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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-19-6085-2019</article-id><title-group><article-title>How robust are stratospheric age of air trends<?xmltex \hack{\break}?> from different reanalyses?</article-title><alt-title>Age of air from different reanalyses and methods</alt-title>
      </title-group><?xmltex \runningtitle{Age of air from different reanalyses and methods}?><?xmltex \runningauthor{F. Ploeger et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1 aff2">
          <name><surname>Ploeger</surname><given-names>Felix</given-names></name>
          <email>f.ploeger@fz-juelich.de</email>
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3">
          <name><surname>Legras</surname><given-names>Bernard</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-3756-7794</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Charlesworth</surname><given-names>Edward</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1323-8881</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Yan</surname><given-names>Xiaolu</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Diallo</surname><given-names>Mohamadou</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-0225-8120</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Konopka</surname><given-names>Paul</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4 aff6">
          <name><surname>Birner</surname><given-names>Thomas</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Tao</surname><given-names>Mengchu</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1071-5953</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff5">
          <name><surname>Engel</surname><given-names>Andreas</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-0557-3935</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Riese</surname><given-names>Martin</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-6398-6493</ext-link></contrib>
        <aff id="aff1"><label>1</label><institution>Institute for Energy and Climate Research: Stratosphere (IEK-7), Forschungszentrum Jülich, Jülich, Germany</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Laboratoire de Météorologie Dynamique, UMR8539, IPSL, UPMC/ENS/CNRS/Ecole Polytechnique, Paris, France</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>Meteorological Institute, Ludwig-Maximilians-Universität München, München, Germany</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt, Germany</institution>
        </aff>
        <aff id="aff6"><label>6</label><institution>Deutsches Zentrum für Luft- und Raumfahrt (DLR), Institut für Physik der Atmosphäre, Oberpfaffenhofen, Germany</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Felix Ploeger (f.ploeger@fz-juelich.de)</corresp></author-notes><pub-date><day>8</day><month>May</month><year>2019</year></pub-date>
      
      <volume>19</volume>
      <issue>9</issue>
      <fpage>6085</fpage><lpage>6105</lpage>
      <history>
        <date date-type="received"><day>9</day><month>December</month><year>2018</year></date>
           <date date-type="rev-request"><day>14</day><month>January</month><year>2019</year></date>
           <date date-type="rev-recd"><day>1</day><month>April</month><year>2019</year></date>
           <date date-type="accepted"><day>16</day><month>April</month><year>2019</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2019 Felix Ploeger et al.</copyright-statement>
        <copyright-year>2019</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019.html">This article is available from https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019.pdf</self-uri>
      <abstract><title>Abstract</title>
    <p id="d1e199">An accelerating Brewer–Dobson circulation (BDC) is a robust signal
of climate change in model predictions but has been questioned by
trace gas observations. We analyse the stratospheric mean age of air and
the full age spectrum as measures for the BDC and its trend. Age
of air is calculated using the Chemical Lagrangian Model of the
Stratosphere (CLaMS) driven by ERA-Interim, JRA-55 and MERRA-2
reanalysis data to assess the robustness of the representation of
the BDC in current generation meteorological reanalyses. We find
that the climatological mean age significantly depends on the
reanalysis, with JRA-55 showing the youngest and MERRA-2 the
oldest mean age. Consideration of the age spectrum indicates that
the older air for MERRA-2 is related to a stronger spectrum tail,
which is likely associated with weaker tropical upwelling and stronger
recirculation. Seasonality of stratospheric transport is robustly
represented in reanalyses, with similar mean age variations
and age spectrum peaks. Long-term changes from 1989 to 2015 turn
out to be similar for the reanalyses with mainly decreasing mean age
accompanied by a shift of the age spectrum peak towards shorter
transit times, resembling the forced response in climate model
simulations to increasing greenhouse gas concentrations. For the
shorter periods, 1989–2001 and 2002–2015, the age of air changes are
less robust. Only ERA-Interim shows the hemispheric dipole pattern
in age changes from 2002 to 2015 as viewed by recent satellite
observations. Consequently, the representation of decadal
variability of the BDC in current generation reanalyses appears less
robust and is a major uncertainty of modelling the BDC.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <?pagebreak page6086?><p id="d1e211">The global circulation of the stratosphere, known as the Brewer–Dobson
circulation <xref ref-type="bibr" rid="bib1.bibx12 bib1.bibx44" id="paren.1"/>, is a crucial factor
controlling the lower stratospheric composition of radiatively active
trace gases; therefore, it plays an important role in the Earth's
radiation budget and in climate. Hence, a realistic representation of
the BDC is a prerequisite for reliable climate model
predictions. However, current climate models and observations disagree
regarding long-term changes of the BDC
<xref ref-type="bibr" rid="bib1.bibx74" id="paren.2"><named-content content-type="pre">e.g.</named-content></xref>. Climate models simulate a strengthening
and accelerating circulation which is not evident from observations,
representing a major uncertainty in current model predictions
<xref ref-type="bibr" rid="bib1.bibx13" id="paren.3"><named-content content-type="pre">see</named-content><named-content content-type="post">for a recent review</named-content></xref>. The BDC is
characterised by the slow upwelling in the tropics from the
troposphere across the tropical tropopause layer (TTL) into the
stratosphere, followed by poleward motion in the stratosphere and
downwelling at middle and high latitudes. From the perspective of
tracer transport, the BDC includes a residual mean mass circulation and
additional two-way eddy mixing, which causes net transport of
tracers but not mass <xref ref-type="bibr" rid="bib1.bibx61" id="paren.4"><named-content content-type="pre">e.g.</named-content></xref>. The residual mean
mass circulation may be separated into two different main branches
<xref ref-type="bibr" rid="bib1.bibx8" id="paren.5"/>. On the one hand, a shallow circulation branch transports air masses
to middle latitude regions at lower levels above the tropopause within
a few months to about 2 years. A deep circulation branch, on the other hand,
causes transport deep into the stratosphere and downwelling at high
latitudes on a timescale of several years <xref ref-type="bibr" rid="bib1.bibx8" id="paren.6"/>. The
stratospheric BDC is mechanically driven by the transfer of momentum from
breaking atmospheric waves to the zonal flow
<xref ref-type="bibr" rid="bib1.bibx42 bib1.bibx44" id="paren.7"/>. The shallow circulation branch is
mainly driven by synoptic and planetary-scale waves, and the deep
branch is mainly driven by planetary waves propagating deep into the
stratosphere <xref ref-type="bibr" rid="bib1.bibx61" id="paren.8"><named-content content-type="pre">e.g.</named-content></xref>. Results from an idealised
model suggest that the strength of the shallow circulation branch is
largely controlled by the strength of wave sources in the troposphere
<xref ref-type="bibr" rid="bib1.bibx36" id="paren.9"/>. The strength of the deep circulation branch, in comparison,
appears to be largely controlled by the propagation conditions for waves in the stratosphere.</p>
      <p id="d1e252">As the BDC is a zonal mean circulation and related wind velocities are
small residuals, directly measuring the circulation is not possible
<xref ref-type="bibr" rid="bib1.bibx13" id="paren.10"><named-content content-type="pre">e.g.</named-content></xref>. A common measure of the BDC is the age
of air, which represents the timescale for transport through the stratosphere. By
definition, age of air measures the speed of the
circulation. Strictly, due to atmospheric mixing processes on a
multitude of scales, a stratospheric air parcel is not characterised by
a single transport timescale but by a transit time distribution. This
transit time distribution is termed the “age of air spectrum”
<xref ref-type="bibr" rid="bib1.bibx38" id="paren.11"/>. Commonly used reference surfaces for measuring the
transit time are the tropical tropopause or the tropical surface
<xref ref-type="bibr" rid="bib1.bibx75" id="paren.12"><named-content content-type="pre">e.g.</named-content></xref>. The first moment of the age spectrum
distribution, termed the “mean age of air”, can be estimated from
observations of specific trace gas species with linearly increasing
mixing ratios in the troposphere, as is approximately the case for
<inline-formula><mml:math id="M1" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and SF<inline-formula><mml:math id="M2" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx38" id="paren.13"/>. Similar to a tracer, the mean age is
affected by both the residual mean mass circulation and atmospheric
mixing processes <xref ref-type="bibr" rid="bib1.bibx56 bib1.bibx34" id="paren.14"><named-content content-type="pre">e.g.</named-content></xref>, which complicates an
unambiguous interpretation of mean age changes in terms of
processes. The full age spectrum allows for a clearer interpretation, but
its deduction from observations is much more challenging and usually
hinges on simplifying assumptions like the stationarity of the flow or a
specific parameterization of the age spectrum shape
<xref ref-type="bibr" rid="bib1.bibx4 bib1.bibx69" id="paren.15"><named-content content-type="pre">e.g.</named-content></xref>. Ongoing modelling studies
suggest promising new methods for deducing the age spectrum based on
either an improved parametric approach <xref ref-type="bibr" rid="bib1.bibx40" id="paren.16"/> or an
inversion approach <xref ref-type="bibr" rid="bib1.bibx62" id="paren.17"/>. However, applicability to measurement
data remains to be shown.</p>
      <p id="d1e308">The BDC is characterised by variability on very different timescales.
Seasonal variability in the BDC is caused by seasonality in
wave driving, which is stronger in boreal than austral winter due
to larger wave excitation by orography in the Northern Hemisphere
(NH). As a result, tropical upwelling and related extratropical
downwelling (in the NH) maximise in boreal winter
<xref ref-type="bibr" rid="bib1.bibx77" id="paren.18"><named-content content-type="pre">e.g.</named-content></xref>. On inter-annual timescales, the BDC is
significantly modulated by the stratospheric Quasi-Biennial
Oscillation (QBO) <xref ref-type="bibr" rid="bib1.bibx7" id="paren.19"><named-content content-type="pre">e.g.</named-content></xref>, by the El Niño–Southern Oscillation
(ENSO) <xref ref-type="bibr" rid="bib1.bibx15 bib1.bibx21" id="paren.20"><named-content content-type="pre">e.g.</named-content></xref> and
by stratospheric aerosol injected by volcanic eruptions
<xref ref-type="bibr" rid="bib1.bibx20" id="paren.21"><named-content content-type="pre">e.g.</named-content></xref>. In the long term, climate models simulate
a robust strengthening of the BDC with global warming, resulting in an increase of the
tropical upwelling mass flux as well as in a global decrease of
the stratospheric mean age of air over the last decades and into the
future <xref ref-type="bibr" rid="bib1.bibx14 bib1.bibx13" id="paren.22"><named-content content-type="pre">e.g.</named-content></xref>. In contrast,
estimates of the mean age of air from balloon observations of long-lived
trace gas species in the NH middle latitudes above about 24 km show
no significant long-term trend <xref ref-type="bibr" rid="bib1.bibx26" id="paren.23"/>. Additional recent
balloon measurements corroborate this result <xref ref-type="bibr" rid="bib1.bibx27" id="paren.24"/>. A
recent, improved analysis of the same balloon observations confirms
the insignificant (weakly positive) mean age trend above about 24 km,
but shows a negative mean age trend below this level <xref ref-type="bibr" rid="bib1.bibx66" id="paren.25"/>. Indications
of a negative mean age trend in the lowermost stratosphere around the
year 2000 have also been found from aircraft observations of mean age
<xref ref-type="bibr" rid="bib1.bibx11" id="paren.26"/>. Hence, in particular in the stratosphere above
about 24 km, climate models results are not consistent with observations
regarding trends in the BDC.</p>
      <p id="d1e349">The strengthening BDC trend in models is clearly related to greenhouse
gas-induced tropospheric warming. This warming strengthens the
subtropical jets, thereby shifting the critical levels for wave breaking
upwards and equatorwards and intensifying the mechanical forcing of the
BDC <xref ref-type="bibr" rid="bib1.bibx31 bib1.bibx70 bib1.bibx33" id="paren.27"><named-content content-type="pre">e.g.</named-content></xref>. A recent study by
<xref ref-type="bibr" rid="bib1.bibx57" id="text.28"/> indicates that the BDC trend is consistent
with the expansion of the troposphere and an associated upward shift
of the tropopause with climate change.</p>
      <?pagebreak page6087?><p id="d1e361">Concerning BDC changes over decadal periods, horizontal circulation
shifts in the latitudinal direction also cause important effects. This
has recently been shown for a southward circulation shift from
2002 to 2012 which likely caused a hemispheric dipole mean age change
pattern (the age increased in the NH and decreased in the SH) as observed by the
Michelson Interferometer for Passive Atmospheric Sounding (MIPAS)
satellite instrument <xref ref-type="bibr" rid="bib1.bibx72" id="paren.29"/>. Ensembles of climate model
simulations may include mean age change patterns which are more
complex than a global decrease and even have some resemblance to MIPAS
observations <xref ref-type="bibr" rid="bib1.bibx32" id="paren.30"/>. Hence, to simulate observed past
BDC changes it is important to correctly represent variability on
inter-annual to decadal timescales in the models. For interpreting
mean age trends, the consideration of atmospheric mixing processes turns
out to be particularly important
<xref ref-type="bibr" rid="bib1.bibx67 bib1.bibx59 bib1.bibx22" id="paren.31"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d1e375">Meteorological reanalyses combine a global weather forecast model with
atmospheric observations through a data assimilation system to provide an
optimal estimate of the atmospheric state from the past to present. These
reanalyses are based on an unchanged forecast model version and assimilation
system to minimise artificial changes in the state variables due to changes
in the reanalysis system. However, as the observational data sets included in
the assimilation change over time, abrupt state changes may still occur to
some degree, rendering reanalysis-based trend studies challenging.
Considering more than one reanalysis in such studies increases the
reliability of results considerably. The Stratosphere-troposphere Processes
And their Role in Climate (SPARC) Reanalysis Intercomparison Project
(S-RIP) aims at an inter-comparison of the current generation reanalysis
products, as described by <xref ref-type="bibr" rid="bib1.bibx30" id="text.32"/>. The present paper contributes
to this project by comparing the representation of the stratospheric BDC in
the three most modern reanalysis products: (i) ERA-Interim from the European
Centre for Medium-Range Weather Forecasts (ECMWF), (ii) JRA-55 from the
Japanese Meteorological Agency and (iii) MERRA-2 from the National
Aeronautics and Space Administration (NASA).</p>
      <p id="d1e381">Past analyses have shown that modern reanalyses provide an improved
representation of the BDC <xref ref-type="bibr" rid="bib1.bibx19 bib1.bibx55" id="paren.33"><named-content content-type="pre">e.g.</named-content></xref>
compared with older reanalysis products like the ECMWF's ERA-40 reanalysis
<xref ref-type="bibr" rid="bib1.bibx54" id="paren.34"><named-content content-type="pre">e.g.</named-content></xref>. In particular, ERA-Interim has been
shown to combine a negative mean age trend throughout most regions of
the stratosphere with a weakly positive age trend in the NH above
about 24 km, similar to existing balloon observations
<xref ref-type="bibr" rid="bib1.bibx59" id="paren.35"/>. Moreover, the hemispheric dipole age trend
pattern as observed by MIPAS from 2002 to 2012 turns out to be
reproduced, at least qualitatively, by ERA-Interim-driven simulations
<xref ref-type="bibr" rid="bib1.bibx60" id="paren.36"/>. However, the robustness of these results concerning the
representation of the BDC in different reanalyses is an open question.</p>
      <p id="d1e400">A very recent study by <xref ref-type="bibr" rid="bib1.bibx16" id="text.37"/> compares the BDC in various
reanalyses by using a kinematic transport model (Belgian Assimilation System
for Chemical ObsErvations, BASCOE) within the scope of the S-RIP project.
The results presented here are based on a diabatic transport model (for
further details see Sect. <xref ref-type="sec" rid="Ch1.S2"/>) and therefore complement the
study by <xref ref-type="bibr" rid="bib1.bibx16" id="text.38"/> regarding the representation of vertical
transport. The main goal of our paper is to assess the robustness of the
climatology and seasonality of the BDC as well as its trends in current
generation reanalyses, as imprinted on stratospheric age of air. For that
reason, we calculate and analyse the mean age of air as well as the full
time-dependent stratospheric age spectrum, which has not been used for a
model inter-comparison of the BDC to date.</p>
      <p id="d1e411">The modelling method (transport model and age of air diagnostics) is described
in Sect. <xref ref-type="sec" rid="Ch1.S2"/>. In Sect. <xref ref-type="sec" rid="Ch1.S3"/> the climatology and
seasonality of age of air from different reanalyses is compared before
considering trends in Sect. <xref ref-type="sec" rid="Ch1.S4"/>. Section <xref ref-type="sec" rid="Ch1.S5"/>
provides a comparison to existing observational mean age estimates, and
Sect. <xref ref-type="sec" rid="Ch1.S6"/> discusses the results, in particular compared to
the results from the complementary model study of <xref ref-type="bibr" rid="bib1.bibx16" id="text.39"/>.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Data and method</title>
      <p id="d1e436">The Chemical Lagrangian Model of the Stratosphere (CLaMS) is a Lagrangian
model for calculating transport and chemistry for trace gas species based on
the motion of 3-D forward trajectories and an additional parameterised
representation of atmospheric small-scale mixing processes
<xref ref-type="bibr" rid="bib1.bibx52" id="paren.40"/>. Parameterised mixing in the model is driven by
deformations in the large-scale flow, such that, in regions of large flow
deformations, strong mixing occurs <xref ref-type="bibr" rid="bib1.bibx47" id="paren.41"/>. Model transport is
calculated in an isentropic vertical coordinate framework with potential
temperature <inline-formula><mml:math id="M3" display="inline"><mml:mi mathvariant="italic">θ</mml:mi></mml:math></inline-formula> being the vertical coordinate throughout the
stratosphere and upper troposphere, and with the cross-isentropic vertical
velocity deduced from the total diabatic heating rate (of the respective
reanalysis forecast), including effects of radiative and turbulent heating,
as well as latent heat release. Further details about the CLaMS model set-up
used in this study can be found in <xref ref-type="bibr" rid="bib1.bibx64" id="text.42"/>.</p>
      <?pagebreak page6088?><p id="d1e455">As described by <xref ref-type="bibr" rid="bib1.bibx58" id="text.43"/>, and briefly reviewed in the
following, we calculate the age of air spectrum for each reanalysis
from multiple tracer pulses and the mean age from the spectrum. The age
spectrum <inline-formula><mml:math id="M4" display="inline"><mml:mi>G</mml:mi></mml:math></inline-formula> is a boundary value Greens function for the continuity
equation of a conserved and passive trace gas species
<xref ref-type="bibr" rid="bib1.bibx38 bib1.bibx45" id="paren.44"><named-content content-type="pre">e.g.</named-content></xref> and relates the trace gas mixing
ratio <inline-formula><mml:math id="M5" display="inline"><mml:mrow><mml:mi mathvariant="italic">χ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> at location <inline-formula><mml:math id="M6" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> and time <inline-formula><mml:math id="M7" display="inline"><mml:mi>t</mml:mi></mml:math></inline-formula> to the mixing ratio
<inline-formula><mml:math id="M8" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">χ</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> at the boundary surface, where it is assumed to be uniform
<xref ref-type="bibr" rid="bib1.bibx75" id="paren.45"><named-content content-type="pre">e.g.</named-content></xref>:
          <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M9" display="block"><mml:mrow><mml:mi mathvariant="italic">χ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:munderover><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">τ</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msub><mml:mi mathvariant="italic">χ</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        Here, the integration is taken along transit time <inline-formula><mml:math id="M10" display="inline"><mml:mi mathvariant="italic">τ</mml:mi></mml:math></inline-formula>, and the boundary
surface is usually taken to be the tropical tropopause or the tropical
surface, a particularly common choice in models. The age spectrum calculation
applied in this study is set up analogously to the approach described by
<xref ref-type="bibr" rid="bib1.bibx58" id="text.46"/>, and similarly to the calculation in the GEOS climate
model <xref ref-type="bibr" rid="bib1.bibx49 bib1.bibx50" id="paren.47"/>. The calculation method is based on <inline-formula><mml:math id="M11" display="inline"><mml:mrow><mml:mi>N</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">60</mml:mn></mml:mrow></mml:math></inline-formula>
inert pulse tracers, approximating a delta distribution lower boundary
condition <inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="italic">χ</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mi>i</mml:mi></mml:msubsup><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mi mathvariant="italic">δ</mml:mi><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi>t</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> with <inline-formula><mml:math id="M13" display="inline"><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>,</mml:mo><mml:mi mathvariant="normal">…</mml:mi><mml:mo>,</mml:mo><mml:mn mathvariant="normal">60</mml:mn></mml:mrow></mml:math></inline-formula>, defining
tracer pulses at source times <inline-formula><mml:math id="M14" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. For such a set of pulse tracers, the age
spectrum at transit time <inline-formula><mml:math id="M15" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is related to the tracer mixing ratio of
the <inline-formula><mml:math id="M16" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula>th species via
          <disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M17" display="block"><mml:mrow><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">χ</mml:mi><mml:mi>i</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>;</mml:mo></mml:mrow></mml:math></disp-formula>
        hence the age spectrum can be directly calculated from the pulse
tracer mixing ratios in the simulation.</p>
      <p id="d1e760">To approximate the delta distribution characteristics, pulse tracer mixing
ratios are set to one in the lowest (orography following) model layer
(approximately the boundary layer) in the tropics between
15<inline-formula><mml:math id="M18" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and 15<inline-formula><mml:math id="M19" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N for 30 days. The 60 different species are
pulsed every other month (first species in the first month, second species in the
third month, etc.), such that after 10 years of simulation all species have
been pulsed. Hence, after every 10 years the first species is reset to zero
and pulsed again. This boundary impulse (time-)evolving response (BIER)
method <xref ref-type="bibr" rid="bib1.bibx58" id="paren.48"/> resolves the age spectrum along 10 years of
the transit time axis with a bin size of 2 months.</p>
      <p id="d1e784">The mean age of air is then calculated as the first moment of the age
spectrum:
          <disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M20" display="block"><mml:mrow><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:munderover><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">τ</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        As the mean age strongly depends on the age spectrum tail, which generally
shows an exponential decay after about 4–5 years <xref ref-type="bibr" rid="bib1.bibx49" id="paren.49"><named-content content-type="pre">e.g.</named-content></xref>,
the effect of the finite age spectrum tail on the mean age may be corrected by
fitting an exponentially decaying function
<xref ref-type="bibr" rid="bib1.bibx19 bib1.bibx58" id="paren.50"><named-content content-type="pre">e.g.</named-content></xref>. Hence, a corrected age spectrum may
be defined by extrapolating the spectrum tail for transit times
<inline-formula><mml:math id="M21" display="inline"><mml:mrow><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>&gt;</mml:mo><mml:msup><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>*</mml:mo></mml:msup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">10</mml:mn></mml:mrow></mml:math></inline-formula> using
          <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M22" display="block"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">corr</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>*</mml:mo></mml:msup><mml:mo>)</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi>e</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mstyle scriptlevel="+1"><mml:mfrac><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>-</mml:mo><mml:msup><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>*</mml:mo></mml:msup><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mi mathvariant="italic">ξ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:msup><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        with <inline-formula><mml:math id="M23" display="inline"><mml:mrow><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>*</mml:mo></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> the age spectrum value at 10 years, and the tail
decay timescale <inline-formula><mml:math id="M24" display="inline"><mml:mrow><mml:mi mathvariant="italic">ξ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> (depending on location and time) being
estimated from the exponential fit to the spectrum at transit times between
5 and 10 years. As the full age spectrum is the probability distribution of
transit times, it is generally normalised to unity. However, due to the truncation of
the simulated spectrum at 10 years, the integration of the spectrum over
transit time leads to a norm less than one (see Fig. <xref ref-type="fig" rid="Ch1.F6"/>):
          <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M25" display="block"><mml:mrow><mml:msup><mml:mi>N</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msup><mml:mo>=</mml:mo><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mn mathvariant="normal">10</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">year</mml:mi></mml:mrow></mml:munderover><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">τ</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>&lt;</mml:mo><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:munderover><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">τ</mml:mi><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        Including the exponential tail correction improves the normalisation, but
small differences to unity remain due to the finite resolution along the
transit time axis. On the one hand, including the correction generally
improves comparisons of mean age to observations. On the other hand, MERRA-2
age spectra show a much more pronounced tail without a clear exponential
decay over 10 years in some cases (see Sect. <xref ref-type="sec" rid="Ch1.S5"/>),
violating the necessary assumption for the finite tail correction. Hence, for
most parts of the analysis we simply consider the finite tail age spectra
over 10 years without including the tail correction. This simplifies the
interpretation of the comparison of different reanalyses by only considering
the resolved part of the age spectrum. Effects of the unresolved tail and the
finite tail correction are further discussed in Sect. <xref ref-type="sec" rid="Ch1.S5"/>.</p>
      <p id="d1e1112">Two other age spectrum-based transport diagnostics are the modal age,
which is the transit time of the maximum age spectrum peak, and the
age spectrum width
          <disp-formula id="Ch1.E6" content-type="numbered"><label>6</label><mml:math id="M26" display="block"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msqrt><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:mfrac></mml:mstyle><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mn mathvariant="normal">0</mml:mn><mml:mi mathvariant="normal">∞</mml:mi></mml:munderover><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">τ</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>[</mml:mo><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>-</mml:mo><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:msup><mml:mo>]</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mspace width="0.25em" linebreak="nobreak"/><mml:mi>G</mml:mi><mml:mo>(</mml:mo><mml:mi>r</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi>t</mml:mi><mml:mo>,</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="italic">τ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:msqrt><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        The spectrum width is strongly influenced by long transit times in the
spectrum tail and therefore is usually considered a measure of the strength
of recirculation <xref ref-type="bibr" rid="bib1.bibx49" id="paren.51"><named-content content-type="pre">e.g.</named-content></xref>. The modal age, in comparison,
can be interpreted as a measure of the residual circulation in the tropics
and in the winter stratosphere as it is closely related to the residual
circulation transit time in these regions. As additional diagnostics for the
interpretation of processes affecting zonal mean mean age we consider
residual circulation transit times <xref ref-type="bibr" rid="bib1.bibx8" id="paren.52"><named-content content-type="pre">RCTTs,</named-content></xref> and the net
mixing effect on mean age <xref ref-type="bibr" rid="bib1.bibx34" id="paren.53"><named-content content-type="pre">“ageing by mixing”,</named-content></xref> in
Sect. <xref ref-type="sec" rid="Ch1.S6"/>. The RCTT is the transit time of a (hypothetical) air
parcel if it was transported by the residual circulation alone and, by
definition, solely includes effects of the residual circulation
<xref ref-type="bibr" rid="bib1.bibx8" id="paren.54"/>. For this paper, RCTTs are calculated with the CLaMS
trajectory module and using the zonal mean diabatic residual circulation in
isentropic coordinates <inline-formula><mml:math id="M27" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msup><mml:mover accent="true"><mml:mi>v</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>*</mml:mo></mml:msup><mml:mo>,</mml:mo><mml:msup><mml:mover accent="true"><mml:mi>Q</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>*</mml:mo></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>
<xref ref-type="bibr" rid="bib1.bibx60" id="paren.55"/>. Here, <inline-formula><mml:math id="M28" display="inline"><mml:mi>Q</mml:mi></mml:math></inline-formula> denotes the diabatic heating rate, <inline-formula><mml:math id="M29" display="inline"><mml:mi>v</mml:mi></mml:math></inline-formula> denotes the
meridional velocity component, overlined quantities denote mass-weighted
zonal averages and primed quantities represent the respective fluctuations therefrom
<xref ref-type="bibr" rid="bib1.bibx6" id="paren.56"><named-content content-type="pre">e.g.</named-content><named-content content-type="post">chap. 9.4</named-content></xref>; hence,
<inline-formula><mml:math id="M30" display="inline"><mml:mrow><mml:msup><mml:mover accent="true"><mml:mi>v</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>*</mml:mo></mml:msup><mml:mo>=</mml:mo><mml:mo>(</mml:mo><mml:mover accent="true"><mml:mrow><mml:mi mathvariant="italic">σ</mml:mi><mml:mi>v</mml:mi></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>)</mml:mo><mml:mo>/</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">σ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mrow></mml:math></inline-formula>, and
<inline-formula><mml:math id="M31" display="inline"><mml:mrow><mml:msup><mml:mover accent="true"><mml:mi>Q</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>*</mml:mo></mml:msup><mml:mo>=</mml:mo><mml:mo>(</mml:mo><mml:mover accent="true"><mml:mrow><mml:mi mathvariant="italic">σ</mml:mi><mml:mi>Q</mml:mi></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>)</mml:mo><mml:mo>/</mml:mo><mml:mover accent="true"><mml:mi mathvariant="italic">σ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mrow></mml:math></inline-formula>.</p>
      <?pagebreak page6089?><p id="d1e1348">In addition, the zonal mean mean age <inline-formula><mml:math id="M32" display="inline"><mml:mover accent="true"><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> is affected by mixing
processes in the atmosphere. The local effect of this mixing, the local eddy
mixing tendency, is represented in the zonal mean (isentropic) tracer
continuity equation for mean age by the divergence <inline-formula><mml:math id="M33" display="inline"><mml:mi mathvariant="script">M</mml:mi></mml:math></inline-formula> of a 2-D
mixing flux vector <xref ref-type="bibr" rid="bib1.bibx6" id="paren.57"><named-content content-type="pre">e.g.</named-content><named-content content-type="post">Eq. 9.4.21</named-content></xref>. The net mixing
effect on the zonal mean mean age, the ageing by mixing, is then calculated by
integrating the local eddy mixing tendency <inline-formula><mml:math id="M34" display="inline"><mml:mi mathvariant="script">M</mml:mi></mml:math></inline-formula> along residual
circulation trajectories <inline-formula><mml:math id="M35" display="inline"><mml:mrow><mml:mi>x</mml:mi><mml:mo>(</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx60" id="paren.58"/>:
          <disp-formula id="Ch1.E7" content-type="numbered"><label>7</label><mml:math id="M36" display="block"><mml:mrow><mml:mover accent="true"><mml:mi mathvariant="normal">Γ</mml:mi><mml:mo mathvariant="normal">‾</mml:mo></mml:mover><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>,</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi mathvariant="normal">RCTT</mml:mi></mml:msub><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>,</mml:mo><mml:mi>t</mml:mi><mml:mo>)</mml:mo><mml:mo>+</mml:mo><mml:munderover><mml:mo movablelimits="false">∫</mml:mo><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow><mml:mi>t</mml:mi></mml:munderover><mml:mi mathvariant="script">M</mml:mi><mml:mo>(</mml:mo><mml:mi>x</mml:mi><mml:mo>(</mml:mo><mml:msup><mml:mi>t</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mo>)</mml:mo><mml:mo>)</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">d</mml:mi><mml:msup><mml:mi>t</mml:mi><mml:mo>′</mml:mo></mml:msup><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        Here, <inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">τ</mml:mi><mml:mi mathvariant="normal">RCTT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the RCTT, for transport from the 340 K
isentropic surface in the tropics (30<inline-formula><mml:math id="M38" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S–30<inline-formula><mml:math id="M39" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N), and <inline-formula><mml:math id="M40" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is the
time when the trajectory intersected the 340 K surface. As proposed by
<xref ref-type="bibr" rid="bib1.bibx34" id="text.59"/> and recently further evidenced by <xref ref-type="bibr" rid="bib1.bibx22" id="text.60"/>,
the net eddy mixing effect can be well approximated by the difference between
the mean age and the RCTT. We apply this approximation in the following without
explicitly calculating the mixing effect (see Sect. <xref ref-type="sec" rid="Ch1.S6"/>).
For further details about the RCTT and the ageing by mixing calculation see
<xref ref-type="bibr" rid="bib1.bibx60" id="text.61"/>.</p>
      <p id="d1e1533">The CLaMS simulations are driven with horizontal winds and diabatic heating
rates from the three most recent reanalysis data sets: ERA-Interim, JRA-55
and MERRA-2. The simulations for ERA-Interim and JRA-55 both start on
1 January 1979, whereas the MERRA-2 simulation starts on 1 January 1980. Due
to the specific pulse tracer set-up described above it takes 10 years of
simulation until all pulse tracers have been set and the age spectrum can be
evaluated. To enable the age of air analysis beginning in 1979 (in 1980 for
MERRA-2), for comparison with balloon-borne mean age measurements in
Sect. <xref ref-type="sec" rid="Ch1.S5"/>, a 10-year-long model spin-up is carried out by
repeating conditions of the first simulation year. However, the simulated age
of air before 1989 includes the effect of the spin-up and most parts of the
analysis presented here are restricted to the time period from 1989 to 2015. For
MERRA-2, the year 1989 still includes a very weak spin-up effect, but
without any effect on our conclusions, as all results of the paper could be
analogously derived for the 1990–2015 period (not shown).</p>
      <p id="d1e1538">The three different reanalyses used here have been recently described by
<xref ref-type="bibr" rid="bib1.bibx30" id="text.62"/>, with further details given by <xref ref-type="bibr" rid="bib1.bibx18" id="text.63"/> for
ERA-Interim, by <xref ref-type="bibr" rid="bib1.bibx46" id="text.64"/> for JRA-55 and by <xref ref-type="bibr" rid="bib1.bibx35" id="text.65"/>
for MERRA-2. For driving the CLaMS model simulations, reanalysis horizontal
winds and diabatic heating rates from the reanalysis forecast are used on
native model levels and with a horizontal resolution of <inline-formula><mml:math id="M41" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M42" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> in latitude and longitude. The age of
air results from the different simulations have been interpolated to
potential temperature levels (same for all reanalyses) and monthly zonal mean
climatologies have been created.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><?xmltex \currentcnt{1}?><label>Figure 1</label><caption><p id="d1e1579">Mean age climatology (1989–2015) for December–February (DJF,
<bold>a–c</bold>) and June–August (JJA, <bold>d–f</bold>) for
ERA-Interim <bold>(a, d)</bold>, JRA-55 <bold>(b, e)</bold> and
MERRA-2 <bold>(c, f)</bold>.
Thin solid black lines highlight particular mean age contours, the thin dashed
black lines show pressure levels in hPa, and the thick black line is the
(lapse rate) tropopause <xref ref-type="bibr" rid="bib1.bibx76" id="paren.66"><named-content content-type="pre">calculated from each reanalysis
following</named-content></xref>.</p></caption>
        <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f01.png"/>

      </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><?xmltex \currentcnt{2}?><label>Figure 2</label><caption><p id="d1e1612">Age spectrum on the 500 K potential temperature surface for
December–February in <bold>(a)</bold> the tropics between
20<inline-formula><mml:math id="M43" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and 20<inline-formula><mml:math id="M44" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, <bold>(b)</bold> middle latitudes between
30 and 60<inline-formula><mml:math id="M45" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N and <bold>(c)</bold> polar regions between
60 and 90<inline-formula><mml:math id="M46" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N. Different colours represent different reanalyses
(ERA-Interim is shown using black, JRA-55 is shown using blue and MERRA-2 is shown using red).
Vertical dashed lines indicate the respective mean age. (Note the different <inline-formula><mml:math id="M47" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis range for
tropical and extratropical spectra.)</p></caption>
        <?xmltex \igopts{width=184.942913pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f02.png"/>

      </fig>

</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Seasonal variations in age of air</title>
      <p id="d1e1682">Climatological mean age data (1989–2015) from the three reanalyses for
boreal winter (December–February, DJF) and summer (June–August, JJA) are
compared in Fig. <xref ref-type="fig" rid="Ch1.F1"/>. Throughout most parts of the stratosphere
JRA-55 shows the youngest mean age and MERRA-2 shows the oldest mean age.
Values for ERA-Interim lie in between. However, in the tropical lower
stratosphere below about 700 K potential temperature (about 20 hPa)
ERA-Interim shows the youngest mean age of the three reanalyses, which is
consistent with overly strong tropical upwelling as documented in the literature
<xref ref-type="bibr" rid="bib1.bibx18" id="paren.67"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d1e1692">The MERRA-2 mean age is substantially older than the other reanalyses,
with the largest relative differences in the tropical stratosphere (e.g. about
2.5 years for MERRA-2 at about 500 K (about 50 hPa) compared to about
1.5 years for ERA-Interim). Moreover, at high latitudes the MERRA-2 mean age is
clearly older, reaching maximum values of more than 5.5 years in the southern
polar vortex compared with less than 5 years for ERA-Interim and JRA-55 (note
that these values are calculated from the age spectrum over 10 years and that
actual mean ages are higher).</p>
      <p id="d1e1695">Despite these differences in climatological average mean age values,
seasonal variations (as estimated from December–February to
June–August differences) are very similar in the three
reanalyses. The youngest air is found in the tropical stratosphere
during boreal winter, when the BDC upwelling maximises. Conversely,
the oldest air occurs in the high-latitude stratosphere during
wintertime and is related to the strongest downwelling within the deep
BDC branch in that region and season. Furthermore, a flushing of the
summertime lower stratosphere with young air masses from the tropics
<xref ref-type="bibr" rid="bib1.bibx43 bib1.bibx10" id="paren.68"><named-content content-type="pre">e.g.</named-content></xref> is evident in all
reanalyses. This summertime flushing shows a robust hemispheric
asymmetry, and is stronger in the NH than in the SH <xref ref-type="bibr" rid="bib1.bibx48" id="paren.69"/>.</p>
      <p id="d1e1706">More details about stratospheric transport can be observed in the age
spectrum, presented in Fig. <xref ref-type="fig" rid="Ch1.F2"/> for the tropics, middle and
high latitudes on the 500 K potential temperature surface. The tropical age
spectra show an almost unimodal shape with a clear peak at short transit
times, and only very weak additional peaks and a decaying tail at larger
transit times. In middle and high latitudes the age spectra show distinct
multiple peaks caused mainly by the seasonality of transport into the
stratosphere <xref ref-type="bibr" rid="bib1.bibx68 bib1.bibx49 bib1.bibx19 bib1.bibx58" id="paren.70"><named-content content-type="pre">e.g.</named-content></xref>.
These multiple spectrum peaks are robustly found for all reanalyses, again
indicating robustness in the representation of seasonal variations in
stratospheric transport in modern reanalyses. In general, ERA-Interim and
JRA-55 age spectra are very similar for all regions, but MERRA-2 spectra
differ more substantially. In particular, for MERRA-2 the secondary peaks at
higher ages are delayed by a few months compared with ERA-Interim and JRA-55,
again indicating slower transport for MERRA-2. At high latitudes, the modal
age (transit time of the maximum spectrum peak) for MERRA-2 may occur with a
delay of more than a year (e.g. Fig. <xref ref-type="fig" rid="Ch1.F2"/>c). In all regions the
modal peak is shifted to larger transit times (higher ages) for MERRA-2. In
particular, the spectrum tail is much more pronounced for MERRA-2 (e.g.
Fig. <xref ref-type="fig" rid="Ch1.F2"/>f), with age spectrum values more than twice as large
as ERA-Interim and JRA-55 at transit times larger than about 8
years. Hence, there is a substantially larger fraction of very old air for
MERRA-2 than for ERA-Interim and JRA-55.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><?xmltex \currentcnt{3}?><label>Figure 3</label><caption><p id="d1e1723">Age spectrum (as transit time probability density
function (PDF) in month<inline-formula><mml:math id="M48" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) at 400 K for December–February <bold>(a, b, c)</bold> and
June–August <bold>(d, e, f)</bold> for ERA-Interim <bold>(a, d)</bold>,
JRA-55 <bold>(b, e)</bold> and MERRA-2 <bold>(c, f)</bold>.
Climatological values for 1989–2015 are shown. The black line shows the mean age, and the
white diamonds show the modal age.</p></caption>
        <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f03.png"/>

      </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><?xmltex \currentcnt{4}?><label>Figure 4</label><caption><p id="d1e1762">Same as Fig. <xref ref-type="fig" rid="Ch1.F3"/>, but at the 600 K potential
temperature surface.</p></caption>
        <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f04.png"/>

      </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5"><?xmltex \currentcnt{5}?><label>Figure 5</label><caption><p id="d1e1775">Cross-isentropic vertical velocity <inline-formula><mml:math id="M49" display="inline"><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi mathvariant="italic">θ</mml:mi><mml:mo>/</mml:mo><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:math></inline-formula>
from the total diabatic heating rate for ERA-Interim <bold>(a)</bold>,
JRA-55 <bold>(b)</bold> and MERRA-2 <bold>(c)</bold>. Climatological
annual mean distributions for 1989–2015 are shown. The thin black lines show pressure
contours, and the thick black line is the (lapse rate)
tropopause.</p></caption>
        <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f05.png"/>

      </fig>

      <p id="d1e1809">The global view of the age spectrum in the lowest stratosphere at 400 K is
presented in Fig. <xref ref-type="fig" rid="Ch1.F3"/>. The 400 K isentrope has been
chosen as a representative level for the shallow BDC branch. The robust
representation of transport seasonality is again evident from the similar
occurrence of the<?pagebreak page6090?> multiple spectrum peaks. In particular, the modal peak
(modal age) of the tropical age spectra is shifted to younger ages in boreal
winter, which is consistent with faster wintertime BDC upwelling. The strong flushing
of the Northern Hemisphere <xref ref-type="bibr" rid="bib1.bibx10" id="paren.71"/>, and to a lesser degree also
of the Southern Hemisphere, is clearly visible in the extension of the modal
peak (white diamonds) from the tropics into the summer hemisphere in all
reanalyses. This extension of the tropical young air signal deep into the
summer hemisphere is consistent with the general understanding of a less
isolated tropics and stronger isentropic mixing causing horizontal exchange
between the tropics and the extratropics during summer.</p>
      <p id="d1e1817">The subtropics in Fig. <xref ref-type="fig" rid="Ch1.F3"/> are characterised as
transition regions between approximately monomodal tropical age spectra and
middle- and high-latitude spectra with distinct multiple peaks. The contrast
between tropical and extratropical age spectra is strongest in the respective
winter hemisphere, which is indicative of a stronger subtropical jet and related
transport barrier compared to the summer hemisphere. For MERRA-2, the
transition between tropical and extratropical age spectra is more dilute,
indicating stronger exchange between tropics and middle latitudes in the
lowest stratosphere. This stronger exchange likely results in a stronger
recirculation of extratropical aged air masses into the tropics, causing
older air throughout the stratosphere.</p>
      <p id="d1e1823">Very similar results emerge from the comparison of the age spectra at higher
levels in the stratosphere (here 600 K in Fig. <xref ref-type="fig" rid="Ch1.F4"/>),
where the deep BDC branch dominates transport. The seasonality in tropical
upwelling (faster in boreal winter) as well as in subtropical transport
barriers (stronger in boreal winter) is robustly represented in the different
reanalysis data sets. In particular the older modal age for MERRA-2 in the
tropics, evident at 400 K (Fig. <xref ref-type="fig" rid="Ch1.F3"/>), becomes even
more clear at 600 K.</p>
      <p id="d1e1830">This shift of the tropical modal age to longer transit times is related to a
slower tropical upwelling for MERRA-2, which is consistent with the comparison of
reanalysis climatological total diabatic heating rates shown in
Fig. <xref ref-type="fig" rid="Ch1.F5"/>. In particular throughout the tropical tropopause
layer <xref ref-type="bibr" rid="bib1.bibx28" id="paren.72"><named-content content-type="pre">e.g.</named-content></xref> and up to about 500 K the MERRA-2
heating rates are lower than for the other reanalyses
(Fig. <xref ref-type="fig" rid="Ch1.F5"/>). Below the tropopause around the level of zero
radiative heating (around 360 K) there is even a cooling layer evident in
the MERRA-2 heating rates causing a “bottleneck” structure in annual mean
upwelling. The differences in heating rates could be related to ozone
differences between the reanalyses <xref ref-type="bibr" rid="bib1.bibx17" id="paren.73"><named-content content-type="pre">e.g.</named-content></xref>. ERA-Interim
uses prescribed climatological ozone fields for the radiative calculations,
including a potential high bias in ozone concentrations in the tropical lower
stratosphere <xref ref-type="bibr" rid="bib1.bibx29" id="paren.74"><named-content content-type="pre">e.g.</named-content></xref>. JRA-55, in comparison,
uses prescribed time-varying ozone fields from a model simulations
<xref ref-type="bibr" rid="bib1.bibx46" id="paren.75"/>, and MERRA-2 uses interactive ozone for radiation and
heating rate calculations <xref ref-type="bibr" rid="bib1.bibx73" id="paren.76"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d1e1861">Regarding the age spectrum, MERRA-2 further shows a weaker gradient between
tropical and extratropical age spectra compared with the other reanalyses at
600 K (Fig. <xref ref-type="fig" rid="Ch1.F4"/>). This weaker tropical–extratropical
contrast indicates stronger exchange between tropics and extratropics and a
weaker<?pagebreak page6091?> subtropical transport barrier. Furthermore, the MERRA-2 age spectra
at 600 K show a more pronounced spectrum tail, as previously noted. Differences
in the age spectrum tail at transit times larger than about 5 years cannot
be caused by the differences in the diabatic circulation (in
Fig. <xref ref-type="fig" rid="Ch1.F5"/>) alone, because related transit times along the
residual circulation are generally below about 5 years
<xref ref-type="bibr" rid="bib1.bibx8" id="paren.77"><named-content content-type="pre">e.g.</named-content><named-content content-type="post">Fig. 2</named-content></xref>. Therefore, the more pronounced spectrum
tail for MERRA-2 compared with ERA-Interim and JRA-55 is likely a result of
the stronger recirculation of air into the tropics at lower levels.
Recirculation into the tropics, particularly at low levels, causes air masses
to circulate through the stratosphere within the BDC several times before
sinking back into the troposphere and significantly increases the age
<xref ref-type="bibr" rid="bib1.bibx56 bib1.bibx34" id="paren.78"><named-content content-type="pre">e.g.</named-content></xref>. Therefore, an increased recirculation
enhances the fraction of aged air masses and hence the tail of the age
spectrum <xref ref-type="bibr" rid="bib1.bibx49" id="paren.79"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d1e1885">Figure <xref ref-type="fig" rid="Ch1.F6"/> further compares the characteristics of the spectrum
tail between the three reanalyses by showing the spectrum normalisation
(coloured shading) and the tail decrease timescale (blue contours). The
spectrum norm was calculated as the integral of the age spectrum over
10 years (Eq. <xref ref-type="disp-formula" rid="Ch1.E5"/>), and the tail decrease timescale was calculated as the
exponential decrease rate of the spectrum tail at transit times larger than
5 years (Eq. <xref ref-type="disp-formula" rid="Ch1.E4"/>). As the model age spectra are truncated
after 10 years (see Sect. <xref ref-type="sec" rid="Ch1.S2"/>) a stronger spectrum tail will
result in a less stringent normalisation condition and in a larger difference
of the age spectrum norm from unity. Indeed, Fig. <xref ref-type="fig" rid="Ch1.F6"/> shows that
the MERRA-2 age spectra are less well normalised, with a norm below 0.8
throughout large regions of the stratosphere, whereas for ERA-Interim and
JRA-55 the norm is always above 0.9 (in the lower part of the stratosphere
even above about 0.95). This lack of normalisation of the MERRA-2 age spectra is
clearly related to a much larger tail decrease timescale (global average
5.13 years) compared with ERA-Interim (2.84 years) and JRA-55 (2.91 years).
Compared to the climate model simulated age spectra of <xref ref-type="bibr" rid="bib1.bibx49" id="text.80"/>, with
a global average tail decay timescale of 2.77 years, ERA-Interim and
JRA-55 show comparable values, whereas MERRA-2 differs substantially.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6"><?xmltex \currentcnt{6}?><label>Figure 6</label><caption><p id="d1e1904">Norm of the climatological (1989–2015) age spectra for
ERA-Interim <bold>(a)</bold>, JRA-55 <bold>(b)</bold> and MERRA-2 <bold>(c)</bold>.
Blue contours show the climatological tail decay timescale (in years), the thin
black dashed lines show the pressure levels in hPa, and the thick black line is
the (lapse rate) tropopause.</p></caption>
        <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f06.png"/>

      </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><label>Figure 7</label><caption><p id="d1e1925">Long-term mean age trends for 1989–2015 <bold>(a, b, c)</bold>, decadal
trends for 1989–2001 <bold>(d, e, f)</bold> and decadal trends for
2002–2015 <bold>(g, h, i)</bold>, for ERA-Interim <bold>(a, d, g)</bold>,
JRA-55 <bold>(b, e, h)</bold> and MERRA-2 <bold>(c, f, i)</bold>. The trend
significance, estimated in multiples of the standard deviation <inline-formula><mml:math id="M50" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>, is shown
as grey contours (<inline-formula><mml:math id="M51" display="inline"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula> contour thick grey, and then decreasing in 0.2 steps
as thin lines). The thin black solid contours show the climatological mean age
distribution, the thin black dashed lines show pressure levels in hPa, and the
thick black line is the (lapse rate) tropopause.</p></caption>
        <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f07.png"/>

      </fig>

</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Age of air trends</title>
      <p id="d1e1978">In the following, we analyse trends in age of air for the same periods as
considered by <xref ref-type="bibr" rid="bib1.bibx16" id="text.81"/> to simplify the comparison to their results
in Sect. <xref ref-type="sec" rid="Ch1.S6"/>. We refer to 1989–2015 as “long-term” trends
and to 1989–2001 (“pre-2000” in the following) and 2002–2015
(“post-2000”) as “decadal” trends. It should be noted that even the
long-term period spans only 27 years, which is relatively short compared with
climate model simulation periods but is the longest period we can obtain from
the reanalyses without including spin-up effects in the results (see
Sect. <xref ref-type="sec" rid="Ch1.S2"/>). Throughout the paper, trends are calculated from the
linear regression of monthly mean time series after deseasonalising (by
subtracting the mean annual cycle), and the significance is measured in multiples
of the standard deviation of the linear trend.</p><?xmltex \hack{\newpage}?>
<?pagebreak page6092?><sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Long-term trends from 1989 to 2015</title>
      <p id="d1e1996">Long-term mean age trends for 1989–2015 are presented in
Fig. <xref ref-type="fig" rid="Ch1.F7"/>a–c. Overall, mean age trends are negative
throughout most regions of the lower stratosphere below about 600 K (30 hPa)
and for all three reanalyses. Hence, the representation of long-term changes
in mean age in the lower stratosphere in current reanalyses is largely robust
and indicates an accelerating shallow BDC branch. Mean age trends above about
600 K are not robust, with ERA-Interim showing positive trends in the NH
whereas JRA-55 and MERRA-2 show negative trends. Hence, trends in the deep
BDC branch appear not to be robustly represented in current reanalysis data
sets. The mean age decrease in the shallow BDC branch is in agreement with an
acceleration of the residual circulation in reanalyses
<xref ref-type="bibr" rid="bib1.bibx1 bib1.bibx53" id="paren.82"/>.</p>
      <p id="d1e2004">Closer examination of the 1989–2015 trends in Fig. <xref ref-type="fig" rid="Ch1.F7"/>a–c
reveals detailed differences between the reanalyses. First, ERA-Interim
shows an inhomogeneous pattern with the strongest negative trends in the southern
subtropics, and even weakly positive trends in the NH above about 30 hPa.
Second, JRA-55 provides a very homogeneous picture, showing negative mean
age trends everywhere. Third, MERRA-2 again shows largely negative trends,
maximising in the<?pagebreak page6093?> southern subtropics similarly to ERA-Interim, and positive
trends in the NH lowermost stratosphere below about 400 K.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><label>Figure 8</label><caption><p id="d1e2011">Age spectrum trend (annual mean) at 400 K for
ERA-Interim <bold>(a, d, g)</bold>, JRA-55 <bold>(b, e, h)</bold> and
MERRA-2 <bold>(c, f, i)</bold>, and for the periods 1989–2015 <bold>(a, b, c)</bold>, 1989–2001 <bold>(d, e, f)</bold>, and 2002–2015 <bold>(g, h, i)</bold>. The
thin black contours show the climatological age spectrum, the thick black
line shows the climatological mean age, and the white diamonds show the
climatological modal age.</p></caption>
          <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f08.png"/>

        </fig>

      <p id="d1e2040">Changes in the full age spectrum can shed more light on the processes
involved during each period. Figure <xref ref-type="fig" rid="Ch1.F8"/>a–c shows age
spectrum changes (coloured shading) during the 1989–2015 period in the lower
stratosphere at 400 K and at all latitudes for the different reanalyses,
overlaid with contours of climatological mean age (thick black lines).
Remarkably, trends in the age spectra at young transit times are very
consistent, particularly in the tropics, with all reanalyses showing an
increase in the fraction of air masses with transit times younger than the
modal age, and a simultaneous decrease in the air mass fraction with transit
times just older than modal age. These changes indicate a shift of<?pagebreak page6094?> the
spectrum peak (modal age) to younger transit times over time. Modal age can
be related to the residual circulation transit time <xref ref-type="bibr" rid="bib1.bibx49" id="paren.83"><named-content content-type="pre">e.g.</named-content></xref>,
particularly in the tropics and the winter hemisphere stratosphere
<xref ref-type="bibr" rid="bib1.bibx58" id="paren.84"/>. The shift of the modal age to younger ages in the tropics
indicates an acceleration of the residual mean mass circulation.</p>
      <p id="d1e2053">This decrease in the modal age emerges even more clearly at higher levels (e.g.
600 K in Fig. <xref ref-type="fig" rid="Ch1.F9"/>a–c). Independent of reanalysis
and latitude, the spectrum peak shifts to younger transit times over the
1989–2015 period. Differences in mean age trends between the different
reanalyses appear to be related to differences in the age spectrum tail. Clearly,
the weakly increasing mean age in the NH above about 30 hPa
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>) in ERA-Interim is related to an increasing age
spectrum tail at transit times older than about 4 years
(Fig. <xref ref-type="fig" rid="Ch1.F9"/>a), which is absent in the other two
reanalyses. Note that the 600 K potential temperature level is at the lower
boundary of the region of increasing mean age in ERA-Interim, and that the
described increase of the age spectrum tail becomes even clearer at levels
above. However, 600 K is chosen as it is consistent with the later
2002–2015 trends, which show the mean age dipole change pattern only below
about 20 hPa.</p>
      <p id="d1e2062">In agreement with the general shift of the age spectrum peak towards younger
transit times from 1989 to 2015 the fraction of young air masses, younger than
6 months, robustly increases in the lower stratosphere in all three
reanalyses (Fig. <xref ref-type="fig" rid="Ch1.F10"/>). Differences occur in the NH lowermost
stratosphere, where the young air mass increase is strongest for JRA-55
and is absent for MERRA-2, which is consistent with the respective changes in mean
age (Fig. <xref ref-type="fig" rid="Ch1.F7"/>). Note that the young air mass fraction is a
particularly robust diagnostic as it is independent of the truncation of the
age spectrum<?pagebreak page6095?> to 10 years. Observable changes in the young air mass fraction
are confined below about the 500 K potential temperature level. Above this level, the
air is generally older than 6 months, and the young air mass fraction with
transit times shorter than 6 months almost vanishes. Changes in the old air
mass fraction, older than 2 years, show negative changes in the tropical
stratosphere above about 450 K (not shown), which is consistent with the shift of the
age spectrum towards shorter transit times (also at higher levels).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9" specific-use="star"><?xmltex \currentcnt{9}?><label>Figure 9</label><caption><p id="d1e2071">Same as Fig. <xref ref-type="fig" rid="Ch1.F8"/>, but at the 600 K
potential temperature surface.</p></caption>
          <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f09.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10"><?xmltex \currentcnt{10}?><label>Figure 10</label><caption><p id="d1e2084">Trend in the young air mass fraction (transit time less than 6 months)
from 1989 to 2015 for <bold>(a)</bold> ERA-Interim,
<bold>(b)</bold> JRA-55 and <bold>(c)</bold> MERRA-2, in percent per decade. The
white contours show the young air mass fraction climatology in percent, and the
thick white line is the tropopause.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f10.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Decadal changes during 1989–2001 and 2002–2015</title>
      <p id="d1e2110">The decadal mean age changes over shorter periods are much more
diverse than the long-term trends. Furthermore, certain
characteristics in these decadal changes strongly depend on the
start and end points of the period considered and should not be
taken as representative of long-term trends. Nevertheless, as observational
data sets only exist for restricted periods and several past studies have
focused on circulation changes before and after the year 2000, we
include a discussion of such decadal changes in the following. The
decadal periods considered (1989–2001 and 2002–2015) were chosen for
better comparability with <xref ref-type="bibr" rid="bib1.bibx16" id="text.85"/>.</p>
      <p id="d1e2116">For 1989–2001, ERA-Interim and MERRA-2 show mean age trend patterns
similar to the longer 1989–2015 period (Fig. <xref ref-type="fig" rid="Ch1.F7"/>d and f).
JRA-55, in contrast, shows much stronger negative trends, particularly
in the tropics (Fig. <xref ref-type="fig" rid="Ch1.F7"/>e). These strong negative trends in
JRA-55 are related to a stronger effect of the volcanic eruption of Mt.
Pinatubo in June 1991, which increased mean age in the reanalysis in the
lower stratosphere during the 2–3 years following the eruption
<xref ref-type="bibr" rid="bib1.bibx20" id="paren.86"/>. As the Pinatubo eruption and related ageing of air occurs
close to the beginning of the trend period, 1989–2001 negative decadal mean
age trends appear enhanced for JRA-55 (see Fig. <xref ref-type="fig" rid="Ch1.F11"/>b). More
generally, the strong negative mean age trends in the Southern Hemisphere
(SH) during the 1989–2001 period are likely related to the effects of ozone
depleting substances <xref ref-type="bibr" rid="bib1.bibx63" id="paren.87"/>, with the dominant effect caused by
their chemical impact with respect to depleting ozone <xref ref-type="bibr" rid="bib1.bibx3" id="paren.88"/>. Reanalyses may
include ozone depletion effects by assimilating observed temperatures even
without having realistic ozone fields.</p>
      <?pagebreak page6096?><p id="d1e2135">Mean age trends for the later period 2002–2015 are least consistent among
the three reanalyses (Fig. <xref ref-type="fig" rid="Ch1.F7"/>g–i). MERRA-2 shows negative
trends similar to the 1989–2015 and 1989–2001 periods. Conversely,
JRA-55 shows positive trends throughout almost the entire stratosphere, with
the exception of a small region in the NH lower stratosphere of insignificant
trends. In contrast, ERA-Interim shows decreasing age in the lowest
stratosphere, and a clear dipole pattern above with increasing age in the NH
lower stratosphere, and decreasing age in the SH. This dipole pattern has
been shown to be consistent with mean age trends based on satellite
observations <xref ref-type="bibr" rid="bib1.bibx37 bib1.bibx60" id="paren.89"><named-content content-type="pre">e.g.</named-content></xref> and observed HCl trends
<xref ref-type="bibr" rid="bib1.bibx51" id="paren.90"/>, although for a slightly different period (2002–2012).
Recently, <xref ref-type="bibr" rid="bib1.bibx72" id="text.91"/> related the dipole trend pattern to a southward
shift of the global stratospheric circulation. Obviously, only ERA-Interim
shows this dipole pattern in mean age trends for 2002–2015, whereas the
other two reanalyses provide only very weak indications for slightly more
ageing in the NH (JRA-55) or a weaker age decrease in that region
(MERRA-2).</p>
      <p id="d1e2151">The differences between the reanalyses are larger for the age spectrum
changes over the shorter periods, 1989–2001 and 2002–2015, than for the
long-term, 1989–2015, trend. At the lower potential temperature level of
400 K the spectrum peak may shift towards younger transit times (e.g.
JRA-55 for 1989–2001) or towards older transit times (e.g. MERRA-2 for
2002–2015), and the spectrum tail may decrease or increase depending on the
reanalysis (Fig. <xref ref-type="fig" rid="Ch1.F8"/>d–i). At the upper level of
600 K, more consistent spectrum changes emerge. During the early period
1989–2001 all reanalyses show a shift of the spectrum peak towards younger
transit times (Fig. <xref ref-type="fig" rid="Ch1.F9"/>d–f), which is consistent with
the decreasing mean age over this period. During the later 2002–2015 period
MERRA-2 mainly shows a shift of the spectrum peak to shorter transit times
(Fig. <xref ref-type="fig" rid="Ch1.F9"/>i), which is consistent with decreasing mean age
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>i). JRA-55, in contrast, shows a shift of the
spectrum peak towards longer transit times and an increase in the spectrum
tail (Fig. <xref ref-type="fig" rid="Ch1.F9"/>h), resulting in positive mean age
trends (Fig. <xref ref-type="fig" rid="Ch1.F7"/>h). ERA-Interim shows a hemispheric
asymmetric pattern (Fig. <xref ref-type="fig" rid="Ch1.F9"/>g). In the NH, the
spectrum peak shifts towards longer transit times and the spectrum tail
increases, resulting in an increasing mean age during this period
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>g). In the SH, opposite changes occur, with a
spectrum peak shift towards shorter transit times and a decrease of the
spectrum tail. Hence, the hemispheric asymmetric age<?pagebreak page6097?> spectrum changes in
ERA-Interim for transit times less than 10 years are consistent with the
hemispheric dipole trend in mean age. Clearly, spectrum changes in the tail
at transit times of around 5 years appear critical for the positive mean age
trend in the NH. As 5 years is beyond the timescale of the residual
circulation, mixing effects are likely involved in causing the hemispheric
dipole pattern of mean age changes, as recently concluded from analysis of
different diagnostics <xref ref-type="bibr" rid="bib1.bibx60 bib1.bibx72" id="paren.92"/>. Interestingly, age
spectrum changes in the NH from 2002 to 2015 appear qualitatively consistent
between ERA-Interim and JRA-55, showing decreasing values at transit times
less than about 2 years and increasing values at transit times around
5 years. Hence, the more pronounced NH ageing in ERA-Interim compared with
JRA-55 is the result of a very subtle balance between changes in the age
spectrum at short transit times (less than about 2 years) and in the tail
(around 5 years).</p>
</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Comparison to observations</title>
      <p id="d1e2184">To assess the reliability of the representation of the stratospheric BDC in
different reanalyses, the mean age of air is compared to the mean age estimated from
observations of the long-lived trace gas species SF<inline-formula><mml:math id="M52" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M53" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.
Figure <xref ref-type="fig" rid="Ch1.F11"/>a compares latitude sections of mean age from
reanalysis, airborne in situ observations (same data as shown in
<xref ref-type="bibr" rid="bib1.bibx75" id="altparen.93"/>, based on various measurements;
<xref ref-type="bibr" rid="bib1.bibx9 bib1.bibx5 bib1.bibx25 bib1.bibx65 bib1.bibx39" id="altparen.94"/>) and MIPAS
satellite observations of SF<inline-formula><mml:math id="M54" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx71 bib1.bibx37" id="paren.95"/> at 500 K
potential temperature (20 km for the observations).</p>
      <p id="d1e2228">Overall, the reanalysis mean age lies within the uncertainty range of the
observations. In the tropics, the in situ observed mean age is significantly
lower than the reanalysis age, with only ERA-Interim reaching similar values.
However, MIPAS shows a much older mean age (above 2 years), which is similar to
MERRA-2 values. Compared to the in situ observations, age gradients in the
subtropics are too weak for all reanalyses due to the higher tropical age
values. In the middle and high latitudes, ERA-Interim and JRA-55 agree closely
with <inline-formula><mml:math id="M55" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>-based mean age observations, whereas MERRA-2 agrees better
with the SF<inline-formula><mml:math id="M56" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:math></inline-formula>-based mean age.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11"><?xmltex \currentcnt{11}?><label>Figure 11</label><caption><p id="d1e2253"><bold>(a)</bold> Latitude section of mean age at 20 km from in situ
observations <xref ref-type="bibr" rid="bib1.bibx74" id="paren.96"><named-content content-type="pre">e.g.</named-content></xref> shown using black symbols, from
different reanalysis data sets at 500 K potential temperature (red
represents ERA-Interim, blue represents JRA-55 and green represents MERRA-2) and from MIPAS satellite
observations (grey).  Dashed lines show the reanalysis mean age
including the correction for the finite age spectrum tail (see
text). Grey shading shows the range between maximum and minimum
MIPAS observations at each latitude. <bold>(b)</bold> Mean age time series in
the northern middle latitudes (40–50<inline-formula><mml:math id="M57" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N and
30–5 hPa, 600–1200 K for reanalyses). Coloured lines show the mean
age from the different reanalyses (red dashed line denoted the corrected mean
age for ERA-Interim). Black symbols show the mean age from the balloon
observations of <xref ref-type="bibr" rid="bib1.bibx27" id="text.97"/>, with error bars representing the
uncertainty of the observations.</p></caption>
        <?xmltex \igopts{width=213.395669pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f11.png"/>

      </fig>

      <p id="d1e2285">As the reanalysis age spectrum is truncated at 10 years, the respective mean
age is biased low by definition. This low bias can be corrected by applying a
correction for the finite age spectrum tail (see Sect. <xref ref-type="sec" rid="Ch1.S2"/>), and
the corrected mean ages are also compared to the observations in
Fig. <xref ref-type="fig" rid="Ch1.F11"/>a (dashed lines). For all reanalyses the tail
correction increases the mean age. This effect is moderate for ERA-Interim and
JRA-55, such that the corrected reanalysis mean age remains within the
observational uncertainty range. For MERRA-2, in contrast, the effect of the
tail correction is large, increasing the mean age by more than 2 years at high
latitudes. As a consequence, the tail-corrected MERRA-2 mean age is clearly
out of the observational uncertainty range (the tail correction effects will
be discussed further below).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F12"><?xmltex \currentcnt{12}?><label>Figure 12</label><caption><p id="d1e2294"><bold>(a)</bold> Age spectrum at 46<inline-formula><mml:math id="M58" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N and 700 K potential
temperature for June 1992 from ERA-Interim <bold>(a)</bold> and
MERRA-2 <bold>(b)</bold>. Red lines illustrate the correction method for the
finite age spectrum tail by fitting an exponential function to the tail at
transit times older than 5 years (see Sect. <xref ref-type="sec" rid="Ch1.S2"/>). The dashed red
vertical line shows the mean age for the tail-corrected spectrum, the dashed
black line shows the mean age for the uncorrected case. (Note the logarithmic <inline-formula><mml:math id="M59" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis, varying
over 3 orders of magnitude).</p></caption>
        <?xmltex \igopts{width=213.395669pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f12.png"/>

      </fig>

      <p id="d1e2329">A long-term observational mean age time series only exists for NH middle
latitudes from balloon-borne measurements of SF<inline-formula><mml:math id="M60" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">6</mml:mn></mml:msub></mml:math></inline-formula> and <inline-formula><mml:math id="M61" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CO</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>
<xref ref-type="bibr" rid="bib1.bibx26 bib1.bibx27" id="paren.98"/>. Long-term time series of reanalysis mean age in
the NH middle latitudes (averaged between 40 and 50<inline-formula><mml:math id="M62" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N and 600 and 1200 K,
which is approximately equivalent to the vertical layer for<?pagebreak page6098?> the observations of
30–5 hPa) are compared against this balloon observation time series in
Fig. <xref ref-type="fig" rid="Ch1.F11"/>b (note, that data points before 1989 include spin-up
effects, see Sect. <xref ref-type="sec" rid="Ch1.S2"/>). Clearly, the uncertainty arising from
using different reanalyses is of a similar magnitude as the uncertainty in the
observations, such that no conclusion is possible regarding which reanalysis
scenario is most realistic. However, The mean age trends substantially
differ between the reanalyses with negative trends for JRA-55
(<inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.17</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.01</mml:mn></mml:mrow></mml:math></inline-formula> yr decade<inline-formula><mml:math id="M64" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and MERRA-2 (<inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.18</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.01</mml:mn></mml:mrow></mml:math></inline-formula> yr decade<inline-formula><mml:math id="M66" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and a
positive trend for ERA-Interim (<inline-formula><mml:math id="M67" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.07</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.01</mml:mn></mml:mrow></mml:math></inline-formula> yr decade<inline-formula><mml:math id="M68" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), Hence, ERA-Interim
appears to agree best with the observed (non-significant) trend of
<inline-formula><mml:math id="M69" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.15</mml:mn><mml:mo>±</mml:mo><mml:mn mathvariant="normal">0.18</mml:mn></mml:mrow></mml:math></inline-formula> yr decade<inline-formula><mml:math id="M70" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> by <xref ref-type="bibr" rid="bib1.bibx27" id="text.99"/>. A “best fit” to the
observational time series results from applying the finite tail correction to
the ERA-Interim mean age, which is in remarkably good agreement with the
observations, regarding absolute values, variability and trend (red dashed
line).</p>
      <p id="d1e2473">Figure <xref ref-type="fig" rid="Ch1.F11"/>a shows a much stronger sensitivity to the tail
correction for the MERRA-2 mean age compared with the other reanalyses. This
stronger sensitivity for MERRA-2 results from differences in the spectrum
tail compared with the other two reanalyses (see Fig. <xref ref-type="fig" rid="Ch1.F2"/>), with
a substantially slower tail decrease for MERRA-2. Figure <xref ref-type="fig" rid="Ch1.F12"/>
illustrates a case of extreme differences between the reanalyses (June 1992
at 700 K potential temperature and 46<inline-formula><mml:math id="M71" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N). For ERA-Interim, the age
spectrum values decrease substantially over the<?pagebreak page6099?> 10 years of transit time
(more than an order of magnitude), indicating a strongly decaying spectrum
tail. For MERRA-2, in contrast, the tail decrease is much slower, leading to
a substantially larger tail decay timescale and to a less strict
normalisation, as previously discussed above (Fig. <xref ref-type="fig" rid="Ch1.F6"/>). This longer
tail decay timescale causes the finite tail correction applied to the age
spectra resolved over 10 years to have a much larger effect for MERRA-2
than for ERA-Interim and JRA-55. Figure <xref ref-type="fig" rid="Ch1.F12"/> further
shows that for MERRA-2 even the assumption of an exponentially decaying age
spectrum tail after about 5 years, which has generally been found to be valid for
observations <xref ref-type="bibr" rid="bib1.bibx24" id="paren.100"/> and models <xref ref-type="bibr" rid="bib1.bibx49" id="paren.101"/>, is violated in
some cases. Hence, the exponential finite tail correction is not applicable
for the MERRA-2 age spectra over 10 years of transit time. For that reason, the
inter-comparison presented in this paper is based on the uncorrected age
spectrum.</p>
</sec>
<sec id="Ch1.S6">
  <label>6</label><title>Discussion</title>
      <p id="d1e2510">Potential long-term changes in the stratospheric Brewer–Dobson
circulation and their relation to anthropogenically forced climate
change have been the subject of intense debate over recent
years. Climate models show a significant strengthening and
acceleration of the BDC <xref ref-type="bibr" rid="bib1.bibx13" id="paren.102"/>, resulting in a global
negative mean age trend <xref ref-type="bibr" rid="bib1.bibx14" id="paren.103"><named-content content-type="pre">e.g.</named-content></xref>. Trace gas
observations, in comparison, show no indication of a significant
long-term mean age trend <xref ref-type="bibr" rid="bib1.bibx26 bib1.bibx27" id="paren.104"/>. Studies
based on reanalysis meteorology have also provided a diverse picture
of mean age trends
<xref ref-type="bibr" rid="bib1.bibx19 bib1.bibx55 bib1.bibx59" id="paren.105"><named-content content-type="pre">e.g.</named-content></xref>
which is partly related to the different trend periods considered.</p>
      <p id="d1e2529">In view of such diversity in past published mean age trends, the qualitative
agreement between the “long-term” trends for 1989–2015 in the lower
stratosphere (below about 30 hPa) presented here for the newest three
reanalyses is remarkable (Fig. <xref ref-type="fig" rid="Ch1.F7"/>). In general, the mean age
trend is negative throughout the lower stratosphere with the largest values
in the tropical and SH lower stratosphere, indicating an accelerating shallow
BDC branch. These negative long-term mean age trends in current reanalyses
appear to be largely consistent with mean age trends from climate models over
even longer periods (century), representing the forced response of the BDC to
increasing greenhouse gas levels. Consistent with these negative mean age
trends and the related shift of the age spectrum peak (modal age) towards
shorter transit times (e.g. Fig. <xref ref-type="fig" rid="Ch1.F9"/>), most current
reanalyses show an increasing tropical mass flux <xref ref-type="bibr" rid="bib1.bibx1" id="paren.106"/> and
decreasing residual circulation transit times (Thomas Birner, personal
communication, 2018). However, <xref ref-type="bibr" rid="bib1.bibx1" id="text.107"/> further pointed out that
residual circulation trends may strongly depend on the method used for
calculating upwelling velocities.<?xmltex \hack{\newpage}?></p>
      <p id="d1e2543">Above about 30 hPa mean age trends and related circulation changes
depend more strongly on the respective reanalysis considered.
At these upper levels ERA-Interim shows ageing in the NH, which is not
included in the other two reanalyses. Hence, long-term changes in the
deep BDC branch appear to be less robustly represented in the reanalyses.
The NH ageing in ERA-Interim turns out to be related to a
strengthening age spectrum tail indicating changes in recirculation.
The evidence for recirculation changes agrees with the results of
<xref ref-type="bibr" rid="bib1.bibx59" id="text.108"/>, which showed that atmospheric mixing processes
substantially affect mean age trend patterns, with the strongest effects
on shorter timescales such as decades.</p>
      <p id="d1e2549">Over shorter periods of around a decade the reanalysis age of air trends show
substantial differences. For the pre-2000 period, trends in the NH above
about 600 K (approximately 24 km) are not consistent
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>) due to insignificant ERA-Interim trends
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>d). The strong negative mean age trends in the SH
and tropics, in contrast, consistently emerge from all reanalyses and
likely represent the combined effects of ozone depleting substances to
decrease mean age <xref ref-type="bibr" rid="bib1.bibx63" id="paren.109"/> and of volcanic aerosol from the
Pinatubo eruption to increase mean age at the beginning of the 1989–2001
period <xref ref-type="bibr" rid="bib1.bibx20" id="paren.110"/>. In particular, regarding the effect of Pinatubo
aerosol, differences in the response of the BDC and related differences in
age of air between the reanalyses are evident from the middle latitude mean
age time series in Fig. <xref ref-type="fig" rid="Ch1.F11"/>b. The increase in age after the
Pinatubo eruption is very strong in JRA-55, is weaker in ERA-Interim and
is absent in MERRA-2. These differences point to different representations of
stratospheric volcanic aerosol in the reanalyses causing the differences in
decadal BDC trends. In ERA-Interim and JRA-55 the effects of stratospheric
volcanic aerosol are only included by the assimilation of observed temperature
and wind data, as discussed in more detail by <xref ref-type="bibr" rid="bib1.bibx20" id="text.111"/>, whereas
MERRA-2 additionally assimilates aerosol optical depth <xref ref-type="bibr" rid="bib1.bibx30" id="paren.112"/>.
Furthermore, the effect of ozone depleting substances (ODSs) is very likely differently represented in the
reanalyses due to the usage of different ozone products. ERA-Interim uses an
ozone climatology, JRA-55 uses time-varying ozone fields from another model
simulation and MERRA-2 uses interactive ozone (see Sect. <xref ref-type="sec" rid="Ch1.S3"/>).
Hence, differences in the related effects on the BDC are to be expected.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F13" specific-use="star"><?xmltex \currentcnt{13}?><label>Figure 13</label><caption><p id="d1e2576">Mean age from ERA-Interim <bold>(a)</bold>, and differences to
JRA-55 <bold>(b)</bold> and MERRA-2 <bold>(c)</bold>, for the 1989–2015
climatological mean. The same for residual circulation transit time RCTT is
shown in <bold>(d)</bold>–<bold>(f)</bold>, and for ageing by mixing
in <bold>(g–i)</bold>. The thin black solid contours show the climatology values for
the respective reanalysis (e.g. ERA-Interim mean age in <bold>a</bold>,
MERRA-2 mean age in <bold>c</bold>), the thin black dashed lines show pressure
levels, the thick black solid line show the (WMO) tropopause and the blue contours
in <bold>(e)</bold>–<bold>(f)</bold> show relative differences for RCTTs in percent
(solid for positive and dashed for negative differences).</p></caption>
        <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/6085/2019/acp-19-6085-2019-f13.png"/>

      </fig>

      <?pagebreak page6100?><p id="d1e2616">For the post-2000 period, the age of air trends are even less consistent and no
clear common circulation change emerges from the comparison of the different
reanalyses (Fig. <xref ref-type="fig" rid="Ch1.F7"/>). Remarkably, the largest differences
between the reanalysis trends occur for the most recent period. This is
against the general expectation that a larger consistency between reanalyses
emerges for more recent periods, when observational data and the assimilation
procedures are more consistent. The inconsistency in the post-2000 trends is
mainly related to the fact that JRA-55 and MERRA-2 show opposite mean age
trends during the 2002–2015 period throughout the stratosphere
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>h, i), and that only ERA-Interim shows a
hemispheric dipole pattern (Fig. <xref ref-type="fig" rid="Ch1.F7"/>g). The hemispheric
dipole pattern in the mean age changes in ERA-Interim is related to changes in
the age spectrum tail (increasing tail in the NH and decreasing tail in the SH),
pointing to changes in recirculation that are in agreement with <xref ref-type="bibr" rid="bib1.bibx59" id="text.113"/>.
As the hemispheric dipole age trend pattern has been recently related to a
southward circulation shift by about 5<inline-formula><mml:math id="M72" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx72" id="paren.114"/>,
post-2000 age trend differences between the reanalyses could be caused by
differences in the representation of this circulation shift.</p>
      <p id="d1e2641">Comparison to the recently published reanalysis mean age trends by
<xref ref-type="bibr" rid="bib1.bibx16" id="text.115"/> may reveal interesting differences regarding the
representation of the BDC between kinematic transport models as used in their
study (BASCOE model) and diabatic transport models as used here (CLaMS).
Regarding the climatology, the mean age from MERRA-2 shows substantially higher
values than the other reanalyses for both diabatic and kinematic transport
<xref ref-type="bibr" rid="bib1.bibx16" id="paren.116"><named-content content-type="pre">see Fig. <xref ref-type="fig" rid="Ch1.F1"/>, and</named-content><named-content content-type="post">Fig. 3</named-content></xref>.
The differences in diabatic heating rates, with weaker tropical upwelling for
MERRA-2 (Fig. <xref ref-type="fig" rid="Ch1.F5"/>), are qualitatively consistent with the
differences in mean age in the diabatic model calculation. The fact that
similar mean age differences were found by <xref ref-type="bibr" rid="bib1.bibx16" id="text.117"/> suggests
that differences in the reanalysis vertical winds, which drive their
kinematic model calculations, could be similar to the differences in heating
rates.</p>
      <?pagebreak page6101?><p id="d1e2661">However, as previously earlier, the differences in heating rates alone cannot
fully explain the simulated mean age differences as shown in the following.
Figure <xref ref-type="fig" rid="Ch1.F13"/> shows the ERA-Interim climatological mean age and
residual circulation transit times (RCTTs), and differences to the other
reanalyses. Here, RCTTs are calculated from the diabatic residual circulation
in isentropic coordinates, as described in Sect. <xref ref-type="sec" rid="Ch1.S2"/>. The mean age
from MERRA-2 is older than ERA-Interim by more than 2 years
throughout most parts of the stratosphere (Fig. <xref ref-type="fig" rid="Ch1.F13"/>c), whereas
differences in RCTTs are below 0.5 years (Fig. <xref ref-type="fig" rid="Ch1.F13"/>f). Hence,
differences in the representation of mixing processes must play a role.</p>
      <p id="d1e2672">The net mixing effect on mean age (ageing by mixing), calculated as the
difference between the mean age and the RCTT following <xref ref-type="bibr" rid="bib1.bibx34" id="text.118"/> and further
described in Sect. <xref ref-type="sec" rid="Ch1.S2"/>, is shown in Fig. <xref ref-type="fig" rid="Ch1.F13"/>g–i.
This ageing by mixing is about 2 years larger for MERRA-2 than for
ERA-Interim in most parts of the lower stratosphere, and clearly explains
the large difference in the mean age between the reanalyses. However, ageing by
mixing depends on both local mixing characteristics in the lower stratosphere
and the transit time of tropical upwelling, which controls the timescale for
mixing to affect the ascending air <xref ref-type="bibr" rid="bib1.bibx34 bib1.bibx59" id="paren.119"><named-content content-type="pre">see</named-content></xref>.
Hence, the differences in the ageing by mixing between ERA-Interim and
MERRA-2 may be caused by either differences in local mixing (eddy
diffusivity) or by differences in the RCTTs. From a tropical leaky pipe model
perspective ageing by mixing is even linearly related to RCTT, with a longer
RCTT causing a larger ageing by mixing <xref ref-type="bibr" rid="bib1.bibx56 bib1.bibx23" id="paren.120"/>. In
percent, the differences in RCTTs between MERRA-2 and ERA-Interim in the
tropical lower stratosphere are large (about 50 %, see blue contours in
Fig. <xref ref-type="fig" rid="Ch1.F13"/>f), and likely cause a related difference in ageing by
mixing. Overall, the larger ageing by mixing for MERRA-2 compared with
ERA-Interim clearly causes the differences in mean age. Deeper insight into
potential differences in local mixing characteristics could be gained by a
reanalysis inter-comparison of effective diffusivity
<xref ref-type="bibr" rid="bib1.bibx41 bib1.bibx2" id="paren.121"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d1e2698">For the long-term mean age trends (1989–2015) both diabatic and kinematic
transport representations result in very similar results for all three
reanalyses, as evident from the comparison of Fig. <xref ref-type="fig" rid="Ch1.F7"/> with
Fig. 12 of <xref ref-type="bibr" rid="bib1.bibx16" id="text.122"/>. This good agreement regarding long-term
trends again points to a robust representation of the effect of greenhouse
gas-induced warming in forcing trends in the BDC. However, regarding decadal changes
over shorter periods, the results from diabatic and kinematic transport
models show more substantial differences. The strongest differences emerge for
the pre-2000 period for ERA-Interim and for the post-2000 period for
MERRA-2. For the former case, diabatic transport in CLaMS results in
negative mean age trends throughout the SH and tropical stratosphere
(Fig. <xref ref-type="fig" rid="Ch1.F7"/>d), whereas kinematic transport in BASCOE results in
positive trends in these regions <xref ref-type="bibr" rid="bib1.bibx16" id="paren.123"><named-content content-type="post">Fig. 12</named-content></xref>. As
pre-2000 decadal trends are likely controlled by the effects of ozone
depleting substances and Pinatubo volcanic aerosol on the BDC, the
differences in age trends for this period point to differences in the
representation of these processes between diabatic and kinematic transport.
In particular differences in the effect of volcanic aerosol (e.g. due to the
Pinatubo eruption in June 1991), with increasing mean age for diabatic
transport and no significant age changes for kinematic transport seem to be
critical, and have also been noted by <xref ref-type="bibr" rid="bib1.bibx16" id="text.124"/>. For the latter
case (post-2000 period for MERRA-2), diabatic transport in CLaMS results in
negative trends throughout the stratosphere (Fig. <xref ref-type="fig" rid="Ch1.F7"/>i),
whereas kinematic transport in BASCOE results in positive age trends
<xref ref-type="bibr" rid="bib1.bibx16" id="paren.125"><named-content content-type="post">Fig. 12</named-content></xref>. Furthermore, less striking differences
between diabatic and kinematic mean age trends emerge for MERRA-2 during the
pre-2000 period, where kinematic age trends are more negative compared with
diabatic trends <xref ref-type="bibr" rid="bib1.bibx16" id="paren.126"><named-content content-type="pre">Fig. <xref ref-type="fig" rid="Ch1.F7"/>f and</named-content><named-content content-type="post">Fig. 12</named-content></xref>.
Weak differences also occur for ERA-Interim
from 2002 to 2015, where the NH ageing appears stronger in the diabatic age
trends <xref ref-type="bibr" rid="bib1.bibx16" id="paren.127"><named-content content-type="pre">Fig. <xref ref-type="fig" rid="Ch1.F7"/>g and</named-content><named-content content-type="post">Fig. 12</named-content></xref>. The
causes for the differences regarding decadal trends in the BDC on shorter
periods between diabatic and kinematic transport representations, as well as
between the different reanalyses, are unclear to date, but appear to be a
promising subject for future analysis aiming to improve consistency between
the reanalyses.</p>
</sec>
<sec id="Ch1.S7" sec-type="conclusions">
  <label>7</label><title>Conclusions</title>
      <p id="d1e2750">We compared stratospheric mean age and the full age spectrum from
simulations with the diabatic CLaMS model driven by different
reanalyses (ERA-Interim, JRA-55 and MERRA-2) to investigate the
robustness in the representation of the climatology, seasonality and trends of
the Brewer–Dobson circulation in current generation reanalysis data
sets. Considering the full (time-dependent) age spectrum in a data
inter-comparison is novel and provides clearer insights into circulation differences
than considering mean age alone. Climatological mean age differs
significantly between the different reanalyses, with JRA-55 showing
the youngest age and MERRA-2 showing the oldest age throughout almost
the entire stratosphere. The substantially older mean age for MERRA-2
appears to be related to a more pronounced age spectrum tail,
indicating a stronger effect of the recirculation of air into the
tropics. A comparison of residual circulation and mixing effects on
mean age confirms that the net mixing effect (including recirculation)
is necessary to explain the mean age differences between MERRA-2
and ERA-Interim. The seasonality in the BDC is robustly represented,
with very similar mean age seasonality and similar seasonal age
spectrum peaks emerging for all reanalyses. Comparison to
balloon-borne mean age observations reveals a similarly large spread
in simulated and observed mean ages and allows no clear conclusions to
be drawn regarding the reliability of the different reanalyses.</p>
      <p id="d1e2753">In particular, long-term trends in the lower stratosphere (below about
30 hPa) during the 1989–2015 period are robustly represented in the
reanalyses mainly showing decreasing mean age, which is strongest in the SH and
tropical lower stratosphere. Related to this mean age decrease is a<?pagebreak page6102?> robust
shift of the age spectrum towards shorter transit times and an increase in
the fraction of young air masses. These long-term age of air changes from
reanalyses resemble results from climate model simulations over even longer
periods, which simulate an acceleration of the shallow branch of the
stratospheric BDC as the forced response to increasing greenhouse gas levels.
At upper levels (above 30 hPa), mean age changes in the reanalyses appear
less robust, pointing to a less robust representation of changes in the deep
BDC branch.</p>
      <p id="d1e2756">For shorter periods of about a decade (here 1989–2001 and 2002–2015), the age
of air changes are more diverse and depend on the specific reanalysis
considered. These decadal age changes may even disagree in sign globally for
certain periods. Moreover, the hemispheric asymmetric dipole in mean age
trends for 2002–2015, as viewed by satellite observations, only emerges for
ERA-Interim. Hence, decadal variability in the Brewer–Dobson circulation and
the various factors involved (e.g. QBO, ENSO, ODS and volcanic aerosol) turn
out not to be robustly represented in current generation reanalyses.</p>
</sec>

      
      </body>
    <back><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e2763">The CLaMS model data used for this paper may be requested
from the corresponding author (f.ploeger@fz-juelich.de).</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e2769">FP carried out the ERA-Interim-driven and JRA-55-driven model simulations and the data analysis.
BL and XY prepared the reanalysis data. EC carried out the MERRA-22-driven
simulation. PK, MT, XY and BL contributed code for the analysis.
BL, TB, PK and MD contributed to the design of the analysis. AE provided the
observational mean age data. MD, PK, TB, MT, MR, EC, BL, XY provided helpful
discussions and comments. FP wrote the paper with contributions from all
co-authors.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e2775">The authors declare that they have no conflict of
interest.</p>
  </notes><notes notes-type="sistatement"><title>Special issue statement</title>

      <p id="d1e2781">This article is part of the special issue “The SPARC Reanalysis
Intercomparison Project (S-RIP) (ACP/ESSD inter-journal SI)”. It is not
associated with a conference.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e2787">We thank Marta Abalos, Hella Garny, Aurelien Podglajen and Gebhard Günther
for helpful discussions. We are grateful to Nicole Thomas for programming
support, and the ECMWF, NASA and the Japanese Meteorological Agency for
providing the reanalysis data. This study was funded by the Helmholtz
Association under grant no. VH-NG-1128 (Helmholtz Young Investigators Group
A–SPECi).</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e2793">The article processing charges for this
<?xmltex \hack{\newline}?>open-access publication were covered by a Research
<?xmltex \hack{\newline}?> Centre of the Helmholtz Association.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e2803">This paper was edited by Gabriele Stiller and reviewed by Eric Ray and two anonymous referees.</p>
  </notes><ref-list>
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    <!--<article-title-html>How robust are stratospheric age of air trends from different reanalyses?</article-title-html>
<abstract-html><p>An accelerating Brewer–Dobson circulation (BDC) is a robust signal
of climate change in model predictions but has been questioned by
trace gas observations. We analyse the stratospheric mean age of air and
the full age spectrum as measures for the BDC and its trend. Age
of air is calculated using the Chemical Lagrangian Model of the
Stratosphere (CLaMS) driven by ERA-Interim, JRA-55 and MERRA-2
reanalysis data to assess the robustness of the representation of
the BDC in current generation meteorological reanalyses. We find
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reanalysis, with JRA-55 showing the youngest and MERRA-2 the
oldest mean age. Consideration of the age spectrum indicates that
the older air for MERRA-2 is related to a stronger spectrum tail,
which is likely associated with weaker tropical upwelling and stronger
recirculation. Seasonality of stratospheric transport is robustly
represented in reanalyses, with similar mean age variations
and age spectrum peaks. Long-term changes from 1989 to 2015 turn
out to be similar for the reanalyses with mainly decreasing mean age
accompanied by a shift of the age spectrum peak towards shorter
transit times, resembling the forced response in climate model
simulations to increasing greenhouse gas concentrations. For the
shorter periods, 1989–2001 and 2002–2015, the age of air changes are
less robust. Only ERA-Interim shows the hemispheric dipole pattern
in age changes from 2002 to 2015 as viewed by recent satellite
observations. Consequently, the representation of decadal
variability of the BDC in current generation reanalyses appears less
robust and is a major uncertainty of modelling the BDC.</p></abstract-html>
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