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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-21-6347-2021</article-id><title-group><article-title>Case study of a humidity layer above Arctic stratocumulus <?xmltex \hack{\break}?> and potential turbulent coupling with the cloud top</article-title><alt-title>Case study of a humidity layer above Arctic stratocumulus</alt-title>
      </title-group><?xmltex \runningtitle{Case study of a humidity layer above Arctic stratocumulus}?><?xmltex \runningauthor{U.~Egerer et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>Egerer</surname><given-names>Ulrike</given-names></name>
          <email>egerer@tropos.de</email>
        <ext-link>https://orcid.org/0000-0001-6107-612X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Ehrlich</surname><given-names>André</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-0860-8216</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2 aff4">
          <name><surname>Gottschalk</surname><given-names>Matthias</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-9077-519X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Griesche</surname><given-names>Hannes</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-8696-7359</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3">
          <name><surname>Neggers</surname><given-names>Roel A. J.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-9182-3050</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Siebert</surname><given-names>Holger</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Wendisch</surname><given-names>Manfred</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-4652-5561</ext-link></contrib>
        <aff id="aff1"><label>1</label><institution>Leibniz Institute for Tropospheric Research, Permoserstr. 15, 04318 Leipzig, Germany</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Leipzig Institute for Meteorology, University of Leipzig, Stephanstr. 3, 04103 Leipzig, Germany</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Institute for Geophysics and Meteorology, University of Cologne, Pohligstr. 3, 50969 Cologne, Germany</institution>
        </aff>
        <aff id="aff4"><label>a</label><institution>now at: Deutscher Wetterdienst, Frankfurter Str. 135, 63067 Offenbach, Germany</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Ulrike Egerer (egerer@tropos.de)</corresp></author-notes><pub-date><day>27</day><month>April</month><year>2021</year></pub-date>
      
      <volume>21</volume>
      <issue>8</issue>
      <fpage>6347</fpage><lpage>6364</lpage>
      <history>
        <date date-type="received"><day>11</day><month>June</month><year>2020</year></date>
           <date date-type="accepted"><day>22</day><month>March</month><year>2021</year></date>
           <date date-type="rev-recd"><day>10</day><month>March</month><year>2021</year></date>
           <date date-type="rev-request"><day>25</day><month>June</month><year>2020</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2021 </copyright-statement>
        <copyright-year>2021</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/.html">This article is available from https://acp.copernicus.org/articles/.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/.pdf</self-uri>
      <abstract><title>Abstract</title>
    <p id="d1e158">Specific humidity inversions (SHIs) above low-level cloud
layers have been frequently observed in the Arctic.  The formation of these
SHIs is usually associated with large-scale advection of humid air
masses. However, the potential coupling of SHIs with cloud layers by turbulent
processes is not fully understood.  In this study, we analyze a 3 d
period of a persistent layer of increased specific humidity above a
stratocumulus cloud observed during an Arctic field campaign in June 2017. The
tethered balloon system BELUGA (Balloon-bornE moduLar Utility for profilinG
the lower Atmosphere) recorded vertical profile data of meteorological,
turbulence, and radiation parameters in the atmospheric boundary layer. An
in-depth discussion of the problems associated with humidity measurements in
cloudy environments leads to the conclusion that the observed SHIs do not
result from measurement artifacts.  We analyze two different scenarios for the
SHI in relation to the cloud top capped by a temperature inversion: (i) the
SHI coincides with the cloud top, and (ii) the SHI is vertically separated
from the lowered cloud top. In the first case, the SHI and the cloud layer are
coupled by turbulence that extends over the cloud top and connects the two
layers by turbulent mixing. Several profiles reveal downward virtual sensible
and latent heat fluxes at the cloud top, indicating entrainment of humid air
supplied by the SHI into the cloud layer. For the second case, a downward
moisture transport at the base of the SHI and an upward moisture flux at the cloud
top is observed. Therefore, the area between the cloud top and SHI is supplied
with moisture from both sides.  Finally, large-eddy simulations (LESs)
complement the observations by modeling a case of the first scenario. The
simulations reproduce the observed downward turbulent fluxes of heat and
moisture at the cloud top. The LES realizations suggest that in the presence
of a SHI, the cloud layer remains thicker and the temperature inversion height
is elevated.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e170">The Arctic atmospheric boundary layer (ABL) exhibits numerous particular
features compared to lower latitudes, such as persistent mixed-phase clouds,
multiple cloud layers decoupled from the surface, and ubiquitous temperature
inversions close to the surface. Local ABL and cloud processes are complex and
not completely understood, but they are considered an important component to
explain the rapid warming of the Arctic region <xref ref-type="bibr" rid="bib1.bibx52" id="paren.1"/>. One of
the special features frequently observed in the Arctic are specific humidity
inversions (SHIs), although specific humidity is generally expected to
decrease with height <xref ref-type="bibr" rid="bib1.bibx32 bib1.bibx53" id="paren.2"/>. The relative frequency of
occurrence of low-level SHIs in summer is estimated to be in the range of
70 %–90 % over the Arctic ocean <xref ref-type="bibr" rid="bib1.bibx29" id="paren.3"/>.</p>
      <?pagebreak page6348?><p id="d1e182">Arctic SHIs have been observed during past field campaigns <xref ref-type="bibr" rid="bib1.bibx37 bib1.bibx33" id="paren.4"/>, e.g., the Surface Heat Budget of the Arctic Ocean <xref ref-type="bibr" rid="bib1.bibx48" id="paren.5"><named-content content-type="pre">SHEBA;
</named-content></xref> in 1997–1998, or the Arctic Summer Cloud Ocean Study
<xref ref-type="bibr" rid="bib1.bibx47" id="paren.6"><named-content content-type="pre">ASCOS; </named-content></xref> in 2008. Furthermore, a number of studies
on the climatology of SHIs have been published <xref ref-type="bibr" rid="bib1.bibx29 bib1.bibx3 bib1.bibx6" id="paren.7"><named-content content-type="pre">e.g., </named-content></xref>. SHIs occur most frequently over the Arctic ocean
and are strongest in summer. In the lower troposphere, they often occur in
conjunction with temperature inversions and high relative humidity but are
also linked to the surface energy budget <xref ref-type="bibr" rid="bib1.bibx29" id="paren.8"/>. Formation
processes and interactions of SHIs with clouds have been investigated in large-eddy simulations (LESs). For example, <xref ref-type="bibr" rid="bib1.bibx41" id="text.9"/> showed that a
specific humidity layer becomes important as a moisture source for the cloud
when moisture supply from the surface is limited. <xref ref-type="bibr" rid="bib1.bibx33" id="text.10"/> studied
how the SHIs support the mixed-phase clouds to extend into the temperature and
humidity inversion.</p>
      <p id="d1e213">Mostly, the formation of the summertime SHIs is attributed to large-scale
advection of humid air masses. In the Arctic, especially over sea ice,
moisture advection is the critical factor for cloud formation and development
<xref ref-type="bibr" rid="bib1.bibx43" id="paren.11"/>. SHIs form when warm, moist air is advected over the
cold sea ice surface and moisture is removed through condensation and
precipitation from the lowest ABL part.  This and further simplified formation
processes are discussed by <xref ref-type="bibr" rid="bib1.bibx29" id="text.12"/>.</p>
      <p id="d1e222">SHIs can contribute to the longevity of Arctic mixed-phase clouds
<xref ref-type="bibr" rid="bib1.bibx28 bib1.bibx36" id="paren.13"/>, which dominate the near-surface radiation
heat budget in the Arctic <xref ref-type="bibr" rid="bib1.bibx18" id="paren.14"/>. When a SHI is located closely
above an Arctic stratocumulus, it can provide moisture that may drive the
cloud evolution due to cloud top entrainment. In contrast, in the typical
marine sub-tropical or mid-latitude cloud-topped ABL, dry air from above is
entrained into the cloud <xref ref-type="bibr" rid="bib1.bibx1 bib1.bibx32 bib1.bibx20" id="paren.15"/>. However, SHIs are not well represented in global atmospheric
models, where the SHI strength is typically underestimated <xref ref-type="bibr" rid="bib1.bibx29" id="paren.16"/>,
or the SHIs are not reproduced <xref ref-type="bibr" rid="bib1.bibx42" id="paren.17"/>.</p>
      <p id="d1e241">Previous studies on SHIs have been based on radiosoundings, remote sensing
observations, reanalysis data, or LESs. Most observational studies rely on
profiles of mean thermodynamic parameters from radiosoundings, which might be
influenced by sensor wetting after cloud penetration in the SHI region. A
systematic bias in radiosonde humidity measurements due to sensor wetting or
other error sources is a serious concern when studying SHIs, particularly
under moist and cold conditions. To exclude systematic biases, one aim of this
work is to carefully assess the validity of the SHI observations. Due to the
limited time resolution of radiosondes, those measurements do not allow for
turbulence observations to analyze the exchange processes between the SHI and
cloud top. To date, very few data are available to characterize and
quantify the turbulent and radiative energy fluxes at SHIs. However, in
particular the vertical turbulent exchange of mass and energy is necessary to
understand the importance of SHIs for cloud evolution and lifetime.</p>
      <p id="d1e244"><?xmltex \hack{\newpage}?>To investigate the exchange processes between the cloud layer and the SHI, we
performed tethered balloon-borne high-resolution vertical profile measurements
of turbulence and radiation during a 3 d period in the framework of the
campaign Physical Feedbacks of Arctic Boundary Layer, Sea Ice, Cloud and
Aerosol (PASCAL) <xref ref-type="bibr" rid="bib1.bibx52" id="paren.18"/>. The observations are supplemented by
LES for the same period. We focus on a detailed case study with a persistent
SHI above a stratocumulus deck to answer the following research question: how are the
SHI and the cloud top connected by turbulent mixing?</p>
      <p id="d1e251">The paper is structured as follows: Sect. <xref ref-type="sec" rid="Ch1.S2"/> describes the
observations. In Sect. <xref ref-type="sec" rid="Ch1.S3"/>, we discuss humidity measurements in
cloudy and cold conditions and potential error sources. For the case study,
Sect. <xref ref-type="sec" rid="Ch1.S4"/> analyzes the vertical ABL structure around the SHI
and the relation of SHI, cloud top, and temperature inversion. In
Sect. <xref ref-type="sec" rid="Ch1.S5"/>, we investigate the turbulent coupling between SHI
and the cloud layer, and the turbulent transport of heat and moisture. We
close with a discussion of the impact of the SHI on the cloud by means of
LES in Sect. <xref ref-type="sec" rid="Ch1.S6"/>.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Observations</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>The PASCAL expedition</title>
      <p id="d1e279">The observations analyzed in this study were performed during PASCAL
<xref ref-type="bibr" rid="bib1.bibx52" id="paren.19"/>, which took place in the sea-ice-covered area north of
Svalbard in summer 2017. The RV <italic>Polarstern</italic> <xref ref-type="bibr" rid="bib1.bibx22" id="paren.20"/> carried
a suite of remote sensing and in situ instrumentation. Additionally, an ice
floe camp was erected in the vicinity of the ship
<xref ref-type="bibr" rid="bib1.bibx25" id="paren.21"/>. <xref ref-type="bibr" rid="bib1.bibx21" id="text.22"/> describe the synoptic situation during
the operation of the ice floe camp as climatologically warm with prevailing
warm and moist maritime air masses advected from the south and east. The
meteorological conditions were influenced by a high-pressure ridge east of
Svalbard. The present study is based on measurements with instruments carried
by the tethered balloon system BELUGA <xref ref-type="bibr" rid="bib1.bibx10" id="paren.23"><named-content content-type="pre">Balloon-bornE moduLar Utility for
profilinG the lower Atmosphere; </named-content></xref>. BELUGA was launched from the
sea ice floe at around 82<inline-formula><mml:math id="M1" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 10<inline-formula><mml:math id="M2" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E in the period of
5–14 June 2017. The balloon measurements are complemented by radiosoundings
launched every 6 h <xref ref-type="bibr" rid="bib1.bibx34" id="paren.24"/> and by ship-based remote
sensing observations from a vertical-pointing, motion-stabilized cloud radar
<xref ref-type="bibr" rid="bib1.bibx14" id="paren.25"/>, a lidar <xref ref-type="bibr" rid="bib1.bibx13" id="paren.26"/>, and a
microwave radiometer of the OCEANET platform <xref ref-type="bibr" rid="bib1.bibx15" id="paren.27"/>, which were
processed with the synergistic instrument algorithm Cloudnet
<xref ref-type="bibr" rid="bib1.bibx12" id="paren.28"/>.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><?xmltex \currentcnt{1}?><?xmltex \def\figurename{Figure}?><label>Figure 1</label><caption><p id="d1e339">Temporal development of the specific humidity vertical profile observed by radiosondes. The radar-retrieved cloud top height is depicted as a black line; the cloud base height derived from the lidar near-field channel is indicated as a grey line. The red lines represent the BELUGA flight profiles.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f01.png"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Observation period</title>
      <p id="d1e356">The observational basis for this study is a persistent layer of increased
specific humidity above a single-layer<?pagebreak page6349?> stratocumulus deck during the period
between 5 and 7 June 2017.  Figure <xref ref-type="fig" rid="Ch1.F1"/> illustrates the
temporal development of the vertical specific humidity profile derived from
radiosonde measurements. Cloud top and bottom and the time–height curves of
the corresponding BELUGA flights are added for the investigated period. The
BELUGA flights were conducted around noon on each of the three consecutive
days. A local maximum of specific humidity is observed above the cloud top
throughout almost the entire period, with a slight diurnal cycle peaking at
noon and a maximum specific humidity on 6 June. It is worth noting that the
observations show a well-defined layer of increased specific humidity,
hereafter referred to as the humidity layer, rather than a distinct and sharp SHI
with only a slight decrease above.</p>
      <p id="d1e361">The cloud top and base height in Fig. <xref ref-type="fig" rid="Ch1.F1"/> are estimated from
the cloud radar and lidar (near-field channel) data, averaged over 30 <inline-formula><mml:math id="M3" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula>
and with a vertical resolution of 30 <inline-formula><mml:math id="M4" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. Throughout the 3 d
period, cloud height and thickness decrease to a minimum at noon of 6 June
and thereafter increase again. The cloud is almost permanently of mixed-phase
type with a maximum liquid water content (LWC) between 0.15 and
0.6 <inline-formula><mml:math id="M5" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and an estimated ice water content (IWC) of about
0.03 <inline-formula><mml:math id="M6" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> derived from Cloudnet data (not shown here).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><?xmltex \currentcnt{2}?><?xmltex \def\figurename{Figure}?><label>Figure 2</label><caption><p id="d1e418">BELUGA flight profiles for 5, 6, and 7 June (red lines) with the radar reflectivity <inline-formula><mml:math id="M7" display="inline"><mml:mi>Z</mml:mi></mml:math></inline-formula> and cloud boundaries (black lines, as in Fig. <xref ref-type="fig" rid="Ch1.F1"/>).</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f02.png"/>

        </fig>

      <p id="d1e437">Figure <xref ref-type="fig" rid="Ch1.F1"/> depicts the high variability in cloud top and
bottom heights. To illustrate the cloud situation around the BELUGA flights in
more detail, Fig. <xref ref-type="fig" rid="Ch1.F2"/> shows the radar reflectivity and
cloud boundaries for the particular three balloon flights. On 5 June, the
cloud top height is approximately constant, whereas on 6 June the cloud top
fluctuates between 350 and 230 <inline-formula><mml:math id="M8" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> in the course of the flight. During
the 7 June flight, the cloud layer thins by 110 <inline-formula><mml:math id="M9" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> starting from the cloud
top.</p>
</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><title>BELUGA setup</title>
      <p id="d1e468">The BELUGA system consists of a 90 <inline-formula><mml:math id="M10" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> helium-filled tethered balloon
with a modular setup of different instrument packages to explore the ABL
between the surface and 1500 <inline-formula><mml:math id="M11" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> altitude. BELUGA can operate under
cloudy and light icing conditions in the Arctic. Fixed to the balloon tether,
a fast (50 <inline-formula><mml:math id="M12" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">Hz</mml:mi></mml:mrow></mml:math></inline-formula> resolution) ultrasonic anemometer, supported by an
inertial navigation system, measures the wind velocity vector in an
Earth-fixed coordinate system together with the sonic temperature. Especially
at low specific humidity, the sonic temperature is close to the virtual
temperature, which will be used in the following. Furthermore, barometric
pressure, relative humidity, and the static air temperature are measured with
lower resolution (1 <inline-formula><mml:math id="M13" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">Hz</mml:mi></mml:mrow></mml:math></inline-formula>). Relative humidity (RH) is measured with a
capacitive humidity sensor. The housing of the RH sensor, which has a high
diffusivity for water vapor, also accommodates a temperature sensor for the
sensor-internal temperature. The air temperature is measured with a PT100 for
reference and a thermocouple for temperature fluctuations (at
50 <inline-formula><mml:math id="M14" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">Hz</mml:mi></mml:mrow></mml:math></inline-formula>). A second instrument payload is fixed simultaneously to the
tether, measuring broadband terrestrial and solar net irradiances. Technical
details on BELUGA, its instrumentation, and operation during PASCAL as well
as data processing methods are given by <xref ref-type="bibr" rid="bib1.bibx10" id="text.29"/>.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Specific humidity measurements in a moist environment</title>
      <?pagebreak page6350?><p id="d1e527">A cold and moist environment poses considerable challenges for the measurement
of specific humidity. This can lead to measurement artifacts in the region of
the SHI. Therefore, in this section we discuss the measurement of specific
humidity with BELUGA and radiosondes as well as possible sources of error and
their effects.  Specific humidity <inline-formula><mml:math id="M15" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> is derived from air temperature <inline-formula><mml:math id="M16" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and
RH using

              <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M17" display="block"><mml:mstyle class="stylechange" displaystyle="true"/><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo><mml:mo>⋅</mml:mo><mml:mtext>RH</mml:mtext></mml:mrow><mml:mrow><mml:mi>p</mml:mi><mml:mo>-</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>⋅</mml:mo><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo><mml:mo>⋅</mml:mo><mml:mtext>RH</mml:mtext></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

        <?xmltex \hack{\newpage}?><?xmltex \hack{\noindent}?>with the static pressure <inline-formula><mml:math id="M18" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>, the ratio of specific gas constants of dry air and water vapor <inline-formula><mml:math id="M19" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">d</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">0.622</mml:mn></mml:mrow></mml:math></inline-formula>, and the temperature-dependent saturation vapor pressure <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. In this study, the measurements of RH and <inline-formula><mml:math id="M21" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> are obtained by regular radiosoundings (Vaisala RS92-SGP) and observations with the BELUGA system. Both methods use capacitive RH sensors, suffering from several limitations <xref ref-type="bibr" rid="bib1.bibx51" id="paren.30"/>.</p>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>Error sources for humidity measurements</title>
      <p id="d1e700">Several studies address the associated systematic errors of radiosonde RH and
<inline-formula><mml:math id="M22" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> measurements and identify three main sources, (i) wet-bulbing, (ii) solar
heating, and (iii) time response errors:
<list list-type="custom"><list-item><label>i.</label>
      <p id="d1e712">Wet-bulbing occurs when a water film develops on the sensor during cloud
penetration, with subsequent evaporative cooling under sub-saturated
conditions above the cloud. This effect leads to an overestimation of RH and
underestimation of <inline-formula><mml:math id="M23" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> in the sub-saturated environment until the water film
has completely evaporated. <xref ref-type="bibr" rid="bib1.bibx19" id="text.31"/> show that wet-bulbing is an
issue for the radiosonde type used during PASCAL. However, the error induced
by wet-bulbing is difficult to quantify <xref ref-type="bibr" rid="bib1.bibx7" id="paren.32"/>.</p></list-item><list-item><label>ii.</label>
      <p id="d1e729">Exposure of an RH sensor to direct sunlight above a cloud causes a
radiation dry bias (measured RH is too low) of up to 5 <inline-formula><mml:math id="M24" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">%</mml:mi></mml:mrow></mml:math></inline-formula> in the lower
troposphere <xref ref-type="bibr" rid="bib1.bibx27 bib1.bibx50" id="paren.33"/>. The error is corrected in the
radiosonde data processing algorithm <xref ref-type="bibr" rid="bib1.bibx19" id="paren.34"/>. However, this
correction is intended for cloud-free conditions. Solar heating also
influences temperature measurements <xref ref-type="bibr" rid="bib1.bibx45" id="paren.35"/>, but the effect on
radiosonde temperature is negligible at low altitudes. For BELUGA, the
temperature and RH sensors are shielded against direct solar radiation, but
the sensor surroundings might warm and influence the measurements.
<?xmltex \hack{\newpage}?></p></list-item><list-item><label>iii.</label>
      <p id="d1e751">Furthermore, the time response for RH and <inline-formula><mml:math id="M25" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> measurements is
finite. Compared to the effects (i) and (ii), this part of the sensor behavior
can be quantified by the time constant <inline-formula><mml:math id="M26" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>. Assuming a first-order sensor
response, the time dependence of a measured signal <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> (RH or
<inline-formula><mml:math id="M28" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> in our case) is given by<disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M29" display="block"><mml:mstyle displaystyle="true" class="stylechange"/><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mi mathvariant="italic">τ</mml:mi><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:mfenced><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>with the <inline-formula><mml:math id="M30" display="inline"><mml:mrow><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> time constant <inline-formula><mml:math id="M31" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> and the ambient (“true”) signal
<inline-formula><mml:math id="M32" display="inline"><mml:mrow><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e871">The time-lag-corrected signal is<disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M33" display="block"><mml:mstyle displaystyle="true" class="stylechange"/><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="italic">τ</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>x</mml:mi><mml:mo mathvariant="normal" stretchy="false">̃</mml:mo></mml:mover><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:mfenced open="[" close="]"><mml:mrow><mml:msub><mml:mover accent="true"><mml:mi>x</mml:mi><mml:mo mathvariant="normal" stretchy="false">̃</mml:mo></mml:mover><mml:mi mathvariant="normal">m</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>⋅</mml:mo><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="italic">τ</mml:mi></mml:mrow></mml:msup></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="italic">τ</mml:mi></mml:mrow></mml:msup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>with <inline-formula><mml:math id="M34" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula> being the time step between two consecutive measurement points
<xref ref-type="bibr" rid="bib1.bibx26" id="paren.36"/>. Here, we assume that the time-corrected value (index
<inline-formula><mml:math id="M35" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>) is equal to the ambient value <inline-formula><mml:math id="M36" display="inline"><mml:mrow><mml:msub><mml:mi>x</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The tilde in
Eq. (<xref ref-type="disp-formula" rid="Ch1.E3"/>) represents the low-pass-filtered, measured time
series.</p></list-item></list></p>
      <p id="d1e1001">Although radiosonde data processing routines consider the time response error,
fast humidity changes in cold conditions are still affected <xref ref-type="bibr" rid="bib1.bibx40 bib1.bibx9" id="paren.37"/>. The time constants for the BELUGA RH sensor were estimated in a
laboratory study (see Appendix <xref ref-type="sec" rid="App1.Ch1.S1"/>) and are
<inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mtext>RH</mml:mtext></mml:msub><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M38" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> for RH and <inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:msub><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">70</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M40" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> for the internal temperature. The time constant for the
<inline-formula><mml:math id="M41" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> measurements based on the thermocouple on BELUGA was found to be below
1 <inline-formula><mml:math id="M42" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx10" id="paren.38"/> and, thus, has a minor influence on the
vertical temperature profile compared to the humidity observations.</p>
</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><?xmltex \opttitle{Sensitivity of $q$ to the RH and $T$ profile}?><title>Sensitivity of <inline-formula><mml:math id="M43" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> to the RH and <inline-formula><mml:math id="M44" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> profile</title>
      <p id="d1e1101">We perform sensitivity studies to analyze how the three error sources (cf. Sect. <xref ref-type="sec" rid="Ch1.S3.SS1"/>) for <inline-formula><mml:math id="M45" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and RH measurements combine and
influence the derivation of <inline-formula><mml:math id="M46" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>. The errors are simulated as <inline-formula><mml:math id="M47" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and RH
deviations from a synthetic reference case (grey line in Fig. <xref ref-type="fig" rid="Ch1.F3"/>), which represents a simulated measurement<?pagebreak page6351?> of a
temperature inversion combined with a decrease in RH. The temperature linearly increases by 6 <inline-formula><mml:math id="M48" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:math></inline-formula> in the 200 <inline-formula><mml:math id="M49" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> thick inversion layer, whereas RH linearly decreases from 100 <inline-formula><mml:math id="M50" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">%</mml:mi></mml:mrow></mml:math></inline-formula> to 40 <inline-formula><mml:math id="M51" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">%</mml:mi></mml:mrow></mml:math></inline-formula> in the same height range, resulting in monotonically decreasing specific humidity without a SHI.</p>
      <p id="d1e1162">First, we consider the influence of possible measurement errors in the
temperature inversion region for the <inline-formula><mml:math id="M52" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and RH sensor separately. That is,
only one sensor will be influenced by an increased or decreased signal while
keeping the other sensor reading at the reference value.</p>
      <p id="d1e1172">The magnitude of the simulated deviations (Fig. <xref ref-type="fig" rid="Ch1.F3"/>a and b) is
arbitrary, but the qualitative profile of the affected signal is according to
the error sources, as discussed in Sect. <xref ref-type="sec" rid="Ch1.S3.SS1"/>.</p>
      <p id="d1e1180">The effect of the four errors (<inline-formula><mml:math id="M53" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> or RH too high or too low in the
temperature inversion region) on the specific humidity profile is shown in
Fig. <xref ref-type="fig" rid="Ch1.F3"/>c.  An artificial humidity layer above the cloud can
emerge when the RH sensor overestimates the moisture due to wet-bulbing (but
keeping the temperature sensor unaffected), or when the temperature sensor is
heated in the inversion region but the humidity sensor is unaffected. Vice
versa, <inline-formula><mml:math id="M54" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> shows a deficit compared to the reference when one of the sensors
indicates underestimated values compared to the reference scenario. If a
single phenomenon affects both the temperature and RH sensor (e.g., solar
heating results in underestimated RH and overestimated temperature), the
errors in the determination of <inline-formula><mml:math id="M55" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> have an opposite effect and, therefore, the
overall error in <inline-formula><mml:math id="M56" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> is reduced.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3"><?xmltex \currentcnt{3}?><?xmltex \def\figurename{Figure}?><label>Figure 3</label><caption><p id="d1e1215">Sensitivity of the vertical <inline-formula><mml:math id="M57" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> profile to a deviation of <inline-formula><mml:math id="M58" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and RH compared to a reference case (grey line). Only one parameter (<inline-formula><mml:math id="M59" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> or RH) experiences a deviation in the inversion region, the other parameter is unchanged. Underestimated temperature (blue) or overestimated RH (green) might result from wet-bulbing. Overestimated temperature (purple) or underestimated RH (orange) might result from solar heating. A slow-response RH sensor overestimates RH on the ascent (green) and underestimates RH on the descent (orange).</p></caption>
          <?xmltex \igopts{width=199.169291pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f03.png"/>

        </fig>

      <p id="d1e1245">As a second step, we simulate the influence of different time constants
<inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mtext>RH</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M61" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi>T</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for the RH and temperature measurements. If
both time constants have similar values, the resulting <inline-formula><mml:math id="M62" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> does not change
significantly in magnitude, but the vertical structure shifts upwards or
downwards for an ascent or descent. With a slow-response RH sensor
(<inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mtext>RH</mml:mtext></mml:msub><mml:mo>≫</mml:mo><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi>T</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), the measured RH in the SHI region is
overestimated on the ascent and underestimated on the descent with the effects
on <inline-formula><mml:math id="M64" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> as shown in Fig. <xref ref-type="fig" rid="Ch1.F3"/>c and with an artificial SHI on the
ascent.</p>
      <p id="d1e1305">As a result of these sensitivity studies, the error in <inline-formula><mml:math id="M65" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> is reduced when
both the temperature and humidity sensors are affected by the same error
source (e.g., solar heating on both sensors), and when both sensors have
comparable time constants. Under these conditions, a detected SHI can be
considered as most likely real and does not need to be interpreted as an
artifact.</p>
</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>SHIs measured with BELUGA and radiosondes: natural feature or artifact?</title>
      <p id="d1e1323">A simple and convincing test of the possible influence of the error sources on
the SHI observations is profiling in opposite direction, that is a descent
from the free troposphere through the SHI into the cloud layer. This is
commonly impossible in case of standard radiosoundings, but feasible for the
BELUGA observations.  Figure <xref ref-type="fig" rid="Ch1.F4"/> shows vertical
profiles of RH, <inline-formula><mml:math id="M66" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>, and <inline-formula><mml:math id="M67" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> as measured by radiosounding and BELUGA on 5 June
2017.  Qualitatively, the measurements of both platforms show a similar
vertical structure with a sharp temperature inversion capping the cloud layer.
The cloud top (estimated from the observed downward terrestrial irradiance) is
situated close to the temperature inversion base. However, the cloud top
height derived from radiation observations should be treated with caution due
to the vertical separation of the radiation and thermodynamic sensors by about
20 <inline-formula><mml:math id="M68" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, corresponding to a temporal shift between the observations of
about 20 <inline-formula><mml:math id="M69" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> during profiling. In the course of the measurement period
of almost 2 h, the temperature inversion base and the cloud top remain
at almost constant altitude.  The radiosonde observation shows a layer of
increased <inline-formula><mml:math id="M70" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> between 400 and 550 <inline-formula><mml:math id="M71" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> altitude just above the
temperature inversion base. The increased specific humidity emerges from RH
remaining high within the temperature inversion, before decreasing to the free
troposphere level well above the inversion base.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><?xmltex \currentcnt{4}?><?xmltex \def\figurename{Figure}?><label>Figure 4</label><caption><p id="d1e1376">Vertical profiles of <bold>(a)</bold> relative humidity RH, <bold>(b)</bold> temperature <inline-formula><mml:math id="M72" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>, and <bold>(c)</bold> specific humidity <inline-formula><mml:math id="M73" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> measured by a radiosonde and BELUGA on 5 June 2017 (second profile). RH and <inline-formula><mml:math id="M74" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> for BELUGA are shown before and after the corrections. The radiosonde was launched at 16:50 <inline-formula><mml:math id="M75" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">UTC</mml:mi></mml:mrow></mml:math></inline-formula>; the balloon flew a continuous ascent and descent from 14:15 to 14:40 <inline-formula><mml:math id="M76" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">UTC</mml:mi></mml:mrow></mml:math></inline-formula>. The cloud top (from BELUGA radiation data) is shown as horizontal lines. Solid and dashed lines represent the BELUGA ascent and descent, respectively.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f04.png"/>

        </fig>

      <p id="d1e1432">Before comparing the <inline-formula><mml:math id="M77" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> measurements from the radiosonde to BELUGA
observations, we illustrate the effect of the applied RH correction and the
consequences for the <inline-formula><mml:math id="M78" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> profile.  Figure <xref ref-type="fig" rid="Ch1.F4"/>a shows
the uncorrected and time-response-corrected RH for an ascent and descent. The
uncorrected RH ascent profile deviates strongly from the descent in the cloud
top region. While descending through the cloud, the sensor requires a
150 <inline-formula><mml:math id="M79" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> height difference for rising from 55 <inline-formula><mml:math id="M80" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">%</mml:mi></mml:mrow></mml:math></inline-formula> to 95 <inline-formula><mml:math id="M81" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">%</mml:mi></mml:mrow></mml:math></inline-formula>
RH. The RH hysteresis around the cloud top is visible as a systematic deviation in
all observed flight data (not shown).  A comparison to Fig. <xref ref-type="fig" rid="Ch1.F3"/>
(orange lines) suggests that the major part of the error is due to a slow RH
sensor. Furthermore, the sensor underestimates RH in the cloud on the descent,
which might indicate solar heating.  After applying<?pagebreak page6352?> the time lag correction,
the RH profile shows a significantly reduced difference between ascent and
descent. The remaining difference is qualitatively consistent with the
temperature observations as shown in Fig. <xref ref-type="fig" rid="Ch1.F4"/>b. The
temperature profiles show a warming of the cloud top and inversion region
between 300 and 500 <inline-formula><mml:math id="M82" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> during the descent leading to a reduced RH.</p>
      <p id="d1e1489">The “uncorrected” specific humidity in Fig. <xref ref-type="fig" rid="Ch1.F4"/>c is
calculated from the uncorrected RH and the temperature measured with the
fast-response thermocouple. The resulting <inline-formula><mml:math id="M83" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> profiles show a SHI on the
ascent and the descent of the BELUGA flight with a similar structure and
location compared to the radiosonde data.  The <inline-formula><mml:math id="M84" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> profile as observed during
the descent is shifted to lower <inline-formula><mml:math id="M85" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> values in the region of the hysteresis of
the uncorrected RH.</p>
      <p id="d1e1515">The corrected <inline-formula><mml:math id="M86" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> results from the RH and the sensor-internal temperature
<inline-formula><mml:math id="M87" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> after correcting both signals for the time lag error
according to Eq. (<xref ref-type="disp-formula" rid="Ch1.E3"/>).  We argue that using
<inline-formula><mml:math id="M88" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> should be preferred instead of the thermocouple readings
because RH and <inline-formula><mml:math id="M89" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> have similar time constants, and RH is
measured at <inline-formula><mml:math id="M90" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> instead of the temperature of the atmospheric
environment. The ambient temperature and <inline-formula><mml:math id="M91" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> differ slightly due
to the thermal inertia of the sensor housing.</p>
      <p id="d1e1583">After applying the corrections, the maximum value of the SHI, as observed
during the BELUGA ascent, is reduced by about 0.6 <inline-formula><mml:math id="M92" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> compared
to the uncorrected <inline-formula><mml:math id="M93" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> maximum. After correction, all BELUGA profiles and the
radiosonde data exhibit the SHI with similar structure and amplitude. This
consistency suggests that the observed SHI is a natural feature instead of an
instrumental artifact. We can exclude wet-bulbing as the main reason for the
observed SHIs because the SHI is also present during the descent. The
influence of solar heating and time-lag errors is minimized. Our conclusion
also strengthens the confidence in SHIs as frequently observed by radiosondes.</p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Vertical profiles of mean ABL parameters</title>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Comparison of normalized temperature and humidity profiles</title>
      <p id="d1e1626">Throughout the observation period, we observe a persistent layer of increased
specific humidity above the cloud layer. One of the governing questions of
this analysis is to understand how observed SHIs relate to the general ABL
structure and, in particular, to the temperature
inversion. Figure <xref ref-type="fig" rid="Ch1.F5"/>a and b shows vertical profiles of
potential temperature <inline-formula><mml:math id="M94" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula> and specific humidity <inline-formula><mml:math id="M95" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> recorded in the
period of 5–7 June 2017. Both parameters are normalized to their near-surface
values and plotted in relation to the base height of the temperature inversion
<inline-formula><mml:math id="M96" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The cloud boundaries are shown in
Fig. <xref ref-type="fig" rid="Ch1.F5"/>c for reference.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5"><?xmltex \currentcnt{5}?><?xmltex \def\figurename{Figure}?><label>Figure 5</label><caption><p id="d1e1660">Balloon-borne vertical profiles of <bold>(a)</bold> potential temperature <inline-formula><mml:math id="M97" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula>, <bold>(b)</bold> specific humidity <inline-formula><mml:math id="M98" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>, and <bold>(c)</bold> cloud boundaries for four ascents (solid lines) and descents (dashed lines) on 5, 6, and 7 June 2017. The altitude <inline-formula><mml:math id="M99" display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> is normalized to the temperature inversion base height <inline-formula><mml:math id="M100" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. Potential temperature <inline-formula><mml:math id="M101" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula> and the specific humidity <inline-formula><mml:math id="M102" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> are normalized to their near-surface values. The cloud top is derived from the irradiance profile; the cloud base is derived from Cloudnet data.
The profiles are named after the start time (cf. Fig. <xref ref-type="fig" rid="Ch1.F2"/>).</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f05.png"/>

        </fig>

      <p id="d1e1727">All measurements show a similar vertical structure of <inline-formula><mml:math id="M103" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula> within the
ABL. Below the temperature inversion base <inline-formula><mml:math id="M104" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, the stratification
is near-neutral to weakly stable. Above the inversion, the thermodynamic
stability is higher and exhibits more variability compared to below the
inversion. No systematic difference between ascents and descents is
visible. The ABL is thermodynamically coupled to the surface, which makes
normalizing to surface values meaningful.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><?xmltex \currentcnt{6}?><?xmltex \def\figurename{Figure}?><label>Figure 6</label><caption><p id="d1e1751">Boundary layer observations around the cloud top on 5 June 2017, first profile: vertical profiles of <bold>(a)</bold> potential temperature <inline-formula><mml:math id="M105" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula>, <bold>(b)</bold> RH, <bold>(c)</bold> specific humidity <inline-formula><mml:math id="M106" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>, <bold>(d)</bold>
downward terrestrial irradiance <inline-formula><mml:math id="M107" display="inline"><mml:mrow><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>terr</mml:mtext><mml:mo>↓</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>,
<bold>(e)</bold> horizontal wind velocity <inline-formula><mml:math id="M108" display="inline"><mml:mi>U</mml:mi></mml:math></inline-formula>, and <bold>(f)</bold> Richardson number <inline-formula><mml:math id="M109" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> for BELUGA ascent and descent and the radiosonde launched at 11:00 <inline-formula><mml:math id="M110" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">UTC</mml:mi></mml:mrow></mml:math></inline-formula>.
The triangles indicate where <inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is defined.
The cloud top is shown as horizontal lines (solid for ascents and dashed for descents).</p></caption>
          <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f06.png"/>

        </fig>

      <p id="d1e1843">Within the mixed layer below <inline-formula><mml:math id="M112" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, specific humidity
decreases slightly with height but increases when reaching <inline-formula><mml:math id="M113" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. Above <inline-formula><mml:math id="M114" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, the normalized specific humidity exhibits more variability compared to the normalized temperature. The descent of
7 June 09 <inline-formula><mml:math id="M115" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> shows a temperature inversion with some internal structure in the form of two smaller “steps” in <inline-formula><mml:math id="M116" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula>. We define <inline-formula><mml:math id="M117" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i<?pagebreak page6353?></mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> at the lower step, with the SHI base being located clearly above at the upper step at <inline-formula><mml:math id="M118" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">1.2</mml:mn><mml:mo>⋅</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. For this case, a deficit in <inline-formula><mml:math id="M119" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> is observed below the SHI, which is plausible because between ascent and descent cloud top had decreased to about <inline-formula><mml:math id="M120" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.95</mml:mn><mml:mo>⋅</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e1947">For most profiles, the cloud top coincides with <inline-formula><mml:math id="M121" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and the
increased humidity is observed above the cloud layer.  Only for two profiles
(both descents on 5 June), the lower bound of the SHI is already located below the cloud top.  We do not find clouds penetrating into the temperature
inversion, although such situations have been frequently observed in previous
studies <xref ref-type="bibr" rid="bib1.bibx33 bib1.bibx37 bib1.bibx35 bib1.bibx39 bib1.bibx2" id="paren.39"><named-content content-type="pre">e.g., </named-content></xref>. However, two of the descent profiles (6 June 09 h and
7 June 09 h) show situations where the cloud top had decreased between ascent and descent, and the SHI is vertically separated from the cloud top.</p>
</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Cloud top variability versus SHI height</title>
      <p id="d1e1974">The cloud top variability, here defined as the cloud top height difference
between ascent and subsequent descent for each profile, is related to
<inline-formula><mml:math id="M122" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and the lower boundary of the SHI.  For all 3 d, a
descending cloud top is observed between the ascent and subsequent descent
with a cloud top height difference of 50 to 100 <inline-formula><mml:math id="M123" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. This cloud top
variability is indicated by in situ irradiance and thermodynamic measurements
and also confirmed by radar reflectivity
(cf. Fig. <xref ref-type="fig" rid="Ch1.F2"/>). In order to illustrate the relation of
cloud top height, SHI, and other ABL parameters,
Figs. <xref ref-type="fig" rid="Ch1.F6"/>–<xref ref-type="fig" rid="Ch1.F8"/> show profiles of mean <inline-formula><mml:math id="M124" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula>, RH, <inline-formula><mml:math id="M125" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>, downward
terrestrial irradiance <inline-formula><mml:math id="M126" display="inline"><mml:mrow><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>terr</mml:mtext><mml:mo>↓</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>, horizontal wind
velocity <inline-formula><mml:math id="M127" display="inline"><mml:mi>U</mml:mi></mml:math></inline-formula>, and Richardson number <inline-formula><mml:math id="M128" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> as measured during ascents and
descents on 5, 6, and 7 June, respectively. We analyze only continuous profile
data without longer breaks at certain heights for the first profile of each
day. The cloud top height is defined by the discontinuity of the
<inline-formula><mml:math id="M129" display="inline"><mml:mrow><mml:msubsup><mml:mi>F</mml:mi><mml:mtext>terr</mml:mtext><mml:mo>↓</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> profile and marked with horizontal lines,
whereas <inline-formula><mml:math id="M130" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is indicated with triangles. The Richardson number is
the ratio between thermodynamic stability and wind shear and, therefore, a
measure for the ability of turbulence generation (<inline-formula><mml:math id="M131" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M132" display="inline"><mml:mi mathvariant="italic">≲</mml:mi></mml:math></inline-formula> 1) or
dissipation (<inline-formula><mml:math id="M133" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M134" display="inline"><mml:mi mathvariant="italic">≳</mml:mi></mml:math></inline-formula> 1).</p>
      <p id="d1e2106">On 5 June (Fig. <xref ref-type="fig" rid="Ch1.F6"/>), <inline-formula><mml:math id="M135" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> lowers from 430
to 380 <inline-formula><mml:math id="M136" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> in the course of the BELUGA flight. The temperature
difference across the inversion of <inline-formula><mml:math id="M137" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="italic">θ</mml:mi><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">9</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M138" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:math></inline-formula>, which
is also the strongest observed during our flights, stays constant during
ascent and descent. The RH decreases within the temperature inversion,
accompanied by an increase in <inline-formula><mml:math id="M139" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> above <inline-formula><mml:math id="M140" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of about
0.25 <inline-formula><mml:math id="M141" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> (ascent) and 0.5 <inline-formula><mml:math id="M142" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> (descent). The
radiosonde, launched around 2 h prior to the BELUGA flight, shows a
higher <inline-formula><mml:math id="M143" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> but qualitatively a similar vertical structure of
<inline-formula><mml:math id="M144" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula>, RH, and <inline-formula><mml:math id="M145" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>.  The cloud top agrees well with <inline-formula><mml:math id="M146" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for
the ascent and descent.  The horizontal wind velocity <inline-formula><mml:math id="M147" display="inline"><mml:mi>U</mml:mi></mml:math></inline-formula> is around
2 <inline-formula><mml:math id="M148" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> inside the cloud layer and decreases to
1 <inline-formula><mml:math id="M149" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> in the free troposphere, resulting in horizontal wind
shear.  During the ascent, the wind shear zone is clearly located below
<inline-formula><mml:math id="M150" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> with a sudden increase in <inline-formula><mml:math id="M151" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> to values greater than 1 above
<inline-formula><mml:math id="M152" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud top.  During the descent, the strongest wind shear
is observed around <inline-formula><mml:math id="M153" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and the resulting increase in <inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> is
slightly above <inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. This vertical shift suggests a slightly
stronger turbulent coupling between cloud top and the SHI above, as compared
to the ascent.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><?xmltex \def\figurename{Figure}?><label>Figure 7</label><caption><p id="d1e2350">Same as Fig. <xref ref-type="fig" rid="Ch1.F6"/>, but for 6 June 2017 (first profile).</p></caption>
          <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f07.png"/>

        </fig>

      <?pagebreak page6354?><p id="d1e2362">The general ABL structure observed on 6 June (Fig. <xref ref-type="fig" rid="Ch1.F7"/>)
in terms of the profiles of <inline-formula><mml:math id="M156" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula>, RH, and <inline-formula><mml:math id="M157" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> is quite similar to the
5 June observations, showing a decreasing cloud top height during the balloon
operation. Here, <inline-formula><mml:math id="M158" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> decreases from 290 <inline-formula><mml:math id="M159" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> during the
ascent to about 230 <inline-formula><mml:math id="M160" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> during the descent. The radiosonde, launched
1.5 <inline-formula><mml:math id="M161" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> after the BELUGA flight, shows a similar <inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to the
balloon ascent, indicating that <inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud top recover between
BELUGA descent and radiosounding. This is in agreement with the radar
observations in Fig. <xref ref-type="fig" rid="Ch1.F2"/>.  The lower bound of the SHI with
<inline-formula><mml:math id="M164" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">0.3</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mrow></mml:math></inline-formula> on the ascent and
0.7 <inline-formula><mml:math id="M165" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> on the descent is coupled to <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in both
cases. On the ascent, <inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> coincides with the cloud top. During
the descent, the cloud top is almost 20 <inline-formula><mml:math id="M168" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> below <inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
which could possibly result from cloud top heterogeneity. However, the
temperature gradient is smoother compared to the ascent, which leads to a less
clear determination of <inline-formula><mml:math id="M170" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The humidity structure above the
cloud layer observed by the radiosonde exhibits a distinct SHI with a lower
bound coupled to the temperature inversion. Peak values of <inline-formula><mml:math id="M171" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> are comparable
with BELUGA observations made during the descent. The horizontal wind velocity
is about 5 <inline-formula><mml:math id="M172" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and almost height-constant for the entire ascent but increases by about 2 <inline-formula><mml:math id="M173" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> inside the cloud layer during the
descent. The radiosonde provides a similar picture to the balloon descent.
For the ascent, the sharp increase in <inline-formula><mml:math id="M174" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> is connected to <inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
whereas for the descent this increase in <inline-formula><mml:math id="M176" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> is – similar to the previous
day – about 20 <inline-formula><mml:math id="M177" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> above cloud top, allowing for some turbulent
exchange between the cloud and the SHI above.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><?xmltex \def\figurename{Figure}?><label>Figure 8</label><caption><p id="d1e2622">Same as Fig. <xref ref-type="fig" rid="Ch1.F6"/>, but for 7 June 2017.</p></caption>
          <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f08.png"/>

        </fig>

      <p id="d1e2633">On 7 June, a clear SHI develops with a lower boundary at around 580 <inline-formula><mml:math id="M178" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>,
which is similar in the two BELUGA and the radiosonde profiles
(Fig. <xref ref-type="fig" rid="Ch1.F8"/>). For the BELUGA ascent and the radiosonde
profile, this boundary agrees well with <inline-formula><mml:math id="M179" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud top (for
the radiosonde data cloud top can be roughly estimated from the RH
profile). The radiosonde profile and BELUGA ascent are shifted in time by
about 70 <inline-formula><mml:math id="M180" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> and the remarkable match in <inline-formula><mml:math id="M181" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> should not
be over-interpreted. For the BELUGA descent, the thermal stratification
changes again (similar to the previous days). The temperature inversion
weakens and <inline-formula><mml:math id="M182" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is shifted downward by about 110 to
480 <inline-formula><mml:math id="M183" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, together with the cloud top. Thus, the cloud top and the SHI
base are separated by 110 <inline-formula><mml:math id="M184" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> on the descent. The terrestrial irradiance
inside the cloud layer fluctuates strongly, especially on the descent, which
suggests a patchy cloud with cloud holes.  The horizontal wind velocity agrees
qualitatively for all three profiles. Inside the ABL, a higher wind velocity
of around 6 <inline-formula><mml:math id="M185" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> is observed with the BELUGA observations,
showing a local maximum of 8 <inline-formula><mml:math id="M186" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> slightly below
<inline-formula><mml:math id="M187" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. Above this maximum, <inline-formula><mml:math id="M188" display="inline"><mml:mi>U</mml:mi></mml:math></inline-formula> gradually decreases to
2 <inline-formula><mml:math id="M189" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> in the free troposphere. According to the Richardson
number, wind shear limits turbulence above the cloud top for both ascent and
descent.</p>
      <p id="d1e2774">To resume, we observed mean profiles of several cases where cloud tops
coincide with <inline-formula><mml:math id="M190" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and the SHI base. Although some cloud tops show
more or less strong horizontal wind shear, the stabilizing effect of the
temperature inversion leads to a sudden increase in <inline-formula><mml:math id="M191" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:mrow></mml:math></inline-formula> just above the cloud
layer, which suggests a rather low turbulent exchange with the humidity layers
above. However, for one case a special situation provides a new aspect of this
phenomenon: <inline-formula><mml:math id="M192" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and cloud top height had decreased while the
humidity layer remained at its vertical position, leading to a humidity gap
between cloud top and SHI.</p>
</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Turbulence at cloud top and around the SHI</title>
      <p id="d1e2819">Concerning the question of how the humidity and cloud layer interact and to
what extent these layers exchange energy by turbulent transport, we first
describe the interface between the SHI and cloud top by means of observations
at constant altitude (Sect. <xref ref-type="sec" rid="Ch1.S5.SS1"/>).  We then analyze the
vertical profiles of basic turbulence parameters (Sect. <xref ref-type="sec" rid="Ch1.S5.SS2"/>) and
turbulent energy fluxes (Sect. <xref ref-type="sec" rid="Ch1.S5.SS3"/>).</p><?xmltex \hack{\newpage}?>
<?pagebreak page6355?><sec id="Ch1.S5.SS1">
  <label>5.1</label><title>Observations at constant altitude in the inversion layer</title>
      <p id="d1e2836">To get an insight into the transition from cloud top to the humidity layer
above, measurements were taken at a constant height in the temperature
inversion region. Figure <xref ref-type="fig" rid="Ch1.F9"/> shows a 500 <inline-formula><mml:math id="M193" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula>
time series measured on 6 June at a constant altitude around <inline-formula><mml:math id="M194" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">300</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M195" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> (second last constant altitude segment in
Fig. <xref ref-type="fig" rid="Ch1.F2"/> for 6 June). The local dissipation rate
<inline-formula><mml:math id="M196" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> is evaluated in 2 <inline-formula><mml:math id="M197" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> segments to illustrate the evolving
turbulence intensity.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9"><?xmltex \currentcnt{9}?><?xmltex \def\figurename{Figure}?><label>Figure 9</label><caption><p id="d1e2892">Constant-altitude time series of <bold>(a)</bold> virtual potential temperature <inline-formula><mml:math id="M198" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> specific humidity <inline-formula><mml:math id="M199" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>, <bold>(c)</bold> vertical wind <inline-formula><mml:math id="M200" display="inline"><mml:mi>w</mml:mi></mml:math></inline-formula>, <bold>(d)</bold> co-variance <inline-formula><mml:math id="M201" display="inline"><mml:mrow><mml:msup><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, and <bold>(e)</bold>  dissipation rate <inline-formula><mml:math id="M202" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula>
for
6 June measured at 300 <inline-formula><mml:math id="M203" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> altitude around <inline-formula><mml:math id="M204" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.
</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f09.png"/>

        </fig>

      <p id="d1e2988">Within the first third of the record, the virtual potential temperature
<inline-formula><mml:math id="M205" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (as approximately measured by the ultrasonic anemometer)
shows strong variations on a typical timescale of 30–50 <inline-formula><mml:math id="M206" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> with
amplitudes up to 3 <inline-formula><mml:math id="M207" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:math></inline-formula>. Based on the temperature gradient
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>), the changes in <inline-formula><mml:math id="M208" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> would
correspond to a height variation of <inline-formula><mml:math id="M209" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula>. More likely, parts of
the height-constant measurements (<inline-formula><mml:math id="M210" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>z</mml:mi><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M211" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>) are taken in
potentially colder, drier, and more turbulent air masses at the inversion base,
interrupted by measurements in potentially warmer, more humid, and less turbulent
air masses at higher altitudes well within the <inline-formula><mml:math id="M212" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> inversion. This variability
is also visible in the wind direction (not shown here). Depending on the
relative location of <inline-formula><mml:math id="M213" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to the measurement height, the
co-variance <inline-formula><mml:math id="M214" display="inline"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> is highly intermittent and no mean flux
is derived from these observations.</p>
      <p id="d1e3105">The center part of the record is characterized by a comparably low variability
leading to the conclusion that this part of the observations is performed
entirely inside the descending temperature inversion. Finally, observations
are performed well above <inline-formula><mml:math id="M215" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> inside the stably stratified <inline-formula><mml:math id="M216" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula>
inversion layer, characterized by values of <inline-formula><mml:math id="M217" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> 1 order of
magnitude lower compared to at the inversion base. Here, variations in
<inline-formula><mml:math id="M218" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M219" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> are again correlated and caused by changes in
relative height.</p>
      <p id="d1e3151">The observations do not allow for drawing quantitative conclusions, such as
time and area-averaged turbulent heat fluxes, from this record. However, these
measurements vividly illustrate the difficulties in estimating turbulent
fluxes based on covariance methods in the vicinity of the temperature
inversion, although the measurement height is kept at a remarkably constant
height level. Therefore, the methods for estimating turbulent fluxes based on
mean vertical gradients and slant profiles are more suitable for this study
and are used below.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10" specific-use="star"><?xmltex \currentcnt{10}?><?xmltex \def\figurename{Figure}?><label>Figure 10</label><caption><p id="d1e3156">Vertical profiles of local dissipation rate <inline-formula><mml:math id="M220" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> and TKE for the first ascent and descent of 5, 6, and 7 June 2017. The height is normalized by the temperature inversion base <inline-formula><mml:math id="M221" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The region of increased specific humidity is marked as blue shading, the cloud layer as grey shading.</p></caption>
          <?xmltex \igopts{width=398.338583pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f10.png"/>

        </fig>

</sec>
<sec id="Ch1.S5.SS2">
  <label>5.2</label><title>Vertical profiles of turbulent energy and dissipation</title>
      <?pagebreak page6356?><p id="d1e3191">The vertical distribution of turbulence parameters, such as local dissipation
rate <inline-formula><mml:math id="M222" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> and the turbulent kinetic energy TKE, provide an insight
into the coupling between the cloud layer and the SHI.  The local
<inline-formula><mml:math id="M223" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> values are derived from second-order structure functions by
applying inertial subrange scaling as described by
<xref ref-type="bibr" rid="bib1.bibx10" id="text.40"/>. Different from that study, here <inline-formula><mml:math id="M224" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> is
calculated from non-overlapping, 2 <inline-formula><mml:math id="M225" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> sub-records yielding a vertical
resolution of about 2 <inline-formula><mml:math id="M226" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. Regions without inertial sub-range scaling
are excluded.  Turbulent kinetic energy (<inline-formula><mml:math id="M227" display="inline"><mml:mrow><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn><mml:mo>⋅</mml:mo><mml:msubsup><mml:mi>u</mml:mi><mml:mi>i</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow></mml:math></inline-formula>) is calculated
in a moving 50 <inline-formula><mml:math id="M228" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> window. The observed TKE noise level is about
0.005 <inline-formula><mml:math id="M229" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and is usually reached at <inline-formula><mml:math id="M230" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>/</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M231" display="inline"><mml:mi mathvariant="italic">≳</mml:mi></mml:math></inline-formula> 1.1.</p>
      <p id="d1e3304">Figure <xref ref-type="fig" rid="Ch1.F10"/> shows <inline-formula><mml:math id="M232" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> and TKE for each first
profile of 5, 6, and 7 June as a function of normalized height (the descent of
5 June is excluded due to data issues). The cloud and humidity layers are
shaded for reference.  For the presented cases, turbulence is most pronounced
in the upper cloud layer and around cloud top with typical values of
<inline-formula><mml:math id="M233" display="inline"><mml:mrow><mml:mi mathvariant="italic">ε</mml:mi><mml:mo>∼</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M234" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and
TKE <inline-formula><mml:math id="M235" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 0.02 <inline-formula><mml:math id="M236" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. For 5 and 6 June, the turbulence
intensity is rather constant in the cloud. For 7 June, with increased wind
velocity, a maximum of <inline-formula><mml:math id="M237" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> is evident just below cloud top.</p>
      <p id="d1e3389">Figure <xref ref-type="fig" rid="Ch1.F10"/> also illustrates how the SHI and cloud layer
are either separated or overlap, and how they are connected by turbulent
motion. At a certain height level, <inline-formula><mml:math id="M238" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula> decreases to the
low-turbulence free-troposphere level. The transition is gradual, indicating
turbulent mixing in this region.  On 5 June and the ascents of 6 and 7 June,
the SHI and the cloud are directly coupled by turbulent mixing.  For the
descents of 6 and 7 June, most of the mixing takes place at the interface of
the cloud top with the humidity gap between cloud and SHI. In this case,
inside the SHI the turbulence intensity is reduced almost to the
free-troposphere level and the SHI seems to be decoupled from the cloud layer
via the humidity gap in between.</p>
      <p id="d1e3401">We can only speculate about the reason for the development of this humidity
gap, which is most pronounced for the descent of 7 June.  One explanation
could be long-range advection of increased moisture in the free troposphere
combined with a temporary collapse of the well-mixed cloud layer leading to a
vertical separation of cloud top and SHI. However, this interesting feature
leads to new research questions that require further observations and a more
detailed LES analysis.</p>
</sec>
<sec id="Ch1.S5.SS3">
  <label>5.3</label><title>Vertical profiles of turbulent moisture and heat fluxes</title>
      <p id="d1e3413">The turbulent exchange of moisture can be quantified by the latent heat flux

                <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M239" display="block"><mml:mstyle displaystyle="true" class="stylechange"/><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mi>L</mml:mi><mml:mo>=</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">ρ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>⋅</mml:mo><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mi>q</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          whereas the virtual sensible heat flux is given by

                <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M240" display="block"><mml:mstyle class="stylechange" displaystyle="true"/><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi>H</mml:mi><mml:mo>=</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">ρ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>⋅</mml:mo><mml:msub><mml:mi>c</mml:mi><mml:mi>p</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          with an overline describing an average of the sub-record.  Here,
<inline-formula><mml:math id="M241" display="inline"><mml:mover accent="true"><mml:mi mathvariant="italic">ρ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> is the mean air density, <inline-formula><mml:math id="M242" display="inline"><mml:mrow><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2.5</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">6</mml:mn></mml:msup><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">J</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:mrow></mml:math></inline-formula> is the latent heat of evaporation, and
<inline-formula><mml:math id="M243" display="inline"><mml:mrow><mml:msub><mml:mi>c</mml:mi><mml:mi>p</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1005</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M244" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">J</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">K</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> is the specific heat capacity of air.
This direct calculation of <inline-formula><mml:math id="M245" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M246" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> requires sufficient long, stationary,
and homogeneous records in a certain height to provide time-averaged estimates
of the covariances with statistical significance
<xref ref-type="bibr" rid="bib1.bibx44 bib1.bibx24" id="paren.41"/>. Our observations focus mainly on vertical
profiling, and only a limited number of height-constant records around the
cloud top and inversion region are available. As shown in
Sect. <xref ref-type="sec" rid="Ch1.S5.SS1"/>, the conditions around the temperature inversion are
highly instationary and, thus, we use the vertical profiles to study the
fluxes in this region. We apply two approaches for estimating fluxes from
vertical profiles: (i) describing the flux profile by applying the so-called
“slant profile method” and (ii) relating the turbulent flux to mean
gradients (flux gradient method).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11" specific-use="star"><?xmltex \currentcnt{11}?><?xmltex \def\figurename{Figure}?><label>Figure 11</label><caption><p id="d1e3610">Same as Fig. <xref ref-type="fig" rid="Ch1.F10"/>, but for the virtual sensible heat flux <inline-formula><mml:math id="M247" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> (eddy covariance method) and the latent heat flux <inline-formula><mml:math id="M248" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> (flux gradient method).
</p></caption>
          <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f11.png"/>

        </fig>

      <?pagebreak page6357?><p id="d1e3635">The slant profile method is based on the assumption that for a certain height
range the profile data are considered as a homogeneous record and
Eq. (<xref ref-type="disp-formula" rid="Ch1.E5"/>) can be applied. For this method, instantaneous
values of <inline-formula><mml:math id="M249" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> are estimated for a defined height range, defining also the
length scales contributing to the flux. For our observations, this method
provides only results for <inline-formula><mml:math id="M250" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> due to the lack of fast-response humidity
measurements. Alternatively, <inline-formula><mml:math id="M251" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> can be estimated with the flux gradient
method. This method is based on the relation between the covariances and the
mean gradients of <inline-formula><mml:math id="M252" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M253" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>:

                <disp-formula id="Ch1.E6" content-type="numbered"><label>6</label><mml:math id="M254" display="block"><mml:mstyle class="stylechange" displaystyle="true"/><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msubsup><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi><mml:mo>′</mml:mo></mml:msubsup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:msub><mml:mover accent="true"><mml:mi mathvariant="italic">θ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>z</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          and

                <disp-formula id="Ch1.E7" content-type="numbered"><label>7</label><mml:math id="M255" display="block"><mml:mstyle displaystyle="true" class="stylechange"/><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mover accent="true"><mml:mrow><mml:msup><mml:mi>w</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:msup><mml:mi>q</mml:mi><mml:mo>′</mml:mo></mml:msup></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mi>Q</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mo>∂</mml:mo><mml:mover accent="true"><mml:mi>q</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>z</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>

          with <inline-formula><mml:math id="M256" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M257" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>Q</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> being the turbulent exchange coefficients for
sensible and latent heat, respectively. The coefficients are defined as
positive, which means that the flux is directed against the mean
gradient. Values of <inline-formula><mml:math id="M258" display="inline"><mml:mi>K</mml:mi></mml:math></inline-formula> can be derived from parameterizations based on
turbulence observations such as proposed by <xref ref-type="bibr" rid="bib1.bibx16" id="text.42"/> or by directly
applying Eq. (<xref ref-type="disp-formula" rid="Ch1.E6"/>) with the measured <inline-formula><mml:math id="M259" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula>, yielding
<inline-formula><mml:math id="M260" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. With <inline-formula><mml:math id="M261" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>Q</mml:mi></mml:msub><mml:mo>≈</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx8" id="paren.43"/> for a wide range of
stratification and the mean humidity gradient <inline-formula><mml:math id="M262" display="inline"><mml:mrow><mml:mo>∂</mml:mo><mml:mover accent="true"><mml:mi>q</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>/</mml:mo><mml:mo>∂</mml:mo><mml:mi>z</mml:mi></mml:mrow></mml:math></inline-formula>, we estimate <inline-formula><mml:math id="M263" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> by combining Eqs. (<xref ref-type="disp-formula" rid="Ch1.E7"/>) and
(<xref ref-type="disp-formula" rid="Ch1.E4"/>).</p>
      <p id="d1e3891">Before estimating <inline-formula><mml:math id="M264" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> from the slant profiles by applying
Eq. (<xref ref-type="disp-formula" rid="Ch1.E5"/>), the turbulent fluctuations must be
determined. This is done by applying a high-pass filter of Bessel type with a
filter window of 10 <inline-formula><mml:math id="M265" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula>, corresponding to a horizontal length scale of
about 10 to 70 <inline-formula><mml:math id="M266" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> (depending on the horizontal wind velocity) and a
vertical length scale of about 10 <inline-formula><mml:math id="M267" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. After filtering, the fluxes are
averaged over a moving 50 <inline-formula><mml:math id="M268" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> window by applying
Eq. (<xref ref-type="disp-formula" rid="Ch1.E5"/>). The filter and averaging windows are similar to
the values proposed by <xref ref-type="bibr" rid="bib1.bibx46" id="text.44"/> and <xref ref-type="bibr" rid="bib1.bibx23" id="text.45"/>, who
estimated turbulent fluxes from aircraft-based slant profiles.</p>
      <p id="d1e3944">Figure <xref ref-type="fig" rid="Ch1.F11"/> shows five selected cases
(cf. Fig. <xref ref-type="fig" rid="Ch1.F10"/>) with profiles of <inline-formula><mml:math id="M269" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> based on the slant
profile method and <inline-formula><mml:math id="M270" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> based on the flux gradient method.  The upper part of
the cloud layer is mainly characterized by an upward-oriented heat flux (<inline-formula><mml:math id="M271" display="inline"><mml:mrow><mml:mi>H</mml:mi><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>), most pronounced for the last two profiles with a local maximum between
<inline-formula><mml:math id="M272" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.8</mml:mn><mml:mo>&lt;</mml:mo><mml:mi>z</mml:mi><mml:mo>/</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>. Only for the first ascent of 5 June is the <inline-formula><mml:math id="M273" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula>
flux almost height-constant with much lower values compared to the other
days. For this day, <inline-formula><mml:math id="M274" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> exhibits larger variability around
and slightly above <inline-formula><mml:math id="M275" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, which differs from the typical structure
of a turbulent flow. This variability mainly causes the positive values of <inline-formula><mml:math id="M276" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula>
around <inline-formula><mml:math id="M277" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, which, therefore, should not be misinterpreted. This
is a similar effect to that discussed in Sect. <xref ref-type="sec" rid="Ch1.S5.SS1"/>. A negative peak
of <inline-formula><mml:math id="M278" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> around or slightly above <inline-formula><mml:math id="M279" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is visible for the descent of
6 June and both profiles of 7 June. On 7 June, a secondary, weaker negative
peak in <inline-formula><mml:math id="M280" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> is located at the lower part of the SHI.</p>
      <p id="d1e4076">Although it is known that in general <inline-formula><mml:math id="M281" display="inline"><mml:mrow><mml:mi>K</mml:mi><mml:mo>=</mml:mo><mml:mi>K</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, we estimate a constant
<inline-formula><mml:math id="M282" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for each ascent and descent in the lower region of the SHI, which is
the focus area of our study. In that region, we observe negative <inline-formula><mml:math id="M283" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> fluxes
and positive <inline-formula><mml:math id="M284" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> gradients.  Applying
Eq. (<xref ref-type="disp-formula" rid="Ch1.E6"/>) leads to mean values of <inline-formula><mml:math id="M285" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> between 0.001 and
0.004 <inline-formula><mml:math id="M286" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> for the five profiles. The <inline-formula><mml:math id="M287" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>H</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mi>Q</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> values
for each profile are used for calculating the <inline-formula><mml:math id="M288" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> profile based on the flux
gradient method.</p>
      <p id="d1e4189">A negative peak in <inline-formula><mml:math id="M289" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> is observed for all days in the lower SHI region. The
downward energy flux at cloud top is common for the entrainment region, where
potentially warmer and usually drier air from the free troposphere is mixed
downward into the (cloudy) ABL.  However, for our observations, this downward
flux in the lower SHI region means a downward transport of potentially warmer
but more humid air into the region below. The situation is different for the
descent profile of 7 June, with the vertical humidity gap between cloud top
and SHI. Here, the negative peak in <inline-formula><mml:math id="M290" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> at the lower SHI is accompanied by a
positive <inline-formula><mml:math id="M291" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> at cloud top. This profile does not suggest a significant
transport of humidity into the cloud top. Instead, for the special case where
the cloud and the SHI are separated, the gap in between receives moisture from
both the SHI above and from the cloud layer below.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F12" specific-use="star"><?xmltex \currentcnt{12}?><?xmltex \def\figurename{Figure}?><label>Figure 12</label><caption><p id="d1e4215">LES results (with and without an initial SHI) and BELUGA observations for 7 June 2017: vertical profiles of <bold>(a)</bold> virtual potential temperature <inline-formula><mml:math id="M292" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(b)</bold> specific humidity <inline-formula><mml:math id="M293" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula>, <bold>(c)</bold> liquid (LWC) and ice water content (IWC), <bold>(d)</bold> virtual sensible heat flux <inline-formula><mml:math id="M294" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula>, and <bold>(e)</bold> latent heat flux <inline-formula><mml:math id="M295" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula>. The light blue area is the cloud extent for the observations (cloud top is derived from BELUGA irradiance measurements, cloud base from lidar data).
</p></caption>
          <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f12.png"/>

        </fig>

</sec>
</sec>
<?pagebreak page6358?><sec id="Ch1.S6">
  <label>6</label><title>Possible influence of the humidity layer on ABL and cloud structure: an LES study</title>
      <p id="d1e4281">The observational data discussed so far provide insight into the turbulent
structure of cloudy ABLs that are capped by humidity layers. What remains
unclear is how the presence of such humidity layers might have impacted the
general ABL and clouds as observed on this day. For this purpose numerical
experiments at cloud- and turbulence-resolving resolutions can be used to good effect, providing virtual datasets for detailed process studies and allowing sensitivity tests for hypothesis testing <xref ref-type="bibr" rid="bib1.bibx41" id="paren.46"/>. In this section idealized Lagrangian large-eddy simulations (LESs) are discussed that were generated to match the observed vertical structure of the ABL as closely as possible. For a detailed technical description of the experimental design of these realizations, we refer to Appendix <xref ref-type="sec" rid="App1.Ch1.S2"/>. Two simulations are discussed, one based on an initial profile without a SHI, the other with a SHI superimposed. The LES simulations are Lagrangian, following an air mass from a location 12 <inline-formula><mml:math id="M296" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> upstream of the RV <italic>Polarstern</italic>. This allows for proper model spinup and also gives the SHI ample time to impact the turbulence and clouds below. The simulations are sampled when the air mass arrives at RV <italic>Polarstern</italic> on 7 June 2017 at 10:48 <inline-formula><mml:math id="M297" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">UTC</mml:mi></mml:mrow></mml:math></inline-formula>. The LES output considered includes the mean thermodynamic and cloudy state, as well as the turbulent fluxes of heat <inline-formula><mml:math id="M298" display="inline"><mml:mi>H</mml:mi></mml:math></inline-formula> and moisture <inline-formula><mml:math id="M299" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula>, calculated as the covariance between vertical velocity and perturbations in static energy and humidity, respectively.</p>
      <p id="d1e4326">Figure <xref ref-type="fig" rid="Ch1.F12"/> shows vertical profiles of the LES output (with
and without an initial SHI) and the BELUGA ascent, where cloud top,
<inline-formula><mml:math id="M300" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and SHI base coincide. The LES profiles represent averages
over the horizontal domain over a 900 <inline-formula><mml:math id="M301" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> period. The temperature
differences across the inversion as well as the lapse rates above are
reasonably well reproduced by the LES (Fig. <xref ref-type="fig" rid="Ch1.F12"/>a). The
experiment including an initial SHI features a temperature inversion base
<inline-formula><mml:math id="M302" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and similarly a mixed-layer depth, that agrees well with the
observations. Without the initial humidity layer, <inline-formula><mml:math id="M303" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is
approximately 40 <inline-formula><mml:math id="M304" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> lower. The vertical profile of specific humidity
shows a similar vertical structure and a distinct increase in <inline-formula><mml:math id="M305" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> above the
cloud layer in both the model and the observations
(Fig. <xref ref-type="fig" rid="Ch1.F12"/>b). The strength of the SHI of <inline-formula><mml:math id="M306" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1.1</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M307" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> in the LES is close to the radiosonde SHI strength of
<inline-formula><mml:math id="M308" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.9</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M309" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, but larger than the SHI observed with
BELUGA of <inline-formula><mml:math id="M310" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.6</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M311" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. In the LES without initial SHI,
specific humidity decreases by <inline-formula><mml:math id="M312" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">0.2</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M313" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>
within the temperature inversion height range. Within the mixed layer, both
experiments slightly underestimate <inline-formula><mml:math id="M314" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">θ</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M315" display="inline"><mml:mi>q</mml:mi></mml:math></inline-formula> compared to
the BELUGA soundings. This is probably explained by the calibration of these
experiments to the radiosonde soundings, which show a similar offset compared
to BELUGA (cf. Fig. <xref ref-type="fig" rid="Ch1.F8"/>).</p>
      <p id="d1e4538">Compared to the balloon measurements, a thinner liquid cloud layer forms in
the LES, as indicated in the LWC profiles in
Fig. <xref ref-type="fig" rid="Ch1.F12"/>c. While the observed mixed-phase cloud is around
500 <inline-formula><mml:math id="M316" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> thick, the simulations result in a liquid cloud of about
300 <inline-formula><mml:math id="M317" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> vertical extent. Note that significant ice water is present
below the liquid cloud base in the model, for which lidar readings are
sensitive <xref ref-type="bibr" rid="bib1.bibx5" id="paren.47"/>. For this reason, the model bias in cloud base
height could be artificial. Without a humidity layer, the liquid cloud is
thinner, extending only 260 <inline-formula><mml:math id="M318" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>. The cloud top is simulated at around
600 <inline-formula><mml:math id="M319" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> altitude for the scenario with SHI and at 560 <inline-formula><mml:math id="M320" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> altitude
for the scenario without SHI, respectively. In the SHI case, the higher cloud
top reflects the larger mixed-layer depth compared to the case without SHI.</p>
      <?pagebreak page6359?><p id="d1e4587">The LES provides a positive (i.e., upward-directed) virtual sensible heat flux
inside the cloud layer (Fig. <xref ref-type="fig" rid="Ch1.F12"/>d). The negative virtual
heat flux at cloud top is seen with and without initial SHI.  The LES, with or
without an initial SHI, shows a positive moisture flux <inline-formula><mml:math id="M321" display="inline"><mml:mi>L</mml:mi></mml:math></inline-formula> between surface and
cloud top (Fig. <xref ref-type="fig" rid="Ch1.F12"/>e). In the presence of an initial SHI,
the cloud top region exhibits a negative moisture flux.  This negative
moisture flux coincides with the negative virtual sensible heat flux and
indicates that downward humidity transport takes place between the humidity
layer and the underlying mixed layer. Lacking the initial SHI, the total
moisture flux is close to zero near the inversion. This means that in this
case dry air, rather than humidity, is entrained into the mixed layer from
above. The direction of fluxes is in agreement with the flux estimates in
Sect. <xref ref-type="sec" rid="Ch1.S5.SS3"/> for 7 June, where a SHI is present above cloud top
on the ascent.</p>
      <p id="d1e4604">More research is necessary to further investigate how the additional entrained
moisture of the humidity layer is processed in the cloud (e.g., through phase
transition) and how exactly the humidity layer contributes to the cloud
evolution (e.g., the role of clouds penetrating into the inversion or
thermodynamically decoupled clouds).</p>
</sec>
<sec id="Ch1.S7" sec-type="conclusions">
  <label>7</label><title>Summary and conclusion</title>
      <p id="d1e4615">A persistent layer of increased specific humidity above a stratocumulus deck
has been observed by tethered-balloon-borne instrumentation in the Fram Strait
northwest of Svalbard (82<inline-formula><mml:math id="M322" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, 10<inline-formula><mml:math id="M323" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) in the period from 5
to 7 June 2017. Vertical profiles of thermodynamic parameters, wind velocity,
and terrestrial irradiance were sampled in situ. An in-depth discussion of the
problems associated with humidity measurements in cloudy and cold environments
led to the conclusion that the observed SHIs are a natural feature and not a
result of measurement artifacts.  The high resolution of the measurements
allows for estimating local turbulence parameters such as local energy
dissipation rates. Based on slant profiles, the turbulent virtual sensible
heat flux was estimated by applying the eddy covariance method. The vertical
profile of the latent heat flux was calculated by applying the flux gradient
method.  The observations allow for the first time detailed analyses of the
relative position of the SHI, cloud top, and the temperature inversion height
<inline-formula><mml:math id="M324" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and give a first qualitative indication of how these
different layers are coupled by turbulent transport.</p>
      <p id="d1e4647"><?xmltex \hack{\newpage}?>We observed two different scenarios: (i) the base of the SHI qualitatively
coincides with <inline-formula><mml:math id="M325" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and the cloud top height and (ii) cloud top
height and <inline-formula><mml:math id="M326" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> had decreased with the SHI base remaining at a
constant height, leading to a “humidity gap” between cloud top and SHI base.
Turbulence, as described by local <inline-formula><mml:math id="M327" display="inline"><mml:mi mathvariant="italic">ε</mml:mi></mml:math></inline-formula>, decreases gradually above
<inline-formula><mml:math id="M328" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> suggesting that turbulent energy exchange is possible in that
region. Vertical profiles of latent heat fluxes qualitatively show a downward
moisture transport at the base of the SHIs for all profiles. When the SHI
coincides with the cloud top as in the first scenario (i), this suggests the
cloud is being supplied with moisture from the overlying SHI. For the second
scenario (ii), the sign of the latent heat fluxes suggests upward humidity
transport from the cloud together with downward humidity transport from the
SHI base, both feeding the vertical gap between the SHI base and the cloud top
with moisture.</p>
      <p id="d1e4691">For one case study of the first type of scenario, LESs were performed. The
simulations support the observational findings by showing a negative moisture
flux at the SHI base towards the cloud region below. Further, the LESs show
that the moisture supply does directly influence the dynamics of the cloudy
ABL by increasing <inline-formula><mml:math id="M329" display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mi mathvariant="normal">i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and the cloud layer thickness.</p>
      <p id="d1e4705">For more general conclusions beyond case studies, further observations over a
larger measurement period are necessary. An improvement for future
measurements would be a fast-response humidity sensor that operates reliably
under cold and cloudy conditions. Those observations would allow for
quantifying the vertical moisture transport by applying the eddy covariance
method instead of relying on estimating the exchange coefficient and mean
humidity gradients.</p>
      <p id="d1e4709">Furthermore, we suggest a thorough LES study driven by our observations. These
studies are capable of investigating the consequences of the two observed
scenarios on ABL dynamics and cloud lifetime and will help to answer the
question of how important the SHIs are for the Arctic cloudy ABL.</p><?xmltex \hack{\clearpage}?>
</sec>

      
      </body>
    <back><app-group>

<?pagebreak page6360?><app id="App1.Ch1.S1">
  <?xmltex \currentcnt{A}?><label>Appendix A</label><title>Estimating the time constants of the BELUGA humidity sensor</title>

      <?xmltex \floatpos{h!}?><fig id="App1.Ch1.S1.F13"><?xmltex \currentcnt{A1}?><?xmltex \def\figurename{Figure}?><label>Figure A1</label><caption><p id="d1e4726">Time response of the humidity sensor to a step function experiment: <bold>(a)</bold> sensor-internal temperature <inline-formula><mml:math id="M330" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <bold>(b)</bold> RH at 8.6 <inline-formula><mml:math id="M331" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> with fitted time constants <inline-formula><mml:math id="M332" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>. Panel <bold>(c)</bold> shows the time constants depending on the flow speed. A root fit function is added to the values.</p></caption>
        <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/21/6347/2021/acp-21-6347-2021-f13.png"/>

      </fig>

      <p id="d1e4780"><?xmltex \hack{\noindent}?>We determine the time constants for the BELUGA humidity sensor in laboratory
experiments by analyzing the sensor response to a step-like change of the
surrounding thermodynamical parameters. The sensor is brought from a calm and
saturated environment into a sub-saturated airstream with constant <inline-formula><mml:math id="M333" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and RH.
The flow speed of the sub-saturated air is varied between 2 and
9 <inline-formula><mml:math id="M334" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>.  In addition to RH, the sensor provides a measure for the
internal sensor temperature <inline-formula><mml:math id="M335" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, which is determined by a PT-1000.</p>
      <p id="d1e4819">Figure <xref ref-type="fig" rid="App1.Ch1.S1.F13"/>a and b show an example for the time response of the
humidity sensor on BELUGA. The time constants <inline-formula><mml:math id="M336" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mtext>RH</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M337" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> are obtained from an exponential fit to the response
function at a constant flow speed of
8.6 <inline-formula><mml:math id="M338" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">s</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. Figure <xref ref-type="fig" rid="App1.Ch1.S1.F13"/>c summarizes the
resulting time constants for different flow speeds. The time constant of a
temperature and RH sensor is influenced by the heat and moisture transfer,
which scale with the flow speed <inline-formula><mml:math id="M339" display="inline"><mml:mrow><mml:mo>∝</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:msqrt><mml:mi>U</mml:mi></mml:msqrt></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx4" id="paren.48"><named-content content-type="pre">e.g.,</named-content><named-content content-type="post">for heat
transfer</named-content></xref>. Based on this relationship, a least-square fit to the
observations yields the <inline-formula><mml:math id="M340" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> values depending on the flow speed.  For flow
speeds typical for atmospheric observations, we estimate time constants of
<inline-formula><mml:math id="M341" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:msub><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">70</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M342" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M343" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mtext>RH</mml:mtext></mml:msub><mml:mo>≈</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M344" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">s</mml:mi></mml:mrow></mml:math></inline-formula>. Similar to <xref ref-type="bibr" rid="bib1.bibx26" id="text.49"/>, we multiply the estimated
time constant with a factor of 0.8 before the time series reconstruction to
avoid potential over-correction.</p>
      <p id="d1e4954">For the reconstruction of the time series, <inline-formula><mml:math id="M345" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula> is evaluated for each
measurement point with the measured wind velocity by applying
Eq. (<xref ref-type="disp-formula" rid="Ch1.E3"/>). Low-pass filtering in
Eq. (<xref ref-type="disp-formula" rid="Ch1.E3"/>) is realized by a Savitzky–Golay filter with a
window length of <inline-formula><mml:math id="M346" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>.  This low-pass filtering is necessary to avoid
amplification of gradients caused by signal noise or digitization steps
<xref ref-type="bibr" rid="bib1.bibx26" id="paren.50"/>.  The time-response correction is applied to the RH
and the internal temperature data.</p><?xmltex \hack{\newpage}?>
</app>

<app id="App1.Ch1.S2">
  <?xmltex \currentcnt{B}?><label>Appendix B</label><title>LES model configuration</title>
      <p id="d1e4987">In this study the LES configuration as designed by <xref ref-type="bibr" rid="bib1.bibx31" id="text.51"/> for the
PASCAL observation period 5–7 June 2017 is adopted. For the full details of
this method, we refer to this publication, the essence of which can be
summarized as follows. The Dutch Atmospheric Large-Eddy Simulation model
<xref ref-type="bibr" rid="bib1.bibx17" id="paren.52"><named-content content-type="pre">DALES,</named-content></xref> is used, being equipped with a well-established
double-moment mixed-phase microphysics scheme <xref ref-type="bibr" rid="bib1.bibx38" id="paren.53"/>. A
Lagrangian framework is adopted, following cloudy mixed layers as embedded in
warm air masses moving towards the RV <italic>Polarstern</italic>. The large-scale
forcings along the 950 <inline-formula><mml:math id="M347" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">hPa</mml:mi></mml:mrow></mml:math></inline-formula> back trajectory are derived from an
amalgamation of analysis and short-range forecast data of the European Centre
for Medium-range Weather Forecasts (ECMWF), using the method as described by
<xref ref-type="bibr" rid="bib1.bibx49" id="text.54"/>. The initial profiles are obtained by sampling the ECMWF
data at a specified location and time point upstream of the ship and are
further adjusted in a reverse engineering approach to yield a good agreement
with the RV <italic>Polarstern</italic> radiosonde in terms of mixed-layer depth and
thermodynamic state. The surface temperature along the trajectory is
prescribed, while the surface fluxes are interactive, resulting in weakly
coupled cloudy mixed layers. In this setup, the low-level turbulence and
clouds are free to evolve.</p>
      <p id="d1e5019"><xref ref-type="bibr" rid="bib1.bibx31" id="text.55"/> thoroughly evaluated these LES simulations against PASCAL
measurements, reporting satisfactory agreement concerning the thermodynamic
state, clouds, and surface radiative fluxes. The observed SHIs were less well
reproduced, with their strength and depth somewhat underestimated. To improve
on this underestimation, and to cater to the specific needs of this study, two
new simulations were conducted for 7 June 2017, adopting a configuration that
slightly differs from the setup described above at the following points:
<list list-type="bullet"><list-item>
      <p id="d1e5026">Instead of 48 <inline-formula><mml:math id="M348" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> the model initializes only 12 <inline-formula><mml:math id="M349" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> before the arrival of the simulated air mass at RV <italic>Polarstern</italic>. A shorter lead time facilitates the adjustment of the initial profile for obtaining a good agreement with the observed sounding in terms of temperature and inversion height. On the other hand, a period of 12 <inline-formula><mml:math id="M350" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi></mml:mrow></mml:math></inline-formula> is still long enough to allow complete spinup of the mixed-phase clouds and turbulence.</p></list-item><list-item>
      <p id="d1e5057">The simulated doubly periodic and homogeneously forced domain has dimensions of <inline-formula><mml:math id="M351" display="inline"><mml:mrow><mml:mn mathvariant="normal">2.56</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">2.56</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1.28</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M352" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">km</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> discretized at a spatial resolution of <inline-formula><mml:math id="M353" display="inline"><mml:mrow><mml:mn mathvariant="normal">20</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">20</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M354" display="inline"><mml:mrow class="unit"><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>, adopting flexible time-stepping to ensure numerical stability.</p></list-item><list-item>
      <p id="d1e5115">The initial state derived from the ECMWF data is adjusted by lowering the thermal inversion height, following the method of <xref ref-type="bibr" rid="bib1.bibx31" id="text.56"/>. A second initial profile is then obtained by superimposing a humidity layer of 200 <inline-formula><mml:math id="M355" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> depth and 0.5 <inline-formula><mml:math id="M356" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> strength on this<?pagebreak page6361?> initial profile, placed immediately above the new temperature inversion. These values reflect the structure of the observed SHIs.</p></list-item><list-item>
      <p id="d1e5147">The surface sensible and latent heat fluxes are switched off, in effect decoupling the cloud layer from the surface. Imposing a surface decoupling has proven to be an effective way to maintain humidity inversions <xref ref-type="bibr" rid="bib1.bibx41" id="paren.57"/>. It should be noted that no measurements were made of the surface heat fluxes along the upstream trajectory, preventing us from assessing the validity of this modification.</p></list-item></list>
<?xmltex \hack{\newpage}?><?xmltex \hack{\noindent}?>These modifications yield two cases, one with and one without an initial SHI. These cases are idealized but include one realization in which the strength and depth of the humidity layer agree well with the observations. In combination, the SHI and no-SHI experiments provide insight into the impact of this feature on the observed evolution and behavior of turbulence and clouds on this day.</p><?xmltex \hack{\clearpage}?>
</app>
  </app-group><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e5162">Observational data related to the present article are available with open access through PANGAEA – Data Publisher for Earth &amp; Environmental Science: <ext-link xlink:href="https://doi.org/10.1594/PANGAEA.899803" ext-link-type="DOI">10.1594/PANGAEA.899803</ext-link> <xref ref-type="bibr" rid="bib1.bibx11" id="paren.58"/>. The full LES case configuration, as well as a selection of standard output, are available online at <uri>https://doi.pangaea.de/10.1594/PANGAEA.919946</uri> <xref ref-type="bibr" rid="bib1.bibx30" id="paren.59"/>.</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e5180">UE and MG performed the measurements and analyzed the observational data. HS was responsible for the overall balloon system. HS, MW, and AE contributed to the data analysis. RN performed the LES and analyzed the results. HG provided the remote sensing data and advice on the data. UE drafted the paper with contributions from all co-authors.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e5186">The authors declare that they have no conflict of interest.</p>
  </notes><notes notes-type="sistatement"><title>Special issue statement</title>

      <p id="d1e5192">This article is part of the special issue “Arctic mixed-phase clouds as studied during the ACLOUD/PASCAL campaigns in the framework of (AC)<inline-formula><mml:math id="M357" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> (ACP/AMT/ESSD inter-journal SI)”. It is not associated with a conference.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e5208">We gratefully acknowledge the funding by the Deutsche Forschungsgemeinschaft
(DFG, German Research Foundation) – project number 268020496 – TRR 172,
within the Transregional Collaborative Research Center “ArctiC Amplification: Climate Relevant Atmospheric and SurfaCe Processes, and Feedback Mechanisms (AC)<inline-formula><mml:math id="M358" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula>” in sub-project A02. We greatly appreciate the participation in RV <italic>Polarstern</italic> cruise PS 106.1 (expedition grant number AWI-PS106-00). We thank ECMWF for providing access to the large-scale model analyses and forecast fields used to force the LES. We gratefully acknowledge the Regional Computing Centre of the University of Cologne (RRZK) for granting us access to the CHEOPS cluster. The Gauss Centre for Supercomputing e.V. (<uri>http://www.gauss-centre.eu</uri>, last access: 26 April 2021) is acknowledged for providing computing time on the GCS Supercomputer JUWELS at the Jülich Supercomputing Centre (JSC) under project no. HKU28.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e5228">This research has been supported by the Deutsche
Forschungsgemeinschaft (DFG, German Research Foundation) (grant
no. Projektnummer 268020496 – TRR 172). <?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>
The publication of this article was funded by the <?xmltex \notforhtml{\newline}?> Open Access Fund of the Leibniz Association.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e5239">This paper was edited by Radovan Krejci and reviewed by two anonymous referees.</p>
  </notes><ref-list>
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    <!--<article-title-html>Case study of a humidity layer above Arctic stratocumulus  and potential turbulent coupling with the cloud top</article-title-html>
<abstract-html><p>Specific humidity inversions (SHIs) above low-level cloud
layers have been frequently observed in the Arctic.  The formation of these
SHIs is usually associated with large-scale advection of humid air
masses. However, the potential coupling of SHIs with cloud layers by turbulent
processes is not fully understood.  In this study, we analyze a 3&thinsp;d
period of a persistent layer of increased specific humidity above a
stratocumulus cloud observed during an Arctic field campaign in June 2017. The
tethered balloon system BELUGA (Balloon-bornE moduLar Utility for profilinG
the lower Atmosphere) recorded vertical profile data of meteorological,
turbulence, and radiation parameters in the atmospheric boundary layer. An
in-depth discussion of the problems associated with humidity measurements in
cloudy environments leads to the conclusion that the observed SHIs do not
result from measurement artifacts.  We analyze two different scenarios for the
SHI in relation to the cloud top capped by a temperature inversion: (i) the
SHI coincides with the cloud top, and (ii) the SHI is vertically separated
from the lowered cloud top. In the first case, the SHI and the cloud layer are
coupled by turbulence that extends over the cloud top and connects the two
layers by turbulent mixing. Several profiles reveal downward virtual sensible
and latent heat fluxes at the cloud top, indicating entrainment of humid air
supplied by the SHI into the cloud layer. For the second case, a downward
moisture transport at the base of the SHI and an upward moisture flux at the cloud
top is observed. Therefore, the area between the cloud top and SHI is supplied
with moisture from both sides.  Finally, large-eddy simulations (LESs)
complement the observations by modeling a case of the first scenario. The
simulations reproduce the observed downward turbulent fluxes of heat and
moisture at the cloud top. The LES realizations suggest that in the presence
of a SHI, the cloud layer remains thicker and the temperature inversion height
is elevated.</p></abstract-html>
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