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  <front>
    <journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>

    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-16-2997-2016</article-id><title-group><article-title>Fingerprints of a riming event on cloud radar Doppler spectra: observations
and modeling</article-title>
      </title-group><?xmltex \runningtitle{Fingerprints of a riming event on cloud radar Doppler spectra}?><?xmltex \runningauthor{H. Kalesse et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1 aff3">
          <name><surname>Kalesse</surname><given-names>Heike</given-names></name>
          <email>kalesse@tropos.de</email>
        <ext-link>https://orcid.org/0000-0001-6699-7040</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Szyrmer</surname><given-names>Wanda</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff4">
          <name><surname>Kneifel</surname><given-names>Stefan</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-2220-2968</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff5">
          <name><surname>Kollias</surname><given-names>Pavlos</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Luke</surname><given-names>Edward</given-names></name>
          
        </contrib>
        <aff id="aff1"><label>1</label><institution>McGill University Montreal, Montréal, QC, Canada</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Brookhaven National Laboratory, Upton, NY,
USA</institution>
        </aff>
        <aff id="aff3"><label>a</label><institution>now at: Leibniz-Institute for Tropospheric Research,
Leipzig, Germany</institution>
        </aff>
        <aff id="aff4"><label>b</label><institution>now at: University of Cologne, Cologne,
Germany</institution>
        </aff>
        <aff id="aff5"><label>c</label><institution>now at: Stony Brook University, Stony Brook, NY, USA</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Heike Kalesse (kalesse@tropos.de)</corresp></author-notes><pub-date><day>9</day><month>March</month><year>2016</year></pub-date>
      
      <volume>16</volume>
      <issue>5</issue>
      <fpage>2997</fpage><lpage>3012</lpage>
      <history>
        <date date-type="received"><day>23</day><month>July</month><year>2015</year></date>
           <date date-type="rev-request"><day>22</day><month>October</month><year>2015</year></date>
           <date date-type="rev-recd"><day>11</day><month>February</month><year>2016</year></date>
           <date date-type="accepted"><day>16</day><month>February</month><year>2016</year></date>
      </history>
      <permissions>
<license license-type="open-access">
<license-p>This work is licensed under a Creative Commons Attribution 3.0 Unported License. To view a copy of this license, visit <ext-link ext-link-type="uri" xlink:href="http://creativecommons.org/licenses/by/3.0/">http://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions><self-uri xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016.html">This article is available from https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016.pdf</self-uri>


      <abstract>
    <p>Radar Doppler spectra measurements are exploited to study a riming event when
precipitating ice from a seeder cloud sediment through a supercooled liquid
water (SLW) layer. The focus is on the “golden sample” case study for this
type of analysis based on observations collected during the deployment of the
Atmospheric Radiation Measurement Program's (ARM) mobile facility AMF2 at
Hyytiälä, Finland, during the Biogenic Aerosols – Effects on Clouds
and Climate (BAECC) field campaign. The presented analysis of the height
evolution of the radar Doppler spectra is a state-of-the-art retrieval with
profiling cloud radars in SLW layers beyond the traditional use of spectral
moments. Dynamical effects are considered by following the particle
population evolution along slanted tracks that are caused by horizontal
advection of the cloud under wind shear conditions. In the SLW layer, the
identified liquid peak is used as an air motion tracer to correct the Doppler
spectra for vertical air motion and the ice peak is used to study the radar
profiles of rimed particles. A 1-D steady-state bin microphysical model is
constrained using the SLW and air motion profiles and cloud top radar
observations. The observed radar moment profiles of the rimed snow can be
simulated reasonably well by the model, but not without making several
assumptions about the ice particle concentration and the relative role of
deposition and aggregation. This suggests that in situ observations of key
ice properties are needed to complement the profiling radar observations
before process-oriented studies can effectively evaluate ice microphysical
parameterizations.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

      <?xmltex \hack{\newpage}?>
<sec id="Ch1.S1" sec-type="intro">
  <title>Introduction</title>
      <p>Mixed-phase clouds are ubiquitous, long-lived, and cover extended areas (e.g.,
Shupe et al., 2008; Zhang et al., 2010; Kanitz et al., 2011). However, the
factors governing the formation, maintenance, and dissipation of mixed-phase
clouds are poorly understood and consequently not well represented in weather
and climate models (Cantrell and Heymsfield, 2005; Lebo et al., 2008; Barrett
et al., 2010). The complex interaction between atmospheric vertical motions,
aerosol particles, water vapor, liquid water, and ice determine the radiative
and microphysical properties of mixed-phase clouds to a large extent (Gregory
and Morris, 1996). Microphysical processes such as water vapor diffusion,
collision, coalescence, aggregation, and riming are controlled by the
variable mass ratio between liquid water and ice (Pruppacher and Klett,
1997). The ongoing increase in the temporal and spatial resolution of
numerical models suggests that cloud microphysical processes will be modeled
in ever more detail in the coming decades (Klein et al., 2013). In that
context, the development of process-level understanding has been found to be
a key for success in addressing the complicated nature of mixed-phase clouds
and improving their representation in numerical models (Morrison et al.,
2012).</p>
      <p>Mixed-phase clouds pose a serious observational challenge due to the
difficulty of identifying the presence of supercooled liquid
water (SLW) layers embedded in cloud regions dominated by ice (Luke et al., 2010). Existing mixed-phase cloud
classifications are highly uncertain and lead to a misrepresentation of these
clouds in models (Illingworth et al., 2007). Moving beyond the detection of
SLW layers and into process-oriented studies (e.g., riming) requires
synergetic observations with cloud Doppler radars and microwave radiometers
(MWRs) in combination with backscatter and Doppler lidars (e.g., Verlinde et
al., 2013). As highlighted in Kollias et al. (2007a) spectral Doppler
information is expected to be one of the main tools for future observational
studies on cloud microphysics (see Sect. 2.3 for details).</p>
      <p>Here, a 35 GHz cloud Doppler radar is used in synergy with a microwave
radiometer to identify and characterize a SLW layer within a mixed-phase
cloud and its effect on the cloud microphysics. The recorded radar Doppler
spectra are bimodal, thus comprised of a liquid and an ice spectral peak
(e.g., Shupe et al., 2004). As in Shupe et al. (2004), the vertical air
motion within the SLW layer is retrieved from cloud radar Doppler spectra.
The liquid peak radar reflectivity is used to retrieve the SLW profile while
the spectral peak associated with typical ice and snow terminal velocities is
used to detect and follow the evolution of riming. The temporal (height)
evolution of the radar Doppler spectrum is analyzed along slanted fall
streaks from cloud top to cloud base to optimally follow the particles'
history in order to gain insight into microphysical processes occurring in
different layers of the mixed-phase cloud (Marshall, 1953; Hogan and Kew,
2005).</p>
      <p>This study illustrates the objective steps in identifying the impact of a
microphysical process (riming) on radar observations (fingerprints) and the
steps required to analyze a multi-sensor data set containing radar Doppler
spectra. While the implementation of the aforementioned retrieval and
analysis technique is valuable, this is not purely a retrieval effort. The
main question this study aims to address is to what extent such
process-oriented studies (i.e., fingerprinting studies) can be used to
evaluate existing riming efficiency parameterizations (e.g., Hall, 1980;
Cober and List, 1993; Lohmann, 2004). To accomplish this, a 1-D steady-state
bin microphysics model is used to model the riming event. Restating that this
is not a retrieval contribution, the goal is not to reproduce the evolution
of riming ice spectra peak moments but rather to assess whether the
observations can sufficiently constrain other parameters and factors that can
affect the model output.</p>
      <p>The structure of the paper is as follows. The data, instrumentation, and
background of radar Doppler spectra processing are introduced in Sect. 2.
Section 3 gives a detailed analysis of the snowfall case study including a
description of the synoptic situation (Sect. 3.1), the in situ observations
(Sect. 3.2), the cloud radar and MWR observations as well as the fall streak
tracking technique, and the evolution of the cloud radar Doppler spectrum
(Sect. 3.3). In Sect. 3.4 the 1-D microphysical bin model used to reproduce
the rimed-mode radar moments is described and a comparison of observations
with model results is discussed. A summary and conclusions are provided in
Sect. 4.</p>
</sec>
<sec id="Ch1.S2">
  <title>Data, instrumentation, and Doppler spectra processing</title>
<sec id="Ch1.S2.SS1">
  <title>BAECC field campaign overview</title>
      <p>From 1 February to 12 September 2014 the Biogenic Aerosols – Effects on
Clouds and Climate (BAECC) field experiment (Petäjä et al., 2016) –
a joint project of the University of Helsinki, the Finnish Meteorological
Institute, and the US Department of Energy (DOE) Atmospheric Radiation
measurement (ARM) program – took place in the boreal forest of southern
Finland. For that purpose, extensive remote sensing and in situ
instrumentation was installed at the Station for Measuring
Ecosystem–Atmosphere Relations (SMEAR II, Hari and Kulmala, 2005) at the
Hyytiälä field station of the University of Helsinki located at
61<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>50<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>′</mml:mo></mml:msup></mml:math></inline-formula>37.114<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:math></inline-formula> N and 24<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>17<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>′</mml:mo></mml:msup></mml:math></inline-formula>15.709<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>′</mml:mo><mml:mo>′</mml:mo></mml:mrow></mml:msup></mml:math></inline-formula> E, 150 m above
sea level. Within that frame, an intensive observation period focusing
on winter precipitation (BAECC-Snowfall Experiment (SNEX)) organized in
collaboration with the National Aeronautics and Space Administration (NASA)
Global Precipitation Measurement (GPM) ground validation program and Colorado
State University was conducted from 1 February to 30 April 2014.</p>
</sec>
<sec id="Ch1.S2.SS2">
  <title>Instrumentation</title>
      <p>The second ARM Mobile Facility (AMF2), consisting of an extensive suite of
remote sensing instruments such as a Ka-band ARM Zenith-pointing Radar
(KAZR), a W-, <?xmltex \hack{\mbox\bgroup}?>Ka-,<?xmltex \hack{\egroup}?> and X-band Scanning ARM Cloud Radar (Kollias et al., 2014),
a micropulse lidar (MPL), a High Spectral Resolution Lidar (HSRL), and a
two-channel MWR (Cadeddu et al., 2013) was deployed at the observation site.
The lidars are used for detection of cloud base height and cloud particle
phase, the radars for characterization of cloud and precipitation
microphysics, and the MWR for determination of column-integrated amounts of
liquid water and water vapor. For this study, data from the Ka-band ARM
Zenith-pointing Radar (KAZR) operating at 35 GHz, as well as the MWR are
used.</p>
      <p>Ground-based in situ sensors included a Particle Imaging Package (PIP),
which is a new version of the Snow Video Imager (Newman et al., 2009).
Pluvio weighing gauges were employed to measure precipitation rate and
snowfall accumulation. Pluvios were also used in combination with the PIP
for determination of total particle concentration, particle size
distribution (PSD), and particle terminal fall velocities from which fall
velocity–size relations were derived at high temporal resolution.</p>
      <p>For a detailed description of the measurement site setup as well as the
in situ and remote sensing instrumentation and data processing please refer
to Kneifel et al. (2015). In addition to the mentioned instrumentation,
radiosondes were launched four times daily for profiling of the atmospheric
state variables.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><caption><p>Vertical profiles of temperature (blue, left) and dew point
temperature (red, left), relative humidity (middle, black), as well as
horizontal wind speed (right, black) and wind direction (right, blue) from a
radiosonde launched at 23:20 UTC (23.33 UTC) on 21 February 2014 in Hyytiälä.
The red line in the middle panel refers to the humidity at which the air is
saturated with respect to ice; i.e., if the relative humidity is to
the right of the red line, the air is supersaturated ice (grey
shading).</p></caption>
          <?xmltex \igopts{width=298.753937pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f01.pdf"/>

        </fig>

</sec>
<sec id="Ch1.S2.SS3">
  <title>Doppler spectra processing</title>
      <p>The mean Doppler velocity from profiling radars has been used in past studies
to detect and study riming. Initially, Weiss and Hobbs (1975) distinguished
ice crystal growth by riming from growth by water vapor deposition by
observing the different rates of change of mean Doppler velocity with height.
Mosimann (1995) used a vertically pointing Doppler radar in combination with
snow crystal in situ measurements to quantitatively determine an index of the
degree of riming in stratiform precipitation, a technique which has been used
in further studies (e.g., Borys et al., 2003; Baschek et al., 2004).</p>
      <p>Today, advancements in signal processing and radar technology and decreasing
storage costs have enabled the routine recording of the full radar Doppler
spectrum. The radar Doppler spectrum often contains unique signatures that
can be used to retrieve cloud microphysics and dynamics (Kollias et al.,
2007b). In particular, the presence of liquid cloud droplets in the radar
sampling volume allows use of the Doppler spectra peak of the liquid
particles to derive the mean vertical air motion of the sampling volume.
This approach is based on the assumption that the terminal velocity of small
cloud droplets is negligible compared to typical vertical air motions in
clouds (Kollias et al., 2001). Thus, the location of the peak caused by
liquid droplets in the Doppler spectrum can act as a tracer for vertical air
motion.</p>
      <p>This implies that in SLW layers also containing ice particles, if the liquid
spectral peak does not significantly overlap the ice peak in velocity, then
the cloud dynamics (vertical air motion and eddy dissipation rate) can be
retrieved (Kollias et al., 2001; Shupe et al., 2004). The potential of using
multimodal cloud radar Doppler spectra for characterizing the liquid- and
ice-phase components in mixed-phase clouds has been previously demonstrated
(e.g., Shupe et al., 2004; Luke et al., 2010; Luke and Kollias, 2013;
Rambukkange et al., 2011; Verlinde et al., 2013; Yu et al., 2014).</p>
      <p>Here, in addition to the objective detection and analysis of the SLW spectral
peaks, the temporal evolution of the radar Doppler spectrum is analyzed along
slanted fall streaks from cloud top to cloud base to gain insight into
microphysical processes occurring in different layers in mixed-phase clouds.
As already highlighted in Marshall (1953), this is necessary in situations
when vertical wind shear is observed. Under these conditions, following the
particle evolution along straight vertical paths is not suitable for detailed
fingerprinting studies. To track radar moments in cirrus, this technique has
been refined in Hogan and Kew (2005). Similar to their approach, we do not
simply follow the fall streaks in the observations but compare them with
simulated fall streaks by using the horizontal wind profile and Doppler fall
velocity. In this way we can ensure consistency between the expected fall
streak shape, which is solely based on dynamics and particles' fall velocity,
and the observations. This approach helps to avoid a subjective and
potentially false identification of a fall streak in the observations that
might be caused, e.g., by different generating processes and levels or
directional wind shear that would hamper the derivation of particle history
along the fall streak. To our knowledge, this is the first study in which the
evolution of the full Doppler spectrum along <italic>slanted</italic> fall streak
paths is analyzed.</p>
      <p>Finally, the SLW radar reflectivity is extracted from the SLW spectral peak
and used to derive the profile of SLW content within the SLW layer while the
ice rimed spectral peak is used to derive the radar observables of the rimed
particles.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><caption><p>KAZR-observed primary Doppler spectrum peak moments on
21 February 2014 in Hyytiälä. Panel <bold>(a)</bold> shows reflectivity (dBZ),
<bold>(b)</bold> mean Doppler velocity (m s<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, and <bold>(c)</bold> spectrum
width of the primary Doppler spectrum peak (m s<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. Negative Doppler
velocities indicate downward motion.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f02.pdf"/>

        </fig>

</sec>
</sec>
<sec id="Ch1.S3">
  <title>Case study analysis</title>
<sec id="Ch1.S3.SS1">
  <?xmltex \opttitle{Synoptic situation in Hyyti\"{a}l\"{a} on 21~February~2014}?><title>Synoptic situation in Hyytiälä on 21 February 2014</title>
      <p>On 21 February 2014 a low-pressure system situated between Iceland and the
British Isles influenced the weather in most parts of Europe. Several surface
fronts associated with the weather system moved to the east/northeast. The
most prominent one was a partially occluded front that crossed western Europe
and reached the stage of a fully developed occlusion further east. Due to
increased vertical mixing, it had the characteristics of a warm occlusion
near the surface with rising temperatures behind the passage of the front.
The advection of warm air is indicated by a veering vertical wind profile in
the radio sounding launched at 23.2 UTC as shown in Fig. 1. With
warm air sliding over cold air, the first clouds associated with this system
were found at higher levels (around 8 km).</p>
      <p>Prior to the arrival of the warm occlusion in Hyytiälä, multiple
cloud layers were present which are obvious in the radiosonde launched at
23.33 UTC. The cloud base of the frontal system was continuously lowering
with the approaching warm occlusion. Also, the reflectivity of the cloud as
observed by the 35 GHz vertically pointing cloud radar KAZR (cf. Fig. 2)
showed tilted fall streak features above 3.5 km altitude, indicating vertical
wind shear consistent with the radio sounding profile of horizontal wind. The
temperature profile shows two inversion layers, a boundary layer inversion at
0.5–0.8 km at which a shallow low-level cloud had formed and a second one
at 2.8–3 km where a mid-level cloud had formed as illustrated in Fig. 3.
Cloud top temperatures of the warm occlusion front and the mid-level cloud
were <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>50 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C (at 8 km) and <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>12 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C (at 3.4 km), while
the surface temperature was <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>3 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C, respectively. The ambient
relative humidity profile shows layers of saturated/subsaturated conditions
associated with the two distinct cloud layers extending from 2.3 km and
higher as well as from 0.2 to 0.9 km. Subsaturated conditions leading to
sublimation prevailed between 0.8 and 2.3 km as well as below 0.2 km. Thus,
snowfall associated with the onset of the frontal system (22.7–22.8 UTC)
experienced sublimation before reaching the ground.</p>
</sec>
<sec id="Ch1.S3.SS2">
  <title>In situ observations</title>
      <p>During the period of interest when the snow front moved in (22.7–22.8 UTC),
in situ observations showed low snowfall rates below (0.3 mm h<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> and
low total ice particle concentrations (<inline-formula><mml:math display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 100 m<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>. PIP images were
often out of focus; however, the structure of several individual ice
particles was identified: in addition to small and large oriented dendrites,
fast-falling roundish particles with high density – an indication of riming
– were observed. In the PIP 22 min time integration interval
22.52–22.88 UTC, area-equivalent maximum observed diameters were less than
1.5 mm (D. Moisseev, personal communication, 2015). Afterwards (PIP integration time interval
22.88–23.06 UTC), the maximum particle size increased to 3 mm and snowfall
rate was still low but doubled to 0.6 mm h<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Later on (after
23.06 UTC) heavy snowfall of large low-density aggregates was observed with
the ground-based instruments and multi-frequency radar measurements as
discussed in Kneifel et al. (2015). During the time of interest of this
study, the X-SACR was not operated in vertically pointing mode.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3"><caption><p>A schematic diagram of the cloud layers present in Hyytiälä
on 21 February 2014. Sketch is overlying the KAZR reflectivity.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f03.jpg"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS3">
  <title>KAZR and MWR observations</title>
      <p>In Fig. 2 the time–height plots of the first three moments (effective radar
reflectivity factor Ze, subsequently called reflectivity; mean Doppler
velocity <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, and spectral width (<inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>)) of the primary peak of
the KAZR Doppler spectrum are shown. The primary peak is defined to be the
noise-separated peak containing the bin with maximum power spectral density
(cf. Fig. 4; Kollias et al., 2007b). This is the peak used in the standard
ARM radar moments data products. The ARM MicroARSCL data product (Kollias et
al., 2007b) extends the reported moments to skewness and kurtosis for both
the primary peak and an additional noise-separated secondary peak, if one
exists. The peak power densities and modal velocities of up to two local
maxima occurring within the primary peak are also reported. Mean and maximum
spectral noise power are determined using the technique described in
Hildebrand and Sekhon (1974). If only one hydrometeor population is present
in the radar volume (cf. Fig. 4a), the radar Doppler spectrum is usually
characterized by a single peak above noise floor, which is controlled by the
width of the PSD and sub-volume turbulence. In cases with more than one
hydrometeor class in the radar volume (e.g, liquid droplets and snow) it is
possible to have sufficient fall velocity separation between the two
hydrometeor classes so that the radar Doppler spectra is bimodal. As
mentioned in Luke and Kollias (2013), strongly multimodal situations can be
considered to be “golden” samples as they make it easy to separate the
contributions of the individual hydrometeor populations to the total radar
return. Here, we classify all peaks which are separated by the mean noise
floor into three categories (liquid droplets, freshly generated ice, and
(rimed) snow). Peaks are grouped into these classes according to their mean
Doppler velocity and spectrum width. However, in many observations, the
terminal fall velocity difference between two different particle size
distributions is not large enough to produce individual peaks separated by
the mean noise floor. Instead, broad merged peaks consisting of the
contribution of two or more PSDs occur (cf. Fig. 4d). This is also the reason
why only a short time period is analyzed in this study; synoptic situations
in which ice particles from a “seeder” cloud above are falling through a
SLW layer where they experience riming occurred at least half a dozen times
during the BAECC-SNEX period but unfortunately, for all other events, only
merged peaks were observed in the KAZR Doppler spectra.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><caption><p>Examples of KAZR Doppler spectra at different times and heights.
Notice the different <inline-formula><mml:math display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> scales. Maximum and mean noise floor
determined according to Hildebrand and Sekhon (1974) are indicated by grey
and black horizontal lines, respectively. The primary peak is labeled as 1st,
the secondary peak as 2nd. The mean Doppler velocity of primary peak is shown
by the vertical grey line. The plots are created with the Doppler Spectrum
Visualizer, a visualization toolkit which is publicly available at
<uri>http://www.gim.bnl.gov/armclouds/specvis_java_toolkit/</uri>.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f04.png"/>

        </fig>

      <p>An objective way to distinguish spherical supercooled liquid droplets from
freshly generated nonspherical ice would be the use of spectral linear
depolarization ratio (LDR). Unfortunately though, no KAZR cross-polarization
channel data were gathered during BAECC-SNEX and thus no LDR could be
determined. However, microphysical modeling sensitivity tests (not shown)
showed that unrealistically high ice particle number concentrations – on the
order of a few hundreds to a few thousands per liter for ice particle sizes
of a few hundred microns – would be required to produce a peak of about
<inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>20 to <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>15 dBZ at 0.15 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. For this regime of sizes, the
observed ice particle number concentration reported in the literature is
below 10 per liter (e.g., Zhang et al., 2014; Lloyd et al., 2015). We can
thus assume that power spectrum peaks at small velocities are due to liquid
droplets and not ice particles.</p>
      <p>In this study, the focus is on the period when the upper level snow band
moves in, roughly from 22.4 UTC when first detected by the KAZR to the end
of the first snow shower at around 22.77 UTC. In the KAZR reflectivity field
(cf. Fig. 2a) the onset of snowfall is clearly visible by the high Ze
(<inline-formula><mml:math display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>5 dBZ) area extending from a fall streak feature at a height of
8 km downwards. The Ze structure is strongly tilted above 3.5 km due to
horizontal wind shear. The decrease in Ze at 22.7–22.77 UTC below 1 km can
likely be attributed to sublimation in an ice-subsaturated layer (cf.
humidity profile in Fig. 1).</p>
      <p>Before the arrival of the snow band in Hyytiälä, a liquid-topped
mixed-phase cloud with cloud top at 3.4 km is observed (see Fig. 3). Its
roughly 500 m thick SLW layer can clearly be distinguished by mean Doppler
velocities of around 0.0 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in Fig. 2b, as well as very narrow
spectrum width values below 0.08 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and low reflectivity values
(Ze <inline-formula><mml:math display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>15 dBZ). A typical KAZR Doppler spectrum example within this
liquid layer is shown in Fig. 4a. Within this SLW layer new ice formation
took place at about <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>12 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C; subsequently, the ice sedimented and
grew in size as reflected by a gradual increase of Ze (22.4–22.69 UTC)
between 2.9 and 0.9 km, as well as an increase of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>. A
Doppler spectrum example of this freshly generated ice mode is shown in
Fig. 4c. The rapid increase of Ze below 0.9 km prior to the snowfall
indicates ice particle riming which is confirmed by the ground-based in situ
observations of rimed ice crystals during that time period. The riming most
likely occurred in another SLW layer at the lower inversion at 0.7–0.9 km,
characterized by mostly non-noise-floor-separated liquid peaks in the Doppler
spectra (not shown). Strong surface turbulence below 0.8 km is obvious in
highly variable <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and high <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>. The strong turbulence in the
surface layer led to a broadening of the Doppler spectra peaks which resulted
in broad merged peaks (not separated by the noise floor) and thus hampered
the application of our microphysical retrievals for that SLW layer.</p>
      <p>When the snow band starts falling through the SLW layer, the primary peak
moments are not sufficient to capture the radar view of the microphysics. The
coincidence of liquid and ice particle size distributions within the KAZR
sampling volume leads to multimodal KAZR radar Doppler spectra due to the
terminal fall velocity difference between the liquid droplets and the falling
snow (Fig. 4b). As obvious in Fig. 4b, the snow falling through the SLW layer
has a higher dynamic range than the liquid mode and is thus classified as the
principle peak, leading to a sudden change of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> values in Fig. 2b
after 22.69 UTC and below 3.4 km. Similarly, the sudden high values of
<inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> at 22.68–22.7 UTC and below 2 km can be explained by a merged
peak of the freshly generated ice and the snow which are no longer separated
by the mean noise floor, as illustrated in Fig. 4d. The strong increase of
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> (on the order of 0.5 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, cf. Fig. 2b) within the SLW
layer indicates riming of particles, as also seen in the in situ measurements
(cf. Sect. 3.2).</p>
      <p>Observations supporting the presence of riming when the snow fall streak
intercepts the SLW layer are provided in the temporal evolution of the MWR
liquid water path (LWP) shown in Fig. 5b. While the LWP varies between
320 and 400 g m<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> before 22.69 UTC when only the liquid-topped
mixed-phase cloud is present, it rapidly decreases from 400 to
250 g m<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> within 3 min (22.69–22.74 UTC). The observed reduction in
the LWP can partly be attributed to the capturing of SLW droplets by the
falling snowflakes, leading to rimed particles with high density and fast
fall velocities.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5"><caption><p>Zoomed view (2–4 km, 22.54–22.77 UTC) of the snow front on
21 February 2014. Panel <bold>(a)</bold> shows KAZR total reflectivity,
<bold>(b)</bold> microwave radiometer (MWR) liquid water path (LWP),
<bold>(c)</bold> reflectivity of the liquid peak, <bold>(d)</bold> mean Doppler
velocity of the liquid peak used as vertical air motion tracer. The dotted
lines depict individual fall streaks starting at different generating levels
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:math></inline-formula> km (black), <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn>2.9</mml:mn></mml:mrow></mml:math></inline-formula> km
(blue)). All subsequent averaged profiles refer to the area between the two
black fall streaks.</p></caption>
          <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f05.pdf"/>

        </fig>

      <p>It should be noted that the vertically integrated value of LWP cannot be
entirely attributed to the layer of SLW at 2.9–3.4 km. Unfortunately, the
entire vertical distribution of SLW cannot be reconstructed because the lidar
signal was already extinguished by a thin SLW layer at 0.2–0.4 km. However,
two more thin SLW layers were detected by KAZR Doppler spectrum analysis at
0.8–0.9 and 1.5–1.7 km (see Fig. 3). These layers however were
intermittent and coincide in time with the periods of the highest values of
LWP around 22.6–22.65 and 22.7 UTC. When these intermittent layers were
observed, the LWP increased by 60–80 g m<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>; we use this values as the
estimate of their combined contribution to the total LWP. The SLW layer that
had formed at the lower temperature inversion at 0.8 km is a remnant
signature of the long-lived thin mixed-phase cloud with cloud top at just
below 0.9 km that was present since before 14 UTC.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><caption><p>Panels <bold>(a, d)</bold> show KAZR reflectivity (Ze) field. There, the
location of the SLW layer is indicated by thin horizontal black lines. The upper
middle and upper right panels show range and time spectrograms of vertical
profile which is indicated by a black vertical line in <bold>(a)</bold>; the lower
middle and lower right panels along slanted fall streak are shown in <bold>(d)</bold>
as a dashed line. Panel <bold>(b)</bold> shows vertical range spectrogram along vertical black
line in upper left panel, <bold>(c)</bold> time spectrogram at 3.16 km,
<bold>(e)</bold> slanted range spectrogram along dashed line in <bold>(d)</bold>.
Panel <bold>(f)</bold> shows the air-motion-corrected time spectrogram at 3.16 km.</p></caption>
          <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f06.pdf"/>

        </fig>

      <p><?xmltex \hack{\newpage}?>Based on the liquid peak reflectivity (Fig. 5c) of the SLW layer at
2.9–3.4 km the mean liquid water path of this layer (averaged between the
two slanted paths in Fig. 5) was estimated to be 80–90 g m<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
<sec id="Ch1.S3.SS3.SSS1">
  <title>Fall streak tracking</title>
      <p>When vertical wind shear is observed, the analysis of vertical profiles is
not sufficient to correctly trace the paths of evolution of hydrometeor
populations, as already stated in Marshall (1953). Instead, it is necessary
to follow the falling hydrometeor populations along slanted fall streaks if
we want to estimate their microphysical evolution from the particle-generating level (<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> to height <inline-formula><mml:math display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula>. As illustrated in Hogan and
Kew (2005), the slanted fall streak patterns can be simulated in the radar
time–height observation space by taking the mean Doppler velocity
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> as average fall velocity of the particle population and using
the horizontal wind profile <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>u</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, e.g., from radio soundings closest in time
to account for advection:

                  <disp-formula id="Ch1.E1" content-type="numbered"><mml:math display="block"><mml:mrow><mml:mtext>d</mml:mtext><mml:mi>z</mml:mi><mml:mo>/</mml:mo><mml:mtext>d</mml:mtext><mml:msub><mml:mi>t</mml:mi><mml:mtext>rad</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mi>u</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>)</mml:mo><mml:mo>)</mml:mo><mml:mo>/</mml:mo><mml:mo>(</mml:mo><mml:mi>u</mml:mi><mml:mo>(</mml:mo><mml:mi>z</mml:mi><mml:mo>)</mml:mo><mml:mo>-</mml:mo><mml:mi>u</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>)</mml:mo><mml:mo>)</mml:mo><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>

            Here, <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>u</mml:mi><mml:mo>(</mml:mo><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is the horizontal wind velocity at the particle-generating level <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> which is assumed to be close to cloud top
(<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:math></inline-formula> km) and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mtext>rad</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is the radar time (<inline-formula><mml:math display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> axis in
time–height plots in vertically pointing mode). It is important to note that
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mtext>rad</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is usually different from the sedimentation time of the
particle population and that fall streaks are not identical to particle
trajectories but are a result of overlapping trajectories as they are
advected over the radar (Bohren and Fraser, 1992). As in Hogan and
Kew (2005), we use the finite difference equivalent of Eq. (1) and work our
way downward level-by-level considering the displacement at level <inline-formula><mml:math display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> in the
determination of displacement at level <inline-formula><mml:math display="inline"><mml:mrow><mml:mi>z</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>. We use this technique to
determine a fall streak for each radar time step. Subsequently, all averaged
profiles (means and standard deviations) are determined for the fall streaks
spanned between the two black slanted fall streaks in Fig. 5. Our focus of
interest will be the uppermost SLW layer at the height range 2.9–3.4 km.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><caption><p>Slanted profile moments of SLW (blue), ice generated in the SLW
layer (red), and frontal snow (black). Means and standard deviations of
<bold>(a)</bold> reflectivity, <bold>(b)</bold> mean Doppler velocity, and
<bold>(c)</bold> mode width are shown for the slanted paths encompassed by the
two dashed lines in Fig. 5. Within the SLW layer, the velocities are
corrected for vertical air motion.</p></caption>
            <?xmltex \igopts{width=270.301181pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f07.pdf"/>

          </fig>

      <p>The closest radio sounding in time was launched at 23.2 UTC, approximately
45 min after the snow front was first observed with the KAZR. Ideally,
horizontal wind profiles at the time of interest should be used; however,
overall agreement of the slope of the black simulated fall streaks in Fig. 5
with the slope of the reflectivity features (above 2.9 km) seems to confirm
that the horizontal wind field did not change considerably within these
45 min. Below 3 km the slope of the black simulated fall streaks does not
fit well with the Ze feature, which is tilted in the opposite direction
compared to the fall streak above. Additional fall streak simulations
(depicted in blue in Fig. 5a) show that this backward tilted slope is well
matched by simulations if we assume <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>z</mml:mi><mml:mtext>gen</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn>2.9</mml:mn></mml:mrow></mml:math></inline-formula>–3 km and the mean
Doppler velocity of the rimed snow mode in Eq. (1). The lower-level Ze
feature thus corresponds to the fall streaks of those snow particles that
experience riming in the SLW layer and indicates – as expected – the SLW
layer as the correct generating level for the rimed particle population.</p>
</sec>
<sec id="Ch1.S3.SS3.SSS2">
  <title>Doppler spectrum evolution</title>
      <p>Figure 6 illustrates the necessity of tracking particle populations along
slanted paths in conditions of wind shear by contrasting the KAZR Doppler
spectrum evolution along the vertical line at 22.69 UTC in Fig. 6a versus
along the estimated slanted fall streak in Fig. 6d. Clearly, the vertical
range spectrogram in Fig. 6b shows some non-microphysical features – such as
the discontinuity of spectral reflectivity at around 4 km – caused by
taking a vertical profile when a slanted one is more representative. The
range spectrogram along the slanted path in Fig. 6e tells a much more
consistent microphysical evolution story of the particles when the frontal
system moves in: above the 3.4 km height, snow with a mean Doppler velocity
of around 1 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> is observed. A few shallow layers of increased
turbulence as well as thicker layers of up-/downdrafts result in a shift of
the entire Doppler spectrum to more positive/negative values, respectively.
At 2.9–3.4 km, the layer of SLW with <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> fluctuating around
0 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> is obvious in Fig. 6e as well as in the time spectrogram in
Fig. 6c. Due to their small size, the terminal fall velocity of SLW
droplets is negligible, so their <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> (also illustrated in Fig. 5d)
can be used as an air motion tracer as done in previous studies (e.g., Shupe
et al., 2004; Rambukkange et al., 2011). The <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> offset of the
liquid mode from 0 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> gives us an estimate of radar volume mean
vertical air motion. Thus, in the SLW layer, the fall velocity of ice
particles can be corrected for vertical air motion as illustrated in Fig. 6f.
In Fig. 6e, the same air-motion correction is applied in regions with SLW.
Again, the increase of <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> of the snow falling from higher layers
into the SLW layers indicates riming. Also, the new ice mode generated in the
SLW layer is revealed, as its <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> quickly increases from a few
tens of cm s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to 0.8 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> between 2.8
and 2 km.</p><?xmltex \hack{\newpage}?>
</sec>
<sec id="Ch1.S3.SS3.SSS3">
  <title>Profiles and probability density functions (PDFs) of radar
moments</title>
      <p>Although the given observations cannot fully disentangle microphysical and
dynamical effects, a fairly consistent picture of the evolution of the
present hydrometeor populations can be formed (cf. Fig. 6). The means and
standard deviations of Ze, <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, and <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> of slanted profiles of
the three hydrometeor populations (SLW, ice generated in the SLW layer, and
frontal snow) are shown in Fig. 7. The average profile and standard
deviations are based on all 110 simulated fall streaks encompassed by the two
dashed lines in Fig. 5. Since in the Rayleigh scattering regime radar
reflectivity is proportional to the number of particles <inline-formula><mml:math display="inline"><mml:mi>N</mml:mi></mml:math></inline-formula> and to <inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi>D</mml:mi><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula>
(with <inline-formula><mml:math display="inline"><mml:mi>D</mml:mi></mml:math></inline-formula> being the diameter of the droplets), the reflectivity of the SLW
droplets is very low (<inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>18 to <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>22 dBZ on average, cf. Fig. 7a). The
reflectivity of the ice generated in the SLW layer increases between 3.2 and
2 km from <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>16 to <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>10 dBZ because the ice particles grow due to water
vapor deposition and aggregation. At the same time, the <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> of the
ice mode increases from 0.2 to 0.7 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (cf. Fig. 7b). The absence of
an air motion tracer outside of the SLW layer does not allow for vertical air
motion contributions to the observed <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> to be accounted for. As a
result, the observed <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is not equal to the terminal fall velocity
of the ice particles but could be higher (in updrafts) or lower (in
downdrafts). Due to its large particles, the greatest contribution to the
total radar return is of course given by the frontal snow mode. The total
increase of mean Ze of this mode from 6 to 2 km is 12 dBZ; however, from
6 km to the top of the SLW layer, the mean increase of Ze and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>
of the snow mode is only moderate (5 dBZ and 0.15 m s<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>, suggesting
only moderate growth of the snow particles, which is likely due to water
vapor deposition in higher parts of the cloud. <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> of the frontal
snow mode increases from 1 to 1.65 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> between 3.2 and 2 km.
Spectrum width profiles in Fig. 7c show several thin turbulent layers in
which the standard deviation of <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> is high. <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> of the SLW mode is
smallest (0.05–0.07 m s<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> while <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> of the new ice and frontal
snow mode are on the order of 0.1–0.2 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. As previously mentioned,
larger <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> can be caused by a superposition of broad PSD and sub-volume
turbulence.</p>
      <p>Probability density functions (PDFs) of the moments of the three hydrometeor
populations are shown in Fig. 8. Only data points from below the SLW layer
top (3.4 km) down to the surface and between the two black dashed fall
streaks in Fig. 5 are considered. For Ze and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> there is very
little overlap in the PDF of each hydrometeor population. In uniform
beam-filling conditions and sub-volume turbulence, the Doppler spectrum of a
cloud droplet PSD is symmetrical and near-Gaussian, resulting in zero
skewness (Kollias et al., 2011). In contrast, the PDF of the observed SLW
mode is skewed towards negative values, indicating the presence of
supercooled drizzle at around <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>12 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C. The presence of drizzle is
also indicated in Fig. 9 where the joint PDF of skewness and Ze is shown.
While liquid-mode skewness fluctuates around zero for Ze below <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>20 dBZ, it
becomes increasingly negative at higher Ze values of <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>20 to <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>16 dBZ. The
existence of drizzle in SLW layers at the temperature range of <inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>5 to
<inline-formula><mml:math display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>12 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C was also found by Verlinde et al. (2013) for Arctic
multilayered mixed-phase clouds; the skewness-reflectivity signature as
shown in Fig. 9 is qualitatively similar to the signatures observed in warm
drizzle clouds (Luke and Kollias, 2013).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8"><caption><p>Probability density functions (PDFs) of noise-separated peaks of SLW
(blue), ice generated in the SLW layer (red), and frontal snow (black) for
the slanted paths encompassed by the two dashed lines in Fig. 4. Only data
from surface to below top of the SLW layer (3.4 km) are considered. Please
note that the PDF of SLW <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> is cut at 20 %.</p></caption>
            <?xmltex \igopts{width=236.157874pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f08.pdf"/>

          </fig>

</sec>
</sec>
<sec id="Ch1.S3.SS4">
  <title>1-D microphysical bin modeling</title>
      <p>The comprehensive observations were used as input to a one-dimensional (1-D)
bin microphysical model. The model is based on the warm rain model first
presented in Szyrmer et al. (2005) and modified to include the ice processes
of deposition, aggregation, and riming. The leading question is whether it is
possible to reproduce the evolution of the observed radar moments of the
rimed snow mode in the SLW layer using radar forward modeling of the
microphysical model output. Forcing the model output to agree with the
observations could help us to evaluate different proposed riming efficiency
schemes that have been implemented as options in the model (see Appendix A).
The microphysical modeling was limited to the SLW layer between 2.9 and 3.4 km
and focused on the evolution of the moments (Ze, <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) of
the frontal snow mode.</p>
<sec id="Ch1.S3.SS4.SSS1">
  <title>Model description</title>
      <p>The 1-D steady-state model simulates the height evolution
of the bin-resolved snow PSD introduced at the model's uppermost level (which
in this study is the top of the SLW layer at 3.4 km). The model input
includes the vertical profiles of temperature, pressure, relative humidity
(taken from the radio sounding, cf. Fig. 1) and vertical air motion (derived
from the SLW-mode <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>; cf. Fig. 10). The cloud droplet PSD at each
level within the SLW layer is calculated from the liquid peak reflectivity
profile, assuming that the cloud droplets follow a log-normal size distribution
with a height-independent prescribed droplet number concentration <inline-formula><mml:math display="inline"><mml:mi>N</mml:mi></mml:math></inline-formula> and
dispersion parameter <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mtext>PSD</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> (<inline-formula><mml:math display="inline"><mml:mrow><mml:mi>N</mml:mi><mml:mo>=</mml:mo><mml:mn>30</mml:mn></mml:mrow></mml:math></inline-formula> cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">3</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">σ</mml:mi><mml:mtext>PSD</mml:mtext></mml:msub><mml:mo>=</mml:mo><mml:mn>0.4</mml:mn></mml:mrow></mml:math></inline-formula>) which are also taken for calculations of liquid
water content (LWC) in Fig. 10.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9"><caption><p>A joint PDF of frequency of occurrence (number of pixels) of skewness
and reflectivity of supercooled liquid mode encompassed by the two black fall
streaks in Fig. 5.</p></caption>
            <?xmltex \igopts{width=199.169291pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f09.pdf"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10"><caption><p>Mean vertical air motion profile (<inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>air</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, left) derived from
liquid-mode mean Doppler velocity and liquid water content (LWC, right)
derived from liquid peak reflectivity between the two black fall streaks in
Fig. 5, respectively.</p></caption>
            <?xmltex \igopts{width=199.169291pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f10.pdf"/>

          </fig>

      <p>The evolution of the snow mode along the fall streak is simulated by
explicitly calculating the contribution to particle growth by the
microphysical processes of water vapor diffusion, aggregation, and riming. In
the model setup used in the presented simulations, the water vapor deposition
and aggregation processes conserve the area ratio, aspect ratio, and
mass–size relationships. The deposition calculations use the results of Field
et al. (2008) to describe the capacitance, except for the smaller particles
for which the electrostatic capacitance approximation for thin plates is
assumed, and the ventilation factor proposed by Hall and Pruppacher (1976) is
adapted. The value of aggregation efficiency is set to 0.2. Details of the
riming parameterizations are presented in Appendix A.</p>
      <p>The frontal snow PSD is introduced at the uppermost model level in a
functional form of a generalized gamma function with melted diameter
representing particle size. The values of the two shape parameters are taken
from Delanoë et al. (2005) for the form that is most consistent with the
observations. The initial mass–size relation of a power law form with
exponent 2 and prefactor 0.0012 g cm<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> is used. The rimed fraction of
the snow particles at the model's uppermost level is set to 0. The initial
area ratio is calculated from the empirical relation between area ratio and
particle density in Heymsfield et al. (2002) for side plane aggregates
(particle density <inline-formula><mml:math display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 0.18 area ratio<inline-formula><mml:math display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mn>1.5</mml:mn></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11" specific-use="star"><caption><p>A comparison of observed and modeled moments of the frontal snow
mode in the SLW layer. Black solid and dashed lines refer to the mean and
standard deviation of the slanted paths encompassed by the two black fall
streaks in Fig. 5. Model results based on riming efficiencies by Hall &amp;
Cober as well as Lohmann are shown in red and blue, respectively (see text
for details). Model results assuming area ratio increase with mass and rimed
fraction (solid red and blue line) as well as with mass only (dotted red and
blue) are shown.</p></caption>
            <?xmltex \igopts{width=284.527559pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/2997/2016/acp-16-2997-2016-f11.pdf"/>

          </fig>

</sec>
<sec id="Ch1.S3.SS4.SSS2">
  <title>Comparison of model output and observations</title>
      <p>In Fig. 11, KAZR-observed profiles of snow-mode radar moments and the modeled
moments are compared. Backscattering calculations are performed using Mie
spheres with nonuniform mass distribution (Fabry and Szyrmer, 1999). The
terminal velocity of snow particles – unrimed at the top and partially rimed
below – is calculated based on the method proposed by Heymsfield and
Westbrook (2010). However, two different possibilities for the evolution of
the area ratio with riming are implemented. In the first approach (denoted by
1 in Fig. 11) for a given particle maximum diameter, the increase of the
area ratio from the initial value is parameterized as a function of the
aspect ratio modified by riming. In the second approach (denoted by 2 in
Fig. 11) the increase of the area ratio is smaller and is obtained assuming
that the initial relation between area ratio and particle density is
maintained, i.e., the increase of the area ratio results from the increase of
mass only.</p>
      <p>In addition to the sensitivity of the terminal velocity of the rimed snow
particles to the evolution of the area ratio relationship, the sensitivity of
the modeled radar moments of the rimed snow mode to different riming
efficiencies is evaluated. Specifically, in one model realization, the riming
efficiency parameterizations from Hall (1980) and Cober and List (1993) for
small and large ice particles are used, respectively. Model results using
this particular parameterization are denoted as Hall Cober in Fig. 11. In
another model realization, the riming efficiency parameterization proposed by
Lohmann (2004), assuming plates for small D and aggregates for large D is
adapted. Model results using this approach are denoted as Lohmann in
Fig. 11.</p>
      <p>Two effects can explain some of the discrepancies between the observed and
modeled profiles. First, dynamical effects such as turbulence are not
included in the radar forward model that estimates the radar Doppler spectrum
width profile. Thus, the forward simulation cannot reproduce the spectrum
broadening of the rimed mode below 3 km (cf. Fig. 11c). Second, there are
uncertainties in the exact slope of the fall streaks due to the fact that the
horizontal wind profile from the sounding is not taken at the time of
interest but 45 min later. Overall, the evolution of the rimed snow-mode
moments in the SLW layer can be reproduced by the model (within the standard
deviations). In Fig. 11a, the observed and modeled Ze profile shows an
increase from the top of the SLW layer to about 3.15 km which is attributed to an increase of
mass of the snow when the liquid droplets attach to the snowflakes. Below
3.15 km, the <inline-formula><mml:math display="inline"><mml:mrow><mml:mtext>d</mml:mtext><mml:mtext>Ze</mml:mtext><mml:mo>/</mml:mo><mml:mtext>d</mml:mtext><mml:mi>z</mml:mi></mml:mrow></mml:math></inline-formula> is slightly reduced because even
with the increase of mass, the increase of backscatter is very low and at the
same time there is a reduction of particle number concentration. Except for
the aforementioned influence of turbulence on spectrum width, the model
reproduces the mean Doppler velocity and spectrum width profiles well. With
the increase in mass and density during the riming process, particle fall
velocities of the rimed snow steadily increase from top to bottom of the SLW
layer from about 0.95 to 1.2 m s<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The model is also capable of
reproducing the small decrease in the spectrum width due to differences in
the riming efficiency of small and large particles, leading to a small
reduction in the spread of the rimed particles' fall velocities.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S4" sec-type="conclusions">
  <title>Summary and conclusions</title>
      <p>For a frontal winter snowfall event observed at the SMEAR II site in
Hyytiälä in Finland during the BAECC-SNEX field experiment in 2014,
we show that by disentangling the contributions of the different hydrometeor
populations to total vertically pointing cloud radar returns, it is possible
to follow the microphysical evolution of the present cloud and
precipitation particles. For that purpose, we work with the entire radar
Doppler spectrum instead of only considering cloud radar moments, which are
integrated parameters of the spectrum.</p>
      <p>The analysis presented here focuses on a band of snow that falls through a
SLW layer, where it experiences riming and where new ice particle formation
also takes place. A detailed analysis of the vertical evolution of radar
moments of the frontal snow, SLW droplets, and freshly generated ice in terms
of their evolution of radar moments (Ze, <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>, <inline-formula><mml:math display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) is
presented.</p>
      <p>The extensive analysis accounts for the vertical shear of the horizontal wind
and the tracking of particle populations is performed along slanted paths
instead of vertical profiles. Furthermore, the multiple noise-floor-separated
modes of the radar Doppler spectra are analyzed and the moments of the SLW,
ice, and rimed snow determined separately. From the <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> and Ze of
the SLW droplets we estimate vertical air motion and LWC within the SLW
layer, respectively.</p>
      <p>The observations were used to set up and evaluate a 1-D steady-state bin
microphysical model that accounts for the processes of deposition,
aggregation, and riming. In particular, the profiles of vertical air motion
and SLW content, along with thermodynamic variables from the nearest sounding
were used to set up the steady-state conditions within the SLW layer. The
radar moments at the top of the SLW layer were used to initiate the unrimed
snow PSD. The radar Doppler spectrum analysis enabled isolation of the radar
moments of the rimed snow within the SLW layer.</p>
      <p>The microphysical model output (PSD of rimed snow particles) is used as input
to a simple radar forward model that reproduces the three radar Doppler
moments. The scattering model used to estimate the backscattering
cross section of the snow particles is based on a two-layer spherical model
introduced by Fabry and Szyrmer (1999). The uncertainties associated with
this backscattering computation have been discussed in Szyrmer et al. (2012).
While there are several different methods to prescribe the scattering
calculations of snow particles (e.g., Tyynelä et al., 2013; Hogan and
Westbrook, 2014), the height
evolution of the radar moments of the rimed snow mode is not very sensitive
to the scattering method used. Also, the very small particle sizes observed
at the surface indicate that larger snowflakes which produce more complex Mie
scattering, as for example seen later on 21 February 2014 (Kneifel et al.,
2015), were not present during the period of interest.</p>
      <p>Assuming a generalized gamma function with melted diameter representing
particle size and using two different methods to estimate the terminal fall
velocity of the rimed particles as well as two different methods to estimate
the riming efficiency of the snow particles, we were able to reproduce the
observed profiles (Fig. 11). Modeling was also performed, assuming an
exponential snow PSD form (not shown). For this PSD form it is found that the
modeled profiles of the rimed snow Ze and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> are similar to those
modeled using the generalized gamma function PSD. However, for the
exponential PSD assumption, the modeled radar Doppler spectrum width profile
had much less sensitivity to riming efficiency parameterization or choice of
area ratio increase.</p>
      <p>The case presented here was carefully selected to represent a scenario where
riming is the dominant process that modulates the snow radar moments (riming
fingerprinting). The simulations indicate that for fixed parameterizations
for deposition and aggregation, the number of combinations of the riming and
velocity parameterizations resulting in profiles that are comparable to the
observations is rather limited. However, changing any of these factors may
lead to different results. In other words, the effect of choosing different
riming efficiency parameterizations is on the same order as choosing
different options for area ratio increase, and thus also fall velocity
calculations, as indicated by a equidistant spread of modeled profiles of Ze,
and <inline-formula><mml:math display="inline"><mml:mrow><mml:msub><mml:mi>V</mml:mi><mml:mtext>d</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula> in Fig. 11.</p>
      <p>Thus, no clear conclusions can be made as to which riming parameterization
is more appropriate in this particular case due to large sensitivity of the
model simulations to several factors other that those we assume, because of
a lack of additional observational constraints. The profiling radar
observations provide a height evolution perspective, which is a critical
constraint for fingerprinting studies that aim to “isolate” a vertical
layer where a particular microphysical process dominates particle growth.
However, as it is evident from the sensitivity of the simulations, in situ
observations giving exact velocity–size relations, particle size and
density estimates, and information about particle shape are needed to
further limit the choices in the model setup leading to true advancement in
our understanding of riming and other ice microphysical processes. While
extensive ground-based in situ data were gathered during BAECC-SNEX, the
period of interest was characterized by low precipitation rates which
hampered the ground-based microphysical retrievals. Furthermore,
measurements of the LWC and ice PSD at the top of the SLW layer would have
been key parameters to constrain the model runs. This points to the future
need for coordinated (aircraft-based) in situ observations combined with
profiling and scanning radar observations. The DOE ARM Program and the ARM
Aerial Facility (AAF) are well positioned to conduct such targeted
observational–modeling studies in the future.</p>
      <p>The present riming case study was selected from the extensive BAECC campaign
data set due to its nearly ideal situation in which the fall velocity
separation of the different hydrometeor classes is strong enough to produce
individual peaks separated by the mean<?xmltex \hack{\vadjust{\newpage}}?> noise floor
in the cloud radar Doppler spectra. During other riming cases, cloud radar
Doppler spectra multimodalities were observed; however, these peaks were
usually merged. These cases are more complicated to disentangle, most likely
due to a more complex mixture of dominant ice growth processes (water vapor
deposition, aggregation, and riming) which all played an important role.
Fingerprinting studies of <italic>one</italic> particular microphysical growth
process – such as riming – requires more simple microphysical situations as
we think is the case in the presented study.</p>
      <p>In situations with merged broad peaks it is very challenging to define
<italic>objective</italic> peak separation criteria and to thus disentangle the
relative contributions of different hydrometeor populations to the total
radar returns. In a previous mixed-phase cloud radar Doppler spectra study
(Shupe et al., 2004) empirical “peak-picking” criteria were developed by
manual inspection of the peak-picking results. There, it was emphasized that
the criteria depend on the observed mixed-phase cloud cases and cloud radar
sampling parameters (such as temporal resolution and number of fast Fourier transform points).
The development of robust cloud radar Doppler spectra peak separation
criteria in mixed-phase clouds is the topic of future studies; the data set
gathered during the BAECC campaign offers great potential for such studies.</p>
<sec id="Ch1.S4.SSx1" specific-use="unnumbered">
  <title>Data availability</title>
      <p>All data used in this study are publicly accessible at the ARM data archive:
<uri>www.archive.arm.gov</uri>.</p><?xmltex \hack{\clearpage}?>
</sec>
</sec>

      
      </body>
    <back><app-group>

<app id="App1.Ch1.S1">
  <?xmltex \opttitle{Parameterizations of riming efficiency\hack{\break} and physics}?><title>Parameterizations of riming efficiency<?xmltex \hack{\break}?> and physics</title>
      <p>The increase in mass of an individual snow particle via the riming process is
calculated with the stochastic collection equation. Different options for the
calculations of the riming efficiency, the evolution of area ratio and aspect
ratio via the riming process, and the related increase in particle fall
velocity are included in the model. Size-dependent riming efficiency
parameterizations proposed in the literature and introduced in the model can
be separated into two groups. The first group describes the efficiency of
smaller pristine crystals, mainly at the first stage of riming, based on
numerical simulations of Pitter and Pruppacher (1974), Pitter (1977), and
Wang and Ji (2000), and proposed by Hall (1980), Young (1993),
Geresdi (1998), and
Lohman (2004) taken from Mitchell (1990). The second group of
parameterizations introduced in the model are more suitable for larger more
spherical particles; the parameterization developed for the
accretional growth of raindrops (Beard and Grover, 1974), a parameterization
derived for graupel (Cober and List, 1993), and the one proposed by
Lohmann (2004) for aggregates based on the experimental results of Lew et
al. (1986) are included. Some examples of the dependence of the riming efficiency on the
snow particle size calculated for different cloud droplet diameters are shown
in the supporting information of Leinonen and Szyrmer (2015).</p>
      <p><?xmltex \hack{\newpage}?>Different approaches to describing the physics of riming result in different
descriptions of the changes of the properties of particles undergoing riming
growth. Aggregates and branched particles appear to grow by “filling in”,
resulting in an increase of particle effective density while the major
dimension does not change. Mainly, the minor dimension is expected to
increase; but when the particle effective density is large enough, associated
with a quasi-spherical shape, the filling process has to be replaced by an
increase of both dimensions with the aspect ratio maintained (e.g., Morrison
and Grabowski, 2010).
Different options of change of particle aspect ratio accompanying the growth
by riming in the model use the rime density calculated from empirical
formulas (Macklin, 1962; Pflaum and Pruppacher, 1979; Heymsfield and Pflaum,
1985). The following options for the evolution of the area ratio for a given
increase of the rimed fraction can be selected in the model: (i) using one of
the empirical relations of mass–density–area ratio (by choosing an
appropriate relation from the table in Szyrmer et al., 2012 or others), or
(ii) obtained by interpolation based on rimed fraction between the values
associated with the unrimed particle and graupel (as in Lin and Colle, 2011),
or (iii) calculated from the assumed relation of particle geometry between
area ratio and aspect ratio (e.g., Avramov et al., 2011; Jensen and
Harrington, 2015).</p><?xmltex \hack{\clearpage}?>
</app>
  </app-group><ack><title>Acknowledgements</title><p>The authors thank the entire BAECC-SNEX science team, the AMF2 team, and the
SMEAR II staff for data acquisition and analysis, as well as Dimitri Moisseev
for discussion of in situ observational results. The Department of Energy
(DOE) Atmospheric System Research (ASR) program provided funding to conduct
this research through the ASR radar science grant. Heike Kalesse conducted
this work within the framework of the DFG project COMPoSE, GZ: KA 4162/1-1. Work
contributed by Stefan Kneifel was also supported by a PostDoc fellowship from
the German Academic Exchange Service (DAAD).<?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>
Edited by: T. Petäjä</p></ack><ref-list>
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<abstract-html><p class="p">Radar Doppler spectra measurements are exploited to study a riming event when
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assumptions about the ice particle concentration and the relative role of
deposition and aggregation. This suggests that in situ observations of key
ice properties are needed to complement the profiling radar observations
before process-oriented studies can effectively evaluate ice microphysical
parameterizations.</p></abstract-html>
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