOD) at the site was about
425 % of the multi-years' average level, with the extreme value centre overlapping the area of that of fire spots' density. Similar to the
distribution of TA-AOD and OC-AOD, the peripheral areas of the maximum value
centre are covered with isopleths, showing the characteristics of free
diffusion. BC is well known as a kind of absorbing aerosol, which is reported
to have a wider range of absorbing band than greenhouse gases, which can
absorb broadband radiation from visible light to infrared wavelength (Zhang
et al., 2017). During the daytime, it can<?pagebreak page430?> absorb solar radiation, longwave
radiation from the warmer land and shortwave radiation from local fires.
During night-time, it has a warming effect on both the atmosphere and Earth's
surface through longwave radiation. As a result, it has a warming effect on
the Earth–atmosphere system, including the surface of the regional land–sea system, so there is a soaring of temperature, shown in Fig. 4b. The soaring
BC during the mega fire heated the local atmosphere, which was like adding a
heater in the air. The heater then gave out downward longwave radiation
to the regional land–sea system. Just like the Sun during daytime, this
could trigger a SW circulation anomaly, weakening LW circulation.
Considering the BC burst during mega fires, there is nothing weird about its
dominant role in the local land temperature increase during night-time. The
mechanism proposed above can be summarized as follows. During night-time, the
formation of LW originates from the process of heat release from both land
and sea. As they both lose heat at different paces due to different heat
capacities, the TDLS is enlarged. During the mega fires, the upper
atmosphere of the regional land–sea system is heated, so that the vertical
temperature gradient is weakened, which is unfavourable for heat release from
both sea and land surfaces. As a result, the TDLS is significantly weakened.</p>
      <p id="d1e920">Another potential contributing accelerator is CO<inline-formula><mml:math id="M42" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, which is also the
product of fires due to the combustion of plants and trees. CO<inline-formula><mml:math id="M43" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is a
kind of greenhouse gas which is likely to be engaged in the same mechanism
as BC to reduce TDLS during night-time, except that CO<inline-formula><mml:math id="M44" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> cannot affect the
downwelling solar radiation. Details about this are not repeated again.
However we should note that the effect of CO<inline-formula><mml:math id="M45" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is based on theoretical
analysis rather than observational verification due to the lack of accurate
observation data. Both BC and CO<inline-formula><mml:math id="M46" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>'s warming effects increase TDLS
during daytime, which partially offsets the strong negative radiative forcing
effect of total aerosols, but their combined warming effect is more
significant during night-time than during daytime. That is most likely the
reason (at least partially) that SW speed had a negative anomaly but was less
significant than LW speed.</p>
      <p id="d1e968">What we discussed above are all factors whose influences were restrained to
a small scale. Although SLB is a small-scale system, it can still be
affected by the variations of signals on a large scale, since the local
temperature is affected by both regional forcing and the variation of the large-scale background temperature field. In our previous study, we weighed their
contributions qualitatively (Shen et al., 2019). In this study, we simply
discuss the potential effect<?pagebreak page431?> of the change in large-scale SST. Hirsch and
Koren (2021) emphasized the effect of record-breaking aerosol emission from
this mega fire on the cooling of the oceanic areas. On a large scale, its average
radiative forcing on sea surface was <inline-formula><mml:math id="M47" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.0 <inline-formula><mml:math id="M48" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 W/m<inline-formula><mml:math id="M49" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>. The
temperature decrease of large-scale sea surface could have negative forcing
on the SST at a regional scale, though the specific temperature variation of
the sea surface where the SLB vertical stream lies might not be the same.</p>
      <p id="d1e994">We summarized all the influencing factors of TDLS at both regional and large
scales in Table 2. Among all these factors, aerosols, BC, OC and CO<inline-formula><mml:math id="M50" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
had direct forcing on TDLS by changing the solar radiation reaching the
regional sea–land system. In contrast, the heating effect of fire spots and
large-scale SST signal had forcing on land temperature and regional SST
respectively, thus further having different forcing effects on TDLS during
daytime and night-time. During the 2019 Australian mega fires, TDLS during daytime
and night-time both decreased under their combined forcing effects, which
could be inferred from the anomalies of SLB speed. Clearly, the directions
of all forcing effects of different factors were the same during night-time.
That was why LW speed decreased much more significantly than SW speed did.
The negative radiative forcing effect of total aerosols was the determinant
cause for TDLS decrease during daytime, which could only be partially offset
by other factors.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T2" specific-use="star"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e1010">Summary of the effect of different factors on TDLS. Factors marked
in bold represent that they are either a weak factor or a potential factor
derived from theoretical analysis but not verified by observation.
</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="5cm"/>
     <oasis:colspec colnum="3" colname="col3" align="center"/>
     <oasis:colspec colnum="4" colname="col4" align="center"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col2" align="center">Influencing factors </oasis:entry>
         <oasis:entry colname="col3">Forcing on daytime TDLS</oasis:entry>
         <oasis:entry colname="col4">Forcing on night=time TDLS</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Large-scale forcing</oasis:entry>
         <oasis:entry colname="col2">Cooling of SST on a large scale (Hirsch and Koren, 2021)</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M51" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M52" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Regional forcing</oasis:entry>
         <oasis:entry colname="col2"><bold>Heating effect of nearby fire spots</bold></oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M53" display="inline"><mml:mo mathvariant="bold">+</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M54" display="inline"><mml:mo mathvariant="bold">-</mml:mo></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Total aerosols</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M55" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M56" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">BC</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M57" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M58" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">OC</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M59" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M60" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"><bold>CO</bold> <inline-formula><mml:math id="M61" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="bold">2</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M62" display="inline"><mml:mo mathvariant="bold">+</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M63" display="inline"><mml:mo mathvariant="bold">-</mml:mo></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S3.SS5">
  <label>3.5</label><title>Source of aerosols</title>
<sec id="Ch1.S3.SS5.SSS1">
  <label>3.5.1</label><title>Fire centre's emission</title>
      <p id="d1e1219">As indicated earlier, the year 2020 did not have advantages over other years in
terms of local and nearby fire spot density and FRP in January. Note that
certain land-cover types could also increase the aerosol emissions. For
example, if there was more combustible land cover such as forests or plants, the fires
could emit more carbonaceous aerosols in the form of smoke. Considering this
possibility, we further checked the latest version of land cover in
Australia online (<uri>http://maps.elie.ucl.ac.be/CCI/viewer/index.php</uri>, last access: 1 April 2021). It was
updated to 2019, which overlapped with the starting time of the 2019 Australian
mega fires. It showed that the areas and density of flora near the site were
stable over the years, implying that the soaring in local aerosols during mega
fires was not likely caused by the change of land cover either.</p>
      <?pagebreak page432?><p id="d1e1225">As Figs. 6, 8, 11 and 12 show, the distributions of fire spots, TA-AOD,
BC-AOD and OC-AOD were quite similar to each other. In the fire centre, both
the density and FRP of fire spots were much higher in January 2020 than
in January of other years, which are all based on distribution
characteristics at a large scale. In order to show the fire situation at the
fire centre more accurately, we magnified the FRP map to restrain the areas
to merely the fire centre, which is shown in Fig. 13. As shown, the fire
spot density was quite high in this region, especially along coastal areas.
Compared with other areas, the fire centre had much more fire spots with
higher FRP. The spots with FRP from 235 to 864 MW were evenly distributed in
all fire areas, surrounded by low FRP spots with high density. There were
quite a few spots with even higher FRP ranging from 864 to 2194 MW, which
could not be found in other peripheral areas (Fig. 7a). In some areas at
the fire centre, we could even find fire spots with FRP ranging from 2194
to 5232 MW. All these distribution characteristics of fire spots suggest
the possibility of large amounts of aerosols including smoke being emitted
into the atmosphere, after which a great concentration gradient in the
horizontal direction is formed between the fire centre and farther areas. Based
on basic chemistry law, irreversible free diffusion would happen in this
process. As the concentration gap increases, the diffusion efficiency also
increases. The distribution of contour lines in Figs. 8, 11 and 12 also
shows the characteristics of free diffusion. A similar mechanism works out for
the spatial distribution of CO<inline-formula><mml:math id="M64" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> during the fire events.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F13"><?xmltex \currentcnt{13}?><?xmltex \def\figurename{Figure}?><label>Figure 13</label><caption><p id="d1e1239">The detailed distribution of fire spots and their FRP in the fire
centre during January 2020.</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f13.png"/>

          </fig>

</sec>
<sec id="Ch1.S3.SS5.SSS2">
  <label>3.5.2</label><title>Analysis on the background wind field</title>
      <p id="d1e1256">Apart from free diffusion, wind is crucial for pollution transport including
aerosols (Walcek, 2002). Also, wind is a key factor of the near-surface
CO<inline-formula><mml:math id="M65" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> distribution (Cao et al., 2017). Zhang et al. (2017) confirmed that
BC could be transported over long distances in mid-latitude areas. The
transport distance of OC was even longer than that of BC. It is necessary
for us to look into the background wind field in order to know the likely
aerosol transport from the fire centre to the site. Yang et al. (2021)
retrieved the average status of the vertical distribution of various
aerosols in southeastern Australia during the 2019 Australian mega fires and
found most of them accumulated under 3 km, which is about 700 hPa. Figure 14
shows the monthly average background wind field based on wind information
at pressure levels from 1000 to 700 hPa in January 2020. The red
cross symbols represent the fire spots in this figure. The average background
wind field clearly revealed the existence of the Southern Hemisphere's
westerlies and a subtropical high. The fire centre was approximately located
at the intersection of the northern boundary of the westerlies and the southwestern
boundary of the subtropical high. Since January is the middle month of
Australian summer, the subtropical high developed quite vigorously, some of
which stretched into the eastern part of the Australian continent. It covered
the areas where most fire spots were located. At a large scale, this caused
quite a hot and dry background meteorological field, which was favourable for
the development and persistence of wild fires. Based on the average status
of wind fields at different pressure levels, the subtropical high and
westerlies together formed a background wind field blowing from the site to
the fire centre, which was unfavourable for the aerosol transport from the fire
centre to the site. However, we should notice that this figure<?pagebreak page433?> merely
describes the monthly average status; it ignores the status of wind flows at
a more accurate fine timescale. In other words, it is still possible that
aerosols from the fire centre were transported to the site within some short
periods in January 2020, contributing to the significant positive
anomalies in AODs shown in Figs. 8, 9, 11 and 12. Based on the specific
dates of SLB days during mega fires identified in the previous section, which
were 4, 14, 20 and 28 January respectively, we divided January 2020 into five short time periods by excluding the identified SLB
days. These five short time periods were all named the “no-SLB period”. We
did the backward trajectory analysis during each no-SLB period to see if the
aerosols from the fire centre were transported to the site with the help of
the background wind field, thus further confirming this period to be a no-SLB period
through all the mechanisms mentioned above. It is easy to understand that
the near-surface concentration of aerosol should be at a high level in
general, not only because it was near the fire spots, but also because it was
within the boundary layer. Considering these aspects, the backward
trajectory analysis was carried out at 500 m over the site. Figure 15a–e
show the wind backward trajectories at this site during the five no-SLB periods respectively. During the no-SLB periods of (a), (c), (d) and (e), the winds
mainly came from the southern Pacific to the east of Australia continent,
which could not transport aerosols from the fire centre. There were winds
coming from the fire centre merely during period (b). The northern edge of
the wind flow beam was quite near the fire centre, and then it went further towards
the northeastern direction in the southern Pacific. When it reached the
general position of the subtropical high, it turned back to the direction of
northwest before finally reaching the site. The high-pressure gradient
between the centre and edge of the subtropical high was opposite to its
moving direction, which might be the cause of its abrupt turning. Although
the southwestern edge of the subtropical high itself had wind flows whose
directions were away from the Australian continent at a monthly average
(Fig. 14), the wind flows from the northern edge of the Southern Hemisphere's
westerlies could still move along its southwestern edge as soon as they
intersected with each other if a smaller timescale and a single level were
considered (Fig. 15b). Figure 15f showed the contributions of the main
backward trajectories based on the whole month's statistics. The main
backward trajectories were calculated after the clustering of all
trajectories, whose number was based on a certain mathematical method like the
calculation of total spatial variation (TSV). More details of this
clustering method and contribution calculation can be found on the official
website of this software (<uri>http://meteothink.org/docs/trajstat/cluster_cal.html</uri>, last access: 31 March 2021). It
can be seen that the wind flows which could potentially bring aerosols from
the fire centre still had a little contribution, which accounted for
9.32 % (2.87 % <inline-formula><mml:math id="M66" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> 6.45 %). In contrast, winds coming from the Pacific
to the east and northeast of the Australian continent dominated the wind
field at the site, whose contributions were 25.09 % and 54.12 %
respectively. Thus, the contribution of wind transport to increasing local
aerosols should be limited, which was only found during one period with a time
length less than 10 d in January 2020. From the perspective of
multi-layers of the atmosphere (0–3 km), the multi-layers of the background wind
fields as a whole did not contribute to the aerosol and CO<inline-formula><mml:math id="M67" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> transport
from the fire centre to the site. Therefore, the soaring of aerosols including
BC and OC at the site should mainly be caused by the combined effect of
combustion in the fire centre and great free diffusion caused by a significant
concentration gradient, with a likely relatively weak contribution of the wind
transport.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F14"><?xmltex \currentcnt{14}?><?xmltex \def\figurename{Figure}?><label>Figure 14</label><caption><p id="d1e1289">Monthly average background wind field based on wind information
at pressure levels from 100 to 700 hPa in January 2020. The red crosses
present fire spots, and the black star represents the site location.</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f14.png"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F15" specific-use="star"><?xmltex \currentcnt{15}?><?xmltex \def\figurename{Figure}?><label>Figure 15</label><caption><p id="d1e1300">The site's wind backward trajectories at 500 m during January 2020. The wind backward trajectories during the first no-SLB period from 1 to 3 January <bold>(a)</bold>, the wind backward trajectories during the second no-SLB period from 5 to 13 January <bold>(b)</bold>, the wind backward trajectories during
the third no-SLB period from 15 to 19 January <bold>(c)</bold>, the wind backward
trajectories during the fourth no-SLB period from 21 to 27 January <bold>(d)</bold>, the
wind backward trajectories during the fifth no-SLB period from 29 to 31 January <bold>(e)</bold> and the contribution of the four main wind clusters based on the wind
backward trajectories during the whole month of January 2020 <bold>(f)</bold>.</p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f15.png"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F16" specific-use="star"><?xmltex \currentcnt{16}?><?xmltex \def\figurename{Figure}?><label>Figure 16</label><caption><p id="d1e1331">The site's wind backward trajectories at 3 km during January 2020. The wind backward trajectories during the first no-SLB period from 1  to 3  January <bold>(a)</bold>, the wind backward trajectories during the second no-SLB period from 5  to 13  January <bold>(b)</bold>, the wind backward trajectories during the
third no-SLB period from 15 to 19 January <bold>(c)</bold>, the wind backward
trajectories during the fourth no-SLB period from 21 to 27 January <bold>(d)</bold>, the
wind backward trajectories during the fifth no-SLB period from 29 to 31
January <bold>(e)</bold> and the contribution of the four main wind clusters based on the wind
backward trajectories during the whole month of January 2020 <bold>(f)</bold>.</p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f16.png"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F17" specific-use="star"><?xmltex \currentcnt{17}?><?xmltex \def\figurename{Figure}?><label>Figure 17</label><caption><p id="d1e1361">The summary of mechanisms containing influencing factors of local
SLB during daytime and night-time. The larger fire cluster represents the
centre of mega fires with a higher concentration of all types of aerosols.
During the Australian mega fires, aerosols were transported to the local site by
means of free diffusion, which was caused by the great concentration gap of
aerosols between the fire centre and the local site. The width of arrows of
“shortwave radiation” represents the magnitude of shortwave radiation.</p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://acp.copernicus.org/articles/22/419/2022/acp-22-419-2022-f17.png"/>

          </fig>

      <p id="d1e1370">Most aerosols are generally within the atmospheric boundary layer under normal
conditions, while this might be different under the situation during mega fires
considering the boost of vertical movement due to the great heat release from
fires and astonishing amounts of aerosol emissions. Smoke, as a kind of
unique aerosol emission produced in great amounts during fire events, could be
essential to SW and LW speed anomalies due to its absorptive radiative
properties, making it particularly valuable to examine its transport
individually. Yang et al. (2021) analysed the vertical distribution of smoke
on southeastern parts of Australia, which included the fire centre and the
site, and found that the smoke accumulated at 3 km generally. Considering
this aspect, we also did the backward trajectory analysis at 3 km, whose time
division was the same as that at 500 m. The results are shown in Fig. 16.
As shown, the wind flow scattered more evenly at 3 km than at 500 m. There
were more wind flows coming from the southwestern direction of the site.
This is probably due to the fact that the magnitude and stretching area of
westerlies are larger in the upper atmosphere than in layers closer to the
surface. During period (a), (b) and (e), there were clusters of wind flows coming
from the fire centre or near the fire centre, which could bring aerosols to
the site. Specifically, there were wind flows penetrating the fire centre directly during period (a) and (e), while the wind flows during period (b) are
only adjacent to the north edge of fire centre. Since the period (b) was the
longest among all no-SLB periods, it did not necessarily mean that the
wind's aerosol transport effect during this period was less than that
during other periods, although the wind flows were not directly from the fire
centre. Their moving paths were similar to those of wind flows in
Fig. 15b, which all showed an abrupt turn on the Pacific to the southeast
of the site. This is probably because the Southern Hemisphere's
subtropical high developed to be quite strong during the middle of<?pagebreak page435?> summer,
making the pressure gradient exist both at 500 m and 3 km (Fig. 14).
Figure 16f shows the contribution of wind flows on monthly average, whose
clustering number was also 4. There were four main directions of wind
flows, whose contributions were 28.67 %, 21.86 %, 11.47 % and 37.99 %
respectively. For clarity, we define these four main wind
flows as wind flow clusters. The wind flow clusters with contributions of
21.86 % and 11.47 % were generally adjacent to the north edge of the
fire centre, which contained a contribution of wind flows from the fire
centre. Due to the clustering limitation of Meteoinfo, we could not extract
the specific contributions of wind flows blowing directly from the fire centre from the total contributions of wind flow clusters (21.86 % and
11.47 %). But based on analysis from shorter time periods, their
contributions were larger than those at 500 m because there were more no-SLB periods with wind flows blowing from the fire centre.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S4" sec-type="conclusions">
  <label>4</label><title>Summary and discussion</title>
      <p id="d1e1383">In this study, the SLB day number, SLB speed, daytime temperature and
night-time temperature at Brisbane Archerfield in January were calculated
from 2001 to 2020 using observation data from automatic meteorological
stations. We have taken three steps in total to exclude the interference of
winds from synoptic-scale systems in order to extract the real SLB signals.
First, we used a SRWF method to verify the OE-SLB and then extracted the SLB
signal from original observation. Second, we defined the SLB days as when the whole
SLB circulation is most significant and integrated. Finally, we used SLB
signals during PTS (PTL) on SLB days to calculate the monthly average of SW
(LW) speed. In the corresponding months over the years, regional cloud
fraction, COD, fire spot and FRP distribution in Australia were revealed
using the MODIS product. Comparison with MODIS and site observations confirmed
the good quality of the MERRA-2 product to reveal the variation of aerosols
during mega fires. Consequently, aerosols' distributions in eastern
Australia were revealed in the form of AOD using the MERRA-2 product, including
that of total aerosols, OC and BC. Furthermore, the background wind field
and backward wind trajectory were analysed using the ERA5 product and HYSPLIT
respectively. The main findings of this study are as follows.
<list list-type="order"><list-item>
      <p id="d1e1388">There was a significant slump in SLB day number (33.3 % of the average
level) and LW speed (decreased by 22.3 % of the average level) at the
site. While SW speed also decreased by 14.8 % of the average level, it was
not significant.</p></list-item><list-item>
      <p id="d1e1392">There was a burst of aerosols at the site, with TA-AOD, BC-AOD and
OC-AOD being approximately 240 %, 425 % and 630 % of the multi-years'
averages. TDLS is a direct cause of SLB, while other factors influence SLB
through their effects on TDLS. The variation of night-time land temperature
could generally represent the variation of TDLS during night-time, while TDLS
during daytime could not be simply represented by daytime land temperature.
Specifically, the significant aerosol burst was mainly responsible for the
decrease of SW speed. The burst of BC at the site, as well as the large-scale
SST decrease during mega fires, was mainly responsible for the slump of LW
speed. CO<inline-formula><mml:math id="M68" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emitted by<?pagebreak page436?> nearby fire spots or transmitted from the fire
centre was a potential and weak factor of the slump of LW speed. The
heating effect of nearby fires on TDLS was weak during both daytime and
night-time.</p></list-item><list-item>
      <p id="d1e1405">Emissions from the fire centre were mainly responsible for the local
positive aerosol anomaly during mega fires. On average, the background wind
fields from the near surface to 3 km were unfavourable for aerosol and CO<inline-formula><mml:math id="M69" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
transport. But there was likely aerosol and CO<inline-formula><mml:math id="M70" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> transport through
a large-scale wind field at single levels during shorter periods within
January 2020. Specifically, the wind flow transport at 3 km was stronger
than that at 500 m, which was particularly important for smoke transport
since the smoke from fires gathered at the same level. In general, free
diffusion due to a large concentration gradient was mainly responsible for
aerosol transport and the potential CO<inline-formula><mml:math id="M71" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> transport, while the effect of
background wind field played a secondary role.</p></list-item></list>
In order to make the influencing factors of SLB clear and concise, we
summarized their potential mechanisms in a local sea–land system (Fig. 17).
During the daytime, a negative anomaly of SW speed was found at the site in
January 2020 when the Australian mega fires were most intense. The local
cloud fraction and COD were almost on an average level, while there were significantly more aerosols during mega fires, which mainly came from the fire centre by free
diffusion. They significantly weakened the in situ downwelling solar radiation, thus
further narrowing the TDLS, which was the direct cause of SW speed decrease.
BC and CO<inline-formula><mml:math id="M72" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> heated the atmosphere and warmed the earth–atmosphere system
by longwave radiation from the heated atmosphere. The warming effect of BC and
CO<inline-formula><mml:math id="M73" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, the decrease of SST at a large scale and the weak heating effect
of nearby fire spots partially offset the effect of aerosols on narrowing
TDLS, making the negative SW speed anomaly not exceed the multi-years'
oscillation range. During night-time, the heating effect of nearby fire spots
was still weak but more significant than that during daytime. The warming
effect of BC and CO<inline-formula><mml:math id="M74" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> was like adding a heater in the atmosphere, which
triggered a SW circulation anomaly, thus resulting in a slump in LW speed. The
decrease of SST at a large scale further boosted the decrease of LW speed.
The slumps in both SLB speed and SLB day number could help to accumulate the
local aerosols (Shen and Zhao, 2020), which further catalysed the physical
processes mentioned in the mechanism and finally formed a positive feedback
mechanism under a scenario of mega fires.</p>
      <p id="d1e1463">Essentially, a narrowed TDLS was the direct cause of SLB speed decrease, which
was affected by various factors in the form of either shortwave radiation or
longwave radiation. It not only weakened the SLB speed, but also brought
about a slump in the SLB day number. The in situ radiation, including both longwave and
shortwave radiation reaching the ground, has a direct impact on the TDLS
considering the basic physical mechanism of SLB formation. Note that the
specific weather condition, cloud fraction, COD and the type of clouds and
aerosols could all affect the in situ radiation. Apart from in situ radiation, the heat
release in urban areas, heat waves, heating effect of nearby heat sources,
large-scale signals of SST and land surface temperature variation could all
affect TDLS by changing either the local land temperature or SST. The
large-scale signals of temperature variations could be caused by either
natural variability or human variability. Normally, SLB forms when the TDLS
is obvious and the background wind field is mild. So the condition of a large-scale wind field such as a monsoon is also an important influencing factor of
SLB. Apart from the slump in both SLB day number and LW speed during mega
fire events, there were smaller fluctuations in both of their trends, which
need to be studied further in future.</p>
</sec>

      
      </body>
    <back><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e1471">The Dynamic Land Cover Dataset (DLCD)
can be accessed thorough Geoscience Australia
(<uri>http://www.ga.gov.au/scientific-topics/earth-obs/accessing-satellite-imagery/landcover</uri>,
Lymburner et al., 2015). MERRA-2 Reanalysis data can be accessed through
the NASA Global Modeling and Assimilation Office
(<uri>https://gmao.gsfc.nasa.gov/reanalysis/MERRA-2/</uri>, Global Modeling and
Assimilation Office (GMAO), 2015). MODIS observation data can be accessed
through the Earthdata centre managed by NOAA (<uri>https://earthdata.nasa.gov/search?q=MCD06</uri>, MODIS Atmosphere Science Team, 2015; <uri>http://earthdata.nasa.gov/search?q=MOD08</uri>, Hubanks et al., 2015). GDAS data used
in HYSPLIT data are accessible through the NOAA READY website (<uri>http://www.ready.noaa.gov</uri>, NOAA, 2016). Fire spot and FRP data can be
accessed from the MODIS MCD14 product managed by NOAA (<uri>https://earthdata.nasa.gov/search?q=MCD14</uri>, The Land, Atmosphere Near real-time Capability for EOS MODIS (LANCEMODIS) Team, 2015). The wind and
temperature observation data from the NOAA global observation network can be
accessed on NOAA's official website (<uri>http://www1.ncdc.noaa.gov/pub/data/noaa/</uri>, Baldwin et al., 2020). The ERA5 data can be accessed
through the official website of the Copernicus project
(<uri>https://climate.copernicus.eu/climate-reanalysis</uri>, Hersbach et al., 2021).</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e1502">CZ and LS developed the
ideas and designed the study. LS, XY, YY and PZ contributed to collection
and analyses of data. LS and XY performed the analysis and prepared the
manuscript. CZ supervised and modified the manuscript. All authors made
substantial contributions to this work.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e1508">The contact author has declared that neither they nor their co-authors have any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <?pagebreak page437?><p id="d1e1514">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e1520">This work was supported by the Ministry
of Science and Technology of China National Key Research and Development
Program (2019YFA0606803), the National Natural Science Foundation of China
(41925022), the State Key Laboratory of Earth Surface Processes and
Resources Ecology and the Fundamental Research Funds for the Central
Universities.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e1525">This research has been supported by the National Key Research and Development Program of China (grant no. 2019YFA0606803) and the National Outstanding Youth Science Fund Project of the National Natural Science Foundation of China (grant no. 41925022).</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e1531">This paper was edited by Jianping Huang and reviewed by two anonymous referees.</p>
  </notes><ref-list>
    <title>References</title>

      <ref id="bib1.bib1"><label>1</label><?label 1?><mixed-citation>Albrecht, B. A.: Aerosols, Cloud Microphysics, and Fractional Cloudiness,
Science, 245, 1227–1230, <ext-link xlink:href="https://doi.org/10.1126/science.245.4923.1227" ext-link-type="DOI">10.1126/science.245.4923.1227</ext-link>,
1989.</mixed-citation></ref>
      <ref id="bib1.bib2"><label>2</label><?label 1?><mixed-citation>Baldwin, R., Wright, V., Anders, D. D., Brinegar, D., Lott, N., Jones, P., Smith, F., and Boreman, B.: The FCC Integrated Surface Hourly Database, A New Resource of Global Climate Data [data set], Data center of NOAA, available at: <uri>http://www1.ncdc.noaa.gov/pub/data/noaa/</uri> (last access: 31 March 2021), 2020.</mixed-citation></ref>
      <ref id="bib1.bib3"><label>3</label><?label 1?><mixed-citation>Cao, L. Z., Chen, X., Zhang, C., Kurban, A., Yuan, X. L., Pan, T., and
Maeyer, P.: The temporal and spatial distributions of the near-surface
CO<inline-formula><mml:math id="M75" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations in central Asia and analysis of their controlling
factors, Atmosphere, 8, 1–14, <ext-link xlink:href="https://doi.org/10.3390/atmos8050085" ext-link-type="DOI">10.3390/atmos8050085</ext-link>, 2017.</mixed-citation></ref>
      <ref id="bib1.bib4"><label>4</label><?label 1?><mixed-citation>Charlson, R. J., Schwartz, S. E., Hales, J. M., Cess, R. D., Coakley, J. A.,
Hansen, J. E., and Hofmann, D. J.: Climate forcing by anthropogenic
aerosols, Science, 255, 423–430, 1992.</mixed-citation></ref>
      <ref id="bib1.bib5"><label>5</label><?label 1?><mixed-citation>Chuang, C. C., Penner, J. E., Prospero, J. M., Grant, K. E., Rau, G. H., and
Kawamoto, K.: Cloud susceptibility and the first aerosol indirect forcing:
Sensitivity to black carbon and aerosol concentrations, J. Geophys.
Res.-Atmos., 107, 4564, <ext-link xlink:href="https://doi.org/10.1029/2000JD000215" ext-link-type="DOI">10.1029/2000JD000215</ext-link>, 2002.</mixed-citation></ref>
      <ref id="bib1.bib6"><label>6</label><?label 1?><mixed-citation>Cuxart, J., Jiménez, M. A., Prtenjak, M. T., and Grisogono, B.: Study of a
sea-breeze case through momentum, temperature, and turbulence budgets, J.
Appl. Meteorol. Climatol., 53, 2589–2609, 2014.</mixed-citation></ref>
      <ref id="bib1.bib7"><label>7</label><?label 1?><mixed-citation>Garrett, T. J. and Zhao, C.: Increased Arctic cloud longwave emissivity
associated with pollution from mid-latitudes, Nature, 440, 787–789,
<ext-link xlink:href="https://doi.org/10.1038/nature04636" ext-link-type="DOI">10.1038/nature04636</ext-link>, 2006.</mixed-citation></ref>
      <ref id="bib1.bib8"><label>8</label><?label 1?><mixed-citation>Giglio, L., Schroeder, W., and Justice, C. O.: The collection 6 MODIS active
fire detection algorithm and fire products, Remote Sens. Environ., 178,
31–41, <ext-link xlink:href="https://doi.org/10.1016/j.rse.2016.02.054" ext-link-type="DOI">10.1016/j.rse.2016.02.054</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib9"><label>9</label><?label 1?><mixed-citation>Global Modeling and Assimilation Office (GMAO): MERRA-2 tavgM_2d_aer_Nx: 2d, Monthly mean, Time-averaged, Single-Level, Assimilation, Aerosol Diagnostics V5.12.4, Greenbelt, MD, USA, Goddard Earth Sciences Data and Information Services Center (GES DISC) [data set], <ext-link xlink:href="https://doi.org/10.5067/FH9A0MLJPC7N" ext-link-type="DOI">10.5067/FH9A0MLJPC7N</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib10"><label>10</label><?label 1?><mixed-citation>Grandey, B. S., Lee, H.-H., and Wang, C.: Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires, Atmos. Chem. Phys., 16, 14495–14513, <ext-link xlink:href="https://doi.org/10.5194/acp-16-14495-2016" ext-link-type="DOI">10.5194/acp-16-14495-2016</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib11"><label>11</label><?label 1?><mixed-citation>Han, W., Li, Z., Wu, F., Zhang, Y., Guo, J., Su, T., Cribb, M., Fan, J., Chen, T., Wei, J., and Lee, S.-S.: The mechanisms and seasonal differences of the impact of aerosols on daytime surface urban heat island effect, Atmos. Chem. Phys., 20, 6479–6493, <ext-link xlink:href="https://doi.org/10.5194/acp-20-6479-2020" ext-link-type="DOI">10.5194/acp-20-6479-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib12"><label>12</label><?label 1?><mixed-citation>Hersbach, H., Bell, B., Berrisford, P., Biavati, G., Horányi, A., Muñoz Sabater, J., Nicolas, J., Peubey, C., Radu, R., Rozum, I., Schepers, D., Simmons, A., Soci, C., Dee, D., and Thépaut, J.-N.: ERA5 monthly averaged data on single levels from 1979 to present, Copernicus Climate Change Service (C3S) Climate Data Store (CDS) [data set], available at: <uri>https://climate.copernicus.eu/climate-reanalysis</uri> (last access: 31 March 2021), 2019.</mixed-citation></ref>
      <ref id="bib1.bib13"><label>13</label><?label 1?><mixed-citation>Hirsch, E. and Koren, I.: Record-breaking aerosol levels explained by smoke
injection into the stratosphere, Science, 371, 1269–1274,
<ext-link xlink:href="https://doi.org/10.1126/science.abe1415" ext-link-type="DOI">10.1126/science.abe1415</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bib14"><label>14</label><?label 1?><mixed-citation>Hubanks, P., Platnick, S., King, M., and Ridgway, B.:  MODIS Atmosphere L3 Monthly Product. NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data set], USA, <ext-link xlink:href="https://doi.org/10.5067/MODIS/MOD08_M3.061" ext-link-type="DOI">10.5067/MODIS/MOD08_M3.061</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib15"><label>15</label><?label 1?><mixed-citation>IPCC: Intergovernmental Panel on Climate Change, Climate Change 2013: The Physical
Science Basis, Contribution of Working Group I to the Fifth Assessment
Report of the Intergovernmental Panel on Climate Change, Cambridge
Univ. Press, Cambridge, UK, and New York, 1535 pp., 2013.</mixed-citation></ref>
      <ref id="bib1.bib16"><label>16</label><?label 1?><mixed-citation>Jacobson, M. Z.: Strong radiative heating due to the mixing state of black
carbon in atmospheric aerosols, Nature, 409, 695–697, 2001.</mixed-citation></ref>
      <ref id="bib1.bib17"><label>17</label><?label 1?><mixed-citation>Jacobson, M. Z.: Effects of biomass burning on climate, accounting for heat
and moisture fluxes, black and brown carbon, and cloud absorption effects,
J. Geophys. Res.-Atmos., 119, 8980–9002,
<ext-link xlink:href="https://doi.org/10.1002/2014jd021861" ext-link-type="DOI">10.1002/2014jd021861</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bib18"><label>18</label><?label 1?><mixed-citation>Jia, S. Q., Jing, J. L., Ju, E. D., and Chi, W. B.: Discussions on the
temperature and pressure fields in a mega forest fire zone, J. Nort. Fore.
Uni., 15, 226–232, <ext-link xlink:href="https://doi.org/10.13759/j.cnki.dlxb.1987.s4.028" ext-link-type="DOI">10.13759/j.cnki.dlxb.1987.s4.028</ext-link>, 1987.</mixed-citation></ref>
      <ref id="bib1.bib19"><label>19</label><?label 1?><mixed-citation>Kloss, C., Berthet, G., Sellitto, P., Ploeger, F., Bucci, S., Khaykin, S., Jégou, F., Taha, G., Thomason, L. W., Barret, B., Le Flochmoen, E., von Hobe, M., Bossolasco, A., Bègue, N., and Legras, B.: Transport of the 2017 Canadian wildfire plume to the tropics via the Asian monsoon circulation, Atmos. Chem. Phys., 19, 13547–13567, <ext-link xlink:href="https://doi.org/10.5194/acp-19-13547-2019" ext-link-type="DOI">10.5194/acp-19-13547-2019</ext-link>, 2019.</mixed-citation></ref>
      <ref id="bib1.bib20"><label>20</label><?label 1?><mixed-citation>Kusaka, H., Kimura, F., Hirakuchi, H., and Mizutori, M.: The effects of
land-use alteration on the sea breeze and daytime heat island in the Tokyo
metropolitan area, J. Meteorol. Soc. Jpn., 78, 405–420,
<ext-link xlink:href="https://doi.org/10.2151/jmsj1965.78.4_405" ext-link-type="DOI">10.2151/jmsj1965.78.4_405</ext-link>, 2000.</mixed-citation></ref>
      <ref id="bib1.bib21"><label>21</label><?label 1?><mixed-citation>Li, J. W., Yang, L. Q., Li, X. W., and Zheng, H. R.: Visualization of local
wind field based forest-fire's forecast modelin<?pagebreak page438?>g for transportation
planning, Multimed. Tools. Appl., 1, 1–15,
<ext-link xlink:href="https://doi.org/10.1007/s11042-016-3357-7" ext-link-type="DOI">10.1007/s11042-016-3357-7</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib22"><label>22</label><?label 1?><mixed-citation>Luhar, A. K., Mitchell, R. M., Meyer, C. P., Qin, Y., Campbell, S., Gras, J.
L., and Parry, D.: Biomass burning emissions over northern Australia
constrained by aerosol measurements: II–Model validation, and impacts on air quality and radiative
forcing, Atmos. Environ., 42, 1647–1664,
<ext-link xlink:href="https://doi.org/10.1016/j.atmosenv.2007.12.040" ext-link-type="DOI">10.1016/j.atmosenv.2007.12.040</ext-link>, 2008.</mixed-citation></ref>
      <ref id="bib1.bib23"><label>23</label><?label 1?><mixed-citation>Lymburner, L., Tan, P., McIntyre, A., Thankappan, M., and Sixsmith, J.:
Dynamic Land Cover Dataset Version 2.1. Geoscience Australia, Canberra,
available at: <uri>http://pid.geoscience.gov.au/dataset/ga/83868</uri> (last access: 31
January 2021), 2015.</mixed-citation></ref>
      <ref id="bib1.bib24"><label>24</label><?label 1?><mixed-citation>Ma, Y., Gao, R. Z., and Miao, S. G.: Impacts of urbanization on summer-time
SLB circulation in Qingdao, Acta. Sci. Circumst., 33, 1690–1696,
<ext-link xlink:href="https://doi.org/10.13671/j.hjkxxb.2013.06.030" ext-link-type="DOI">10.13671/j.hjkxxb.2013.06.030</ext-link>, 2013.</mixed-citation></ref>
      <ref id="bib1.bib25"><label>25</label><?label 1?><mixed-citation>Mallet, M. D., Desservettaz, M. J., Miljevic, B., Milic, A., Ristovski, Z. D., Alroe, J., Cravigan, L. T., Jayaratne, E. R., Paton-Walsh, C., Griffith, D. W. T., Wilson, S. R., Kettlewell, G., van der Schoot, M. V., Selleck, P., Reisen, F., Lawson, S. J., Ward, J., Harnwell, J., Cheng, M., Gillett, R. W., Molloy, S. B., Howard, D., Nelson, P. F., Morrison, A. L., Edwards, G. C., Williams, A. G., Chambers, S. D., Werczynski, S., Williams, L. R., Winton, V. H. L., Atkinson, B., Wang, X., and Keywood, M. D.: Biomass burning emissions in north Australia during the early dry season: an overview of the 2014 SAFIRED campaign, Atmos. Chem. Phys., 17, 13681–13697, <ext-link xlink:href="https://doi.org/10.5194/acp-17-13681-2017" ext-link-type="DOI">10.5194/acp-17-13681-2017</ext-link>, 2017.</mixed-citation></ref>
      <ref id="bib1.bib26"><label>26</label><?label 1?><mixed-citation>McCoy, D. T. and Hartmann, D. L.: Observations of a substantial
cloud-aerosol indirect effectduring the 2014–2015
Bárðarbunga-Veiðivötnssure eruption in Iceland, Geophys.
Res. Lett., 42, 10409–10414, <ext-link xlink:href="https://doi.org/10.1002/2015GL067070" ext-link-type="DOI">10.1002/2015GL067070</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib27"><label>27</label><?label 1?><mixed-citation>Meyer, C. P., Luhar, A. K., and Mitchell, R. M.: Biomass burning emissions
over northern Australia constrained by aerosol measurements: I – Modelling
the distribution of hourly emissions, Atmos. Environ., 42, 1629–1646,
<ext-link xlink:href="https://doi.org/10.1016/j.atmosenv.2007.10.089" ext-link-type="DOI">10.1016/j.atmosenv.2007.10.089</ext-link>, 2008.</mixed-citation></ref>
      <ref id="bib1.bib28"><label>28</label><?label 1?><mixed-citation>Miller, S. T. K., Keim, B. D., Talbot, R. W., and Mao, H.: Sea breeze:
Structure, forecasting, and impacts, Rev. Geophys., 41, 1011,
<ext-link xlink:href="https://doi.org/10.1029/2003RG000124" ext-link-type="DOI">10.1029/2003RG000124</ext-link>, 2013.</mixed-citation></ref>
      <ref id="bib1.bib29"><label>29</label><?label 1?><mixed-citation>Mitchell, R. M., O'Brien, D. M., and Campbell, S. K.: Characteristics and
radiative impact of the aerosol generated by the Canberra firestorm of
January 2003, J. Geophys. Res.-Atmos., 111, D02204,
<ext-link xlink:href="https://doi.org/10.1029/2005jd006304" ext-link-type="DOI">10.1029/2005jd006304</ext-link>, 2006.</mixed-citation></ref>
      <ref id="bib1.bib30"><label>30</label><?label 1?><mixed-citation>Mitchell, R. M., Forgan, B. W., Campbell, S. K., and Qin, Y.: The
climatology of Australian tropical aerosol: Evidence for regional
correlation, Geophys. Res. Lett., 40, 2384–2389,
<ext-link xlink:href="https://doi.org/10.1002/grl.50403" ext-link-type="DOI">10.1002/grl.50403</ext-link>, 2013.</mixed-citation></ref>
      <ref id="bib1.bib31"><label>31</label><?label 1?><mixed-citation>MODIS Atmosphere Science Team: MODIS Cloud Properties Level 3 Monthly Product, NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data set], USA, <ext-link xlink:href="https://doi.org/10.5067/MODIS/MCD06COSP_M3_MODIS.061" ext-link-type="DOI">10.5067/MODIS/MCD06COSP_M3_MODIS.061</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib32"><label>32</label><?label 1?><mixed-citation>Nai, F. B., Zhao, L. N., and Wu, J. R.: Impacts of sea-land and
mountain-valley circulations on the air pollution in Beijing-Tianjin-Hebei:
a case study, Environ. Pollut., 234, 429–438,
<ext-link xlink:href="https://doi.org/10.1016/j.envpol.2017.11.066" ext-link-type="DOI">10.1016/j.envpol.2017.11.066</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bib33"><label>33</label><?label 1?><mixed-citation>NOAA: GDAS – Daily Tar Files (1<inline-formula><mml:math id="M76" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> by 1<inline-formula><mml:math id="M77" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>), NCEI's NOAA National Operational Model Archive and Distribution System (NOMADS) [data set], available at: <uri>ftp://ftp.arl.noaa.gov/pub/archives/gdas1</uri> (last access: 31 March 2021), 2016.</mixed-citation></ref>
      <ref id="bib1.bib34"><label>34</label><?label 1?><mixed-citation>Ohneiser, K., Ansmann, A., Baars, H., Seifert, P., Barja, B., Jimenez, C., Radenz, M., Teisseire, A., Floutsi, A., Haarig, M., Foth, A., Chudnovsky, A., Engelmann, R., Zamorano, F., Bühl, J., and Wandinger, U.: Smoke of extreme Australian bushfires observed in the stratosphere over Punta Arenas, Chile, in January 2020: optical thickness, lidar ratios, and depolarization ratios at 355 and 532 nm, Atmos. Chem. Phys., 20, 8003–8015, <ext-link xlink:href="https://doi.org/10.5194/acp-20-8003-2020" ext-link-type="DOI">10.5194/acp-20-8003-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib35"><label>35</label><?label 1?><mixed-citation>Portin, H., Mielonen, T., Leskinen, A., Arola, A., Pärjälä, E.,
Romakkaniemi, S., Laaksonen, A., Lehtinen, K. E. J., and Komppula, M.:
Biomass burning aerosols observed in Eastern Finland during the Russian
wildfires in summer 2010 e Part 1: In-situ aerosol characterization, Atmos.
Environ., 47, 269–278, http:// <ext-link xlink:href="https://doi.org/10.1016/j.atmosenv.2011.10.067" ext-link-type="DOI">10.1016/j.atmosenv.2011.10.067</ext-link>, 2012.</mixed-citation></ref>
      <ref id="bib1.bib36"><label>36</label><?label 1?><mixed-citation>Rajib, P. and Heekwa, L.: Estimation of the effective zone of sea/land
breeze in a coastal area, Atmos. Pollut. Res., 2, 106–115,
<ext-link xlink:href="https://doi.org/10.5094/APR.2011.013" ext-link-type="DOI">10.5094/APR.2011.013</ext-link>, 2010.</mixed-citation></ref>
      <ref id="bib1.bib37"><label>37</label><?label 1?><mixed-citation>Ramana, M. V., Ramanathan, V., Feng, Y., Yoon, S. C., Kim, S. W.,
Carmichael, G. R., and Schauer, J. J.: Warming influenced by the ratio of
black carbon to sulphate and the black-carbon source, Nat. Geosci., 1,
542–545, <ext-link xlink:href="https://doi.org/10.1038/NGEO918" ext-link-type="DOI">10.1038/NGEO918</ext-link>, 2010.</mixed-citation></ref>
      <ref id="bib1.bib38"><label>38</label><?label 1?><mixed-citation>Sarker, A., Saraswat, R. S., Chandrasekar, A.: Numerical study of the
effects of urban heat island on the characteristic features of the sea
breeze circulation, P. Indian As.-Eng. Sci., 107, 127–137, 1998.</mixed-citation></ref>
      <ref id="bib1.bib39"><label>39</label><?label 1?><mixed-citation>Shen, L. X. and Zhao, C. F.: Dominance of Shortwave Radiative Heating in
the Sea-Land Breeze Amplitude and its Impacts on Atmospheric Visibility in
Tokyo, Japan, J. Geophys. Res.-Atmos., 125, 1–19,
<ext-link xlink:href="https://doi.org/10.1029/2019jd031541" ext-link-type="DOI">10.1029/2019jd031541</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib40"><label>40</label><?label 1?><mixed-citation>Shen, L. X., Zhao, C. F., Ma, Z. S., Li, Z. Q., Li, J. P., and Wang, K. C.:
Observed decrease of summer sea-land breeze in Shanghai from 1994 to 2014
and its association with urbanization, Atmos. Res., 227, 198–209,
<ext-link xlink:href="https://doi.org/10.1016/j.atmosres.2019.05.007" ext-link-type="DOI">10.1016/j.atmosres.2019.05.007</ext-link>, 2019.</mixed-citation></ref>
      <ref id="bib1.bib41"><label>41</label><?label 1?><mixed-citation>Shen, L. X., Zhao, C. F., and Yang, X. C.: Insight Into the Seasonal
Variations of the Sea-Land Breeze in Los Angeles With Respect to the Effects
of Solar Radiation and Climate Type, J. Geophys. Res.-Atmos., 126, 1–21,
<ext-link xlink:href="https://doi.org/10.1029/2019jd033197" ext-link-type="DOI">10.1029/2019jd033197</ext-link>, 2021a.</mixed-citation></ref>
      <ref id="bib1.bib42"><label>42</label><?label 1?><mixed-citation>Shen, L. X., Zhao, C. F., and Yang, X. C.: Climate-Driven Characteristics of
Sea-Land Breezes Over the Globe, Geophys. Res. Lett., 48, 1–10,
<ext-link xlink:href="https://doi.org/10.1029/2020GL092308" ext-link-type="DOI">10.1029/2020GL092308</ext-link>, 2021b.</mixed-citation></ref>
      <ref id="bib1.bib43"><label>43</label><?label 1?><mixed-citation>Sun, R. Y., Krueger, S. K., Jenkins, M. A., Zulauf, M. A., and Charney, J. J.: The importance of fire–atmosphere coupling and boundary-layer turbulence to wildfire spread, Int. J. Wildland Fire., 18, 50–60, <ext-link xlink:href="https://doi.org/10.1071/WF07072" ext-link-type="DOI">10.1071/WF07072</ext-link>, 2009.</mixed-citation></ref>
      <ref id="bib1.bib44"><label>44</label><?label 1?><mixed-citation>The Land, Atmosphere Near real-time Capability for EOS MODIS (LANCEMODIS) Team:  MODIS/Aqua Terra Thermal Anomalies/Fire locations 1 km FIRMS V006 NRT (Vector data), NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data set], USA, <ext-link xlink:href="https://doi.org/10.5067/FIRMS/MODIS/MCD14DL.NRT.006" ext-link-type="DOI">10.5067/FIRMS/MODIS/MCD14DL.NRT.006</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib45"><label>45</label><?label 1?><mixed-citation>Torres, O., Jethva, H., Ahn, C., Jaross, G., and Loyola, D. G.: TROPOMI aerosol products: evaluation and observations of synoptic-scale carbonaceous aerosol plume<?pagebreak page439?>s during 2018–2020, Atmos. Meas. Tech., 13, 6789–6806, <ext-link xlink:href="https://doi.org/10.5194/amt-13-6789-2020" ext-link-type="DOI">10.5194/amt-13-6789-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib46"><label>46</label><?label 1?><mixed-citation>Turnock, S. T., Spracklen, D. V., Carslaw, K. S., Mann, G. W., Woodhouse, M. T., Forster, P. M., Haywood, J., Johnson, C. E., Dalvi, M., Bellouin, N., and Sanchez-Lorenzo, A.: Modelled and observed changes in aerosols and surface solar radiation over Europe between 1960 and 2009, Atmos. Chem. Phys., 15, 9477–9500, <ext-link xlink:href="https://doi.org/10.5194/acp-15-9477-2015" ext-link-type="DOI">10.5194/acp-15-9477-2015</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib47"><label>47</label><?label 1?><mixed-citation>van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Kasibhatla, P. S., and Arellano Jr., A. F.: Interannual variability in global biomass burning emissions from 1997 to 2004, Atmos. Chem. Phys., 6, 3423–3441, <ext-link xlink:href="https://doi.org/10.5194/acp-6-3423-2006" ext-link-type="DOI">10.5194/acp-6-3423-2006</ext-link>, 2006.</mixed-citation></ref>
      <ref id="bib1.bib48"><label>48</label><?label 1?><mixed-citation>Vermote, E., Ellicott, E., Dubovik, O., Lapyonok, T., Chin, M., Giglio, L.,
and Roberts, G. J.: An approach to estimate global biomass burning emissions
of organic and black carbon from MODIS fire radiative power, J. Geophys.
Res.-Atmos., 114, D18205, <ext-link xlink:href="https://doi.org/10.1029/2008jd011188" ext-link-type="DOI">10.1029/2008jd011188</ext-link>, 2009.</mixed-citation></ref>
      <ref id="bib1.bib49"><label>49</label><?label 1?><mixed-citation>Walcek, C. J.: Effects of wind shear on pollution dispersion, Atmos.
Environ., 36, 511–517, <ext-link xlink:href="https://doi.org/10.1016/s1352-2310(01)00383-1" ext-link-type="DOI">10.1016/s1352-2310(01)00383-1</ext-link>, 2002.</mixed-citation></ref>
      <ref id="bib1.bib50"><label>50</label><?label 1?><mixed-citation>Wang, Y., Jiang, J. H., and Su, H.: Atmospheric responses to the
redistribution of anthropogenic aerosols, J. Geophys. Res.-Atmos., 120,
9625-9641, <ext-link xlink:href="https://doi.org/10.1002/2015JD023665" ext-link-type="DOI">10.1002/2015JD023665</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib51"><label>51</label><?label 1?><mixed-citation>Xue, D. Q., Zheng, Q. L., and Qian, X. Z.: Features of sea-land circulation
with its influence over Shandong Peninsula, J. Nanjing Inst. Meteorol., 18,
293–299, <ext-link xlink:href="https://doi.org/10.13878/j.cnki.dqkxxb.1995.02.021" ext-link-type="DOI">10.13878/j.cnki.dqkxxb.1995.02.021</ext-link>, 1995.</mixed-citation></ref>
      <ref id="bib1.bib52"><label>52</label><?label 1?><mixed-citation>Yan, H. and Anthes, R. A.: The effect of latitude on the sea breeze, Mon.
Weather Rev., 115, 936–956, 1987.
 </mixed-citation></ref><?xmltex \hack{\newpage}?>
      <ref id="bib1.bib53"><label>53</label><?label 1?><mixed-citation>Yang, X., Zhao, C. F., Zhou, L., Wang, Y., and Liu, X.: Distinct impact of
different types of aerosols on surface solar radiation in China, J. Geophys.
Res. Atmos., 121, 6459-6471, <ext-link xlink:href="https://doi.org/10.1002/2016JD024938" ext-link-type="DOI">10.1002/2016JD024938</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib54"><label>54</label><?label 1?><mixed-citation>Yang, X., Zhao, C., Yang, Y., Yan, X., and Fan, H.: Statistical aerosol properties associated with fire events from 2002 to 2019 and a case analysis in 2019 over Australia, Atmos. Chem. Phys., 21, 3833–3853, <ext-link xlink:href="https://doi.org/10.5194/acp-21-3833-2021" ext-link-type="DOI">10.5194/acp-21-3833-2021</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bib55"><label>55</label><?label 1?><mixed-citation>Zhang, H., Wang, Z. L., and Zhao, S. Y.: Atmospheric aerosols and their
climatological effect, China Meteorological Press, Beijing, China, ISBN:
978-7-5029-6676-8, 2017.</mixed-citation></ref>
      <ref id="bib1.bib56"><label>56</label><?label 1?><mixed-citation>Zhao, C. and Garrett, T. J.: Effects of Arctic haze on surface cloud radiative forcing, Geophys. Res. Lett., 42, 557–564, <ext-link xlink:href="https://doi.org/10.1002/2014gl062015" ext-link-type="DOI">10.1002/2014gl062015</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bib57"><label>57</label><?label 1?><mixed-citation>Zhao, C., Lin, Y., Wu, F., Wang, Y., Li, Z., Rosenfeld, D., and Wang, Y.:
Enlarging rainfall area of tropical cyclones by atmospheric aerosols,
Geophys. Res. Lett., 45, 8604–8611, <ext-link xlink:href="https://doi.org/10.1029/2018GL079427" ext-link-type="DOI">10.1029/2018GL079427</ext-link>,
2018.</mixed-citation></ref>
      <ref id="bib1.bib58"><label>58</label><?label 1?><mixed-citation>Zhao, C. F., Yang, Y. K., Fan, H., Huang, J. P., Fu, Y. F., Zhang, X. Y.,
Kang, S. C., Cong, Z. Y., Husi, L., and Menenti, M.: Aerosol characteristics
and impacts on weather and climate over Tibetan Plateau, Nat. Sci. Rev., 7,
492–495, <ext-link xlink:href="https://doi.org/10.1093/nsr/nwz184" ext-link-type="DOI">10.1093/nsr/nwz184</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib59"><label>59</label><?label 1?><mixed-citation>Zhu, L., Meng, Z., Zhang, F., and Markowski, P. M.: The influence of sea- and land-breeze circulations on the diurnal variability in precipitation over a tropical island, Atmos. Chem. Phys., 17, 13213–13232, <ext-link xlink:href="https://doi.org/10.5194/acp-17-13213-2017" ext-link-type="DOI">10.5194/acp-17-13213-2017</ext-link>, 2017.</mixed-citation></ref>

  </ref-list></back>
    <!--<article-title-html>Observed slump of sea land breeze in Brisbane under the effect of aerosols from remote transport during 2019 Australian mega fire events</article-title-html>
<abstract-html/>
<ref-html id="bib1.bib1"><label>1</label><mixed-citation>
Albrecht, B. A.: Aerosols, Cloud Microphysics, and Fractional Cloudiness,
Science, 245, 1227–1230, <a href="https://doi.org/10.1126/science.245.4923.1227" target="_blank">https://doi.org/10.1126/science.245.4923.1227</a>,
1989.
</mixed-citation></ref-html>
<ref-html id="bib1.bib2"><label>2</label><mixed-citation>
Baldwin, R., Wright, V., Anders, D. D., Brinegar, D., Lott, N., Jones, P., Smith, F., and Boreman, B.: The FCC Integrated Surface Hourly Database, A New Resource of Global Climate Data [data set], Data center of NOAA, available at: <a href="http://www1.ncdc.noaa.gov/pub/data/noaa/" target="_blank"/> (last access: 31 March 2021), 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib3"><label>3</label><mixed-citation>Cao, L. Z., Chen, X., Zhang, C., Kurban, A., Yuan, X. L., Pan, T., and
Maeyer, P.: The temporal and spatial distributions of the near-surface
CO<sub>2</sub> concentrations in central Asia and analysis of their controlling
factors, Atmosphere, 8, 1–14, <a href="https://doi.org/10.3390/atmos8050085" target="_blank">https://doi.org/10.3390/atmos8050085</a>, 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib4"><label>4</label><mixed-citation>Charlson, R. J., Schwartz, S. E., Hales, J. M., Cess, R. D., Coakley, J. A.,
Hansen, J. E., and Hofmann, D. J.: Climate forcing by anthropogenic
aerosols, Science, 255, 423–430, 1992.
</mixed-citation></ref-html>
<ref-html id="bib1.bib5"><label>5</label><mixed-citation>Chuang, C. C., Penner, J. E., Prospero, J. M., Grant, K. E., Rau, G. H., and
Kawamoto, K.: Cloud susceptibility and the first aerosol indirect forcing:
Sensitivity to black carbon and aerosol concentrations, J. Geophys.
Res.-Atmos., 107, 4564, <a href="https://doi.org/10.1029/2000JD000215" target="_blank">https://doi.org/10.1029/2000JD000215</a>, 2002.
</mixed-citation></ref-html>
<ref-html id="bib1.bib6"><label>6</label><mixed-citation>Cuxart, J., Jiménez, M. A., Prtenjak, M. T., and Grisogono, B.: Study of a
sea-breeze case through momentum, temperature, and turbulence budgets, J.
Appl. Meteorol. Climatol., 53, 2589–2609, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib7"><label>7</label><mixed-citation>Garrett, T. J. and Zhao, C.: Increased Arctic cloud longwave emissivity
associated with pollution from mid-latitudes, Nature, 440, 787–789,
<a href="https://doi.org/10.1038/nature04636" target="_blank">https://doi.org/10.1038/nature04636</a>, 2006.
</mixed-citation></ref-html>
<ref-html id="bib1.bib8"><label>8</label><mixed-citation>Giglio, L., Schroeder, W., and Justice, C. O.: The collection 6 MODIS active
fire detection algorithm and fire products, Remote Sens. Environ., 178,
31–41, <a href="https://doi.org/10.1016/j.rse.2016.02.054" target="_blank">https://doi.org/10.1016/j.rse.2016.02.054</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib9"><label>9</label><mixed-citation>
Global Modeling and Assimilation Office (GMAO): MERRA-2 tavgM_2d_aer_Nx: 2d, Monthly mean, Time-averaged, Single-Level, Assimilation, Aerosol Diagnostics V5.12.4, Greenbelt, MD, USA, Goddard Earth Sciences Data and Information Services Center (GES DISC) [data set], <a href="https://doi.org/10.5067/FH9A0MLJPC7N" target="_blank">https://doi.org/10.5067/FH9A0MLJPC7N</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib10"><label>10</label><mixed-citation>Grandey, B. S., Lee, H.-H., and Wang, C.: Radiative effects of interannually varying vs. interannually invariant aerosol emissions from fires, Atmos. Chem. Phys., 16, 14495–14513, <a href="https://doi.org/10.5194/acp-16-14495-2016" target="_blank">https://doi.org/10.5194/acp-16-14495-2016</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib11"><label>11</label><mixed-citation>Han, W., Li, Z., Wu, F., Zhang, Y., Guo, J., Su, T., Cribb, M., Fan, J., Chen, T., Wei, J., and Lee, S.-S.: The mechanisms and seasonal differences of the impact of aerosols on daytime surface urban heat island effect, Atmos. Chem. Phys., 20, 6479–6493, <a href="https://doi.org/10.5194/acp-20-6479-2020" target="_blank">https://doi.org/10.5194/acp-20-6479-2020</a>, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib12"><label>12</label><mixed-citation>
Hersbach, H., Bell, B., Berrisford, P., Biavati, G., Horányi, A., Muñoz Sabater, J., Nicolas, J., Peubey, C., Radu, R., Rozum, I., Schepers, D., Simmons, A., Soci, C., Dee, D., and Thépaut, J.-N.: ERA5 monthly averaged data on single levels from 1979 to present, Copernicus Climate Change Service (C3S) Climate Data Store (CDS) [data set], available at: <a href="https://climate.copernicus.eu/climate-reanalysis" target="_blank"/> (last access: 31 March 2021), 2019.
</mixed-citation></ref-html>
<ref-html id="bib1.bib13"><label>13</label><mixed-citation>Hirsch, E. and Koren, I.: Record-breaking aerosol levels explained by smoke
injection into the stratosphere, Science, 371, 1269–1274,
<a href="https://doi.org/10.1126/science.abe1415" target="_blank">https://doi.org/10.1126/science.abe1415</a>, 2021.
</mixed-citation></ref-html>
<ref-html id="bib1.bib14"><label>14</label><mixed-citation>
Hubanks, P., Platnick, S., King, M., and Ridgway, B.:  MODIS Atmosphere L3 Monthly Product. NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data set], USA, <a href="https://doi.org/10.5067/MODIS/MOD08_M3.061" target="_blank">https://doi.org/10.5067/MODIS/MOD08_M3.061</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib15"><label>15</label><mixed-citation>IPCC: Intergovernmental Panel on Climate Change, Climate Change 2013: The Physical
Science Basis, Contribution of Working Group I to the Fifth Assessment
Report of the Intergovernmental Panel on Climate Change, Cambridge
Univ. Press, Cambridge, UK, and New York, 1535 pp., 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib16"><label>16</label><mixed-citation>Jacobson, M. Z.: Strong radiative heating due to the mixing state of black
carbon in atmospheric aerosols, Nature, 409, 695–697, 2001.
</mixed-citation></ref-html>
<ref-html id="bib1.bib17"><label>17</label><mixed-citation>Jacobson, M. Z.: Effects of biomass burning on climate, accounting for heat
and moisture fluxes, black and brown carbon, and cloud absorption effects,
J. Geophys. Res.-Atmos., 119, 8980–9002,
<a href="https://doi.org/10.1002/2014jd021861" target="_blank">https://doi.org/10.1002/2014jd021861</a>, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib18"><label>18</label><mixed-citation>Jia, S. Q., Jing, J. L., Ju, E. D., and Chi, W. B.: Discussions on the
temperature and pressure fields in a mega forest fire zone, J. Nort. Fore.
Uni., 15, 226–232, <a href="https://doi.org/10.13759/j.cnki.dlxb.1987.s4.028" target="_blank">https://doi.org/10.13759/j.cnki.dlxb.1987.s4.028</a>, 1987.
</mixed-citation></ref-html>
<ref-html id="bib1.bib19"><label>19</label><mixed-citation>Kloss, C., Berthet, G., Sellitto, P., Ploeger, F., Bucci, S., Khaykin, S., Jégou, F., Taha, G., Thomason, L. W., Barret, B., Le Flochmoen, E., von Hobe, M., Bossolasco, A., Bègue, N., and Legras, B.: Transport of the 2017 Canadian wildfire plume to the tropics via the Asian monsoon circulation, Atmos. Chem. Phys., 19, 13547–13567, <a href="https://doi.org/10.5194/acp-19-13547-2019" target="_blank">https://doi.org/10.5194/acp-19-13547-2019</a>, 2019.
</mixed-citation></ref-html>
<ref-html id="bib1.bib20"><label>20</label><mixed-citation>Kusaka, H., Kimura, F., Hirakuchi, H., and Mizutori, M.: The effects of
land-use alteration on the sea breeze and daytime heat island in the Tokyo
metropolitan area, J. Meteorol. Soc. Jpn., 78, 405–420,
<a href="https://doi.org/10.2151/jmsj1965.78.4_405" target="_blank">https://doi.org/10.2151/jmsj1965.78.4_405</a>, 2000.
</mixed-citation></ref-html>
<ref-html id="bib1.bib21"><label>21</label><mixed-citation>Li, J. W., Yang, L. Q., Li, X. W., and Zheng, H. R.: Visualization of local
wind field based forest-fire's forecast modeling for transportation
planning, Multimed. Tools. Appl., 1, 1–15,
<a href="https://doi.org/10.1007/s11042-016-3357-7" target="_blank">https://doi.org/10.1007/s11042-016-3357-7</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib22"><label>22</label><mixed-citation>Luhar, A. K., Mitchell, R. M., Meyer, C. P., Qin, Y., Campbell, S., Gras, J.
L., and Parry, D.: Biomass burning emissions over northern Australia
constrained by aerosol measurements: II–Model validation, and impacts on air quality and radiative
forcing, Atmos. Environ., 42, 1647–1664,
<a href="https://doi.org/10.1016/j.atmosenv.2007.12.040" target="_blank">https://doi.org/10.1016/j.atmosenv.2007.12.040</a>, 2008.
</mixed-citation></ref-html>
<ref-html id="bib1.bib23"><label>23</label><mixed-citation>Lymburner, L., Tan, P., McIntyre, A., Thankappan, M., and Sixsmith, J.:
Dynamic Land Cover Dataset Version 2.1. Geoscience Australia, Canberra,
available at: <a href="http://pid.geoscience.gov.au/dataset/ga/83868" target="_blank"/> (last access: 31
January 2021), 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib24"><label>24</label><mixed-citation>Ma, Y., Gao, R. Z., and Miao, S. G.: Impacts of urbanization on summer-time
SLB circulation in Qingdao, Acta. Sci. Circumst., 33, 1690–1696,
<a href="https://doi.org/10.13671/j.hjkxxb.2013.06.030" target="_blank">https://doi.org/10.13671/j.hjkxxb.2013.06.030</a>, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib25"><label>25</label><mixed-citation>Mallet, M. D., Desservettaz, M. J., Miljevic, B., Milic, A., Ristovski, Z. D., Alroe, J., Cravigan, L. T., Jayaratne, E. R., Paton-Walsh, C., Griffith, D. W. T., Wilson, S. R., Kettlewell, G., van der Schoot, M. V., Selleck, P., Reisen, F., Lawson, S. J., Ward, J., Harnwell, J., Cheng, M., Gillett, R. W., Molloy, S. B., Howard, D., Nelson, P. F., Morrison, A. L., Edwards, G. C., Williams, A. G., Chambers, S. D., Werczynski, S., Williams, L. R., Winton, V. H. L., Atkinson, B., Wang, X., and Keywood, M. D.: Biomass burning emissions in north Australia during the early dry season: an overview of the 2014 SAFIRED campaign, Atmos. Chem. Phys., 17, 13681–13697, <a href="https://doi.org/10.5194/acp-17-13681-2017" target="_blank">https://doi.org/10.5194/acp-17-13681-2017</a>, 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib26"><label>26</label><mixed-citation>McCoy, D. T. and Hartmann, D. L.: Observations of a substantial
cloud-aerosol indirect effectduring the 2014–2015
Bárðarbunga-Veiðivötnssure eruption in Iceland, Geophys.
Res. Lett., 42, 10409–10414, <a href="https://doi.org/10.1002/2015GL067070" target="_blank">https://doi.org/10.1002/2015GL067070</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib27"><label>27</label><mixed-citation>Meyer, C. P., Luhar, A. K., and Mitchell, R. M.: Biomass burning emissions
over northern Australia constrained by aerosol measurements: I – Modelling
the distribution of hourly emissions, Atmos. Environ., 42, 1629–1646,
<a href="https://doi.org/10.1016/j.atmosenv.2007.10.089" target="_blank">https://doi.org/10.1016/j.atmosenv.2007.10.089</a>, 2008.
</mixed-citation></ref-html>
<ref-html id="bib1.bib28"><label>28</label><mixed-citation>Miller, S. T. K., Keim, B. D., Talbot, R. W., and Mao, H.: Sea breeze:
Structure, forecasting, and impacts, Rev. Geophys., 41, 1011,
<a href="https://doi.org/10.1029/2003RG000124" target="_blank">https://doi.org/10.1029/2003RG000124</a>, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib29"><label>29</label><mixed-citation>Mitchell, R. M., O'Brien, D. M., and Campbell, S. K.: Characteristics and
radiative impact of the aerosol generated by the Canberra firestorm of
January 2003, J. Geophys. Res.-Atmos., 111, D02204,
<a href="https://doi.org/10.1029/2005jd006304" target="_blank">https://doi.org/10.1029/2005jd006304</a>, 2006.
</mixed-citation></ref-html>
<ref-html id="bib1.bib30"><label>30</label><mixed-citation>Mitchell, R. M., Forgan, B. W., Campbell, S. K., and Qin, Y.: The
climatology of Australian tropical aerosol: Evidence for regional
correlation, Geophys. Res. Lett., 40, 2384–2389,
<a href="https://doi.org/10.1002/grl.50403" target="_blank">https://doi.org/10.1002/grl.50403</a>, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib31"><label>31</label><mixed-citation>
MODIS Atmosphere Science Team: MODIS Cloud Properties Level 3 Monthly Product, NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data set], USA, <a href="https://doi.org/10.5067/MODIS/MCD06COSP_M3_MODIS.061" target="_blank">https://doi.org/10.5067/MODIS/MCD06COSP_M3_MODIS.061</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib32"><label>32</label><mixed-citation>Nai, F. B., Zhao, L. N., and Wu, J. R.: Impacts of sea-land and
mountain-valley circulations on the air pollution in Beijing-Tianjin-Hebei:
a case study, Environ. Pollut., 234, 429–438,
<a href="https://doi.org/10.1016/j.envpol.2017.11.066" target="_blank">https://doi.org/10.1016/j.envpol.2017.11.066</a>, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib33"><label>33</label><mixed-citation>
NOAA: GDAS – Daily Tar Files (1° by 1°), NCEI's NOAA National Operational Model Archive and Distribution System (NOMADS) [data set], available at: <a href="ftp://ftp.arl.noaa.gov/pub/archives/gdas1" target="_blank"/> (last access: 31 March 2021), 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib34"><label>34</label><mixed-citation>Ohneiser, K., Ansmann, A., Baars, H., Seifert, P., Barja, B., Jimenez, C., Radenz, M., Teisseire, A., Floutsi, A., Haarig, M., Foth, A., Chudnovsky, A., Engelmann, R., Zamorano, F., Bühl, J., and Wandinger, U.: Smoke of extreme Australian bushfires observed in the stratosphere over Punta Arenas, Chile, in January 2020: optical thickness, lidar ratios, and depolarization ratios at 355 and 532 nm, Atmos. Chem. Phys., 20, 8003–8015, <a href="https://doi.org/10.5194/acp-20-8003-2020" target="_blank">https://doi.org/10.5194/acp-20-8003-2020</a>, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib35"><label>35</label><mixed-citation>Portin, H., Mielonen, T., Leskinen, A., Arola, A., Pärjälä, E.,
Romakkaniemi, S., Laaksonen, A., Lehtinen, K. E. J., and Komppula, M.:
Biomass burning aerosols observed in Eastern Finland during the Russian
wildfires in summer 2010 e Part 1: In-situ aerosol characterization, Atmos.
Environ., 47, 269–278, http:// <a href="https://doi.org/10.1016/j.atmosenv.2011.10.067" target="_blank">https://doi.org/10.1016/j.atmosenv.2011.10.067</a>, 2012.
</mixed-citation></ref-html>
<ref-html id="bib1.bib36"><label>36</label><mixed-citation>Rajib, P. and Heekwa, L.: Estimation of the effective zone of sea/land
breeze in a coastal area, Atmos. Pollut. Res., 2, 106–115,
<a href="https://doi.org/10.5094/APR.2011.013" target="_blank">https://doi.org/10.5094/APR.2011.013</a>, 2010.
</mixed-citation></ref-html>
<ref-html id="bib1.bib37"><label>37</label><mixed-citation>Ramana, M. V., Ramanathan, V., Feng, Y., Yoon, S. C., Kim, S. W.,
Carmichael, G. R., and Schauer, J. J.: Warming influenced by the ratio of
black carbon to sulphate and the black-carbon source, Nat. Geosci., 1,
542–545, <a href="https://doi.org/10.1038/NGEO918" target="_blank">https://doi.org/10.1038/NGEO918</a>, 2010.
</mixed-citation></ref-html>
<ref-html id="bib1.bib38"><label>38</label><mixed-citation>Sarker, A., Saraswat, R. S., Chandrasekar, A.: Numerical study of the
effects of urban heat island on the characteristic features of the sea
breeze circulation, P. Indian As.-Eng. Sci., 107, 127–137, 1998.
</mixed-citation></ref-html>
<ref-html id="bib1.bib39"><label>39</label><mixed-citation>Shen, L. X. and Zhao, C. F.: Dominance of Shortwave Radiative Heating in
the Sea-Land Breeze Amplitude and its Impacts on Atmospheric Visibility in
Tokyo, Japan, J. Geophys. Res.-Atmos., 125, 1–19,
<a href="https://doi.org/10.1029/2019jd031541" target="_blank">https://doi.org/10.1029/2019jd031541</a>, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib40"><label>40</label><mixed-citation>Shen, L. X., Zhao, C. F., Ma, Z. S., Li, Z. Q., Li, J. P., and Wang, K. C.:
Observed decrease of summer sea-land breeze in Shanghai from 1994 to 2014
and its association with urbanization, Atmos. Res., 227, 198–209,
<a href="https://doi.org/10.1016/j.atmosres.2019.05.007" target="_blank">https://doi.org/10.1016/j.atmosres.2019.05.007</a>, 2019.
</mixed-citation></ref-html>
<ref-html id="bib1.bib41"><label>41</label><mixed-citation>Shen, L. X., Zhao, C. F., and Yang, X. C.: Insight Into the Seasonal
Variations of the Sea-Land Breeze in Los Angeles With Respect to the Effects
of Solar Radiation and Climate Type, J. Geophys. Res.-Atmos., 126, 1–21,
<a href="https://doi.org/10.1029/2019jd033197" target="_blank">https://doi.org/10.1029/2019jd033197</a>, 2021a.
</mixed-citation></ref-html>
<ref-html id="bib1.bib42"><label>42</label><mixed-citation>Shen, L. X., Zhao, C. F., and Yang, X. C.: Climate-Driven Characteristics of
Sea-Land Breezes Over the Globe, Geophys. Res. Lett., 48, 1–10,
<a href="https://doi.org/10.1029/2020GL092308" target="_blank">https://doi.org/10.1029/2020GL092308</a>, 2021b.
</mixed-citation></ref-html>
<ref-html id="bib1.bib43"><label>43</label><mixed-citation>
Sun, R. Y., Krueger, S. K., Jenkins, M. A., Zulauf, M. A., and Charney, J. J.: The importance of fire–atmosphere coupling and boundary-layer turbulence to wildfire spread, Int. J. Wildland Fire., 18, 50–60, <a href="https://doi.org/10.1071/WF07072" target="_blank">https://doi.org/10.1071/WF07072</a>, 2009.
</mixed-citation></ref-html>
<ref-html id="bib1.bib44"><label>44</label><mixed-citation>
The Land, Atmosphere Near real-time Capability for EOS MODIS (LANCEMODIS) Team:  MODIS/Aqua Terra Thermal Anomalies/Fire locations 1&thinsp;km FIRMS V006 NRT (Vector data), NASA MODIS Adaptive Processing System, Goddard Space Flight Center [data set], USA, <a href="https://doi.org/10.5067/FIRMS/MODIS/MCD14DL.NRT.006" target="_blank">https://doi.org/10.5067/FIRMS/MODIS/MCD14DL.NRT.006</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib45"><label>45</label><mixed-citation>
Torres, O., Jethva, H., Ahn, C., Jaross, G., and Loyola, D. G.: TROPOMI aerosol products: evaluation and observations of synoptic-scale carbonaceous aerosol plumes during 2018–2020, Atmos. Meas. Tech., 13, 6789–6806, <a href="https://doi.org/10.5194/amt-13-6789-2020" target="_blank">https://doi.org/10.5194/amt-13-6789-2020</a>, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib46"><label>46</label><mixed-citation>Turnock, S. T., Spracklen, D. V., Carslaw, K. S., Mann, G. W., Woodhouse, M. T., Forster, P. M., Haywood, J., Johnson, C. E., Dalvi, M., Bellouin, N., and Sanchez-Lorenzo, A.: Modelled and observed changes in aerosols and surface solar radiation over Europe between 1960 and 2009, Atmos. Chem. Phys., 15, 9477–9500, <a href="https://doi.org/10.5194/acp-15-9477-2015" target="_blank">https://doi.org/10.5194/acp-15-9477-2015</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib47"><label>47</label><mixed-citation>van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Kasibhatla, P. S., and Arellano Jr., A. F.: Interannual variability in global biomass burning emissions from 1997 to 2004, Atmos. Chem. Phys., 6, 3423–3441, <a href="https://doi.org/10.5194/acp-6-3423-2006" target="_blank">https://doi.org/10.5194/acp-6-3423-2006</a>, 2006.
</mixed-citation></ref-html>
<ref-html id="bib1.bib48"><label>48</label><mixed-citation>Vermote, E., Ellicott, E., Dubovik, O., Lapyonok, T., Chin, M., Giglio, L.,
and Roberts, G. J.: An approach to estimate global biomass burning emissions
of organic and black carbon from MODIS fire radiative power, J. Geophys.
Res.-Atmos., 114, D18205, <a href="https://doi.org/10.1029/2008jd011188" target="_blank">https://doi.org/10.1029/2008jd011188</a>, 2009.
</mixed-citation></ref-html>
<ref-html id="bib1.bib49"><label>49</label><mixed-citation>Walcek, C. J.: Effects of wind shear on pollution dispersion, Atmos.
Environ., 36, 511–517, <a href="https://doi.org/10.1016/s1352-2310(01)00383-1" target="_blank">https://doi.org/10.1016/s1352-2310(01)00383-1</a>, 2002.
</mixed-citation></ref-html>
<ref-html id="bib1.bib50"><label>50</label><mixed-citation>Wang, Y., Jiang, J. H., and Su, H.: Atmospheric responses to the
redistribution of anthropogenic aerosols, J. Geophys. Res.-Atmos., 120,
9625-9641, <a href="https://doi.org/10.1002/2015JD023665" target="_blank">https://doi.org/10.1002/2015JD023665</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib51"><label>51</label><mixed-citation>Xue, D. Q., Zheng, Q. L., and Qian, X. Z.: Features of sea-land circulation
with its influence over Shandong Peninsula, J. Nanjing Inst. Meteorol., 18,
293–299, <a href="https://doi.org/10.13878/j.cnki.dqkxxb.1995.02.021" target="_blank">https://doi.org/10.13878/j.cnki.dqkxxb.1995.02.021</a>, 1995.
</mixed-citation></ref-html>
<ref-html id="bib1.bib52"><label>52</label><mixed-citation>Yan, H. and Anthes, R. A.: The effect of latitude on the sea breeze, Mon.
Weather Rev., 115, 936–956, 1987.

</mixed-citation></ref-html>
<ref-html id="bib1.bib53"><label>53</label><mixed-citation>Yang, X., Zhao, C. F., Zhou, L., Wang, Y., and Liu, X.: Distinct impact of
different types of aerosols on surface solar radiation in China, J. Geophys.
Res. Atmos., 121, 6459-6471, <a href="https://doi.org/10.1002/2016JD024938" target="_blank">https://doi.org/10.1002/2016JD024938</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib54"><label>54</label><mixed-citation>Yang, X., Zhao, C., Yang, Y., Yan, X., and Fan, H.: Statistical aerosol properties associated with fire events from 2002 to 2019 and a case analysis in 2019 over Australia, Atmos. Chem. Phys., 21, 3833–3853, <a href="https://doi.org/10.5194/acp-21-3833-2021" target="_blank">https://doi.org/10.5194/acp-21-3833-2021</a>, 2021.
</mixed-citation></ref-html>
<ref-html id="bib1.bib55"><label>55</label><mixed-citation>Zhang, H., Wang, Z. L., and Zhao, S. Y.: Atmospheric aerosols and their
climatological effect, China Meteorological Press, Beijing, China, ISBN:
978-7-5029-6676-8, 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib56"><label>56</label><mixed-citation>
Zhao, C. and Garrett, T. J.: Effects of Arctic haze on surface cloud radiative forcing, Geophys. Res. Lett., 42, 557–564, <a href="https://doi.org/10.1002/2014gl062015" target="_blank">https://doi.org/10.1002/2014gl062015</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib57"><label>57</label><mixed-citation>Zhao, C., Lin, Y., Wu, F., Wang, Y., Li, Z., Rosenfeld, D., and Wang, Y.:
Enlarging rainfall area of tropical cyclones by atmospheric aerosols,
Geophys. Res. Lett., 45, 8604–8611, <a href="https://doi.org/10.1029/2018GL079427" target="_blank">https://doi.org/10.1029/2018GL079427</a>,
2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib58"><label>58</label><mixed-citation>Zhao, C. F., Yang, Y. K., Fan, H., Huang, J. P., Fu, Y. F., Zhang, X. Y.,
Kang, S. C., Cong, Z. Y., Husi, L., and Menenti, M.: Aerosol characteristics
and impacts on weather and climate over Tibetan Plateau, Nat. Sci. Rev., 7,
492–495, <a href="https://doi.org/10.1093/nsr/nwz184" target="_blank">https://doi.org/10.1093/nsr/nwz184</a>, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib59"><label>59</label><mixed-citation> Zhu, L., Meng, Z., Zhang, F., and Markowski, P. M.: The influence of sea- and land-breeze circulations on the diurnal variability in precipitation over a tropical island, Atmos. Chem. Phys., 17, 13213–13232, <a href="https://doi.org/10.5194/acp-17-13213-2017" target="_blank">https://doi.org/10.5194/acp-17-13213-2017</a>, 2017.
</mixed-citation></ref-html>--></article>
