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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-20-625-2020</article-id><title-group><article-title>A very high-resolution assessment and modelling of <?xmltex \hack{\break}?>urban air quality</article-title><alt-title>A very high-resolution assessment</alt-title>
      </title-group><?xmltex \runningtitle{A very high-resolution assessment}?><?xmltex \runningauthor{T.~Wolf et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes">
          <name><surname>Wolf</surname><given-names>Tobias</given-names></name>
          <email>tobias_wolf1@gmx.de</email>
        <ext-link>https://orcid.org/0000-0001-6004-2374</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Pettersson</surname><given-names>Lasse H.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6005-7514</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Esau</surname><given-names>Igor</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-4122-6340</ext-link></contrib>
        <aff id="aff1"><institution>Nansen Environmental and Remote Sensing Center, Thormøhlens gate 47, 5006, Bergen, Norway</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Tobias Wolf (tobias_wolf1@gmx.de)</corresp></author-notes><pub-date><day>20</day><month>January</month><year>2020</year></pub-date>
      
      <volume>20</volume>
      <issue>2</issue>
      <fpage>625</fpage><lpage>647</lpage>
      <history>
        <date date-type="received"><day>27</day><month>March</month><year>2019</year></date>
           <date date-type="rev-request"><day>8</day><month>August</month><year>2019</year></date>
           <date date-type="rev-recd"><day>5</day><month>November</month><year>2019</year></date>
           <date date-type="accepted"><day>16</day><month>November</month><year>2019</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2020 Tobias Wolf et al.</copyright-statement>
        <copyright-year>2020</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020.html">This article is available from https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020.pdf</self-uri>
      <abstract><title>Abstract</title>
    <p id="d1e97">Urban air quality is one of the most prominent
environmental concerns for modern city residents and authorities. Accurate
monitoring of air quality is difficult due to intrinsic urban landscape
heterogeneity and superposition of multiple polluting sources. Existing
approaches often do not provide the necessary spatial details and peak
concentrations of pollutants, especially at larger distances from monitoring
stations. A more advanced integrated approach is needed. This study presents
a very high-resolution air quality assessment with the Parallelized Large-Eddy Simulation Model (PALM), capitalising on local measurements. This fully three-dimensional
primitive-equation hydrodynamical model resolves both structural details of
the complex urban surface and turbulent eddies larger than 10 m in size. We
ran a set of 27 meteorological weather scenarios in order to assess the
dispersion of pollutants in Bergen, a middle-sized Norwegian city embedded
in a coastal valley. This set of scenarios represents typically observed
weather conditions with high air pollution from nitrogen dioxide (<inline-formula><mml:math id="M1" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>)
and particulate matter (<inline-formula><mml:math id="M2" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>). The modelling methodology helped to
identify pathways and patterns of air pollution caused by the three main
local air pollution sources in the city. These are road vehicle traffic,
domestic house heating with wood-burning fireplaces and ships docked in the
harbour area next to the city centre. The study produced vulnerability maps,
highlighting the most impacted districts for each weather and emission
scenario. Overall, the largest contribution to air pollution over inhabited
areas in Bergen was caused by road traffic emissions for <inline-formula><mml:math id="M3" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
wood-burning fireplaces for <inline-formula><mml:math id="M4" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> pollution. The effect of emission
from ships in the port was mostly restricted to the areas close to the
harbour and moderate in comparison. However, the results have contributed to
implementation of measures to reduce emissions from ships in Bergen harbour,
including provision of shore power.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e153">Patterns of atmospheric pollution in the urban environment are rather
variable and spatially heterogeneous. Air quality may regularly deteriorate
to harmful levels in the vicinity of near-surface emission sources, such as
major traffic junctions and low-raised chimneys. Widely accepted statistical
models provide reasonably accurate assessment of pollutant concentrations
near the strong emission sources assuming availability of representative
meteorological input (e.g. Isakov et al.,
2017). At larger distances from the sources, or in more complex flow
settings, however, their accuracy drastically deteriorates. It has been
understood that pockets of polluted air could be trapped in a weakly
turbulent (weakly diffusive) flow and transported over longer distances.
This turbulent transport by larger eddies cannot be successfully described
by phenomenological statistical methods. Its adequate representation
requires hydrodynamic modelling where at least the largest carrying eddies
would be explicitly resolved. Moreover, intricate configurations of
buildings, streets and other urban surface objects create preferable
pathways for wind and turbulent diffusion. Along those pathways, the
pollutants disperse over much larger distances, thus raising air quality
concerns in distant districts that otherwise would be considered as
unaffected.</p>
      <p id="d1e156">The highest concentrations of atmospheric pollutants are often found under
persistent calm and cold weather conditions. This is also the case for the
coastal city of Bergen, Norway, that is subject to this study. Such
conditions are<?pagebreak page626?> characterised by a stably stratified lower atmosphere and
strongly suppressed turbulent diffusion (Davy and
Esau, 2016; Zilitinkevich and Esau, 2005). In the most extreme cases, known
as temperature inversions, the air temperature is increasing with height
(Wolf et al., 2014), trapping the turbulence,
and therefore pollutants, in a shallow layer near the surface. Even in such
conditions, there could be non-negligible turbulence as well as horizontal
transport of pollutants driven by local circulations
(Wolf-Grosse et al., 2017a). If the calm
weather conditions persist sufficiently long, concentrations of air
pollutants may reach levels in excess of regulatory thresholds for air
pollution (Bergen Kommune, 2019; European Commission, 2019),
while their spatial pattern would be highly heterogeneous.</p>
      <p id="d1e159">Local air quality is frequently assessed with simplified statistical models,
such as a family of Gaussian models, e.g. CALINE, or with more sophisticated
models, which include parameterised turbulent diffusion, e.g. AIRMOD
(Daly and Zannetti, 2007). A set of models recommended by the
US and European environmental protection agencies could be found
correspondingly on EPA (2019) and on EEA (2019). Statistical models are poor in predicting horizontal pollution
transport in turbulent atmospheric boundary layers (ABLs), as they do not
account for turbulent eddies, meandering flows and flow–surface structure
interactions (Sun et al., 2016). In recent years,
computational fluid dynamics models have been tried in assessments of the
urban and road-level dispersion. As an example, one may mention simulations
by Steffens et al. (2014) of the wind tunnel experiment
conducted by Heist et al. (2009). This study
investigated concentration gradients of a tracer gas under 12 different
roadway configurations. It concluded that near-road structures impact
dispersion of pollutants near roadways, and therefore atmospheric modelling
is needed to design barriers to control the impact of vehicular emissions.</p>
      <p id="d1e162">Recent advances in computational fluid dynamics and growing performance of
parallel computers open an opportunity to further extend the model-based
urban air quality assessment. Turbulence-resolving, or at least
turbulence-permitting, large-eddy simulation models have been already used
in several cities to investigate turbulent flows and atmospheric pollution
(e.g. Castillo et al., 2009; Gronemeier et al., 2017; Keck et al., 2014; Letzel et
al., 2008; Park et al., 2015; Resler et al., 2017).
Cécé et al. (2016)
used a turbulence-permitting model to study air quality (nitrogen oxides,
<inline-formula><mml:math id="M5" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) in a coastal mountain area of a tropical island where local
circulations are well developed and influential. A consistent description of
the circulation and pollution effects in a coastal mountain valley can be
found in Fernando et al. (2010). These
and other studies convinced us that the large-eddy simulation models could
accurately resolve the dispersion of pollutants even in a complex
environment without the current need for potentially unsuitable statistical
fitting.</p>
      <p id="d1e177">This study makes the next step on the bridge between idealised feasibility
studies and applied air quality assessments. It utilises the Parallelized Large-Eddy Simulation (LES) Model (PALM) (Maronga
et al., 2015) to investigate the dispersion of pollutants in a weakly
turbulent ABL under archetypical, but frequently observed, weather
conditions, which lead to dangerous deterioration of the air quality, in our
case in Bergen. Bergen is embedded in a relatively deep and narrow valley
ending in a large ocean fjord. The minimum distance between the mountains is
approximately 1 km when measured across the valley floor; it is
approximately 4 km when measured between the mountain peaks, being up to 650 m high. The polluted air during cold winter days tends to accumulate
and stagnate in the bottom of the valley, whereas local circulations
redistribute the pollution across the central city districts. Thus, the
local circulations are likely to determine air quality for the districts'
populations. The effect of the local circulations could be accounted for in
the PALM simulations (Wolf-Grosse et al.,
2017a) but not in statistical models relying on coarse spatial resolution
(<inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> km) mesoscale models.</p>
      <p id="d1e190">In this study, the dispersion of nitrogen dioxide (<inline-formula><mml:math id="M7" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) and
small-fraction particulate matter (<inline-formula><mml:math id="M8" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) is modelled over densely
populated central Bergen under weak winds and typical scenarios of measured
severe air pollution. As such, this study presents a necessary element of
an integrated urban pollution assessment and warning system envisaged in
Baklanov et al. (2007). The chosen
approach could be useful for the design of high-resolution local climate
information services assessing informed decision-making at the municipal
level (e.g. Bauer et
al., 2015; Letzel et al., 2012; Ronda et al., 2017). Results from this study
have already been adopted by the Bergen Port Authority (BOH) to assist their
routine assessment of the impact of exhaust from ships in the harbour.</p>
      <p id="d1e215">The paper has the following structure. The next section describes the
local geographical and data context for the city of Bergen. The third
section presents the modelling approach with PALM and the analysed
meteorological scenarios. The fourth section presents the analysis and
modelling results of this study. The fifth section provides a broader
discussion with generalisations of the methodology, data usage and policy
implications. The final section briefly summarises the conclusions.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Data</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>Site description</title>
      <p id="d1e233">The western coast of Norway is known for its picturesque mountain landscapes
with sea inlets (fjords) penetrating deep into coastal valleys. Similar, if
not as dramatic, settings with coastal valleys opening into sea inlets and
bays are frequently accommodating harbour cities in other parts of the globe
as<?pagebreak page627?> well. Therefore, as we believe, the methodology and experience described
in this study might be of interest to the research and urban management
communities worldwide.</p>
      <p id="d1e236">Bergen is the second largest city in Norway. This coastal city is located at
60.4<inline-formula><mml:math id="M9" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N and 5.3<inline-formula><mml:math id="M10" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E. The mountains around the city have
peak elevations between 284 and 643 m a.s.l. They protect the
valley from storms, significantly reducing the surface layer wind speed
(Jonassen et al., 2013). The northern
location with its weak solar irradiation during wintertime and cold air
pooling in lower parts of the relief causes frequently observed but highly
local temperature inversions during periods with persistently calm and clear
weather. These inversions can last through several days. The resulting weak
turbulent mixing of the lower valley atmosphere fosters the accumulation of
locally emitted pollutants despite only moderate emissions. A climatology of
temperature inversions and air pollution events in Bergen was previously
reported in Wolf et al. (2014).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><?xmltex \currentcnt{1}?><label>Figure 1</label><caption><p id="d1e259"><bold>(a)</bold> Topographic map of the Bergen area. The black square
indicates the final model domain used for the PALM simulations; the gray
square indicates the focus area for the analysis of the PALM simulations.
<bold>(b)</bold> Emission map for Bergen city centre used in the PALM simulations.
Colour shading indicates the number of parcels of land with registered
active fireplaces (for domestic heating) per <inline-formula><mml:math id="M11" display="inline"><mml:mrow><mml:mn mathvariant="normal">10</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> m<inline-formula><mml:math id="M12" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> grid square.
Black/gray lines indicate the location of main/side roads. The main harbour
areas, Jekteviken (southwest, 2) and Skolten (northeast, 1), are indicated
with two red squares. The numbered arrows point at the location of the
automatic weather stations at (1) Skolten, (2) Jekteviken, (4) Florida and
(6) Ulriken, and the air pollution stations at (3) Rådhuset and (5) Danmarksplass.</p></caption>
          <?xmltex \igopts{width=369.885827pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f01.png"/>

        </fig>

      <p id="d1e295">Bergen has more than 275 000 inhabitants. More than 75 000 of them reside in
the central districts, located in the elongated central Bergen valley, which
is the focus of this study. The valley opens toward a sea inlet (Byfjorden)
in the northwest. It widens towards a large brackish water lake and more
residential areas in the southwest. Figure 1 shows the relief of the studied
area, the model simulation domain, as well as the location of the major air
pollution sources in the city.</p>
      <p id="d1e298">A reader may like to know that the air quality in Bergen has been monitored
continuously since 2002 with an increasing number of measurement stations.
In addition, a routine air quality forecast exists within the “Bedre
Byluft” national project for monitoring and prediction of air pollution in
Norwegian cities. The results from the measurements are available under
NILU (2019). The predictions can be found under
Miljødirektoratet (2019). Both measurements and predictions
are regularly summarised (Bergen Kommune, 2018; Tarrasón
et al., 2017). The forecast system has recently been changed. It was based
on the AirQuis/EPISODE air quality model using meteorological input from a 1 km mesoscale numerical weather prediction (NWP) model specifically run for
this application. The new forecast system is based on the “Nasjonalt
Bergningsverktøy” (NBV) tool. The NBV uses uEMEP as a dispersion model
and the control run of the standard METCoOp ensemble prediction system
(MEPS) for Norway with a 2.5 km spatial resolution to calculate physics in
the dynamical spectral model as meteorological input (Denby and
Süld, 2015). With this, the previous AirQuis/EPISODE model at least to
some degree included the valley topography into the dispersion calculations
via a higher resolution of the meteorological input and a meteorological
pre-processor that created a divergence-free wind field in the valley
(Baklanov et al., 2007; The World Bank,
2009).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e304">Datasets used for this study.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="156pt"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="118pt"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="115pt"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Dataset</oasis:entry>
         <oasis:entry colname="col2">Source</oasis:entry>
         <oasis:entry colname="col3">Format, data type (period)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3" align="left">Topographic data </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Laser measurements from over the square area of size <inline-formula><mml:math id="M13" display="inline"><mml:mrow><mml:mn mathvariant="normal">10</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> km centred over Bergen city hall</oasis:entry>
         <oasis:entry colname="col2">Bergen municipality, already <?xmltex \hack{\hfill\break}?>combined and filtered in <?xmltex \hack{\hfill\break}?>previous project</oasis:entry>
         <oasis:entry colname="col3">LAS point cloud</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Topographic height for Bergen <?xmltex \hack{\hfill\break}?>municipality</oasis:entry>
         <oasis:entry colname="col2">Bergen municipality</oasis:entry>
         <oasis:entry colname="col3">DSM, GeoTiff, 10 m horizontal <?xmltex \hack{\hfill\break}?>resolution</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Topographic height for surrounding <?xmltex \hack{\hfill\break}?>municipalities</oasis:entry>
         <oasis:entry colname="col2">Norwegian mapping authority</oasis:entry>
         <oasis:entry colname="col3">DSM, GeoTiff, 10 m horizontal <?xmltex \hack{\hfill\break}?>resolution</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Water surfaces</oasis:entry>
         <oasis:entry colname="col2">Bergen municipality</oasis:entry>
         <oasis:entry colname="col3">Shape file, polygon</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3" align="left">Local measurements and large-scale circulation </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Microwave radiometer measurements <?xmltex \hack{\hfill\break}?>(inversions)</oasis:entry>
         <oasis:entry colname="col2">Own data, NERSC</oasis:entry>
         <oasis:entry colname="col3">ASCII, time series (2011–2016)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Geophysical Institute weather stations  <?xmltex \hack{\hfill\break}?></oasis:entry>
         <oasis:entry colname="col2">University of Bergen (UiB)</oasis:entry>
         <oasis:entry colname="col3">ASCII, time series (2011–2016)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">ERA-Interim (large-scale meteorology) <?xmltex \hack{\hfill\break}?></oasis:entry>
         <oasis:entry colname="col2">European Centre for Medium- <?xmltex \hack{\hfill\break}?>Range Weather Forecasts <?xmltex \hack{\hfill\break}?>(ECMWF)</oasis:entry>
         <oasis:entry colname="col3">NetCDF, map with different <?xmltex \hack{\hfill\break}?>resolutions and timescales</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Weather stations at Skolten and <?xmltex \hack{\hfill\break}?>Jekteviken</oasis:entry>
         <oasis:entry colname="col2">BOH</oasis:entry>
         <oasis:entry colname="col3">ASCII, time series (2014–2016)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Air pollution measurements</oasis:entry>
         <oasis:entry colname="col2">Norwegian Institute for Air <?xmltex \hack{\hfill\break}?>Research (NILU, 2019)</oasis:entry>
         <oasis:entry colname="col3">ASCII, time series (2003–2016)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3" align="left">Emission data </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Main streets (centre line and traffic) <?xmltex \hack{\hfill\break}?></oasis:entry>
         <oasis:entry colname="col2">Bergen municipality</oasis:entry>
         <oasis:entry colname="col3">Shape file, traffic information</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Side streets (centre line and traffic) <?xmltex \hack{\hfill\break}?></oasis:entry>
         <oasis:entry colname="col2">National road authority</oasis:entry>
         <oasis:entry colname="col3">Shape file, traffic information</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Traffic at Danmarksplass</oasis:entry>
         <oasis:entry colname="col2">National road authority</oasis:entry>
         <oasis:entry colname="col3">Excel list with traffic counts for <?xmltex \hack{\hfill\break}?>different time periods</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Properties with fireplaces <?xmltex \hack{\hfill\break}?></oasis:entry>
         <oasis:entry colname="col2">Bergen fire department</oasis:entry>
         <oasis:entry colname="col3">Shape file, point data, list</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Harbour log</oasis:entry>
         <oasis:entry colname="col2">BOH</oasis:entry>
         <oasis:entry colname="col3">Excel list with ship type, name, <?xmltex \hack{\hfill\break}?>arrival and departure, docking <?xmltex \hack{\hfill\break}?>time (2015–2016)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Datasets</title>
      <p id="d1e579">This study demonstrates the high-resolution modelling methodology using the
comprehensive local data context. The model simulations require
high-resolution topographic data, emission inventories for the different
sources of pollution and vertical profiles of the large-scale (geostrophic)
wind and temperature. All data sources are summarised in Table 1. Their
detailed description is presented below.</p>
      <p id="d1e582">The added value of the high-resolution model simulations is created by their
ability to resolve the local relief features, which control the air flow and
the turbulent dispersion. We run the PALM model with 10 m spatial
resolution. To obtain the adequate relief, we used a topographic laser-based
dataset, as described in Wolf-Grosse
et al. (2017a). These topographic data were processed to ensure consistency
and eliminate artefacts in the airborne laser data. The processed data
constitute a digital elevation model (DEM) for the Bergen municipality.
However, this DEM does not cover the entire simulation domain, as we run the
simulations over a significantly larger area to resolve multiple local flows
steered by the topographic relief. We extended the DEM, adopting digital
surface model (DSM) data. The DSM does not include buildings (the DEM does),
but outside the urbanised central districts, and sufficiently far away from
the focus area, we assume that it is sufficient to resolve the major
features of the relief and coastal line.</p>
      <p id="d1e585">We selected the typical air pollution scenarios for this study based on
joint air quality and meteorological data analysis. Routine air pollution
measurements since 2003 have been available from two of the local air pollution
stations, namely the Danmarksplass (DP) and Rådhuset (RH) stations
in the central Bergen districts (see Fig. 1). The DP station represents an
area affected by heavy road traffic, whereas the RH station serves as an
urban background reference. We jointly analysed the air quality and
meteorological records for several pollution episodes, when high
concentrations of <inline-formula><mml:math id="M14" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M15" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> were observed. As local
meteorological data, we used measurements from the automatic weather stations
located in the Florida neighbourhood (on top of the Geophysical Institute),
the Ulriken summit and in the Jekteviken and Skolten harbour areas. For the
large-scale weather conditions, we used data from the retrospective
meteorological ERA-Interim analysis
(Dee et
al., 2011) and from the local boundary layer temperature profiles observed
by a microwave radiometer MTP-5HE, which the Nansen Center has been operating on
top of the Geophysical Institute since 2011.</p>
      <p id="d1e610">The central Bergen districts are affected by emissions from three major
polluting sources: vehicles on the road network; ships in the Bergen
harbour; and wood-burning fireplaces in private residences. There are no
major industrial sources. The road network is contributing to both
emissions of <inline-formula><mml:math id="M16" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M17" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. To specify these emissions, we used
the gridded traffic density per road segment. It was available from
registers<?pagebreak page628?> at the national road authority for the main streets and from a
traffic model run by the national road authority for the side streets.</p>
      <p id="d1e636">Emissions from ships at berth in the harbour are contributing to both
emissions of <inline-formula><mml:math id="M18" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M19" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The Bergen harbour is located in the
historic city centre, and therefore ships docked at berth in the harbour
can directly contribute to the local air pollution. Here, we considered only
emissions from supply vessels for the offshore oil industry, during their
periods at berth in Bergen harbour. Due to their often-large number and
their large sizes, these ships are major contributors to the emissions from
the harbour compared to other relevant ship types like the frequent, but
small, short-range public transportation ferries or the less frequent, but
larger, freight or passenger ships. In summertime, emissions from cruise
ships can exceed the emissions from the offshore supply vessels in the
harbour. In recent years, the cruise traffic seemed to expand also into other
seasons. The impact of these supply vessels, that are docked right in the
city centre of Bergen for extensive periods of time, on local air pollution
is still highly disputed by the local population and therefore a matter of
public interest and concern. The BOH provided us with data to specify the
ships' location in the harbour between January 2015 and March 2016. For the
emission rates per ship, we used the emission factors from the certification
documentation of two representative ships.</p>
      <p id="d1e661">Domestic heating with wood-burning fireplaces only contributes to emissions
of <inline-formula><mml:math id="M20" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. We assessed these emissions through accounting for estates
with registered active fireplaces. These data were provided by the Bergen
fire department. For the emission rates per fireplace, we used typical
emission factors for the existing mixture of new, clean burning wood ovens
and older ones with higher emissions. All three emission sources are
graphically summarised in Fig. 1.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Model</title>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>The PALM model</title>
      <p id="d1e691">The high-resolution air quality assessment requires a proper atmospheric
model which can resolve the most energetic turbulence eddies in fully
three-dimensional simulations. This ability to resolve the turbulent motions
and interactions across a multitude of scales distinguishes the
turbulence-resolving, or at least turbulence-permitting, LES models from
more traditional meteorological and cloud-resolving models. The traditional
meteorological models have the whole turbulence spectrum collapsed in their
closure schemes, even if those models are running at 1 km or sometimes
higher resolutions. The turbulence closure schemes are designed for weakly
stratified, horizontally homogenous ABLs over a flat terrain. Their
application to a strongly stable stratified ABL commonly results in
excessive vertical mixing and hence in erroneous pollutant transport. The
results of the GABLS intercomparison exercises are instructive to one
working with this issue
(Cuxart
et al., 2006; Holtslag et al., 2013; Vignon et al., 2017).</p>
      <p id="d1e694">We used the PALM (version 4.0, revision 1550) code in this study. The PALM
code is developed by the PALM group<?pagebreak page629?> at the Leibniz University of Hannover,
Germany (Maronga et al., 2015). This
model solves the primitive hydro- and thermodynamic equations for
incompressible Boussinesq fluids. We ran the model for dry atmospheric
conditions. This choice simplifies the model setup and is motivated by the
fact that the worst air quality was always observed during fair-weather
conditions, under prolonged occurrence of temperature inversions in the
Bergen valley. Thus, the model was initiated only with temperature and wind
profiles. The initial wind profiles also serve as geostrophic wind profiles
or forcing, which drives the PALM simulations via the geostrophic wind term.</p>
      <p id="d1e697">We ran PALM over a geographical domain centred on Bergen municipality. The
domain spans 12.79 km in the zonal (east–west) and 17.27 km in the
meridional (north–south) directions (Fig. 1a). The surface
geometry was set by the DEM-DSM data. The lateral boundary conditions in the
model runs were periodic. The domain includes a 1000 m wide buffer zone at
the outer boundaries of the model domain. This buffer was necessary to
linearly interpolate the<?pagebreak page630?> surface geometry, making it periodic in both
lateral directions. We set the model grid resolution to 10 m. The grid is
vertically stretched by 1 % for each subsequent grid level above 750 m. In
total, there were 128 vertical grid levels reaching 1450 m a.s.l.,
which is more than 2 times the height of the highest mountain peak
within the model domain. The surface boundary conditions were different for
the land and water surfaces. We used the Neumann (constant flux) condition
for the land grid cells, as they have low heat capacity and quickly adjust
the skin temperature. For the water grid cells, we used the Dirichlet
(constant temperature) condition, as water has a large heat capacity and
retains an almost constant skin temperature over the simulation time window.</p>
      <p id="d1e700">Turbulent mixing is an irreversible process. It changes the temperature
stratification and the wind profiles in the model also during the model
spin-up. We counteract this difficulty by introducing a nudging routine. It
relaxes the horizontally averaged temperature profile towards the initial
temperature profile. This nudging is enabled starting from the second grid
level above the local surface. The relaxation timescale is <inline-formula><mml:math id="M21" display="inline"><mml:mrow><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">43</mml:mn></mml:mrow></mml:math></inline-formula> 200 s
at elevations <inline-formula><mml:math id="M22" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">400</mml:mn></mml:mrow></mml:math></inline-formula> m a.s.l. This timescale linearly decreases to <inline-formula><mml:math id="M23" display="inline"><mml:mrow><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1800</mml:mn></mml:mrow></mml:math></inline-formula> s at <inline-formula><mml:math id="M24" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">600</mml:mn></mml:mrow></mml:math></inline-formula> m.
Nudging is therefore very weak in the lower parts of the atmosphere,
allowing the temperature profile inside the Bergen valley to be determined
dynamically through the boundary conditions. In the free atmosphere above
the mountains, we applied much stronger nudging, retaining the initial
temperature profile. A simpler setup of the PALM model has been tested
successfully in its application to the stably stratified ABL inside the
Bergen valley (Wolf-Grosse et al.,
2017a).</p>
      <p id="d1e752">In order to simulate the dispersion of pollutants from the relevant sources,
we used constant emission rates per grid cell in the model. The emission
rates were set separately for each of the three emission sources. Hence,
<inline-formula><mml:math id="M25" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M26" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> tracers from the harbour, chimneys and roads are
simulated independently. In the applied model version of PALM, all
pollutants are treated as passive tracers. We argue that this is a
reasonable choice for the wintertime air quality assessment in a local
high-latitude domain. The background near-surface ozone (<inline-formula><mml:math id="M27" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) that could
serve as a source of additional <inline-formula><mml:math id="M28" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> from existing NO is greatly
depleted during the winter months. Sunlight that could lead to a photolytic
conversion of <inline-formula><mml:math id="M29" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> to NO and <inline-formula><mml:math id="M30" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is largely absent. The nucleation
of <inline-formula><mml:math id="M31" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> into nitrate particles is slow compared to the transport and
mixing processes. The particle growth beyond the <inline-formula><mml:math id="M32" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> limits is also a
slow process, whereas the particle wet scavenging is minimal under the clear-sky conditions considered in this study. Gravitational settling of particles
for the size range below 2.5 <inline-formula><mml:math id="M33" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m is slow.</p><?xmltex \hack{\newpage}?>
</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Scenarios</title>
      <p id="d1e861">The high-resolution environmental assessment and modelling is still a costly
and computationally demanding exercise. Therefore, we selected the most
relevant and impactful scenarios of high air pollution using joint
statistical analysis of the long-term air quality and meteorological
observations
(Wolf-Grosse
et al., 2017b; Wolf et al., 2014; Wolf and Esau, 2014). Here, we will not
repeat the details of that analysis. Nevertheless, a brief summary might be
useful for new readers. Studies of the extreme deterioration of the air
quality may frequently benefit from the fact that the high concentrations of
pollutants are reached after several hours (or even days) of persistently
calm clear-sky weather. Such weather conditions are limited to a few
specific sets of local values of the meteorological parameters. The high
concentrations are mostly observed under southeasterly winds over the
Bergen valley. Due to a complex interaction between the locally forced
circulation and the large-scale winds, the wind direction in the city is
mostly southeasterly, too. That means the air moves from the city towards
the Bergen fjord and harbour. The local wind therefore transports air
pollution from the locations with the most intensive emission and towards
the fjord. The efficiency of this transport is dependent on a convergence
zone that can, dependent on the interplay between the local and larger-scale
drivers, be located either over the fjord or over the city areas in
proximity to the harbour. Different inhabited areas might therefore be
affected by emissions from some or all local emission sources.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><?xmltex \currentcnt{2}?><label>Figure 2</label><caption><p id="d1e866">The mean vertical temperature profile used for nudging in the PALM
model domain.</p></caption>
          <?xmltex \igopts{width=113.811024pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f02.png"/>

        </fig>

<sec id="Ch1.S3.SS2.SSS1">
  <label>3.2.1</label><title>Meteorological conditions</title>
      <p id="d1e882">As the baseline scenario for this study, we used the dominant weather
conditions, which were observed during the cases with measured hourly mean
<inline-formula><mml:math id="M34" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations above the regulatory threshold of 200 <inline-formula><mml:math id="M35" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M36" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> at the DP site (Bergen Kommune, 2019). The initial and
nudging temperature profile is the average of the temperature profiles
measured over central Bergen during these high-air-pollution conditions<?pagebreak page631?> as
shown in Fig. 2. The geostrophic wind profile is the mean of the wind
profile taken from the ERA-Interim reanalysis over all high-air-pollution
conditions. Due to the low resolution of ERA-Interim and the specific
topography at the Norwegian west coast, the lowest grid level from
ERA-Interim is located at around <inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">410</mml:mn></mml:mrow></mml:math></inline-formula> m, dependent on large-scale air
pressure. Therefore, the local scale flows are missing. To define a wind
profile adapted to the realistic topography, we modified the wind speed
profile to linearly increase from zero below <inline-formula><mml:math id="M38" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">300</mml:mn></mml:mrow></mml:math></inline-formula> m to the actual
ERA-Interim value at <inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">450</mml:mn></mml:mrow></mml:math></inline-formula> m. Additional sensitivity experiments
included the wind speed being 0.5 and 1.5 times the baseline wind speed.
The geostrophic wind direction in the baseline scenario was set to wd <inline-formula><mml:math id="M40" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 110<inline-formula><mml:math id="M41" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>.
Sensitivity experiments used the wind directions of wd <inline-formula><mml:math id="M42" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 90<inline-formula><mml:math id="M43" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and wd <inline-formula><mml:math id="M44" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 130<inline-formula><mml:math id="M45" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, which cover the interval of the
relevant wind directions found in the ERA-Interim data. The wind profiles
for the different scenarios are shown in Fig. 3.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3"><?xmltex \currentcnt{3}?><label>Figure 3</label><caption><p id="d1e1004">Mean wind speed <bold>(a)</bold> and wind direction <bold>(b)</bold> profiles in the three considered scenarios and sensitivity experiments. In
addition, the original ERA-Interim profiles (ERAI) are given as dashed
lines.</p></caption>
            <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f03.png"/>

          </fig>

      <p id="d1e1019">During each single PALM simulation, we kept the model forcing constant,
meaning that we conducted simulations with static boundary conditions. This
is a necessary simplification in order to limit the computational efforts.
Each scenario was initialised with a precursor simulation running over 12 h
in order to stabilise the model circulation. At the end of the
precursor run, the mean meteorological parameters were not drifting any
longer. After the initialisation, the simulations were continued for another
6 h with emissions applied. For multiple simulations of the same
meteorological condition, we used a restart option.</p>
      <p id="d1e1023">We do not have consistent surface heat budget observations in Bergen. To
circumvent this problem, we inferred an approximate budget. The reviewed
literature (Brümmer and Schultze, 2015; Nordbo et
al., 2012) suggested as a reasonable value for the scenario a constant
kinematic heat flux of <inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:msub><mml:mi>H</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.02</mml:mn></mml:mrow></mml:math></inline-formula> K m s<inline-formula><mml:math id="M47" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M48" display="inline"><mml:mrow><mml:mo>≈</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">20</mml:mn></mml:mrow></mml:math></inline-formula> W m<inline-formula><mml:math id="M49" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) over the land cells. Over the water cells (lakes and fjord), we
applied a constant surface temperature to reflect the very high heat
capacity of the water mixed layer. We run three sensitivity experiments with
the water surface temperature set to 0, 2.5 and
5 <inline-formula><mml:math id="M50" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C. The baseline scenario is characterised by temperature
inversions in the shallow ABL over Bergen.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T2"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e1091">Parameters for the different meteorological scenarios<inline-formula><mml:math id="M51" display="inline"><mml:msup><mml:mi/><mml:mo>∗</mml:mo></mml:msup></mml:math></inline-formula>.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.95}[.95]?><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Parameter</oasis:entry>
         <oasis:entry colname="col2">Name</oasis:entry>
         <oasis:entry colname="col3">Description</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">Wind speed</oasis:entry>
         <oasis:entry colname="col2">ws01</oasis:entry>
         <oasis:entry colname="col3">Vertical profile baseline scenario</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">ws02</oasis:entry>
         <oasis:entry colname="col3">0.5 times baseline scenario</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">ws03</oasis:entry>
         <oasis:entry colname="col3">1.5 times baseline scenario</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Wind direction</oasis:entry>
         <oasis:entry colname="col2">wd01</oasis:entry>
         <oasis:entry colname="col3">Baseline scenario, 110<inline-formula><mml:math id="M53" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">wd02</oasis:entry>
         <oasis:entry colname="col3">90<inline-formula><mml:math id="M54" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">wd03</oasis:entry>
         <oasis:entry colname="col3">130<inline-formula><mml:math id="M55" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Surface temperature</oasis:entry>
         <oasis:entry colname="col2">ft01</oasis:entry>
         <oasis:entry colname="col3">Baseline scenario, 2.5 <inline-formula><mml:math id="M56" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Bergen fjord</oasis:entry>
         <oasis:entry colname="col2">ft02</oasis:entry>
         <oasis:entry colname="col3">5 <inline-formula><mml:math id="M57" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">ft03</oasis:entry>
         <oasis:entry colname="col3">0 <inline-formula><mml:math id="M58" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e1103"><inline-formula><mml:math id="M52" display="inline"><mml:msup><mml:mi/><mml:mo>∗</mml:mo></mml:msup></mml:math></inline-formula> As a brief syntax for the naming of the different model scenarios, we use the three meteorological parameters
(wind speed, wind direction and sea surface temperature in the fjord) separated by underscores, e.g. ws01_wd01_ft01 for the baseline scenario.</p></table-wrap-foot></table-wrap>

      <p id="d1e1298">All meteorological conditions for the different scenarios are summarised in
Table 2. As a brief syntax for the naming of the different model scenarios,
we use the three meteorological parameters (wind speed, wind direction and sea
surface temperature in the fjord) separated by underscores, e.g. ws01_wd01_ft01 for the baseline scenario. For
all possible 27 combinations of meteorological scenarios, we conducted the 12 h precursor runs, including dummy emissions from large streets (see below).
These were not used for the final in-detail dispersion assessments but
allowed for an initial assessment of the dispersion patterns in the valley
for each meteorological scenario. The strong topographic steering in the
valley restricts deviations in the simulated patterns produced by the
sensitivity runs. The precursor sensitivity simulations therefore showed
similar geographical concentration patterns but with varying accumulation
strengths. In order to reduce the computational load from repeating all
emission simulations for all 27 meteorological scenarios, we conducted
emission simulations only for the most notably different meteorological
scenarios. These were the six scenarios: ws01_wd01_ft01, ws02_wd01_ft01,
ws03_wd01_ft01, ws03_wd02_ft01, ws03_d02_t02 and
ws03_wd02_ft03.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS2">
  <label>3.2.2</label><title>Emissions</title>
      <?pagebreak page632?><p id="d1e1310">We obtained the road traffic emission rates from the annual mean daily
traffic data. For this, we converted the traffic counts in the grid cell <inline-formula><mml:math id="M59" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula>
of the PALM model to the emission rates, <inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, as
              <disp-formula id="Ch1.Ex1"><mml:math id="M61" display="block"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">r</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>N</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>l</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M62" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the annual mean daily number of vehicles (ADT) passing a
certain grid cell; <inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msub><mml:mi>l</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the length of the road links per grid cell;
<inline-formula><mml:math id="M64" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">r</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is a suitable emission factor for the existing park of vehicles and
their emission characteristics in Bergen. The calculation of the emission
factors for <inline-formula><mml:math id="M65" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M66" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> from road traffic is described in detail
in Appendix A.</p>
      <p id="d1e1421">We obtained the emission rates from wood-burning fireplaces (only
<inline-formula><mml:math id="M67" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>), <inline-formula><mml:math id="M68" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, in a grid cell <inline-formula><mml:math id="M69" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula> as
              <disp-formula id="Ch1.Ex2"><mml:math id="M70" display="block"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>n</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M71" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the number of real estate properties with at least one
registered wood-burning fireplace, per model grid cell <inline-formula><mml:math id="M72" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula>; <inline-formula><mml:math id="M73" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the
typical emission factor for the wood-burning fireplaces. The calculation of
this emission factor is described in detail in Appendix B.</p>
      <p id="d1e1510">Both emission rates (<inline-formula><mml:math id="M74" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M75" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are defined as the surface fluxes in
the model. It should be noted here that the a posteriori evaluation of the <inline-formula><mml:math id="M76" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in the simulations revealed that the provided emission
rates from wood-burning fireplaces are too high. Therefore, we keep the
concentration patterns but uniformly scale the calculated magnitudes by a
factor of 0.1 in order to achieve reasonable concentrations compared to the
available measurements. This inconsistency in the emission rates may be
because either the emission rates per oven were overestimated or the
fireplaces are much less used than suggested by the local fire department.
There is also a degree of uncertainty related to the actual effective
emission height. In the areas with the highest densities of chimneys, they
typically have their exhaust at the heights between the third and fourth
floor. The effect of the emission height in the complex settings on the
Bergen area should be assessed in more detail in future studies. However, at
least the relative distribution of the pollutants should be reasonably
represented, assuming that the usage of ovens is similar between different
neighbourhoods.</p>
      <p id="d1e1546">We obtained emission factors <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for the grid cell <inline-formula><mml:math id="M78" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula>, in which the
offshore supply vessels typically are docked as
              <disp-formula id="Ch1.Ex3"><mml:math id="M79" display="block"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>v</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where <inline-formula><mml:math id="M80" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the average emission factor per fuel spent for two
representative ships provided by a local ship owning company; and <inline-formula><mml:math id="M81" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is
the typical fuel usage for the ships while at berth. Both numbers are
factors describing the emissions from the ship's secondary engines that are
smaller than the main engines used for travel and provide the ships with
power while at berth. The calculation of this emission factor is described
in detail in Appendix C.</p>
      <p id="d1e1618">To compare to the most severe air pollution conditions in Bergen, all
emission factors are calculated for typical high-emission conditions,
meaning rush-hour traffic, active usage of ovens for heating and standard
ship emissions at berth for a busy day in the harbour in terms of the number
of ships at berth.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><?xmltex \currentcnt{4}?><label>Figure 4</label><caption><p id="d1e1623">The meteorological conditions averaged over the last 15 min of the
12 h precursor simulation for the baseline scenario ws01_wd01_ ft01. The conditions were sampled in two areas: <bold>(a)</bold> the
harbour area at the northwest end of the city centre where the profiles 1
and 2 were sampled; <bold>(b)</bold> the heavy traffic and densely populated area at the
southeast end of the city centre where the profiles 3, 4 and 5 were sampled.
The temperature profiles <bold>(c)</bold> and the wind speed <bold>(d)</bold> and direction <bold>(e)</bold> profiles were averaged over the sub-areas shown by the white rectangles.</p></caption>
            <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f04.png"/>

          </fig>

<?xmltex \hack{\newpage}?>
</sec>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Results</title>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Baseline scenario simulations</title>
      <p id="d1e1666">The scenario ws01_wd01_ft01 is the baseline
scenario for the air quality simulations (see Table 2). This scenario
describes the most typical meteorological conditions during episodes with
high air pollution in Bergen. The baseline scenario maintains a low-level
(surface) temperature inversion in the lowermost 100 m a.s.l.
almost everywhere over land in the Bergen simulation domain. The weak winds
and wind channelling by the valley relief could be noted over the lowermost
400 m. Figure 4 shows the relief and vertical temperature and wind profiles
in two selected areas of interest and five selected sub-areas for more detailed
analysis. Area (a) represents the harbour area in the city centre, while
area (b) represents an area with dense population and heavy traffic in the
southwest of the city centre. Area (a) is strongly affected by the
sea–land temperature contrast. The enhanced mixing over the water surface
dilutes the temperature inversion there. Area (b) includes the heavily
trafficked road junctions at DP and its direct surroundings (sub-area
4). It also includes the Bergen meteorological observatory with a large
amount of meteorological instrumentation collocated in sub-area 3.</p>
      <p id="d1e1669">The wind speed and directions in the baseline scenario clearly indicate a
low-level air transport in the Bergen valley towards its opening into
Byfjorden – the sea inlet where the harbour is located. This channelled
local circulation is likely enhanced by the land–sea temperature contrast as
it has been described already through statistical analysis in
Wolf et al. (2014) and dynamical analysis
in Wolf-Grosse et al. (2017a). The
latter study also addressed the distinct rotation in the wind direction from
down-valley near the ground to up-valley at around <inline-formula><mml:math id="M82" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">300</mml:mn></mml:mrow></mml:math></inline-formula> m and down-valley
again above that altitude. This rotation with altitude is believed to be
caused by an interaction between the large-scale meteorological circulation,
the local topographic steering and the local forcing through the land–sea
temperature contrast.</p>
      <p id="d1e1684">The temperature inversion in the simulated baseline scenario was most
pronounced in sub-area 4. We assume this sub-area to be the most
representative of the interior valley. The other sub-areas show more or less
pronounced effects of the cold air passing over warm water bodies. The
simulated inversion profiles show multiple inversion layers that are not
resolved in the measured vertical temperature observations (resolution at 50 m). The maximum heights of the inversion profiles in the simulations are
somewhat shallower than what is typically observed. A more thorough
discussion of the simulated and observed inversion profiles in Bergen can be
found in Wolf-Grosse et al. (2017).</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F5" specific-use="star"><?xmltex \currentcnt{5}?><label>Figure 5</label><caption><p id="d1e1690">The simulated <inline-formula><mml:math id="M83" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration pattern in the baseline
scenario ws01_wd01_ft01 in the central part of
the model domain. The emission source is the road traffic (cars). The
concentrations were sampled at 5 m above the surface. Concentrations below 5 <inline-formula><mml:math id="M84" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M85" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> are omitted. The wind vectors characterise the flow 55 m
above the surface. The sampled data were averaged over the last 15 min of
the 6 h dispersion run. The concentrations are given by semi-transparent
colour shading overlaying the grayscale land and water surface taken from map
data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=284.527559pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f05.png"/>

        </fig>

      <?xmltex \floatpos{p}?><fig id="Ch1.F6" specific-use="star"><?xmltex \currentcnt{6}?><label>Figure 6</label><caption><p id="d1e1732">The same as in Fig. 5 but for the <inline-formula><mml:math id="M86" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration
pattern. The emission source of <inline-formula><mml:math id="M87" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> here was associated with the
wood-burning fireplaces. The concentrations are given by semi-transparent
colour shading overlaying the grayscale land and water surface taken from map
data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=284.527559pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f06.png"/>

        </fig>

      <p id="d1e1763">Due to its high spatial resolution, the PALM simulations created a detailed
geographical dispersion pattern of the <inline-formula><mml:math id="M88" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M89" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in and around the city. Figure 5 shows the <inline-formula><mml:math id="M90" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentration pattern created by the road traffic emission in the baseline
scenario. The underlying<?pagebreak page633?> geographical map (land and water surfaces) is given
in gray shading as a Google Maps<sup>®</sup>  picture. The use of
geoinformation tools to visualise the model simulations may facilitate the
use of the simulated quantitative information in decision-making processes.
The familiar map design simplifies orientation of and identification with
the complicated pollution pattern.</p>
      <p id="d1e1802">The simulations revealed that emissions from road traffic are the dominant
emission source for <inline-formula><mml:math id="M91" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> over the populated parts of the Bergen valley
during high-air-pollution episodes. This was also confirmed with a detailed
analysis of the timing of peak pollution levels from the local measurements
at the two reference stations together with considerations of the local mean
measured wind directions during high-air-pollution conditions (not shown).
The baseline scenario indicates that the <inline-formula><mml:math id="M92" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations are rather
high (<inline-formula><mml:math id="M93" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">100</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M94" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M95" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) not only in direct proximity to
the major roads but also in many adjacent urban areas. The exact shape and
structure of the valley topography imprint strongly on the local dispersion
conditions. Downwind of the major road transecting through the valley, areas
with a channelled flow appear. These are visible as streaks of elevated
pollution concentrations sometimes as high as 150 <inline-formula><mml:math id="M96" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M97" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. These
streaks are separated by areas with pollutant concentrations below 50 <inline-formula><mml:math id="M98" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M99" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The atmospheric channelling follows the areas with the
lowest topographic height. In addition, the small water bodies (lakes and
fjords) appear as areas with relatively lower air pollutant concentrations
due to their comparatively higher surface temperature and the subsequent
enhanced ventilation of the lowest air layers. This fine-scale structure of
the dispersion pattern is especially relevant, since the simulations
indicated elevated concentrations also in areas without continuous
measurements with a sufficient temporal resolution. Some urban areas might
be affected by pollution transport over several kilometres and accumulation
of emitted substances strongly different from the emission pattern.</p>
      <?pagebreak page635?><p id="d1e1898">The dominant emission sources for <inline-formula><mml:math id="M100" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> during high-air-pollution
episodes in the central Bergen valley turned out to be the wood-burning
fireplaces. This was visible in the PALM simulations as well as in the
detailed analysis of the available air pollution observations at the two
reference stations (not shown). Therefore, one could expect the highest
concentrations of the <inline-formula><mml:math id="M101" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the densely populated areas. Figure 6
shows the pattern of the <inline-formula><mml:math id="M102" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in the baseline scenario.
Distinct to the <inline-formula><mml:math id="M103" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> pattern, the <inline-formula><mml:math id="M104" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> pattern is more evenly
distributed over the entire city. The concentrations peak in the areas of
the near-surface flow convergence in the lower parts of the relief. Since
the wind is weak, areas with higher density of fireplaces are clearly
identifiable (Fig. 1).</p>
</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>The simulated patterns from different emission sources</title>
      <p id="d1e1964">A major advantage of the high-resolution modelling is related to the model's
ability to simulate separately the impact and patterns of the different
emission sources. As for <inline-formula><mml:math id="M105" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, the most significant emission sources in
Bergen are related to the ships in the harbour and the road traffic. This is
likely a typical situation for many coastal cities around the globe. We have
a reasonably good estimation of the absolute ship and traffic (road
vehicles) emission rates and their spatial distribution to run independent
simulations of their pathways and the <inline-formula><mml:math id="M106" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration patterns. The
combined assessment of the absolute and relative contributions from these
two local air pollution sources is provided in Fig. 7. The road traffic
emission dominates the urban air pollution almost everywhere in the city.
The absolute emission rate per ship in port is, however, quite high.
Assuming that within the assessed time, each vehicle is moved by 10 km, the
emission from each ship would correspond to the emission from 1377 typical
vehicles in Bergen. Using the concrete counts of the cars passing the
central area, it gives us that 16 ships at berth in the harbour emit about
127 % of the total car emission in the considered area. Such a
significantly higher emission has, however, smaller contribution to the
street-level concentrations of air pollutants. The ships emit at higher
elevations. As the vertical mixing is strongly reduced, their emission does
not reach the ground before they are either transported offshore over the
Byfjorden or diluted by the horizontal air movements.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><label>Figure 7</label><caption><p id="d1e1991">The same as in Fig. 5 but for the road traffic emission (red
shading) and the ships in the harbour emission (green shading) plotted
together through the artificial colour palette. Concentrations below 5 <inline-formula><mml:math id="M107" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M108" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> are omitted. The relative contribution of the ship
emissions into the total local <inline-formula><mml:math id="M109" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration are given by contours.
The concentrations are given by semi-transparent colour shading overlaying the
grayscale land and water surface taken from map data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=293.063386pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f07.png"/>

        </fig>

      <?xmltex \floatpos{p}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><label>Figure 8</label><caption><p id="d1e2033">The same as in Fig. 7 but for the <inline-formula><mml:math id="M110" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions from the
road traffic (red shading), ships in the harbour (green shading) and
wood-burning fireplaces (blue shading). Due to the dominating impact of the
emissions from wood-burning fireplaces, the red and green colours are only
visible at their emission hot spots in the harbour and at the major roads in
the southeastern part of the domain. The concentrations are given by
semi-transparent colour shading overlaying the grayscale land and water
surface taken from map data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=293.063386pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f07.png"/>

        </fig>

      <p id="d1e2054">There are three major sources of the <inline-formula><mml:math id="M111" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emission in Bergen, namely
ships, road traffic and wood-burning fireplaces. Figure 8 shows that
fireplaces dominate in their contribution to the local pollutant loadings,
even after the rescaling to provide more reasonable concentrations. The
emissions per ship are approximately 34 times that from a single
wood-burning fireplace after applying the scaling factor of 0.1. However,
the fireplaces are emitting at lower heights above the ground and clustered
in the most populated area. The ships emit the <inline-formula><mml:math id="M112" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the harbour
area where the emitted pollution is, in many weather conditions, effectively
transported offshore and diluted over the unpopulated fjord area. The
<inline-formula><mml:math id="M113" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations from the road traffic are overall low.</p>
      <p id="d1e2090">At this point, however, the high uncertainty of <inline-formula><mml:math id="M114" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions should
be emphasised, as emissions by road, tire and break abrasion have been
neglected in this study, in addition to the necessary correction of the
emission strength. Deposition of small- and larger-sized particulate matter (PM) may
in addition play a crucial role and correct the simulated pattern to some
degree. PM deposited on the ground can lead to high peak PM concentrations,
when moist urban surfaces are drying off after several days with fair
weather. This is especially relevant for major roads, where car-induced
turbulence can lead to a resuspension of dust greater than what the local
wind conditions would generate.</p>
</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Air pollution pattern sensitivity to meteorological scenarios</title>
      <p id="d1e2112">The baseline weather scenario represents the most typical meteorological
conditions leading to build-up of the air pollution in the city. The
concrete observed weather conditions, however, vary and may differ from the
considered scenario. Therefore, the air quality assessment needs to
characterise sensitivity of the pollution distribution patterns to imposed
perturbations of the meteorological parameters. The strong topographic
steering in the valley restricts deviations in the simulated patterns
produced by the sensitivity runs. Overall, the precursor sensitivity
simulations showed very similar geographical concentration patterns but with
varying accumulation strengths. The baseline and sensitivity scenarios are
listed in Table 2. Only the weather scenarios with the most notable
differences in the local dispersion conditions will be discussed below for
shortness of presentation.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F9" specific-use="star"><?xmltex \currentcnt{9}?><label>Figure 9</label><caption><p id="d1e2117">The same as in Fig. 7 but for the scenario ws03_wd02_ft02. The concentrations are given by semi-transparent
colour shading overlaying the grayscale land and water surface taken from map
data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=312.980315pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f09.png"/>

        </fig>

      <?xmltex \floatpos{p}?><fig id="Ch1.F10" specific-use="star"><?xmltex \currentcnt{10}?><label>Figure 10</label><caption><p id="d1e2128">The same as in Fig. 8 but for the scenario ws03_wd02_ft02. The concentrations are given by semi-transparent
colour shading overlaying the grayscale land and water surface taken from map
data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=312.980315pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f10.png"/>

        </fig>

      <p id="d1e2138">The stronger off-shore (easterly) wind (scenarios ws03_wd02_ ft01 and ws03_wd02_ft02)
deflect the pollutant plumes over the fjord water (Fig. 9 for <inline-formula><mml:math id="M115" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
Fig. 10 for <inline-formula><mml:math id="M116" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>), reducing the pollutant transport out of the
inhabited city centre and the harbour area. The waterfront takes most of the
impact. The concentration patterns in the valley interior remain largely
unchanged. We note that the pollution patterns became more fragmented in
those scenarios, indicating somewhat reduced stagnation and accumulation of
pollutants in the valley.</p>
      <?pagebreak page638?><p id="d1e2163">The most influential weather scenario with respect to the local dispersion
conditions is ws03_wd02_ft03 (see Figs. 11 and
12). A reversal of the flow at some elevation can be recognised from the
up-valley transport of the emissions from ships in the harbour in Fig. 11,
while the wind vectors at the lower (<inline-formula><mml:math id="M117" display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">55</mml:mn></mml:mrow></mml:math></inline-formula> m) level still suggests a
down-valley flow closer to the ground. This reversal was already visible in
the vertical profiles in Fig. 4 but at the higher levels, so that it was
invisible in the plume dispersion at the surface (Fig. 7). The flow reversal
is also vertically more extended in this simulation (not shown). The reason
for this is a change of the interplay between the locally forced circulation
due to the land–sea temperature contrast, the topographic steering and the
large-scale meteorological circulation. The weaker convergence over the
fjord due to the lower water surface temperatures and the stronger
large-scale winds weakens the down-valley circulation, reducing venting of
the pollutants from inhabited areas to the water surface in Byfjorden.
Hence, the populated areas close to the waterfront experience increased
accumulation of pollutants, especially visible for the <inline-formula><mml:math id="M118" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations in Fig. 12. This result is counterintuitive, as a stronger
large-scale wind allows for the increased accumulation. At the same time,
the highest concentrations of <inline-formula><mml:math id="M119" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> are reduced, as the large road
junctions in the interior of the valley are now affected by stronger winds
and hence dispersion of the pollutants.</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F11" specific-use="star"><?xmltex \currentcnt{11}?><label>Figure 11</label><caption><p id="d1e2202">The same as in Fig. 7 but for the scenario ws03_wd02_ft03. The concentrations are given by semi-transparent
colour shading overlaying the grayscale land and water surface taken from map
data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=312.980315pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f11.png"/>

        </fig>

      <?xmltex \floatpos{p}?><fig id="Ch1.F12" specific-use="star"><?xmltex \currentcnt{12}?><label>Figure 12</label><caption><p id="d1e2213">The same as in Fig. 8 but for the scenario ws03_wd02_ft03. The concentrations are given by semi-transparent
colour shading overlaying the grayscale land and water surface taken from map
data ©2019 Google.</p></caption>
          <?xmltex \igopts{width=312.980315pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f12.png"/>

        </fig>

</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Discussion</title>
      <p id="d1e2232">The routine monitoring of urban air quality with a few accredited
measurement stations is nowadays the main instrument of environmental
protection and control mechanisms. The decision-making process is frequently
assisted with statistical assessment, zonation and forecasting of the
concentrations of pollution levels. As the monitoring becomes cheaper and
more accessible, a more detailed monitoring of the concentration levels in
the urban environment gradually emerges (see, e.g., the CurieuzeNeuzen
project; CurieuzeNeuzen, 2019). For example, the area of the Bergen
municipality is monitored today with five stations measuring
the air quality characteristic of the
most populous districts.
However, as we demonstrate in this study, such an observational network is
sub-optimal and not fully representing the complexity caused by the
topography of a coastal valley environment. The typical spatial scales of
the surface topography and heterogeneity require in principle a denser
monitoring network and refinement of the forecast models in order to reach a
deeper understanding of the local dispersion conditions at adequate spatial
scales. In the case of Bergen, the model resolutions of a hundred metres
or finer are necessary in order to resolve the processes for distribution and
accumulation of air pollutants near the surface
(Cheynet et al., 2017).</p>
      <p id="d1e2235">Such high-resolution models are now available. The existing computer
capacity allows running the model simulations for several typical
meteorological scenarios, which are associated with the typically observed
air pollution episodes. In Bergen, it was found that mainly a few
meteorological scenarios result in high pollution concentrations
(Wolf et al., 2014). Therefore,
high-resolution scenario modelling is not only technically feasible but also
would create an added value for the risk and vulnerability assessment for
urban areas. In future, high-resolution models could be coupled with
existing routine numerical weather forecasts and data assimilated from
measurement stations. The present study was, however, limited to the air
quality assessment tasks, which are related to a local policy-making and
planning processes. It does not intend to advance to the routine local air
quality forecast.</p>
      <p id="d1e2238">All emissions of air pollution are harmful to the environment at large;
however, in development of pollution policies and mitigation strategies,
quantification of the major sources of pollution and in particular their
impact on the observed elevated concentrations of the polluting substances
at the street level is needed. This is a difficult assessment task as the
emitted pollution is transported and dispersed by an intricate pattern of
the turbulent local flows in an urban environment. The dynamic nature of the
concentration patterns and their sensitivity to the variations of the
meteorological conditions are not fully considered. This study demonstrates
that the use of high-resolution atmospheric models can contribute to
overcoming this challenge. The models can simulate the dynamics and specific
contribution of each of the individual air pollution sources into the total
concentration of each pollutant, here demonstrated for <inline-formula><mml:math id="M120" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M121" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. Such simulation results might be utilised to tune policies and
regulations in a dialogue with the major polluters and the citizens. In the
presented case of the Bergen port authorities, they assess the simulated
concentration patterns to minimise the impact of the ship exhaust on the
city air quality.</p>
      <p id="d1e2263">It should be noted here that the high-resolution dispersion pattern produced
in this study is based on physical meteorological fields with an equally
high resolution, thus including the effect of topographic steering and other
local forcing, consistent with how the simulations are defined. Other
attempts to produce high-resolution dispersion patterns in Bergen and other
places are to our knowledge based on lower-resolution meteorological fields
but high-resolution emission maps (e.g. Miljødirektoratet,
2019). This gives the maps an erroneously high-resolution appearance that
however neglects the important impact of local flow steering.</p>
      <p id="d1e2267">The high-resolution modelling is a relatively new approach in meteorology
and air quality studies. Several scientific challenges need to be resolved
in future studies. Model simulations with this amount of spatial detail are
difficult to validate against observations. While it is possible to state
that the simulated pollutant pattern and meteorological conditions are
reasonably similar to the observations, a rigorous validation is
challenging. Usual validation against operational weather stations run by
meteorological services is not possible due to a too-low spatial density of
the observations. Including the abundantly available citizen observations
might be a pathway for future validation
(Johansson et al., 2015; Schneider et al.,
2017; Zilitinkevich et al., 2015) but goes beyond the scope of this study.
General validation of the modelling technique is required with dedicated
measurement campaigns or experiments (e.g. Hertwig, 2013). The
Bergen test bed with its high density of meteorological observations could
serve as a proper validation case.</p>
      <?pagebreak page640?><p id="d1e2270">The scenarios for the initialisation of the model simulations should be
improved in order to increase correspondence between observed and modelled
conditions (e.g. Maronga et al., 2019). This is necessary
both for improving the realism of the simulations and  for their
validation. The subset of simulated conditions needs to be compared to the
relevant subset of observed conditions. For this, a better correspondence
with observed cases is necessary. It is clear that model simulations with
periodic boundary conditions, as used in this study, are only an
intermediate step. Simultaneously, a reduction of the computational costs
should be assessed. Both could be achieved through nesting of model domains
with different spatial resolutions, as it is already routinely done for
coarser-scale simulations with, e.g. the Weather Research and Forecasting
(WRF) model
(Cécé et al.,
2016; Muñoz-Esparza et al., 2017).</p>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <label>6</label><title>Conclusions</title>
      <p id="d1e2281">This study applied the turbulence-resolving model PALM in the local air
quality context to assess the conditions and consequences of low-level
emission of nitrogen dioxide (<inline-formula><mml:math id="M122" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) and particulate matter (<inline-formula><mml:math id="M123" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>)
from the major polluters in the city of Bergen, Norway. We ran simulations
at 10 m resolution over a very large geographic domain spanning 12.79 km in
the zonal (east–west) and 17.27 km in the meridional (north–south)
directions. In order to assess the possible bandwidth of circulation
conditions inside the valley, we conducted a set of eight sensitivity runs
with varying model forcing in addition to the baseline scenario, reflecting
the most typically observed air pollution conditions. We simulated
separately the emissions from the three major local emission sources of air
pollution. These are car traffic, heating in wood-burning fireplaces and
emissions from offshore supply vessels docked in the harbour area, located
next to the city centre.</p>
      <p id="d1e2306">The results support the following conclusions: the very high-resolution
numerical atmospheric simulations change our perspective on the magnitude
and dynamics of the air quality under the most typical air quality hazard
situations. Small topographic features like the shape of the valley floor or
local water bodies strongly affect the dispersion and accumulation
conditions for air pollutants. This results in areas with a channelled flow,
where air with a high pollution load (in excess of 150 <inline-formula><mml:math id="M124" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M125" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for
<inline-formula><mml:math id="M126" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) can be transported over several hundred metres or even kilometres.
Especially for <inline-formula><mml:math id="M127" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> both areas with maximum emissions and areas
with minimum ventilation show higher concentrations in the dispersion maps.
The sensitivity runs highlight the relevance of the interplay between the
local surface conditions and the larger-scale atmospheric circulation.
Attempts to model the dispersion of pollutants in this city at resolutions
that are unable to resolve this interplay and the local fine-scale
topographic features will most likely fail to produce the necessary details
of the dispersion map.</p>
      <p id="d1e2351"><?xmltex \hack{\newpage}?>The separate analysis of emissions from the three major emission sources was
helpful in a source appointment of the overall pollution levels in the city
centre. An assumed high impact of the ships located in Bergen harbour as the
major polluter in the city was not generally confirmed in the simulations
during winter conditions. Despite the 16 supply vessels in the harbour
emitting 27 % more <inline-formula><mml:math id="M128" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> than all cars in the simulated domain, their
relative impact on the air pollution over inhabited parts of the valley near
the ground exceeds 25 % over a larger area only for one of the simulated
scenarios. This could, however, be different for other, similar harbours, as
our simulations attributed this lower impact to the intrinsic structure of
the local circulations at the waterfront.</p>
      <p id="d1e2366">The usage of high-resolution data and numerical model simulations for
meteorological services gives a so-far unprecedented amount of detail for
end users and allows for a direct connection of the scientific issues with
an understanding of the societal dimensions as stated in the Pan-Eurasian
Experiment (PEEX) white paper addressing a holistic understanding of the
feedbacks and interactions in the land–atmosphere–ocean–society continuum
(Lappalainen et al., 2016). The
BOH deemed the results from this study  helpful
for their efforts to manage and reduce the impact of emissions from ships in
the harbour on the local population. This study serves as a demonstration of
a concept for an approach of statistical dynamical downscaling applied to
high-resolution services by making LES usable for a reduced and therewith
feasible amount of possible model simulations under selected meteorological
scenarios.</p>
</sec>

      
      </body>
    <back><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e2373">The study has used external data from the following sources: Endre Leivestad
and Trond Grindheim – Bergen Municipality, Haso Bradaric – Norwegian
Mapping Authority, Ole Edvard Grov and Joachim Reuder – University of
Bergen, Rita Våler – Norwegian Institute for Air Research, Stig Nyland
Andersen – Norwegian Public Road Authority, Even Husby – BOH and the
European Centre for Medium-Range Weather Forecasts (ECMWF). The PALM model
is developed and maintained at the Institute of Meteorology and Climatology,
Leibniz University Hannover. CPU time was provided through the Norwegian
Supercomputing Project (NOTUR II grant numbers nn2993k and nn9528k). The
illustrations were prepared as a colour-coded semi-transparent contour and
shading layers on top of a Google Maps background (<uri>http://code.google.com/apis/maps/</uri>, last access: 1 March 2019, using the get Google map version 2.0
function from the MathWorks file exchange; <uri>https://se.mathworks.com/matlabcentral/fileexchange/27627-zoharby-plot-google-map</uri>, last access: 1 March 2019, Bar-Yehuda, 2019).</p>
  </notes><?xmltex \hack{\clearpage}?><app-group>

<?pagebreak page641?><app id="App1.Ch1.S1">
  <?xmltex \currentcnt{A}?><label>Appendix A</label><title>Emissions from road traffic</title>
      <p id="d1e2393">The emissions from road traffic vary strongly with the composition of the
vehicle fleet passing a road link. We calculated emission factors
specifically for the vehicle fleet at use in Bergen.</p>

      <?xmltex \floatpos{t}?><fig id="App1.Ch1.S1.F13" specific-use="star"><?xmltex \currentcnt{A1}?><label>Figure A1</label><caption><p id="d1e2398">Annual mean daily traffic flow in vehicle metres
(<inline-formula><mml:math id="M129" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>l</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)
in each PALM grid cell for side streets <bold>(a)</bold> and main roads <bold>(b)</bold>.
Both colour shadings have the unit of metres. Roads in the left panel that
are appearing to go straight into mountainous areas are sporadically used
small utility roads. For simplicity of the underlying traffic model, they are
indicated as straight roads instead of following their actual path.
Emissions from these roads are negligible.</p></caption>
        <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f13.png"/>

      </fig>

<?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T3" specific-use="star"><?xmltex \currentcnt{A1}?><label>Table A1</label><caption><p id="d1e2434">Emission factors <inline-formula><mml:math id="M130" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">r</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for <inline-formula><mml:math id="M131" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M132" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> for the different vehicle types.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="7">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right"/>
     <oasis:thead>
       <oasis:row>

         <oasis:entry colname="col1"/>

         <oasis:entry rowsep="1" namest="col2" nameend="col3" align="center"><inline-formula><mml:math id="M135" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (g km<inline-formula><mml:math id="M136" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)<inline-formula><mml:math id="M137" display="inline"><mml:msup><mml:mi/><mml:mtext>a</mml:mtext></mml:msup></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry rowsep="1" namest="col5" nameend="col6" align="center"><inline-formula><mml:math id="M138" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (g km<inline-formula><mml:math id="M139" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)<inline-formula><mml:math id="M140" display="inline"><mml:msup><mml:mi/><mml:mtext>a</mml:mtext></mml:msup></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col7"/>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">Vehicle</oasis:entry>

         <oasis:entry colname="col2">Congested</oasis:entry>

         <oasis:entry colname="col3">Freely flowing</oasis:entry>

         <oasis:entry colname="col4">Mean emission</oasis:entry>

         <oasis:entry colname="col5">Congested</oasis:entry>

         <oasis:entry colname="col6">Freely flowing</oasis:entry>

         <oasis:entry colname="col7">Mean emission</oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">type</oasis:entry>

         <oasis:entry colname="col2">city traffic</oasis:entry>

         <oasis:entry colname="col3">city traffic</oasis:entry>

         <oasis:entry colname="col4">factors</oasis:entry>

         <oasis:entry colname="col5">city traffic</oasis:entry>

         <oasis:entry colname="col6">city traffic</oasis:entry>

         <oasis:entry colname="col7">factor</oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1"/>

         <oasis:entry colname="col2"/>

         <oasis:entry colname="col3"/>

         <oasis:entry colname="col4">(<inline-formula><mml:math id="M141" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M142" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M143" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)<inline-formula><mml:math id="M144" display="inline"><mml:msup><mml:mi/><mml:mtext>b</mml:mtext></mml:msup></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col5"/>

         <oasis:entry colname="col6"/>

         <oasis:entry colname="col7">(<inline-formula><mml:math id="M145" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M146" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M147" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)<inline-formula><mml:math id="M148" display="inline"><mml:msup><mml:mi/><mml:mtext>b</mml:mtext></mml:msup></mml:math></inline-formula></oasis:entry>

       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1">Passenger car diesel</oasis:entry>

         <oasis:entry rowsep="1" colname="col2">0.350</oasis:entry>

         <oasis:entry rowsep="1" colname="col3">0.183</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry rowsep="1" colname="col5">0.0043</oasis:entry>

         <oasis:entry rowsep="1" colname="col6">0.0017</oasis:entry>

         <oasis:entry colname="col7"/>

       </oasis:row>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1">Passenger car gasoline</oasis:entry>

         <oasis:entry rowsep="1" colname="col2">0.004</oasis:entry>

         <oasis:entry rowsep="1" colname="col3">0.002</oasis:entry>

         <oasis:entry colname="col4">2.51 <inline-formula><mml:math id="M149" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry rowsep="1" colname="col5">0.0009</oasis:entry>

         <oasis:entry rowsep="1" colname="col6">0.0006</oasis:entry>

         <oasis:entry colname="col7"><inline-formula><mml:math id="M150" display="inline"><mml:mrow><mml:mn mathvariant="normal">3.52</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">7</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">Passenger car electric</oasis:entry>

         <oasis:entry colname="col2">0</oasis:entry>

         <oasis:entry colname="col3">0</oasis:entry>

         <oasis:entry colname="col4"/>

         <oasis:entry colname="col5">0</oasis:entry>

         <oasis:entry colname="col6">0</oasis:entry>

         <oasis:entry colname="col7"/>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">Small delivery vans</oasis:entry>

         <oasis:entry colname="col2">0.300</oasis:entry>

         <oasis:entry colname="col3">0.217</oasis:entry>

         <oasis:entry colname="col4">5.47 <inline-formula><mml:math id="M151" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col5">0.0050</oasis:entry>

         <oasis:entry colname="col6">0.0021</oasis:entry>

         <oasis:entry colname="col7">7.51 <inline-formula><mml:math id="M152" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">7</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row rowsep="1">

         <oasis:entry colname="col1">Heavy lorries</oasis:entry>

         <oasis:entry colname="col2">0.899</oasis:entry>

         <oasis:entry colname="col3">0.481</oasis:entry>

         <oasis:entry colname="col4">1.79 <inline-formula><mml:math id="M153" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry colname="col5">0.0904</oasis:entry>

         <oasis:entry colname="col6">0.0385</oasis:entry>

         <oasis:entry colname="col7">1.68 <inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry rowsep="1" colname="col1">City bus diesel</oasis:entry>

         <oasis:entry rowsep="1" colname="col2">2.530</oasis:entry>

         <oasis:entry rowsep="1" colname="col3">1.430</oasis:entry>

         <oasis:entry colname="col4" morerows="1">3.76 <inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

         <oasis:entry rowsep="1" colname="col5">0.0083</oasis:entry>

         <oasis:entry rowsep="1" colname="col6">0.0041</oasis:entry>

         <oasis:entry colname="col7" morerows="1">1.22 <inline-formula><mml:math id="M156" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>

       </oasis:row>
       <oasis:row>

         <oasis:entry colname="col1">City bus gas</oasis:entry>

         <oasis:entry colname="col2">0</oasis:entry>

         <oasis:entry colname="col3">0</oasis:entry>

         <oasis:entry colname="col5">0</oasis:entry>

         <oasis:entry colname="col6">0</oasis:entry>

       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><table-wrap-foot><p id="d1e2470"><inline-formula><mml:math id="M133" display="inline"><mml:msup><mml:mi/><mml:mtext>a</mml:mtext></mml:msup></mml:math></inline-formula> Hagman and Amundsen (2011). <inline-formula><mml:math id="M134" display="inline"><mml:msup><mml:mi/><mml:mtext>b</mml:mtext></mml:msup></mml:math></inline-formula> Calculated for this study.</p></table-wrap-foot></table-wrap>

      <p id="d1e3028">Traffic flow information from the national road authority overlaps with the
traffic flow information from the Bergen municipality (Sect. 2.2). Both
include information on main roads. We assume the measurement-based traffic
flow information from Bergen municipality to be more representative than the
model-based traffic flow information from the national road authority. We
therefore combined both into one consistent dataset giving preference to
information from Bergen municipality wherever possible. The information used
from the two datasets is shown in Fig. A1.</p>

      <?xmltex \floatpos{p}?><fig id="App1.Ch1.S1.F14"><?xmltex \currentcnt{A2}?><label>Figure A2</label><caption><p id="d1e3033">Number of wood-burning fireplaces per PALM grid cell
(<inline-formula><mml:math id="M157" display="inline"><mml:mrow><mml:msub><mml:mi>n</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) after spatial averaging.</p></caption>
        <?xmltex \igopts{width=199.169291pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f14.png"/>

      </fig>

      <?xmltex \floatpos{p}?><fig id="App1.Ch1.S1.F15" specific-use="star"><?xmltex \currentcnt{A3}?><label>Figure A3</label><caption><p id="d1e3055">Ship positions in Bergen harbour. The numbers behind the names of
the harbour docks indicate the number of hours with supply ships docked at
each of the harbour docks from January 2015 to March 2016.</p></caption>
        <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/625/2020/acp-20-625-2020-f15.png"/>

      </fig>

      <p id="d1e3064">We decided to neglect the emissions from tunnels. This is in contrast to
another study recently conducted for the Bergen area based on statistical
modelling (Denby, 2014). This study split all emissions from
within tunnels equally to both ends. This approach neglects the ventilation
system especially at use in longer tunnels that always runs either towards
one side or removes air through vertical ventilation shafts at some distance
from the tunnel ends, mostly away from inhabited areas. This will lead to an
underestimation of street emissions at the positions of the ventilation
shafts and some tunnel exits but avoids the problem of an unknown
overestimation of emissions at all tunnel openings.</p>
      <p id="d1e3067">For the separation of the vehicle fleet in Bergen into different vehicle
classes, we used information from an Oslo-based survey (Hagman and
Amundsen, 2011). In this survey, small passenger cars account for 72 % of
all road traffic. The remaining 28 % are composed of small diesel-driven
delivery cars (15 %), heavy transportation with lorries (10 %) and
busses (3 %). The passenger cars are furthermore divided into 47.6 %
diesel driven cars, 49.7 % gasoline driven cars and 2.6 % electric
cars. Due to the high road taxes for any vehicle other than electric cars and the
increasing number of electric cars over time, especially in the Bergen area,
we assume that electric cars are used 4 times as often as other types.
This leads to the final distribution of passenger cars of 44 % diesel
driven, 46 % gasoline driven and 10 % electric. From the 3 % bus
traffic, 27 % is gas driven (Målfrid Vik Sønstabø, public
transport authority, personal communication, 2016). These are assumed to
have negligible emissions of <inline-formula><mml:math id="M158" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M159" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e3093"><?xmltex \hack{\newpage}?>For the specific emissions per driving distance, we use constant values for
all streets in Bergen and a constant composition of the traffic pattern. Due
to a lack of information on the specific vehicles, speeds and driving
patterns along each street we assume all vehicles to have emission class
Euro 5 and that the vehicles are standing in congested traffic for 50 %
of the time. This gives some errors due to different driving pattern or
vehicle-fleet compositions along specific roads, but a more detailed
specification of the emissions would be beyond the scope of this work. The
emission factors per distance and vehicle type are stated in Table A1.</p>
      <p id="d1e3097">The traffic flow information is given in annual mean daily traffic flow.
Typically, the highest <inline-formula><mml:math id="M160" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> pollutant concentrations are measured
between 07:00 and 17:00 UTC during working days and in February. For the
assessment of the traffic during these times, we used the traffic information
from Danmarksplass, close to the DP air pollution reference station. This
area should be representative of the traffic in Bergen, as it is one of the
main streets handling the city traffic. During the 10 h 67 % and 75 % of all traffic happens with passenger cars/small delivery vans and
heavy lorries/city buses, respectively. In addition, 1.125 and 1.011 times
the annual mean daily traffic happen during working days and February
for passenger cars/small delivery vans. The corresponding numbers for heavy
lorries/city buses are 0.965 and 1.298, respectively.</p>
      <p id="d1e3111">The resulting total emission factors for road traffic are thus
<inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">r</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">5.54</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M162" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g (m<inline-formula><mml:math id="M163" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M164" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> s)  for <inline-formula><mml:math id="M165" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">r</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">2.10</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M167" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g (m<inline-formula><mml:math id="M168" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M169" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> s) for <inline-formula><mml:math id="M170" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> distributed
over the 100 m<inline-formula><mml:math id="M171" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> large grid cells. All emissions from road traffic are
averaged over <inline-formula><mml:math id="M172" display="inline"><mml:mrow><mml:mn mathvariant="normal">3</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:math></inline-formula> grid cells to follow the width of large streets, where
most of the emissions take place and include the effects of vehicle-induced
turbulence.</p><?xmltex \hack{\clearpage}?>
</app>

<?pagebreak page644?><app id="App1.Ch1.S2">
  <?xmltex \currentcnt{B}?><label>Appendix B</label><title>Emissions from wood-burning fireplaces</title>
      <p id="d1e3266">The emission factors from wood-burning fireplaces assume constant emissions
per oven according to the existing mix of oven types in Bergen and their
estimated typical usage (both provided by the Bergen fire department).
According to these numbers, there are 25 % modern ovens with catalysators,
25 % modern ovens without catalysators and 50 % old ovens presently in
use in Bergen. These have emissions factors of 5, 10 and 30 g kg<inline-formula><mml:math id="M173" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> burned
wood, of which 90 % are assumed in the size fraction <inline-formula><mml:math id="M174" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. Like the
street-related emissions, we averaged the emissions per oven over <inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:mn mathvariant="normal">3</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:math></inline-formula> grid
cells.</p>
      <p id="d1e3304">Overall, 70 % of all wood-burning fireplaces are assumed in use during cold winter
days. In addition, each property that is registered to have fireplaces might
have at least one fireplace, possibly more. Together, it is therefore roughly
assumed that one wood-burning fireplace per property might be used on a
daily basis. Figure A2 shows the number of wood-burning fireplaces per grid
cell after special averaging. During a typical firing cycle, a total of 11 kg of
wood are assumed to be used, and we assume that most use of the firing
occurs between 16:00 and 23:00 UTC, after people come home from work. The
final emission factor per property with a fireplace registered is therefore
<inline-formula><mml:math id="M176" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">c</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">74.21</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M177" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M178" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s for
<inline-formula><mml:math id="M179" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> distributed over the 100 m<inline-formula><mml:math id="M180" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> large grid cells. Wood-burning
fireplaces are assumed not to contribute significantly to the local <inline-formula><mml:math id="M181" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
emissions.</p>
</app>

<app id="App1.Ch1.S3">
  <?xmltex \currentcnt{C}?><label>Appendix C</label><title>Emissions from ships</title>
      <p id="d1e3382">Figure A3 shows the position of the harbour docks frequented by supply ships
in Bergen together with the number of hours with supply ships docked at
these locations from January 2015 to March 2016. In order to identify the
most typically used locations, we specified emissions in PALM from all
harbour docks with more than 20 h of ship docking time in the analysed
period. This reduced the number of supply ships with emissions specified in
the PALM simulations to 16. This can be seen as a higher threshold for the
number of supply ships typically in the harbour, describing a busy day. For
the emissions, we assumed that the ships were running their secondary engines
for onboard energy supply during docking.</p>
      <p id="d1e3385">For the assessment of the emissions per ship, we used the mean numbers for
two offshore oil-exploration-related ship types that are the most typical in
Bergen. These are the smaller offshore platform supply vessels (represented
by Normand Carrier, Solstad Shipping) and the larger anchor handling vessels
(represented by Normand Ranger, Solstad Shipping); both are for simplicity
reasons referred to as offshore supply vessels in this study. The larger
ship had a weight of 3051 gross tonnage (GT) and typical <inline-formula><mml:math id="M182" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions
of 41.05 g kg<inline-formula><mml:math id="M183" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> spent fuel. The smaller ship had a weight of 4750 GT and
typical <inline-formula><mml:math id="M184" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions of 39.28 g kg<inline-formula><mml:math id="M185" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> spent fuel. According to Volker
Matthias (Helmholtz Centre for Materials and Coastal Research Geesthacht,
personal communication, 2016), of the total <inline-formula><mml:math id="M186" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions from these
ships, 10 % are <inline-formula><mml:math id="M187" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The average <inline-formula><mml:math id="M188" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emission of both ships is
therefore <inline-formula><mml:math id="M189" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">4.02</mml:mn></mml:mrow></mml:math></inline-formula> g kg<inline-formula><mml:math id="M190" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> spent fuel. We calculated the typical fuel usage
of the ships based on their weight, as suggested in
Hulskotte et al. (2014). The typical mean fuel usage
for both ships, when at berth was <inline-formula><mml:math id="M191" display="inline"><mml:mrow><mml:msub><mml:mi>v</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">67</mml:mn></mml:mrow></mml:math></inline-formula> kg h<inline-formula><mml:math id="M192" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the mean ship weight of 3900 GT. This results in a typical
emission factor per supply ship of 275 g h<inline-formula><mml:math id="M193" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> or <inline-formula><mml:math id="M194" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">763.31</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M195" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g (m<inline-formula><mml:math id="M196" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> s) distributed over the 100 m<inline-formula><mml:math id="M197" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> large grid cells. For the <inline-formula><mml:math id="M198" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions, we used
<inline-formula><mml:math id="M199" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1.5</mml:mn></mml:mrow></mml:math></inline-formula> g kg<inline-formula><mml:math id="M200" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> spent fuel for both ships with 90 % of the
particles in the <inline-formula><mml:math id="M201" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> size range (Volker Matthias, Helmholtz Centre
for Materials and Coastal Research Geesthacht, personal communication,
2016). This led to emission factors of 90 g h<inline-formula><mml:math id="M202" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> or <inline-formula><mml:math id="M203" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">251.03</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M204" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g (m<inline-formula><mml:math id="M205" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> s) distributed over the 100 m<inline-formula><mml:math id="M206" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> large grid cells for <inline-formula><mml:math id="M207" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. All these numbers assume that no
specific fuel cleaning technology was in use while the ships are at berth, as
recommended by Even Husby (BOH, personal communication, 2016). The emission
numbers are in agreement with measurements of ship plumes some distance from
the ships in Finland
(Pirjola et al.,
2014).</p>
      <p id="d1e3691">In order to account for the elevated emission from ships, we artificially
increased topography at the location of the ships to a typical height of the
chimneys on top of the assessed supply vessels plus an offset to account for
initial plume rise. This way, we could specify the emissions as fluxes from
the ground. Elevated fluxes were not readily available in the used PALM
version. The total increase of the topographic height at the location of the
ships is 40 m. This gives an elevated plume rise but not too strong
disturbance of the local flow pattern, since the increase in topographic
height for the entire domain only covered 16 grid points. Additional plume
rise is considered by setting a positive surface heat flux on top of the
elevated topography of 1000 W m<inline-formula><mml:math id="M208" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
</app>

<app id="App1.Ch1.S4">
  <?xmltex \currentcnt{D}?><label>Appendix D</label><title>A list of publications on the use of PALM for urban air quality studies.</title>
      <p id="d1e3714">The PALM model has been used in a number of peer-review research articles and online materials certifying its quality and applicability for urban air quality, turbulent dynamics and pollution diffusion studies. Here we would like to provide a quick reference list of these publications for interested readers: Castillo et al. (2009), Gronemeier et al. (2016), Kanda et al. (2013), Kurppa et al. (2018), Letzel et al. (2008, 2012), Maronga et al. (2015, 2019), Pavlik et al. (2019) and Park et al. (2012).</p><?xmltex \hack{\clearpage}?>
</app>
  </app-group><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e3722">All co-authors conceptualised the study and designed the applied
methodology. LHP and TW collected the data. LHP and TW acquired the funding.
IE was the project manager. IE and TW designed and applied the software. IE
had a role of supervision for TW. TW developed the visualisation with
support from IE and LHP. IE initialised the manuscript. TW wrote the first
manuscript. All authors contributed to the review and editing of the
manuscript.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e3728">The authors declare that they have no conflict of interest.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e3734">This study is performed within the GC Rieber Climate Research Institute at the Nansen Center, under a contract with Port of Bergen (BOH). Ulrik Jørgensen, Sverre Østvold, Nils Møllerup and Even Husby – BOH, and Eva Britt Isager and Per Vikse – Climate section, Mette Iversen and Nils-Eino Langhelle – Section for Plan and
Geodata, Per Hallstein Fauske and Arve Bang, Health Care Agency, all Bergen municipality, provided the user perspective and
valuable cooperation.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e3739">This research has been supported by Port of Bergen and  strategic institute funding (RCN grant no. 218857). The initial developments were funded by grants from the GC Rieber foundation.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e3746">This paper was edited by Ashu Dastoor and reviewed by two anonymous referees.</p>
  </notes><ref-list>
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<abstract-html><p>Urban air quality is one of the most prominent
environmental concerns for modern city residents and authorities. Accurate
monitoring of air quality is difficult due to intrinsic urban landscape
heterogeneity and superposition of multiple polluting sources. Existing
approaches often do not provide the necessary spatial details and peak
concentrations of pollutants, especially at larger distances from monitoring
stations. A more advanced integrated approach is needed. This study presents
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weather conditions with high air pollution from nitrogen dioxide (NO<sub>2</sub>)
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identify pathways and patterns of air pollution caused by the three main
local air pollution sources in the city. These are road vehicle traffic,
domestic house heating with wood-burning fireplaces and ships docked in the
harbour area next to the city centre. The study produced vulnerability maps,
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scenario. Overall, the largest contribution to air pollution over inhabited
areas in Bergen was caused by road traffic emissions for NO<sub>2</sub> and
wood-burning fireplaces for PM<sub>2.5</sub> pollution. The effect of emission
from ships in the port was mostly restricted to the areas close to the
harbour and moderate in comparison. However, the results have contributed to
implementation of measures to reduce emissions from ships in Bergen harbour,
including provision of shore power.</p></abstract-html>
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