<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing with OASIS Tables v3.0 20080202//EN" "journalpub-oasis3.dtd">
<article xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:oasis="http://docs.oasis-open.org/ns/oasis-exchange/table" xml:lang="en" dtd-version="3.0">
  <front>
    <journal-meta><journal-id journal-id-type="publisher">ACP</journal-id><journal-title-group>
    <journal-title>Atmospheric Chemistry and Physics</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1680-7324</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-19-10217-2019</article-id><title-group><article-title>The MetVed model: development and evaluation of emissions<?xmltex \hack{\break}?> from residential wood combustion at high spatio-temporal resolution in Norway</article-title><alt-title>MetVed model for RWC</alt-title>
      </title-group><?xmltex \runningtitle{MetVed model for RWC}?><?xmltex \runningauthor{H. Grythe et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes">
          <name><surname>Grythe</surname><given-names>Henrik</given-names></name>
          <email>heg@nilu.no</email>
        <ext-link>https://orcid.org/0000-0001-5074-4858</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Lopez-Aparicio</surname><given-names>Susana</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-0426-9667</ext-link></contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Vogt</surname><given-names>Matthias</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Vo Thanh</surname><given-names>Dam</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Hak</surname><given-names>Claudia</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Halse</surname><given-names>Anne Karine</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Hamer</surname><given-names>Paul</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no">
          <name><surname>Sousa Santos</surname><given-names>Gabriela</given-names></name>
          
        </contrib>
        <aff id="aff1"><institution>Norwegian Institute for Air Research (NILU), P.O. Box 100, 2027  Kjeller, Norway</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Henrik Grythe (heg@nilu.no)</corresp></author-notes><pub-date><day>13</day><month>August</month><year>2019</year></pub-date>
      
      <volume>19</volume>
      <issue>15</issue>
      <fpage>10217</fpage><lpage>10237</lpage>
      <history>
        <date date-type="received"><day>30</day><month>January</month><year>2019</year></date>
           <date date-type="rev-request"><day>22</day><month>March</month><year>2019</year></date>
           <date date-type="rev-recd"><day>27</day><month>June</month><year>2019</year></date>
           <date date-type="accepted"><day>5</day><month>July</month><year>2019</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2019 </copyright-statement>
        <copyright-year>2019</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://acp.copernicus.org/articles/.html">This article is available from https://acp.copernicus.org/articles/.html</self-uri><self-uri xlink:href="https://acp.copernicus.org/articles/.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/.pdf</self-uri>
      <abstract><title>Abstract</title>
    <p id="d1e143">We present here emissions estimated from a newly developed emission model for residential wood combustion (RWC) at high spatial and temporal resolution, which we name the MetVed model. The model estimates hourly emissions resolved on a 250 <inline-formula><mml:math id="M1" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid resolution for several compounds, including particulate matter (<inline-formula><mml:math id="M2" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">PM</mml:mi></mml:mrow></mml:math></inline-formula>), black carbon (<inline-formula><mml:math id="M3" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">BC</mml:mi></mml:mrow></mml:math></inline-formula>) and polycyclic aromatic hydrocarbons (<inline-formula><mml:math id="M4" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">PAHs</mml:mi></mml:mrow></mml:math></inline-formula>) in Norway for a 12-year period. The model uses novel input data and calculation methods that combine databases built with an unprecedented high level of detail and near-national coverage. The model establishes wood burning potential at the grid based on the dependencies between variables that influence emissions: i.e. outdoor temperature, number of and type and size of dwellings, type of available heating technologies, distribution of wood-based heating installations and their associated emission factors. RWC activity with a 1 h temporal profile was produced by combining heating degree day and hourly and weekday activity profiles reported by wood consumers in official statistics. This approach results in an improved characterisation of the spatio-temporal distribution of wood use, and subsequently of emissions, required for urban air quality assessments. Whereas most variables are calculated based on bottom-up approaches on a 250 <inline-formula><mml:math id="M5" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> spatial grid, the MetVed model is set up to use official wood consumption at the county level and then distributes consumption to individual grids proportional to the physical traits of the residences within it. MetVed combines consumption with official emission factors that makes the emissions also upward scalable from the 250 <inline-formula><mml:math id="M6" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid to the national level.</p>
    <p id="d1e195">The MetVed spatial distribution obtained was compared at the urban scale to other existing emissions at the same scale. The annual urban emissions, developed according to different spatial proxies, were found to have differences up to an order of magnitude. The MetVed total annual <inline-formula><mml:math id="M7" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions in the urban domains compare well to emissions adjusted based on concentration measurements. In addition, hourly <inline-formula><mml:math id="M8" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations estimated by an Eulerian dispersion model using MetVed emissions were compared to measurements at air quality stations. Both hourly daily profiles and the seasonality of <inline-formula><mml:math id="M9" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> show a slight overestimation of <inline-formula><mml:math id="M10" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> levels. However, a comparison with black carbon from biomass burning and benzo(a)pyrene measurements indicates higher emissions during winter than that obtained by MetVed. The accuracy of urban emissions from RWC relies on the accuracy of the wood consumption (activity data), emission factors and the spatio-temporal distribution. While there are still knowledge gaps regarding emissions, MetVed represents a vast improvement in the spatial and temporal distribution of RWC.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e251">Wood burning for residential heating emits to the atmosphere primary aerosol particles, short-lived climate gases, and organic volatile and semi-volatile compounds (<inline-formula><mml:math id="M11" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">VOCs</mml:mi></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M12" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">SVOCs</mml:mi></mml:mrow></mml:math></inline-formula>), which can condense on existing primary particles, which in turn leads to increased particulate matter mass <xref ref-type="bibr" rid="bib1.bibx34" id="paren.1"><named-content content-type="pre">e.g.</named-content></xref>. These aerosol particles play an important role in air quality and hence on human health. Throughout most urban areas, natural aerosol concentrations are augmented by anthropogenic emission sources, such as particles emitted<?pagebreak page10218?> from traffic and residential heating. Combined with strong emission sources, the conditions in urban areas often prevent efficient dilution of atmospheric pollutants, causing citizens to be disproportionately exposed to high local pollution levels. Together with nitrogen oxides (<inline-formula><mml:math id="M13" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">NO</mml:mi><mml:mi>x</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), elevated particulate matter (<inline-formula><mml:math id="M14" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">PM</mml:mi></mml:mrow></mml:math></inline-formula>) concentrations remain among the major concerns for human health. In particular, fine <inline-formula><mml:math id="M15" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">PM</mml:mi></mml:mrow></mml:math></inline-formula> from combustion sources is consistently associated with cardiovascular diseases and mortality <xref ref-type="bibr" rid="bib1.bibx28" id="paren.2"><named-content content-type="pre">e.g.</named-content></xref>.</p>
      <p id="d1e308">The emissions from residential wood combustion (RWC) are considered a main contributor to harmful atmospheric pollutants in many European cities <xref ref-type="bibr" rid="bib1.bibx11" id="paren.3"><named-content content-type="pre">e.g.</named-content></xref>. For aerosol particles, the mass contribution from RWC is highlighted as a large source across Europe <xref ref-type="bibr" rid="bib1.bibx17" id="paren.4"/>. In Nordic countries, RWC is an especially large source of aerosols, contributing more than 50 % of the total urban and national <inline-formula><mml:math id="M16" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> anthropogenic emissions, making it the single largest source. RWC has been found to account for as much as 50 %–80 % of urban <inline-formula><mml:math id="M17" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> mass concentrations <xref ref-type="bibr" rid="bib1.bibx18" id="paren.5"/>. In Nordic countries, there is a strong tradition tied to wood burning. The combination of readily available wood supply with an especially strong aesthetic appeal of wood burning stoves <xref ref-type="bibr" rid="bib1.bibx20" id="paren.6"/> for the Nordic population leads to many residential buildings relying in part on heating by wood burning during the extended winter period <xref ref-type="bibr" rid="bib1.bibx5" id="paren.7"/>. This tradition is widespread across the Nordic area, but there are also some important differences among the Nordic countries. Boilers are commonly used in Sweden and Denmark, whereas masonry and sauna stoves are more common in Finland <xref ref-type="bibr" rid="bib1.bibx2" id="paren.8"/>. In Norway, the installations for RWC mainly consist of stoves and open fireplaces, which are predominantly small space heaters, in contrast to boilers, which are typically larger heating devices. This is manifested through an estimated 2.1 million domestic wood burning heating installations in the 2.4 million Norwegian households, with an additional 900 000 in the 1 million cabins and summer houses of Norway (Norsk Varme, personal communication, 2018).</p>
      <p id="d1e354">Emissions from RWC are dependent on many factors such as the type and size of the wood (e.g. logs, chips, pellets), the burning efficiency of the wood installation, the draft conditions, fuel load, burning conditions, the moisture content of the wood, and the operation itself <xref ref-type="bibr" rid="bib1.bibx2" id="paren.9"><named-content content-type="pre">e.g. automatic or manual feeding</named-content></xref>. The resulting outdoor concentration of pollutants from RWC emissions is in addition dependent on the emission altitude, atmospheric conditions and removal efficiency (deposition and dilution). As high RWC activity is often combined with low temperatures, when the frequent presence of temperature inversions enhances pollution levels, meteorological conditions also play an important role. A temperature inversion occurs when the air temperature rises with altitude, resulting in reduced buoyancy of air masses at the surface, and consequently the vertical mixing of air is reduced. Since RWC is generally produced within the boundary layer, temperature inversions trap the pollution at low altitudes, leading to increased concentration levels.</p>
      <p id="d1e362">In Norway, where there are approximately 3 million individual wood burning installations, establishing the emissions from each individual point source constitutes a challenge. Besides, emissions from RWC largely differ both temporally and spatially within a city and across regions. It is therefore essential to develop accurate emission inventories, with a high level of both spatial and temporal resolution, that capture both modes of variability. This will support the understanding of the processes that lead to high pollution episodes in winter, predict them, assess the potential impact on human health and evaluate measures to reduce RWC emissions.</p>
      <p id="d1e366">The Norwegian emissions for RWC reported to the Convention on Long-Range Transboundary Air Pollution (CLRTAP; <uri>http://www.ceip.at</uri>, last access: 12 June 2019) are calculated based on wood consumption at a county level, derived from self-reporting questionnaires and information about the available technology, distinguishing between open fireplaces and wood stoves produced before 1998 and after 1998 <xref ref-type="bibr" rid="bib1.bibx1" id="paren.10"/>. Wood consumption per technology is thereafter combined with official Norwegian emission factors that represent real-world firing conditions <xref ref-type="bibr" rid="bib1.bibx33" id="paren.11"/>. Different emission factors are used in and around the three largest urban centres in Norway, based on the assumption of different firing habits in urban areas from those used for the rest of the country <xref ref-type="bibr" rid="bib1.bibx26" id="paren.12"/>.</p>
      <p id="d1e381">There exist several methods to allocate and grid emissions from RWC down to the urban scale. Common to all these RWC emission methodologies is that they use a downscaling approach to try to resolve household-differentiated emissions. To enable this, accurate and detailed input data down to the urban scale are required. Data availability determines to a large extent the type of proxy that can be used to spatially distribute emissions for RWC at high resolution. Thus, the initial and crucial step in the development of high-resolution RWC emission inventories is the collection of suitable data.</p>
      <p id="d1e384">For the spatial distribution and gridding of emissions from RWC, the most common method is a downscaling approach applied to existing lower-resolution emissions or activity data by means of auxiliary data <xref ref-type="bibr" rid="bib1.bibx40 bib1.bibx10" id="paren.13"/>. The most common parameters used for downscaling have been population or dwelling density. The underlying assumption is that emissions are equal from all households and therefore it positively correlates with the increase in population or dwelling density. Across European countries, this assumption has led to overestimation of emissions in urban areas <xref ref-type="bibr" rid="bib1.bibx40" id="paren.14"/>. In southern European countries, RWC is more common in rural than in urban areas, and therefore emissions per household decrease with increases in population density <xref ref-type="bibr" rid="bib1.bibx39" id="paren.15"><named-content content-type="pre">e.g.</named-content></xref>. In Nordic countries, on the contrary, RWC is common also in urban areas, and new proxies have been developed to capture the variability at the urban scale. In Denmark, a differential distribution of emissions according to the type of<?pagebreak page10219?> dwelling is proposed, and accordingly detached houses are assumed to have higher activity than, for instance, apartments <xref ref-type="bibr" rid="bib1.bibx27" id="paren.16"/>. In Sweden, national total emissions are calculated based on the domestic energy budget calculations and emission factors, and then the gridding of emissions is done based on the number of wood boilers, wood stoves, pellet boilers and oil boilers on a municipality level <xref ref-type="bibr" rid="bib1.bibx3" id="paren.17"/>.</p>
      <p id="d1e404">Uncertainties in emissions for RWC at the urban scale are due to the activity data (i.e. wood consumption), emission factors per technology and on the spatio-temporal distribution of emissions. In this work, we aim to contribute to the improvement of the distribution of RWC emissions at high spatial and temporal resolutions, and we subsequently aim to reduce the uncertainties on emissions and dispersion modelling at the urban scale. Hereby, we describe the MetVed model based on defining the wood burning potential at 250 <inline-formula><mml:math id="M18" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> resolution resulting from the analysis of several combined databases built with an unprecedented high level of detail. Near-national coverage of the amount and types of dwellings, the type of available residential heating technologies (e.g. district heating, heat pump) and individual wood stove appliances set up the basis of the model. Emissions are distributed in time based on heating demand, which is based on the outdoor temperature. In addition, the model distributes emissions in two vertical layers depending on whether wood consumption occurs in houses or apartments, resulting in a lower or upper injection layer, respectively. The MetVed model constitutes a significant step forward in the development and improvement of high-resolution emissions from RWC.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Model input data</title>
      <p id="d1e423">The MetVed model is set up with several routines for the calculation of wood consumption at the at 250 <inline-formula><mml:math id="M19" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid level. A schematic of the model calculations is shown in Fig. <xref ref-type="fig" rid="Ch1.F1"/>. Emission factors for three different burning technologies are provided by <xref ref-type="bibr" rid="bib1.bibx33" id="text.18"/>: old stoves (pre-dates 1998), new stoves (1998) and open fireplaces. Emission factors are combined with aggregated consumption statistics at the county level with the same differentiation. The other main input data sets are the location of fireplaces from the fire and rescue agencies registry, data on dwelling types and available residential heating technology obtained from the largest real estate advertisement portal in Norway, and energy consumption from the Norwegian Energy Labelling System (ENOVA). The model additionally uses outdoor temperature together with a diurnal and weekly variation of woodfuel consumption in Norway to establish the time dependence of emissions. As with most emission models, the accuracy and level of detail depends on the available input data. For MetVed, the model output resolution is determined by the resolution of the input dwelling information (i.e. 250 <inline-formula><mml:math id="M20" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><?xmltex \currentcnt{1}?><label>Figure 1</label><caption><p id="d1e449">Schematic representation of the data flow and calculations done in MetVed.</p></caption>
        <?xmltex \igopts{width=483.69685pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f01.png"/>

      </fig>

      <p id="d1e458"><?xmltex \hack{\newpage}?>As the above data sets constitute the basis for the analysis of RWC in Norwegian households we provide a detailed description of each data set in this section. The utilisation of high-resolution data is important for the MetVed model to produce valuable results. The principle behind building an emission model with more bottom-up principles relies heavily on gathered underlying data. Thus, to achieve accurate emissions, new avenues for data gathering is an important field of development.</p>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>Wood consumption</title>
      <p id="d1e470">The use of wood for residential heating for the years from 2005 to 2016 is provided based on the responses to the Statistics Norway's Travel and Holiday Survey. Data on wood consumption are collected and officially reported by Statistics Norway at the county level. The survey gathers data in four quarterly surveys covering the preceding 12 months. The calculated consumption of wood is the average of five consecutive quarterly surveys. The survey contains 25 questions regarding wood burning for residential heating. The sampling pool of the survey is drawn at a nationwide level and is considered representative for all counties. Wood consumption in each of the three technology classes (open fireplace, stove produced before 1998 and stove produced after 1998) is available for each county, and these data are used in the MetVed model as input because finer resolution is not available.</p>
      <p id="d1e473">Reported wood mass (<inline-formula><mml:math id="M21" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kg</mml:mi></mml:mrow></mml:math></inline-formula>) from questionnaires is recalculated to represent dry wood consumption by assuming an 18 % water content. In that way, wood consumption corresponds with emission factors that represent grams of pollutant per kilogram of dried wood. According to Statistics Norway, there are several elements of uncertainty in the wood consumption data, such as the survey sample size and the employed conversion factors (e.g. mass of bags of wood reported as volume). Statistics Norway concluded that the coefficient of variation of the total wood consumption is below 3 % based on an uncertainty study carried out in 2011 <xref ref-type="bibr" rid="bib1.bibx36" id="paren.19"/>. The uncertainty is higher at the county level as the values are based on smaller samples. Large-scale production of fuelwood and sales of wood (estimated 70 % of consumption) are nearly exclusively birch, and also untraded wood will contain significant birch. As no other information is available, consumption is assumed to be birch, in accordance with emission factors.</p>
</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Emission factors</title>
      <?pagebreak page10220?><p id="d1e495">The Norwegian emission factors are listed in Table <xref ref-type="table" rid="Ch1.T1"/> and were established by <xref ref-type="bibr" rid="bib1.bibx33" id="text.20"/> for three categories: (i) open fireplaces, (ii) stoves produced before 1998 and (iii) stoves produced after 1998. The emissions factors are determined by laboratory experiments following the Norwegian standard for testing enclosed wood heaters and smoke emissions <xref ref-type="bibr" rid="bib1.bibx25" id="paren.21"/> and are considered as representative of real-world conditions. The particle sampling is carried out in a dilution tunnel in order to mimic the dilution and cooling effects when the smoke exits the chimney. In this way, the particle sampling also accounts for condensed matter. The Norwegian standard requires that the type of wood used is birch, so all emission factors are based on birch wood.</p>

<table-wrap id="Ch1.T1"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e508">Emission factors as amount of pollutant per amount of dry wood <xref ref-type="bibr" rid="bib1.bibx33" id="paren.22"/>.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Pollutant</oasis:entry>
         <oasis:entry colname="col2">Open</oasis:entry>
         <oasis:entry colname="col3">Wood stove</oasis:entry>
         <oasis:entry colname="col4">Wood stove</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">fireplace</oasis:entry>
         <oasis:entry colname="col3">(–1998)</oasis:entry>
         <oasis:entry colname="col4">(1998–)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">CO (g kg<inline-formula><mml:math id="M22" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">126.3</oasis:entry>
         <oasis:entry colname="col3">150</oasis:entry>
         <oasis:entry colname="col4">50.5</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M23" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CH</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> (g kg<inline-formula><mml:math id="M24" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">5.3</oasis:entry>
         <oasis:entry colname="col3">5.3</oasis:entry>
         <oasis:entry colname="col4">5.3</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PM<inline-formula><mml:math id="M25" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:math></inline-formula> (g kg<inline-formula><mml:math id="M26" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">17.0</oasis:entry>
         <oasis:entry colname="col3">17.1</oasis:entry>
         <oasis:entry colname="col4">12.0</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PM<inline-formula><mml:math id="M27" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> (g kg<inline-formula><mml:math id="M28" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">16.4</oasis:entry>
         <oasis:entry colname="col3">16.5</oasis:entry>
         <oasis:entry colname="col4">11.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BC (% PM<inline-formula><mml:math id="M29" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">9</oasis:entry>
         <oasis:entry colname="col3">1.01</oasis:entry>
         <oasis:entry colname="col4">0.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PAH<inline-formula><mml:math id="M30" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">TOTAL</mml:mi></mml:msub></mml:math></inline-formula> (g t<inline-formula><mml:math id="M31" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">17.4</oasis:entry>
         <oasis:entry colname="col3">52</oasis:entry>
         <oasis:entry colname="col4">0.0226</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d1e760"><xref ref-type="bibr" rid="bib1.bibx33" id="text.23"/> proposed two sets of emission factors depending on different firing conditions in Norwegian cities and rural areas. The reasoning behind the two emission factors is that users in the countryside fire their stove with low air intake during the night and other users do not <xref ref-type="bibr" rid="bib1.bibx12" id="paren.24"/>. To our knowledge, there is not a solid and updated study that supports this assumption; thus we presume the same firing conditions as in large cities across all of Norway.</p>
</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><title>Dwelling number</title>
      <p id="d1e776">The data set containing the type and number of dwellings is obtained from Statistics Norway <xref ref-type="bibr" rid="bib1.bibx4" id="paren.25"/>. The data set originates from the state tax agency registry (SERG), and that covers all households in Norway. It can be considered complete and up to date. The gridded version at 250 <inline-formula><mml:math id="M32" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> of this registry maps the number of dwellings, the number of detached houses, duplexes, townhouses, the number of dwellings in apartment blocks and other dwellings. An example of the dwelling number data set (for the municipality of Stavanger) is shown in Fig. <xref ref-type="fig" rid="Ch1.F2"/>. The grid number of total houses (Fig. <xref ref-type="fig" rid="Ch1.F2"/>a) has the highest density of dwellings in downtown Stavanger. This is also where apartments (Fig. <xref ref-type="fig" rid="Ch1.F2"/>c) have their highest density, while detached houses (Fig. <xref ref-type="fig" rid="Ch1.F2"/>b) are much more uniformly spread through out the municipality. This illustrates a typical feature of most urban areas, where a city centre typically consists of mainly apartment blocks, whereas detached houses and duplexes are more prevalent in suburban areas. In Norway in 2017, there were around 2.5 million registered dwellings of which 50 % are detached houses, 9 % duplexes, 12 % townhouses, 24 % apartments and 5 % are classified as others. The spatial distribution of dwelling types differs across region and area. This is especially so for the apartment share, which ranges from 77 % in the Oslo municipality to 0 % in many rural municipalities.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><?xmltex \currentcnt{2}?><label>Figure 2</label><caption><p id="d1e801">Example of part of the input data used in the MetVed model in the Municipality of Stavanger. <bold>(a)</bold> Total dwelling number at 250 <inline-formula><mml:math id="M33" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid resolution. <bold>(b)</bold> Number of detached hours. <bold>(c)</bold> Number of apartments. <bold>(d)</bold> Individual wood burning installations from the fire and rescue agency. <bold>(e)</bold> Density of wood burning installations. <bold>(f)</bold> Share (%) of wood-based installations for residential heating obtained from the web-crawled data set.  Background map: © OpenStreetMap contributors 2019. Distributed under a Creative Commons BY-SA License.</p></caption>
          <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f02.jpg"/>

        </fig>

<?xmltex \hack{\newpage}?>
</sec>
<?pagebreak page10221?><sec id="Ch1.S2.SS4">
  <label>2.4</label><title>Fire and rescue agencies registry</title>
      <p id="d1e847">In Norway, there are 620 fire stations divided among <inline-formula><mml:math id="M34" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">300</mml:mn></mml:mrow></mml:math></inline-formula> fire department agencies. The fire and rescue agencies are responsible for inspecting and assessing all firing installations. These are dominated by residential heating installations, but the database also contains a small number of cooking appliances. The agencies carry out routine inspections as part of fire hazard safety procedures. During these inspections, information such as geographical location and type of installation is collected in a local database by each agency.</p>
      <p id="d1e860">In this study, we contacted 270 fire and rescue agencies in Norway to gain access to their data set on firing installations. We successfully obtained the complete information from a total of 101 municipalities, covering almost half (1 million) of Norwegian residencies, including the five largest cities. The data set provides detailed information on all residential addresses inspected, including the geographical location of the pipe, the installation type, technology and model, and whether the technology can be classified as a clean burning technology (i.e. true/false).</p>
      <p id="d1e863">The fire and rescue agency registry, if complete, should include all firing installations including those in residential households. There are however a few caveats to these data. Inspections are carried out continuously and over time, and the data obtained generally did not indicate when the inspection was done and some data could be obsolete. There is also a lack of uniform sampling method among the municipalities, and the type of data supplied was different for each fire departments system. For instance, there were 795 different housing types in the total fire agency data, which were filtered to each of the residential types of buildings and others.<?pagebreak page10222?> Classification of the installation ranged from a general description to a complete brand and model type, in all consisting of 890 different descriptions. Each one was placed in one of the three categories of wood burning installation or classified as non-wood based. It also appears that the coverage is not fully complete and must be considered partial even in the municipality where all fire agency data were provided. For example, the fire agency in the Oslo municipality informed us of continual dodging of inspections by house owners for various reasons, which results in an estimated 10 % unregistered firing installations (Oslo Fire Department, personal communication, 2018). As a result, the data are used as a statistical input to the MetVed model. Cross referencing wood consumption and firing installation statistics shows that there is a relatively good agreement with other existing data, and therefore it could also be used directly in the model. Figure <xref ref-type="fig" rid="Ch1.F2"/>d shows all the inspected installations in the Stavanger municipality with a density heat map Fig. <xref ref-type="fig" rid="Ch1.F2"/>e. The highest density of wood burning installations is obtained in the Stavanger city centre, but there are also other less densely populated areas where fireplace frequency per dwelling is much higher (e.g. Testa, which is north-west of the city centre).</p>
</sec>
<sec id="Ch1.S2.SS5">
  <label>2.5</label><title>Web-crawled database</title>
      <p id="d1e878">The web-crawled data set is derived from the web-crawling program GoodOvening that scrapes data in a systematic way from a real state advertisement portal satisfying certain search criteria. It structures data obtained for further data analysis <xref ref-type="bibr" rid="bib1.bibx23" id="paren.26"><named-content content-type="pre">for more details see</named-content></xref>. The web-crawled data set is continually updated and consisted of 444 000 geo-positioned data points within Norway at the time the data was extracted for the MetVed model. Along with the geographical location, the web-crawling extracts data on the characteristics of each dwelling such as the type that they belong to (i.e. detached house, townhouse, duplex, apartment, etc.), the size and the type of the available energy system for residential heating (i.e. wood burning installation, district heating, heat pump, etc.). The web-crawling database is aggregated to the 250 <inline-formula><mml:math id="M35" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid resolution and it allows us to establish, with a high level of detail, grids with low or high RWC potential. A zero RWC potential is assigned to those grids with dwellings with no wood-based heating installations. The highest potential would be to those grids with dwellings where a wood-based installation is the sole residential heating source. Between these, the potential is determined as a proportion of wood-based installation to other residential heating technologies.</p>
      <p id="d1e894">Figure <xref ref-type="fig" rid="Ch1.F2"/>f shows the proportion of wood-based installations for residential heating relative to other listed technologies (e.g. district heating, heat pump, electricity) at 250 <inline-formula><mml:math id="M36" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> resolution. The city centre shows a low proportion of wood-based technologies (i.e. from 0 % to 30 %) even though the same area shows the highest number of residential dwellings (Fig. <xref ref-type="fig" rid="Ch1.F2"/>a) and the highest density of wood-based technologies (Fig. <xref ref-type="fig" rid="Ch1.F2"/>b). The highest proportion of wood-based technologies is observed spread out in the areas outside the city centre. We see similar spatial patterns at the grid level for the proportion of wood-based heating technologies in and around other Norwegian cities.</p>
</sec>
<sec id="Ch1.S2.SS6">
  <label>2.6</label><title>Database from the Norwegian Energy Labelling System for Dwellings (ENOVA)</title>
      <p id="d1e919">The ENOVA energy labelling system was implemented in Norway in July 2010 and is a self-assessment report performed by owners of dwellings and buildings, or qualified experts in the case of new buildings. The ENOVA data set consists of about <inline-formula><mml:math id="M37" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">650</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mn mathvariant="normal">000</mml:mn></mml:mrow></mml:math></inline-formula> entries that include (i) the size of the dwelling, (ii) building type (e.g. apartment, small house, office building), (iii) building year, (iv) energy consumption of the dwelling (<inline-formula><mml:math id="M38" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kWh</mml:mi></mml:mrow></mml:math></inline-formula>), (v) primary and secondary heating installations, (vi) energy consumption per fuel and (vii) geographical information. While individual buildings are listed in the data, the data accessed were used on a municipal and postal code resolution due to data privacy. The information from these data supplements the two preceding data sets and also provides a relation between energy consumption for total heating, RWC and building size/type. Wood consumption input statistics to MetVed were used on the county level to correspond with wood consumption data.</p>
</sec>
<sec id="Ch1.S2.SS7">
  <label>2.7</label><title>Outdoor temperature</title>
      <p id="d1e952">Outdoor temperature is an important controlling factor for RWC because the main purpose of most RWC is the heating supply. The MetVed model uses observed temperatures as input meteorological data. Observed daily mean temperatures were obtained for the years from 2005 to 2016 for 57 official Norwegian temperature measurement stations through the eKlima database <xref ref-type="bibr" rid="bib1.bibx8" id="paren.27"/> to form the basis for time variation of emissions for MetVed. For now we have ensured that urban areas have an observation point within them.</p>
</sec>
<sec id="Ch1.S2.SS8">
  <label>2.8</label><title>Other data</title>
      <p id="d1e966">In addition to geospatial information of Norway, such as municipal and county administrative borders, we have ancillary data responses to questionnaires on wood consumption in Akershus/Oslo and Sarpsborg/Fredrikstad <xref ref-type="bibr" rid="bib1.bibx22" id="paren.28"/>. Together with all of the individual answers of respondents to the questionnaires of the Statistics Norway Holiday Survey (where wood consumption is reported), they form the basis of establishing assumptions on variability between primary and supplementary wood heating habits.</p>
      <?pagebreak page10223?><p id="d1e972">To assess emissions, dispersion modelling has been used and the results have been compared with observations. To do this, measurement data of <inline-formula><mml:math id="M39" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> were taken from the Norwegian air quality network monitoring stations that report to the European air quality database (<uri>https://www.eea.europa.eu</uri>, last access: 14 June 2019). <inline-formula><mml:math id="M40" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">PM</mml:mi></mml:mrow></mml:math></inline-formula> is measured by applying methods equivalent to the reference method (i.e. TEOM 1400A and Grimm-EDM180) that continuously monitor and log with a time resolution of 1 h. Measurements of <inline-formula><mml:math id="M41" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">BC</mml:mi></mml:mrow></mml:math></inline-formula> in Oslo were obtained at two roadside monitoring stations in the winters 2014/2015 and 2015/2016. The measurements were performed with an Aethalometer (Magee Scientific) that measured aerosol light absorption at seven specific wavelengths at 1 <inline-formula><mml:math id="M42" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">min</mml:mi></mml:mrow></mml:math></inline-formula> resolution <xref ref-type="bibr" rid="bib1.bibx13" id="paren.29"/>. The results at the specific wavelengths are used to determine the contribution from traffic and wood burning to <inline-formula><mml:math id="M43" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">BC</mml:mi></mml:mrow></mml:math></inline-formula> concentration based on the model established by <xref ref-type="bibr" rid="bib1.bibx31" id="text.30"/>. Benzo(a)pyrene (BaP) measurements were taken from the Norwegian monitoring network through active air sampling. The monthly <inline-formula><mml:math id="M44" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> values are derived from the analysis of particle filters, which are collected with a 3 d frequency. The identification and quantification of <inline-formula><mml:math id="M45" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> is carried out by GC/LRMS.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>The MetVed model</title>
      <p id="d1e1069">For the MetVed model MatLab was chosen since there is a wide variety in the type form and file format of the input data, and it allows for easy reading, visualisation and inspection of data flows in the model. The MetVed model contains different routines to estimate emissions at the 250 <inline-formula><mml:math id="M46" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid. In order to calculate emissions, MetVed first calculate gridded wood consumption and emission factors. Spatial and temporal distribution of emissions further requires information on location, type and activity of wood burning installations. These are all derived from the input data, which have different scales and resolutions (e.g. county, municipality, grid, point). MetVed calculations take into account the physical properties of households and their heating systems, but they do not account for most human behavioural differences. The main calculation of MetVed is to pre-process the input data to arrive at gridded emissions, calculated as
          <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M47" display="block"><mml:mrow><mml:mi>E</mml:mi><mml:mo>(</mml:mo><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mi>C</mml:mi><mml:mo>(</mml:mo><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:mi mathvariant="normal">EF</mml:mi><mml:mo>(</mml:mo><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi><mml:mo>)</mml:mo><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where <inline-formula><mml:math id="M48" display="inline"><mml:mrow><mml:mi>E</mml:mi><mml:mo>(</mml:mo><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is emissions (<inline-formula><mml:math id="M49" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">yr</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) in a grid, <inline-formula><mml:math id="M50" display="inline"><mml:mi>c</mml:mi></mml:math></inline-formula>, for the year, yr, and <inline-formula><mml:math id="M51" display="inline"><mml:mi>C</mml:mi></mml:math></inline-formula> and EF are the wood consumption (<inline-formula><mml:math id="M52" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kg</mml:mi></mml:mrow></mml:math></inline-formula>) and emission factor (<inline-formula><mml:math id="M53" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">kg</mml:mi><mml:msup><mml:mi/><mml:mo>-</mml:mo></mml:msup><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>), respectively. Though several calculation methods are available in MetVed, the main method to calculate grid EFs and consumption is based on consumption per technology at the county scale.  The initial step is thus to calculate a consumption-weighted average EF for the year of interest, yr:
          <disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M54" display="block"><mml:mrow><?xmltex \hack{\hbox\bgroup\fontsize{9.5}{9.5}\selectfont$\displaystyle}?><mml:mi mathvariant="normal">EF</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">yr</mml:mi><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="normal">EF</mml:mi><mml:mi mathvariant="normal">new</mml:mi></mml:msub><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">new</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="normal">EF</mml:mi><mml:mi mathvariant="normal">old</mml:mi></mml:msub><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">old</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="normal">EF</mml:mi><mml:mi mathvariant="normal">open</mml:mi></mml:msub><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">open</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">total</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo><?xmltex \hack{$\egroup}?></mml:mrow></mml:math></disp-formula>
        where EF<inline-formula><mml:math id="M55" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">old</mml:mi></mml:msub></mml:math></inline-formula>, EF<inline-formula><mml:math id="M56" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">new</mml:mi></mml:msub></mml:math></inline-formula> and EF<inline-formula><mml:math id="M57" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">open</mml:mi></mml:msub></mml:math></inline-formula> refer to the emission factors for old stoves, new stoves and open fireplaces, respectively (Table <xref ref-type="table" rid="Ch1.T1"/>), and similarly <inline-formula><mml:math id="M58" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">new</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M59" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">old</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M60" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mrow><mml:mi mathvariant="normal">open</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula> refer to the consumption in the different technology classes.</p>
      <p id="d1e1365">To distribute consumption to each grid, MetVed calculates a wood burning potential (WP) in a hierarchical fashion up from dwelling to grid to municipal level and finally up to county, to match the consumption input data resolution. The WP is calculated to distribute in a consistent way the available consumption at the county level, and this establishes the share of total consumption assigned to each grid. The WP is dependent on statistical and physical properties of each residence (e.g. the type and the size), and it has two components:
          <disp-formula id="Ch1.E3" content-type="numbered"><label>3</label><mml:math id="M61" display="block"><mml:mrow><mml:mi mathvariant="normal">WP</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi>W</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        a consumption weight (<inline-formula><mml:math id="M62" display="inline"><mml:mrow><mml:msub><mml:mi>W</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and a frequency of wood-based installation for residential heating (<inline-formula><mml:math id="M63" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), calculated per dwelling type (HT) in each county. <inline-formula><mml:math id="M64" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is calculated based on the fraction of dwellings of each type in each county that have listed wood burning installations in the web-crawled data set. For the consumption weight <inline-formula><mml:math id="M65" display="inline"><mml:mrow><mml:msub><mml:mi>W</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, a linear dependence between energy consumption and dwelling size is applied for each HT and is specific to each county. The linear dependency is established from the ENOVA data set, and the dwelling size applied is the HT average size determined from the web-crawled data set per county.</p>
      <p id="d1e1436">Survey data on wood consumption, however, indicate very skewed consumption statistics that are not explained by total heating demand of a dwelling. According to the surveys, a few high-intensity users burn up to 30–50 times the average amount of wood consumed, which can amount to more than 10 % of the wood consumed in a given county. This differential usage introduces uncertainty and it will also affect consumption. In broad terms we can distribute the usage rate into three categories: (i) inactive (existing installations not in use), (ii) secondary usage (used as supplementary heating), and (iii) primary heating source. At the moment, there is no way to establish exactly which of the listed installations are in disuse. Therefore, we only consider two categories, i.e. installations for secondary usage and as primary heating source. As an example, the Bergen fire department estimated that roughly 15 % of the wood burning installations are inactive, 70 % are sporadically used for social or secondary heating, and the remaining 15 % are primary heating sources.
To detail out further the activity level of fireplaces, further data could be collected. In some municipalities, amount of residue material from chimneys swept is kept record of and graded on a scale from 1 to 9 (clean to dirty). These and similar data (if collected) could be used directly to estimate the activity in each chimney but would need a proper framework. Also the consumption questionnaire presently asks respondents first if they have a wood firing installation and then if it is in use, so this also supports finding the average share of inactive fireplaces.</p>
      <p id="d1e1439">These usage shares will have geographical variations because climate, wood availability and prices of heating vary across the country. It is therefore necessary to improve the information on installation usage. This is done by the analysis of the web-crawling data set <xref ref-type="bibr" rid="bib1.bibx23" id="paren.31"/>.<?pagebreak page10224?> This data set provides good statistics on the relative occurrence of both wood burning installations and other heating technologies at high geographical resolution. When it is established that other heating technologies are available (e.g. district heating, heat pump), wood burning installations are assumed to be used as a secondary heating source.</p>
      <p id="d1e1446">The difference in wood consumption between a RWC installation that is used as a primary heating source and another that is used as a secondary source has been established through the ancillary data in questionnaires <xref ref-type="bibr" rid="bib1.bibx22" id="paren.32"/>. We define the ratio (<inline-formula><mml:math id="M66" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula>) between wood consumption for households with primary (<inline-formula><mml:math id="M67" display="inline"><mml:mrow><mml:msub><mml:mi>h</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) and secondary (<inline-formula><mml:math id="M68" display="inline"><mml:mrow><mml:msub><mml:mi>h</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) RWC heating as <inline-formula><mml:math id="M69" display="inline"><mml:mrow><mml:mi>R</mml:mi><mml:mo>=</mml:mo><mml:msub><mml:mi>h</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub><mml:mo>/</mml:mo><mml:msub><mml:mi>h</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. To represent <inline-formula><mml:math id="M70" display="inline"><mml:mrow><mml:msub><mml:mi>h</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, we used the 15th percentile of consumption and for <inline-formula><mml:math id="M71" display="inline"><mml:mrow><mml:msub><mml:mi>h</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the average wood consumption to get a conservative estimate of <inline-formula><mml:math id="M72" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> of 4. In the questionnaire data, RWC as primary heating source occurs only in detached houses, and therefore this is only applied to this type of dwellings, where 10 % of detached houses are assumed to use wood as their primary heating source.</p>
      <p id="d1e1533">We establish the ratio of wood burning installations to dwellings as
          <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M73" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="normal">PF</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="normal">NFP</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where <inline-formula><mml:math id="M74" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the number of dwellings of a specific type and NFP<inline-formula><mml:math id="M75" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:math></inline-formula> is the number of installations per HT. The ratio predicted by web-crawling and rescue and fire agencies data sets predicts roughly 1.7 million installations, while in an existing national survey predicts about 1.9 million houses with wood-based installations (Norstat 2016 survey, Norsk Varme, personal communication, 2018). Therefore, an adjustment was done to the detached houses to assign enough total installations to residences based on web-crawling that gave about 10 % fewer total installations in residential buildings than reported. The probability of having an installation for RWC (<inline-formula><mml:math id="M76" display="inline"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is then calculated:
          <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M77" display="block"><mml:mrow><mml:msub><mml:mi>P</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi mathvariant="normal">PF</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi mathvariant="normal">PP</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>×</mml:mo><mml:mi>R</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where PP is the fraction of primary heating for each type of dwelling (HT). Finally, the consumption in each grid is calculated by distributing the municipal consumption <inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to each grid depending on the number of dwellings of each type (<inline-formula><mml:math id="M79" display="inline"><mml:mrow><mml:msub><mml:mi>N</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) at the grid, <inline-formula><mml:math id="M80" display="inline"><mml:mi>c</mml:mi></mml:math></inline-formula>, and their associated WP<inline-formula><mml:math id="M81" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:math></inline-formula>:
          <disp-formula id="Ch1.E6" content-type="numbered"><label>6</label><mml:math id="M82" display="block"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi>c</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mo>∑</mml:mo><mml:mrow><mml:mi mathvariant="normal">m</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">HT</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi>N</mml:mi><mml:mrow><mml:mi mathvariant="normal">m</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">HT</mml:mi></mml:mrow></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi mathvariant="normal">WP</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>×</mml:mo><mml:munder><mml:mo movablelimits="false">∑</mml:mo><mml:mrow><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">HT</mml:mi></mml:mrow></mml:munder><mml:msub><mml:mi>N</mml:mi><mml:mrow><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">HT</mml:mi></mml:mrow></mml:msub><mml:mo>×</mml:mo><mml:msub><mml:mi mathvariant="normal">WP</mml:mi><mml:mi mathvariant="normal">HT</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
        where the <inline-formula><mml:math id="M83" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi mathvariant="normal">m</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is calculated in the same way as <inline-formula><mml:math id="M84" display="inline"><mml:mrow><mml:msub><mml:mi>C</mml:mi><mml:mi>c</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in Eq. (<xref ref-type="disp-formula" rid="Ch1.E6"/>) based on wood consumption at the county. For each year, emissions (<inline-formula><mml:math id="M85" display="inline"><mml:mrow><mml:mi>E</mml:mi><mml:mo>(</mml:mo><mml:mi>c</mml:mi><mml:mo>,</mml:mo><mml:mi mathvariant="normal">yr</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>) are finally calculated at the grid by multiplying Eqs. (<xref ref-type="disp-formula" rid="Ch1.E6"/>) and (<xref ref-type="disp-formula" rid="Ch1.E2"/>) at the grid.</p><?xmltex \hack{\newpage}?>
<sec id="Ch1.S3.SSx1" specific-use="unnumbered">
  <title>Time variation</title>
      <p id="d1e1799">From an annual baseline consumption, MetVed estimates the hourly distribution of wood usage through a calendar year. The time variation of RWC activity is defined to be dependent on the heating demand defined by the outdoor temperature. Therefore the heating degree day (HDD) concept is used <xref ref-type="bibr" rid="bib1.bibx29" id="paren.33"/>. MetVed looks up the geographically nearest meteorological station to obtain the outdoor temperature data set.  Thereafter the HDD is calculated as
            <disp-formula id="Ch1.E7" content-type="numbered"><label>7</label><mml:math id="M86" display="block"><mml:mrow><mml:mi mathvariant="normal">HDD</mml:mi><mml:mo>=</mml:mo><mml:mo movablelimits="false">max⁡</mml:mo><mml:mfenced open="(" close=")"><mml:mrow><mml:mn mathvariant="normal">0</mml:mn><mml:mo>,</mml:mo><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">Threshold</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:mi>T</mml:mi></mml:mrow></mml:mfenced><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where T is the outdoor daily average temperature in degree Celsius. Regarding <inline-formula><mml:math id="M87" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">Threshold</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, we follow <xref ref-type="bibr" rid="bib1.bibx37" id="text.34"/> and use 15 <inline-formula><mml:math id="M88" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C (HDD<inline-formula><mml:math id="M89" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:math></inline-formula>). Hourly resolution is obtained by coupling the daily consumption to the diurnal heating cycle in Norway. The time of day when RWC occurs is obtained by a survey covering dwellings that provides information regarding the use of the RWC installations both during the day and week <xref ref-type="bibr" rid="bib1.bibx1" id="paren.35"/>. The obtained weekly and hourly activity shows a strong diurnal cycle, where RWC is higher after 17:00 CET. Hourly consumption is obtained by multiplying the daily HDD derived consumption with the hourly average reported activity, which is also weekday dependent. There is higher activity during weekends than weekdays <xref ref-type="bibr" rid="bib1.bibx12" id="paren.36"/>. The consumption differences between weekdays and weekends are smaller than what is suggested by <xref ref-type="bibr" rid="bib1.bibx9" id="text.37"/> and <xref ref-type="bibr" rid="bib1.bibx18" id="text.38"/>. However, the diurnal pattern of concentrations they found for RWC is similar to the emissions profile derived based on the activity data, which assumes an emission profile that takes into account emissions of the later stages of the firing cycle <xref ref-type="bibr" rid="bib1.bibx15 bib1.bibx32" id="paren.39"><named-content content-type="pre">e.g.</named-content></xref>. Fixed public holidays and Easter are treated as weekends.</p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Emission results and discussion</title>
<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Time evolution of wood consumption in Norway</title>
      <?pagebreak page10225?><p id="d1e1900">The primary model output from MetVed is gridded emissions for Norway in the period of 2005–2016. Figure <xref ref-type="fig" rid="Ch1.F3"/> shows the spatial distributions of emissions from RWC obtained with MetVed at a 250 <inline-formula><mml:math id="M90" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid resolution in southern Norway and seven domains selected for the evaluation of urban emissions. The distribution of RWC emissions on the 250 <inline-formula><mml:math id="M91" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid is concentrated where there are residential buildings. This is in cities, valleys and along the coast, and consequently they cover a small proportion of the surface area in Norway. Each grid cell has emissions relative to their proportion of the wood burning  determined by the number and type of dwellings and available residential heating technology within it. In the urban domains, the lowest emissions (i.e. in the range 0–0.14 <inline-formula><mml:math id="M92" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">t</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">yr</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> per grid) are obtained in the outskirts of the urban areas (blue grids in Fig. <xref ref-type="fig" rid="Ch1.F3"/>), whereas the highest emissions (i.e. 0.30–1.50 <inline-formula><mml:math id="M93" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">t</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">yr</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> per grid) are centred in the urban areas. The internal distribution within each urban domain varies among the cities, as it depends on the distribution characteristics of apartments and houses, as well as the availability of non-wood-based residential heating technologies.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><?xmltex \currentcnt{3}?><label>Figure 3</label><caption><p id="d1e1960">MetVed emissions (<inline-formula><mml:math id="M94" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">t</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">yr</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) in 2015 in the south of Norway and in seven urban domains at a 250 <inline-formula><mml:math id="M95" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid. The squares in the map of the south of Norway represent the zoomed in domains on the right, labelled from 1 to 7 (named on the left panel), which are used for the assessment of urban emissions and dispersion modelling. The black circles represent the location of the air quality monitoring stations in Figs. <xref ref-type="fig" rid="Ch1.F7"/>, <xref ref-type="fig" rid="Ch1.F8"/> and <xref ref-type="fig" rid="Ch1.F9"/>.  Background map: © OpenStreetMap contributors 2019. Distributed under a Creative Commons BY-SA License.</p></caption>
          <?xmltex \igopts{width=497.923228pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f03.jpg"/>

          <p id="d1e1999">.</p>
        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><?xmltex \currentcnt{4}?><label>Figure 4</label><caption><p id="d1e2005"><bold>(a)</bold> Historical evolution of the officially reported consumption of firewood and emissions of <inline-formula><mml:math id="M96" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> since 1990. <bold>(b)</bold> Consumption per technology class for new, old and open in yellow, blue and green, respectively. Red bars show the stock of new ovens assuming a constant sale over time. <bold>(c)</bold> The coloured bars show the EF of ovens sold in a given year. EF MetVed (blue) is the emission factor used in the MetVed model. EF CLRTAP is derived from officially reported emission and consumption numbers. The yellow dashed line shows the emission factor one would get from the assumed oven sales (red bars in panel <bold>a</bold>) and equal consumption in all ovens. The deviating dotted dark blue line shows the derived annual emission factor when manufacturer information on emission factors is used for each year. <bold>(d)</bold> Annual average emission factors for each year of each component in the MetVed emissions, based on consumption statistics.</p></caption>
          <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f04.png"/>

        </fig>

      <p id="d1e2040">Total annual MetVed emissions are closely linked to the total emissions in Norway reported to CLRTAP (Fig. <xref ref-type="fig" rid="Ch1.F4"/>a) as both are estimated using the same wood consumption data and  emission factors. MetVed wood consumption is only for residential heating, and the difference with emissions reported to CLRTAP is that the latter includes consumption in cabins. The peak year of wood consumption is 2010, coinciding with an especially cold winter across Norway. Since 2010, consumption has gone down every year except in 2012. Before 2005, there was a general decline in reported emissions. This is mainly associated with a reduction in wood consumption and an increase in the share of newer technology ovens. From 2005 until 2016, consumption in open fireplaces is relatively constant, varying between 3 % and 5 %, whereas the share of consumption in new stoves has nearly doubled, from 34 % in 2005 to 62 % in 2016 Fig. <xref ref-type="fig" rid="Ch1.F4"/>b).</p>
</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>Effects of technological advances</title>
      <p id="d1e2055">In 1998, regulations were put into place to reduce emission for newly sold stoves, which should not emit more than 12 <inline-formula><mml:math id="M97" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M98" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. The bars in Fig. <xref ref-type="fig" rid="Ch1.F4"/>c show the assumed average EF of stoves sold in that year. Assuming ovens have equal usage, the share in a given year predicted by an exchange of stoves by sales is shown as a dashed yellow line. This EF fits very well with the derived emission factor for <inline-formula><mml:math id="M99" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> from both MetVed and from the CLRTAP emissions since 2005. Similarly as for <inline-formula><mml:math id="M100" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, all other compounds (Fig. <xref ref-type="fig" rid="Ch1.F4"/>d) except <inline-formula><mml:math id="M101" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">CH</mml:mi><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> show a general decline in EFs since 2005. This decline in EFs is the main driver for the decreasing trend in emissions in Norway, as an increasing fraction of wood is consumed in new stoves. BC is the only EF that does not decrease uniformly. The reason is that the EF for open fireplaces is an order of magnitude higher than those for stoves, and the slight variability in the consumption estimates in open fireplaces drives the change.</p>
      <p id="d1e2124">The MetVed input data were analysed to evaluate both the share of stoves and their use. In the fire and rescue agency data, roughly 70 % indicate the age of the installation, of which only 34 % of residential stoves are noted to be newer than 1998. A recent survey carried out in Norway in 2016 shows around 64 % of the wood burning installations in 2016 are new stoves (Norstat 2016 survey, Norsk Varme, personal communication, 2018). Sales estimates based on this survey indicate that the transfer to cleaner technologies therefore will go on for the next several decades. Similarly, the increased efficiency of newer ovens from an estimated 50 % to 75 % for new ovens <xref ref-type="bibr" rid="bib1.bibx33" id="paren.40"/> will act to reduce consumption. Thus, based on this, future emissions are expected to go down further. The red bars in Fig. <xref ref-type="fig" rid="Ch1.F4"/>b show an assumed share of existing stove technology assuming annual sales of new ovens to the residential sector of 67 500 units per year. This sale is derived from a fit to emission factors and will be influenced by consumption differences. Based on the Norstat 2016 survey, annual sales are close to 40 000 installations per year (Norsk Varme, personal communication, 2018). This difference indicates that there are large consumption differences and that on average a new installation may involve a higher consumption of fuelwood. Therefore, what the real effect of exchanging an old for a new installation will have on the overall consumption, and therefore on emissions, is still uncertain.</p>
      <p id="d1e2132">It is worth noting that the two stove technologies new and old are comprised of an assembly of stoves. Producers of stoves today claim to have significantly reduced <inline-formula><mml:math id="M102" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions even further since 1998, to about 2 <inline-formula><mml:math id="M103" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> in 2016 (Norsk Varme, personal communication, 2018). Both Norwegian emissions reported to CLRTAP and MetVed assume constant EF for the new oven assembly. The dotted lines in Fig. <xref ref-type="fig" rid="Ch1.F4"/>c show the EF with a continuing reduction down to 2 <inline-formula><mml:math id="M104" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> in 2016, both for ovens sold in that year (light blue) and for the share of stoves in that year (green). Were EF based on this it would act to significantly reduce 2016 <inline-formula><mml:math id="M105" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> EF from 13.5 to 7.4 <inline-formula><mml:math id="M106" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">g</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> and thus nearly halving emissions.</p>
</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Temperature dependence of wood consumption</title>
      <p id="d1e2219">Consumption of fuelwood follows the change in demand for heating energy. In Fig. <xref ref-type="fig" rid="Ch1.F5"/>a the total annual number for HDD<inline-formula><mml:math id="M107" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:math></inline-formula> at observation sites (57 meteorological stations) across the simulation domains in Norway is weighted by the total number of dwellings in the domain covered by each station. The MetVed  annual consumption is from the CLRTAP (Fig. <xref ref-type="fig" rid="Ch1.F4"/>a), which is derived independently from the temperature. The linear fit to the period 2005 to 2016 indicates that consumption is reduced by <inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:math></inline-formula> % per year, whereas a slight increase in HDD demand is observed over the same period (Fig. <xref ref-type="fig" rid="Ch1.F7"/>c). Residuals from both trends show that the temperature can explain about 63 % of the variance in consumption (<inline-formula><mml:math id="M109" display="inline"><mml:mrow><mml:mi>r</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.79</mml:mn></mml:mrow></mml:math></inline-formula> Fig. <xref ref-type="fig" rid="Ch1.F5"/>b). HDD would therefore provide a good indicator for present and future annual consumption variations, but long-term trends depending on the physical properties of residences must also be considered. It is also important to note that the trend of decreasing consumption between 2005 and 2016 is not due to increasing average winter temperatures.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5" specific-use="star"><?xmltex \currentcnt{5}?><label>Figure 5</label><caption><p id="d1e2264"><bold>(a)</bold> The HDD in the simulation domains in Fig. <xref ref-type="fig" rid="Ch1.F3"/> weighted by the population in each domain along with the annually reported consumption 2005–2016. The dashed line is the linear trend. <bold>(b)</bold> Normalised residuals to linear trends 2005–2016. <bold>(c)</bold> The blue line show the linear trend in consumption. Explanatory variables for this change (2005–2016) are changes in heating demand (HDD; in red), the efficiency of wood ovens (assumed 75 % for new, 50 % for old and 15 % for open; in yellow), the reduced energy required to heat buildings due to improved insulation (purple), and the decreasing  share of total domestic energy consumption that comes from wood (green).</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f05.png"/>

        </fig>

      <p id="d1e2283">In the MetVed model, the concept of HDD is only used to distribute wood consumption within a year, and only to days with a heating demand. The model determines the total number of HDDs in a year over which the consumption is distributed. The choice of a threshold HDD, i.e. the coldest temperature where no heating is required, only influences the temperature sensitivity of consumption within a year. A lower HDD threshold would therefore only lead to higher<?pagebreak page10226?> emissions in winter and less during spring and autumn. In the cold year 2010, consumption increased by 25 %, and the number of HDDs with threshold 20<inline-formula><mml:math id="M110" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M111" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">20</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) increased by 23 % relative to the 2005–2016 mean. In contrast, <inline-formula><mml:math id="M112" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M113" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M114" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> showed an increase of 36 %, 65 %, 135 %, respectively. Thus a lower threshold temperature will thus increase temperature sensitivity of emissions. From the residual consumption and <inline-formula><mml:math id="M115" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> in Fig. <xref ref-type="fig" rid="Ch1.F5"/>b we derived the relation for the period 2005–2016:
            <disp-formula id="Ch1.E8" content-type="numbered"><label>8</label><mml:math id="M116" display="block"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>C</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.77</mml:mn><mml:mspace linebreak="nobreak" width="0.25em"/><mml:mi mathvariant="normal">Δ</mml:mi><mml:mspace width="0.25em" linebreak="nobreak"/><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where <inline-formula><mml:math id="M117" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>C</mml:mi></mml:mrow></mml:math></inline-formula> is the change in consumption and <inline-formula><mml:math id="M118" display="inline"><mml:mi mathvariant="normal">Δ</mml:mi></mml:math></inline-formula><inline-formula><mml:math id="M119" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> the change in the <inline-formula><mml:math id="M120" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, both unitless. The relation between the outdoor average temperature and consumption is 0.32 kg dwelling<inline-formula><mml:math id="M121" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> HDD<inline-formula><mml:math id="M122" display="inline"><mml:mrow><mml:msubsup><mml:mi/><mml:mn mathvariant="normal">15</mml:mn><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e2445">As other factors also influence wood consumption, household energy consumption per square metre has been examined from the output of the Norwegian energy balance model (<uri>https://www.ssb.no/energi-og-industri/statistikker/husenergi/hvert-3-aar/2014-07-14</uri>, last access: 18 December 2018) and shown in Fig. <xref ref-type="fig" rid="Ch1.F5"/>c. An increase in the number of energy-efficient houses and a lower wood energy share reduce the annual wood energy demand (both by <inline-formula><mml:math id="M123" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> % per year in Fig. <xref ref-type="fig" rid="Ch1.F5"/>c). <xref ref-type="bibr" rid="bib1.bibx33" id="text.41"/> report an energy efficiency of 15 %, 50 % and 75 % for open fireplaces, old stoves and new stoves, respectively, which are also used in the Norwegian energy balance model. Consumption per technology in 2012 gives a 61 % average stove efficiency, at a constant energy output. The effect of newer, more-efficient installations has influenced the decrease in consumption by 0.5 % per year (“oven efficiency” in Fig. <xref ref-type="fig" rid="Ch1.F5"/>c).</p>
      <p id="d1e2471">In 2012, the average reported dwellings in Norway received 16 % of their energy, about 3200 <inline-formula><mml:math id="M124" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kWh</mml:mi></mml:mrow></mml:math></inline-formula>, from wood. This is significantly higher than the average energy share suggested by the MetVed input data from ENOVA, where the annual average energy from wood is 960 <inline-formula><mml:math id="M125" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kWh</mml:mi></mml:mrow></mml:math></inline-formula>, although only 3 % reported using wood for heating. The reason for the lower reported wood consumption in the ENOVA data set is not clear but may be related to conscious under-reporting to achieve a better energy certificate by the dwelling owners. Birch wood, which is the most common fuelwood in Norway, has a dry (0 % moisture) energy content of 4.395 <inline-formula><mml:math id="M126" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kWh</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">kg</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> <xref ref-type="bibr" rid="bib1.bibx30" id="paren.42"/>. To achieve the stated energy, an average Norwegian household would then in 2012 have to burn 1195 <inline-formula><mml:math id="M127" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kg</mml:mi></mml:mrow></mml:math></inline-formula> of dry birch wood. The same conversion of the ENOVA-reported consumption gives 7.2 <inline-formula><mml:math id="M128" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kg</mml:mi></mml:mrow></mml:math></inline-formula> of dry wood for<?pagebreak page10227?> an average Norwegian household. Based on the official wood consumption data, the total residential consumption in 2012 was 1460 <inline-formula><mml:math id="M129" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kt</mml:mi></mml:mrow></mml:math></inline-formula>, which equates to 589 <inline-formula><mml:math id="M130" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kg</mml:mi></mml:mrow></mml:math></inline-formula> of wood consumption per dwelling (800 <inline-formula><mml:math id="M131" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">kg</mml:mi></mml:mrow></mml:math></inline-formula> per dwelling with a wood-based installation). Due to large differences in the input data, the housing type and size and energy dependencies calculated within MetVed are only based on the ENOVA-reported total energy consumption.</p>
</sec>
<sec id="Ch1.S4.SS4">
  <label>4.4</label><?xmltex \opttitle{PM${}_{{2.5}}$ emissions at the urban scale}?><title>PM<inline-formula><mml:math id="M132" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:math></inline-formula> emissions at the urban scale</title>
      <p id="d1e2569">The main aim of MetVed was to improve the spatial and temporal distribution of emissions from RWC. Resulting emissions of <inline-formula><mml:math id="M133" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> within each of the urban domains in Fig. <xref ref-type="fig" rid="Ch1.F3"/> from MetVed are shown with four other emission inventories available to do urban modelling in Norway in Fig. <xref ref-type="fig" rid="Ch1.F6"/>a. These domains contain the largest cities in Norway and together cover 44 % of Norwegian dwellings. With the exception of Norsk BeregningsVerktøy (NBV) emissions, all urban emission inventories are obtained by downscaling national emissions submitted to the CLRTAP (<uri>http://www.ceip.at</uri>). Though the year of reference varies between inventories, the magnitude of total national emission is comparable. The difference within these domains is therefore to a large extent<?pagebreak page10228?> determined by the method of spatially distributing the emissions.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><?xmltex \currentcnt{6}?><label>Figure 6</label><caption><p id="d1e2592"><bold>(a)</bold> Total emissions within domains shown in Fig. <xref ref-type="fig" rid="Ch1.F3"/>. <bold>(b)</bold> The percent of houses with at least one fireplace  (left <inline-formula><mml:math id="M134" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis) and the consumption per fireplace for each of the domains (right <inline-formula><mml:math id="M135" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis). <bold>(c)</bold> The distribution of housing types for each domain.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f06.png"/>

        </fig>

      <p id="d1e2625">Total emissions within each domain are computed by first-order conservative remapping emissions for each inventory to the domain <xref ref-type="bibr" rid="bib1.bibx16" id="paren.43"><named-content content-type="pre">e.g.</named-content></xref>. The European Monitoring and Evaluation Programme (EMEP) emissions are distributed on a <inline-formula><mml:math id="M136" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">0.1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula> grid and represent the lowest urban emissions in all domains, except Oslo, having an order of magnitude lower emissions than the remaining domains. To our knowledge, detailed information about the method used to downscale the EMEP emissions is not publicly available, but the data are openly available at <uri>https://ceip.at</uri>. <xref ref-type="bibr" rid="bib1.bibx26" id="text.44"/> states that when the activity data used to estimate emissions are available at a higher geographical resolution than national, they are used to distribute emissions. In Norway, wood consumption is available at the county level; thus we assume that EMEP emissions from RWC are distributed at this level. This is consistent with the visualisation of emissions where the county administrative borders are visible, and emissions are widely distributed in the Norwegian geography, covering also unpopulated areas. The TNO_MACC_III emissions have a resolution of <inline-formula><mml:math id="M137" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.125</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">0.625</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>, similar to EMEP, but have much higher emissions within each urban domain than EMEP. TNO_MACC_III uses internal approaches based on population density and a function to describe proximity to wood as their downscaling method <xref ref-type="bibr" rid="bib1.bibx19" id="paren.45"/>.</p>
      <?pagebreak page10229?><p id="d1e2684">NWA emissions (NordicWelfAir, <uri>http://projects.au.dk/nordicwelfair/</uri>, last access: 16 June 2019) are on a 1 <inline-formula><mml:math id="M138" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> grid and are based on scaling down wood consumption per technology from county level based on dwelling number at 250 <inline-formula><mml:math id="M139" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> resolution. Different RWC activity is assumed for apartments and houses, and the Norwegian official emission factors (Table <xref ref-type="table" rid="Ch1.T1"/>) is used. Thereafter emissions are re-gridded to a 1 <inline-formula><mml:math id="M140" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> resolution. NBV emissions, also on a 1 <inline-formula><mml:math id="M141" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> grid, result from downscaling wood consumption per technology by dwelling number at the district level resolution also using the Norwegian official emission factors <xref ref-type="bibr" rid="bib1.bibx38" id="paren.46"/>. The domain of Oslo in NBV is an exception. In this case emissions are reported in <xref ref-type="bibr" rid="bib1.bibx22" id="text.47"/>. In NBV, a multiplication scaling factor was derived for each urban domain individually based on the ratio of concentration levels obtained by atmospheric dispersion modelling to observed <inline-formula><mml:math id="M142" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> levels. These factors vary from 0.42 to 0.27, i.e, dividing the total emissions in these areas by a factor of 2.3–3.7. For the MetVed emission inventory, the total emissions within the area are dependent on all the input parameters detailed in Sect. <xref ref-type="sec" rid="Ch1.S3"/>.</p>
      <p id="d1e2744">The total emissions within each domain is for all inventories (with the exception of EMEP)  closely related to the number of houses within each domain (Fig. <xref ref-type="fig" rid="Ch1.F6"/>b), either directly or indirectly through population. Note that the sizes of the domains vary somewhat and all have different total area (Fig. <xref ref-type="sec" rid="Ch1.S3"/>), but they all cover a city and their area of influence. The dependency on dwelling or population density differs among the methods, and thus emissions at the urban scale vary accordingly. TNO_MACC_III results in the highest emissions at the urban scale followed by NWA emissions, but EMEP results in very low emissions at the same scale, as the downscaling approach distributes and diffuses emissions at the county level. In the MetVed model, the emissions are determined by the physical properties of the houses and their installed heating technologies within each domain (also done on the 250 <inline-formula><mml:math id="M143" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> grid). In our study, we consider NBV emissions as a tuned emission data set, as they have been obtained by comparing results from dispersion modelling and observations, and then scaling emissions. The correction factors vary among the domains and therefore the methodology lacks consistency. However, MetVed emissions are produced at high resolution at the national level following a consistent methodology and relationships between variables that influence emissions. In addition, MetVed emissions at national levels equal the official emissions reported to the CLRTAP which gives it consistency as a national emission inventory. The results from the MetVed model at the urban scale are consistent with NBV for most of the domains. MetVed emissions within the urban domains have, for most of the domains, lower emissions than those derived as a result of downscaling approaches based on population (TNO_MACC_III) or dwelling density (NWA). The MetVed emissions are the most similar to the locally corrected NBV emissions. This lowering of urban emissions in MetVed relative to emissions from the downscaling approach is the result of taking into account the share of wood-based technologies from the web-crawled input data. In that way, we account for lower wood consumption when heating technologies other than wood-based technologies are available <xref ref-type="bibr" rid="bib1.bibx27" id="paren.48"/>.</p>
      <p id="d1e2762">There are a number of dependencies in the consumption and wood installation statistics for these domains (Fig. <xref ref-type="fig" rid="Ch1.F6"/>b). For instance Trondheim, which has the fourth highest population, is located in the county with the second highest<?pagebreak page10230?> consumption per dwelling, and it has the second highest consumption per wood installation (after Grenland) of any domain. For NBV emissions, this leads to an observation-based emission correction of 0.33. In MetVed, Trondheim's high share of apartments (Fig. <xref ref-type="fig" rid="Ch1.F6"/>c) and low frequency of fireplaces (Fig. <xref ref-type="fig" rid="Ch1.F6"/>b) gives the lowest emissions for all of the MetVed domains, which shows that these properties act well to explain the reduced consumption. Dwelling size is an important factor for calculating consumption in MetVed, and it plays a significant role because apartments in the Trondheim city centre are generally small. The Oslo domain similarly has low emissions per dwelling, but in this case it is also driven by a low consumption per wood burning installation.</p>
      <p id="d1e2771">An increased prevalence of wood installations is positively correlated (<inline-formula><mml:math id="M144" display="inline"><mml:mrow><mml:msup><mml:mi>R</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.44</mml:mn></mml:mrow></mml:math></inline-formula>) with higher consumption within the domains (Fig. <xref ref-type="fig" rid="Ch1.F6"/>c). This is a result of the MetVed calculations, where the combination of regional consumption statistics and the prevalence of wood installations is found by the web-crawled statistics. This acts to support assumptions made in previous studies, e.g. proximity to wood and rural consumption being higher than urban consumption, but is in MetVed represented in dwellings' heating installations and their usage rate. Additionally, MetVed considers the dwelling size which further increases a rural amplification of firewood use, as rural properties are on average larger.</p>
</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Comparison with observations and evaluation</title>
      <p id="d1e2801">Atmospheric dispersion modelling was carried out for <inline-formula><mml:math id="M145" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> for the year 2015 with supplementary runs for <inline-formula><mml:math id="M146" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">BC</mml:mi></mml:mrow></mml:math></inline-formula> and additional investigation of benzo[a]pyrene (<inline-formula><mml:math id="M147" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula>) concentrations at sites where measurements were available. In the selected Norwegian areas, <inline-formula><mml:math id="M148" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> measurements may be considered a tracer for wood burning activity. The black carbon from biomass burning (<inline-formula><mml:math id="M149" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) measurements available enables the comparison with RWC BC concentrations. The evaluation of <inline-formula><mml:math id="M150" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">BC</mml:mi></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M151" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> adds to the comparisons to <inline-formula><mml:math id="M152" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> measurements, which have the added uncertainty of other sources. The combined outcomes from these evaluations will add to the understanding of the uncertainties associated with emissions from RWC and their contribution to air pollution levels in urban areas.</p>
      <p id="d1e2902">RWC emissions from MetVed for 2015 were used as input in the air quality model  EPISODE <xref ref-type="bibr" rid="bib1.bibx14" id="paren.49"/>, an offline Eulerian dispersion model frequently applied to assess air quality in Norwegian cities. EPISODE is driven by meteorology from the AROME model <xref ref-type="bibr" rid="bib1.bibx35" id="paren.50"/> at 1 <inline-formula><mml:math id="M153" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> resolution. <inline-formula><mml:math id="M154" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> boundary conditions come from CAMS daily forecast re-gridded to the same vertical and horizontal grid as the EPISODE model <xref ref-type="bibr" rid="bib1.bibx24" id="paren.51"/>. In EPISODE, <inline-formula><mml:math id="M155" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is treated as an inert particle, subject only to removal by transport, which limits the size of the modelling domains. Furthermore, EPISODE requires emissions on the same scale as the meteorology; therefore MetVed emissions were regridded to the meteorological field grid (1 <inline-formula><mml:math id="M156" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula>) within each domain.</p>
<sec id="Ch1.S5.SS1">
  <label>5.1</label><?xmltex \opttitle{Particulate matter ({$\protect\chem{PM_{{2.5}}}$})}?><title>Particulate matter (<inline-formula><mml:math id="M157" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
      <p id="d1e2972">The dispersion modelling in the seven domains of <inline-formula><mml:math id="M158" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> was compared to available measurements of total <inline-formula><mml:math id="M159" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentration. Comparisons must therefore include all anthropogenic emissions in the urban areas. The additional emission inventories include, along with RWC, emissions by shipping, off-road machinery, traffic exhaust and suspension of road dust. Urban emissions are estimated based on high-resolution input data that thereafter are aggregated to a 1 <inline-formula><mml:math id="M160" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> grid and combined with time variation functions to result in emissions at 1 <inline-formula><mml:math id="M161" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">h</mml:mi><mml:mspace width="0.125em" linebreak="nobreak"/><mml:msup><mml:mi mathvariant="normal">km</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> resolution <xref ref-type="bibr" rid="bib1.bibx38 bib1.bibx21" id="paren.52"><named-content content-type="pre">for more details see</named-content></xref>. Non-exhaust emissions associated with tyre and road wearing processes and the suspension of road dust were modelled by the vehicle abrasion and suspension model NORTRIP <xref ref-type="bibr" rid="bib1.bibx6" id="paren.53"/>. Emission domains and the year of reference (2015) were chosen to be able to compare with modelled concentrations obtained based on NBV emissions <xref ref-type="bibr" rid="bib1.bibx38" id="paren.54"/>. Similarly, measurement stations were selected to coincide with the existing model concentrations and assess a potential improvement when comparing with previous estimates.</p>
      <p id="d1e3031">With few exceptions, the air quality stations are classified as traffic stations and are operated by the road authorities. Few measurements are therefore ideally located with regards to a detailed evaluation of the spatial distribution of emissions from RWC within each domain. The main difference of the spatial distribution provided by MetVed and that by other methods not differentiating housing types (and size) and available residential heating technologies can best be seen through comparison between stations situated between different types of buildings. In Oslo for instance, only one monitoring station (Smestad) could be qualified as located in an area dominated by detached houses, together with similarly located monitoring stations Vaaland in Stavanger and Lensmannsdalen in Grenland. The remaining stations are in close proximity to apartments or a diversity of dwelling types, along with roads with large emissions. Together with the contributed uncertainty from other sources the differentiation on housing types is therefore hard to evaluate, and so the main focus is on evaluating total emissions within each domain.</p>

<table-wrap id="Ch1.T2" specific-use="star"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e3036">The 2015 hourly concentrations fit to observations for EPISODE simulations of <inline-formula><mml:math id="M162" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> for each of the stations. The hourly <inline-formula><mml:math id="M163" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> is the Pearson correlation coefficient and bias is calculated as model minus observation.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="6">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Station</oasis:entry>
         <oasis:entry colname="col2">Domain</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M164" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> MetVed</oasis:entry>
         <oasis:entry colname="col4">Bias MetVed</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M165" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> NBV</oasis:entry>
         <oasis:entry colname="col6">Bias NBV</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">Aakerbergveien</oasis:entry>
         <oasis:entry colname="col2">Oslo</oasis:entry>
         <oasis:entry colname="col3">0.58</oasis:entry>
         <oasis:entry colname="col4">0.63</oasis:entry>
         <oasis:entry colname="col5">0.56</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.57</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Hjortnes</oasis:entry>
         <oasis:entry colname="col2">Oslo</oasis:entry>
         <oasis:entry colname="col3">0.52</oasis:entry>
         <oasis:entry colname="col4">1.73</oasis:entry>
         <oasis:entry colname="col5">0.52</oasis:entry>
         <oasis:entry colname="col6">0.34</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Sofienbergparken</oasis:entry>
         <oasis:entry colname="col2">Oslo</oasis:entry>
         <oasis:entry colname="col3">0.35</oasis:entry>
         <oasis:entry colname="col4">1.21</oasis:entry>
         <oasis:entry colname="col5">0.33</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.24</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Danmarks Plass</oasis:entry>
         <oasis:entry colname="col2">Bergen</oasis:entry>
         <oasis:entry colname="col3">0.43</oasis:entry>
         <oasis:entry colname="col4">1.16</oasis:entry>
         <oasis:entry colname="col5">0.44</oasis:entry>
         <oasis:entry colname="col6">0.10</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Vaaland</oasis:entry>
         <oasis:entry colname="col2">Stavanger</oasis:entry>
         <oasis:entry colname="col3">0.40</oasis:entry>
         <oasis:entry colname="col4">1.44</oasis:entry>
         <oasis:entry colname="col5">0.33</oasis:entry>
         <oasis:entry colname="col6">1.36</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">St. Croix</oasis:entry>
         <oasis:entry colname="col2">Nedre Glomma</oasis:entry>
         <oasis:entry colname="col3">0.64</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M168" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.50</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.52</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M169" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.28</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Elgeseter</oasis:entry>
         <oasis:entry colname="col2">Trondheim</oasis:entry>
         <oasis:entry colname="col3">0.43</oasis:entry>
         <oasis:entry colname="col4">2.62</oasis:entry>
         <oasis:entry colname="col5">0.38</oasis:entry>
         <oasis:entry colname="col6">2.74</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Lensmannsdalen</oasis:entry>
         <oasis:entry colname="col2">Grenland</oasis:entry>
         <oasis:entry colname="col3">0.33</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M170" display="inline"><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1.58</mml:mn></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">0.31</oasis:entry>
         <oasis:entry colname="col6">0.23</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Total</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">0.46</oasis:entry>
         <oasis:entry colname="col4">0.93</oasis:entry>
         <oasis:entry colname="col5">0.42</oasis:entry>
         <oasis:entry colname="col6">0.33</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

      <p id="d1e3354">Hourly correlation coefficients and biases are shown in Table <xref ref-type="table" rid="Ch1.T2"/>. Compared to NBV emissions, which were calibrated with a weekly correction factor, the MetVed temporal emission profile generally improves correlation. The bias is not improved, because the MetVed emissions are generally higher, and so the overestimation by the model is increased. The Oslo comparison shows a strong overestimation, and a possible reason is that the MetVed approach has a limited effect in Oslo, as it is in itself a county, and so total<?pagebreak page10231?> consumption and emissions are direct results of the input wood consumption. In the Trondheim domain, the NBV emissions results from applying a factor of 0.33 to the dwelling density derived emissions <xref ref-type="bibr" rid="bib1.bibx38" id="paren.55"/>, and MetVed produces similar results to NBV at the Elgeseter monitoring station. The consideration of dwelling type and size and the fireplace information accounted for in MetVed account similarly for lower emissions and concentrations in urban areas as the local scalings applied individually in NBV.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><label>Figure 7</label><caption><p id="d1e3364">Average concentration of <inline-formula><mml:math id="M171" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> averaged at air quality stations and as a total annual average. Bottom right: the annual average diurnal variability concentration as indicated by measurements (black) and the model (blue). The orange line shows the contribution from wood burning and the shaded area is calculated as the measurement hourly average in winter (NDJF) – summer (JJA). The bars show the monthly average concentration by sector and the black line the measurement monthly average.</p></caption>
          <?xmltex \igopts{width=369.885827pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f07.png"/>

        </fig>

      <p id="d1e3384">The annually averaged observed concentration at the sites is 8.0 <inline-formula><mml:math id="M172" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, and using MetVed emissions this is 8.7 <inline-formula><mml:math id="M173" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. Monthly observed concentrations at each station are shown in Fig. <xref ref-type="fig" rid="Ch1.F7"/> as a black line, and the modelled concentrations are shown as bars, coloured by sector.  Both model and observations show a pronounced seasonal cycle in <inline-formula><mml:math id="M174" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations with a winter peak primarily driven by the background concentration and RWC contributions, and the remaining sectors have a similar cycle but contribute less to the <inline-formula><mml:math id="M175" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> seasonality. Model concentrations, including RWC, have a winter to summer (i.e. DJF to JJA) ratio of <inline-formula><mml:math id="M176" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula>, and the measurements have the winter (DJF) to summer (JJA) ratio of 1.45, indicating that the seasonality in model concentration is more than twice as strong. As wood burning for residential heating is an intensive winter activity in Norway, it is hard to envision that there should be no seasonality in RWC, and therefore the uncertainty on the seasonality of other contributing sectors must be considered. <xref ref-type="bibr" rid="bib1.bibx41" id="text.56"/> reported, based on simultaneous measurements in Oslo and a regional background site (Hurdal, 70 <inline-formula><mml:math id="M177" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">km</mml:mi></mml:mrow></mml:math></inline-formula> NE of Oslo), similar <inline-formula><mml:math id="M178" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> values in summer at both sites, 7.6 and 7.7 <inline-formula><mml:math id="M179" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, respectively. However, in winter, <inline-formula><mml:math id="M180" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">1</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations in Oslo were similar to summer concentrations, i.e. 7.8 <inline-formula><mml:math id="M181" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, but at the regional background site they were 45 % lower than in summer, i.e. 4.3 <inline-formula><mml:math id="M182" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>. Source apportionment also indicated that the elevated urban wintertime concentration consisted largely of organic mass from biomass burning. These results indicate a strong urban source rather than influence from regional background levels during winter.</p>
      <p id="d1e3551">The diurnal evening <inline-formula><mml:math id="M183" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> peak in winter (Fig. <xref ref-type="fig" rid="Ch1.F7"/>, bottom right) is also more pronounced in the model than that in the observations. While the difference between the summer and the winter diurnal pattern is also enhanced by meteorological conditions, the absolute difference between winter and summer (i.e. DFJ–JJA grey shape in Fig. <xref ref-type="fig" rid="Ch1.F7"/>, bottom right) is much less prominent than the diurnal winter contribution of RWC alone (orange line in Fig. <xref ref-type="fig" rid="Ch1.F7"/>, bottom right). The assessment of the diurnal variation also suggests that the total modelled influence of RWC on the air quality station <inline-formula><mml:math id="M184" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is too strong.</p>
      <p id="d1e3582">In Oslo, three model simulations were used to assess the sensitivity of surface concentrations to emission altitude. In urban Oslo, the annual average RWC concentration of <inline-formula><mml:math id="M185" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> at 2 <inline-formula><mml:math id="M186" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula> was 4.41 <inline-formula><mml:math id="M187" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> when all RWC emissions were emitted in the surface layer (0–30 <inline-formula><mml:math id="M188" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>). When apartment emissions were emitted in the second layer, the surface concentration was reduced to 3.76 <inline-formula><mml:math id="M189" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:msup><mml:mi mathvariant="normal">g</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>, and when smaller buildings emit in the second layer, a further reduction to 3.19 <inline-formula><mml:math id="M190" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:msup><mml:mi mathvariant="normal">g</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> was observed. The wintertime diurnal cycle of <inline-formula><mml:math id="M191" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> has a more pronounced peak, and the seasonal cycle of <inline-formula><mml:math id="M192" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> similarly indicates a too-strong seasonal cycle obtained with all emission estimates, when compared to observations, and so the total contribution of RWC to <inline-formula><mml:math id="M193" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations seems to be overall overestimated. This is supported by the new emission inventory developed by <xref ref-type="bibr" rid="bib1.bibx7" id="text.57"/> for particulate emissions from RWC. When assessing organic carbon emissions, <xref ref-type="bibr" rid="bib1.bibx7" id="text.58"/> establish that while emissions in most of Europe are underestimated, in Norway they are overestimated.</p>
</sec>
<sec id="Ch1.S5.SS2">
  <label>5.2</label><title>Black carbon</title>
      <p id="d1e3711">During both winter 2014–2015 and 2015–2016, hourly concentrations of aerosol absorption were measured at two sites in Oslo (Smestad and RV4 Fig. <xref ref-type="fig" rid="Ch1.F8"/>). The first period was at Smestad (17 December 2014–18 March 2015) and the second at RV4 (20 November 2015–30 May 2016). The decomposition of the absorbing aerosols includes BC from biomass burning (<inline-formula><mml:math id="M194" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), which in Oslo (in winter) should be equivalent to BC from RWC. While both measurements were done<?pagebreak page10232?> in close proximity to larger trunk roads, Smestad is surrounded by a large area of detached houses, while the RV4 sampling site is characterised by apartment buildings and a hospital. Even though the number of dwellings in the area surrounding RV4 is higher with nearly 30 % more residences within 300 <inline-formula><mml:math id="M195" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>, MetVed emissions in the grid of RV4 are 10 % lower, as the area is characterised by a high share of apartment buildings with low MetVed emissions.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8" specific-use="star"><?xmltex \currentcnt{8}?><label>Figure 8</label><caption><p id="d1e3737"><bold>(a)</bold> The left <inline-formula><mml:math id="M196" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis shows modelled RWC BC (blue) and measured <inline-formula><mml:math id="M197" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> data at Smestad and RV4 (in red and yellow respectively). The right <inline-formula><mml:math id="M198" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis shows the time series of temperature at Blindern (grey). <bold>(b)</bold> Aethalometer concentrations of BC from wood burning against temperature measured at two sites in Oslo from winter 2015 to spring 2016 (red symbols) and EPISODE concentrations (RWC BC) in winter and spring for the calendar year of 2015 (blue symbols). <bold>(c)</bold> The diurnal profile of <inline-formula><mml:math id="M199" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">RWC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> averaged over winter 2015 to spring 2016 as measured by the Aethalometer (blue). The diurnal profile of firing habits as reported by wood consumers in <xref ref-type="bibr" rid="bib1.bibx1" id="text.59"/> shown in dashed lines for weekdays and weekends (red dashed lines). The dotted lines show the diurnal variability in emission in MetVed.</p></caption>
          <?xmltex \igopts{width=441.017717pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f08.png"/>

        </fig>

      <p id="d1e3794">The modelled year (2015) does not completely overlap with either of the two measurements (Fig. <xref ref-type="fig" rid="Ch1.F8"/>a), and therefore model data are shown for the temperature range (<inline-formula><mml:math id="M200" display="inline"><mml:mrow><mml:mi>T</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">8</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M201" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C), which is the temperature range covered by the observations in Fig. <xref ref-type="fig" rid="Ch1.F8"/>b. Daily average <inline-formula><mml:math id="M202" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> concentrations at both sites show a similar dependence on temperature Fig. <xref ref-type="fig" rid="Ch1.F8"/>c, though overall lower concentration levels are observed in RV4, which is probably influenced by the measurements continuing further into spring. The difference between the two sites is somewhat smaller in the model. Model concentrations show a similar but weaker temperature dependence, suggesting that daily emissions could increase more than emissions obtained by <inline-formula><mml:math id="M203" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e3848">The modelled diurnal variability in concentration (Fig. <xref ref-type="fig" rid="Ch1.F8"/>c) agrees well with <inline-formula><mml:math id="M204" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The diurnal time variation of wood consumption and the subsequent MetVed emissions is in agreement with the <inline-formula><mml:math id="M205" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> observations. The diurnal weekend emission profile is similar to the observed hourly concentration profile, and the total average model concentration fits (<inline-formula><mml:math id="M206" display="inline"><mml:mrow><mml:mi>T</mml:mi><mml:mo>&lt;</mml:mo><mml:mn mathvariant="normal">8</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M207" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C) well with the levels of measured <inline-formula><mml:math id="M208" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
</sec>
<?pagebreak page10233?><sec id="Ch1.S5.SS3">
  <label>5.3</label><title>Benzo(a)pyrene</title>
      <p id="d1e3917">For most of the air quality stations, dispersion model results show an overestimation of winter <inline-formula><mml:math id="M209" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations, and a similar underestimation of summer concentrations. While <inline-formula><mml:math id="M210" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> has many sources, <inline-formula><mml:math id="M211" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> filter measurements offer a way to more directly investigate the RWC contribution.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9" specific-use="star"><?xmltex \currentcnt{9}?><label>Figure 9</label><caption><p id="d1e3960">Monthly average Benzo(a)pyrene air concentrations at five urban sites in Norway along with the annually averaged concentration on Birkenes, a rural background station in the south of Norway. The shaded areas show the monthly RWC activity predicted by HDD with a temperature threshold of 5, 10 and 15 <inline-formula><mml:math id="M212" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C.</p></caption>
          <?xmltex \igopts{width=455.244094pt}?><graphic xlink:href="https://acp.copernicus.org/articles/19/10217/2019/acp-19-10217-2019-f09.png"/>

        </fig>

      <p id="d1e3978">Figure <xref ref-type="fig" rid="Ch1.F9"/> shows monthly average concentrations between 2015 and 2017 at different urban sites, within the domains in Fig. <xref ref-type="fig" rid="Ch1.F3"/>, along with the annual average <inline-formula><mml:math id="M213" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> concentration at Birkenes, a regional background air quality observatory. All urban measurement sites show the same <inline-formula><mml:math id="M214" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> seasonality with the highest values in January. The most pronounced <inline-formula><mml:math id="M215" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> profile is obtained in Lillehammer, followed by Oslo and Drammen, where measurements show similar monthly profiles and concentration levels, and Trondheim, where the lowest <inline-formula><mml:math id="M216" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> levels are obtained. The <inline-formula><mml:math id="M217" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> annual mean concentration in all urban areas varies from 0.18, 0.30 and 0.20 ng m<inline-formula><mml:math id="M218" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in Trondheim to 0.56, 0.61 and 0.68 ng m<inline-formula><mml:math id="M219" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in Lillehammer in 2015, 2016 and 2017, respectively. These levels are below the <inline-formula><mml:math id="M220" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> European target value (i.e. 1 ng m<inline-formula><mml:math id="M221" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) but above the reference value established by the World Health Organisation (i.e. 0.12 ng m<inline-formula><mml:math id="M222" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Unlike in Birkenes, where values represent regional background levels, <inline-formula><mml:math id="M223" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> annual mean concentrations are below the WHO reference value, measured at 0.013, 0.010 and 0.011 ng m<inline-formula><mml:math id="M224" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in 2015, 2016 and 2017, respectively. Figure <xref ref-type="fig" rid="Ch1.F9"/> shows in addition the monthly normalised <inline-formula><mml:math id="M225" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math id="M226" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">10</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M227" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> obtained for Oslo (grey shades areas) based on outdoor temperatures for the same period. In MetVed, the monthly normalised HDD relates outdoor temperature with activity (i.e. wood consumption). Figure <xref ref-type="fig" rid="Ch1.F9"/> shows the effect that different thresholds (i.e. 5, 10 or 15 <inline-formula><mml:math id="M228" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C) would have on monthly wood consumption and therefore emissions. A higher temperature threshold will increase activity into spring and autumn, and a lower temperature threshold will limit activity to wintertime. The overall <inline-formula><mml:math id="M229" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> best fit to these profiles is obtained using <inline-formula><mml:math id="M230" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, suggesting a more intense source during winter than what is obtained with <inline-formula><mml:math id="M231" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>. This is in agreement with the BC observations, which is the opposite of what is observed based on <inline-formula><mml:math id="M232" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> measurements.</p>
      <?pagebreak page10234?><p id="d1e4257">The annual <inline-formula><mml:math id="M233" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> average level at each site is indicative of total RWC activity in the area, and the levels are well in agreement with the spatial distribution of emissions in the MetVed model. Lillehammer, with the highest <inline-formula><mml:math id="M234" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> levels, is the least densely populated area of those considered here but has high emissions from RWC due to high wood consumption in the region, and the area surrounding the station is made up of mainly detached houses with a high wood burning potential. Trondheim, with the lowest <inline-formula><mml:math id="M235" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> levels, is a highly populated urban area located in a county with a high wood consumption. The proxies behind MetVed entail the lowest emissions compared with other urban areas (Fig. <xref ref-type="fig" rid="Ch1.F6"/>a) as a result of the high share of apartments with alternative residential heating sources other than wood based, which represent the observed <inline-formula><mml:math id="M236" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> differences well.</p>
</sec>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <label>6</label><title>Conclusions</title>
      <p id="d1e4335">The uncertainties in emissions from RWC at the urban scale rely on those in the activity (wood consumption), emission factors and spatio-temporal distribution of the emissions. With the development of the MetVed model, our aim was to reduce the uncertainties associated with the spatio-temporal distribution of RWC emissions for their use in air quality modelling at the urban scale. As the spatial distribution alone cannot explain the large uncertainties, a detailed evaluation of the estimations and evolution of wood consumption and emission factors was also performed. The emissions from RWC in Norway show a significant declining trend. This is driven primarily by the increased use of new technologies for RWC along with a general decline in heating demand from wood-based installations through a lower heating demand per square metre and a lower share of total demand being filled from RWC.</p>
      <p id="d1e4338"><?xmltex \hack{\newpage}?>MetVed takes into account the physical properties of residences and, based on the frequency, size and type of dwelling and its available heating technologies, estimates a wood burning potential at the grid level. Even though MetVed takes into account most of the variables that affect emissions from RWC, there are still factors not considered which may affect local emissions, e.g. human behaviour, or specific geo-localised information on which installations are unused. Compared with existing emission inventories, MetVed has a higher spatial resolution, which is supported by detailed input data. The unique set of input data, and the established relationships, lead to an improved horizontal and vertical spatial distribution of emissions. One of the main effects of the MetVed approach, when comparing with other methods, is that emissions are displaced from highly populated downtown areas to the urban outskirts. As a result, MetVed gives lower emissions in highly populated areas than those established by downscaling approaches based on population or housing density, and it is moreover in agreement with total local emissions developed by combining results from dispersion modelling and observations. The new approach may have implications when estimating population exposure to pollution levels associated with RWC, as lower population exposure may be expected.</p>
      <p id="d1e4342">Downscaled emissions derived from annual wood consumption with national emission factors have in the past produced outcomes that did not compare well with observations in Norwegian cities. When comparing with air quality monitoring stations measuring <inline-formula><mml:math id="M237" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>, which exist predominantly in urban areas, modelled results have shown a strong tendency to overestimate concentrations. The MetVed model<?pagebreak page10235?> applies several new data sources to the effect of drastically reducing the emissions in urban domains when comparing with direct downscaling methods, and the results are similar to those adjusted by measurement data. The overall correlation is improved even compared to emissions adjusted with observations (NBV emissions), and this highlights the advantages of the MetVed methodology for improving the temporal variability. However, MetVed emissions still overestimate <inline-formula><mml:math id="M238" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> concentrations. The comparison of <inline-formula><mml:math id="M239" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> indicates, for the same domain where <inline-formula><mml:math id="M240" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is overestimated, that emissions are on the contrary lower and less temperature dependent than observations should predict. A potential reason for these discrepancies is that the <inline-formula><mml:math id="M241" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> Norwegian emission factor applied could be too high, which would fit well with all the inter-comparisons with observations. This is also supported by the diurnal cycle concentration profile of MetVed emissions, which have a very similar but stronger profile to that predicted by observations of <inline-formula><mml:math id="M242" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M243" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, which implies that <inline-formula><mml:math id="M244" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> emissions are somewhat overestimated.</p>
      <p id="d1e4434">The temporal emission distribution follows the heating degree day (HDD) combined with a diurnal consumption derived from consumer statistics. The applied HDD improves correlation against measurements relative to the emissions adjusted based on observations. However, this gives more intense emissions during winter and a stronger diurnal variability compared with profiles inferred from <inline-formula><mml:math id="M245" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> observations. The Annual average bias is only 0.23 <inline-formula><mml:math id="M246" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">g</mml:mi><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msup><mml:mi mathvariant="normal">m</mml:mi><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> (or 3.83 %), where the winter overestimation is compensated for by the summer underestimation. Across all stations for which simulations were done, the same general temporal pattern is seen. Substantially higher RWC emissions in the summer months or that emissions occur much earlier in the day across all domains are not plausible reasons for the observed discrepancies between winter and summer. Besides, observed <inline-formula><mml:math id="M247" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">BC</mml:mi><mml:mi mathvariant="normal">BB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M248" display="inline"><mml:mrow class="chem"><mml:mi mathvariant="normal">B</mml:mi><mml:mo>(</mml:mo><mml:mi mathvariant="normal">a</mml:mi><mml:mo>)</mml:mo><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math></inline-formula> indicate a stronger dependency on temperature, which would produce a stronger seasonality, than predicted by <inline-formula><mml:math id="M249" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">HDD</mml:mi><mml:mn mathvariant="normal">15</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> used in MetVed. We are confident that the spatial distribution of emissions given by the MetVed model entails lower uncertainties than previous methods based on downscaling approaches using population or dwelling number. Thus, further investigation of the accuracy and representativeness of the activity data (wood consumption) and the official Norwegian emission factors is needed. In addition, the main contributor to the seasonality in <inline-formula><mml:math id="M250" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is, along with RWC, the background concentration which does not have a diurnal cycle. The evaluation of the <inline-formula><mml:math id="M251" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> seasonality shows the need for improving the time variation of all contributing emitting sectors.</p>
      <p id="d1e4529">EPISODE RWC <inline-formula><mml:math id="M252" display="inline"><mml:mrow class="unit"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> surface concentrations in Oslo decreased by 18 % when apartment emissions were shifted from the surface layer (<inline-formula><mml:math id="M253" display="inline"><mml:mrow><mml:mo>&gt;</mml:mo><mml:mn mathvariant="normal">30</mml:mn></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M254" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>) to the second model layer (30–60 <inline-formula><mml:math id="M255" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">m</mml:mi></mml:mrow></mml:math></inline-formula>). A similar effect at the surface was (further reduction of 14 %) observed for moving all emissions up into the model second layer. This shows the sensitivity to emission altitude when comparing with surface concentrations.</p>
      <p id="d1e4569">Even though the model is developed for Norway, the principles behind it and the methodology can be applicable in other European countries where similar input data could be made available. Besides, the principles applied in MetVed, which is based on high-resolution data collection, could be expanded to other emitting sectors. To further improve RWC emission inventories, there is a need for more measurements specifically targeting RWC in Norway, as most measurements are limited to <inline-formula><mml:math id="M256" display="inline"><mml:mrow class="chem"><mml:msub><mml:mi mathvariant="normal">PM</mml:mi><mml:mn mathvariant="normal">2.5</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> at roadside stations in urban areas where the signal-to-noise ratio of RWC is very low. The results and evidence from our study point to even higher emissions from RWC than predicted by observations. As MetVed reduced the uncertainties associated with spatio-temporal distribution of emissions, there is a need to revise the activity data and emission factors used for the official reporting of emissions.</p>
</sec>

      
      </body>
    <back><notes notes-type="dataavailability"><title>Data availability</title>

      <p id="d1e4587">Both MetVed input and output data will be distributed freely upon contact with the corresponding author. Model input data are openly available from their stated source or upon contact with the corresponding author. For underlying ENOVA data, which were obtained under a confidentiality agreement, we refer to ENOVA for distribution. Measurement data can be obtained from the corresponding author or through their source portal.</p>
  </notes><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e4593">HG and SLA contributed equally to the text and work within this paper. SLA did all the MetVed EPISODE model simulations. MV contributed to both the writing of the text and method and model development. CH provided the BC measurement data and contributed comments and corrections to the manuscript. AKH provided the B(a)P as well as comments and corrections to the manuscript. DVT did data processing and supplied emissions for other sectors. PH supplied background concentrations and commented on and proofread the manuscript. GSS did all the EPISODE NBV simulations and provided technical assistance with EPISODE and existing emissions.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e4599">The authors declare that they have no conflict of
interest.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e4605">We thank ENOVA for sharing their anonymous data on residence energy consumption, as well as all 90 fire and rescue agencies that supplied data on firing installations.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e4610">This research has been supported by the Norwegian Environment Agency project MetVed (grant no. 2017/8676), NFR (grant no. 247884/O70), NordForsk NordicWelfAir Project (grant no. 75007), and NILU Institute Strategic Initiative MASTER (grant no. B118006).</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <?pagebreak page10236?><p id="d1e4616">This paper was edited by Jennifer G. Murphy and reviewed by two anonymous referees.</p>
  </notes><ref-list>
    <title>References</title>

      <ref id="bib1.bibx1"><label>Aasestad(2010)</label><?label Aasestad2010?><mixed-citation>
Aasestad, K.: Vedforbruk, fyringsvaner og svevestøv Dokumentasjon og resultater fra undersøkelse i Drammen 2006/2007 Statistics Norway, Oslo, Norway, ISBN 978-82-537-7823-5, 2010.</mixed-citation></ref>
      <ref id="bib1.bibx2"><label>ACAP(2014)</label><?label ACAP2014?><mixed-citation>
ACAP: Reduction of Black Carbon Emissions from Residential Wood Combustion in the Arctic – Black Carbon Inventory, Abatement Instruments and Measures. Arctic Contaminants Action Program (ACAP), Oslo, Norway,
ISBN 978-82-999755-1-3, 164 pp., 2014.</mixed-citation></ref>
      <ref id="bib1.bibx3"><label>Andersson et al.(2015)</label><?label Andersson2015?><mixed-citation>
Andersson, S., Arvelius, J., Brodl, L., Verbova, M., Ortiz, C., Jonsson, M., Svanström, S., Gerner, A., Danielsson, H., and Yaramenka, K.: Metod- och kvalitetsbeskrivning för geografiskt fördelade emissioner till luft (submission 2018). SMED Rapport Nr10 2018, Sveriges Meteorologiska och Hydrologiska Institut, Norrköping, Sweden, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx4"><label>Bloch(2018)</label><?label Bloch2018?><mixed-citation>Bloch, V. V. H.: Registerbasert boligstatistikk, Dokumentasjon og videre arbeid. 2018/2 Statistcs Norway ISBN 978-82-537-9676-5, available at: <uri>http://www.ssb.no/natur-og-miljo</uri>, last access: 9 December 2018.</mixed-citation></ref>
      <ref id="bib1.bibx5"><label>Denby(2009)</label><?label Denby2009?><mixed-citation>
Denby, B.: Source-Receptor and Inverse Modelling to quantify urban PARTiculate emissions (SRIMPART). Nordic Council of Ministers, Copenhagen, Denmark, 2009.</mixed-citation></ref>
      <ref id="bib1.bibx6"><label>Denby et al.(2013)</label><?label Denby2013?><mixed-citation>
Denby, B., Sundvor, I., Johansson, C., Pirjola, L., Ketzel, M., Norman, M.,  Kupiainen, K., Gustafsson, M., Blomqvist, G., and Omstedt, G.: A coupled road dust and surface moisture model to predict non-exhaust road traffic induced particle emissions (NORTRIP). Part 1: Road dust loading and suspension modelling, Atmos. Environ., 77, 283–300, 2013.</mixed-citation></ref>
      <ref id="bib1.bibx7"><label>Denier van der Gon et al.(2015)</label><?label vandergon2015?><mixed-citation>Denier van der Gon, H. A. C., Bergström, R., Fountoukis, C., Johansson, C., Pandis, S. N., Simpson, D., and Visschedijk, A. J. H.: Particulate emissions from residential wood combustion in Europe – revised estimates and an evaluation, Atmos. Chem. Phys., 15, 6503–6519, <ext-link xlink:href="https://doi.org/10.5194/acp-15-6503-2015" ext-link-type="DOI">10.5194/acp-15-6503-2015</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx8"><label>eKlima(2018)</label><?label eklima?><mixed-citation>eKlima: Weather and climate data from Norwegian Meteorological Institute from historical data to real time observations, Norwegian Meteorological Institute, available at:  <uri>http://eklima.no</uri>, last access: 14 August 2018.</mixed-citation></ref>
      <ref id="bib1.bibx9"><label>Finstad et al.(2004)</label><?label Finstad2004?><mixed-citation>
Finstad, A., Flugsrud, K.,  Haakonsen G., and  Aasestad, K.: Vedforbruk, fyringsvaner og svevestøv: Undersøkelse om vedforbruk og fyringsvaner i Trondheim og Bergen 2003 2006/2007 Statistics Norway, Oslo, Norway, ISBN 82-537-6700-5, 2004.</mixed-citation></ref>
      <ref id="bib1.bibx10"><label>GAINS(2000)</label><?label GAINS?><mixed-citation>GAINS:  Greenhouse  gas  and  Air  pollution  Interaction  Model, IIASA,  Laxenburg,  available  at: <uri>http://gains.iiasa.ac.at/models/</uri> (last access: 12 September 2018), 2000.</mixed-citation></ref>
      <ref id="bib1.bibx11"><label>Genberg et al.(2011)</label><?label Genberg2011?><mixed-citation>Genberg, J., Hyder, M., Stenström, K., Bergström, R., Simpson, D., Fors, E. O., Jönsson, J. Å., and Swietlicki, E.: Source apportionment of carbonaceous aerosol in southern Sweden, Atmos. Chem. Phys., 11, 11387–11400, <ext-link xlink:href="https://doi.org/10.5194/acp-11-11387-2011" ext-link-type="DOI">10.5194/acp-11-11387-2011</ext-link>, 2011.</mixed-citation></ref>
      <ref id="bib1.bibx12"><label>Haakonsen and Kvingedal(2001)</label><?label HAA2001?><mixed-citation>
Haakonsen, G. and Kvingedal, E.: Utslipp til luft fra vedfyring i Norge. Utslippsfaktorer, ildstedsbestand og fyringsvaner. Statistics Norway, Repport 2001/36. Oslo–Kongsvinger, Norway, 2001.</mixed-citation></ref>
      <ref id="bib1.bibx13"><label>Hak(2017)</label><?label H2017?><mixed-citation>
Hak, C.: Vurdering av Black Carbon (BC) og CO2 langs veg i Oslo. NILU/OR Report 11/2017, Norwegian Institute for Air Research, Kjeller, Norway, 2017 (in Norwegian).</mixed-citation></ref>
      <ref id="bib1.bibx14"><label>Hamer et al.(2019)</label><?label Hamer2019?><mixed-citation>Hamer, P. D., Walker, S.-E., Sousa-Santos, G., Vogt, M., Vo-Thanh, D., Lopez-Aparicio, S., Ramacher, M. O. P., and Karl, M.: The urban dispersion model EPISODE. Part 1: A Eulerian and subgrid-scale air quality model and its application in Nordic winter conditions, Geosci. Model Dev. Discuss., <ext-link xlink:href="https://doi.org/10.5194/gmd-2019-199" ext-link-type="DOI">10.5194/gmd-2019-199</ext-link>, in review, 2019.</mixed-citation></ref>
      <ref id="bib1.bibx15"><label>Heringa et al.(2012)</label><?label Heringa2012?><mixed-citation>
Heringa, M. F., DeCarlo, P. F., Chirico, R., Lauber, A., Doberer, A., Good, J., and Miljevic, B.: Time-resolved characterization of primary emissions from residential wood combustion appliances, Environ. Sci. Technol., 46, 11418–11425, 2012.</mixed-citation></ref>
      <ref id="bib1.bibx16"><label>Jones(1999)</label><?label Jones1999?><mixed-citation>Jones, P. W.: First- and second-order conservative remapping schemes for grids in spherical coordinates, Mon. Weather Rev., 127, 2204–2210, <ext-link xlink:href="https://doi.org/10.1175/1520-0493(1999)127&lt;2204:FASOCR&gt;2.0.CO;2" ext-link-type="DOI">10.1175/1520-0493(1999)127&lt;2204:FASOCR&gt;2.0.CO;2</ext-link>, 1999.</mixed-citation></ref>
      <ref id="bib1.bibx17"><label>Karagulian et al.(2015)</label><?label Karagulian2015?><mixed-citation>
Karagulian, F., Belis, C. A., Dora, C. F. C., Prüss-Ustün, A. M., Bonjour, S., Adair-Rohani, H., and Amann, M.: Contributions to cities' ambient particulate matter (PM): A systematic review of local source contributions at global level, Atmos. Environ., 120, 475–483, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx18"><label>Krecl et al.(2008)</label><?label Kercl2008?><mixed-citation>Krecl, P., Hedberg Larsson, E., Ström, J., and Johansson, C.: Contribution of residential wood combustion and other sources to hourly winter aerosol in Northern Sweden determined by positive matrix factorization, Atmos. Chem. Phys., 8, 3639–3653, <ext-link xlink:href="https://doi.org/10.5194/acp-8-3639-2008" ext-link-type="DOI">10.5194/acp-8-3639-2008</ext-link>, 2008.</mixed-citation></ref>
      <ref id="bib1.bibx19"><label>Kuenen et al.(2014)</label><?label Kuenen2014?><mixed-citation>Kuenen, J. J. P., Visschedijk, A. J. H., Jozwicka, M., and Denier van der Gon, H. A. C.: TNO-MACC_II emission inventory; a multi-year (2003–2009) consistent high-resolution European emission inventory for air quality modelling, Atmos. Chem. Phys., 14, 10963–10976, <ext-link xlink:href="https://doi.org/10.5194/acp-14-10963-2014" ext-link-type="DOI">10.5194/acp-14-10963-2014</ext-link>, 2014.</mixed-citation></ref>
      <ref id="bib1.bibx20"><label>Levander and Bodin (2014)</label><?label Levander2014?><mixed-citation>Levander, T. and Bodin, S.: Controlling Emissions from Wood Burning. Legislation and Regulation in Nordic Countries to Control Emissions from Residential Wood Burning. An Examination of Past Experience. TemaNord 2014:517. Nordic Council of Ministers, Copenhagen, Denmark, available at: <uri>http://www.diva-portal.org/smash/get/diva2:710531/FULLTEXT01.pdf</uri> (last access: 15 September 2016), 2014.</mixed-citation></ref>
      <ref id="bib1.bibx21"><label>Lopez-Aparicio and Vo Thanh(2017)</label><?label Susana2017?><mixed-citation>
Lopez-Aparicio, S. and Vo Thanh, D.: Emission estimates for Norwegian cities. NBV Emission Database v.0, NILU (NILU OR, 35/2015), Kjeller, Norway, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx22"><label>Lopez-Aparicio et al.(2017b)</label><?label Susana2017c?><mixed-citation>
López-Aparicio, S., Guevara, M., Thunis, P., Cuvelierd, K., and Tarrasón, L.: Assessment of discrepancies between bottom-up and regional emission inventories in Norwegian urban areas, Atmos. Environ., 154, 285–296, 2017b.</mixed-citation></ref>
      <ref id="bib1.bibx23"><label>Lopez-Aparicio et al.(2018)</label><?label Susana2018?><mixed-citation>Lopez-Aparicio, S., Grythe, H., Vogt, M. , Pierson, M., and Vallejo, I.: Webcrawling and Machine Learning as a New Approach for the Spatial Distribution of Atmospheric Emissions, PLoS ONE, 13, e0200650, <ext-link xlink:href="https://doi.org/10.1371/journal.pone.0200650" ext-link-type="DOI">10.1371/journal.pone.0200650</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bibx24"><label>Marécal et al.(2015)</label><?label Marecal2015?><mixed-citation>Marécal, V., Peuch, V.-H., Andersson, C., Andersson, S., Arteta, J., Beekmann, M., Benedictow, A., Bergström, R., Bessagnet, B., Cansado, A., Chéroux, F., Colette, A., Coman, A., Curier, R. L., Denier van der Gon, H. A. C., Drouin, A., Elbern, H., Emili, E., Engelen, R. J., Eskes, H. J., Foret, G., <?pagebreak page10237?>Friese, E., Gauss, M., Giannaros, C., Guth, J., Joly, M., Jaumouillé, E., Josse, B., Kadygrov, N., Kaiser, J. W., Krajsek, K., Kuenen, J., Kumar, U., Liora, N., Lopez, E., Malherbe, L., Martinez, I., Melas, D., Meleux, F., Menut, L., Moinat, P., Morales, T., Parmentier, J., Piacentini, A., Plu, M., Poupkou, A., Queguiner, S., Robertson, L., Rouïl, L., Schaap, M., Segers, A., Sofiev, M., Tarasson, L., Thomas, M., Timmermans, R., Valdebenito, Á., van Velthoven, P., van Versendaal, R., Vira, J., and Ung, A.: A regional air quality forecasting system over Europe: the MACC-II daily ensemble production, Geosci. Model Dev., 8, 2777–2813, <ext-link xlink:href="https://doi.org/10.5194/gmd-8-2777-2015" ext-link-type="DOI">10.5194/gmd-8-2777-2015</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx25"><label>Norsk Standard 3059(1994)</label><?label NS1994?><mixed-citation>Norsk Standard 3059: Enclosed wood heaters – Smoke emission – Requirements, available at: <uri>https://www.standard.no/nettbutikk/produktkatalogen/produktpresentasjon/?ProductID=133351</uri> (last access: 9 December 2018), 1994.</mixed-citation></ref>
      <ref id="bib1.bibx26"><label>NEA(2018)</label><?label NEA2018?><mixed-citation>
Norwegian Environment Agency (NEA): Informative Inventory Report (IIIR) 2018 Norway. Air Pollutant Emissions 1990–2018. Rapport M-967, Oslo, Norway, 2018.</mixed-citation></ref>
      <ref id="bib1.bibx27"><label>Plejdrup et al.(2016)</label><?label Plejdrup2016?><mixed-citation>Plejdrup, M. S., Nielsen, O.-K., and Brandt, J.: Spatial emission modelling for residential wood combustion in Denmark, Atmos. Environ., 144, 389–396, <ext-link xlink:href="https://doi.org/10.1016/j.atmosenv.2016.09.013" ext-link-type="DOI">10.1016/j.atmosenv.2016.09.013</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bibx28"><label>Pope(2000)</label><?label Pope2000?><mixed-citation>
Pope, C. A.: Review: Epidemiological Basis for Particulate Air Pollution Health Standards, Aerosol Sci. Tech., 32, 4–14, 2000.</mixed-citation></ref>
      <ref id="bib1.bibx29"><label>Quayle and Diaz(1980)</label><?label Quayle1980?><mixed-citation>
Quayle, R. G. and Diaz, H. F.: Heating degree-day data applied to residential heating energy consumption, J. Appl. Meteorol., 19, 241–246, 1980.</mixed-citation></ref>
      <ref id="bib1.bibx30"><label>Raymer(2006)</label><?label Raymer2006?><mixed-citation>Raymer, A. K. P.: A comparison of avoided greenhouse gas emissions when using different kinds of wood energy, Biomass and Bioenergy, 30, 605–617, <ext-link xlink:href="https://doi.org/10.1016/j.biombioe.2006.01.009" ext-link-type="DOI">10.1016/j.biombioe.2006.01.009</ext-link>, 2006.</mixed-citation></ref>
      <ref id="bib1.bibx31"><label>Sandradewi et al.(2008)</label><?label S2008?><mixed-citation>
Sandradewi, J., Prévôt, A. S. H., Szidat, S., Perron, N., Alfarra, M. R., Lanz, V. A., Weingartner, E., and Baltensperger, U.: Using aerosol light absorption measurements for the quantitative determination of wood burning and traffic emission contributions to particulate matter, Environ. Sci. Technol., 42, 3316–3323, 2008.</mixed-citation></ref>
      <ref id="bib1.bibx32"><label>Sciare et al.(2013)</label><?label Sciare2013?><mixed-citation>Sciare, J., Sarda-Esteve, R., Favez, O., Cachier, H., Aymoz, G., and Laj, P.: Nighttime residential wood burning evidenced from an indirect method for estimating real-time concentration of particulate organic matter (POM), Atmos. Environ., 42, 2158–2172, 2008.
 </mixed-citation></ref><?xmltex \hack{\newpage}?>
      <ref id="bib1.bibx33"><label>Seljeskog et al.(2013)</label><?label Seljeskog2013?><mixed-citation>
Seljeskog, M., Goile, F., Sevault, A., and Lamberg, H.: Particle emission factors for wood stove firing in Norway, SINTEF Energi AS, Trondheim, Norway, 2013.</mixed-citation></ref>
      <ref id="bib1.bibx34"><label>Seljeskog et al.(2017)</label><?label Seljeskog2017?><mixed-citation>Seljeskog, M., Goile, F., and Skreiberg, Ø.: Recommended revisions of Norwegian emission factors for wood stoves, Energy Procedia, 105, 1022–1028, <ext-link xlink:href="https://doi.org/10.1016/j.egypro.2017.03.447" ext-link-type="DOI">10.1016/j.egypro.2017.03.447</ext-link>, 2017.</mixed-citation></ref>
      <ref id="bib1.bibx35"><label>Seity et al.(2011)</label><?label Seity2011?><mixed-citation>
Seity, Y., Brousseau, P., Malardel, S., Hello, G., Bénard, P., Bouttier, F., Lac, C., and Masson, V.: The AROME‐France convective‐scale operational model, Mon. Weather Rev., 139, 976–991, 2011.</mixed-citation></ref>
      <ref id="bib1.bibx36"><label>SSB(2018)</label><?label SSB2018?><mixed-citation>SSB: <uri>https://www.ssb.no/en/energi-og-industri/statistikker/energiregnskap</uri>, last access: 19 September 2018.</mixed-citation></ref>
      <ref id="bib1.bibx37"><label>Stohl et al.(2013)</label><?label Stohl2013?><mixed-citation>Stohl, A., Klimont, Z., Eckhardt, S., Kupiainen, K., Shevchenko, V. P., Kopeikin, V. M., and Novigatsky, A. N.: Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions, Atmos. Chem. Phys., 13, 8833–8855, <ext-link xlink:href="https://doi.org/10.5194/acp-13-8833-2013" ext-link-type="DOI">10.5194/acp-13-8833-2013</ext-link>, 2013.</mixed-citation></ref>
      <ref id="bib1.bibx38"><label>Tarrasón et al.(2017)</label><?label Leonor2017?><mixed-citation>
Tarrasón, L., Sousa Santos, G., Vo Thanh, D., Vogt, M., López-Aparicio, S., Denby, B., Tønnesen, D., Sundvor, I., Røen, H. V., and Høiskar, B. A. K.: Air quality in Norwegian cities in 2015. Evaluation report for NBV main results (NILU report 21/2017), NILU, Kjeller, Norway, 2017.</mixed-citation></ref>
      <ref id="bib1.bibx39"><label>Terrenoire et al.(2015)</label><?label Terrenoire2015?><mixed-citation>Terrenoire, E., Bessagnet, B., Rouïl, L., Tognet, F., Pirovano, G., Létinois, L., Beauchamp, M., Colette, A., Thunis, P., Amann, M., and Menut, L.: High-resolution air quality simulation over Europe with the chemistry transport model CHIMERE, Geosci. Model Dev., 8, 21–42, <ext-link xlink:href="https://doi.org/10.5194/gmd-8-21-2015" ext-link-type="DOI">10.5194/gmd-8-21-2015</ext-link>, 2015.</mixed-citation></ref>
      <ref id="bib1.bibx40"><label>Timmermans et al.(2013)</label><?label Timmermans2013?><mixed-citation>
Timmermans, R. M. A., van der Gon, H. D., Kuenen, J. J. P., Segers, A. J.,  Honoré, C., Perrussel, O., Builtjesa, P. J. H., and Schaap, M.: Quantification of the urban air pollution increment and its dependency on the use of down-scaled and bottom-up city emission inventories, Urban Climate, 6, 44–62, 2013.</mixed-citation></ref>
      <ref id="bib1.bibx41"><label>Yttri et al.(2011)</label><?label Yttri2011?><mixed-citation>Yttri, K. E., Simpson, D., Stenström, K., Puxbaum, H., and Svendby, T.: Source apportionment of the carbonaceous aerosol in Norway – quantitative estimates based on <inline-formula><mml:math id="M257" display="inline"><mml:mrow class="chem"><mml:msup><mml:mi/><mml:mn mathvariant="normal">14</mml:mn></mml:msup><mml:mi mathvariant="normal">C</mml:mi></mml:mrow></mml:math></inline-formula>, thermal-optical and organic tracer analysis, Atmos. Chem. Phys., 11, 9375–9394, <ext-link xlink:href="https://doi.org/10.5194/acp-11-9375-2011" ext-link-type="DOI">10.5194/acp-11-9375-2011</ext-link>, 2011.</mixed-citation></ref>

  </ref-list></back>
    <!--<article-title-html>The MetVed model: development and evaluation of emissions from residential wood combustion at high spatio-temporal resolution in Norway</article-title-html>
<abstract-html><p>We present here emissions estimated from a newly developed emission model for residential wood combustion (RWC) at high spatial and temporal resolution, which we name the MetVed model. The model estimates hourly emissions resolved on a 250&thinsp;m grid resolution for several compounds, including particulate matter (PM), black carbon (BC) and polycyclic aromatic hydrocarbons (PAHs) in Norway for a 12-year period. The model uses novel input data and calculation methods that combine databases built with an unprecedented high level of detail and near-national coverage. The model establishes wood burning potential at the grid based on the dependencies between variables that influence emissions: i.e. outdoor temperature, number of and type and size of dwellings, type of available heating technologies, distribution of wood-based heating installations and their associated emission factors. RWC activity with a 1&thinsp;h temporal profile was produced by combining heating degree day and hourly and weekday activity profiles reported by wood consumers in official statistics. This approach results in an improved characterisation of the spatio-temporal distribution of wood use, and subsequently of emissions, required for urban air quality assessments. Whereas most variables are calculated based on bottom-up approaches on a 250&thinsp;m spatial grid, the MetVed model is set up to use official wood consumption at the county level and then distributes consumption to individual grids proportional to the physical traits of the residences within it. MetVed combines consumption with official emission factors that makes the emissions also upward scalable from the 250&thinsp;m grid to the national level.</p><p>The MetVed spatial distribution obtained was compared at the urban scale to other existing emissions at the same scale. The annual urban emissions, developed according to different spatial proxies, were found to have differences up to an order of magnitude. The MetVed total annual PM<sub>2.5</sub> emissions in the urban domains compare well to emissions adjusted based on concentration measurements. In addition, hourly PM<sub>2.5</sub> concentrations estimated by an Eulerian dispersion model using MetVed emissions were compared to measurements at air quality stations. Both hourly daily profiles and the seasonality of PM<sub>2.5</sub> show a slight overestimation of PM<sub>2.5</sub> levels. However, a comparison with black carbon from biomass burning and benzo(a)pyrene measurements indicates higher emissions during winter than that obtained by MetVed. The accuracy of urban emissions from RWC relies on the accuracy of the wood consumption (activity data), emission factors and the spatio-temporal distribution. While there are still knowledge gaps regarding emissions, MetVed represents a vast improvement in the spatial and temporal distribution of RWC.</p></abstract-html>
<ref-html id="bib1.bib1"><label>Aasestad(2010)</label><mixed-citation>
Aasestad, K.: Vedforbruk, fyringsvaner og svevestøv Dokumentasjon og resultater fra undersøkelse i Drammen 2006/2007 Statistics Norway, Oslo, Norway, ISBN 978-82-537-7823-5, 2010.
</mixed-citation></ref-html>
<ref-html id="bib1.bib2"><label>ACAP(2014)</label><mixed-citation>
ACAP: Reduction of Black Carbon Emissions from Residential Wood Combustion in the Arctic – Black Carbon Inventory, Abatement Instruments and Measures. Arctic Contaminants Action Program (ACAP), Oslo, Norway,
ISBN 978-82-999755-1-3, 164 pp., 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib3"><label>Andersson et al.(2015)</label><mixed-citation>
Andersson, S., Arvelius, J., Brodl, L., Verbova, M., Ortiz, C., Jonsson, M., Svanström, S., Gerner, A., Danielsson, H., and Yaramenka, K.: Metod- och kvalitetsbeskrivning för geografiskt fördelade emissioner till luft (submission 2018). SMED Rapport Nr10 2018, Sveriges Meteorologiska och Hydrologiska Institut, Norrköping, Sweden, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib4"><label>Bloch(2018)</label><mixed-citation>
Bloch, V. V. H.: Registerbasert boligstatistikk, Dokumentasjon og videre arbeid. 2018/2 Statistcs Norway ISBN 978-82-537-9676-5, available at: <a href="http://www.ssb.no/natur-og-miljo" target="_blank">http://www.ssb.no/natur-og-miljo</a>, last access: 9 December 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib5"><label>Denby(2009)</label><mixed-citation>
Denby, B.: Source-Receptor and Inverse Modelling to quantify urban PARTiculate emissions (SRIMPART). Nordic Council of Ministers, Copenhagen, Denmark, 2009.
</mixed-citation></ref-html>
<ref-html id="bib1.bib6"><label>Denby et al.(2013)</label><mixed-citation>
Denby, B., Sundvor, I., Johansson, C., Pirjola, L., Ketzel, M., Norman, M.,  Kupiainen, K., Gustafsson, M., Blomqvist, G., and Omstedt, G.: A coupled road dust and surface moisture model to predict non-exhaust road traffic induced particle emissions (NORTRIP). Part 1: Road dust loading and suspension modelling, Atmos. Environ., 77, 283–300, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib7"><label>Denier van der Gon et al.(2015)</label><mixed-citation>
Denier van der Gon, H. A. C., Bergström, R., Fountoukis, C., Johansson, C., Pandis, S. N., Simpson, D., and Visschedijk, A. J. H.: Particulate emissions from residential wood combustion in Europe – revised estimates and an evaluation, Atmos. Chem. Phys., 15, 6503–6519, <a href="https://doi.org/10.5194/acp-15-6503-2015" target="_blank">https://doi.org/10.5194/acp-15-6503-2015</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib8"><label>eKlima(2018)</label><mixed-citation>
eKlima: Weather and climate data from Norwegian Meteorological Institute from historical data to real time observations, Norwegian Meteorological Institute, available at:  <a href="http://eklima.no" target="_blank">http://eklima.no</a>, last access: 14 August 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib9"><label>Finstad et al.(2004)</label><mixed-citation>
Finstad, A., Flugsrud, K.,  Haakonsen G., and  Aasestad, K.: Vedforbruk, fyringsvaner og svevestøv: Undersøkelse om vedforbruk og fyringsvaner i Trondheim og Bergen 2003 2006/2007 Statistics Norway, Oslo, Norway, ISBN 82-537-6700-5, 2004.
</mixed-citation></ref-html>
<ref-html id="bib1.bib10"><label>GAINS(2000)</label><mixed-citation>
GAINS:  Greenhouse  gas  and  Air  pollution  Interaction  Model, IIASA,  Laxenburg,  available  at: <a href="http://gains.iiasa.ac.at/models/" target="_blank">http://gains.iiasa.ac.at/models/</a> (last access: 12 September 2018), 2000.
</mixed-citation></ref-html>
<ref-html id="bib1.bib11"><label>Genberg et al.(2011)</label><mixed-citation>
Genberg, J., Hyder, M., Stenström, K., Bergström, R., Simpson, D., Fors, E. O., Jönsson, J. Å., and Swietlicki, E.: Source apportionment of carbonaceous aerosol in southern Sweden, Atmos. Chem. Phys., 11, 11387–11400, <a href="https://doi.org/10.5194/acp-11-11387-2011" target="_blank">https://doi.org/10.5194/acp-11-11387-2011</a>, 2011.
</mixed-citation></ref-html>
<ref-html id="bib1.bib12"><label>Haakonsen and Kvingedal(2001)</label><mixed-citation>
Haakonsen, G. and Kvingedal, E.: Utslipp til luft fra vedfyring i Norge. Utslippsfaktorer, ildstedsbestand og fyringsvaner. Statistics Norway, Repport 2001/36. Oslo–Kongsvinger, Norway, 2001.
</mixed-citation></ref-html>
<ref-html id="bib1.bib13"><label>Hak(2017)</label><mixed-citation>
Hak, C.: Vurdering av Black Carbon (BC) og CO2 langs veg i Oslo. NILU/OR Report 11/2017, Norwegian Institute for Air Research, Kjeller, Norway, 2017 (in Norwegian).
</mixed-citation></ref-html>
<ref-html id="bib1.bib14"><label>Hamer et al.(2019)</label><mixed-citation>
Hamer, P. D., Walker, S.-E., Sousa-Santos, G., Vogt, M., Vo-Thanh, D., Lopez-Aparicio, S., Ramacher, M. O. P., and Karl, M.: The urban dispersion model EPISODE. Part 1: A Eulerian and subgrid-scale air quality model and its application in Nordic winter conditions, Geosci. Model Dev. Discuss., <a href="https://doi.org/10.5194/gmd-2019-199" target="_blank">https://doi.org/10.5194/gmd-2019-199</a>, in review, 2019.
</mixed-citation></ref-html>
<ref-html id="bib1.bib15"><label>Heringa et al.(2012)</label><mixed-citation>
Heringa, M. F., DeCarlo, P. F., Chirico, R., Lauber, A., Doberer, A., Good, J., and Miljevic, B.: Time-resolved characterization of primary emissions from residential wood combustion appliances, Environ. Sci. Technol., 46, 11418–11425, 2012.
</mixed-citation></ref-html>
<ref-html id="bib1.bib16"><label>Jones(1999)</label><mixed-citation>
Jones, P. W.: First- and second-order conservative remapping schemes for grids in spherical coordinates, Mon. Weather Rev., 127, 2204–2210, <a href="https://doi.org/10.1175/1520-0493(1999)127&lt;2204:FASOCR&gt;2.0.CO;2" target="_blank">https://doi.org/10.1175/1520-0493(1999)127&lt;2204:FASOCR&gt;2.0.CO;2</a>, 1999.
</mixed-citation></ref-html>
<ref-html id="bib1.bib17"><label>Karagulian et al.(2015)</label><mixed-citation>
Karagulian, F., Belis, C. A., Dora, C. F. C., Prüss-Ustün, A. M., Bonjour, S., Adair-Rohani, H., and Amann, M.: Contributions to cities' ambient particulate matter (PM): A systematic review of local source contributions at global level, Atmos. Environ., 120, 475–483, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib18"><label>Krecl et al.(2008)</label><mixed-citation>
Krecl, P., Hedberg Larsson, E., Ström, J., and Johansson, C.: Contribution of residential wood combustion and other sources to hourly winter aerosol in Northern Sweden determined by positive matrix factorization, Atmos. Chem. Phys., 8, 3639–3653, <a href="https://doi.org/10.5194/acp-8-3639-2008" target="_blank">https://doi.org/10.5194/acp-8-3639-2008</a>, 2008.
</mixed-citation></ref-html>
<ref-html id="bib1.bib19"><label>Kuenen et al.(2014)</label><mixed-citation>
Kuenen, J. J. P., Visschedijk, A. J. H., Jozwicka, M., and Denier van der Gon, H. A. C.: TNO-MACC_II emission inventory; a multi-year (2003–2009) consistent high-resolution European emission inventory for air quality modelling, Atmos. Chem. Phys., 14, 10963–10976, <a href="https://doi.org/10.5194/acp-14-10963-2014" target="_blank">https://doi.org/10.5194/acp-14-10963-2014</a>, 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib20"><label>Levander and Bodin (2014)</label><mixed-citation>
Levander, T. and Bodin, S.: Controlling Emissions from Wood Burning. Legislation and Regulation in Nordic Countries to Control Emissions from Residential Wood Burning. An Examination of Past Experience. TemaNord 2014:517. Nordic Council of Ministers, Copenhagen, Denmark, available at: <a href="http://www.diva-portal.org/smash/get/diva2:710531/FULLTEXT01.pdf" target="_blank">http://www.diva-portal.org/smash/get/diva2:710531/FULLTEXT01.pdf</a> (last access: 15 September 2016), 2014.
</mixed-citation></ref-html>
<ref-html id="bib1.bib21"><label>Lopez-Aparicio and Vo Thanh(2017)</label><mixed-citation>
Lopez-Aparicio, S. and Vo Thanh, D.: Emission estimates for Norwegian cities. NBV Emission Database v.0, NILU (NILU OR, 35/2015), Kjeller, Norway, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib22"><label>Lopez-Aparicio et al.(2017b)</label><mixed-citation>
López-Aparicio, S., Guevara, M., Thunis, P., Cuvelierd, K., and Tarrasón, L.: Assessment of discrepancies between bottom-up and regional emission inventories in Norwegian urban areas, Atmos. Environ., 154, 285–296, 2017b.
</mixed-citation></ref-html>
<ref-html id="bib1.bib23"><label>Lopez-Aparicio et al.(2018)</label><mixed-citation>
Lopez-Aparicio, S., Grythe, H., Vogt, M. , Pierson, M., and Vallejo, I.: Webcrawling and Machine Learning as a New Approach for the Spatial Distribution of Atmospheric Emissions, PLoS ONE, 13, e0200650, <a href="https://doi.org/10.1371/journal.pone.0200650" target="_blank">https://doi.org/10.1371/journal.pone.0200650</a>, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib24"><label>Marécal et al.(2015)</label><mixed-citation>
Marécal, V., Peuch, V.-H., Andersson, C., Andersson, S., Arteta, J., Beekmann, M., Benedictow, A., Bergström, R., Bessagnet, B., Cansado, A., Chéroux, F., Colette, A., Coman, A., Curier, R. L., Denier van der Gon, H. A. C., Drouin, A., Elbern, H., Emili, E., Engelen, R. J., Eskes, H. J., Foret, G., Friese, E., Gauss, M., Giannaros, C., Guth, J., Joly, M., Jaumouillé, E., Josse, B., Kadygrov, N., Kaiser, J. W., Krajsek, K., Kuenen, J., Kumar, U., Liora, N., Lopez, E., Malherbe, L., Martinez, I., Melas, D., Meleux, F., Menut, L., Moinat, P., Morales, T., Parmentier, J., Piacentini, A., Plu, M., Poupkou, A., Queguiner, S., Robertson, L., Rouïl, L., Schaap, M., Segers, A., Sofiev, M., Tarasson, L., Thomas, M., Timmermans, R., Valdebenito, Á., van Velthoven, P., van Versendaal, R., Vira, J., and Ung, A.: A regional air quality forecasting system over Europe: the MACC-II daily ensemble production, Geosci. Model Dev., 8, 2777–2813, <a href="https://doi.org/10.5194/gmd-8-2777-2015" target="_blank">https://doi.org/10.5194/gmd-8-2777-2015</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib25"><label>Norsk Standard 3059(1994)</label><mixed-citation>
Norsk Standard 3059: Enclosed wood heaters – Smoke emission – Requirements, available at: <a href="https://www.standard.no/nettbutikk/produktkatalogen/produktpresentasjon/?ProductID=133351" target="_blank">https://www.standard.no/nettbutikk/produktkatalogen/produktpresentasjon/?ProductID=133351</a> (last access: 9 December 2018), 1994.
</mixed-citation></ref-html>
<ref-html id="bib1.bib26"><label>NEA(2018)</label><mixed-citation>
Norwegian Environment Agency (NEA): Informative Inventory Report (IIIR) 2018 Norway. Air Pollutant Emissions 1990–2018. Rapport M-967, Oslo, Norway, 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib27"><label>Plejdrup et al.(2016)</label><mixed-citation>
Plejdrup, M. S., Nielsen, O.-K., and Brandt, J.: Spatial emission modelling for residential wood combustion in Denmark, Atmos. Environ., 144, 389–396, <a href="https://doi.org/10.1016/j.atmosenv.2016.09.013" target="_blank">https://doi.org/10.1016/j.atmosenv.2016.09.013</a>, 2016.
</mixed-citation></ref-html>
<ref-html id="bib1.bib28"><label>Pope(2000)</label><mixed-citation>
Pope, C. A.: Review: Epidemiological Basis for Particulate Air Pollution Health Standards, Aerosol Sci. Tech., 32, 4–14, 2000.
</mixed-citation></ref-html>
<ref-html id="bib1.bib29"><label>Quayle and Diaz(1980)</label><mixed-citation>
Quayle, R. G. and Diaz, H. F.: Heating degree-day data applied to residential heating energy consumption, J. Appl. Meteorol., 19, 241–246, 1980.
</mixed-citation></ref-html>
<ref-html id="bib1.bib30"><label>Raymer(2006)</label><mixed-citation>
Raymer, A. K. P.: A comparison of avoided greenhouse gas emissions when using different kinds of wood energy, Biomass and Bioenergy, 30, 605–617, <a href="https://doi.org/10.1016/j.biombioe.2006.01.009" target="_blank">https://doi.org/10.1016/j.biombioe.2006.01.009</a>, 2006.
</mixed-citation></ref-html>
<ref-html id="bib1.bib31"><label>Sandradewi et al.(2008)</label><mixed-citation>
Sandradewi, J., Prévôt, A. S. H., Szidat, S., Perron, N., Alfarra, M. R., Lanz, V. A., Weingartner, E., and Baltensperger, U.: Using aerosol light absorption measurements for the quantitative determination of wood burning and traffic emission contributions to particulate matter, Environ. Sci. Technol., 42, 3316–3323, 2008.
</mixed-citation></ref-html>
<ref-html id="bib1.bib32"><label>Sciare et al.(2013)</label><mixed-citation>
Sciare, J., Sarda-Esteve, R., Favez, O., Cachier, H., Aymoz, G., and Laj, P.: Nighttime residential wood burning evidenced from an indirect method for estimating real-time concentration of particulate organic matter (POM), Atmos. Environ., 42, 2158–2172, 2008.

</mixed-citation></ref-html>
<ref-html id="bib1.bib33"><label>Seljeskog et al.(2013)</label><mixed-citation>
Seljeskog, M., Goile, F., Sevault, A., and Lamberg, H.: Particle emission factors for wood stove firing in Norway, SINTEF Energi AS, Trondheim, Norway, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib34"><label>Seljeskog et al.(2017)</label><mixed-citation>
Seljeskog, M., Goile, F., and Skreiberg, Ø.: Recommended revisions of Norwegian emission factors for wood stoves, Energy Procedia, 105, 1022–1028, <a href="https://doi.org/10.1016/j.egypro.2017.03.447" target="_blank">https://doi.org/10.1016/j.egypro.2017.03.447</a>, 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib35"><label>Seity et al.(2011)</label><mixed-citation>
Seity, Y., Brousseau, P., Malardel, S., Hello, G., Bénard, P., Bouttier, F., Lac, C., and Masson, V.: The AROME‐France convective‐scale operational model, Mon. Weather Rev., 139, 976–991, 2011.
</mixed-citation></ref-html>
<ref-html id="bib1.bib36"><label>SSB(2018)</label><mixed-citation>
SSB: <a href="https://www.ssb.no/en/energi-og-industri/statistikker/energiregnskap" target="_blank">https://www.ssb.no/en/energi-og-industri/statistikker/energiregnskap</a>, last access: 19 September 2018.
</mixed-citation></ref-html>
<ref-html id="bib1.bib37"><label>Stohl et al.(2013)</label><mixed-citation>
Stohl, A., Klimont, Z., Eckhardt, S., Kupiainen, K., Shevchenko, V. P., Kopeikin, V. M., and Novigatsky, A. N.: Black carbon in the Arctic: the underestimated role of gas flaring and residential combustion emissions, Atmos. Chem. Phys., 13, 8833–8855, <a href="https://doi.org/10.5194/acp-13-8833-2013" target="_blank">https://doi.org/10.5194/acp-13-8833-2013</a>, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib38"><label>Tarrasón et al.(2017)</label><mixed-citation>
Tarrasón, L., Sousa Santos, G., Vo Thanh, D., Vogt, M., López-Aparicio, S., Denby, B., Tønnesen, D., Sundvor, I., Røen, H. V., and Høiskar, B. A. K.: Air quality in Norwegian cities in 2015. Evaluation report for NBV main results (NILU report 21/2017), NILU, Kjeller, Norway, 2017.
</mixed-citation></ref-html>
<ref-html id="bib1.bib39"><label>Terrenoire et al.(2015)</label><mixed-citation>
Terrenoire, E., Bessagnet, B., Rouïl, L., Tognet, F., Pirovano, G., Létinois, L., Beauchamp, M., Colette, A., Thunis, P., Amann, M., and Menut, L.: High-resolution air quality simulation over Europe with the chemistry transport model CHIMERE, Geosci. Model Dev., 8, 21–42, <a href="https://doi.org/10.5194/gmd-8-21-2015" target="_blank">https://doi.org/10.5194/gmd-8-21-2015</a>, 2015.
</mixed-citation></ref-html>
<ref-html id="bib1.bib40"><label>Timmermans et al.(2013)</label><mixed-citation>
Timmermans, R. M. A., van der Gon, H. D., Kuenen, J. J. P., Segers, A. J.,  Honoré, C., Perrussel, O., Builtjesa, P. J. H., and Schaap, M.: Quantification of the urban air pollution increment and its dependency on the use of down-scaled and bottom-up city emission inventories, Urban Climate, 6, 44–62, 2013.
</mixed-citation></ref-html>
<ref-html id="bib1.bib41"><label>Yttri et al.(2011)</label><mixed-citation>
Yttri, K. E., Simpson, D., Stenström, K., Puxbaum, H., and Svendby, T.: Source apportionment of the carbonaceous aerosol in Norway – quantitative estimates based on <sup>14</sup>C, thermal-optical and organic tracer analysis, Atmos. Chem. Phys., 11, 9375–9394, <a href="https://doi.org/10.5194/acp-11-9375-2011" target="_blank">https://doi.org/10.5194/acp-11-9375-2011</a>, 2011.
</mixed-citation></ref-html>--></article>
