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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-20-10667-2020</article-id><title-group><article-title>The impact of ship emissions on air quality and human health in<?xmltex \hack{\break}?> the
Gothenburg area – Part II: Scenarios for 2040</article-title><alt-title>Part II: Scenarios for 2040</alt-title>
      </title-group><?xmltex \runningtitle{Part II: Scenarios for 2040}?><?xmltex \runningauthor{M. O. P. Ramacher et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1">
          <name><surname>Ramacher</surname><given-names>Martin O. P.</given-names></name>
          <email>martin.ramacher@hzg.de</email>
        <ext-link>https://orcid.org/0000-0001-5813-2258</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2 aff3">
          <name><surname>Tang</surname><given-names>Lin</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Moldanová</surname><given-names>Jana</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1737-2391</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Matthias</surname><given-names>Volker</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-0519-8805</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Karl</surname><given-names>Matthias</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-0821-018X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Fridell</surname><given-names>Erik</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4">
          <name><surname>Johansson</surname><given-names>Lasse</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>Helmholtz-Zentrum Geesthacht, 21502 Geesthacht, Germany</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>IVL, Swedish Environmental Research Institute, P.O. Box 53021, 40014 Gothenburg, Sweden</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>WSP Environment Sweden, P.O. Box 13033, 40251 Gothenburg, Sweden</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki,
Finland</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Martin O. P. Ramacher (martin.ramacher@hzg.de)</corresp></author-notes><pub-date><day>11</day><month>September</month><year>2020</year></pub-date>
      
      <volume>20</volume>
      <issue>17</issue>
      <fpage>10667</fpage><lpage>10686</lpage>
      <history>
        <date date-type="received"><day>2</day><month>April</month><year>2020</year></date>
           <date date-type="rev-request"><day>14</day><month>April</month><year>2020</year></date>
           <date date-type="rev-recd"><day>29</day><month>June</month><year>2020</year></date>
           <date date-type="accepted"><day>8</day><month>July</month><year>2020</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2020 </copyright-statement>
        <copyright-year>2020</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/.html">This article is available from https://acp.copernicus.org/articles/.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/.pdf</self-uri>
      <abstract><title>Abstract</title>
    <p id="d1e157">Shipping is an important source of air pollutants, from
the global to the local scale. Ships emit substantial amounts of
sulfur dioxides, nitrogen dioxides, and particulate matter in the vicinity
of coasts, threatening the health of the coastal population, especially in
harbour cities. Reductions in emissions due to shipping have been targeted
by several regulations. Nevertheless, effects of these regulations come into
force with temporal delays, global ship traffic is expected to grow in the
future, and other land-based anthropogenic emissions might decrease. Thus,
it is necessary to investigate combined impacts to identify the impact of
shipping activities on air quality, population exposure, and health effects
in the future.</p>
    <p id="d1e160">We investigated the future effect of shipping emissions on air quality and
related health effects considering different scenarios of the development of
shipping under current regional trends of economic growth and already
decided regulations in the Gothenburg urban area in 2040. Additionally, we
investigated the impact of a large-scale implementation of shore electricity
in the Port of Gothenburg. For this purpose, we established a one-way nested
chemistry transport modelling (CTM) system from the global to the urban
scale, to calculate pollutant concentrations, population-weighted
concentrations, and health effects related to <inline-formula><mml:math id="M1" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M2" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M3" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
    <p id="d1e194">The simulated concentrations of <inline-formula><mml:math id="M4" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M5" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> in future scenarios
for the year 2040 are in general very low with up to 4 ppb for <inline-formula><mml:math id="M6" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
up to 3.5 <inline-formula><mml:math id="M7" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M8" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> PM<inline-formula><mml:math id="M9" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> in the urban areas which
are not close to the port area. From 2012 the simulated overall exposure to
PM<inline-formula><mml:math id="M10" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> decreased by approximately 30 % in simulated future scenarios;
for <inline-formula><mml:math id="M11" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the decrease was over 60 %. The simulated concentrations of
<inline-formula><mml:math id="M12" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> increased from the year 2012 to 2040 by about 20 %. In general, the
contributions of local shipping emissions in 2040 focus on the harbour area
but to some extent also influence the rest of the city domain. The simulated
impact of onshore electricity implementation for shipping in 2040 shows
reductions for <inline-formula><mml:math id="M13" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the port of up to 30 %, while increasing
<inline-formula><mml:math id="M14" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> of up to 3 %. Implementation of onshore electricity for ships at
berth leads to additional local reduction potentials of up to 3 % for
PM<inline-formula><mml:math id="M15" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and 12 % for <inline-formula><mml:math id="M16" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the port area. All future scenarios
show substantial decreases in population-weighted exposure and health-effect
impacts.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e341">Shipping is an important source of air pollutants, from the global to the
local scale. Nearly 70 % of ship emissions occur within 400 km of
coastlines (Corbett et al., 1999), causing air quality problems through
emissions of sulfur dioxide (<inline-formula><mml:math id="M17" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>), nitrogen dioxides (<inline-formula><mml:math id="M18" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and
particulate matter (PM). An increase in shipping activity in the North Sea
and the Baltic Sea has resulted in higher emissions of air pollutants and
subsequently concentrations of pollutants in air, in particular of <inline-formula><mml:math id="M19" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
especially in and around several major ports (Kalli et al., 2013). The high
contribution of shipping to emissions of sulfur and consequently to acid
deposition and air pollution with particulate matter, mainly originating
from the oxidation of the <inline-formula><mml:math id="M20" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions, has been targeted<?pagebreak page10668?> by the
International Maritime Organization (IMO) by setting limits on the maximum
sulfur content of marine fuels (IMO, 2008). While on the global level a
fuel sulfur content limit of 0.5 %, from previously 3.5 %, came
into force on 1 January 2020, the Baltic Sea and the North Sea were declared Sulfur Emission Control Areas (SECAs) in 2006, gradually
decreasing the fuel sulfur limit to 1.5, 1, and 0.1 % in 2006, 2010, and
2015, respectively (IMO, 2008). Additionally, a fuel sulfur limit of 0.1 % applies for ships at berth in all European harbours since 2010 (EU,
2005), and a limit of 1.5 % applies for all passenger ships in regular line traffic in
European waters outside the SECA (EU, 2012). To face the rising <inline-formula><mml:math id="M21" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
emissions, the IMO has designated the North Sea and Baltic Sea <inline-formula><mml:math id="M22" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
Emission Control Areas (NECAs) starting from 1 January 2021 onwards (IMO,
2017). The NECA regulation applies to all vessels built after 2021 and
requires approx. 80 % <inline-formula><mml:math id="M23" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emission reductions (IMO, 2014). Due to
the long lifetime of ships, it will take at least 30 years until the entire
ship fleet is renewed, which means that <inline-formula><mml:math id="M24" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions will only
decrease gradually. In combination with the increasing ship traffic, which
grows by roughly 2 % per year, and the future foreseeable significant
decrease in emissions from other anthropogenic sectors (e.g. traffic,
heating), the relative importance of <inline-formula><mml:math id="M25" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions from shipping for
urban air quality will thus likely remain high.</p>
      <p id="d1e444">To control emissions of greenhouse gases IMO has adopted a package of
technical measures including the Energy Efficiency Design Index (EEDI). The
EEDI regulation entered into force in 2013 and included requirements on
minimum mandatory energy efficiency performance levels, increasing over time
through different phases (IMO, 2011). In 2018 IMO adopted a resolution on
the “Initial IMO Strategy on reduction in GHG emissions from ships” stating
the objective to reduce the total annual greenhouse gas (GHG) emissions from international
shipping by at least 50 % by 2050 compared to 2008 (IMO, 2018). Reaching
this objective implies both efficiency gains and an increased use of
renewable fuels. There is still a great potential for efficiency gains
through better ship and engine design and through operational measures,
mainly lower speeds. State of the art ships can be almost 50 % more
efficient than ships that are 10–20 years old. Biofuels, wind power, and
electrification could play an important part in closing the gap between the
potential of an improved engine design together with operational measures
and the 50 % target for the entire sector, which, on the other hand, is
expected to continue to grow in terms of transported volume in the upcoming
decades.</p>
      <p id="d1e447">An important effect of the emission reductions in <inline-formula><mml:math id="M26" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M27" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is
the resulting reduction in atmospheric concentrations of PM, especially secondary particulate sulfate and nitrate. Sofiev et al. (2018) have shown that the global limit on sulfur content in ship fuels
decreases concentrations of particulate sulfate by 2–4 <inline-formula><mml:math id="M28" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M29" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the vicinity of busy ship lanes on a global scale,
leading to significant reductions in PM<inline-formula><mml:math id="M30" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> (particles with a diameter
of less than 2.5 <inline-formula><mml:math id="M31" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>m). The burden of PM<inline-formula><mml:math id="M32" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> over the Baltic Sea
region is predicted to decrease by 35 %–37 % between 2012 and 2040 as
a result of the regulation of <inline-formula><mml:math id="M33" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M34" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions and due to energy
savings in shipping (Karl et al., 2019a). Importantly, the atmospheric
transformation of <inline-formula><mml:math id="M35" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emitted from shipping is also relevant for ozone
(<inline-formula><mml:math id="M36" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) formation (Eyring et al., 2010). The introduction of a NECA is
thus critical for reducing concentrations of <inline-formula><mml:math id="M37" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M38" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and
PM<inline-formula><mml:math id="M39" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> at the same time.</p>
      <p id="d1e595">In this study we investigate impacts of shipping on urban air quality and
the associated health of the population in several future scenarios. We
combine the development of emissions due to the implementation of the IMO
rules on air pollutants and energy efficiency with changes in traffic
volumes, fleet composition, and fuel types used. In addition, the impact of a
wide use of shoreside electricity by ships at berth is investigated. Only
few studies considering impacts of shipping in future scenarios specifically
relevant for the Baltic Sea region can be found in the literature (Cofala et
al., 2018; Karl et al., 2019b, 2019a; Jonson et al., 2019, 2015). However, the abatement measures considered as well as
the methods used differ from our approach. The first part of our study (Tang
et al., 2020) gives a brief overview of previous studies about the impacts of
shipping emissions on air quality and health on the Swedish west coast. It
provides discussion on how the legislation changed between the base year
used in our study (2012) and the situation today. Also, different methods of
health impact assessment used in these studies are briefly reviewed. In Tang
et al. (2020) we discuss that shipping in Gothenburg in 2012 was a
significant source of air pollution, contributing 35 % and 12.5 %
to the annual exposure to <inline-formula><mml:math id="M40" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M41" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, respectively, and that
the regional shipping outside the city was responsible for 20 % and 10 % of the <inline-formula><mml:math id="M42" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M43" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure, contributing more than the
local shipping in and around the harbours. According to the study of Karl et al. (2019a), the introduction of the SECA with a fuel sulfur limit of 0.1 % decreased the exposure to PM<inline-formula><mml:math id="M44" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> on the Swedish west coast by
approximately 35 %. This can be seen as the regional part of the shipping
contribution because the maximum fuel sulfur content for ships at berth
was limited to 0.1 % already in 2010. Sofiev et al. (2018) assessed
the impact of the currently introduced global 0.5 % fuel sulfur content
(FSC) limit on a global scale in terms of health benefits and found that the
introduction of the global 0.5 % FSC cap in 2020 leads to an avoidance of
<inline-formula><mml:math id="M45" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">2000</mml:mn></mml:mrow></mml:math></inline-formula> (5 % of cases due to shipping without the 0.5 %
cap) premature deaths annually in Europe and <inline-formula><mml:math id="M46" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">137</mml:mn></mml:mrow></mml:math></inline-formula> 000 (38 % of cases) globally. The impact on the west coast of Sweden was,
however, found to be very small because the North and Baltic seas have been SECAs
with a maximum FSC of 0.1 % since 2015.</p>
      <p id="d1e669">Cofala et al. (2018) assessed impacts of the implementation of emission
control areas for <inline-formula><mml:math id="M47" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M48" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in all European seas in several
alternative scenarios studying the years 2030, 2040, and 2050 and also provided cost–benefit analyses for these different alternatives. Different
options of<?pagebreak page10669?> emission control areas in southern Europe had very limited impact
in northern Europe; the study, however, also considered two different base
scenarios, one of them including climate policy options for shipping.
A comparison of the data supplement in Cofala et al. (2018) shows that the
PM<inline-formula><mml:math id="M49" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>-related mortalities caused by shipping decreased in the “climate
measures” scenario compared to the “no-climate-measures” scenario. The decrease was 0.8 %
and 2 % (4 and 13 cases) in 2030 and 2050, respectively, in Sweden and 1 % and 3.7 % (3000 and 12 000 cases) in all of Europe. Cofala et al. (2018) also show the overall impact of shipping on the urban scale for the
model grid cells including Mediterranean harbours. In the scenario without
climate measures in 2030 the shipping contributions to annual mean
PM<inline-formula><mml:math id="M50" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> concentrations vary from <inline-formula><mml:math id="M51" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">0.2</mml:mn></mml:mrow></mml:math></inline-formula> to 2 <inline-formula><mml:math id="M52" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M53" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, while an introduction of additional SECA and NECA rules as in the
North and Baltic seas has the potential to avoid approximately 50 % of
PM<inline-formula><mml:math id="M54" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>. In 2050 the shipping contributions to PM<inline-formula><mml:math id="M55" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> were higher,
with concentrations of up to 3 <inline-formula><mml:math id="M56" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M57" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The reduction potential of the SECA plus NECA introduction is about 65 %. This is more than in 2030
because the NECA effects move forward at a slow pace.</p>
      <p id="d1e781">The health benefit of cleaner ship fuels and other emission reduction
techniques in densely populated harbour cities is estimated to be much
greater than on the open sea. In order to quantify the future impact of
shipping, scenarios for transported cargo volumes, composition of the fleet,
and energy efficiency improvements need to be developed and put into
perspective with probable emission reductions on land.</p>
      <p id="d1e784">The goal of the present study is to investigate the future effect of
shipping emissions on air quality and related health effects considering the
development of shipping under current regional trends of economic growth and
already decided regulations in the Gothenburg urban area in 2040.
Additionally, we investigate the impact of a large-scale implementation of
shore electricity in the Port of Gothenburg. For this purpose, we
established a one-way nested chemistry transport modelling (CTM) system from
the global to the urban scale. This paper is the second part of a study
about the current and future air quality situation in the Gothenburg urban
area. Part 1 by Tang et al. (2020) is published in the same special issue.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Chemistry transport and health-effect modelling</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>The city of Gothenburg</title>
      <p id="d1e802">The city of Gothenburg (Fig. 1) is located on the western coast of Sweden,
with about 0.57 million inhabitants and an area of 450 km<inline-formula><mml:math id="M58" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>.
The dominant wind direction in Gothenburg is south-west with an average wind
speed of 3.5 m s<inline-formula><mml:math id="M59" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, indicating the major transport path from the sea to the
land, especially in summer. The geomorphology of the Gothenburg area is
described as a fissure valley landscape dominated by a few large valleys in
north–south and east–west directions. The major air pollution sources in
Gothenburg are above all road traffic and industry, wood burning, shipping,
agriculture, working machines, and long-range transport (LRT) from the
European continent and other parts of Sweden. The harbour and shipping
activities are important emission sources and directly influence the urban
air quality. The centre of the city is situated on the southern shore of the
Göta älv. The Port of Gothenburg receives between 6000 and
6500 calls per year and an additional 600–700 ships pass to and from ports
upstream and on the Göta älv. The port annually handles
approximately 900 000 containers, <inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:mn mathvariant="normal">20</mml:mn><mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> t  of petroleum, and half a
million roll-on/roll-off (RoRo) units (Fridell et al., 2015). Passenger
traffic in Gothenburg is also very busy with 1.5 million passengers who
ferry to and from Gothenburg to Denmark, Germany, etc., on Stena Line ferries
each year. This makes the port the largest cargo port in Scandinavia. Annual
analyses of air quality monitoring data by the Environmental Administration of City
of Gothenburg show exceedances of both the target and the limit values for
<inline-formula><mml:math id="M61" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> at several stations in Gothenburg in 2012 with decreasing trends
towards exceedances of only the limit value at traffic stations in 2019. For
PM<inline-formula><mml:math id="M62" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> the levels were well below the limit value but exceeded the
target value in 2012 without any significant trend towards the present with
exception of the urban background, where a slightly decreasing trend was
observed and the annual mean was below the target value of 15 <inline-formula><mml:math id="M63" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M64" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the last 4 years. The measured concentration levels of
PM<inline-formula><mml:math id="M65" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> have been below the target value without any significant trend at
Gothenburg monitoring stations. Concentrations of ozone have a slightly
increasing trend from the year 2012 onwards and tend to exceed the limit values
for maximum hourly and 8 h means on a number of occasions each year
(Miljöförvaltningen, 2019).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><?xmltex \currentcnt{1}?><label>Figure 1</label><caption><p id="d1e891">The Gothenburg research domain. The light red grid indicates the
domain extent and the horizontal grid-cell size of 250 m. Red areas indicate
port areas and grey lines indicates the city boundaries as given by the
Copernicus Urban Atlas 2012 dataset. Maps are created with ArcGIS with the underlying basemap sources Esri, HERE, Garmin, GEBCO, National Geographic,
NOAA, and GIS User Community.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f01.png"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Global- to urban-scale CTM system setup</title>
      <p id="d1e908">For the urban-scale, the prognostic meteorology dispersion model TAPM (The
Air Pollution Model; Hurley et al., 2005) was used as part of a one-way
nested CTM system from the global to the
urban scale (Fig. 2). TAPM has been successfully applied to investigate
urban air quality and scenarios in coastal urban areas all over the world
(e.g. Matthaios et al., 2018; Ramacher et al., 2020; Gallego et al., 2016;
Fridell et al., 2014). TAPM consists of a meteorological component and an air
quality component. The meteorological component of TAPM is an
incompressible, non-hydrostatic, primitive equation model with a
terrain-following vertical sigma coordinate system for 3-D simulations. In
the meteorological component, it is possible to assimilate wind observations
to add a nudging term to the horizontal momentum equations. The air
pollution component uses data from the meteorological component and consists
of three modules: first, the Eulerian grid module solves prognostic
equations for mean and variance of concentrations; second, the Lagrangian
particle<?pagebreak page10670?> module can be used to represent near-source dispersion more
accurately; and third, the plume rise module is used to account for plume
momentum and buoyancy effects for point sources. The model also includes
gas-phase reactions based on a generic reaction set (Azzi et al., 1984) to
represent the basic photochemical cycle of <inline-formula><mml:math id="M66" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, NO, and <inline-formula><mml:math id="M67" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, gas- and aqueous-phase chemical reactions for sulfur dioxide and particles, and a dust mode for total suspended particles (PM<inline-formula><mml:math id="M68" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, PM<inline-formula><mml:math id="M69" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula>, PM<inline-formula><mml:math id="M70" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">20</mml:mn></mml:msub></mml:math></inline-formula>, and PM<inline-formula><mml:math id="M71" display="inline"><mml:mrow><mml:msub><mml:mi/><mml:mn mathvariant="normal">30</mml:mn></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. Wet and dry deposition effects are also included.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><?xmltex \currentcnt{2}?><label>Figure 2</label><caption><p id="d1e975">Study design to calculate future concentrations, population
exposure, and health effects.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f02.png"/>

        </fig>

<sec id="Ch1.S2.SS2.SSS1">
  <label>2.2.1</label><title>Boundary conditions</title>
      <p id="d1e991">For the Gothenburg urban area, we coupled TAPM offline to regional CTM
simulations with the Community Multi-scale Air Quality (CMAQ) model v5.0.1 (Byun and Schere, 2006) as performed
by Karl et al. (2019a) for the Baltic Sea region in 2012. Karl et al. (2019a) used global hemispheric pollutant concentrations from APTA global
reanalysis (Sofiev et al., 2018) to consider global chemical boundaries and
accounted for meteorological conditions with meteorological fields
calculated for the Consortium for Small-scale Modelling
(COSMO) Climate Limited-area Modelling Community
(CLM) mesoscale meteorological model version 5.0
(Rockel et al., 2008) for the year 2012 using the ERA-Interim reanalysis as
forcing data (Geyer, 2014). Furthermore, they accounted for regional
land-based emissions in 2012, represented by hourly gridded emissions of
<inline-formula><mml:math id="M72" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, sulfur oxides, carbon monoxide (CO), <inline-formula><mml:math id="M73" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NH</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M74" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, coarse
PM, and non-methane volatile organic compounds (NMVOCs) with the Sparse Matrix
Operator Kernel Emissions for Europe model (SMOKE-EU; Bieser et al., 2011).
Regional Shipping emissions for the Baltic Sea and North Sea with high
spatial and temporal resolution were obtained from the Ship Traffic Emission
Assessment Model (STEAM; Jalkanen et al., 2009; Jalkanen et al., 2012;
Johansson et al., 2013). Fridell et al. (2015) also accounted for future
emission conditions with future scenarios for land-based and shipping
emissions in the Baltic Sea in 2040 which are consistent with the scenarios
used in this study. Details of the regional air quality simulation setup
including shipping emissions, the evaluations of simulated pollutant
concentrations in 2012, and results for the year 2040 scenarios in the
Baltic Sea region are described in Karl et al. (2019a).</p>
      <p id="d1e1025">These simulations are used to interpolate chemical boundary conditions for
TAPM. Concentrations simulated with CMAQ for the vertical model layer 7 with
a mid-layer height of approximately 385 m above ground are used for this
purpose. Since TAPM allows only one single boundary concentration value for
the entire urban domain, these values are calculated every hour using
horizontal wind components on each of the four lateral boundaries to give
more weight to the concentrations upwind of the urban domain (Fridell et al.,
2014). CMAQ simulations with and without ship emissions for 2012 and 2040 in
the Baltic Sea and the North Sea were used as boundary conditions in the
respective TAPM simulation runs with and without ship emissions for 2012 and
2040. This procedure allows for an analysis of regional influences on the
Gothenburg area.</p><?xmltex \hack{\newpage}?>
</sec>
<?pagebreak page10671?><sec id="Ch1.S2.SS2.SSS2">
  <label>2.2.2</label><title>Meteorological fields</title>
      <p id="d1e1038">The spatial resolution of the urban domain for the TAPM air pollution
component is <inline-formula><mml:math id="M75" display="inline"><mml:mrow><mml:mn mathvariant="normal">250</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">250</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula>. With an extent of <inline-formula><mml:math id="M76" display="inline"><mml:mrow><mml:mn mathvariant="normal">25</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">25</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula> this domain covers the city of Gothenburg and the harbour area along the shores of the
Göta river running through the city. The urban domain for the TAPM air
pollution component is nested in <inline-formula><mml:math id="M77" display="inline"><mml:mrow><mml:mn mathvariant="normal">30</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">30</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula> (500 m horizontal resolution)
hourly meteorological fields taken from the innermost domain of nested
simulations with the meteorological component of TAPM. We chose a smaller
domain for the TAPM air pollution component because of a higher efficiency
in computing time while having all important city features covered.</p>
      <p id="d1e1101">TAPM includes a nested approach for meteorology, which allows us to zoom-in to
a local region of interest, while the outer boundaries of the grid are
driven by synoptic-scale analyses. We applied the meteorological component
with four nested domains from a <inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:mn mathvariant="normal">480</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">480</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> extent at the
outer domain (D1) to a <inline-formula><mml:math id="M79" display="inline"><mml:mrow><mml:mn mathvariant="normal">30</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">30</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> extent at the inner domain
(D4). The outer domain (D1) was forced by ECMWF ERA5 synoptic meteorological
reanalyses ensemble means with 30 vertical layers, and <inline-formula><mml:math id="M80" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.3</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">0.3</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> horizontal and 3-hourly temporal resolution.
Additionally, hourly local wind fields of four measurement stations (Femman,
Gothenburg, Landvetter, Vinga) operated by the Swedish Meteorological and
Hydrological Institute (SMHI) have been assimilated in the meteorological
component to force the meteorological fields to be closer to the
measurements. Since this study focuses on the impact of changes in shipping
emissions in 2040 and not on meteorological effects, the 2040 simulations
also use 2012 meteorological fields. Details on meteorological and chemical
component configurations in TAPM as well as air quality results and their
evaluation for 2012 can be found in the accompanying paper by Tang et al. (2020). Based on the temperature anomalies and precipitation anomalies for
the decade 2004–2014 for the Baltic Proper, the year 2012 was chosen as the
meteorological reference year for the CTM simulations in Part I of the
Gothenburg study as well as in regional studies for current (2012) and
future (2040) conditions and shipping scenarios (Karl et al., 2019b; Tang et
al., 2020).</p>
</sec>
<sec id="Ch1.S2.SS2.SSS3">
  <label>2.2.3</label><title>Current and future land-based emission inventories</title>
      <p id="d1e1170">A bottom–up emission inventory for the Gothenburg urban area has been
created to account for road traffic, industrial processes, and other sources
of land-based emissions in 2012. The road traffic emissions are calculated
with traffic activity data from the database of the Environmental
Administration, City of Gothenburg (Miljöförvatningen), and a set of
emission factors for the Swedish road vehicle fleet in 2035 (latest year
available) by HBEFA v. 3.2 (Hand Book of Emission Factors for Road
Transport; Keller et al., 2017). The traffic sources are treated as line
emission sources in TAPM. For the 10 biggest industrial sources, emission
fluxes assigned with coordinates and emission heights were obtained from the
Swedish Environmental Emission Data (SMED) for 2012 and modelled as area
sources in TAPM. The remaining sources, which are non-road activities, waste and
sewage, domestic heating, energy production, combustion in industry for
energy purposes, non-road working machinery, domestic aviation, and solvents
from product use and agriculture, are gathered from the SMED gridded
inventory. They are geographically distributed on a <inline-formula><mml:math id="M81" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula> grid and
modelled as gridded area sources. The land-based emission inventory created
in this way takes into account all relevant emission sources for <inline-formula><mml:math id="M82" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>,
<inline-formula><mml:math id="M83" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M84" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula>, PM<inline-formula><mml:math id="M85" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and volatile organic compounds (VOCs) in 2012. For land-based emissions
in 2040, the 2012 emission inventory was scaled to 2040 conditions using
source-specific approaches. The road traffic emission inventory in 2040 uses
detailed activity data for 2012 scaled with a traffic volume development
scenario in Sweden specific for light- and heavy-duty vehicles and busses
(Transport administration, 2016, 2018). Combined with emission factors,
which were calculated for the expected Swedish car fleet in 2035 using the HBEFA
v.3.2 database (the year 2040 was not available), a road traffic emission
inventory for 2040 was calculated. The annual road traffic emissions in 2040
are 265 t <inline-formula><mml:math id="M86" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M87" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 193 t VOC yr<inline-formula><mml:math id="M88" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and 141 t PM<inline-formula><mml:math id="M89" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M90" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and thus about 89 %, 62 %, and 12 % lower than in 2012 in the Gothenburg area (Fig. 2).</p>
      <p id="d1e1290">The area emissions, covering all emission sectors except road traffic and
shipping, are scaled from 2012 to 2040 with factors which describe the
change in Swedish emissions between 2010 and 2040. These factors were
calculated with emissions obtained from the Greenhouse Gas – Air Pollution
Interactions and Synergies (GAINS) model using the emission scenario
ECLIPSE_V5a_CLE_base
(Kiesewetter et al., 2014) and can be found in Supplement 1. The scenario
emissions for the time period 2000–2040 were provided as national
emissions for European countries, including Sweden, specified for GAINS
emission sector categories by Zbigniew Klimont, IIASA (personal
communication, 3 March 2016). These categories were translated into the emission
categories of Swedish Environmental Emission Data (SMED), and the 2040/2010
factors were applied to the 2012 area emission sectors to derive a
land-based emissions scenario for 2040 (CLE2040). The year 2012 is not
available for ECLIPSE_V5a_CLE_base, but the change between 2010 and 2012 is small on the 30-year horizon.
Based on these factors, the annual industrial emissions in 2040 are 468 t <inline-formula><mml:math id="M91" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M92" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 9958 t VOC yr<inline-formula><mml:math id="M93" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 85 t PM<inline-formula><mml:math id="M94" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M95" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and 189 t <inline-formula><mml:math id="M96" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M97" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and thus about 19 % lower, 45 % higher, 7 % lower, and 2 % lower than in
2012 in the Gothenburg area (Fig. 2). The reason for an increase in VOC
emissions in the future is a scaling factor of 1.45 for the sector
“Combustion in industry for energy purposes”, which 6 out of 10
industrial sources in the Gothenburg area belong to. As part of the CTM
chain, the treatment of area emissions for the<?pagebreak page10672?> urban area of Gothenburg is
consistent with the method used in the regional-scale CMAQ simulations.
Thus, the boundary conditions in the local TAPM runs were taken from
corresponding regional-scale simulations of the CMAQ model with consistently
derived emissions for 2012 and 2040 (Karl et al., 2019a).</p>
</sec>
</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><title>Exposure and health impact assessment</title>
      <p id="d1e1382">The impacts of exposure to air pollutants on the health of people living in
the Gothenburg region were assessed with the ALPHA-RiskPoll model (ARP;
Holland et al., 2013), which calculates a wide range of air-pollutant-specific health effects in the assessed year. The RAINS methodology, which
calculates years of life lost over the expected lifetime of a population
(Amman et al., 2004), has been used as well to enable a comparison with other
studies. Both methods are based on national population statistics for
European countries and on a forecast of the age distribution of the
population, as well as mortality and morbidity data for 2040. In addition,
effect-specific dose–response relationships are taken into account. In the case
of the RAINS methodology only all-cause mortality from PM<inline-formula><mml:math id="M98" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure
has been considered. In the ARP analysis, impacts of exposure to PM<inline-formula><mml:math id="M99" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>,
ozone, and <inline-formula><mml:math id="M100" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> have been considered (Heroux et al., 2013). Only the most
serious impacts, i.e. losses of lives, are presented, taking into account
impacts of chronic exposure to PM<inline-formula><mml:math id="M101" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, short-term exposure to ozone, and short-term exposure to <inline-formula><mml:math id="M102" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, i.e. the impacts marked A* in the
HRAPIE (Health risks of air pollution in Europe) study (Heroux et al.,
2013). For ozone, the indicator SOMO35 is used, standing for the annual sum
of the daily maximum of the 8 h mean ozone concentrations above a
threshold of 35 ppb. The health impacts of some pollutants are correlated,
and that is why the premature deaths attributed to each pollutant cannot
simply be added up. The concentration-response functions (CRFs) for all-cause
mortality used in ARP are those from the WHO (Heroux et al., 2013): 6.2 % (95 % confidence interval 4.0 %–8.3 %) relative risk increase per 10 <inline-formula><mml:math id="M103" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M104" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> increased exposure for the long-term PM<inline-formula><mml:math id="M105" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure,
0.29 % (95 % confidence interval 0.14 %–0.43 %) relative risk
increase per 10 <inline-formula><mml:math id="M106" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M107" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> increased exposure for the short-term
ozone exposure, and 0.27 % (95 % confidence interval 0.16 %–0.38 %) relative risk increase per 10 <inline-formula><mml:math id="M108" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M109" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> increased exposure for
the short-term <inline-formula><mml:math id="M110" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> exposure. The RAINS methodology uses 5.8 %
relative risk increase per 10 <inline-formula><mml:math id="M111" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M112" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> increased exposure to
PM<inline-formula><mml:math id="M113" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>. The health impacts of some pollutants are correlated, and that is
why the premature deaths attributed to each pollutant cannot simply be added
up. In particular, it has been estimated that adding premature deaths
attributed to PM<inline-formula><mml:math id="M114" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> to those attributed to <inline-formula><mml:math id="M115" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> could result in
double counting of around 30 % (Heroux et al., 2013). More details on the
methodology can be found in Part 1 of these papers (Tang et al., 2020).</p>
      <p id="d1e1566">The exposure calculation was based on the concentration fields of
PM<inline-formula><mml:math id="M116" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, <inline-formula><mml:math id="M117" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M118" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> calculated for the examined future
scenarios by the modelling system described above. Annual means and SOMO35
were calculated from hourly ozone concentration fields. Population data at
a <inline-formula><mml:math id="M119" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula> resolution were obtained from Statistics Sweden (SCB) for
2015, with a population of 572 779 in the city of Gothenburg, and used for
calculating the population-weighted average concentrations (PWCs) for the
model domain in 2012 (Tang et al., 2020). For the 2040 scenarios the PWCs
were calculated using the same population data for 2015 since a
geographically resolved prognosis for 2040 was not available. In ARP the
PWCs are applied to the population statistics for Sweden for the year 2040
and scaled to the population of Gothenburg with the help of the year 2012
“Gothenburg population”<inline-formula><mml:math id="M120" display="inline"><mml:mo>/</mml:mo></mml:math></inline-formula>“total Swedish population” ratio. This approach
neglects any potential trend of increase in urbanization in the country, which would lead to higher impacts than calculated with our approach.</p>
      <p id="d1e1627">With the introduced study design, it is possible to estimate the impact of
shipping-related air pollution on the health of citizens in the Gothenburg
area regarding current and future emission scenarios and to identify the
effectiveness of several air pollution abatement measures. For this purpose,
it is necessary to create a set of scenarios with emphasis on shipping
activities in the future, translate them into emission inventories, and
simulate the health effects with the introduced CTM–exposure–health-effect
modelling system.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Current and future shipping emissions scenarios</title>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>Ship emission inventories for the Gothenburg area</title>
      <p id="d1e1646">A shipping emission inventory for the area of Gothenburg with high temporal
and spatial resolution was calculated with STEAM for the year 2012,
representing the present situation (Tang et al., 2020) and giving a baseline
to be compared with future scenarios. In STEAM, position data of individual
ships taken from reports from the Automatic Identification System (AIS) is
used to model fuel consumption and emissions as a function of vessel
activity, engine, and fuel type. The calculation of ship emission inventories
for the Gothenburg area follows the approach that has been applied for the
North and Baltic Sea region and which is described in Karl et al. (2019a). The
emission inventory in this work is therefore consistent with the one in Karl
et al. (2019a). Nevertheless, the regional shipping emission inventory
contains hourly updated emission data on a <inline-formula><mml:math id="M121" display="inline"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">2</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula> grid, while
the local emission inventory comes with a resolution of <inline-formula><mml:math id="M122" display="inline"><mml:mrow><mml:mn mathvariant="normal">250</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">250</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula> for the local research domain. The ship emissions in the Gothenburg area
include combustion emissions from all ship engines (boilers, auxiliary, and
main engines) for the compounds <inline-formula><mml:math id="M123" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M124" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, CO, <inline-formula><mml:math id="M125" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, NMHC, and
PM. Tang et al. (2020) used STEAM shipping emission inventory in<?pagebreak page10673?> the
Gothenburg area and applied it in the presented global-to-local CTM system
to identify the impact of shipping on urban air quality in the year 2012. In
2012, the local ship emissions in Gothenburg hold with 308 t <inline-formula><mml:math id="M126" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M127" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 2089 t <inline-formula><mml:math id="M128" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M129" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 91 t PM<inline-formula><mml:math id="M130" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M131" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and 23 t VOC yr<inline-formula><mml:math id="M132" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for
about 60 % of <inline-formula><mml:math id="M133" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, 40 % of <inline-formula><mml:math id="M134" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, 25 % of PM<inline-formula><mml:math id="M135" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula>, and 1 % of VOC, respectively, to the total emission situation (Fig. 3). Thus,
shipping emissions are a major contributor to the urban air quality in
Gothenburg in 2012.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><?xmltex \currentcnt{3}?><label>Figure 3</label><caption><p id="d1e1836">Present-day and future 2040BAU scenario emission
inventories for the local CTM simulation in Gothenburg.</p></caption>
          <?xmltex \igopts{width=369.885827pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f03.png"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Future scenarios for shipping emissions</title>
      <p id="d1e1853">The scenarios used in this work describe future developments of policy and
technology regarding energy efficiency and exhaust gas emissions from ships
in the North and Baltic Sea region as well as in the Port of Gothenburg all
taking the following into account:
<list list-type="bullet"><list-item>
      <p id="d1e1858">the development of ship traffic and transport volumes,</p></list-item><list-item>
      <p id="d1e1862">fleet development of different ship types,</p></list-item><list-item>
      <p id="d1e1866">changes in fuel mixture,</p></list-item><list-item>
      <p id="d1e1870">the use of abatement measures and other technologies that influence
emissions from shipping,</p></list-item><list-item>
      <p id="d1e1874">regulations influencing emissions and fuel consumption,</p></list-item><list-item>
      <p id="d1e1878">possible local port actions in Gothenburg, e.g. the use of shoreside
electricity for ships at berth.</p></list-item></list>
The scenarios were created in the BONUS SHEBA (Sustainable Shipping and Environment of the
Baltic Sea Region) project and are based on
literature reviews and expert and stakeholder consultations to assess
shipping in the future within different developments (Fridell et al., 2015;
Karl et al., 2019a). The ship traffic volumes are expected to continue to
grow with about 1 % per year on average (it varies with ship type); the
current trend of using larger vessels is expected to continue as well (Kalli
et al. (2013). The trends in cargo volumes, passenger numbers, and ship sizes
are described in detail in Fridell et al. (2015) and translated to emission
scenarios in Karl et al. (2019). The overall goal was to investigate changes
in impacts of shipping on the marine and terrestrial environment as well as
on human health in the Baltic Sea region. The scenario results have been
used to assess urban-scale impacts on air quality and human health in the
Gothenburg area and several other Baltic Sea harbour cities (Ramacher et
al., 2019). In this work shipping in the urban area of Gothenburg in the
future is modelled in four scenarios for 2040:
<list list-type="bullet"><list-item>
      <p id="d1e1884">BAU2040 – business as usual 2040, this scenario is the future reference
scenario including all currently adopted regulations including climate
measures with high energy improvements in energy efficiency (Kalli et al.,
2013) (still not achieving the IMO 2018 Initial Strategy to reduce <inline-formula><mml:math id="M136" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
emissions by 50 % relative to 2008 by the year 2050);</p></list-item><list-item>
      <p id="d1e1899">BAU2040LP – BAU2040 with additional implementation of shoreside
electricity;</p></list-item><list-item>
      <p id="d1e1903">EEDI2040 – as BAU2040, but fuel efficiency just follows the Energy Efficiency Design Index regulation of the IMO;</p></list-item><list-item>
      <p id="d1e1907">EEDI2040LP – EEDI2040 with additional implementation of shoreside
electricity.</p></list-item></list></p>
<sec id="Ch1.S3.SS2.SSS1">
  <label>3.2.1</label><title>Future reference scenario BAU2040</title>
      <p id="d1e1917">The BAU2040 scenario is based on current trends in shipping and takes into
account already decided policy measures (Table 1). This represents a
conservative development of shipping in line with the Shared Socioeconomic
Pathway (SSP) II “Middle of the Road” scenario (Zandersen et al., 2019),
which is developed for the climate community and adapted for shipping in the
Baltic Sea. The trends in shipping were analysed from AIS data from recent
years and combined with an analysis of the different shipping sectors to
obtain the development regarding transport work, ship size, ship speed, and
number of ships for different ship types as done for the regional scale by
Karl et al. (2019a). In combination with assumptions on ship age
distribution and upcoming regulations (Fridell et al., 2015), this allows
for the calculation of emissions to air. The following regulations affecting
emissions to air were applied in BAU2040 (Table 1).
<list list-type="order"><list-item>
      <p id="d1e1922">Sulfur regulation: the Baltic and North seas are SECAs, where the maximum allowed sulfur content in marine fuel was
lowered from 1 % to 0.1 % in 2015. For sea areas outside SECAs the
maximum fuel sulfur content is 0.5 % from 2020 onwards. For ships berthing in EU
ports the maximum allowed fuel sulfur content is 0.1 %; these
regulations directly influence the emissions of <inline-formula><mml:math id="M137" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and have a strong
impact on the PM emissions. These regulations are also applied in the
EEDI2040 scenarios.</p></list-item><list-item>
      <p id="d1e1937"><inline-formula><mml:math id="M138" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> regulation: <inline-formula><mml:math id="M139" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions from marine engines have been regulated
with Tier I for new ships since 2000 and Tier II since 2011. Tier III is
applied in <inline-formula><mml:math id="M140" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> Emission Control Areas for new ships operating in the
Baltic and North seas from 2021. These regulations are also applied in the
EEDI2040 scenarios.</p></list-item><list-item>
      <p id="d1e1973">Energy efficiency: the regulation by IMO regarding the EEDI (IMO, 2018) requires new ships to become gradually more
fuel-efficient. The improvements in energy efficiency, fuel use reductions
and emissions are assumed to be proportional.</p></list-item></list>
The BAU2040 scenario assumes a share of ships driven by liquefied natural
gas (LNG) of about 10 % in the ship fleet in 2040. This is modelled as a
fraction of new ships introduced each year that will use LNG since
retrofitting of existing ships from fuel oil to LNG is assumed less likely
due to high costs. Since LNG is used as a means to comply with the sulfur
and <inline-formula><mml:math id="M141" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> regulations, ship types that operate mainly within SECAs are
modelled as being more likely to use LNG. The BAU2040 scenario also assumes
that on average 20 % of the ships in the Baltic Sea use scrubbers. This
measure, however, does not affect emissions to air in our study since the
scrubbers are required to reach <inline-formula><mml:math id="M142" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions equivalent to using magnesium oxide (MGO) and
that the PM emissions are similar as for MGO (Fridell and Salo, 2016). The
energy efficiency for new ships in BAU2040 is assumed to improve further
than what is required from the EEDI regulation, following recent trends and
assumptions from Kalli et al. (2013), assuming annual efficiency increases
of 1.3 % to 2.25 %, depending on ship type (corresponding efficiency
increase values required by the IMO EEDI regulation are 0.65 % to 1.04 %), which significantly reduces shipping fuel consumption.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e2002">Major regulation changes for the different scenarios.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="8">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="left"/>
     <oasis:colspec colnum="6" colname="col6" align="left"/>
     <oasis:colspec colnum="7" colname="col7" align="right"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">FSC in</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M143" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M144" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">FSC in</oasis:entry>
         <oasis:entry colname="col3">FSC in</oasis:entry>
         <oasis:entry colname="col4">Gothenburg</oasis:entry>
         <oasis:entry colname="col5">regulation</oasis:entry>
         <oasis:entry colname="col6">regulation in</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Scenario</oasis:entry>
         <oasis:entry colname="col2">global</oasis:entry>
         <oasis:entry colname="col3">SECA area</oasis:entry>
         <oasis:entry colname="col4">area</oasis:entry>
         <oasis:entry colname="col5">in NECA</oasis:entry>
         <oasis:entry colname="col6">Gothenburg area</oasis:entry>
         <oasis:entry colname="col7">LNG</oasis:entry>
         <oasis:entry colname="col8">Scrubbers</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">2012 reference</oasis:entry>
         <oasis:entry colname="col2">3.5 %</oasis:entry>
         <oasis:entry colname="col3">1.0 %</oasis:entry>
         <oasis:entry colname="col4">0.1 %</oasis:entry>
         <oasis:entry colname="col5">Tier II standard</oasis:entry>
         <oasis:entry colname="col6">Tier II standard</oasis:entry>
         <oasis:entry colname="col7">–</oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2040 scenarios</oasis:entry>
         <oasis:entry colname="col2">0.5 %</oasis:entry>
         <oasis:entry colname="col3">0.1 %</oasis:entry>
         <oasis:entry colname="col4">0.1 %</oasis:entry>
         <oasis:entry colname="col5">Tier III standard</oasis:entry>
         <oasis:entry colname="col6">Tier III standard</oasis:entry>
         <oasis:entry colname="col7">10 %</oasis:entry>
         <oasis:entry colname="col8">20 %</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d1e2183">Based on these assumptions scaling factors for 2040/2012 were calculated by
applying fleet development, fuel mix, abatement technology implementation,
and improvements in energy efficiency trends to fleet composition in the
Gothenburg area calculated with STEAM for the year 2012. These have been
applied to the 2012 gridded shipping emissions inventory to calculate the
BAU2040 emission scenario. Compared to the present situation in 2012, the
annual shipping emissions in BAU2040 are decreased to 466 t <inline-formula><mml:math id="M145" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M146" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M147" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">78</mml:mn></mml:mrow></mml:math></inline-formula> %), 23 t VOC yr<inline-formula><mml:math id="M148" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M149" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">31</mml:mn></mml:mrow></mml:math></inline-formula> %), 91 t PM<inline-formula><mml:math id="M150" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M151" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M152" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">85</mml:mn></mml:mrow></mml:math></inline-formula> %), 27 t <inline-formula><mml:math id="M153" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M154" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">91</mml:mn></mml:mrow></mml:math></inline-formula> %) (Fig. 4). While the shipping emissions in 2012
were a major contributor to the overall air pollution (Fig. 3), in 2040
the relevance of shipping emissions decreases in comparison to industry,
road traffic, and other sources to 19 % for <inline-formula><mml:math id="M156" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, 1 % for VOC, and 2 % for PM<inline-formula><mml:math id="M157" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M158" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
</sec>
<?pagebreak page10674?><sec id="Ch1.S3.SS2.SSS2">
  <label>3.2.2</label><title>Future scenario EEDI2040</title>
      <p id="d1e2346">As the scenario work revealed that energy effectivization has large impact
on emissions in the target year, encompassing at the same time great
uncertainty, we have chosen to include an alternative scenario with
a different effectivization level. In the EEDI2040 scenario, improvements in
fuel efficiency strictly follow the requirements of the EEDI regulation of the International Maritime
Organization. Annual efficiency increases of 0.65 % to 1.04 %,
depending on ship type, are assumed in the EEDI2040 scenario, while the
corresponding values in the BAU2040 scenario are 1.3 % to 2.25 %. From
the difference between BAU2040 and EEDI2040, the effect of the higher fuel
efficiency increase than required by the EEDI regulation can be deduced.</p>
      <p id="d1e2349">Based on these assumptions, scaling factors have been calculated in the same
manner as for the BAU2040 scenario and applied to the 2012 shipping
emissions inventory. Compared to the present situation in 2012, the annual
shipping emissions in EEDI2040 are decreased to 666 t <inline-formula><mml:math id="M159" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M160" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">68</mml:mn></mml:mrow></mml:math></inline-formula> %),
22 t VOC yr<inline-formula><mml:math id="M162" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula> %), 19 t PM<inline-formula><mml:math id="M164" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M165" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">79</mml:mn></mml:mrow></mml:math></inline-formula> %), and 38 t <inline-formula><mml:math id="M167" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M168" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">88</mml:mn></mml:mrow></mml:math></inline-formula> %) (Fig. 4). In comparison to 2012, the relevance of shipping
emissions in the EEDI2040 scenario decreases in comparison to industry, road
traffic, and other sources to 26 % for <inline-formula><mml:math id="M170" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, 1 % for VOC, and 3 %
for PM<inline-formula><mml:math id="M171" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M172" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
</sec>
<?pagebreak page10675?><sec id="Ch1.S3.SS2.SSS3">
  <label>3.2.3</label><title>Future shoreside electricity scenarios – BAU2040LP and EEDI2040LP</title>
      <p id="d1e2512">In addition to regional developments and regulations, which are reflected in
the BAU2040 and EEDI2040 scenarios, large-scale implementation of shoreside
electricity (or land power, LP) in the Port of Gothenburg was studied in
both scenarios. Concerns about air quality in port cities as well as
policies on greenhouse gas emissions have led to measures aimed at reducing
the use of auxiliary engines by ships at berth and thereby reducing
emissions of air pollutants and greenhouse gases as well as noise through
the use of shoreside electricity.</p>
      <p id="d1e2515">A gridded emission inventory with large-scale shoreside electricity use in
2040 was calculated with STEAM in the following way: all RoRo, RoPax, and
cruise ships and 50 % of all other ships use shoreside electricity.
Scaling factors have been calculated in the same way as for the future
scenarios BAU2040 and EEDI2040, except that emission from ships at berth
were reduced as described. These factors were then applied in the gridded
emission inventories, resulting in 165 t <inline-formula><mml:math id="M173" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M174" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 5 t VOC yr<inline-formula><mml:math id="M175" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 5 t PM<inline-formula><mml:math id="M176" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M177" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and 17 t <inline-formula><mml:math id="M178" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M179" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> emissions in Gothenburg in the
BAU2040LP scenario (Fig. 4). The EEDI2040LP annual shipping emissions result
in 234 t <inline-formula><mml:math id="M180" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M181" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 7 t VOC yr<inline-formula><mml:math id="M182" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 7 t PM<inline-formula><mml:math id="M183" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M184" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and 24 t <inline-formula><mml:math id="M185" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> yr<inline-formula><mml:math id="M186" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.
Compared to the BAU2040 and EEDI2040 scenario, the annual emissions in both
the BAU2040LP and EEDI2040LP scenario are 65 % lower for <inline-formula><mml:math id="M187" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, 68 % lower for VOC, 62 % lower for PM<inline-formula><mml:math id="M188" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula>, and 37 % lower for
<inline-formula><mml:math id="M189" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. While the shipping emissions in 2012 have been a major contributor
to the overall air pollution (Fig. 3), in 2040 the relevance of shipping
emissions decreases in comparison to industry, road traffic, and other
sources to 19 % for <inline-formula><mml:math id="M190" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, 1 % for VOC, and 2 % for PM<inline-formula><mml:math id="M191" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> and
<inline-formula><mml:math id="M192" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the BAU2040LP scenario.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><?xmltex \currentcnt{4}?><label>Figure 4</label><caption><p id="d1e2743">Annual shipping emissions of <inline-formula><mml:math id="M193" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, VOC, PM<inline-formula><mml:math id="M194" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M195" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
for the local CTM simulation in Gothenburg for 2012, BAU2040, and BAU2040LP
emissions scenarios.</p></caption>
            <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f04.png"/>

          </fig>

</sec>
</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>Scenario setup</title>
      <p id="d1e2792">The introduced land-based (CLE2040) and shipping (BAU2040, BAU2040LP,
EEDI2040, and EEDI2040LP) emission inventories for 2040 have been applied in
the established global-to-local CTM system to identify
<list list-type="order"><list-item>
      <p id="d1e2797">the impact on air quality in Gothenburg through a change in total emissions from 2012 to 2040,</p></list-item><list-item>
      <p id="d1e2801">the impact of local shipping activities in 2040 in two different scenarios, and</p></list-item><list-item>
      <p id="d1e2805">the additional impact of local port measures (shoreside electricity) in scenarios for 2040.</p></list-item></list>
Moreover, simulations for all months in 2012 have been performed as
described in Tang et al. (2020). The meteorological conditions were held
constant for all regional and local CTM runs as our focus is on the impact
of changing emissions. The regional boundary conditions applied to the
local-scale TAPM simulations for the BAU2040LP and EEDI2040LP were taken
from regional CTM simulations with BAU2040 and EEDI2040 emissions including
shipping emissions (Table 2). By using the local land-based emissions in
line with the regional land-based emissions and varying the local shipping
emissions, this scenario setup allows for the assessment of local shipping
impacts in different local scenarios. To derive the contribution of ships to
the selected pollutant concentrations, two model runs for each scenario – one
including and one excluding local shipping emissions in TAPM simulations – were performed. The difference is regarded as the contribution of ships to
the individual pollutant. For the scenarios, the difference between two
model runs with different shipping emissions is regarded as the change in
the contribution of ships between the respective scenarios. In the
discussion of the results, the BAU2040 scenario will be discussed as the
future reference scenario. Consequently, we will show results for the
BAU2040 scenario in the main paper, while results for EEDI2040 are available
in Supplement 3.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T2" specific-use="star"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e2812">Meteorology, regional boundary conditions, and emissions
setup for the calculated scenarios.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:colspec colnum="5" colname="col5" align="left"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Scenario</oasis:entry>
         <oasis:entry colname="col2">Meteorology</oasis:entry>
         <oasis:entry colname="col3">Reg. boundary</oasis:entry>
         <oasis:entry rowsep="1" namest="col4" nameend="col5" align="center">Local emissions </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Land based</oasis:entry>
         <oasis:entry colname="col5">Shipping</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">2012 Reference</oasis:entry>
         <oasis:entry colname="col2">2012</oasis:entry>
         <oasis:entry colname="col3">2012 (incl. shipping)</oasis:entry>
         <oasis:entry colname="col4">2012</oasis:entry>
         <oasis:entry colname="col5">2012</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BAU2040</oasis:entry>
         <oasis:entry colname="col2">2012</oasis:entry>
         <oasis:entry colname="col3">BAU2040 (incl. shipping)</oasis:entry>
         <oasis:entry colname="col4">CLE2040</oasis:entry>
         <oasis:entry colname="col5">BAU2040</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BAU2040LP</oasis:entry>
         <oasis:entry colname="col2">2012</oasis:entry>
         <oasis:entry colname="col3">BAU2040 (incl. shipping)</oasis:entry>
         <oasis:entry colname="col4">CLE2040</oasis:entry>
         <oasis:entry colname="col5">BAU2040LP</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EEDI2040</oasis:entry>
         <oasis:entry colname="col2">2012</oasis:entry>
         <oasis:entry colname="col3">EEDI2040 (incl. shipping)</oasis:entry>
         <oasis:entry colname="col4">CLE2040</oasis:entry>
         <oasis:entry colname="col5">EEDI2040</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EEDI2040LP</oasis:entry>
         <oasis:entry colname="col2">2012</oasis:entry>
         <oasis:entry colname="col3">EEDI2040 (incl. shipping)</oasis:entry>
         <oasis:entry colname="col4">CLE2040</oasis:entry>
         <oasis:entry colname="col5">EEDI2040LP</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

</sec>
</sec>
<?pagebreak page10676?><sec id="Ch1.S4">
  <label>4</label><title>Future impact of shipping on concentrations of pollutants</title>
      <p id="d1e2966">BAU2040 serves as a reference scenario all other scenarios are compared to. It
was first compared to the present-day air quality situation in 2012, which
is discussed in detail in the accompanying paper by Tang et al. (2020). Ship
activities in Gothenburg 2012 contribute to peak values, in particularly in
the north of the city port and the river Göta due to the dominant SW
wind. The local shipping contribution to <inline-formula><mml:math id="M196" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in
Gothenburg was about 14 % (around 0.5 ppb) to the annual mean averaged
over the entire model domain. These contributions were higher in summer due
to higher ship activities. Emissions of <inline-formula><mml:math id="M197" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from ships added up with
land-based <inline-formula><mml:math id="M198" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions and enhanced the local ozone loss by NO
titration. The negative effect of <inline-formula><mml:math id="M199" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions from local shipping on
<inline-formula><mml:math id="M200" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in summer was <inline-formula><mml:math id="M201" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula> % (around <inline-formula><mml:math id="M202" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> ppb) on average.
For PM<inline-formula><mml:math id="M203" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, the local ship emissions contributed about 2 % (around
0.07 <inline-formula><mml:math id="M204" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M205" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> to the annual mean, while the annual average
<inline-formula><mml:math id="M206" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations from local shipping were the major contributor to
local <inline-formula><mml:math id="M207" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions with 0.2–0.5 ppb along major shipping lanes. In
the following, maps illustrating changes in annually averaged concentrations
of <inline-formula><mml:math id="M208" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M209" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M210" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M211" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> are shown for the total change
in ambient air concentrations from 2012 to 2040BAU (Fig. 5), the impact of
change in shipping emissions from 2012 to BAU2040 on shipping contribution
to ambient concentrations of these air pollutants (Fig. 6), and impact of a large-scale introduction of shoreside electricity in the
BAU2040LP and EEDI2040LP scenarios on the contribution of shipping compared
to BAU2040 and EEDI2040, respectively (Fig. 7 for BAU2040 results; Supplement 3 for EEDI2040 results). Seasonal plots for summer and winter
months can be found in Supplements 2 and 3.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5" specific-use="star"><?xmltex \currentcnt{5}?><label>Figure 5</label><caption><p id="d1e3144">The total modelled present-day concentration for <inline-formula><mml:math id="M212" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M213" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>,
PM<inline-formula><mml:math id="M214" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M215" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (column 1), as well as the concentration in BAU2040
(column 2) and the difference between the present day and BAU2040 in
absolute (column 3) and relative (column 4) values. ©OpenStreetMap
contributors 2019. Distributed under a Creative Commons BY-SA License.</p></caption>
        <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f05.png"/>

      </fig>

<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Air quality changes in 2040 compared to the present day</title>
      <p id="d1e3202">The local concentration of <inline-formula><mml:math id="M216" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, given as an annual average over the model
domain, decreased by 74 % (around 2.8 ppb) from about 3.7 ppb in 2012 to 0.9 ppb in the future reference scenario BAU2040. The highest changes in
<inline-formula><mml:math id="M217" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> are located in the centre of Gothenburg with an average <inline-formula><mml:math id="M218" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
reduction of up to 80 % (and 8 ppb) next to major roads. Besides the high
reductions due to road traffic, a reduction in <inline-formula><mml:math id="M219" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration due to
the reduction in emissions from industrial sources is visible in the western
part of the Gothenburg domain with reductions of up to 7 ppb
(<inline-formula><mml:math id="M220" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> %). The smaller relative reduction in industrial
areas is due to the comparatively low change in industrial <inline-formula><mml:math id="M221" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
emissions and their already high contribution to <inline-formula><mml:math id="M222" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration in
the western part of the city in 2012, on one side, and the high reduction in
road traffic emissions and a high density of highways and road traffic in
the eastern part of the Gothenburg domain, on the other side. The port area,
which is located westward of the centre, shows a comparably high reduction
potential with up to 70 %. The nearby industrial sources might hide
reductions in <inline-formula><mml:math id="M223" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> from other sources due to their high absolute
contributions and relatively low reduction from 2012 to BAU2040.</p>
      <p id="d1e3293">When it comes to changes in <inline-formula><mml:math id="M224" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations, there is an increase in
the city centre by up to 15 % (about 4 ppb) from 2012 to BAU2040,
especially near major roads. This contrary trend follows the principles of
ground-level ozone formation, which is produced in photochemical reaction
cycles involving the precursors <inline-formula><mml:math id="M225" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and VOCs. The ozone–precursor
relationship in urban environments is a consequence of the fundamental
division into an <inline-formula><mml:math id="M226" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>-sensitive and a VOC-sensitive regime (Sillman, 1999).
VOC-sensitive regimes in dense urban areas with many emission sources lead
to higher <inline-formula><mml:math id="M227" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> with increasing VOC and lower <inline-formula><mml:math id="M228" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> with increasing
<inline-formula><mml:math id="M229" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Karl et al., 2019a). Therefore, the contribution of local ship
emissions with ozone precursors <inline-formula><mml:math id="M230" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and VOCs can selectively be very
significant, in terms of both increasing the <inline-formula><mml:math id="M231" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> levels in urban areas
and decreasing them in the outskirts. Figure 5 shows that both the absolute
and the relative change in impact of shipping activities between 2012 and
BAU2040 becomes more visible for <inline-formula><mml:math id="M232" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> than for <inline-formula><mml:math id="M233" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the western
parts of the city, due to the higher ozone formation in the absence of
<inline-formula><mml:math id="M234" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> sources in the BAU2040 scenario.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><?xmltex \currentcnt{6}?><label>Figure 6</label><caption><p id="d1e3420">Absolute contributions of local ship emissions to annual
mean concentration levels in Gothenburg in 2012 (column 1) and BAU2040
(column 2), as well as the relative contributions (columns 3 and 4).
©OpenStreetMap contributors 2019. Distributed under a
Creative Commons BY-SA License.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f06.png"/>

        </fig>

      <p id="d1e3430">For PM<inline-formula><mml:math id="M235" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M236" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the high impact of some industrial sources in
the west of Gothenburg is even more visible. While in 2012 the average
PM<inline-formula><mml:math id="M237" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> concentrations peak at 53 <inline-formula><mml:math id="M238" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M239" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the
vicinity of the largest point sources, in BAU2040 they peak at 48 <inline-formula><mml:math id="M240" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M241" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The domain-averaged PM<inline-formula><mml:math id="M242" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> concentrations are
much lower with 4 <inline-formula><mml:math id="M243" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M244" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in 2012 and 2.7 <inline-formula><mml:math id="M245" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M246" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in BAU2040; thus they are reduced by 33 % on average. Slightly higher reductions close to roads are caused by lower
PM<inline-formula><mml:math id="M247" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> road traffic emissions. Reductions in the northeast of the urban
area of Gothenburg are probably due to less secondary particle formation.
This pattern also holds true for <inline-formula><mml:math id="M248" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. There is an absolute reduction
potential for <inline-formula><mml:math id="M249" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> of up to 1 <inline-formula><mml:math id="M250" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M251" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and a
relative reduction potential of up to 75 % in the port area, following
shipping routes. Nevertheless, the characteristic industrial point sources
bear the highest absolute <inline-formula><mml:math id="M252" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> reductions and therefore partly diminish
the relative <inline-formula><mml:math id="M253" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> reduction potential in the port area of Gothenburg.</p>
      <p id="d1e3627">In total, the air quality situation with respect to <inline-formula><mml:math id="M254" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M255" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and
<inline-formula><mml:math id="M256" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is clearly improving in the urban area of Gothenburg in the BAU2040
scenario. However, the large industrial point sources, such as three
refineries (Preem Gothenburg, St1 Refinery AB, Nynäs Gothenburg), are
identified as large contributors to spatially selective high concentrations
of <inline-formula><mml:math id="M257" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M258" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M259" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and still contain a high reduction
potential compared to all other sources of air pollution in the urban area
of Gothenburg. When it comes to<?pagebreak page10677?> ozone there is an average increase of up to
1 ppb in summer, probably due to a lower background concentration and
consequently less ozone titration by the lower <inline-formula><mml:math id="M260" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emission in 2040.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><label>Figure 7</label><caption><p id="d1e3706">Relative changes in annual mean
<inline-formula><mml:math id="M261" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M262" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M263" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations for BAU2040LP compared to 2040BAU scenario. © OpenStreetMap contributors 2019. Distributed under a
Creative Commons BY-SA License.</p></caption>
          <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f07.png"/>

        </fig>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T3" specific-use="star"><?xmltex \currentcnt{3}?><label>Table 3</label><caption><p id="d1e3749">Population-weighted exposure in the Gothenburg area to
<inline-formula><mml:math id="M264" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (in ppb), PM<inline-formula><mml:math id="M265" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> (in
<inline-formula><mml:math id="M266" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M267" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), and ozone (as sum of hourly means over
35 ppb) in 2012 and in the BAU2040 and EEDI2040 scenarios. The exposure
caused by local shipping, local and regional shipping, and ships at berth is
given separately.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Population-weighted concentration (PWC)</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M270" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">PM<inline-formula><mml:math id="M271" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">SOMO35</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(ppb)</oasis:entry>
         <oasis:entry colname="col3">(<inline-formula><mml:math id="M272" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M273" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col4">(ppb h<inline-formula><mml:math id="M274" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Year 2012</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Total base</oasis:entry>
         <oasis:entry colname="col2">4.70</oasis:entry>
         <oasis:entry colname="col3">4.12</oasis:entry>
         <oasis:entry colname="col4">19 698</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Local shipping<inline-formula><mml:math id="M275" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">0.68</oasis:entry>
         <oasis:entry colname="col3">0.09</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M276" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1186</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Local <inline-formula><mml:math id="M277" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> regional shipping</oasis:entry>
         <oasis:entry colname="col2">1.65</oasis:entry>
         <oasis:entry colname="col3">0.51</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M278" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1115</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Year 2040</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Total BAU2040</oasis:entry>
         <oasis:entry colname="col2">1.16</oasis:entry>
         <oasis:entry colname="col3">2.80</oasis:entry>
         <oasis:entry colname="col4">18 723</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Local shipping BAU2040<inline-formula><mml:math id="M279" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">0.08</oasis:entry>
         <oasis:entry colname="col3">0.02</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M280" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">115</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Local <inline-formula><mml:math id="M281" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> regional shipping BAU2040</oasis:entry>
         <oasis:entry colname="col2">0.18</oasis:entry>
         <oasis:entry colname="col3">0.31</oasis:entry>
         <oasis:entry colname="col4">35</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Shipping emissions at berth<inline-formula><mml:math id="M282" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> BAU2040</oasis:entry>
         <oasis:entry colname="col2">0.12</oasis:entry>
         <oasis:entry colname="col3">0.01</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M283" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">241</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Total EEDI2040</oasis:entry>
         <oasis:entry colname="col2">1.39</oasis:entry>
         <oasis:entry colname="col3">2.83</oasis:entry>
         <oasis:entry colname="col4">18 434</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Local shipping EEDI2040</oasis:entry>
         <oasis:entry colname="col2">0.28</oasis:entry>
         <oasis:entry colname="col3">0.01</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M284" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">727</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Shipping emissions at berth<inline-formula><mml:math id="M285" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> EEDI2040</oasis:entry>
         <oasis:entry colname="col2">0.18</oasis:entry>
         <oasis:entry colname="col3">0.01</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M286" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">267</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><table-wrap-foot><p id="d1e3792"><inline-formula><mml:math id="M268" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> Includes emissions at berth.
<inline-formula><mml:math id="M269" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> Emissions avoided by being replaced by land power in the BAU2040LP and
EEDI2040LP scenarios.</p></table-wrap-foot></table-wrap>

</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Influence of ship emissions in the future scenarios: BAU</title>
      <?pagebreak page10679?><p id="d1e4191">The modelled contributions of local shipping to atmospheric concentrations
and relative contributions to the overall air pollution in Gothenburg in the
BAU2040 scenario show high reductions relative to the year 2012 for all
pollutants under investigation except of <inline-formula><mml:math id="M287" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, which is slightly
increasing (Fig. 6). Higher absolute and relative contributions of local
shipping are detected in and around the port area, while there are some
minor impacts in the northern urban area of Gothenburg due to predominant
winds from the southwest. This general pattern also holds true for the EEDI2040
scenario. The maximum value for the contribution to annual mean <inline-formula><mml:math id="M288" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations in BAU2040 merely reaches 1 ppb in the port area and is about
80 % lower compared to a maximum of 4.1 ppb in 2012. In the EEDI2040
scenario the maximum ship contribution to <inline-formula><mml:math id="M289" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is slightly higher with
1.4 ppb. The relative contribution of shipping given as annual average in
the entire model domain changed from 14 % to 6 % in BAU2040. In the
EEDI2040 scenario, the relative contribution of local shipping to the
annually averaged grid means reaches 18 %. The relative contributions of
shipping in the port area of Gothenburg is up to 25 % in BAU2040 and up
to 45 % in EEDI2040. In 2012, <inline-formula><mml:math id="M290" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations due to shipping are
involved as a precursor in the photochemical reaction-cycle of <inline-formula><mml:math id="M291" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
formation and form a depletion pattern around the harbour area with up to <inline-formula><mml:math id="M292" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:math></inline-formula> ppb <inline-formula><mml:math id="M293" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. Following the principles of <inline-formula><mml:math id="M294" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> formation in a
high-<inline-formula><mml:math id="M295" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> environment the pattern shows ozone formation from shipping
emissions further from the harbour area. The same pattern is visible in
future scenarios but with only a small depletion of <inline-formula><mml:math id="M296" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula> ppb <inline-formula><mml:math id="M297" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> at most in BAU2040 and <inline-formula><mml:math id="M298" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.2</mml:mn></mml:mrow></mml:math></inline-formula> ppb <inline-formula><mml:math id="M299" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in EEDI2040. While in 2012,
<inline-formula><mml:math id="M300" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations increase by up to 8 % (<inline-formula><mml:math id="M301" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula> ppb)
outside the port area, in the future scenarios shipping-related <inline-formula><mml:math id="M302" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations are on average around 0, except for the area with industrial
emission sources in the west. Here, high VOC emissions from the industrial
sources react with <inline-formula><mml:math id="M303" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions from nearby shipping and form about 1 ppb <inline-formula><mml:math id="M304" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> at most, which can be accounted to shipping activities.
Nevertheless, the overall contribution of shipping to increased <inline-formula><mml:math id="M305" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M306" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations is very low in both future scenarios.</p>
      <p id="d1e4413">The pollutants PM<inline-formula><mml:math id="M307" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M308" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> show similar reduction patterns in
the future scenarios. The huge reductions in PM<inline-formula><mml:math id="M309" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math id="M310" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">85</mml:mn></mml:mrow></mml:math></inline-formula> %) and
<inline-formula><mml:math id="M311" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math id="M312" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">91</mml:mn></mml:mrow></mml:math></inline-formula> %) emissions are consequently leading to a reduced impact
of shipping in BAU2040. The contribution of PM<inline-formula><mml:math id="M313" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> from local ship
emissions is relatively low in 2012 (maximum of 0.9 <inline-formula><mml:math id="M314" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M315" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the western port area), and even lower (maximum of
0.15 <inline-formula><mml:math id="M316" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M317" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the western port area) in the BAU2040
scenario. The <inline-formula><mml:math id="M318" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in the Gothenburg area are driven by
industrial and shipping emissions, which account for more than 99 % of
the total, both in 2012 and in BAU2040. Between 2012 and BAU2040 the
<inline-formula><mml:math id="M319" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions from shipping decreased by 91 % and therefore the
concentration of <inline-formula><mml:math id="M320" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> decreased as well. While there has been a relative
contribution of shipping to <inline-formula><mml:math id="M321" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in summer of about 70 % in the harbour and its surrounding areas in 2012 (concentration
contribution maxima of up to 0.7 <inline-formula><mml:math id="M322" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M323" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), in the
2040BAU scenario the contributions are below 20 % with a maximum
concentration contribution of less than 0.2 <inline-formula><mml:math id="M324" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M325" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to
the summer mean. To summarize, the air pollution from shipping in the
BAU2040 scenario reflects the large emission reductions compared to 2012,
resulting in very low contributions to atmospheric pollution levels.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><label>Figure 8</label><caption><p id="d1e4614">Absolute contributions of total concentration changes
between 2012 and 2040 to PWC in Gothenburg <bold>(a–c)</bold>. Contribution of all
shipping (regional <inline-formula><mml:math id="M326" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> local) in BAU2040 to PWC <bold>(d–f)</bold>. Contribution
of local shipping in BAU2040 to PWC <bold>(g–i)</bold>. Impact of implementation of
shoreside electricity on PWC <bold>(j–l)</bold>. ©OpenStreetMap contributors
2019. Distributed under a Creative Commons BY-SA License.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/20/10667/2020/acp-20-10667-2020-f08.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Influence of shoreside electricity use in future
scenarios</title>
      <p id="d1e4650">The model simulations show that the contribution of shipping to air
pollution in Gothenburg in the future scenarios is focussed on the port
area (Fig. 6). The results for the shoreside electricity scenario BAU2040LP
show visible reductions in <inline-formula><mml:math id="M327" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M328" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M329" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations in the port area (Fig. 7). For <inline-formula><mml:math id="M330" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, local concentration
reductions in the port area are up to 25 % in comparison to BAU2040, and
for the EEDI2040LP scenario, the <inline-formula><mml:math id="M331" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> reduction due to the shoreside
electricity is up to 30 % (Fig. 6). In the surrounding areas of
Gothenburg, the reductions range between 1 % and 15 %. In terms of
<inline-formula><mml:math id="M332" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, replacement of emissions from auxiliary engines at berth with
electricity (BAU2040LP scenario) causes an increase of up to 2.5 %. In
the EEDI2040LP scenario the relative increase in annual mean <inline-formula><mml:math id="M333" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations compared to the EEDI2040 scenario is up to 3 % (Fig. 7).
In both scenarios, the decrease in <inline-formula><mml:math id="M334" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions leads to an increase
in <inline-formula><mml:math id="M335" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations due to less titration of <inline-formula><mml:math id="M336" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The results for
PM<inline-formula><mml:math id="M337" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M338" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> show similar characteristics. BAU2040LP and
EEDI2040LP lead to additional local reduction potentials of up to 3 % for
PM<inline-formula><mml:math id="M339" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and 12 % for <inline-formula><mml:math id="M340" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the port area, but almost no
difference can be seen outside the port area. EEDI2040LP shows a slightly
higher reduction potential than BAU2040LP. In total, the implementation of
shoreside electricity is clearly beneficial to reduce the impact of
shipping emissions and therefore increase the air quality in areas close to
the port.</p>

<?xmltex \floatpos{p}?><table-wrap id="Ch1.T4" orientation="landscape"><?xmltex \currentcnt{4}?><label>Table 4</label><caption><p id="d1e4806">Health impacts calculated for BAU2040 and EEDI2040
scenarios with ARP and RAINS methodologies: emissions at berth – impacts
potentially avoided by the shore-site electricity implementation (BAU2040 –
BAU2040-LP and EEID2040 – EEID2040LP); local shipping – impacts of all
local shipping emissions in the model domain, including emissions at berth;
local <inline-formula><mml:math id="M341" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> regional shipping – impacts of all shipping emissions
including the regional shipping emissions in the Baltic Sea and the North
Sea in the model boundary conditions; total exposure – impacts of the total
PWC for PM<inline-formula><mml:math id="M342" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, <inline-formula><mml:math id="M343" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and ozone as SOMO35 in the model domain.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="10">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right" colsep="1"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:colspec colnum="9" colname="col9" align="right"/>
     <oasis:colspec colnum="10" colname="col10" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry rowsep="1" namest="col4" nameend="col7" align="center" colsep="1">BAU2040 </oasis:entry>
         <oasis:entry rowsep="1" namest="col8" nameend="col10" align="center">EEDI2040 </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Emissions</oasis:entry>
         <oasis:entry colname="col5">Local</oasis:entry>
         <oasis:entry colname="col6">Local<inline-formula><mml:math id="M344" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">Total</oasis:entry>
         <oasis:entry colname="col8">Emissions</oasis:entry>
         <oasis:entry colname="col9">Local</oasis:entry>
         <oasis:entry colname="col10">Total</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Pollutant</oasis:entry>
         <oasis:entry colname="col2">Impact</oasis:entry>
         <oasis:entry colname="col3">Unit</oasis:entry>
         <oasis:entry colname="col4">at berth*</oasis:entry>
         <oasis:entry colname="col5">shipping**</oasis:entry>
         <oasis:entry colname="col6">regional shipping</oasis:entry>
         <oasis:entry colname="col7">exposure</oasis:entry>
         <oasis:entry colname="col8">at berth*</oasis:entry>
         <oasis:entry colname="col9">shipping**</oasis:entry>
         <oasis:entry colname="col10">exposure</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">PM<inline-formula><mml:math id="M345" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Chronic mortality</oasis:entry>
         <oasis:entry colname="col3">Life years lost per year</oasis:entry>
         <oasis:entry colname="col4">2.7</oasis:entry>
         <oasis:entry colname="col5">6.6</oasis:entry>
         <oasis:entry colname="col6">106</oasis:entry>
         <oasis:entry colname="col7">955</oasis:entry>
         <oasis:entry colname="col8">3.9</oasis:entry>
         <oasis:entry colname="col9">4.8</oasis:entry>
         <oasis:entry colname="col10">967</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PM<inline-formula><mml:math id="M346" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Chronic mortality</oasis:entry>
         <oasis:entry colname="col3">Premature deaths per year</oasis:entry>
         <oasis:entry colname="col4">0.3</oasis:entry>
         <oasis:entry colname="col5">0.8</oasis:entry>
         <oasis:entry colname="col6">13</oasis:entry>
         <oasis:entry colname="col7">120</oasis:entry>
         <oasis:entry colname="col8">0.5</oasis:entry>
         <oasis:entry colname="col9">0.6</oasis:entry>
         <oasis:entry colname="col10">122</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PM<inline-formula><mml:math id="M347" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Chronic mortality</oasis:entry>
         <oasis:entry colname="col3">YOLLs per person</oasis:entry>
         <oasis:entry colname="col4">0.0002</oasis:entry>
         <oasis:entry colname="col5">0.0006</oasis:entry>
         <oasis:entry colname="col6">0.009</oasis:entry>
         <oasis:entry colname="col7">0.084</oasis:entry>
         <oasis:entry colname="col8">0.0003</oasis:entry>
         <oasis:entry colname="col9">0.0004</oasis:entry>
         <oasis:entry colname="col10">0.085</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PM<inline-formula><mml:math id="M348" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Chronic mortality (RAINS)</oasis:entry>
         <oasis:entry colname="col3">YOLLs per person</oasis:entry>
         <oasis:entry colname="col4">0.0003</oasis:entry>
         <oasis:entry colname="col5">0.0007</oasis:entry>
         <oasis:entry colname="col6">0.011</oasis:entry>
         <oasis:entry colname="col7">0.096</oasis:entry>
         <oasis:entry colname="col8">0.0004</oasis:entry>
         <oasis:entry colname="col9">0.0005</oasis:entry>
         <oasis:entry colname="col10">0.097</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M349" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Acute mortality</oasis:entry>
         <oasis:entry colname="col3">Premature deaths</oasis:entry>
         <oasis:entry colname="col4">0.23</oasis:entry>
         <oasis:entry colname="col5">0.17</oasis:entry>
         <oasis:entry colname="col6">0.36</oasis:entry>
         <oasis:entry colname="col7">2.28</oasis:entry>
         <oasis:entry colname="col8">0.35</oasis:entry>
         <oasis:entry colname="col9">0.55</oasis:entry>
         <oasis:entry colname="col10">2.74</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M350" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Acute mortality</oasis:entry>
         <oasis:entry colname="col3">Premature deaths</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M351" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.1</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M352" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.1</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">0.02</oasis:entry>
         <oasis:entry colname="col7">9.0</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M353" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.1</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M354" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.4</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col10">8.9</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><table-wrap-foot><p id="d1e4836">* Emissions at berth avoided by being replaced by land power in the LP
scenarios. ** Includes emissions at berth.</p></table-wrap-foot></table-wrap>

</sec>
</sec>
<?pagebreak page10680?><sec id="Ch1.S5">
  <label>5</label><title>Impacts of future shipping on exposure to air pollutants and related health effects</title>
<sec id="Ch1.S5.SS1">
  <label>5.1</label><title>Impact of future shipping on population exposure</title>
      <p id="d1e5262">Table 3 shows PWCs for <inline-formula><mml:math id="M355" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>,
PM<inline-formula><mml:math id="M356" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and <inline-formula><mml:math id="M357" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (expressed as SOMO35) in the inner model domain for
the year 2012 and the investigated scenarios BAU2040 and EEDI2040. PWCs
attributed to local and regional shipping in the Gothenburg area and the
effect of shoreside electricity in BAU2040LP and EEDI2040LP are also shown.</p>
      <?pagebreak page10681?><p id="d1e5296">The calculated exposure to PM<inline-formula><mml:math id="M358" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> was <inline-formula><mml:math id="M359" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">2.8</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M360" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M361" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the scenarios BAU2040 and EEDI2040 with a large part of the
exposure originating from the regional background. The calculated decrease
due to the reductions in anthropogenic emissions between 2012 and 2040 is one-third. The contribution of local shipping to PM<inline-formula><mml:math id="M362" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure was
less than 1 % (<inline-formula><mml:math id="M363" display="inline"><mml:mrow><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">0.02</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M364" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M365" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> in all scenarios. In the
BAU2040 scenario, emissions from ships at berth which can be replaced by
shoreside electricity in the BAU2040LP scenario caused approximately 50 % of the PM<inline-formula><mml:math id="M366" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure attributed to the local shipping. In the
EEDI2040LP scenario the shipping emissions at berth are responsible for more
than 90 % of the exposure attributed to local shipping. Although the
BAU2040LP and EEDI2040LP scenarios imply a relative emission reduction of 62 % (compared to BAU2040 and EEDI2040, respectively) due to shoreside
electricity use at berth, the impact in terms of absolute concentrations is
less than 0.01 <inline-formula><mml:math id="M367" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M368" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in both scenarios. When
additionally the contribution of emissions from regional shipping in the
Baltic Sea and the North Sea is considered, the contribution of shipping to
PM<inline-formula><mml:math id="M369" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure in the BAU2040 scenario of 11 % (0.3 <inline-formula><mml:math id="M370" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M371" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is substantially larger than that of the local shipping. This is due
to the large impact of secondary particulate matter formed during the
atmospheric transport of the more distant emissions. This secondary PM is
calculated in the CMAQ model providing the boundary conditions for the TAPM
simulations, and it considers mainly particulate sulfate and nitrate since
VOC emissions from shipping are not included in that simulation.</p>
      <p id="d1e5443">The contribution of shipping to the PWC of <inline-formula><mml:math id="M372" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is about 10 % in the
BAU2040 scenario and 20 % in the EEDI2040 scenario (0.1 and 0.3 ppb
contributions, respectively). Thus, there is a clear impact of higher
improved energy efficiency. When the contribution of regional shipping
is also considered in the BAU2040 scenario, the contribution of all shipping to
the <inline-formula><mml:math id="M373" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> exposure is 16 % (0.18 ppb); the regional shipping
contribution is not as important as in the case of exposure to PM<inline-formula><mml:math id="M374" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>.
One reason is that emissions of primary PM from shipping are approximately 30 times lower than emissions of <inline-formula><mml:math id="M375" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M376" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:math></inline-formula>  times lower than emissions of <inline-formula><mml:math id="M377" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, which makes the contribution of
secondary PM formed from the more distant emissions relatively more
important compared to the local emissions of primary PM. Another reason is
the longer lifetime of secondary components in the atmosphere.</p>
      <p id="d1e5510">In all modelled scenarios the impact of local shipping decreased the
population exposure to <inline-formula><mml:math id="M378" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> due to less titration in the absence
of <inline-formula><mml:math id="M379" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> sources. Nevertheless, when the impact of regional shipping is
included in the BAU2040 scenario, shipping emissions cause small increases
in exposure to <inline-formula><mml:math id="M380" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The <inline-formula><mml:math id="M381" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> exposure attributed to local shipping, however, only considers population in the local region, while one can expect
<inline-formula><mml:math id="M382" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> formation to cause an increase in exposure for the population living
further away from the city.</p>
      <p id="d1e5569">In total, a very low impact of PM<inline-formula><mml:math id="M383" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> due to local shipping activities
was simulated for the scenarios with and without shoreside electricity. In
all cases, the regional background can be considered as the main contributor
to PM<inline-formula><mml:math id="M384" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure in the urban area. For <inline-formula><mml:math id="M385" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the contribution of
shipping-related concentrations to the total air pollution is significant
within both scenarios (with and without shoreside electricity reduction
scenarios) in 2040, with important, but lower, contributions from regional
background concentrations compared to PM<inline-formula><mml:math id="M386" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>. Nevertheless, the
BAU2040LP and EEDI2040LP scenarios show a high reduction potential and
benefits for the air quality in densely located areas.</p>
      <?pagebreak page10682?><p id="d1e5610">The contribution of air pollution levels to the overall population exposure
expressed as PWC depends on the relationship between spatial distribution of
concentrations of air pollutants and the population density. Figure 8 shows
products of mean concentration and population in each model grid cell with a
resolution of <inline-formula><mml:math id="M387" display="inline"><mml:mrow><mml:mn mathvariant="normal">250</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">250</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:mrow></mml:math></inline-formula>, which represent exposure in the domain.
Compared to the air quality situation in 2012 (Fig. 8a–c), the exposure
to <inline-formula><mml:math id="M388" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M389" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> will decrease in the densely populated area in
2040, especially due to reduced emissions from road traffic. On the other
hand, <inline-formula><mml:math id="M390" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> exposure is increasing correspondingly because of reduced
local <inline-formula><mml:math id="M391" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> titration caused by decreased <inline-formula><mml:math id="M392" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions in most parts
of the city. The spatial patterns of <inline-formula><mml:math id="M393" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M394" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> exposure from
local shipping (Fig. 8g–i) are dominated by gradients in the
concentration fields with highest reduction around the city ports north of
the Göta älv. The contribution of regional and local shipping
to total exposure (Fig. 8d–f) for <inline-formula><mml:math id="M395" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M396" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> is higher in
a larger city area since regional-shipping-related <inline-formula><mml:math id="M397" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M398" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>
exposure is evenly distributed over the city. The introduction of onshore
electricity (Fig. 8j–l) gives visible reductions in the port area for
exposure to <inline-formula><mml:math id="M399" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math id="M400" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">200</mml:mn></mml:mrow></mml:math></inline-formula> ppb <inline-formula><mml:math id="M401" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> capita) and PM<inline-formula><mml:math id="M402" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>
(<inline-formula><mml:math id="M403" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mo>-</mml:mo><mml:mn mathvariant="normal">50</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M404" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M405" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> due to the emissions avoided by
shoreside electricity.</p>
</sec>
<sec id="Ch1.S5.SS2">
  <label>5.2</label><title>Impact of future shipping on health effects</title>
      <p id="d1e5831">Table 4 gives an overview of health impacts calculated for the exposure to
PM<inline-formula><mml:math id="M406" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, <inline-formula><mml:math id="M407" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math id="M408" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in terms of mortalities and years of life
lost (YOLLs). The results show that in 2040 all shipping-related PM<inline-formula><mml:math id="M409" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>,
including the regional shipping, would cause 13 premature deaths per year
corresponding to a shortened lifetime of 0.009 years per person (3.4 d)
in the BAU2040 scenario. The majority of the impact (over 90 %) can be
associated with the regional shipping outside the city. Impacts from local
shipping in Gothenburg were found to be small: less than one premature death
in the city, corresponding to 0.0006 and 0.0004 YOLLs per person in the BAU2040
and EEDI2040 scenario, respectively (<inline-formula><mml:math id="M410" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">0.2</mml:mn></mml:mrow></mml:math></inline-formula> d). Shoreside
electricity reduced the impact of PM<inline-formula><mml:math id="M411" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> from local shipping by ca. 40 % and 80 % in the BAU2040LP and EEDI2040LP scenarios, respectively,
but only by a few percent if regional shipping is also considered in the
BAU2040 scenario. The impacts from the short-term exposure to <inline-formula><mml:math id="M412" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> were
calculated to be 0.36 premature deaths per year in the model domain for all
shipping in the BAU2040 scenario, 0.17 premature death (46 %) being
attributed to local shipping. In the EEDI2040 scenario the <inline-formula><mml:math id="M413" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> impact
from local shipping was larger, 0.55 premature deaths per year. Impacts from
short-term exposure to <inline-formula><mml:math id="M414" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> associated with shipping were calculated as being 0.02 premature deaths in the BAU2040 scenario when all shipping is
considered. As emissions from the local shipping lead to a decrease in
<inline-formula><mml:math id="M415" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in the city, the impact of local shipping would
decrease mortalities with 0.1 and 0.4 premature deaths per year in the
BAU2040 and EEDI2040 scenarios, respectively.</p>
      <p id="d1e5938">The impact of climate policy measures in the shipping sector has been
addressed in Cofala et al. (2018), too, in a study using similar methods as
here. The study includes two base scenarios, one without and one with
climate policy measures; the former keeps the shipping emissions 45 % higher than the latter in 2040. Comparison of the data supplement in
Cofala et al. (2018) shows that the PM<inline-formula><mml:math id="M416" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>-related mortalities caused by
shipping decreased by 1.7 % (<inline-formula><mml:math id="M417" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">300</mml:mn></mml:mrow></mml:math></inline-formula> YOLLs per year) for
Sweden and by 2 % (<inline-formula><mml:math id="M418" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">35</mml:mn></mml:mrow></mml:math></inline-formula> 000 YOLLs per year) for the EU
including UK, Norway, and Switzerland in the climate measures' scenario compared to the
scenario without measures. Mortalities caused by <inline-formula><mml:math id="M419" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> exposure
related to shipping emissions decreased between these two scenarios by 4.3 % (6 premature deaths) for Sweden and by 5.4 % (848 premature deaths)
for the EU in 2040. The results for PM<inline-formula><mml:math id="M420" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> are in line with our findings,
and if we scale up our results to all of Sweden and account for the
difference between the relative emission change in the scenarios by Cofala
et al. (2018) and ours, we find rather similar result (<inline-formula><mml:math id="M421" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> % difference). For <inline-formula><mml:math id="M422" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the change between the scenarios in our study
is of opposite sign than in Cofala et al. (2018), indicating a difference in
the <inline-formula><mml:math id="M423" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> formation regime in the two air pollution models used.</p>
</sec>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <label>6</label><title>Conclusions</title>
      <p id="d1e6032">We investigated the future effect of shipping emissions on air quality and
related health effects considering different scenarios of the development of
shipping under current regional trends of economic growth and already
decided regulations in the Gothenburg urban area in 2040. Additionally, we
investigated the impact of a large-scale implementation of shoreside
electricity in the Port of Gothenburg. For this purpose, we established a
one-way nested CTM system from the global to
the urban scale, to calculate pollutant concentrations, population-weighted
concentrations, and health effects related to <inline-formula><mml:math id="M424" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, PM<inline-formula><mml:math id="M425" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>, and
<inline-formula><mml:math id="M426" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. This paper is the second part of a study about the current and
future air quality situation in the Gothenburg urban area. Part 1 by Tang et al. (2020) introduced, evaluated, and discussed air pollutant concentrations,
population-weighted concentration, and health effects for the year 2012 and is
published in the same special issue.</p>
      <p id="d1e6066">The simulated concentrations of <inline-formula><mml:math id="M427" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M428" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> in future scenarios
for the year 2040 are in general very low with up to 4 ppb for <inline-formula><mml:math id="M429" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
up to 3.5 <inline-formula><mml:math id="M430" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>g m<inline-formula><mml:math id="M431" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for PM<inline-formula><mml:math id="M432" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> in the urban areas
distant to the port area. Nevertheless, two hotspots of <inline-formula><mml:math id="M433" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
PM<inline-formula><mml:math id="M434" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> with higher concentrations are located west of the city. These
hotspots are due to industrial emissions, in particular from refineries.
Compared to 2012 the simulated overall exposure to PM<inline-formula><mml:math id="M435" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> decreased by
approximately 30 % in the BAU scenario for 2040. For <inline-formula><mml:math id="M436" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the
decrease was more than 60 %. The simulated concentrations of ozone
increased between 2012 and 2040 by about 20 %. This increase results from
both higher concentrations simulated in the regional model domain and
transported through the boundaries into the city domain and from lower
<inline-formula><mml:math id="M437" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> titration by reduced <inline-formula><mml:math id="M438" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions. Local shipping also contributes to the titration causing negative contributions to <inline-formula><mml:math id="M439" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations. The impact of the background shipping, however, causes
<inline-formula><mml:math id="M440" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> formation in the city domain, and the overall impact of shipping on
<inline-formula><mml:math id="M441" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations is a net <inline-formula><mml:math id="M442" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> formation.</p>
      <p id="d1e6237">In general, the contributions of local shipping emissions in 2040 focus on
the harbour area. Only to some extent do they influence the rest of the city
domain. For <inline-formula><mml:math id="M443" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> there are in maximum local shipping contributions of
more than 30 %<?pagebreak page10683?> to the total concentrations, located in the port and the
area surrounding it, while contributions of the local shipping activities to
the <inline-formula><mml:math id="M444" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in other parts of the city are up to 10 %
only. The contributions of PM<inline-formula><mml:math id="M445" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> by shipping activities are generally
much lower (up to 3 % at most) and follow the same trend with higher
contributions located in the harbour area and its surroundings and lower
impacts in the other areas.</p>
      <p id="d1e6271">The simulated impact of a wide use of shoreside electricity for shipping in
2040 shows similar spatial patterns for <inline-formula><mml:math id="M446" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M447" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>. For
<inline-formula><mml:math id="M448" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, local concentration reductions in the port area range between 25 % and 30 % at most, depending on the individual scenario. In the
surrounding areas of Gothenburg, the reductions range between 1 % and 15 %. In terms of <inline-formula><mml:math id="M449" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, replacement of emissions from auxiliary engines
at berth with electricity causes an increase of up to 2.5 %–3 %,
depending on the scenario. Implementation of shoreside electricity for
ships at berth leads to an additional local reduction potential of up to 3 % for PM<inline-formula><mml:math id="M450" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and 12 % for <inline-formula><mml:math id="M451" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">SO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in the port area, but almost
no difference can be seen outside the port area. In total, the
implementation of shoreside electricity is clearly beneficial to reduce the
impact of shipping emissions, and it therefore improves air quality in areas
close to the port. Moreover, the strict regulations as simulated in the
BAU2040 scenario are of a high value for an improved air quality in the urban
area of Gothenburg.</p>
      <p id="d1e6338">In 2040 simulations the air quality situation in the city improves
considerably and the concentrations will be below the air quality limit and
target values both for <inline-formula><mml:math id="M452" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M453" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> in the city, even if the
potential underestimates of the model system are accounted for (Tang et al.,
2020). From the static point of view of the year 2040 the conclusion that additional
measures to reduce air pollution levels beyond those in the BAU scenario
would not be necessary could be drawn. However, in perspective, taking also
the temporal development into consideration, the measures reducing
concentrations of <inline-formula><mml:math id="M454" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> will be implemented only at a slow pace and the full
impact of many of them, especially those targeting shipping, will first be
seen in the time horizon of 2040. The local measures could, on the other
hand, be implemented faster and the significant reduction in <inline-formula><mml:math id="M455" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
concentrations from the implementation of onshore electricity could thus reduce
the time before the air quality targets are met in the city.</p>
      <p id="d1e6383">Calculated population-weighted concentrations and health impacts follow the
same trends. The PM<inline-formula><mml:math id="M456" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> contribution of local shipping to PWC of
PM<inline-formula><mml:math id="M457" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> is below 1 % for all scenarios, but the contribution of
regional shipping outside the city domain is still of importance: in the
BAU2040 scenario, its contribution is about 10 %. Relative to 2012 the
exposure to PM<inline-formula><mml:math id="M458" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> from local shipping decreased by more than 80 % in
all scenarios for 2040, while the impact of all shipping including the
regional contribution decreased by only 40 %. The local shipping
contribution to PWC of <inline-formula><mml:math id="M459" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is much more pronounced, being 10 % for
the BAU2040 and 20 % for the EEDI2040 scenario. In the BAU scenario,
regional shipping contributed an additional 6 % to the PWC of <inline-formula><mml:math id="M460" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. In
comparison to 2012, exposure to <inline-formula><mml:math id="M461" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> from local shipping decreased by
approximately 50 % for the EEDI2040 scenario and by more than 80 % for
the BAU2040 scenario. In the BAU2040 scenario exposure to <inline-formula><mml:math id="M462" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> from all
shipping, including the regional contribution, decreased by 86 %. The PWC
of ozone, given as SOMO35, increased in the model domain by about 20 %, following the trends in concentrations.</p>
      <p id="d1e6458">The most serious health effects were associated with PM<inline-formula><mml:math id="M463" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>. It needs to
be emphasized that the effects presented in Table 3 cannot be added due to a
risk of double-counting, especially concerning PM<inline-formula><mml:math id="M464" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M465" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.
Between 2012 and 2040 we can see a large decrease in mortality caused by
PM<inline-formula><mml:math id="M466" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> associated with shipping; in the future reference scenario
(BAU2040) the total decrease is 86 %. For the whole city domain, this
results in nine premature deaths per year that are avoided, corresponding to 67 YOLLs per year. This decrease is mainly associated with the decrease in emissions
due to strengthened SECA legislation introduced in 2015. The introduction of
the NECA legislation in 2021, with a rather slow uptake of abatement
technologies for the reduction in <inline-formula><mml:math id="M467" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions, as well as climate
policy measures implemented in terms of energy effectivization of the fleet,
will lead to an additional reduction in <inline-formula><mml:math id="M468" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions and those of
other air pollutants. Partial impacts of these three aspects have not been
studied here.</p>
      <p id="d1e6522">As already discussed in Tang et al. (2020), Jonson et al. (2019) studied the
impact of an introduction of strengthened sulfur limits in 2015 and found an approximately 35 % reduction in the impact from the regional shipping
contribution to PM<inline-formula><mml:math id="M469" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> around Gothenburg. The global study of Sofiev et al. (2018) shows that the impact of the global cap down to 0.5 % FSC does
not have any significant impact on a further reduction in shipping-related
air pollution around the Swedish west coast. The calculated decrease in
PM<inline-formula><mml:math id="M470" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> was below 1 %. Only limited impacts of these two regulations
on emission from the local shipping in Gothenburg can be expected since
ships at berth have been using fuels with maximum FSC of 0.1 % since 2010 already.</p>
      <p id="d1e6543">In this study, the impact of the improved energy efficiency can be obtained
by comparing the BAU scenario with the EEDI scenario, the latter showing
approx. 30 % higher emissions. The impact on health effects from exposure
to PM<inline-formula><mml:math id="M471" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> in the city domain is rather low: 1.2 % only. The impact of
the higher emissions on exposure to <inline-formula><mml:math id="M472" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is much more important with 17 %,
while exposure to ozone is 1.6 % lower in the EEDI scenario compared
to BAU.</p>
      <p id="d1e6566">Nevertheless, when it comes to the applied static exposure approach to
calculate PWC and health effects, the underlying assumption is that people
are at residential addresses throughout the time. Thus, static exposure does
not account for spatial and temporal variability of population activities
and will lead to uncertainties in calculated exposure and introduce
potential bias in the quantification of human health<?pagebreak page10684?> effects. Several
exposure modelling studies have overcome this traditional approach and are
using population activity data, derived from surveys, individual GIS data or
generic data, and models to account for the diurnal variation in population
numbers in different locations (e.g. Beckx et al., 2009; Smith et al., 2016;
Ramacher et al., 2019; Ramacher and Karl, 2020; Reis et al., 2018; Soares
et al., 2014). Thus, to model population numbers suitable for exposure
calculations, it is generally necessary to know the population distribution
and characterization and therefore the number of people and diurnal activity
patterns of different characteristic population groups. In future studies we
plan to account for population dynamics by applying averaged generic
population activity profiles, which are additionally diversified by
demographic groups in different microenvironments, such as residential
environments, work environments, or traffic environments. This will allow for
a better representation of pollutant concentrations people are exposed to
and the related health effects that are based on exposure calculations.</p>
      <p id="d1e6570">Impacts of the local shipping emissions on air quality and human health are
further discussed and evaluated for the year 2012 in the Part I paper (Tang
et al., 2020).</p>
</sec>

      
      </body>
    <back><notes notes-type="codeavailability"><title>Code availability</title>

      <p id="d1e6577">The TAPM model is a commercial software available at CSIRO, Australia
(<ext-link xlink:href="https://doi.org/10.1016/j.envsoft.2004.04.006" ext-link-type="DOI">10.1016/j.envsoft.2004.04.006</ext-link>,  Hurley et al., 2005). STEAM is the intellectual property of the
Finnish Meteorological Institute and is not publicly available. The ARP tool (Holland et al. 2013) is the intellectual property of Mike Holland and Joe Sparado (mike.holland@emrc.co.uk) and is not publicly available.</p>
  </notes><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e6586">The model output data are available upon request from the corresponding
authors.</p>
  </notes><app-group>
        <supplementary-material position="anchor"><p id="d1e6589">The supplement related to this article is available online at: <inline-supplementary-material xlink:href="https://doi.org/10.5194/acp-20-10667-2020-supplement" xlink:title="pdf">https://doi.org/10.5194/acp-20-10667-2020-supplement</inline-supplementary-material>.</p></supplementary-material>
        </app-group><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e6598">MOPR, LT, JM, and VM designed the model
simulations. LJ calculated ship emissions with STEAM
and contributed text about the shipping emissions. LT prepared ship
emission files for the model simulations. EF prepared future scenarios. LT and JM prepared emission data from other sources.
MK prepared data from the regional-scale simulation used for the
boundary. MOPR and LT prepared the model setup and other input
data, performed the model simulations, and evaluated the model results. LT calculated exposures, and JM calculated the health
impacts. MOPR and JM wrote the major part of the text with assistance from LT and VM.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e6604">The authors declare that they have no conflict of interest.</p>
  </notes><notes notes-type="sistatement"><title>Special issue statement</title>

      <p id="d1e6610">This article is part of the special issue “Shipping and the Environment – From Regional to Global Perspectives (ACP/OS inter-journal SI)”. It is a result of the Shipping and the Environment – From Regional to Global Perspectives, Gothenburg, Sweden, 23–24 October 2017.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e6616">The air quality model CMAQ is developed and maintained by the U.S.
Environmental Protection Agency (US EPA). COSMO-CLM is the community model
of German climate research (<uri>https://wiki.coast.hzg.de/clmcom</uri>, last access: 8 September 2020). The simulations with
COSMO-CLM and CMAQ were performed at the German Climate Computing Centre
(DKRZ) within the project “Regional Atmospheric Modelling” (Project Id
0302). The Swedish Meteorological and Hydrological Institute (SMHI) is
thanked for making available the precipitation data from rain gauge stations
in Sweden. Zbigniew Klimont  (IIASA) is thanked for emission data for the 2040 CLE
scenario from ECLIPSE v5. The NILU (Norsk institutt for luftforskning) is thanked for the EBAS database maintenance
and data provision. Sara Jutterström (IVL) is thanked for good
collaboration and discussion of model results on deposition of nitrogen and
sulfur.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e6625">This research has been supported by BONUS (grant no. Call 2014-41, BONUS SHEBA project) and the INTERREG Baltic Sea Region (grant no. C006 Project platform CSHIPP).<?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>The article processing charges for this open-access <?xmltex \hack{\newline}?> publication  were covered by a Research <?xmltex \hack{\newline}?> Centre of the Helmholtz Association.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e6638">This paper was edited by Huan Liu and reviewed by two anonymous referees.</p>
  </notes><ref-list>
    <title>References</title>

      <ref id="bib1.bib1"><label>1</label><?label 1?><mixed-citation>Amman, M., Cofala, J., Heyes, C., Klimont, Z., Mechler, R., Posch, M., and
Schöpp, W.: The RAINS model: Documentation of the model approach
prepared for the RAINS peer review 2004, Interim Report IR-04-075, available at: <uri>http://pure.iiasa.ac.at/id/eprint/7307/1/IR-04-075.pdf</uri>, last access: 8 January 2020, 2004.</mixed-citation></ref>
      <ref id="bib1.bib2"><label>2</label><?label 1?><mixed-citation>
Azzi, M., Johnson, G. M., and Cope, M.: An introduction to the generic
reaction set photochemical smog mechanism, in: Proceedings of the 8th
International Clean Air Conference, Clean Air Society of Australia &amp; New
Zealand (Ed.), 8th International Clean Air Conference, Melbourne, 6–11 May,
Melbourne, 1984.</mixed-citation></ref>
      <ref id="bib1.bib3"><label>3</label><?label 1?><mixed-citation>Beckx, C., Int Panis, L., Arentze, T., Janssens, D., Torfs, R., Broekx, S.,
and Wets, G.: A dynamic activity-based population modelling approach to
evaluate exposure to air pollution: Methods and application to a Dutch urban
area, Euro. Env. Imp. Assess., 29, 179–185,
<ext-link xlink:href="https://doi.org/10.1016/j.eiar.2008.10.001" ext-link-type="DOI">10.1016/j.eiar.2008.10.001</ext-link>, 2009.</mixed-citation></ref>
      <ref id="bib1.bib4"><label>4</label><?label 1?><mixed-citation>Bieser, J., Aulinger, A., Matthias, V., Quante, M., and Builtjes, P.: SMOKE for Europe – adaptation, modification and evaluation of a comprehensive emission model for Europe, Geosci. Model Dev., 4, 47–68, <ext-link xlink:href="https://doi.org/10.5194/gmd-4-47-2011" ext-link-type="DOI">10.5194/gmd-4-47-2011</ext-link>, 2011.</mixed-citation></ref>
      <ref id="bib1.bib5"><label>5</label><?label 1?><mixed-citation>Byun, D. and Schere, K. L.: Review of the Governing Equations, Computational
Algorithms, and Other Components of the Models-3 Community Multiscale Air
Quality (CMAQ) Modeling System, Appl. Mech. Rev., 59, 51–77,
<ext-link xlink:href="https://doi.org/10.1115/1.2128636" ext-link-type="DOI">10.1115/1.2128636</ext-link>, 2006.</mixed-citation></ref>
      <ref id="bib1.bib6"><label>6</label><?label 1?><mixed-citation>
Cofala, J., Amann, M., Borken-Kleefeld, J., Gomez-Sanabria, A., Heyes, C.,
Kiesewetter, G., Sander, R., Schoepp, W., Holland, M., Fagerli, H., and
Nyiri, A.: The potential for cost-effective air emission reductions from
international shipping through designation of further Emission Control Areas
in EU waters with focus on the Mediterranean Sea: IIASA Research Report,
International Institute for Applied Systems Analysis (IIASA), Laxenburg,
Austria, 2018.</mixed-citation></ref>
      <ref id="bib1.bib7"><label>7</label><?label 1?><mixed-citation>Corbett, J. J., Fischbeck, P. S., and Pandis, S. N.: Global nitrogen and
sulfur inventories for oceangoing ships, J. Geophys. Res., 104, 3457–3470,
<ext-link xlink:href="https://doi.org/10.1029/1998JD100040" ext-link-type="DOI">10.1029/1998JD100040</ext-link>, 1999.</mixed-citation></ref>
      <ref id="bib1.bib8"><label>8</label><?label 1?><mixed-citation>EU: DIRECTIVE 2005/33/EC OF THE EUROPEAN PARLIAMENT AND OF THE COUNCIL of 6
July 2005 amending Directive 1999/32/EC as regards the sulphur content of
marine fuels:
available at: <uri>https://eur-lex.europa.eu/LexUriServ/LexUriServ.do?uri=OJ:L:2005:191:0059:0069:EN:PDF</uri> (last access: 25 March 2020), 2005.</mixed-citation></ref>
      <ref id="bib1.bib9"><label>9</label><?label 1?><mixed-citation>EU: DIRECTIVE 2012/33/EC OF THE EUROPEAN PARLIAMENT AND OF THE COUNCIL of 21
November 2012 amending Directive 1999/32/EC as regards the sulphur content
of marine fuels:
available at: <uri>https://eur-lex.europa.eu/LexUriServ/LexUriServ.do?uri=OJ:L:2012:327:0001:0013:en:PDF</uri> (last access: 25 March 2020), 2012.</mixed-citation></ref>
      <ref id="bib1.bib10"><label>10</label><?label 1?><mixed-citation>Eyring, V., Isaksen, I. S. A., Berntsen, T., Collins, W. J., Corbett, J. J.,
Endresen, O., Grainger, R. G., Moldanova, J., Schlager, H., and Stevenson,
D. S.: Transport impacts on atmosphere and climate: Shipping, Atmos.
Environ., 44, 4735–4771, <ext-link xlink:href="https://doi.org/10.1016/j.atmosenv.2009.04.059" ext-link-type="DOI">10.1016/j.atmosenv.2009.04.059</ext-link>, 2010.</mixed-citation></ref>
      <ref id="bib1.bib11"><label>11</label><?label 1?><mixed-citation>Fridell, E. and Salo, K.: Measurements of abatement of particles and exhaust
gases in a marine gas scrubber, Proc. IMechE, 230, 154–162,
<ext-link xlink:href="https://doi.org/10.1177/1475090214543716" ext-link-type="DOI">10.1177/1475090214543716</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib12"><label>12</label><?label 1?><mixed-citation>Fridell, E., Haeger-Eugensson, M., Moldanova, J., Forsberg, B., and
Sjöberg, K.: A modelling study of the impact on air quality and health
due to the emissions from E85 and petrol fuelled cars in Sweden, Atmos.
Environ., 82, 1–8, <ext-link xlink:href="https://doi.org/10.1016/j.atmosenv.2013.10.002" ext-link-type="DOI">10.1016/j.atmosenv.2013.10.002</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bib13"><label>13</label><?label 1?><mixed-citation>Fridell, E., Winnes, H., Parsmo, R., Boteler, B., Troeltzsch, J., Kowalczyk,
U., Piotrowicz, J., Jalkanen, J.-P., Johansson, L., Matthias, V., and
Ytreberg, E.: Sustainable Shipping and Environment of the Baltic Sea Region
(SHEBA) Deliverable 1.4, type RE: Future Scenarios:
available at: <uri>https://www.sheba-project.eu/imperia/md/content/sheba/deliverables/sheba_d1.4_final.pdf</uri> (last access: 7 September 2020), 2015.</mixed-citation></ref>
      <ref id="bib1.bib14"><label>14</label><?label 1?><mixed-citation>Gallego, E., Roca, F. J., Perales, J. F., Guardino, X., Gadea, E., and
Garrote, P.: Impact of formaldehyde and VOCs from waste treatment plants
upon the ambient air nearby an urban area (Spain), The Sci. Total
Environ., 568, 369–380, <ext-link xlink:href="https://doi.org/10.1016/j.scitotenv.2016.06.007" ext-link-type="DOI">10.1016/j.scitotenv.2016.06.007</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib15"><label>15</label><?label 1?><mixed-citation>Geyer, B.: High-resolution atmospheric reconstruction for Europe 1948–2012: coastDat2, Earth Syst. Sci. Data, 6, 147–164, <ext-link xlink:href="https://doi.org/10.5194/essd-6-147-2014" ext-link-type="DOI">10.5194/essd-6-147-2014</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bib16"><label>16</label><?label 1?><mixed-citation>
Heroux, M. E., Braubach, M., Korol, N., Krzyzanowski, M., Paunovic, E., and
Zastenskaya, I.: The main conclusions about the medical aspects of air
pollution: The projects REVIHAAP and HRAPIE WHO/EC, Gigiena i sanitariia,
9–14, 2013.</mixed-citation></ref>
      <ref id="bib1.bib17"><label>17</label><?label 1?><mixed-citation>
Holland, M. R., Pye, S., and Jones, G.: EC4MACS Modelling Methodology – The
ALPHA Benefit Assessment Model, 2013.</mixed-citation></ref>
      <ref id="bib1.bib18"><label>18</label><?label 1?><mixed-citation>Hurley, P. J., Physick, W. L., and Luhar, A. K.: TAPM: A practical approach
to prognostic meteorological and air pollution modelling, Environ.
Modell. Softw., 20, 737–752, <ext-link xlink:href="https://doi.org/10.1016/j.envsoft.2004.04.006" ext-link-type="DOI">10.1016/j.envsoft.2004.04.006</ext-link>,
2005.</mixed-citation></ref>
      <ref id="bib1.bib19"><label>19</label><?label 1?><mixed-citation>IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto (Revised MARPOL Annex
VI): Resolution MEPC 176 (58), availble at:
<uri>http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.176(58).pdf</uri>
(last access: 25 March 2020), 2008.</mixed-citation></ref>
      <ref id="bib1.bib20"><label>20</label><?label 1?><mixed-citation>IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto. (Inclusion of
regulations on energy efficiency for ships in MARPOL Annex VI),
available at: <uri>http://www.imo.org/en/OurWork/Environment/PollutionPrevention/AirPollution/Documents/Technical and Operational Measures/Resolution MEPC.203(62).pdf</uri>
(last access: 25 March 2020), 2011.</mixed-citation></ref>
      <ref id="bib1.bib21"><label>21</label><?label 1?><mixed-citation>IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto. (Amendments to
regulations 2, 13, 19, 20 and 21 and the Supplement to the IAPP Certificate
under MARPOL Annex VI and certification of dual-fuel engines under the NOX
Technical Code 2008): Resolution MEPC 251(66):
available at: <uri>http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.251(66).pdf</uri>
(last access: 25 March 2020), 2014.</mixed-citation></ref>
      <ref id="bib1.bib22"><label>22</label><?label 1?><mixed-citation>IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto. (Designation of the
Baltic Sea and the North Sea Emission Control Areas for NOX Tier III
control): Resolution MEPC 286(71),
available at: <uri>http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.286(71).pdf</uri>
(last access: 25 March 2020), 2017.</mixed-citation></ref>
      <ref id="bib1.bib23"><label>23</label><?label 1?><mixed-citation>IMO: Initial IMO strategy on reduction of GHG emissions from ships:
Resolution MEPC 304(72):
available at: <uri>http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.304(72).pdf</uri>
(last access: 25 March 2020), 2018.</mixed-citation></ref>
      <ref id="bib1.bib24"><label>24</label><?label 1?><mixed-citation>Jalkanen, J.-P., Brink, A., Kalli, J., Pettersson, H., Kukkonen, J., and Stipa, T.: A modelling system for the exhaust emissions of marine traffic and its application in the Baltic Sea area, Atmos. Chem. Phys., 9, 9209–9223, <ext-link xlink:href="https://doi.org/10.5194/acp-9-9209-2009" ext-link-type="DOI">10.5194/acp-9-9209-2009</ext-link>, 2009.</mixed-citation></ref>
      <?pagebreak page10686?><ref id="bib1.bib25"><label>25</label><?label 1?><mixed-citation>Jalkanen, J.-P., Johansson, L., Kukkonen, J., Brink, A., Kalli, J., and Stipa, T.: Extension of an assessment model of ship traffic exhaust emissions for particulate matter and carbon monoxide, Atmos. Chem. Phys., 12, 2641–2659, <ext-link xlink:href="https://doi.org/10.5194/acp-12-2641-2012" ext-link-type="DOI">10.5194/acp-12-2641-2012</ext-link>, 2012.</mixed-citation></ref>
      <ref id="bib1.bib26"><label>26</label><?label 1?><mixed-citation>Johansson, L., Jalkanen, J.-P., Kalli, J., and Kukkonen, J.: The evolution of shipping emissions and the costs of regulation changes in the northern EU area, Atmos. Chem. Phys., 13, 11375–11389, <ext-link xlink:href="https://doi.org/10.5194/acp-13-11375-2013" ext-link-type="DOI">10.5194/acp-13-11375-2013</ext-link>, 2013.</mixed-citation></ref>
      <ref id="bib1.bib27"><label>27</label><?label 1?><mixed-citation>Jonson, J. E., Jalkanen, J. P., Johansson, L., Gauss, M., and Denier van der Gon, H. A. C.: Model calculations of the effects of present and future emissions of air pollutants from shipping in the Baltic Sea and the North Sea, Atmos. Chem. Phys., 15, 783–798, <ext-link xlink:href="https://doi.org/10.5194/acp-15-783-2015" ext-link-type="DOI">10.5194/acp-15-783-2015</ext-link>, 2015.
 </mixed-citation></ref>
      <ref id="bib1.bib28"><label>28</label><?label 1?><mixed-citation>Jonson, J. E., Gauss, M., Jalkanen, J.-P., and Johansson, L.: Effects of strengthening the Baltic Sea ECA regulations, Atmos. Chem. Phys., 19, 13469–13487, <ext-link xlink:href="https://doi.org/10.5194/acp-19-13469-2019" ext-link-type="DOI">10.5194/acp-19-13469-2019</ext-link>, 2019.</mixed-citation></ref>
      <ref id="bib1.bib29"><label>29</label><?label 1?><mixed-citation>Kalli, J., Jalkanen, J.-P., Johansson, L., and Repka, S.: Atmospheric
emissions of European SECA shipping: long-term projections, WMU J. Marit.
Affairs, 12, 129–145, <ext-link xlink:href="https://doi.org/10.1007/s13437-013-0050-9" ext-link-type="DOI">10.1007/s13437-013-0050-9</ext-link>, 2013.</mixed-citation></ref>
      <ref id="bib1.bib30"><label>30</label><?label 1?><mixed-citation>Karl, M., Bieser, J., Geyer, B., Matthias, V., Jalkanen, J.-P., Johansson, L., and Fridell, E.: Impact of a nitrogen emission control area (NECA) on the future air quality and nitrogen deposition to seawater in the Baltic Sea region, Atmos. Chem. Phys., 19, 1721–1752, <ext-link xlink:href="https://doi.org/10.5194/acp-19-1721-2019" ext-link-type="DOI">10.5194/acp-19-1721-2019</ext-link>, 2019a.</mixed-citation></ref>
      <ref id="bib1.bib31"><label>31</label><?label 1?><mixed-citation>Karl, M., Jonson, J. E., Uppstu, A., Aulinger, A., Prank, M., Sofiev, M., Jalkanen, J.-P., Johansson, L., Quante, M., and Matthias, V.: Effects of ship emissions on air quality in the Baltic Sea region simulated with three different chemistry transport models, Atmos. Chem. Phys., 19, 7019–7053, <ext-link xlink:href="https://doi.org/10.5194/acp-19-7019-2019" ext-link-type="DOI">10.5194/acp-19-7019-2019</ext-link>, 2019b.</mixed-citation></ref>
      <ref id="bib1.bib32"><label>32</label><?label 1?><mixed-citation>Keller, M., Hausberger, S., Matzer, C., Wüthrich, P., and Notter, B.:
HBEFA Version 3.3: Background Documentation,
available at: <uri>http://www.hbefa.net/e/documents/HBEFA33_Documentation_20170425.pdf</uri> (last access: 8 January 2020), 2017.</mixed-citation></ref>
      <ref id="bib1.bib33"><label>33</label><?label 1?><mixed-citation>Kiesewetter, G., Borken-Kleefeld, J., Schöpp, W., Heyes, C., Thunis, P., Bessagnet, B., Terrenoire, E., Gsella, A., and Amann, M.: Modelling <inline-formula><mml:math id="M473" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations at the street level in the GAINS integrated assessment model: projections under current legislation, Atmos. Chem. Phys., 14, 813–829, <ext-link xlink:href="https://doi.org/10.5194/acp-14-813-2014" ext-link-type="DOI">10.5194/acp-14-813-2014</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bib34"><label>34</label><?label 1?><mixed-citation>Matthaios, V. N., Triantafyllou, A. G., Albanis, T. A., Sakkas, V., and
Garas, S.: Performance and evaluation of a coupled prognostic model TAPM
over a mountainous complex terrain industrial area, Theor. Appl. Climatol.,
132, 885–903, <ext-link xlink:href="https://doi.org/10.1007/s00704-017-2122-9" ext-link-type="DOI">10.1007/s00704-017-2122-9</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bib35"><label>35</label><?label 1?><mixed-citation>Miljöförvaltningen: Luften i Göteborg: Årsrapport 2019, available at: <uri>https://goteborg.se/wps/wcm/connect/10808596-7471-4e9e-af8a-2f7f517140af/R+2020_12+Luften+i+G 6teborg+-+ rsrapport+2019.pdf?MOD=AJPERES</uri>,
last access: 29 June 2020.</mixed-citation></ref>
      <ref id="bib1.bib36"><label>36</label><?label 1?><mixed-citation>Ramacher, M. O. P. and Karl, M.: Integrating Modes of Transport in a Dynamic
Modelling Approach to Evaluate Population Exposure to Ambient <inline-formula><mml:math id="M474" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M475" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>
Pollution in Urban Areas, IJERPH, 17, 2099, 1–35, <ext-link xlink:href="https://doi.org/10.3390/ijerph17062099" ext-link-type="DOI">10.3390/ijerph17062099</ext-link>,
2020.</mixed-citation></ref>
      <ref id="bib1.bib37"><label>37</label><?label 1?><mixed-citation>Ramacher, M. O. P., Karl, M., Bieser, J., Jalkanen, J.-P., and Johansson, L.: Urban population exposure to <inline-formula><mml:math id="M476" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions from local shipping in three Baltic Sea harbour cities – a generic approach, Atmos. Chem. Phys., 19, 9153–9179, <ext-link xlink:href="https://doi.org/10.5194/acp-19-9153-2019" ext-link-type="DOI">10.5194/acp-19-9153-2019</ext-link>, 2019.</mixed-citation></ref>
      <ref id="bib1.bib38"><label>38</label><?label 1?><mixed-citation>
Ramacher, M. O. P., Karl, M., Aulinger, A., and Bieser, J.: Population
Exposure to Emissions from Industry, Traffic, Shipping and Residential
Heating in the Urban Area of Hamburg, in: Air Pollution Modeling and its
Application XXVI, edited by: Mensink, C., Gong, W., and Hakami, A.,  Springer
Proceedings in Complexity, Springer International Publishing, Cham,
177–183, 2020.</mixed-citation></ref>
      <ref id="bib1.bib39"><label>39</label><?label 1?><mixed-citation>Reis, S., Liška, T., Vieno, M., Carnell, E. J., Beck, R., Clemens, T.,
Dragosits, U., Tomlinson, S. J., Leaver, D., and Heal, M. R.: The influence
of residential and workday population mobility on exposure to air pollution
in the UK, Environ. Int., 121, 803–813,
<ext-link xlink:href="https://doi.org/10.1016/j.envint.2018.10.005" ext-link-type="DOI">10.1016/j.envint.2018.10.005</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bib40"><label>40</label><?label 1?><mixed-citation>Rockel, B., Will, A., and Hense, A.: The Regional Climate Model COSMO-CLM
(CCLM), Metz, 17, 347–348, <ext-link xlink:href="https://doi.org/10.1127/0941-2948/2008/0309" ext-link-type="DOI">10.1127/0941-2948/2008/0309</ext-link>, 2008.</mixed-citation></ref>
      <ref id="bib1.bib41"><label>41</label><?label 1?><mixed-citation>Sillman, S.: The relation between ozone, <inline-formula><mml:math id="M477" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and hydrocarbons in urban and
polluted rural environments, Atmos. Environ., 33, 1821–1845,
<ext-link xlink:href="https://doi.org/10.1016/S1352-2310(98)00345-8" ext-link-type="DOI">10.1016/S1352-2310(98)00345-8</ext-link>, 1999.</mixed-citation></ref>
      <ref id="bib1.bib42"><label>42</label><?label 1?><mixed-citation>Smith, J. D., Mitsakou, C., Kitwiroon, N., Barratt, B. M., Walton, H. A.,
Taylor, J. G., Anderson, H. R., Kelly, F. J., and Beevers, S. D.: London
Hybrid Exposure Model: Improving Human Exposure Estimates to <inline-formula><mml:math id="M478" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and PM<inline-formula><mml:math id="M479" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>
in an Urban Setting, Environ. Sci. Technol., 50,
11760–11768, <ext-link xlink:href="https://doi.org/10.1021/acs.est.6b01817" ext-link-type="DOI">10.1021/acs.est.6b01817</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib43"><label>43</label><?label 1?><mixed-citation>Soares, J., Kousa, A., Kukkonen, J., Matilainen, L., Kangas, L., Kauhaniemi, M., Riikonen, K., Jalkanen, J.-P., Rasila, T., Hänninen, O., Koskentalo, T., Aarnio, M., Hendriks, C., and Karppinen, A.: Refinement of a model for evaluating the population exposure in an urban area, Geosci. Model Dev., 7, 1855–1872, <ext-link xlink:href="https://doi.org/10.5194/gmd-7-1855-2014" ext-link-type="DOI">10.5194/gmd-7-1855-2014</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bib44"><label>44</label><?label 1?><mixed-citation>Sofiev, M., Winebrake, J. J., Johansson, L., Carr, E. W., Prank, M., Soares,
J., Vira, J., Kouznetsov, R., Jalkanen, J.-P., and Corbett, J. J.: Cleaner
fuels for ships provide public health benefits with climate tradeoffs,
Nat. Commun., 9, 406, 1–12, <ext-link xlink:href="https://doi.org/10.1038/s41467-017-02774-9" ext-link-type="DOI">10.1038/s41467-017-02774-9</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bib45"><label>45</label><?label 1?><mixed-citation>Tang, L., Ramacher, M. O. P., Moldanová, J., Matthias, V., Karl, M., Johansson, L., Jalkanen, J.-P., Yaramenka, K., Aulinger, A., and Gustafsson, M.: The impact of ship emissions on air quality and human health in the Gothenburg area – Part 1: 2012 emissions, Atmos. Chem. Phys., 20, 7509–7530, <ext-link xlink:href="https://doi.org/10.5194/acp-20-7509-2020" ext-link-type="DOI">10.5194/acp-20-7509-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib46"><label>46</label><?label 1?><mixed-citation>
Transport administration: Prognos för persontrafiken 2040: Trafikverkets
Basprognoser 2016, Report 2016:062, Transport administration (Trafikverket),
2016.</mixed-citation></ref>
      <ref id="bib1.bib47"><label>47</label><?label 1?><mixed-citation>
Transport administration: Prognos för persontrafiken 2040: Trafikverkets
Basprognoser 2018-04-01, Report 2018:089, Transport administration
(Trafikverket), 2018.</mixed-citation></ref>
      <ref id="bib1.bib48"><label>48</label><?label 1?><mixed-citation>Zandersen, M., Hyytiäinen, K., Meier, H. E. M., Tomczak, M. T., Bauer,
B., Haapasaari, P. E., Olesen, J. E., Gustafsson, B. G., Refsgaard, J. C.,
Fridell, E., Pihlainen, S., Le Tissier, M. D. A., Kosenius, A.-K., and van
Vuuren, D. P.: Shared socio-economic pathways extended for the Baltic Sea:
exploring long-term environmental problems, Reg. Environ. Change, 19,
1073–1086, <ext-link xlink:href="https://doi.org/10.1007/s10113-018-1453-0" ext-link-type="DOI">10.1007/s10113-018-1453-0</ext-link>, 2019.</mixed-citation></ref>

  </ref-list></back>
    <!--<article-title-html>The impact of ship emissions on air quality and human health in the Gothenburg area – Part II: Scenarios for 2040</article-title-html>
<abstract-html><p>Shipping is an important source of air pollutants, from
the global to the local scale. Ships emit substantial amounts of
sulfur dioxides, nitrogen dioxides, and particulate matter in the vicinity
of coasts, threatening the health of the coastal population, especially in
harbour cities. Reductions in emissions due to shipping have been targeted
by several regulations. Nevertheless, effects of these regulations come into
force with temporal delays, global ship traffic is expected to grow in the
future, and other land-based anthropogenic emissions might decrease. Thus,
it is necessary to investigate combined impacts to identify the impact of
shipping activities on air quality, population exposure, and health effects
in the future.</p><p>We investigated the future effect of shipping emissions on air quality and
related health effects considering different scenarios of the development of
shipping under current regional trends of economic growth and already
decided regulations in the Gothenburg urban area in 2040. Additionally, we
investigated the impact of a large-scale implementation of shore electricity
in the Port of Gothenburg. For this purpose, we established a one-way nested
chemistry transport modelling (CTM) system from the global to the urban
scale, to calculate pollutant concentrations, population-weighted
concentrations, and health effects related to NO<sub>2</sub>, PM<sub>2.5</sub>, and O<sub>3</sub>.</p><p>The simulated concentrations of NO<sub>2</sub> and PM<sub>2.5</sub> in future scenarios
for the year 2040 are in general very low with up to 4&thinsp;ppb for NO<sub>2</sub> and
up to 3.5&thinsp;µg&thinsp;m<sup>−3</sup> PM<sub>2.5</sub> in the urban areas which
are not close to the port area. From 2012 the simulated overall exposure to
PM<sub>2.5</sub> decreased by approximately 30&thinsp;% in simulated future scenarios;
for NO<sub>2</sub> the decrease was over 60&thinsp;%. The simulated concentrations of
O<sub>3</sub> increased from the year 2012 to 2040 by about 20&thinsp;%. In general, the
contributions of local shipping emissions in 2040 focus on the harbour area
but to some extent also influence the rest of the city domain. The simulated
impact of onshore electricity implementation for shipping in 2040 shows
reductions for NO<sub>2</sub> in the port of up to 30&thinsp;%, while increasing
O<sub>3</sub> of up to 3&thinsp;%. Implementation of onshore electricity for ships at
berth leads to additional local reduction potentials of up to 3&thinsp;% for
PM<sub>2.5</sub> and 12&thinsp;% for SO<sub>2</sub> in the port area. All future scenarios
show substantial decreases in population-weighted exposure and health-effect
impacts.</p></abstract-html>
<ref-html id="bib1.bib1"><label>1</label><mixed-citation>
Amman, M., Cofala, J., Heyes, C., Klimont, Z., Mechler, R., Posch, M., and
Schöpp, W.: The RAINS model: Documentation of the model approach
prepared for the RAINS peer review 2004, Interim Report IR-04-075, available at: <a href="http://pure.iiasa.ac.at/id/eprint/7307/1/IR-04-075.pdf" target="_blank"/>, last access: 8 January 2020, 2004.
</mixed-citation></ref-html>
<ref-html id="bib1.bib2"><label>2</label><mixed-citation>
Azzi, M., Johnson, G. M., and Cope, M.: An introduction to the generic
reaction set photochemical smog mechanism, in: Proceedings of the 8th
International Clean Air Conference, Clean Air Society of Australia &amp; New
Zealand (Ed.), 8th International Clean Air Conference, Melbourne, 6–11 May,
Melbourne, 1984.
</mixed-citation></ref-html>
<ref-html id="bib1.bib3"><label>3</label><mixed-citation>
Beckx, C., Int Panis, L., Arentze, T., Janssens, D., Torfs, R., Broekx, S.,
and Wets, G.: A dynamic activity-based population modelling approach to
evaluate exposure to air pollution: Methods and application to a Dutch urban
area, Euro. Env. Imp. Assess., 29, 179–185,
<a href="https://doi.org/10.1016/j.eiar.2008.10.001" target="_blank">https://doi.org/10.1016/j.eiar.2008.10.001</a>, 2009.
</mixed-citation></ref-html>
<ref-html id="bib1.bib4"><label>4</label><mixed-citation>
Bieser, J., Aulinger, A., Matthias, V., Quante, M., and Builtjes, P.: SMOKE for Europe – adaptation, modification and evaluation of a comprehensive emission model for Europe, Geosci. Model Dev., 4, 47–68, <a href="https://doi.org/10.5194/gmd-4-47-2011" target="_blank">https://doi.org/10.5194/gmd-4-47-2011</a>, 2011.
</mixed-citation></ref-html>
<ref-html id="bib1.bib5"><label>5</label><mixed-citation>
Byun, D. and Schere, K. L.: Review of the Governing Equations, Computational
Algorithms, and Other Components of the Models-3 Community Multiscale Air
Quality (CMAQ) Modeling System, Appl. Mech. Rev., 59, 51–77,
<a href="https://doi.org/10.1115/1.2128636" target="_blank">https://doi.org/10.1115/1.2128636</a>, 2006.
</mixed-citation></ref-html>
<ref-html id="bib1.bib6"><label>6</label><mixed-citation>
Cofala, J., Amann, M., Borken-Kleefeld, J., Gomez-Sanabria, A., Heyes, C.,
Kiesewetter, G., Sander, R., Schoepp, W., Holland, M., Fagerli, H., and
Nyiri, A.: The potential for cost-effective air emission reductions from
international shipping through designation of further Emission Control Areas
in EU waters with focus on the Mediterranean Sea: IIASA Research Report,
International Institute for Applied Systems Analysis (IIASA), Laxenburg,
Austria, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib7"><label>7</label><mixed-citation>
Corbett, J. J., Fischbeck, P. S., and Pandis, S. N.: Global nitrogen and
sulfur inventories for oceangoing ships, J. Geophys. Res., 104, 3457–3470,
<a href="https://doi.org/10.1029/1998JD100040" target="_blank">https://doi.org/10.1029/1998JD100040</a>, 1999.
</mixed-citation></ref-html>
<ref-html id="bib1.bib8"><label>8</label><mixed-citation>
EU: DIRECTIVE 2005/33/EC OF THE EUROPEAN PARLIAMENT AND OF THE COUNCIL of 6
July 2005 amending Directive 1999/32/EC as regards the sulphur content of
marine fuels:
available at: <a href="https://eur-lex.europa.eu/LexUriServ/LexUriServ.do?uri=OJ:L:2005:191:0059:0069:EN:PDF" target="_blank"/> (last access: 25 March 2020), 2005.
</mixed-citation></ref-html>
<ref-html id="bib1.bib9"><label>9</label><mixed-citation>
EU: DIRECTIVE 2012/33/EC OF THE EUROPEAN PARLIAMENT AND OF THE COUNCIL of 21
November 2012 amending Directive 1999/32/EC as regards the sulphur content
of marine fuels:
available at: <a href="https://eur-lex.europa.eu/LexUriServ/LexUriServ.do?uri=OJ:L:2012:327:0001:0013:en:PDF" target="_blank"/> (last access: 25 March 2020), 2012.
</mixed-citation></ref-html>
<ref-html id="bib1.bib10"><label>10</label><mixed-citation>
Eyring, V., Isaksen, I. S. A., Berntsen, T., Collins, W. J., Corbett, J. J.,
Endresen, O., Grainger, R. G., Moldanova, J., Schlager, H., and Stevenson,
D. S.: Transport impacts on atmosphere and climate: Shipping, Atmos.
Environ., 44, 4735–4771, <a href="https://doi.org/10.1016/j.atmosenv.2009.04.059" target="_blank">https://doi.org/10.1016/j.atmosenv.2009.04.059</a>, 2010.
</mixed-citation></ref-html>
<ref-html id="bib1.bib11"><label>11</label><mixed-citation>
Fridell, E. and Salo, K.: Measurements of abatement of particles and exhaust
gases in a marine gas scrubber, Proc. IMechE, 230, 154–162,
<a href="https://doi.org/10.1177/1475090214543716" target="_blank">https://doi.org/10.1177/1475090214543716</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib12"><label>12</label><mixed-citation>
Fridell, E., Haeger-Eugensson, M., Moldanova, J., Forsberg, B., and
Sjöberg, K.: A modelling study of the impact on air quality and health
due to the emissions from E85 and petrol fuelled cars in Sweden, Atmos.
Environ., 82, 1–8, <a href="https://doi.org/10.1016/j.atmosenv.2013.10.002" target="_blank">https://doi.org/10.1016/j.atmosenv.2013.10.002</a>, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib13"><label>13</label><mixed-citation>
Fridell, E., Winnes, H., Parsmo, R., Boteler, B., Troeltzsch, J., Kowalczyk,
U., Piotrowicz, J., Jalkanen, J.-P., Johansson, L., Matthias, V., and
Ytreberg, E.: Sustainable Shipping and Environment of the Baltic Sea Region
(SHEBA) Deliverable 1.4, type RE: Future Scenarios:
available at: <a href="https://www.sheba-project.eu/imperia/md/content/sheba/deliverables/sheba_d1.4_final.pdf" target="_blank"/> (last access: 7 September 2020), 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib14"><label>14</label><mixed-citation>
Gallego, E., Roca, F. J., Perales, J. F., Guardino, X., Gadea, E., and
Garrote, P.: Impact of formaldehyde and VOCs from waste treatment plants
upon the ambient air nearby an urban area (Spain), The Sci. Total
Environ., 568, 369–380, <a href="https://doi.org/10.1016/j.scitotenv.2016.06.007" target="_blank">https://doi.org/10.1016/j.scitotenv.2016.06.007</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib15"><label>15</label><mixed-citation>
Geyer, B.: High-resolution atmospheric reconstruction for Europe 1948–2012: coastDat2, Earth Syst. Sci. Data, 6, 147–164, <a href="https://doi.org/10.5194/essd-6-147-2014" target="_blank">https://doi.org/10.5194/essd-6-147-2014</a>, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib16"><label>16</label><mixed-citation>
Heroux, M. E., Braubach, M., Korol, N., Krzyzanowski, M., Paunovic, E., and
Zastenskaya, I.: The main conclusions about the medical aspects of air
pollution: The projects REVIHAAP and HRAPIE WHO/EC, Gigiena i sanitariia,
9–14, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib17"><label>17</label><mixed-citation>
Holland, M. R., Pye, S., and Jones, G.: EC4MACS Modelling Methodology – The
ALPHA Benefit Assessment Model, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib18"><label>18</label><mixed-citation>
Hurley, P. J., Physick, W. L., and Luhar, A. K.: TAPM: A practical approach
to prognostic meteorological and air pollution modelling, Environ.
Modell. Softw., 20, 737–752, <a href="https://doi.org/10.1016/j.envsoft.2004.04.006" target="_blank">https://doi.org/10.1016/j.envsoft.2004.04.006</a>,
2005.
</mixed-citation></ref-html>
<ref-html id="bib1.bib19"><label>19</label><mixed-citation>
IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto (Revised MARPOL Annex
VI): Resolution MEPC 176 (58), availble at:
<a href="http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.176(58).pdf" target="_blank"/>
(last access: 25 March 2020), 2008.
</mixed-citation></ref-html>
<ref-html id="bib1.bib20"><label>20</label><mixed-citation>
IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto. (Inclusion of
regulations on energy efficiency for ships in MARPOL Annex VI),
available at: <a href="http://www.imo.org/en/OurWork/Environment/PollutionPrevention/AirPollution/Documents/Technical and Operational Measures/Resolution MEPC.203(62).pdf" target="_blank"/>
(last access: 25 March 2020), 2011.
</mixed-citation></ref-html>
<ref-html id="bib1.bib21"><label>21</label><mixed-citation>
IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto. (Amendments to
regulations 2, 13, 19, 20 and 21 and the Supplement to the IAPP Certificate
under MARPOL Annex VI and certification of dual-fuel engines under the NOX
Technical Code 2008): Resolution MEPC 251(66):
available at: <a href="http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.251(66).pdf" target="_blank"/>
(last access: 25 March 2020), 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib22"><label>22</label><mixed-citation>
IMO: Amendments to the Annex of the Protocol of 1997 to Amend the
International Convention for the Prevention of Pollution from Ships, 1973,
as Modified by the Protocol of 1978 Relating thereto. (Designation of the
Baltic Sea and the North Sea Emission Control Areas for NOX Tier III
control): Resolution MEPC 286(71),
available at: <a href="http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.286(71).pdf" target="_blank"/>
(last access: 25 March 2020), 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib23"><label>23</label><mixed-citation>
IMO: Initial IMO strategy on reduction of GHG emissions from ships:
Resolution MEPC 304(72):
available at: <a href="http://www.imo.org/en/KnowledgeCentre/IndexofIMOResolutions/Marine-Environment-Protection-Committee-(MEPC)/Documents/MEPC.304(72).pdf" target="_blank"/>
(last access: 25 March 2020), 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib24"><label>24</label><mixed-citation>
Jalkanen, J.-P., Brink, A., Kalli, J., Pettersson, H., Kukkonen, J., and Stipa, T.: A modelling system for the exhaust emissions of marine traffic and its application in the Baltic Sea area, Atmos. Chem. Phys., 9, 9209–9223, <a href="https://doi.org/10.5194/acp-9-9209-2009" target="_blank">https://doi.org/10.5194/acp-9-9209-2009</a>, 2009.
</mixed-citation></ref-html>
<ref-html id="bib1.bib25"><label>25</label><mixed-citation>
Jalkanen, J.-P., Johansson, L., Kukkonen, J., Brink, A., Kalli, J., and Stipa, T.: Extension of an assessment model of ship traffic exhaust emissions for particulate matter and carbon monoxide, Atmos. Chem. Phys., 12, 2641–2659, <a href="https://doi.org/10.5194/acp-12-2641-2012" target="_blank">https://doi.org/10.5194/acp-12-2641-2012</a>, 2012.
</mixed-citation></ref-html>
<ref-html id="bib1.bib26"><label>26</label><mixed-citation>
Johansson, L., Jalkanen, J.-P., Kalli, J., and Kukkonen, J.: The evolution of shipping emissions and the costs of regulation changes in the northern EU area, Atmos. Chem. Phys., 13, 11375–11389, <a href="https://doi.org/10.5194/acp-13-11375-2013" target="_blank">https://doi.org/10.5194/acp-13-11375-2013</a>, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib27"><label>27</label><mixed-citation>
Jonson, J. E., Jalkanen, J. P., Johansson, L., Gauss, M., and Denier van der Gon, H. A. C.: Model calculations of the effects of present and future emissions of air pollutants from shipping in the Baltic Sea and the North Sea, Atmos. Chem. Phys., 15, 783–798, <a href="https://doi.org/10.5194/acp-15-783-2015" target="_blank">https://doi.org/10.5194/acp-15-783-2015</a>, 2015.
 </mixed-citation></ref-html>
<ref-html id="bib1.bib28"><label>28</label><mixed-citation>
Jonson, J. E., Gauss, M., Jalkanen, J.-P., and Johansson, L.: Effects of strengthening the Baltic Sea ECA regulations, Atmos. Chem. Phys., 19, 13469–13487, <a href="https://doi.org/10.5194/acp-19-13469-2019" target="_blank">https://doi.org/10.5194/acp-19-13469-2019</a>, 2019.
</mixed-citation></ref-html>
<ref-html id="bib1.bib29"><label>29</label><mixed-citation>
Kalli, J., Jalkanen, J.-P., Johansson, L., and Repka, S.: Atmospheric
emissions of European SECA shipping: long-term projections, WMU J. Marit.
Affairs, 12, 129–145, <a href="https://doi.org/10.1007/s13437-013-0050-9" target="_blank">https://doi.org/10.1007/s13437-013-0050-9</a>, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib30"><label>30</label><mixed-citation>
Karl, M., Bieser, J., Geyer, B., Matthias, V., Jalkanen, J.-P., Johansson, L., and Fridell, E.: Impact of a nitrogen emission control area (NECA) on the future air quality and nitrogen deposition to seawater in the Baltic Sea region, Atmos. Chem. Phys., 19, 1721–1752, <a href="https://doi.org/10.5194/acp-19-1721-2019" target="_blank">https://doi.org/10.5194/acp-19-1721-2019</a>, 2019a.
</mixed-citation></ref-html>
<ref-html id="bib1.bib31"><label>31</label><mixed-citation>
Karl, M., Jonson, J. E., Uppstu, A., Aulinger, A., Prank, M., Sofiev, M., Jalkanen, J.-P., Johansson, L., Quante, M., and Matthias, V.: Effects of ship emissions on air quality in the Baltic Sea region simulated with three different chemistry transport models, Atmos. Chem. Phys., 19, 7019–7053, <a href="https://doi.org/10.5194/acp-19-7019-2019" target="_blank">https://doi.org/10.5194/acp-19-7019-2019</a>, 2019b.
</mixed-citation></ref-html>
<ref-html id="bib1.bib32"><label>32</label><mixed-citation>
Keller, M., Hausberger, S., Matzer, C., Wüthrich, P., and Notter, B.:
HBEFA Version 3.3: Background Documentation,
available at: <a href="http://www.hbefa.net/e/documents/HBEFA33_Documentation_20170425.pdf" target="_blank"/> (last access: 8 January 2020), 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib33"><label>33</label><mixed-citation>
Kiesewetter, G., Borken-Kleefeld, J., Schöpp, W., Heyes, C., Thunis, P., Bessagnet, B., Terrenoire, E., Gsella, A., and Amann, M.: Modelling NO<sub>2</sub> concentrations at the street level in the GAINS integrated assessment model: projections under current legislation, Atmos. Chem. Phys., 14, 813–829, <a href="https://doi.org/10.5194/acp-14-813-2014" target="_blank">https://doi.org/10.5194/acp-14-813-2014</a>, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib34"><label>34</label><mixed-citation>
Matthaios, V. N., Triantafyllou, A. G., Albanis, T. A., Sakkas, V., and
Garas, S.: Performance and evaluation of a coupled prognostic model TAPM
over a mountainous complex terrain industrial area, Theor. Appl. Climatol.,
132, 885–903, <a href="https://doi.org/10.1007/s00704-017-2122-9" target="_blank">https://doi.org/10.1007/s00704-017-2122-9</a>, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib35"><label>35</label><mixed-citation>
Miljöförvaltningen: Luften i Göteborg: Årsrapport 2019, available at: <a href="https://goteborg.se/wps/wcm/connect/10808596-7471-4e9e-af8a-2f7f517140af/R+2020_12+Luften+i+G 6teborg+-+ rsrapport+2019.pdf?MOD=AJPERES" target="_blank"/>,
last access: 29 June 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib36"><label>36</label><mixed-citation>
Ramacher, M. O. P. and Karl, M.: Integrating Modes of Transport in a Dynamic
Modelling Approach to Evaluate Population Exposure to Ambient NO<sub>2</sub> and PM<sub>2.5</sub>
Pollution in Urban Areas, IJERPH, 17, 2099, 1–35, <a href="https://doi.org/10.3390/ijerph17062099" target="_blank">https://doi.org/10.3390/ijerph17062099</a>,
2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib37"><label>37</label><mixed-citation>
Ramacher, M. O. P., Karl, M., Bieser, J., Jalkanen, J.-P., and Johansson, L.: Urban population exposure to NO<sub><i>x</i></sub> emissions from local shipping in three Baltic Sea harbour cities – a generic approach, Atmos. Chem. Phys., 19, 9153–9179, <a href="https://doi.org/10.5194/acp-19-9153-2019" target="_blank">https://doi.org/10.5194/acp-19-9153-2019</a>, 2019.
</mixed-citation></ref-html>
<ref-html id="bib1.bib38"><label>38</label><mixed-citation>
Ramacher, M. O. P., Karl, M., Aulinger, A., and Bieser, J.: Population
Exposure to Emissions from Industry, Traffic, Shipping and Residential
Heating in the Urban Area of Hamburg, in: Air Pollution Modeling and its
Application XXVI, edited by: Mensink, C., Gong, W., and Hakami, A.,  Springer
Proceedings in Complexity, Springer International Publishing, Cham,
177–183, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib39"><label>39</label><mixed-citation>
Reis, S., Liška, T., Vieno, M., Carnell, E. J., Beck, R., Clemens, T.,
Dragosits, U., Tomlinson, S. J., Leaver, D., and Heal, M. R.: The influence
of residential and workday population mobility on exposure to air pollution
in the UK, Environ. Int., 121, 803–813,
<a href="https://doi.org/10.1016/j.envint.2018.10.005" target="_blank">https://doi.org/10.1016/j.envint.2018.10.005</a>, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib40"><label>40</label><mixed-citation>
Rockel, B., Will, A., and Hense, A.: The Regional Climate Model COSMO-CLM
(CCLM), Metz, 17, 347–348, <a href="https://doi.org/10.1127/0941-2948/2008/0309" target="_blank">https://doi.org/10.1127/0941-2948/2008/0309</a>, 2008.
</mixed-citation></ref-html>
<ref-html id="bib1.bib41"><label>41</label><mixed-citation>
Sillman, S.: The relation between ozone, NO<sub><i>x</i></sub> and hydrocarbons in urban and
polluted rural environments, Atmos. Environ., 33, 1821–1845,
<a href="https://doi.org/10.1016/S1352-2310(98)00345-8" target="_blank">https://doi.org/10.1016/S1352-2310(98)00345-8</a>, 1999.
</mixed-citation></ref-html>
<ref-html id="bib1.bib42"><label>42</label><mixed-citation>
Smith, J. D., Mitsakou, C., Kitwiroon, N., Barratt, B. M., Walton, H. A.,
Taylor, J. G., Anderson, H. R., Kelly, F. J., and Beevers, S. D.: London
Hybrid Exposure Model: Improving Human Exposure Estimates to NO<sub>2</sub> and PM<sub>2.5</sub>
in an Urban Setting, Environ. Sci. Technol., 50,
11760–11768, <a href="https://doi.org/10.1021/acs.est.6b01817" target="_blank">https://doi.org/10.1021/acs.est.6b01817</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib43"><label>43</label><mixed-citation>
Soares, J., Kousa, A., Kukkonen, J., Matilainen, L., Kangas, L., Kauhaniemi, M., Riikonen, K., Jalkanen, J.-P., Rasila, T., Hänninen, O., Koskentalo, T., Aarnio, M., Hendriks, C., and Karppinen, A.: Refinement of a model for evaluating the population exposure in an urban area, Geosci. Model Dev., 7, 1855–1872, <a href="https://doi.org/10.5194/gmd-7-1855-2014" target="_blank">https://doi.org/10.5194/gmd-7-1855-2014</a>, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib44"><label>44</label><mixed-citation>
Sofiev, M., Winebrake, J. J., Johansson, L., Carr, E. W., Prank, M., Soares,
J., Vira, J., Kouznetsov, R., Jalkanen, J.-P., and Corbett, J. J.: Cleaner
fuels for ships provide public health benefits with climate tradeoffs,
Nat. Commun., 9, 406, 1–12, <a href="https://doi.org/10.1038/s41467-017-02774-9" target="_blank">https://doi.org/10.1038/s41467-017-02774-9</a>, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib45"><label>45</label><mixed-citation>
Tang, L., Ramacher, M. O. P., Moldanová, J., Matthias, V., Karl, M., Johansson, L., Jalkanen, J.-P., Yaramenka, K., Aulinger, A., and Gustafsson, M.: The impact of ship emissions on air quality and human health in the Gothenburg area – Part 1: 2012 emissions, Atmos. Chem. Phys., 20, 7509–7530, <a href="https://doi.org/10.5194/acp-20-7509-2020" target="_blank">https://doi.org/10.5194/acp-20-7509-2020</a>, 2020.
</mixed-citation></ref-html>
<ref-html id="bib1.bib46"><label>46</label><mixed-citation>
Transport administration: Prognos för persontrafiken 2040: Trafikverkets
Basprognoser 2016, Report 2016:062, Transport administration (Trafikverket),
2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib47"><label>47</label><mixed-citation>
Transport administration: Prognos för persontrafiken 2040: Trafikverkets
Basprognoser 2018-04-01, Report 2018:089, Transport administration
(Trafikverket), 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib48"><label>48</label><mixed-citation>
Zandersen, M., Hyytiäinen, K., Meier, H. E. M., Tomczak, M. T., Bauer,
B., Haapasaari, P. E., Olesen, J. E., Gustafsson, B. G., Refsgaard, J. C.,
Fridell, E., Pihlainen, S., Le Tissier, M. D. A., Kosenius, A.-K., and van
Vuuren, D. P.: Shared socio-economic pathways extended for the Baltic Sea:
exploring long-term environmental problems, Reg. Environ. Change, 19,
1073–1086, <a href="https://doi.org/10.1007/s10113-018-1453-0" target="_blank">https://doi.org/10.1007/s10113-018-1453-0</a>, 2019.
</mixed-citation></ref-html>--></article>
