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  <front>
    <journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>

    <article-meta>
      <article-id pub-id-type="doi">10.5194/acp-16-14421-2016</article-id><title-group><article-title>Pan-Eurasian Experiment (PEEX): towards a holistic understanding of the feedbacks and interactions in the
land–atmosphere–ocean–society continuum in the northern Eurasian region</article-title>
      </title-group><?xmltex \runningtitle{Pan-Eurasian Experiment (PEEX)}?><?xmltex \runningauthor{H.~K.~Lappalainen et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1 aff2 aff36">
          <name><surname>Lappalainen</surname><given-names>Hanna K.</given-names></name>
          <email>hanna.k.lappalainen@helsinki.fi</email>
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Kerminen</surname><given-names>Veli-Matti</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-0706-669X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff36">
          <name><surname>Petäjä</surname><given-names>Tuukka</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1881-9044</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3">
          <name><surname>Kurten</surname><given-names>Theo</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff4 aff5">
          <name><surname>Baklanov</surname><given-names>Aleksander</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-5396-8440</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff6">
          <name><surname>Shvidenko</surname><given-names>Anatoly</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff7">
          <name><surname>Bäck</surname><given-names>Jaana</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6107-667X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Vihma</surname><given-names>Timo</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6557-7084</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Alekseychik</surname><given-names>Pavel</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff8">
          <name><surname>Andreae</surname><given-names>Meinrat O.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-1968-7925</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff9">
          <name><surname>Arnold</surname><given-names>Stephen R.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff10">
          <name><surname>Arshinov</surname><given-names>Mikhail</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-4599-8287</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Asmi</surname><given-names>Eija</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff10">
          <name><surname>Belan</surname><given-names>Boris</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-1481-6847</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff11">
          <name><surname>Bobylev</surname><given-names>Leonid</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff12">
          <name><surname>Chalov</surname><given-names>Sergey</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6937-7020</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff8">
          <name><surname>Cheng</surname><given-names>Yafang</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-4912-9879</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff12">
          <name><surname>Chubarova</surname><given-names>Natalia</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-8889-0885</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff2">
          <name><surname>de Leeuw</surname><given-names>Gerrit</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1649-6333</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff13">
          <name><surname>Ding</surname><given-names>Aijun</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-4481-5386</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff12">
          <name><surname>Dobrolyubov</surname><given-names>Sergey</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff14">
          <name><surname>Dubtsov</surname><given-names>Sergei</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff15">
          <name><surname>Dyukarev</surname><given-names>Egor</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff16">
          <name><surname>Elansky</surname><given-names>Nikolai</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff17">
          <name><surname>Eleftheriadis</surname><given-names>Kostas</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-2265-4905</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff18">
          <name><surname>Esau</surname><given-names>Igor</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-4122-6340</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff19">
          <name><surname>Filatov</surname><given-names>Nikolay</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff20">
          <name><surname>Flint</surname><given-names>Mikhail</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff13">
          <name><surname>Fu</surname><given-names>Congbin</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff21">
          <name><surname>Glezer</surname><given-names>Olga</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff22">
          <name><surname>Gliko</surname><given-names>Aleksander</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff23">
          <name><surname>Heimann</surname><given-names>Martin</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-6296-5113</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff24">
          <name><surname>Holtslag</surname><given-names>Albert A. M.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-0995-2481</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff25">
          <name><surname>Hõrrak</surname><given-names>Urmas</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff26">
          <name><surname>Janhunen</surname><given-names>Juha</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff27">
          <name><surname>Juhola</surname><given-names>Sirkku</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Järvi</surname><given-names>Leena</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-5224-3448</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Järvinen</surname><given-names>Heikki</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-1879-6804</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff28">
          <name><surname>Kanukhina</surname><given-names>Anna</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff12">
          <name><surname>Konstantinov</surname><given-names>Pavel</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-5064-155X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff29">
          <name><surname>Kotlyakov</surname><given-names>Vladimir</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Kieloaho</surname><given-names>Antti-Jussi</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-9424-3083</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff30">
          <name><surname>Komarov</surname><given-names>Alexander S.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Kujansuu</surname><given-names>Joni</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff31">
          <name><surname>Kukkonen</surname><given-names>Ilmo</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Duplissy</surname><given-names>Ella-Maria</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Laaksonen</surname><given-names>Ari</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1657-2383</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Laurila</surname><given-names>Tuomas</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-1967-0624</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Lihavainen</surname><given-names>Heikki</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6135-4473</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff20">
          <name><surname>Lisitzin</surname><given-names>Alexander</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff5">
          <name><surname>Mahura</surname><given-names>Alexsander</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff32">
          <name><surname>Makshtas</surname><given-names>Alexander</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-9690-9133</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff33">
          <name><surname>Mareev</surname><given-names>Evgeny</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Mazon</surname><given-names>Stephany</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-6788-7828</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff34 aff47">
          <name><surname>Matishov</surname><given-names>Dmitry</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff35 aff36">
          <name><surname>Melnikov</surname><given-names>Vladimir</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff37">
          <name><surname>Mikhailov</surname><given-names>Eugene</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-5736-0996</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Moisseev</surname><given-names>Dmitri</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-4575-0409</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff20">
          <name><surname>Nigmatulin</surname><given-names>Robert</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff38">
          <name><surname>Noe</surname><given-names>Steffen M.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-1514-1140</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff7">
          <name><surname>Ojala</surname><given-names>Anne</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Pihlatie</surname><given-names>Mari</given-names></name>
          
        <ext-link>https://orcid.org/0000-0001-6035-3949</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff39">
          <name><surname>Popovicheva</surname><given-names>Olga</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff40">
          <name><surname>Pumpanen</surname><given-names>Jukka</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff19">
          <name><surname>Regerand</surname><given-names>Tatjana</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff16">
          <name><surname>Repina</surname><given-names>Irina</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff27">
          <name><surname>Shcherbinin</surname><given-names>Aleksei</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff20">
          <name><surname>Shevchenko</surname><given-names>Vladimir</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-9045-297X</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Sipilä</surname><given-names>Mikko</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff16">
          <name><surname>Skorokhod</surname><given-names>Andrey</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-5808-0811</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff9">
          <name><surname>Spracklen</surname><given-names>Dominick V.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff8">
          <name><surname>Su</surname><given-names>Hang</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-4889-1669</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff19">
          <name><surname>Subetto</surname><given-names>Dmitry A.</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-3585-8598</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff41">
          <name><surname>Sun</surname><given-names>Junying</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff19">
          <name><surname>Terzhevik</surname><given-names>Arkady Y.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff37">
          <name><surname>Timofeyev</surname><given-names>Yuri</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff33">
          <name><surname>Troitskaya</surname><given-names>Yuliya</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-3818-9211</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff42">
          <name><surname>Tynkkynen</surname><given-names>Veli-Pekka</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff43">
          <name><surname>Kharuk</surname><given-names>Viacheslav I.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff22">
          <name><surname>Zaytseva</surname><given-names>Nina</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff44">
          <name><surname>Zhang</surname><given-names>Jiahua</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff2">
          <name><surname>Viisanen</surname><given-names>Yrjö</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1">
          <name><surname>Vesala</surname><given-names>Timo</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff7">
          <name><surname>Hari</surname><given-names>Pertti</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff45">
          <name><surname>Hansson</surname><given-names>Hans Christen</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff10">
          <name><surname>Matvienko</surname><given-names>Gennady G.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff12">
          <name><surname>Kasimov</surname><given-names>Nikolai S.</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff44">
          <name><surname>Guo</surname><given-names>Huadong</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff46">
          <name><surname>Bondur</surname><given-names>Valery</given-names></name>
          
        </contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff2 aff12 aff33">
          <name><surname>Zilitinkevich</surname><given-names>Sergej</given-names></name>
          
        <ext-link>https://orcid.org/0000-0002-3909-5436</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff1 aff36">
          <name><surname>Kulmala</surname><given-names>Markku</given-names></name>
          
        <ext-link>https://orcid.org/0000-0003-3464-7825</ext-link></contrib>
        <aff id="aff1"><label>1</label><institution>Department of Physics, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Research and Development, Finnish Meteorological Institute, 00101 Helsinki, Finland</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Department of Chemistry, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>World Meteorological Organization, 1211 Geneva, Switzerland</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>Research and Development Department, Danish Meteorological Institute, 2100 Copenhagen, Denmark</institution>
        </aff>
        <aff id="aff6"><label>6</label><institution>Ecosystem Services and Management, International Institute for Applied Systems Analysis, 2361 Laxenburg, Austria</institution>
        </aff>
        <aff id="aff7"><label>7</label><institution>Department of Forest Sciences, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff8"><label>8</label><institution>Biogeochemistry and Multiphase Chemistry Departments, Max Planck Institute for Chemistry, 55020 Mainz, Germany</institution>
        </aff>
        <aff id="aff9"><label>9</label><institution>Institute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, LS2 9JT, UK</institution>
        </aff>
        <aff id="aff10"><label>10</label><institution>Institute of Atmospheric Optics, Russian Academy of Sciences, Tomsk 634021, Russia</institution>
        </aff>
        <aff id="aff11"><label>11</label><institution>Nansen International Environmental and Remote Sensing Center, St. Petersburg, Russia</institution>
        </aff>
        <aff id="aff12"><label>12</label><institution>Faculty of Geography, Lomonosov Moscow State University, Moscow 119899, Russia</institution>
        </aff>
        <aff id="aff13"><label>13</label><institution>Institute for Climate and Global Change Research &amp; School of Atmospheric Sciences,<?xmltex \hack{\newline}?> Nanjing University, 210023 Nanjing, China</institution>
        </aff>
        <aff id="aff14"><label>14</label><institution>Institute of Chemical Kinetics &amp; Combustion, Russian Academy of Sciences, 630090 Novosibirsk, Russia</institution>
        </aff>
        <aff id="aff15"><label>15</label><institution>Institute of Monitoring of Climatic &amp; Ecological Systems SB RAS, 634055 Tomsk, Russia</institution>
        </aff>
        <aff id="aff16"><label>16</label><institution>A. M. Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences, Moscow, Russia</institution>
        </aff>
        <aff id="aff17"><label>17</label><institution>National Centre of Scientific Research “DEMOKRITOS”, Athens, Greece</institution>
        </aff>
        <aff id="aff18"><label>18</label><institution>Nansen Environmental and Remote Sensing Center/Bjerknes Centre for Climate Research, 5006 Bergen, Norway</institution>
        </aff>
        <aff id="aff19"><label>19</label><institution>Northern Water Problems Institute, Karelian Research Center, Russian Academy of Sciences,185003 Petrozavodsk, Russia</institution>
        </aff>
        <aff id="aff20"><label>20</label><institution>P. P. Shirshov, Institute of Oceanology, Russian Academy of Sciences, Russian Academy of Sciences,<?xmltex \hack{\newline}?> 117997 Moscow, Russia</institution>
        </aff>
        <aff id="aff21"><label>21</label><institution>Institute of Geography, Russian Academy of Sciences, Moscow, Russia</institution>
        </aff>
        <aff id="aff22"><label>22</label><institution>Department of Earth Sciences of the Russian Academy of Sciences, Russian Academy of Sciences,<?xmltex \hack{\newline}?> 119991 Moscow, Russia</institution>
        </aff>
        <aff id="aff23"><label>23</label><institution>Max-Planck-Institute for Biogeochemistry, 07745 Jena, Germany</institution>
        </aff>
        <aff id="aff24"><label>24</label><institution>Meteorology and Air Quality, Wageningen University, 6708 Wageningen, the Netherlands</institution>
        </aff>
        <aff id="aff25"><label>25</label><institution>Institute of Physics, University of Tartu, 18 Ülikooli St., 50090 Tartu, Estonia</institution>
        </aff>
        <aff id="aff26"><label>26</label><institution>Department of World Cultures, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff27"><label>27</label><institution>Department of Environmental Sciences, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff28"><label>28</label><institution>Academic Mobility Department, Russian State Hydrometeorological University, 195196 Saint Petersburg, Russia</institution>
        </aff>
        <aff id="aff29"><label>29</label><institution>Institute of Geography, Russian Academy of Sciences, Moscow, Russia</institution>
        </aff>
        <aff id="aff30"><label>30</label><institution>Institute of Physico-chemical &amp; Biological Problems in Soil Science, Russian Academy of Sciences,<?xmltex \hack{\newline}?> 142290 Institutskaya, Russia</institution>
        </aff>
        <aff id="aff31"><label>31</label><institution>Geophysics and Astronomy, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff32"><label>32</label><institution>Actic &amp; Antarctic Research Institute, Russian Academy of Sciences, 199397 St. Petersburg, Russia</institution>
        </aff>
        <aff id="aff33"><label>33</label><institution>Department of Radiophysics, Nizhny Novgorod State University, Nizhny Novgorod, Russia</institution>
        </aff>
        <aff id="aff34"><label>34</label><institution>Southern Center of Russian Academy of Sciences, Rostov on Don, Russia</institution>
        </aff>
        <aff id="aff35"><label>35</label><institution>Tyumen Scientific Center, Siberian Branch, Russian Academy of Science, Tyumen, Russia</institution>
        </aff>
        <aff id="aff36"><label>36</label><institution>Department of Cryosphere, Tyumen State University, 625003 Tyumen, Russia</institution>
        </aff>
        <aff id="aff37"><label>37</label><institution>Department of Atmospheric Physics, Saint Petersburg State University, 7/9 Universitetskaya nab.,<?xmltex \hack{\newline}?> 199034 St. Petersburg Russia</institution>
        </aff>
        <aff id="aff38"><label>38</label><institution>Institute of Agricultural and Environmental Sciences, Estonian University of Life Sciences, 51014 Tartu, Estonia</institution>
        </aff>
        <aff id="aff39"><label>39</label><institution>Department Microelectronics, Skobeltsyn Institute of Nuclear Physics, Moscow State University,  Moscow 119991, Russia</institution>
        </aff>
        <aff id="aff40"><label>40</label><institution>Department of Environmental Science, University of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland</institution>
        </aff>
        <aff id="aff41"><label>41</label><institution>Graduate University of Chinese Academy of Sciences, 100049 Beijing, China</institution>
        </aff>
        <aff id="aff42"><label>42</label><institution>Aleksanteri Institute, Department of Social Research, University of Helsinki, 00014 Helsinki, Finland</institution>
        </aff>
        <aff id="aff43"><label>43</label><institution>Sukachev Forest Institute, Russian Academy of Sciences, Krasnoyarsk 660036, Russia</institution>
        </aff>
        <aff id="aff44"><label>44</label><institution>Institute of Remote Sensing and Digital Earth, Chinese Academy of Sciences, 100094 Beijing, China</institution>
        </aff>
        <aff id="aff45"><label>45</label><institution>Environmental Science and Analytical Chemistry, Stockholm University, Stockholm, Sweden</institution>
        </aff>
        <aff id="aff46"><label>46</label><institution>AEROCOSMOS Research Institute for Aerospace Monitoring, 105064 Moscow, Russia</institution>
        </aff>
        <aff id="aff47"><label>†</label><institution>deceased, 20 August 2015</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Hanna K. Lappalainen (hanna.k.lappalainen@helsinki.fi)</corresp></author-notes><pub-date><day>22</day><month>November</month><year>2016</year></pub-date>
      
      <volume>16</volume>
      <issue>22</issue>
      <fpage>14421</fpage><lpage>14461</lpage>
      <history>
        <date date-type="received"><day>2</day><month>March</month><year>2016</year></date>
           <date date-type="rev-request"><day>6</day><month>April</month><year>2016</year></date>
           <date date-type="rev-recd"><day>20</day><month>September</month><year>2016</year></date>
           <date date-type="accepted"><day>22</day><month>September</month><year>2016</year></date>
      </history>
      <permissions>
<license license-type="open-access">
<license-p>This work is licensed under a Creative Commons Attribution 3.0 Unported License. To view a copy of this license, visit <ext-link ext-link-type="uri" xlink:href="http://creativecommons.org/licenses/by/3.0/">http://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions><self-uri xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016.html">This article is available from https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016.pdf</self-uri>


      <abstract>
    <p>The northern Eurasian regions and Arctic Ocean will very likely
undergo substantial changes during the next decades. The Arctic–boreal
natural environments play a crucial role in the global climate via albedo
change, carbon sources and sinks as well as atmospheric aerosol production
from biogenic volatile organic compounds. Furthermore, it is expected that
global trade activities, demographic movement, and use of natural resources
will be increasing in the Arctic regions. There is a need for a novel
research approach, which not only identifies and tackles the relevant
multi-disciplinary research questions, but also is able to make a holistic
system analysis of the expected feedbacks. In this paper, we introduce the
research agenda of the Pan-Eurasian Experiment (PEEX), a multi-scale,
multi-disciplinary and international program started in 2012
(<uri>https://www.atm.helsinki.fi/peex/</uri>). PEEX sets a research approach
by which large-scale research topics are investigated from a system perspective
and which aims to fill the key gaps in our understanding of the feedbacks
and interactions between the land–atmosphere–aquatic–society continuum in
the northern Eurasian region. We introduce here the state of the art for the
key topics in the PEEX research agenda and present the future prospects of the
research, which we see relevant in this context.</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <title>Introduction</title>
      <p>The global environment is changing rapidly due to anthropogenic influences.
As a result, we are already facing several “grand challenges” in the 21st
century (e.g. Smith, 2010; Bony et al., 2015; IPCC, 2013; Randers, 2012). Two
of these challenges, climate change and air quality, are strongly influenced
by human activities and their impacts on changing atmospheric composition,
more specifically on the concentrations of greenhouse gases (GHG), reactive
trace gases, and aerosol particles. In the future, the Arctic–boreal natural
environment will play a crucial role in the global climate via albedo
changes, carbon sources and sinks as well as aerosol production from biogenic
volatile organic compounds (Arneth et al., 2010, 2014; Ballantyne et al.,
2012; Carslaw et al., 2010; M. Kulmala et al., 2014, 2015).</p>
      <p>In order to advance our understanding on interlinked grand challenges
further, we need a research approach that helps us to construct a holistic
scientific understanding of the feedbacks and interactions within the
continuum of land–atmosphere–aquatic systems and society across different
spatial and temporal scales. Therefore, we have established the Pan-Eurasian
Experiment (PEEX) program (<uri>https://www.atm.helsinki.fi/peex/</uri>),
which is a multi-scale, multi-disciplinary research initiative focusing on
understanding biosphere–ocean–cryosphere–climate–society interactions and
feedbacks (Lappalainen et al., 2014; Kulmala et al., 2015). PEEX fills some
of the most critical scientific gaps needed for a holistic understanding of
the feedback mechanisms characteristic of the northern Eurasian geographical
domain. Boreal forests and peat lands characterize the vast land areas of
northern Eurasia, with a major part of them situated inside Russian
territory. In addition to natural environments, the PEEX research program is
also interested in different human-influenced environments: from urban to
countryside, from megacities to non-populated remote areas, from areas of
dispersed settlements and sparsely-built environments to
heavily industrialized regions. Thus, the research approach covers the
Arctic and boreal regions situated in northern Eurasia, and also the marine
environments of the Arctic Ocean. PEEX operates in an integrative way using
tools from natural and social sciences such as in situ and satellite
observations, laboratory experiments, multi-scale models, and statistical
data analyses, together with socio-economic analyses. The PEEX research
agenda covers spatial scales from regional to global and temporal scales and
from seconds to decades (Kulmala et al., 2011b). The scientific results will
be used for developing new climate scenarios on global and regional scales,
for constructing reliable early warning systems, and for the mitigation and
adaptation planning of the northern societies in the most efficient way.
PEEX aims to contribute to climate policy concerning topics important to the
Northern Eurasian environment, helping societies build a sustainable
future.</p>
</sec>
<sec id="Ch1.S2">
  <title>System perspective approach</title>
      <p>Earth (system) sciences (ESS) has emerged as one of the most rapidly
developing scientific fields. The recent growth of ESS has been facilitated
by the importance of understanding the fundamental scientific processes of
climate change and air quality as well as the increasing societal impact of
this research area. The development has mainly taken place among natural
sciences, while the collaboration between natural and social sciences to
tackle climate change issues has started to emerge relatively slowly. A
multi- and cross-disciplinary approach is thus needed to advance the
solution-oriented understanding of grand challenges and to apply new
knowledge for reliable climate scenario development, mitigation, and
adaptation as well as early warning system development. In addition to
enhanced collaboration between different branches of science, there is a
need for a next generation of multi-disciplinary scientists able to connect
the scientific issues with an understanding of the societal dimensions
related to the grand challenges.</p>
      <p>Climate change can be considered as the main driving force for system
changes and their feedback dynamics, especially in the Arctic–boreal
regions. It has already been estimated that the future warming in northern
high latitudes regions will be, on average, larger than that experienced at
lower latitudes (IPCC, 2013, 2014). The climate-change-driven processes
taking place in the Arctic provide a good example of how important it is to
quantify feedback dynamics and at the same time study the specific research
topics from the land–atmosphere–hydrosphere–cryosphere–societal system
perspective. For example, the surface radiation balance regulates the
melting and freezing of the pack ice, which in turn is a key climate
regulator. Model simulations of Arctic clouds are particularly deficient,
impeding correctly simulated radiative fluxes, which are vital for the
estimation of the snow-/ice-albedo feedback (Vavrus et al., 2009). Important,
yet poorly quantified, players in the Arctic atmospheric system and climate
change are the short-lived climate forcers (SLCF), such as black carbon and
ozone. The climatic impacts of SLCFs are tightly connected with cryospheric
changes of the land system, and associated with human activities. Models
display diverse and often poor skill in simulating SLCF abundances both at
the surface and vertically through the troposphere at high latitudes
(Eckhardt et al., 2015; Emmons et al., 2015; Monks et al., 2015).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><caption><p>The thematic research areas relevant to the Northern Eurasian land
system include land topic 1 “changing ecosystem processes”, land topic 2
“ecosystem structural changes and resilience” and land topic 3 “risk areas
of permafrost thawing”. For the atmospheric system they are atmosphere topic
1 “atmospheric composition and chemistry”, atmosphere topic 2 “Urban air
quality”, are atmosphere topic 3, “atmospheric circulation and weather”,
for the aquatic system they are aquatic topic 1 “Arctic Ocean in the climate
system”, aquatic topic 2 “maritime ecosystems”, aquatic topic 3 “Lakes
and large river systems”, and for the social system they are society topic 1
“natural resources and anthropogenic activities”, society topic 2 “natural
hazards” and society topic 3 “social transformations”.</p></caption>
        <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f01.jpg"/>

      </fig>

      <p>PEEX is setting a research approach where the large-scale research questions
are studied from a system perspective, and which is also filling the key
gaps in our understanding of the feedbacks and interactions between the
land, atmosphere, aquatic, and societal systems in the northern Eurasian
region (Kulmala et al., 2015). We have structured the research agenda so
that we have highlighted three thematic research areas per system (Fig. 1).
The identification of these key thematic research areas has been based on a
bottom-up approach by researchers coming from Europe, Russia, and China,
who have participated in PEEX meetings and conferences since 2012. These
researchers first introduced a wide spectrum of specific research topics
relevant to the Northern Eurasian region, which were then evaluated and
classified. This bottom-up process led to the so-called “system-based”
structure with altogether 12 thematic research areas. This approach will
piece by piece lead into a holistic system understanding, quantifying the
dominant feedbacks and interactions between the systems, and providing an
understanding of the dynamics of Arctic–boreal biogeochemical cycles (e.g.
water, carbon, nitrogen, phosphorus, sulfur). In our approach, climate
change is the key driver in the dynamics of the land, atmosphere, aquatic
and societal systems (Kulmala et al., 2015). The large-scale thematic areas
of each system and many of the research highlight topics introduced by the
PEEX research agenda are fundamentally related to climate-change-driven
shifting GHG and SLCF formation processes and their primary and secondary
feedbacks between socioeconomic and biogeochemical systems. When studying
the Arctic–boreal feedback loops in a wider context, the PEEX agenda
addresses China as the most crucial source area of atmospheric pollution,
having a significant impact on the chemical composition of the atmosphere
over northern Eurasia (Monks et al., 2015). One must keep in mind that
solving air quality–climate interactions is also the key to practical
solutions on local air quality problems in China.</p>
      <p>In this paper, we introduce the state of the art of the selected thematic
research areas and summarize the future research needs at large scale. This
introduction acts as a “White Paper” of the PEEX research community. The
thematic research areas relevant to the land system are related to “Changing
land ecosystem processes” (Sect. 2.1.1), “Ecosystem structural changes and
resilience” (Sect. 2.1.2), and “Risk areas of permafrost thawing”
(Sect. 2.1.2). In the land system research agenda, we address the following
key issues: changing boreal forests biomass, Arctic greening, and permafrost
processes. The main research areas of the atmospheric system research are the
specific characterization of the “Atmospheric composition and chemistry”
(Sect. 2.2.1), “Urban air quality” (Sect. 2.2.2.), and the “Atmospheric
circulation and weather” (Sect. 2.2.3). In terms of atmospheric systems, we
address oxidants, trace gases, greenhouse gases, and aerosols as atmospheric
key components. We highlight that future advances in predicting urban air
quality and improving weather forecasting are strongly based in atmospheric
boundary layer dynamics research (Holtslag et al., 2013).</p>
      <p>The thematic research areas relevant to the Aquatic System are “the Arctic
Ocean in the climate system” (Sect. 2.3.1), the “Arctic maritime
ecosystems” (Sect. 2.3.2), and the “Lakes, wetland, and large-scale rivers
systems” (Sect. 2.3.3). Under these research areas, we focus on topics like
Arctic sea ice changes, marine gross primary production, and Arctic pelagic
food webs under environmental changes. Lakes and large-scale river systems
have multiple roles and aspects of the physical environments, starting from
water chemistry and algal blooms, and ending up with carbon and methane
dynamics.</p>
      <p>The thematic areas of the societal system have a number of dimensions, but in
the first phase the primary interest lies on studying the consequences of
“Land use and natural resources” (Sect. 2.4.1), on the growing number of
“Natural hazards” (Sect. 2.4.2), and on the “Social transformations”
(Sect. 2.4.3) in the northern Eurasian region. We see topics like the future
Siberian forest area together with fuel balance, forest fires effecting the
carbon and nitrogen balance, and societal dimensions related to
infrastructure degradation as the most important future research areas. In
Sect. 3, we investigate the connections and interlinks between those four
systems.</p>
<sec id="Ch1.S2.SS1">
  <title>Land system – state of the art and future research needs</title>
<sec id="Ch1.S2.SS1.SSS1">
  <title>Changing land ecosystem processes</title>
      <p>In the future, many Arctic–boreal processes will respond sensitively to
climate change, affecting ecosystem productivity and functions. These
changes may lead to unprecedented consequences, e.g. in the magnitude of
the ecosystem carbon sinks, production of aerosol precursor gases, and
surface albedo. We need first to develop methods for identifying the land
regions and processes that are especially sensitive to climate change. Only
after that are we able to analyse their responses.</p>
      <p><?xmltex \hack{\newpage}?>Boreal forests are one of the largest terrestrial biomes, and account for
around one-third of the Earth's forested area (Global Forest Watch, 2002;
<uri>http://www.globalforestwatch.org/</uri>). Nearly 70 % of all boreal
forests are located in the Siberian region. The forest biomass, soils, and
peatlands in the boreal forest zone together constitute one of the world's
largest carbon reservoirs (Bolin et al., 2000; Kasischke, 2000; Schepaschenko
et al., 2013). Due to their large forest surface areas and huge stocks of
carbon (<inline-formula><mml:math display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 320 gigatonnes of carbon; GtC), the boreal and Arctic
ecosystems are significant players in the global carbon budget. Furthermore,
permafrost, a dominant feature of Siberian landscapes, stores around
1700 GtC (Tarnocai et al., 2009). Boreal forests form the main vegetation
zone in the catchment areas of large river systems, so they are an important
part of the global water–energy–carbon feedbacks.</p>
      <p>The forest biomass forms a climate feedback via the anticipated changes in
nutrient availability and temperatures, affecting carbon sequestered
into both the aboveground biomass and soil compartment. The Siberian forests
are currently assumed to be a carbon sink, although with a large uncertainty
range of 0–1 PgC yr<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Gurney et al., 2002). However, these ecosystems
are vulnerable to global climate change in many ways, and the effects on
ecosystem properties and functioning are complicated. While higher ambient
CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations and longer growing seasons may increase plant growth
and productivity, as well as the storage of carbon to soil organic matter
(e.g. Ciais et al., 2005; Menzel et al., 2006), warming affects respiration
and ecosystem water relations in the opposite way (Bauerle et al., 2012;
Parmentier et al., 2011). Expected acceleration of fire regimes might also
substantially impact the carbon balance in Arctic and boreal regions
(Shvidenko and Schepaschenko, 2013).</p>
      <p>One example of the potentially large feedbacks is the critical role that
permafrost plays in supporting the larch forest ecotone in northern Siberia.
The boreal forests in the high latitudes of Siberia are a vast, rather
homogenous ecosystem dominated by larch. The total area of larch forests is
around 260 million ha, or almost one-third of all forests in Russia. Larch
forests survive in the semi-arid climate because of the unique symbiotic
relationship they have with permafrost. The permafrost provides enough water
to support larch domination, and the larch in turn blocks radiation,
protecting the permafrost from intensive thawing during the summer season.
The anticipated thawing of permafrost could decouple this relationship, and
may cause a strong positive feedback, intensifying the warming
substantially.</p>
      <p>The ambient temperature, radiation intensity, vegetation type, and foliar
area are the main constraints for the emission of biogenic volatile organic
compounds (BVOCs) (Laothawornkitkul et al., 2009). This makes BVOC emissions
sensitive to both climate and land use changes, via, e.g., increased
ecosystem productivity or the expansion of forests into tundra regions.
Although the inhibitory effect of CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> on the process level may be
important, Arctic greening may strongly enhance the production of BVOCs in
northern ecosystems (Arneth et al., 2007; Sun et al., 2013). Open tundra may
also act as a significant source for BVOCs, especially if the snow cover
period changes (Aaltonen et al., 2012; Faubert et al., 2012). This would lead
to negative climate feedbacks involving either aerosol–cloud or
aerosol–carbon cycle interactions (M. Kulmala et al., 2013,
2014; Paasonen et al., 2013). Linear
trends in the annual maximum normalized difference vegetation index (NDVI)
over 15 years in the northern areas of the Yamalo-Nenets Autonomous Okrug region in Russia, provide supporting evidence
of the increasing biological activity and greening, and the potential for
enhanced BVOC emissions (Fig. 2).</p>
      <p>In summary, even small proportional changes in ecosystem carbon uptake can
switch terrestrial ecosystems from a net carbon sink to a carbon source, with
consequent impacts on atmospheric CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations and global
temperatures (e.g. Bala et al., 2013; Bodman et al., 2013, Mukhortova et al.,
2015). This process has already been observed, particularly in disturbed
forests of northern Asia (Shvidenko and Schepaschenko, 2014). Currently, we
do not fully understand all the factors influencing carbon storage, or the
links between biogeochemical cycles of carbon, water, and nutrients in a
changing climate. However, the changes in these processes may be large, and
their impacts may either amplify or decrease climate change, especially in
the high northern latitudes.</p>
</sec>
<sec id="Ch1.S2.SS1.SSS2">
  <title>Ecosystem structural changes and resilience</title>
      <p>The ecosystem structural changes are tightly connected to adaptation needs,
and to the development of effective mitigation and adaptation strategies.
Predictions concerning the shifting of vegetation zones are important for
estimating the impacts of the region on future global GHG, BVOC, and aerosol
budgets. Furthermore, natural and anthropogenic stresses, such as land use
changes and biotic and abiotic disturbances, are shaping ecosystems in the
Arctic and boreal regions and have many important feedbacks to climate (see,
e.g., the review by Gauthier et al., 2015). In a warmer climate, northern
ecosystems may become susceptible to insect outbreaks, drought, devastating
forest fires, and other natural disasters. In addition, human impacts may
cause sudden or gradual changes in ecosystem functioning. The ecosystem
resilience is dependent on both the rate and magnitude of these changes.
Recent studies have concluded that current estimates very likely overestimate
the resilience of global forests and particularly boreal forests (Allen et
al., 2015). In some cases, the changes may lead to system imbalance and
possibly reaching a tipping point, after which the effects are irreversible. One of
the most relevant research topics for the land system are to determine the
structural changes and tipping points of the ecosystem changes in the
northern pan-Eurasian region.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2"><caption><p>Linear trends in the annual maximum normalized difference vegetation index
(NDVI) obtained from analysis of the MODIS 0.25 km data product for
2000–2014 over the north-western Siberia region in Russia. The trends are
given in the NDVI changes per 15 years. The yellow colours show the decreasing
NDVI, which corresponds to decreasing biological production; the blue colours
show the increasing NDVI. More detailed analysis of the trends is given in
Esau et al. (2016).</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f02.png"/>

          </fig>

      <p><?xmltex \hack{\newpage}?>Part of the expected ecosystem structural changes is related to the
lengthening of the growing season, which is taking place the Arctic–boreal
regions due to climate change. This phenomenon, called “Arctic greening”,
is due to increased plant biomass growth and advancing tree lines, turning
previously open tundra into shrubland or forest (Myneni et al., 1997; Xu et
al., 2015). However, “browning” as a proxy of decreased productivity has
also been observed during recent decades in many boreal regions (Lloyd and
Bunn, 2007), including vast territories of central Siberia, together with a
general downward trend in basal area increment after the mid-20th century
(Berner et al., 2013) and the overall decline in green from 2011 to 2014 in
Arctic regions (Phoenix and Bjerke, 2016). Current predictions on the extent
and magnitude of these processes vary significantly (Tchebakova et al., 2009;
Hickler et al., 2012; Shvidenko et al., 2013a, b).
It has been estimated that the northward shift of bioclimatic zones in
Siberia will be as large as 600 km by the end of this century (Tchebakova et
al., 2009). By taking into account that the natural migration rate of boreal
tree species cannot exceed 200–500 m per year, such a forecast implies
major vegetation changes in huge areas. In addition, we need to have a deeper
understanding of the future role of the browning process and to re-analyse
the previous model predictions of arctic greening: to what extent are they
wrong, and why (Phoenix and Bjerke, 2016)? This has important biophysical
consequences and climatic feedbacks. Changes in vegetation cover can, e.g.,
lead to albedo changes and therefore higher net absorption of radiation in
regions covered by forests compared to open vegetation (Jeong et al., 2011).
This modifies the local heat and vapour fluxes, and affects boundary layer
conditions as well as both local and larger-scale climate (Sellers et al.,
1997).</p>
      <p>Northern peatlands contain a significant part of the global soil organic
matter reservoirs (45 % of the world's soil carbon; Post et al., 1982),
and comprise one of the world's largest GHG sources (in particular CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>)
(IPCC, 2013). The hydrological conditions are a major factor in determining
the functioning of peatlands as carbon source or sink, and the carbon
balance of the vast northern peatlands is extremely sensitive to human
influence, be it through either management or climate change. For example,
thawing of permafrost peatlands in tundra regions might change tundra
ecosystems from a stable state into a dynamically changing and alternating
land–water mosaic, with dramatic impacts on their GHG production (Heikkinen
et al., 2004; Repo et al., 2009). Today, peatland management activities
range from drainage and peat harvesting to establishing crop plantations and
forests. A complete understanding of the climatic effects of peatland
management remains a challenging question (Maljanen et al., 2010).</p>
      <p>Northern ecosystems are frequently suffering from increased stresses and
deterioration. There is seldom a single and clear cause for forest dieback,
but rather the ecosystems are suffering from multiple stresses
simultaneously (e.g. Kurz et al., 2008a, b; Allen et al., 2010). This
implies that a single stress factor may not be very dramatic for the
resilience of the system, but when occurring simultaneously in combination
with others, the system may cross a threshold (i.e. tipping point), and
this may have dramatic consequences. Such perturbations and disturbances can
include not only long-term pollutant exposures, but also stochastic events such as
fires, flooding, windstorms, or insect population outbreaks, and human
activities such as deforestation or the introduction of exotic plant or
animal species. Disturbances of sufficient magnitude or duration can
profoundly affect an ecosystem, and may force an ecosystem to reach a
threshold beyond which a different regime of processes and structures
predominates. Climate warming, precipitation changes during growth periods,
and permafrost changes will substantially increase water stress, and
consequently increase the risk of mortality for trees. This process has
already clearly intensified over the entire circumpolar boreal belt (Allen
et al., 2010). As a consequence, ecosystems may turn into carbon sources
rather than sinks (Parmentier et al., 2011).</p>
      <p>In the future, boreal forest diebacks may occur due to mass infections of
invasive pathogens or herbivores, such as the autumnal moth (<italic>Epirrita autumnata</italic>) or mountain
bark beetle (<italic>Dendroctonus ponderosae</italic>), which have previously been climatically controlled by harsh
winter conditions. The growth and life cycles of herbivores or their habitat
conditions may change in such a way that the outbreak frequencies and
intensities of previously relatively harmless herbivore populations increase
(Hunter et al., 2014). At the same time as climate is changing, boreal
vegetation is also exposed to increased anthropogenic influences by
pollutant deposition and land use changes (Dentener et al., 2006; Bobbink et
al., 2010; Savva and Berninger, 2010). Large industrial complexes may lead
to local forest diebacks, as has been observed in the Kola region (e.g.
Nöjd and Kauppi, 1995; Tikkanen, 1995; Kukkola et al., 1997) and in some
regions of Siberia (Baklanov et al., 2013). Societal transformations may
lead to abandonment of agricultural land or deterioration of previously
managed forests.</p>
</sec>
<sec id="Ch1.S2.SS1.SSS3">
  <title>Risk areas of permafrost thawing</title>
      <p>The major part of the northern Eurasian geographical region is covered by
continuous permafrost. The fate of permafrost soils in high latitudes is
important for global climate with regard to all greenhouse gases. Thawing of
permafrost will also substantially alter the hydrological regimes,
particularly in northern Asia, which will lead to increasing water stress in
forests and explosive enlargement of fire extent and severity as well as post
fire successions (Shvidenko et al., 2013b).
These scenarios underline the urgent need for systematic permafrost
monitoring, together with GHG measurements in various ecosystems. The
treatment of permafrost conditions in climate models is still not fully
developed (Bala et al., 2013). The major question is, how fast will the
permafrost thaw proceed and how will it affect ecosystem processes and
ecosystem–atmosphere feedbacks, including hydrology and greenhouse gas
cycling.</p>
      <p>Understanding of the feedbacks between carbon and water cycling, ecosystem
functioning, and atmospheric composition related to permafrost thawing is
one of the important topics of the land system study (Heimann and
Reichstein, 2008; Schuur et al., 2009; Arneth et al., 2010). In
high-latitude ecosystems with large, immobile carbon pools in peat and soil,
the future net CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> exchange will depend on the extent of
near-surface permafrost thawing, local thermal and hydrological regimes, and
interactions with the nitrogen cycle (Tarnocai et al., 2009). The extra heat
produced during microbial decomposition could accelerate the rate of change
in active-layer depth, potentially triggering a sudden and rapid loss of
carbon stored in carbon-rich Siberian Pleistocene loess (yedoma) soils
(Khvorostyanov et al., 2008).</p>
      <p>The connection between the climate and the thermal conditions in the
subsurface layers (soil and bedrock) is an important aspect. The warming of
the atmosphere will inevitably result in the warming of the permafrost
layer, and is easily observed in deep borehole temperature data. However,
the changes depend on the soil and rock type as well as on the pore filling
fluids. As long as the pore fill is still ice, the climatic changes are
reflected mainly in the thickness of the active layer, and in slow diffusive
temperature changes of the permafrost layer itself. In areas where the
ground is dominated by low ground temperatures and thick layers of porous
soil types (e.g. sand, silt, peat), the latent heat of the pore-filling ice
will efficiently “buffer” and retard the final thawing. This is one of the
reasons why relatively old permafrost exists at shallow depths in
high-porosity soils. On the other hand, quite different conditions prevail
in low-porosity areas, e.g. in crystalline rock areas.</p>
      <p>The permafrost dynamics affect methane fluxes in many ways. Hot spots such as
mud ponds emitting large amounts of CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> may form when permafrost mires
thaw. In contrast, lakes have occasionally disappeared as a result of the
intensification of soil water percolation (Smith et al., 2005). The rapid
loss of summer ice, together with increasing temperature and melting ice
deposits, results in coastal erosion, physical destruction of the surface in
hilly areas, activation of old carbon and elevated CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>
emissions from sea-bottom sediments (Vonk et al., 2012). High methane
emissions have been observed from the East Siberian Arctic
Shelf
(Shakhova et al., 2010).</p>
</sec>
</sec>
<sec id="Ch1.S2.SS2">
  <title>Atmospheric system – state-of-the-art and future research needs</title>
<sec id="Ch1.S2.SS2.SSS1">
  <title>Atmospheric composition and chemistry</title>
      <p>Atmospheric composition plays a central role in the northern Eurasian climate
system. In addition to greenhouse gases and their biogeochemical cycling
discussed in more detail in Sect. 3.2, key compounds in this regard are ozone
and other oxidants, carbon monoxide, numerous organic compounds as well as
different types of aerosols and their precursors (SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> will be discussed
in Sect. 3.5). At the moment, there is a serious gap in our knowledge on
tropospheric composition and chemistry over Russia and China, with
particularly few observation programs being active over Siberia (Crutzen et
al., 1998; Ramonet et al., 2002; Paris et al., 2008; Kozlova et al., 2008;
Uttal et al., 2015, Paris et al., 2010a, b; Sasakawa et al., 2010; Chi et
al., 2013; Saeki et al., 2013; Ding et al., 2013a, b; Berchet et al., 2015;
Heimann et al., 2014).</p>
      <p>There is thus an urgent need for harmonized, coordinated and comprehensive
greenhouse gas, trace gas, and aerosol in situ observations over northern
Eurasia and China (long-term transport aspect) comparable to European and
circumpolar data observations. In Fig. 3 we illustrate the geographical
coverage of the ground stations that will be part of the coordinated,
coherent, and hierarchic observation network in the northern Eurasian region
and in China.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3"><caption><p>Map showing the existing ACTRIS (aerosols, clouds, and trace gases research infrastructure network)
and ICOS (Integrated Carbon Observations System) stations in Europe (blue), stations making atmospheric and/or
ecosystem measurements in Russia (red), INTERACT (International Network for Terrestrial Research and Monitoring in the Arctic)
stations in Russia (light
blue), and China Flux stations in China (yellow). However, all of these
stations need certain upgrades.</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f03.png"/>

          </fig>

</sec>
<sec id="Ch1.S2.SS2.SSSx1" specific-use="unnumbered">
  <title>Main pollutants</title>
      <p>Little is known about whether and how the regional ozone budget in northern
pan-Eurasia differs from that in the rest of the Northern Hemisphere (Ding et
al., 2008; Berchet et al., 2013). Arctic tropospheric ozone is significantly
influenced by long-range import of ozone and precursors from mid-latitude
sources as well as by boreal wildfires (Ding et al., 2009; Wespes et al.,
2012; Paris et al., 2010b; Vivchar et al., 2009). The role of biomass burning
emissions in the ozone budget in high latitudes remains controversial. While
most studies suggest significant ozone production in boreal smoke plumes
(e.g. Paris et al., 2010b; Parrington et al., 2013; Jolleys et al., 2015),
some observations from individual plumes suggest that O<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:math></inline-formula> production in
boreal wildfire plumes may be weaker, or even turn into net destruction,
compared to fire plumes at lower latitudes (Liang et al., 2011; Jaffe and
Wigder, 2012). Recent modelling work has suggested that boreal fires produce
a substantial large-scale enhancement in summertime ozone at high latitudes,
which appears to be highly sensitive to differences in partitioning of
reactive nitrogen among models (Arnold et al., 2015). The boreal biosphere,
on the other hand, provides a large sink for tropospheric ozone (Paris et
al., 2010b; Parrington et al., 2013). Given their importance for air quality
and global greenhouse gas budget, more atmospheric measurements of O<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:math></inline-formula>,
its precursors and other pollutants over Siberia are needed (see Elansky et
al., 2012). This is particularly the case in light of increasing local Arctic
sources of ozone precursors (NO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mi>x</mml:mi></mml:msub></mml:math></inline-formula>, VOCs, volatile organic compounds) from, e.g., shipping and fossil fuel
resource extraction (Roiger et al., 2015). Such data sets would be
particularly useful for the evaluation of atmospheric chemistry models and
satellite products.</p>
      <p><?xmltex \hack{\newpage}?>The changes in the abundance of anthropogenic aerosols and their precursors
in northern Eurasia have been extensive during the last decades (Granier et
al., 2011), and this has almost
certainly contributed to the very different regional warming patterns over
these areas (e.g. Shindell and Faluvegi, 2009). The main anthropogenic
aerosols in this context are primary carbonaceous particles, consisting of
organic and black carbon as well as secondary sulfate particles produced
during the atmospheric transport of sulfur dioxide. These species, as well as
nitrate, have also been found to dominate the aerosol composition at the
Zotino Tall Tower Observation Facility (ZOTTO) site in
central Siberia (Mikhailov et al., 2015a, b; Ryshkevich et al., 2015). These
aerosols cause large perturbations to the regional radiation budget downwind
of major source areas in the northern Eurasian region, and the resulting
changes in cloud properties and atmospheric circulation patterns may be
important even far away from these sources (Koch and Del Genio, 2010; Persad
et al., 2012). In the snow-covered parts of Eurasia, long-range transported
aerosols containing black carbon and deposited onto snow tend to enhance the
spring and early-summer melting of the snow, with concomitant warming over
this region (Flanner et al., 2009; Goldenson et al., 2012; Meinander et al.,
2013; Atlaskina et al., 2015).</p>
      <p>The most important natural aerosol type over large parts of Eurasia is
secondary organic aerosol originating from atmospheric oxidation of BVOCs
emitted by boreal forests and possibly other ecosystems. Studies conducted in
the Scandinavian part of the boreal zone indicate that new particle formation
associated with BVOC emissions is the dominant source of aerosol particles
and cloud condensation nuclei during summer time (Mäkelä et al.,
1997; Kulmala et al., 2001; Tunved et al., 2006; Asmi et al., 2011; Hirsikko
et al., 2011). The production of secondary organic aerosols associated with
BVOC emissions has been estimated to induce large direct and indirect
radiative effects over the boreal forest zone (Spracklen et al., 2008; Tunved
et al., 2006; Lihavainen et al., 2009, 2015; Scott et al., 2014). The few
continuous measurement data sets from Siberia suggest similarities in the
frequency and seasonal pattern of new particle formation events between
Siberia and Nordic stations (Dal Maso et al., 2007; Arshinov et al., 2012;
Asmi et al., 2016). Measurements conducted at the ZOTTO site in central
Siberia have shown that biogenic secondary organic aerosols reach high
concentrations in summer and dominate the aerosol composition during this
season (Mikhailov et al., 2015a, b; Ryshkevich et al., 2015). At this site,
however, new particle formation events are seen much less frequently than at
the Nordic stations (Heintzenberg et al., 2011). At present, relatively
little is known about the overall contribution of biogenic emissions to
aerosol number or mass concentrations, or to the cloud condensation nuclei
budget, in northern Eurasia.</p>
      <p>Other important natural aerosol types in northern Eurasia are sea spray,
mineral dust, and primary biogenic aerosol particles. Sea spray aerosol makes
an important contribution to the atmospheric aerosol over the Arctic Ocean
and its coastal areas (Zábori et al., 2012, 2013), and influences cloud
properties over these regions (Tjernström et al., 2014). The climatic
effects of sea spray are expected to change in the future as a result of
changes in the sea ice cover and ocean temperatures (Struthers et al., 2011).
Mineral dust particles affect regional climate and air quality over large
regions in Asia, especially during periods of high winds and moderate
precipitation. Mineral dust and primary biological aerosol particles (PBAPs)
particles are also effective ice nuclei (Hoose and Möhler, 2012), and
have the potential to influence radiative and other properties of mixed-phase
cold clouds in the Arctic–boreal regions. Over northern Eurasia, PBAPs
typically contribute more than 20 % of PM<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn>2.5</mml:mn></mml:msub></mml:math></inline-formula> (fine particulate
matter with a diameter of 2.5 <inline-formula><mml:math display="inline"><mml:mi mathvariant="normal">µ</mml:mi></mml:math></inline-formula>m or less)
organic aerosol mass concentrations (Heald and Spracklen, 2009) and 25 %
of supermicron aerosol number concentrations (Spracklen and Heald, 2014). Ice
nucleation, in general, is one of the key microphysical processes in the
atmosphere that remain ill understood. However, a novel theoretical approach
(Laaksonen, 2015; Laaksonen and Malila, 2016) has been shown to be superior
to older theories in the case of water nucleation on solid surfaces, and it
may open a completely new avenue in the studies of atmospheric ice formation.</p>
      <p>Satellites provide information about spatial distributions of the
column-integrated concentrations of aerosols (Andreae, 2009) and various
trace gases including ozone and its precursors (Burrows et al., 2011). These
atmospheric constituents are generally retrieved using passive instruments,
which have good sensitivity near the surface. However, retrieving information
on the near-surface concentrations of pollutants requires assumptions on
their vertical distributions. For instance, the retrieval of tropospheric
ozone from satellite observations requires corrections for the high
concentrations in the upper troposphere and lower stratosphere. For aerosols,
which can only be retrieved in clear-sky conditions, the situation may be
complicated when disconnected layers are present with different types of
aerosols. A solution may be the retrieval of aerosol vertical variation or
the height of the aerosol layer using, e.g., active instruments (lidars), or
retrieval using spectrally resolved observations in the oxygen A-band (e.g.
Hollstein and Fisher, 2014), or instruments providing multiple viewing
algorithms such as MISR (Nelson et al., 2013) or AATSR (Virtanen et al.,
2014). Another complication for aerosols may be the vertical variation of the
physical and chemical properties, which renders it difficult to obtain
closure between column and ground-based in situ measurements (Zieger et al.,
2015, and references cited therein). Nevertheless, good progress has been
made in aerosol retrieval, and column-integrated aerosol measurements
(aerosol optical depth, AOD) from satellites and ground-based observations
compare favourably (e.g. de Leeuw et al., 2015; Kolmonen et al., 2015).
Measurements of trace gases from space using wavelengths in the thermal
infrared suffer from low sensitivity in the lower troposphere (Pommier et
al., 2010). All these factors may render the comparison against local
ground-based in situ observations difficult, although a possible way out
could be the use of chemical transport models constrained by the satellite
column measurements (e.g. de Laat et al., 2009; Stavrakou et al., 2012,
2014), possibly together with sub-orbital airborne measurements of relevant
species. Satellite-measured AOD has been successfully applied to obtain
information on ground-based aerosol mass concentrations (PM<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn>2.5</mml:mn></mml:msub></mml:math></inline-formula>) (Xu et
al., 2015; van Donkelaar et al., 2015). In addition, the use of multiple
satellite instruments, with different characteristics, is proposed to obtain
more accurate information on the transport of aerosols and trace gases and
their vertical distribution (e.g. Naeger et al., 2016). Recently, a technique
has been demonstrated that makes it possible to derive CCN (cloud
condensation nuclei) concentrations at cloud base using remote sensing of
cloud properties (Rosenfeld et al., 2016).</p>
</sec>
<sec id="Ch1.S2.SS2.SSSx2" specific-use="unnumbered">
  <title>Large-scale pollutant transport and sources</title>
      <p>Of particular interest is the pollutant transport to Arctic areas, where
they can influence the radiation budget and climate in various ways (Stohl,
2006; Warneke et al., 2009; Meinander et al., 2013; Eckhardt et al., 2015).
Model simulations suggest that European emissions dominate Arctic pollutant
burdens near the surface, with sources from North America and Asia more
important in the mid- and upper troposphere (Monks et al., 2015). The impact
and influence of China and its polluted megacities on Arctic and boreal
areas is a topic of key importance, given recent and rapid Chinese
industrialization. Inter-continental pollution transport has also become of
increased concern due to its potential influence on regional air quality.
The pollutant export from North America and Asia has been characterized by
intensive field campaigns (Fehsenfeld et al., 2006; Singh et al., 2006), but
long-term research approaches are lacking.</p>
      <p>Emissions from forest fires (van der Werf et al., 2006; Sofiev et al., 2013)
and from agricultural fires in southern Siberia, Kazakhstan, and Ukraine
(Korontzi et al., 2006) in spring and summer are large sources of trace
gases such as carbon monoxide (Nédélec et al., 2005; Konovalov et
al., 2014) as well as aerosol particles (Konovalov et al., 2015). Aerosols
emitted by forest fires are of particular interest, since the strength of
this source type depends on both climate change and human behaviour (Pechony
and Shindell, 2010), and since particles emitted by these fires have
potentially large radiative effects over Eurasia (Randerson et al., 2006).
We need comprehensive top-down emissions estimates, using inverse modelling
constrained by satellite observations, in order to provide quantitative
information on the source strength of aerosols and trace gases emitted by
open fires.</p>
      <p>Air pollution in monsoon Asia has two main characteristics. First, the total
pollutant emission rate from fossil fuel combustion sources is very high,
leading to a high concentration of primary and secondary pollutants in Asia,
especially in eastern China and northern India. Observations show that Asia
is the only region where the concentrations of key pollutants, such as
nitrogen oxides (Richter et al., 2005; Mijling et al., 2013) and their
end-product ozone (Ding et al., 2008; Wang et al., 2009; Verstraeten et al.,
2015), are still increasing. Second, in addition to the anthropogenic fossil
fuel combustion pollutants, monsoon Asia is also influenced by intensive
pollution from seasonal biomass burning and dust storms. For example,
intensive forest burning activities often take place in south Asia during
spring and in Siberia during summer, whereas intensive anthropogenic burning
of agricultural straw takes place in the north and east China plains. Dust
storms frequently occur in the Taklimakan and Gobi deserts in north-west
China, and this dust is often transported over eastern China, southern China,
the Pacific Ocean and even the entire globe (Nie et al., 2014). After mixing
with other anthropogenic pollutants, biomass burning and mineral dust
aerosols have been found to cause complex interactions in the climate system
(Ding et al., 2013a; Nie et al., 2014).</p>
</sec>
<sec id="Ch1.S2.SS2.SSS2">
  <title>Urban air quality</title>
      <p>The northern Eurasian urban environments are characterized by cities with
strong anthropogenic emissions from local industry, traffic, and housing in
Russia and China, and by megacity regions with alarming air quality levels
like those of Moscow and Beijing. Bad air quality has serious health effects
and damages ecosystems. In Beijing, for example, concentrations of
atmospheric fine particles have been found to be more than 10 times higher
than the safe level recommended by the World Health Organization (WHO)
(Zheng et al., 2015). Furthermore, atmospheric pollutants and oxidants play
a central role in climate change dynamics via their direct and indirect
effects on global albedo and radiative transfer. A deeper understanding of
the unpredicted chemical reactions between pollutants and identification of
the most relevant feedbacks between air quality and climate at northern high
latitudes and in China is the most urgent task helping us to find practical
solutions for more healthy air (Kulmala, 2015).</p>
      <p>In Siberian cities, the air quality is strongly linked to climatic conditions
typical for Siberia. Stable atmospheric stratification and temperature
inversions are predominant weather patterns for more than half of the year.
This contributes to the accumulation of different pollutants in the lowest
layers of the atmosphere, thus increasing their impact on ecosystems and
humans. In addition to the severe climatic conditions, human impacts on the
environment in industrial areas and large cities continue to increase. In
winter time, shallow and stably stratified planetary boundary layers (PBL)
typical for northern Scandinavia and Siberia are especially sensitive to even
weak impacts and, therefore, deserve particular attention, especially in the
conditions of environmental and climate change (Zilitinkevich and Esau, 2009;
Esau et al., 2012; Davy and Esau, 2014; Wolf et al., 2014; Wolf and Esau,
2014). Unstably stratified PBLs interact with the free atmosphere mainly
through turbulent ventilation at the PBL upper boundary (Zilitinkevich,
2012). This mechanism, still insufficiently understood and poorly modelled,
controls the development of convective clouds, as well as dispersion and
deposition of aerosols and gases, which are essential features of heat waves
and other extreme weather events.</p>
      <p>The worst air pollution episodes are usually associated with stagnant weather
conditions with a shallow PBL, which promotes the accumulation of intensively
emitted pollutants near the surface. The lower PBL is also influenced by the
heavy pollution itself through its direct or indirect effects on solar
radiation and hence the surface sensible heat flux (e.g. Ding et al.,
2013b). The boundary layer–air pollution feedback will decrease the height
of the PBL and result in an even more polluted PBL (Ding et al., 2013b; Wang
et al., 2014; Petäjä et al., 2016). Therefore, considering the
complex land-surface types (city clusters surrounded by agricultural areas)
and pollution sources, improving our understanding of the associated
feedbacks is very important for forecasting extreme air pollution episodes
and for long-term policymaking. In order to understand this topic, more
vertical measurements using aircraft, balloons, and remote sensing
techniques, as well as advanced numerical models including all relevant
processes and their couplings, are needed.</p>
      <p>Planetary boundary layers are subject to diurnal variations, absorb surface
emissions, control microclimate, air pollution, extreme colds, and heat
waves, and are sensitive to human impacts. Very stable stratification in the
atmosphere above the PBL prevents the compounds produced by the surface
fluxes or surface emissions from efficiently penetrating from the PBL into
the free atmosphere. This means that the PBL height and turbulent fluxes
through the PBL upper boundary control local features of climate and extreme
weather events, such as the heat waves associated with convection, or the
strongly stable stratification events triggering the air pollution
(Zilitinkevich et al., 2015). This concept (equally relevant to the
hydrosphere) illustrates the importance of modelling and monitoring the
atmospheric PBL height, which varies from dozens to thousands of metres
(Zilitinkevich, 1991; Zilitinkevich et al., 2007; Zilitinkevich and Esau,
2009). To carry out a comprehensive inventory of the PBL height over
northern Eurasia is urgently needed.</p>
</sec>
<sec id="Ch1.S2.SS2.SSS3">
  <title>Atmospheric circulation and weather</title>
      <p>The ongoing environmental change and its amplification in northern Eurasia
pose special challenges to the prediction of weather-related hazards, and
also to long-term impacts. A key question is how the atmospheric dynamics
(synoptic scale weather, boundary layer characteristics) will change in
Arctic and boreal regions. The recent changes in the Arctic sea ice have
been much more rapid than models and scientists anticipated about 10 years
ago. The role of the Arctic Ocean in the climate system and sea ice changes
have affected mid-latitude weather and climate, with central and eastern
Eurasia among the regions with strongest effects (Vihma, 2014; Overland et
al., 2015) (see Sect. 2.3.1).</p>
</sec>
<sec id="Ch1.S2.SS2.SSSx3" specific-use="unnumbered">
  <title>Atmospheric dynamics</title>
      <p>The reliability of weather forecasts, and the extension of the time range of
useful forecasts is needed for minimizing economic and human losses from
extreme weather and extreme weather-related natural hazards. In Europe, this
range is currently on average about 8–9 days (Bauer et al., 2015), which
allows reliable early warnings to be issued for weather-related hazards,
such as windstorms and extreme precipitation events with flash floods. The
time range of useful forecasts has typically increased by a day per decade
over the past three decades (Uppala et al., 2005). In the northern Eurasian
region, improved predictions can be used, for instance, for better
prediction of thermal comfort conditions in northern cities (Konstantinov
et al., 2014). A strong urban heat island effect has already been observed in
urban areas of the Arctic with complex spatial and temporal structures
(Konstantinov et al., 2015).</p>
      <p>Understanding of PBL processes is particularly
important for improving the weather predictions. The representation of
boundary layer clouds, and their further coupling to convection in stable
conditions is not currently well understood. Quantification of the behaviour
of the PBL over the northern Eurasian region is needed in analyses of
spatial and temporal distribution of the surface fluxes, in predictions of
microclimate and extreme weather events, and in modelling clouds and air
quality.</p>
      <p>The development of diagnostic and modelling methods for aero-electric
structures is important for a study of both convective and electric
processes in the lower troposphere (Shatalina et al., 2005, 2007).
Convection in the PBL leads to the formation of aero-electric structures,
manifested in ground-based measurements as short-period electric-field
pulsations with periods from several seconds to several hundreds of seconds
(Anisimov et al., 1999, 2002). The sizes of such structures are determined
by the characteristic variation scales of aerodynamic and electrodynamics
parameters of the atmosphere, including the PBL and surface-layer height as
well as by the inhomogeneities in the ground (water) surface. Formed as a
result of convective processes and the capture of positive and negative
charged particles (both ions and aerosols) by convective elements (cells),
aero-electric structures move with the airflow along the Earth's surface.
The further evolution of convective cells results, in particular, in cloud
formation.</p>
</sec>
<sec id="Ch1.S2.SS2.SSSx4" specific-use="unnumbered">
  <title>Global electric circuit</title>
      <p>The global electric circuit (GEC) is an important factor connecting the solar
activity and upper atmospheric processes with the Earth's environment,
including the biosphere and climate (Dolezalek et al., 1976; Singh et al.,
2004). Thunderstorm activity maintains this circuit, whose appearance is
dependent on atmospheric conductance variations over a wide altitude range.
The anthropogenic impact on the GEC through aviation, forest fires, and
electromagnetic pollution has been noted with great concern, and the
importance of lightning activity in climate processes has been recognized.
The GEC forms for two reasons: the continuous operation of ionization
sources, which provides an exponential growth of the conductivity in the
lower atmosphere, and the continuous operation of thunderstorm generators,
providing a high rate of electrical energy generation and dissipation in the
troposphere. Therefore, the GEC is influenced by both geophysical and
meteorological factors, and can serve as a convenient framework for the
analysis of possible inter-connections between atmospheric electrical
phenomena and climate processes. Further exploration of the GEC as part of
the climate system studies, specifically its effect on the balance between
the Earth's ionosphere and global circuit, requires accurate modelling of the
GEC stationary state and its dynamics (Mareev, 2010). Special attention
should be paid to the observations and modelling of generators
(thunderstorms, electrified shower clouds, mesoscale convective systems) in
the global circuit.</p>
</sec>
</sec>
<sec id="Ch1.S2.SS3">
  <title>Aquatic system – state of the art and future research needs</title>
<sec id="Ch1.S2.SS3.SSS1">
  <title>The Arctic Ocean in the climate system</title>
      <p>The essential processes related to the interaction between the Arctic ocean
and other components of the Earth system include the air–sea exchange of
momentum, heat, and matter (e.g. moisture, aerosol, trace gases, CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>,
and CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>) as well as the dynamics and thermodynamics of sea ice. The most
dramatic change in the Arctic Ocean has been the rapid decline of the sea
ice cover. Since the early the 1980s, the Arctic sea ice extent has
decreased by roughly 50 % in summer and autumn (Cavalieri and Parkinson,
2012), while the winter sea ice thickness in the central Arctic has
decreased by approximately 50 % (Kwok and Rothrock, 2009). Arctic sea ice
changes have serious teleconnections. Despite the warming climate,
wintertime cold spells in East Asia have become more frequent, stronger and
longer lasting in this century compared with the 1990s (Kim et al., 2014).
It also seems that the strong decline of the Arctic sea ice has favoured
atmospheric pressure patterns that generate cold-air outbreaks from the
Arctic to East Asia (Mori et al., 2014; Kug et al., 2015; Overland et al.,
2015). The reasons for and the future evolution of the sea ice decline, as
well as its effects on the ocean, atmosphere and surrounding continents are
among the current topics of study on the Arctic climate system. Other major
issues include the role of the ocean in the Arctic amplification of climate
change, greenhouse gas exchange between the ocean, sea ice, and atmosphere as well as aerosol budgets in the marine Arctic (Smedsrud et al., 2013). The key
question here is related to the changes of sea ice extent and thickness, and
to the terrestrial snow cover change.</p>
      <p>Many of the processes considered to be responsible for the Arctic
amplification of climate warming are related to the ocean and sea ice
(Döscher et al., 2014). Among these, the snow-/ice-albedo feedback has
received the most attention (e.g. Flanner et al., 2011). This feedback is
strongest when sea ice is replaced by open water, but it starts to play a
significant role already in spring when the snowmelt on top of sea ice
begins. This is because of the large albedo difference between dry snow
(albedo about 0.85) and wet, melting, bare ice (albedo about 0.40). More work
is needed to understand quantitatively the reduction of snow/ice albedo
during the melting season, including the effects of melt ponds and pollutants
in the snow. Other amplification mechanisms related to the ocean include
increased heat transports from lower latitudes to the Arctic (Polyakov et
al., 2010; Döscher et al., 2014) and fall–winter energy loss from the
ocean (Screen and Simmonds, 2010). Furthermore, the melting of sea ice
strongly affects evaporation, and hence the water vapour and cloud radiative
feedbacks (Sedlar et al., 2011), and the PBL thickness, which controls the
sensitivity of the air temperature to heat input into the PBL (Esau et al.,
2012; Davy and Esau, 2016). The relative importance of the mechanisms
affecting the Arctic amplification of climate warming are not yet well known
(see also Pithan and Mauritsen, 2014; Cohen et al., 2014).</p>
      <p>The rapid decline of the Arctic sea ice cover has tremendous effects on
navigation and exploration of natural resources. To be able to predict the
future evolution of the sea ice cover, the first priority is to better
understand the reasons, including the role of black carbon (see Bond et al.,
2013), behind the past and ongoing sea ice evolution. Several processes have
contributed to the decline of Arctic sea ice cover, but the role of these
processes needs better quantification (Smedsrud et al., 2013; Vihma et al.,
2014). Further studies are needed on the impacts of changes in cloud cover
and radiative forcing (Kay et al., 2008), atmospheric heat transport (Kapsch
et al., 2013) and oceanic heat transport (Döscher et al., 2014). In
addition, as the ice thickness has decreased, the sea ice cover becomes
increasingly sensitive to the ice-albedo feedback (Perovich et al., 2008).
Other issues calling for more attention include the reasons for the earlier
onset of the spring melt (Maksimovich and Vihma, 2012), changes in the phase
of precipitation (Screen and Simmonds, 2012), and large-scale interaction
between the sea ice extent, sea surface temperature distribution, and
atmospheric dynamics (cyclogenesis, cyclolysis, and cyclone tracks) as
discussed, e.g. by Outten et al. (2013).</p>
      <p>In addition to thermodynamic processes, another factor affecting the sea ice
cover in the Arctic is the drift of sea ice. The momentum flux from the
atmosphere to the ice is the main driver of sea-ice drift, which is poorly
represented in climate models (Rampal et al., 2011). This currently hinders
a realistic representation of sea-ice drift patterns in large-scale climate
models. Furthermore, the progressively thinning ice pack is becoming
increasingly sensitive to wind forcing (Vihma et al., 2012). In the future,
research has to address the main processes that determine the momentum
transfer from the atmosphere to the sea ice, including the effects of
atmospheric stratification and sea ice roughness.</p>
      <p>To understand better the links between the Arctic Ocean and terrestrial
Eurasia, there is a particular need to study the effects of Arctic sea ice
decline on Eurasian weather and climate (Sect. 2.2.3) Another poorly
studied problem related to the Arctic Ocean is the role of sea ice as a
source of aerosol precursors, and in the gas exchange between the ocean and
atmosphere (Parmentier et al., 2013). Preliminary results of field studies
at the drifting stations North Pole 35 and 36 (Makshtas et al., 2011) showed
that the shrinking sea ice cover could be the reason for increasing CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
uptake from the atmosphere over the annual cycle, and for the growth of the
seasonal amplitude of CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations in the Arctic.</p>
      <p>Climate models project that air temperatures and precipitation will increase
over the Arctic Ocean, and that this may have important effects on the
structure of sea ice. Increased snow load on a thinner ice may in the future
cause flooding of seawater on ice in the Arctic, which results in the
formation of snow ice. Increased snowmelt and rain, on the other hand,
results in increased percolation of water to the snow–ice interface, where
it re-freezes, forming super-imposed ice (Cheng et al., 2008). Snow ice and
super-imposed ice have granular structures, and differ thermodynamically and
mechanically from the sea ice that currently prevails in the Arctic.</p>
      <p>The changes in the Arctic Ocean have opened some, albeit limited,
possibilities for seasonal prediction. These are mostly related to the large
heat capacity of the ocean: if there is little sea ice in the late summer and
early autumn, this tends to cause large heat and moisture fluxes to the
atmosphere, favouring warm, cloudy weather in late autumn and early winter
(Liu et al., 2011; Stroeve et al., 2012). On the other hand, the reduction of
the sea ice thickness may decrease the possibilities for seasonal forecasting
of ice conditions in the most favourable navigation season in late
summer–early autumn. This is because a thin ice is very sensitive to
unpredictable anomalies in the atmospheric forcing. For example, in
August 2012 a single storm caused a reduction of the sea ice extent by
approximately 1 million km<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>. The reduced sea ice extent in the winter
months has significant impacts on convective clouds. Observations revealed a
gradually increasing frequency of the convective cloud fields over Norwegian
and Barents seas (Chernokulsky and Mokhov, 2012; Esau and Chernokulsky,
2015). The unusually strong atmospheric convection and weaker virtual
potential temperature inversions create favourable conditions for the extreme
Arctic cold outbreaks and meso-scale cyclones known as polar lows (Kolstad et
al., 2009).</p>
      <p>It is vital to enhance routine observations, data assimilation techniques
and prediction models in order to properly monitor the physical state of the
environment. Longer-term impacts of the reduced ice cover are largely
unknown, because the scientific community has had only little time to create
new knowledge on essential climate variables across the domain (see Sect. 2.3.1). To improve preparedness, new observational evidence is therefore
needed to reduce uncertainties in the system dynamics both on short and
longer time-scales.</p>
</sec>
<sec id="Ch1.S2.SS3.SSS2">
  <title>Arctic marine ecosystem</title>
      <p>The ice cover of the Arctic Ocean is undergoing fast changes, including a
decline of summer ice extent and ice thickness (see Sect. 2.3.1). This results in
a significant increase of the ice-free sea surface in the vegetation season,
and an increase in the duration of the growing season itself. The key topic
of future research is the joint effect of Arctic warming, ocean freshening,
pollution load, and acidification on the Arctic marine ecosystem, primary
production, and carbon cycle.</p>
      <p>New ice-free areas of the Arctic Ocean could result in a pronounced growth
of the annual gross primary production (GPP), increased phytoplankton
biomass, and a loss of ice-rich algae communities associated with the low ice
sheet surface (Bluhm et al., 2011). Progressive increase of oil and natural
gas drilling and transportation over the shelf areas will be escalating the
environmental changes of the Arctic marine ecosystems. Furthermore, there is
a risk of irreversible changes in marine Arctic productivity and key
biogeochemical cycles, and the potential for CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> absorption by marine
ecosystem. Processes involving the Arctic may also affect adjacent boreal
areas.</p>
      <p>We do not know how the climatically induced increase in GPP and
phytoplankton biomass will influence the productivity of higher trophic
levels of the Arctic ecosystem. In typical Arctic ecosystems, the most
important consumers are large-sized herbivorous copepods, which have life
cycles synchronized with the temperature as well as the seasonal algae
dynamics (Kosobokova, 2012). Another important consumer community are the
small-sized herbivorous copepods, which are important especially in shelf
ecosystems. An increase in the phytoplankton production in fall, together
with an increase in the sea temperature, may influence the populations of
small-sized copepods, and increase their role in mass and energy flow in the
ecosystems. Our current understanding of the role of small copepods in the
Arctic ecosystems is limited (Arashkevich et al., 2010). An increase in
surface water temperature may “open the Arctic doors” for new species, and
change the Arctic pelagic food webs, energy flows, and biodiversity.</p>
      <p>Increases in the Arctic sea temperature may lead to populations from
neighbouring regions penetrating the Arctic ecosystem, changing the structure
and functioning of native ecosystems. For example, a 1.5 <inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C water
temperature increase in the Bering Sea during the mid-1970s allowed the
Alaskan Pollock to penetrate the Arctic ecosystem, and occupy a place as a
keystone species for several years, supporting one of the world's largest
regional fish harvests (Shuntov et al., 2007). The Bering Sea ecosystem is
very rich compared to the Arctic ecosystems. Currently, we are not aware of
food sources sufficient for supporting massive invader populations even in
case of climate-induced changes in ecosystems. However, the appearance of
aggressive new species even in low numbers may dramatically impact the
sensitive Arctic ecosystems and have effects on the future regulation of
international fisheries in the Arctic.</p>
      <p>We have only recently begun to understand the processes that regulate
freshwater–marine ecosystem interactions in estuarine zones (Flint, 2010).
The mechanisms determining the impact of riverine waters over the Arctic
shelves and the central deep basin, and their dependence on specific
climatic forces, are still poorly understood. In order to determine the
impact of riverine waters, it is important to locate new flagship stations
or permanent observation points in the estuaries of large Siberian rivers.
The changing riverine discharge to the Arctic shelves may amplify the impact
of climate warming on the Arctic marine ecosystems. Degradation of
permafrost, soil erosion, changes in snow cover and summer precipitation may
all lead to changes in flood timing, and also to an increase in the amount
of fresh water and materials of terrestrial origin, including organic matter
and nutrients, annually delivered to the Arctic shelves, and further to the
Arctic basin (Gustafsson et al., 2011). Human-driven land use changes to
drainage basins and associated river systems have the potential to increase
the speed of delivery of pollutants to the Arctic sea.</p>
</sec>
<sec id="Ch1.S2.SS3.SSS3">
  <title>Lakes, wetlands, and large-scale river systems</title>
      <p>In the last decade, the combined effects of air pollution and climate warming
on fresh-water systems have received increasing attention (Skjelkvåle and
Wright, 1998; Schindler, 2001; Alcamo et al., 2002;
Sanderson et al., 2006; Feuchtmayr et al., 2009; Sereda et al., 2011). It is
important to understand the future role of Arctic–boreal lakes, wetlands,
and large river systems, including thermokarst lakes and running waters of
all size, in biogeochemical cycles, and how these changes affect livelihoods,
agriculture, forestry, and industry. The water chemistry of lakes without any
direct pollution sources in the catchment area can be expected to reflect
regional characteristics of water chemistry, as well as global anthropogenic
processes, such as climate change and long-range air pollution (Müller et
al., 1998; Moiseenko et al., 2001; Battarbee et al., 2005). The current
ground-based streamflow-gauging network over the northern Eurasian region
does not provide adequate spatial coverage for many scientific and water
management applications, including the verification of the land-surface
run-off contribution to the recipients of intra-continental run-off. Special
field laboratories, with joint observation and modelling capabilities in
hydrometeorology, sedimentology, and geochemistry are needed to understand
the spreading of tracers and pollutants as part of current and future global
environmental fluxes.</p>
      <p>The gradient in water chemistry from the tundra to the steppe zones in
Siberia can provide insight into the potential effects of climate change on
water chemistry. In the last century, long-range trans-boundary air pollution
led to changes in the geochemical cycles of sulfur, nitrogen, metals, and
other compounds in many parts of the world (Schlesinger, 1997; Vitousek et
al., 1997a, b; Kvaeven et al., 2001; Skjelkvåle et al., 2001).
Environmental pollution problems also include the waterborne spreading of
nutrients and pesticides from local agricultural areas, heavy metals often
originating from mining areas, and other elements and chemicals, such as
persistent organic pollutants from urban and industrial areas. Shifts in
downstream loads cause changes in river and delta dynamics. One example of
important study area is the Selenga River basin, which is located in the
centre of Eurasia, extends from northern Mongolia into southern Siberia
(Russia), and has its outlet at Lake Baikal. The Selenga River basin and Lake
Baikal are located in the upstream part of the Yenisei River system, which
discharges into the Arctic Ocean. Lake Baikal has the largest lake volume in
the world at about 23 000 km<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msup></mml:math></inline-formula> (comprising 20 % of all unfrozen
freshwater in the world), hosts a unique ecosystem (Granina, 1997), and is an
important regional water resource (Garmaev and Khristoforov, 2010; Brunello
et al., 2006). There are numerous industries and agricultural activities
within the Selenga River basin, which affect the water quality of the lake
and its tributaries. Mining is well-developed in the region (e.g. Karpoff and
Roscoe, 2005; Byambaa and Todo, 2011), and heavy metals accumulate in biota
and in sediments of the Selenga River delta and Lake Baikal (Boyle et al.,
1998; Rudneva et al., 2005; Khazheeva et al., 2008).</p>
      <p>In addition to water chemistry, the role of aquatic systems as a net sink or
source for atmospheric CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is presently under debate. When
precipitation or other processes transport large volumes of organic matter
from land into nearby lakes and streams, the carbon of this matter
effectively disappears from the carbon budget of the terrestrial ecosystem
(Huotari et al., 2011). The enhanced decomposition of soil organic matter
may significantly affect the transport of terrestrial carbon to rivers,
estuaries, and the coastal ocean. The contribution of this process to the
global and regional carbon budgets is unknown. Thus, the biological
processes taking place in the terrestrial ecosystem (e.g. photosynthesis,
respiration, and decomposition) and in the aquatic ecosystem are
interlinked. The observed higher temperature response of aquatic ecosystems
compared to terrestrial ecosystems indicates that a substantial part of the
carbon respired or emitted from the aquatic system must be of terrestrial
origin (Yvon-Durocher et al., 2012). Long-term measurements carried out
during all seasons in the littoral zone of Lake Baikal showed that maximum
CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink and emission rates are observed in August and December (during
the pre-ice period), respectively, and the total CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux from the
atmosphere into the littoral zone of Lake Baikal was estimated to be 3–5 g CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> m<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Domysheva et al., 2013).</p>
      <p>The Siberian lakes situated in tundra and forest–tundra zones are in general
poorly studied. In their natural state, their productivity is low, but their
ecosystems are highly sensitive to external influences. Profuse blooming of
cyanobacteria is usually associated with urban and industrial effluents and
nutrient run-off. An assessment is needed of the impact of climate change in
the northern Eurasian region on eutrophication, accompanied by blooms of
cyanobacteria. Besides, the northern Eurasian region is characterized by thaw
lakes, which comprise 90 % of the lakes in the Russian permafrost zone
(Romanovsky et al., 2002). These lakes, which are formed in melting
permafrost, have long been known to emit CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>. The latest observations of
the lakes in the permafrost zone of northern Siberia indicate that they are
releasing much more CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> into the atmosphere than previously thought.
Rather than being emitted in a constant flow, 95 % of CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> comes from
random bubbling in disperse locations. In coming decades, this could become a
more significant factor in global climate change (Walter et al., 2006).</p>
      <p>One direct consequence of climate change is the explosive reproduction of
toxic cyanobacteria (<italic>Nodularia, Microcystis, Anabaena, Aphanizomenon, Planktothrix</italic>) and diatoms (<italic>Pseudo-nitzschia</italic>) (Moore et al., 2008; Paerl and
Huisman, 2009). These blooms occur in ponds, lakes, reservoirs, and bays of
the sea. Cyanobacteria and diatoms excrete especially dangerous carcinogens
and neurotoxins into the water. The toxicity of some cyanotoxins exceeds the
toxicity of currently banned warfare agents. Antidotes to these toxins do
not exist at the moment.</p>
      <p>Water conservation has received an increasing attention in China, and
multiple new projects have been initiated recently. Especially the
construction of water transfer, reservoir, and irrigation schemes have
received much attention, because the central and western regions of China are
suffering from water shortages. These projects are expected to improve water
usage and security, especially for agricultural activities, and to provide
sufficient water resources for local societies. In China, the river systems
are dominated by rivers flowing from the Tibetan plateau to the Pacific
Ocean. The Yangtze is the longest river in China, and flows from the Tibetan
plateau to Shanghai. The Yellow river is the second longest in China, and it
is characterized by seasonal flooding, which causes great economic and
societal losses. The Amur River forms the northern border with Russia. The
Haihe River flows through Beijing to Tianjin, and is under heavy stress from
the highly populated and industrialized capital metropolitan region. Only one
river from China flows to the Arctic Ocean: the Ertix River, which flows to
the north through Kazakhstan, across Siberian Russia, finally joining the Ob
River, which flows to the Arctic Ocean.</p>
</sec>
</sec>
<sec id="Ch1.S2.SS4">
  <title>Social system – state-of-the-art and future research needs</title>
<sec id="Ch1.S2.SS4.SSS1">
  <title>Land use and natural resources</title>
      <p>The fundamental large-scale task is to estimate how human actions such as
land use changes, energy production, the use of natural resources, changes in
energy efficiency, and the use of renewable energy sources will influence the
environments and societies of the northern Eurasian region. For example, the
industrial development of Siberia should be considered as one of most
important drivers of future land use and land cover changes in Russia.
Siberia is a treasure chest of natural resources of Russia, containing
85 % of its prospected gas reserves, 75 % of its coal reserves, and
65 % of its oil reserves. Siberia has more than 75 % of Russia's
lignite, 95 % of its lead, approximately 90 % of its molybdenum,
platinum, and platinoids, 80 % of its diamonds, 75 % of its gold, and
70 % of its nickel and copper (Korytnyi, 2009).</p>
      <p>During the 20th century, a considerable transformation of landscapes in
the tundra and taiga zones in northern Eurasia has occurred as a result of
various industrial, socio-economic and demographic processes, leading to the
industrial development of previously untouched territories (Bergen et al.,
2013). This has led to a decrease in the rural population and, mostly after
the 1990s, to decrease in agricultural activities. There has also been a
significant reduction in agricultural land use, and its partial replacement
by zonal forest ecosystems (Lyuri et al., 2010). According to recent
estimates, the total area of abandoned agricultural land in Russia in the
1990s to 2010s is at about 57 million ha, of which 18 million ha have been
restored by forests and 6 million ha of this are located in Asian Russia
(Schepaschenko et al., 2015). As a result, these areas have become active
accumulators of atmospheric CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (Kalinina et al., 2009). These new
forests (substituting resources) could form the basis for sustainable
development in these regions, in case relevant management programs for the
forests re-established on abandoned lands are going to be implemented.</p>
      <p>The dynamics of land cover, particularly forests, have been documented since
1961 when the results of the first complete inventory of Russian forests were
published. According to official statistics, the area of forests in Asian
Russia increased by around 80 million ha during 1961–2009, mostly before
the middle of the 1990s. This large increase is explained by improved quality
of forest inventories in remote territories, natural reforestation, mostly
during the Soviet era as a result of forest fire suppression, and encroaching
forest vegetation in previously non-forested land. Based on official
statistics, the area of cultivated agricultural land in the region decreased
by around 10 million ha between 1990 and 2009. After the year 2000, the
forested area in Siberia decreased, mostly due to fire and the impacts of
industrial transformations in high latitudes (Shvidenko and Schepaschenko,
2014). A critical decrease in the forest area has also been observed in the
most populated areas with intensive forest harvesting particularly in the
southern part of Siberia and the Far East. For example, in the Krasnoyarsk
Krai, the total area of forests decreased by 5 %, while that of mature
coniferous forests decreased by 25 %. Overall, the typical processes in
these regions are a dramatic decline in the quality of forests, unsustainable
use of forest resources, and insufficient governance and forest management in
the region, including frequent occurrence of illegal logging, natural, and
human-induced disturbances (Shvidenko et al., 2013a).</p>
      <p>Future land use and land cover changes will crucially depend on how
successfully the strategy of sustainable development of northern territories
is developed and implemented. An effective system for the adaptation of
boreal forests to global change needs to be developed and implemented in the
region. An “ecologization” of the current practices of industrial
development of previously untouched territories would allow a substantial
decrease in the physical destruction of landscapes, and halt the decline of
surrounding ecosystems due to air pollution and water and soil contamination
(Kotilainen et al., 2008).</p>
      <p>The expected changes in the climate and environment will have multiple and
complicated impacts on ecosystems, with consequent land cover changes. The
alteration of fire regimes and the thawing of permafrost will intensify the
process of “green desertification” in large areas. Climate warming will
have multiple effects on soil–vegetation–snow interactions. For example, in
a warmer climate, mosses and other vegetation grow faster, providing a
better thermal insulation of the permafrost in summer, and better feeding
conditions for reindeer. However, snow can also more easily accumulate on
thicker vegetation, thus protecting the deeper soil from cooling during the
winter (Tishkov, 2012).</p>
      <p>Both north and east Russia possess abundant mineral resources (Korytnyi,
2009). The resource orientation of northern and eastern Russia's economy,
which has not changed for centuries, increased in the post-Soviet period,
and has been influenced primarily by the product market. It is also expected
that the natural resource development sector will continue to dominate the
economy in the majority of these territories for the next decades.</p>
      <p>A crucial factor in greenhouse gas emission dynamics is the fuel balance. In
Russia, features of the fuel balance have led to an increased pollution. On
average, specific emissions in the northern and eastern cities of Russia,
where coal accounts for most of the power generation, are 3 times higher
than in cities where power is generated mainly from gas or fuel oil (Bondur,
2011a). The geographical location, undeveloped infrastructure, harsh climate,
and coal burning are the main reasons for increased levels of anthropogenic
pollution in these areas (Bondur and Vorobev, 2015; Bondur, 2014). In small
towns, low-capacity boiler rooms are the main source of emissions. Usually,
the lack of financial resources leads to the use of low-quality coal and
obsolete boilers. In the steppe zone of Asian Russia, Mongolia, Kazakhstan,
and Buryatia, the main source of emissions is the burning of harvest
residues.</p>
      <p>The dynamics of GHG emissions in Russia are largely determined by the
economic conditions of production. The economic crisis in 1990–1998 slowed
down environmental degradation to some extent: emissions generally decreased
by 40 %. However, the underlying environmental problems not only remained
unresolved, but significantly deepened, and turned into systemic problems.
The most polluting industries were more resistant to the decline in
production. Technological degradation took place, cleaning systems were
eliminated, and production shifted to part-time, leading to inefficient
capacity utilization. Significant amounts of pollution continued to be
emitted from the domestic sector. Emissions decreased in most regions of the
country, and in 83 % of the cities, but much more slowly than production.
As a result, the specific emissions (per product cost at comparable prices)
had grown by the end of the 1990s in all categories of cities, except cities
with more than 1 million inhabitants (Bityukova et al., 2010). All this can
cause negative impacts on ecosystems. For example, there are about
2 million ha of technogenic deserts around Norilsk. Norilsk is probably the
biggest smelter in the world, and produces more than 2 million t of
pollutants per year (Groisman et al., 2013).</p>
</sec>
<sec id="Ch1.S2.SS4.SSS2">
  <title>Natural hazards</title>
</sec>
<sec id="Ch1.S2.SS4.SSSx1" specific-use="unnumbered">
  <title>Extreme weather and fire occurrence</title>
      <p>The frequency and intensity of weather extremes have increased substantially
during the last decades in Europe, Russia, and China. Further acceleration
is expected in the future (IPCC, 2013). The evolving impacts, risks, and costs
of weather extremes on population, environment, transport, and industry have
so far not been properly assessed in the northern latitudes of Eurasia. New
knowledge is needed for improving the forecasting of extreme weather events,
for understanding the effect of wildfires on radiative forcing and
atmospheric composition in the region, for estimating the impacts of weather
extremes on major biogeochemical cycles, and for understanding the effects
of disturbances in forests on the emissions of BVOC and VON (volatile
organic nitrogen) (Bondur, 2011b, 2015; Bondur and Ginsburg, 2016). How do
changes in the physical, chemical and biological state of the different
ecosystems and the inland, water, and coastal areas affect the economies and
societies in the region, and vice versa?</p>
      <p>The number of large hydrometeorological events in Russia that cause
substantial economic and social losses has increased by more a factor of 2
from 2001 to 2013 (State Report, 2011). The main hazards are related to
atmospheric processes on various temporal and spatial scales, including
strong winds, floods and landslides caused by heavy precipitation, and fires
caused by drought and extreme temperatures. High temperatures and long
droughts can substantially decrease the productivity and cause high dieback
in dark coniferous forests. Hurricanes occur fairly often in the forest zone.
For example, a hurricane destroyed about 78 000 ha of forest in the Irkutsk
region in July 2004 (Vaschuk and Shvidenko, 2006). However, there are no
reliable statistics on many types of natural hazards.</p>
      <p>In order to build scenarios of the future frequency and properties of
weather-related hazards, one should first analyse the atmospheric mechanisms
behind the circulation structures responsible for these hazards: the
cyclones related to strong winds and heavy precipitation and the
anticyclones related to drought and fires episodes. Studying the
cyclone/anticyclone tracks, frequency and intensity can provide a
statistical basis for understanding the geographical distribution and
properties of the major atmospheric hazards and extremes (e.g. Shmakin and
Popova, 2006). For future climate projections, atmospheric hazards and
extremes should be interpreted from the viewpoint of cyclone/anticyclone
statistics, and possible changes in the cyclone/anticyclone geography and
frequency should be analysed.</p>
      <p>Fires are the most important natural disturbances in the boreal forests.
Fires strongly determine the structure, composition, and functioning of the
forest. Each year, about 0.5–1.5 % of the boreal forest burns. Since
boreal forests cover 15 % of the Earth's land surface, this is a
significant area (Kasischke, 2000; Conard et al., 2002; Bondur, 2011b, 2015).
Climate change already substantially impacts fire regimes in northern
Eurasia. More frequent and severe catastrophic (mega-) fires have become a
typical feature of the fire regimes. Such fires envelope areas of up to a
hundred thousand hectares within large geographical regions, lead to the
degradation of forest ecosystems, decrease the biodiversity, may spread to
usually unburned wetlands, cause large economic losses, deteriorate life
conditions and health of local populations, and lead to “green
desertification”, which is an irreversible transformation of the forest
cover for long periods (Shvidenko and Schepaschenko, 2013; Bondur, 2011b,
2015). Megafires also lead to specific weather conditions over the affected
areas that are comparable in size to large-scale pressure systems
(<inline-formula><mml:math display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 30 million ha and more). The annually burned area in the Russian
territory was estimated to be <inline-formula><mml:math display="inline"><mml:mrow><mml:mn>8.2</mml:mn><mml:mo>±</mml:mo><mml:mn>0.8</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn>10</mml:mn><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> ha during
1998–2010, and about two-thirds of this area consisted of boreal forests.
For this period, the fire carbon balance (total amount of carbon in the burnt
fuel) was estimated to be 121 <inline-formula><mml:math display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 28 Tg C yr<inline-formula><mml:math display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Shvidenko et al.,
2011). Current model projections suggest that the number of fires will double
by the end of this century. The extent of catastrophic fires escaping from
the control and fire intensity are projected to increase. Due to increased
severity of fire and deeper soil, carbon emissions from fires are predicted
to increase by a factor of 2 to 4 (Gromtsev, 2002; Malevsky-Malevich et al.,
2008; Flanningan et al., 2009; Shvidenko et al., 2011). During and after
fires, significant changes take place in the forest ecosystems, including the
soil. These changes include (i) a significant amount of biomass is combusted,
and large amounts of carbon and nitrogen are released to the atmosphere in
the form of carbon dioxide and other gases or particles (Harden et al., 2000;
Andreae and Merlet, 2001; Kaiser et al., 2012; Konovalov et al., 2014;
L. Kulmala et al., 2014); (ii) fire alters the microbial
community structure in the soil as well as the structure of the vegetation
(Dooley and Treseder, 2012; Sun et al., 2015); (iii) fires determine the
structure of the vegetation, succession dynamics and the fragmentation of
forest cover, tree species composition, and the productivity of boreal
forests (Gewehr et al., 2014), and (iv) fire is one of the crucial drivers
controlling the dynamics of the carbon stock of boreal forests (Jonsson and
Wardle, 2010; Köster et al., 2014).</p>
      <p>Disturbances resulting from fire, pest outbreaks, and diseases also have
substantial effects on the emissions of BVOCs and volatile organic nitrogen
compounds (Isidorov, 2001), and consequently on atmospheric aerosol
formation. The acceleration of fire regimes will also affect the amount of
black carbon in the atmosphere, and thus has an effect on the albedo of the
cryosphere.</p>
</sec>
<sec id="Ch1.S2.SS4.SSSx2" specific-use="unnumbered">
  <title>Permafrost degradation and infrastructures</title>
      <p>The degradation of permafrost will cause serious damage both to
infrastructure and to ecosystems and water systems in the northern Eurasian
region. This includes, for example, damage to pipelines and buildings,
deformation of roads and railroads in Russia, Mongolia, and China, variations
in the ion distribution in soil water in young and ancient landslides,
cryogenic landslides, spatial and temporal changes of grass and willow
vegetation, saline water accumulation in local depressions of the permafrost
table, and formation of highly saline lenses of groundwater called “salt
traps”.</p>
      <p>Due to the large extent of permafrost-covered areas in northern Eurasia (for
ecosystem effects, see Sect. 2.1.1 and 2.1.2), there are numerous
infrastructural issues related to possible changes in the thickness and
temperature of the frozen part of the subsurface, and thus in the mechanical
soil properties. Climate change-induced changes in the cryosphere are
probably among the most dramatic issues affecting the infrastructure in
northern Eurasia, as this infrastructure is literally standing on permafrost.
Moreover, an interesting coupling may be related to the decreasing ice-cover
of the Arctic Ocean, which results in increased humidity and precipitation on
the continent, and thus a further thickening and longer duration of the
annual snow cover. Snow is a good thermal insulator, and influences the
average ground surface temperature, thus playing a potentially important role
in speeding up the thawing of permafrost.</p>
      <p>The increased risk of damage to local infrastructure, such as buildings and
roads, can cause significant social problems, and exerts pressure on the
local economies. Thawing permafrost is structurally weak, and places a
variety of infrastructure at risk. For example, the failure of buildings,
roads, pipelines, or railways can have dramatic environmental consequences,
as seen in the 1994 breakdown of the pipeline to the Vozei oilfield in
northern Russia, which resulted in a spill of 160 000 t of oil – the
world's largest terrestrial oil spill (United Nations Environment Program,
2013). Maintenance and repair costs related to permafrost thaw and
degradation of infrastructure in northern Eurasia have recently increased,
and will most probably increase further in the future. This is an especially
prominent problem in discontinuous permafrost regions, where even small
changes in the permafrost temperature can cause significant damage to
infrastructure. Most settlements in permafrost zones are located on the
coast, where strong erosion places structures and roads at risk. After damage
to the infrastructure, local residents and indigenous communities are often
forced to relocate. This can cause changes in, or even disappearances of,
local societies, cultures, and traditions (United Nations Environment
Program, 2013).</p>
</sec>
<sec id="Ch1.S2.SS4.SSSx3" specific-use="unnumbered">
  <title>Changing sea environments and the risk of accidents in coastal
regions</title>
      <p>In northern Eurasia, from the eastern part of the Barents Sea to the Bering
Sea, the permafrost is located directly on the seacoast. In many of these
coastal permafrost areas, sea level rise and continuing permafrost
degradation leads to significant coastal erosion, and to the possibility of
a collapse of coastal constructions, lighthouses, ports, houses, etc.
In this region, the sea level rise is coupled to the permafrost degradation
in a complex way, and should be focused on in future studies.</p>
      <p>Understanding and measuring artificial radionuclides in marine ecosystems is
needed for improving emergency preparedness capabilities, and for developing
risk assessments of potential nuclear accidents. The awareness of the
general public and associated stakeholders across the region should also be
raised concerning the challenges and risks associated with nuclear
technologies, environmental radioactivity, and emergency preparedness. The
current state of radioactive contamination in terrestrial and marine
ecosystems in the European Arctic region will be studied by examining
environmental samples collected from Finnish Lapland, Finnmark, and Troms in
Norway, the Kola Peninsula, and the Barents Sea. The results will provide
updated information on the present levels, occurrence and fate of
radioactive substances in the Arctic environments and food chains. The
results will also allow us to estimate where the radioactive substances
originate from, and what risks they may pose in case of accidents.</p>
      <p>Annual expeditions for sample collection are needed for the development of
models to predict the distribution of radionuclides in the northern marine
environment, and for the assessment of the current state of radioactive
contamination in marine ecosystems in the European Arctic region. In view of
recent developments and increased interests in the European Arctic region
for oil and gas extraction, special attention needs to be given to the
analysis of norms (naturally occurring radioactive materials) in order to
understand current levels. The future focus should be put on atmospheric
modelling, and on the assessment of radionuclide distributions in the case of
accidents leading to the release of radioactive substances to the
environment in the European Arctic region. This includes the assessment of
nuclear accident scenarios for dispersion modelling.</p>
</sec>
<sec id="Ch1.S2.SS4.SSS3">
  <title>Social transformations</title>
      <p>Climate and weather strongly affect the living conditions, mostly in the
Eastern part of the northern Eurasian societies, influencing people's
health, incidence of diseases and adaptive capacity. The vulnerability of
societies, including their adaptive capacity, varies greatly depending on
both their physical environment, and on their demographic structure and
economic activities. There is a need to analyses the scientific
background and robustness of the adaptation and mitigation strategies (AMS)
of the region's societies, and their resilience capacity, with special
emphasis on the forest sector and agriculture. The future research needs are
in understanding what ways populated areas are vulnerable to climate
change; how their vulnerability can be reduced and their adaptive capacities
improved; what responses should be identified to mitigate and adapt to
climate changes.</p>
      <p>Health issues are also important in multi-disciplinary studies of northern
Eurasia, as the living conditions of both humans and livestock are changing
dramatically. SLCF, such as black carbon,
ozone, and aerosol particles, are important players in both air quality and
Arctic climate change and their impacts are not yet quantified. Black carbon
has a special role when designing future emission control strategies, since
it is the only major aerosol component whose reduction is likely to be
beneficial to both climate and human health. These changes can be expressed
through complex parameters combining the direct effects of, e.g.,
temperature and wind speed, with indirect effects of several climatic and
non-climatic factors such as the atmospheric pressure variability, or the
frequency of unfavourable weather events, e.g. heat waves or strong winds.
During the last decades, living conditions in northern Eurasia have
generally improved, but with a significant regional and seasonal variation
(Zolotokrylin et al., 2012).</p>
      <p>Both northern and eastern Eurasia have small and diminishing populations,
mainly due to the migration outflow started in the 1990s due to severe and
unfavourable living conditions combined with changing state policies with
respect to the development of the northern territories. This reversed the
previous long-standing pattern of migration inflow. The combination of
outflow and natural population decrease (with some regional exceptions in
several ethnic republics and autonomous regions (<italic>okrugs</italic>) with oil
and gas industry) led to a steady population decline in most regions in
northern and eastern Russia from 1990s. In the post-soviet period, the
population of eastern Russia decreased by 2.7 million, while the population
of Russia's Arctic zone decreased by nearly by one-third (500 000 people),
in contrast to the majority of the world's Arctic territories (Glezer, 2007a,
b). The population change in north-eastern Russia was particularly
remarkable: the Chukotka
Autonomous Okrug lost 68 % of its
population, the Magadan Oblast lost 59 %, and the Kamchatka Krai lost
33 %.</p>
      <p>Geographical and ethnic factors influence the demography and settlement
pattern in the region. Geographical factors include environmental conditions
and the mixture of urban and rural territories. Areas with a large proportion
of indigenous people employed in traditional nature management were exposed
to relatively small post-soviet transformations in the 1990s and 2000s. In
contrast, the largest transformations occurred in areas with a larger
proportion of Russian people and developed mining industries. The differences
in the transformations between settlements with predominantly indigenous and
predominantly Russian populations are evident. For example, in the Chukotka
Autonomous Okrug, the former remained mostly intact, with only small decreases in
population, while the latter disappeared entirely or were significantly
depopulated (Litvinenko, 2012, 2013).</p>
      <p>When assessing the impacts of climate change and other environmental changes
on human societies, it should be taken into account that the urban
environments in northern Eurasian cities and towns situated in the less
favoured regions are currently incapable of mitigating unfavourable impacts.
The impact of climate parameters, such as temperature (including seasonal,
weekly, and daily cycles, and extreme values), strong winds, snowfall,
snowstorms, and precipitation should be investigated. Both the frequency and
the duration of weather events should be considered. These climate
parameters influence human health, incidence of diseases, adaptation
potential, and economic development in general. Furthermore, it is important
to explore the interactions between the environmental change and post-soviet
transformations of natural resource utilization in northern Eurasia in order
to assess the complexity of their socio-ecological consequences at regional
and local levels (Litvinenko, 2012; Tynkkynen, 2010). The population
dynamics of the northern Russian regions in 1990–2012, and the linkage
between intra-regional differences in population dynamics, spatial
transformations of natural resources utilization, and ethnic composition of
the populations should be clarified. It would be desirable to develop an
“early warning system” for the timely mitigation of the negative
socio-ecological effects of both environmental changes, and changes in the
availability of natural resources as well as accident like leakages in gas
and oil pipelines. Such systems would be useful for federal, regional, and
local authorities as well as for local communities.</p>
      <p>It should also be taken into account that the majority of the world's ethnic
groups are small and engaged in culturally specialized methods of
subsistence, so any change in their immediate environment may lead to their
traditional way of life becoming unsustainable. These changes may be due to
rising sea levels, warming seawater, melting ice cover, thawing permafrost,
flooding rivers, changing rain patterns, or moving vegetational zones. These
are direct effects of climate change and environmental deterioration on
ethnodiversity. However, even more threatening are the indirect effects. The
immediate environment of small ethnic groups is often vulnerable to the
adverse impact of majority populations representing governments and nations.
The effects of climate change may lead to a rapid and massive transfer of
majority populations to areas previously inhabited by small ethnic groups.</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S3">
  <title>From process studies towards system understanding and quantification of
feedbacks of Arctic–boreal regions</title>
      <p>The system understanding helps us to understand the behaviour of feedbacks
between the land, atmosphere, aquatic, and societal/economic systems. To be
able to provide a system understanding, we need to understand the individual
processes, and based on process understanding we are then able to quantify
different biogeochemical cycles. Via biogeochemical cycles, the energy and
matter flows are linked to a wider system context, which enables us to
analyse the feedback phenomena. Feedbacks are essential components of our
climate system, as they either increase or decrease the changes in
climate-related parameters in the presence of external forcings (IPCC,
2013).</p>
      <p>The effects of climate change on biogeochemical cycles are still inadequately
understood, and many feedback mechanisms are difficult to quantify (Arneth et
al., 2010; M. Kulmala et al., 2014). They are related to, for example, the
coupling of carbon and nitrogen cycles, permafrost processes and ozone
phytotoxicity (Arneth et al., 2010), or to the emissions and atmospheric
chemistry of biogenic volatile organic compounds (Grote and Niinemets, 2008;
Mauldin et al., 2012), subsequent aerosol formation processes (Kulmala et
al., 2004b; Tunved et al., 2006; Kulmala et al.,
2011a; Hirsikko et al., 2011) and aerosol–cloud interactions (McComiskey and
Feingold, 2012; Penner et al., 2012; Rosenfeld et al., 2014).</p>
      <p>The northern Eurasian Arctic–boreal geographical region covers a wide range
of interactions and feedback processes between humans and natural systems.
Humans are acting both as the source of climate and environmental changes,
and as recipient of their impacts. The PEEX research agenda is addressing
the most relevant research topics related to the process dynamics in the
land, atmospheric, aquatic, and society systems relevant to northern
regions. PEEX also aims to quantify the range of emissions and fluxes from
different types of ecosystems and environments and links to ecosystem
productivity (see also Su et al., 2011; Kulmala and Petäjä, 2011;
Bäck et al., 2010). This new knowledge helps us to obtain a holistic
view on the changes in biogeochemical cycles and feedbacks in the future
Arctic–boreal system (Fig. 4). PEEX will also to take into consideration that
there may exist previously unknown sources and processes (Su et al., 2011;
Kulmala and Petäjä, 2011; Bäck et al., 2010).</p>
      <p>Holistic representations of feedback loops potentially relevant to
Arctic–boreal systems have been given by Charlson et al. (1987), Quinn and
Bates (2011), and by M. Kulmala et al. (2004a,
2014). The “CLAW” hypothesis (the CLAW acronym
refers to Charlson, Lovelock, Andreae and Warren) connects the ocean
biochemistry and climate via a negative feedback loop involving cloud
condensation nuclei production due to dimethylsulfoniopropionate (DMSP) and
dimethyl sulfide (DMS) biosynthesis by marine phytoplankton (e.g. Quinn and
Bates, 2011; Ducklow et al., 2001; O'Dowd et al., 2004; de Leeuw et al.,
2011; Malin et al., 1993; O'Dowd and de Leeuw, 2007). The COBACC (COntinental
Biosphere–Aerosol–Cloud–Climate) hypothesis suggests two partly
overlapping feedbacks that connect the atmospheric carbon dioxide
concentration, ambient temperature, gross primary production, biogenic
secondary organic aerosol formation, clouds, and radiative transfer (M. Kulmala
et al., 2004a, b, 2014; also see Sect. 2.1.1.).
The quantification of these feedback loops under changing climate is crucial
for reliable Earth system modelling and predictions.</p>
      <p>In the context of the COBACC feedback loop, the key large-scale research
questions are the changing cryospheric conditions and consequent changes in
ecosystem feedbacks affecting the Arctic–boreal climate system and weather.
Furthermore, we should estimate the net effects of various feedback effects
(CLAW, COBACC) on land cover changes, photosynthetic activity, GHG
exchanges, BVOC emissions, aerosol and cloud formation, and radiative
forcing at regional and global scales. In our analysis, we should also take
into account the urbanization processes and social transformations (see
Sect. 2.4.3), which are changing the regional climates. In this task, we
should also study the key gaps of the biogeochemical cycles.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4"><caption><p>In urban and industrialized regions, the process understanding of
biogeochemical cycles includes anthropogenic sources, such as industry and
fertilizers, as essential parts of the biogeochemical cycles.</p></caption>
        <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f04.png"/>

      </fig>

<sec id="Ch1.S3.SS1">
  <title>Hydrological cycle</title>
      <p>Climate change may profoundly affect most of the components of the
hydrological cycle, giving rise to positive or negative feedbacks (Fig. 5).
While variations in the hydrological cycle often take place at regional or
local scales, they can also give rise to large-scale or even global changes.
Knowledge of the hydrological cycle in general and particularly related to
permafrost is crucial for predicting the resilience and transformation of
forest ecosystems coupled with permafrost (Osawa et al., 2010).</p>
      <p>In addition to permafrost processes, another important issue in high
latitudes is precipitation. Precipitation is a critical component of the
hydrological cycle, having a great spatial and temporal variability. The
lack of understanding of some precipitation-related processes, combined with
the lack of global measurements of sufficient detail and accuracy, limits
the quantification of different components of the hydrological cycle such as
precipitation, evapotranspiration, or CCN formation. This is especially
true in high-latitude regions, where observations and measurements are
particularly sparse, and processes poorly understood.</p>
      <p>Recent retrievals of multiple satellite products for each component of the
terrestrial water cycle provide an opportunity to estimate the water budget
globally (Sahoo et al., 2011) (Fig. 5). Global precipitation is retrieved at
very high spatial and temporal resolution by combining microwave and
infrared satellite measurements (Sorooshian et al., 2000; Kummerow et al.,
2001; Joyce et al., 2004; Huffman et al., 2007). Large-scale estimates of
global precipitation have been derived by applying energy balance, process,
and empirical models to satellite-derived surface radiation, meteorology,
and vegetation characteristics (e.g. Mu et al., 2007; Su et al., 2007;
Fisher et al., 2008; Sheffield et al., 2010). The water storage change
component can be obtained from satellite data, and the water level in lakes
and large-scale river systems can be estimated from satellite altimetry with
special algorithms developed for terrestrial waters (Berry et al., 2005;
Velicogna et al., 2012; Troitskaya et al., 2012, 2013).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5"><caption><p>Hydrological cycle schematics.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f05.jpg"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS2">
  <title>Carbon cycle</title>
      <p>It is not clear how future climate will modify incoming terrestrial net
primary production (NPP) and outgoing (e.g. heterotrophic soil respiration,
HSR) carbon fluxes to and from terrestrial ecosystems. It is likely that the
transformation of Russian forests is a tipping element for the climate system
by the end of the century over huge areas, even though uncertainties in such
forecasts are significant (Gauthier et al., 2015). The role of boreal and
Arctic lakes and catchment areas in carbon storage dynamics is poorly
quantified (Fig. 6).</p>
      <p>The terrestrial biosphere is a key regulator of atmospheric chemistry and
climate via its carbon uptake capacity (Arneth et al., 2010; Heimann and
Reichstein, 2008). The Eurasian area holds a large pool of organic carbon
both within the above- and below-ground living biota, in the soil, and in
frozen ground, stored during the Holocene and the last ice age. The area also
contains vast stores of fossil carbon. According to estimates of carbon
fluxes and stocks in Russia made as part of a full carbon account by the
land–ecosystem approach (Shvidenko et al., 2010; Schepaschenko et al., 2011;
Dolman et al., 2012), terrestrial ecosystems in Russia served as a net carbon
sink of 0.5–0.7 Pg(C) per year during the last decade. Forests provided
above 90 % of this sink. The spatial distribution of the carbon budget
shows considerable variation, and substantial areas, particularly in
permafrost regions and in disturbed forests, display both sink and source
behaviour. The already clearly observable greening of the Arctic is going to
have large consequences on the carbon sink in the upcoming decades (Myneni et
al., 1997; Zhou et al., 2001), although future predictions are uncertain. The
net ecosystem carbon budget (NECB) or net biome production (NBP) are usually
a sensitive balance between carbon uptake through forest growth, ecosystem
heterotrophic respiration, and carbon release during and after disturbances
such as fire, insect outbreaks, or weather events, e.g. as exceptionally warm
autumns (Piao et al., 2008; Vesala et al., 2010). This balance is delicate,
and for example in the Canadian boreal forest the estimated net carbon
balance is close to carbon neutral due to fires, insects, and harvesting
cancelling the carbon uptake from forest net primary production (Kurz and
Apps, 1995; Kurz et al., 2008b). Long-term
measurements of the concentrations of CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and other carbon gases at
selected sites, especially using tall towers such as the ZOTTO tower, will be
essential for constraining the large-scale carbon fluxes in the PEEX region
(Heimann et al., 2014).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6"><caption><p>Carbon cycling in the Arctic will change as the climate warms.
Figure after ACIA, 2004 (Arctic Climate Impact Assessment, 2004).</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f06.jpg"/>

        </fig>

      <p>Plant growth and carbon allocation in boreal forest ecosystems depend
critically on the supply of recycled nutrients within the forest ecosystem.
In the nitrogen-limited boreal and Arctic ecosystems, the biologically
available nitrogen (NH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> and NO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">3</mml:mn></mml:msub></mml:math></inline-formula>) is in short supply, although the
flux of assimilated carbon below ground may stimulate the decomposition of
nitrogen-containing soil organic matter (SOM), and the nitrogen uptake of
trees (Drake et al., 2011; Phillips et al., 2011). The changes in easily
decomposable carbon could enhance the decomposition of old SOM (Kuzyakov,
2010; Karhu et al., 2014), and thus increase the turnover rates of nitrogen
in the rhizosphere, with possible growth-enhancing feedbacks on vegetation
(Phillips et al., 2011).</p>
      <p>Arctic warming is promoting terrestrial permafrost thaw and shifting
hydrologic flow paths, leading to fluvial mobilization of ancient carbon
stores (Karthe et al., 2014). Observed permafrost thaw acts as a significant
and preferentially degradable source of bioavailable carbon in Arctic
freshwaters, which is likely to increase as permafrost thaw intensifies,
causing positive climate feedbacks in response to ongoing climate change
(Mann et al., 2012). Significant differences in fluvial carbon input between
headwaters and downstream reaches of large Arctic catchments (Yenisey and
Lena) have been identified, but the problem is until now very poorly
explained. At the same time, the fluvial export by the largest rivers is
considered to be an order of magnitude less than coastal erosion in the East
Siberian Arctic Shelf (Semiletov et al., 2011). The Lena's particulate
organic carbon export is estimated to be 2 orders of magnitude less than the
annual input of eroded terrestrial carbon onto the shelf of the Laptev and
East Siberian seas.</p>
      <p>Although inland waters are especially important as lateral transporters of
carbon, their direct carbon exchange with the atmosphere, so-called
outgassing, has been recognized to be a significant component in the global
carbon budget (Bastviken et al., 2011; Regnier et al., 2013). In the boreal
pristine regions, forested catchment lakes can vent ca. 10 % of the
terrestrial NEE (net ecosystem exchange), thus weakening the terrestrial
carbon sink (Huotari et al., 2011). There is a negative relationship between
the lake size and gas saturation, and especially small lakes are relatively
large sources of CO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> (e.g. Kortelainen et al., 2006; Vesala
et al., 2012). However, on a landscape level, large lakes can still dominate
the GHG fluxes. Small lakes also store relatively larger amounts of carbon in
their sediments than larger lakes. The role of lakes as long-term sinks of
carbon, and simultaneously as clear emitters of carbon-containing gases, is
strongly affected by the physics of the water column. In lakes with very
stable water columns and anoxic hypolimnion sediments, carbon storage is
especially efficient, but at the same time, these types of lakes emit
CH<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>. In general, the closure of landscape-level carbon balances is
virtually impossible without studying the lateral carbon transfer processes
(Pumpanen et al., 2014), and the role of lacustrine ecosystems as GHG
sources/sinks. Besides lakes, these studies should include rivers and
streams, which could be even more important than lakes as transport routes of
terrestrial carbon and as emitters of GHGs (Huotari et al., 2013). In
addition, the role of VOC emissions as a part of the carbon budget needs to
be quantified.</p>
</sec>
<sec id="Ch1.S3.SS3">
  <title>Nitrogen cycle</title>
      <p>Nitrogen is the most abundant element in the atmosphere. However, most of the
atmospheric nitrogen is in the form of inert N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, which is unavailable
most for plants and microbes, and can only be assimilated into terrestrial
ecosystems through biological N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fixation (Canfield et al., 2010). Only
cryptogamic covers and certain organisms living in symbiosis with plants are
capable of nitrogen fixation, making nitrogen the main growth-limiting
nutrient in terrestrial ecosystems (Elbert et al., 2012; Lenhart et al.,
2015). Human perturbations to the natural nitrogen cycle have, however,
significantly increased the availability of nitrogen in the environment
(Fig. 7). These perturbations mainly stem from the use of fertilizers in
order to increase crop production to meet the demands of the growing
population (Sutton et al., 2010), although atmospheric nitrogen deposition
may also play a significant role in some areas. The increased use of
fertilizer nitrogen, and consequent perturbations in nitrogen cycling, also
cause severe environmental problems such as eutrophication of terrestrial and
aquatic ecosystems, atmospheric pollution, and groundwater deterioration
(Sutton et al., 2010).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7"><caption><p>Schematic figure for terrestrial nitrogen cycle.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f07.jpg"/>

        </fig>

      <p>Emission of reactive nitrogen (NO, NO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, HONO, ammonia, amines) from
soils (Su et al., 2011; Korhonen et al., 2013), fossil fuel burning, and
other sources links the nitrogen cycle to atmospheric chemistry and secondary
aerosol formation in the atmosphere. There are indications that emissions of
N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>O from the melting permafrost regions in the Arctic may significantly
influence the global N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>O budget and hence contribute to the positive
radiative forcing by greenhouse gases (Repo et al., 2009; Elberling et al.,
2010).</p>
      <p>In natural terrestrial ecosystems, nitrogen availability limits ecosystem
productivity, linking the carbon and nitrogen cycles closely together
(Gruber and Galloway, 2008). The increasing temperatures due to climatic
warming accelerate nitrogen mineralization in soils, leading to increased
nitrogen availability and transport of reactive nitrogen from terrestrial to
aquatic ecosystems. This perturbed and accelerated nitrogen cycling may lead
to large net increases in the carbon sequestration of ecosystems (Magnani et
al., 2007). The large surface area of boreal and Arctic ecosystems implies
that even small changes in nitrogen cycling or feedbacks to the carbon cycle
may be important on the global scale (Erisman et al., 2011). For instance,
increased atmospheric nitrogen deposition has led to higher carbon
sequestration in boreal forests (Magnani et al., 2007). However, the
feedback mechanisms from increased perturbations of the nitrogen cycle may
change the dynamics of the emissions of other greenhouse gases, hence
complicating the overall effects. For instance, the stimulated carbon uptake
of forests due to increased atmospheric nitrogen deposition can largely be
offset by the simultaneously increased soil N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>O emissions (Zaehle et
al., 2011). In the Arctic, the melting permafrost may lead to high emissions
of N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>O (Repo et al., 2009; Elberling et al., 2010), which may
significantly influence the global N<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>O budget.</p>
      <p>Understanding the processes within the nitrogen cycle, the interactions of
reactive nitrogen with the carbon and phosphorus cycles, atmospheric
chemistry and aerosols, as well as their links and feedback mechanisms, is
therefore essential in order to fully understand how the biosphere affects
the atmosphere and the global climate (Kulmala and Petäjä, 2011).</p><?xmltex \hack{\newpage}?>
</sec>
<sec id="Ch1.S3.SS4">
  <title>Phosphorus cycle</title>
      <p>Phosphorus (P) is, together with nitrogen (N), one of the limiting nutrients
for terrestrial ecosystem productivity and growth, while in marine
ecosystems, phosphorus is the main limiting nutrient for productivity
(Whitehead and Crossmann, 2012). The role of P in nutrient limitation in
natural terrestrial ecosystems has not been recognized as widely as that of
N (Vitousek et al., 2010).</p>
      <p>In the global phosphorus biogeochemical cycle, the main reservoirs are in
continental soils, where phosphorus in mineral form is bound to soil parent
material, and in ocean sediments (Fig. 8). Sedimentary phosphorus originates
from riverine transported material eroded from continental soils. The
atmosphere plays a minor role in the phosphorus cycle, and the phosphorus
cycle does not have a significant atmospheric reservoir. Atmospheric
phosphorus mainly originates from aeolian dust, sea spray, and combustion
(Wang et al., 2014). Gaseous forms of phosphorus are scarce, and their
importance for atmospheric processes is unknown (Glindemann et al., 2005).</p>
      <p>South-western Siberian soils have lately been reported to contain high
concentrations of plant-available phosphorus (Achat et al., 2013), which may
enhance the carbon sequestration of the ecosystems if they are not too
limited by nitrogen. In soils, phosphorus is found mainly in mineral form
and bound to the soil parent material such as apatite minerals. The amount
of phosphorus in the parent material is a defining factor for phosphorus
limitation, and the weathering rate determines the amount of phosphorus
available for ecosystems. In ecosystems, most of the available phosphorus is
in organic forms (Achat et al., 2013; Vitousek et al., 2010). In ecosystems
growing on phosphorus-depleted soils, the productivity is more likely to be
nitrogen-limited in early successional stages, and gradually shift towards
phosphorus limitation as the age of the site increases (Vitousek et al.,
2010). In freshwater ecosystems, excess phosphorus leads to eutrophication,
which has ecological consequences, such as the loss of biodiversity due to
changes in physicochemical properties and in species composition (Conley et
al., 2009). Due to the scarcity of studies focusing on ecosystem phosphorus
cycling, the effects of climate change on physicochemical soil properties
and phosphorus availability, and the interactions of the phosphorus cycle
with the cycles of carbon and nitrogen, are largely unknown.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8"><caption><p>Schematic figure of the phosphorus cycle.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f08.jpg"/>

        </fig>

</sec>
<sec id="Ch1.S3.SS5">
  <title>Sulfur cycle</title>
      <p>Sulfur is released naturally through volcanic activity as well as through
weathering of the Earth's crust. The largest natural atmospheric sulfur
source is the emission of DMS from oceanic phytoplankton
(Andreae, 1990). DMS is converted to sulfur dioxide (SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), sulfuric
acid (H<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>), and methyl sulfonic acid (MSA) via gas-phase oxidation.
However, human activities have a major effect on the global sulfur cycle via
vast emissions of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> from fossil fuel burning and smelting activities.
The main sink of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is oxidation to sulfuric acid in both gas and
liquid phases, and subsequent removal from the atmosphere via precipitation
and dry deposition.</p>
      <p>Global anthropogenic SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions are predicted to decrease
significantly by the year 2100 (IPCC SRES, 2000). Emissions in Europe and
North America started to decrease already in the 1970s, but this decrease is
still overwhelmed on a global scale by increasing emissions in eastern Asia
and other strongly developing regions of the world (Smith et al., 2011). The
current global anthropogenic SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions are about 120 Tg per year,
with Europe, the former Soviet Union and China together responsible for
approximately 50 % (Smith et al., 2011). Global natural emissions of
sulfur, including DMS, are significantly smaller (a few tens of Tg per year;
Smith et al., 2001). Anthropogenic emissions dominate especially over the
continents. The main sources of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> are coal and petroleum combustion,
metal smelting, and shipping, with minor contributions from biomass burning
and other activities.</p>
      <p>SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions in Eurasia have a large spatial variability. Smelters in
the Russian Arctic areas emit vast amounts of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, significantly
affecting the regional environment. In 2007 Blacksmith Institute experts
estimated, that the smelter complexes in Norilsk, with annual emissions of 2
Tg are alone responsible for more than 1.5 % of global SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions. However, the emissions from the smelters in the Kola Peninsula,
while still remarkably high, have decreased significantly during the past
decades (Paatero et al., 2008), thus altering the impact of human activities
on the regional climate and environment. In general, existing anthropogenic
activities are slowly becoming more sulfur-effective and less polluting.
However, the emergence of new sulfur-emitting activities and infrastructures
partially counteracts this development.</p>
      <p>The behaviour of future changes in SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions in the PEEX research
area is uncertain. In northern Eurasia, natural resources like fossil fuels,
metals, minerals, and wood are vast, and their utilization is becoming more
and more attractive due increasing demand. This will most likely lead to an
increase in human activities (e.g. mining, oil drilling, shipping) in this
area (e.g. Smith, 2010, and references therein). For example, sulfur
emissions in China increased rapidly until 2006, and then decreased by
9.2 % to 30.8 Tg in 2010 due to the wide application of flue-gas
desulfurization (FGD) equipment in power plants (Lu et al.,
2011). Sulfur emissions in Europe have
decreased significantly during the last decades (Jones and Harrison, 2011).</p>
      <p>Most of the natural and anthropogenic SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is removed from the
atmosphere by liquid-phase oxidation to H<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>, and subsequent
precipitation. In areas with high sulfur loadings, acid rain leads to
acidification of soils and waters (Fig. 9). The main final sink of sulfur is
the oceans. A fraction of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is oxidized to H<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> in the gas
phase in a reaction chain initiated by the reaction of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with the
hydroxyl radical, OH. Especially in forested areas of Eurasia, reactions of
SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with a second important oxidant type, the stabilized Criegee
intermediates originating from biogenic VOC emissions, also produce
significant amounts of H<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> (Mauldin et al., 2012). Gas-phase
sulfuric acid plays a key role in the Earth's atmosphere by triggering
secondary aerosol formation, thus connecting anthropogenic SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions to global climate via aerosol–cloud interactions. Particles
containing sulfuric acid, or sulfate, are also connected with air quality
problems and human health deterioration. Understanding the spatial and
temporal evolution of SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions in northern Eurasia, along with
atmospheric sulfur chemistry, is crucial for understanding and quantifying
the impacts of anthropogenic activities and SO<inline-formula><mml:math display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions on air
quality, acidification as well as on regional and global climate.</p>
</sec>
</sec>
<sec id="Ch1.S4" sec-type="conclusions">
  <title>From system understanding to mitigation and adaptation strategies and
decision-making</title>
      <p>Climate change and weather extremes are already affecting the living
conditions of northern Eurasian societies. The vulnerability of the northern
environments and societies, including their adaptive capacity and buffering
thresholds, varies greatly depending on their current and future physical
environment as well as their demographic structure and economic activities.
The PEEX program as a whole is built on four pillars, namely (i) research,
(ii) research infrastructure, (iii) impact on society, and (iv) knowledge
transfer and capacity building. The scientific outcome of the first two
pillars will be addressing the future state of the physical environment and
its interactions and feedbacks with the demographic structure and economic
activities in the Arctic–boreal system. Periodic PEEX assessments will be
delivered for constructing mitigation and adaptation strategies of the
Northern societies and for use of regional and governmental decision-making.
The PEEX approach is applicable to China, when taking into account the
specific geographical, climatological, and social characteristics of that
region.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9"><caption><p>Schematic figure of the sulfur cycle.</p></caption>
        <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f09.jpg"/>

      </fig>

      <p>The integrative approach of the PEEX first two pillars provides both
analytical and operational answers to our research questions, which can be
utilized in solving interlinked grand challenges using pillars (iii) and
(iv). These will also contribute to the ESS questions as a whole (see ESS
questions: Schellnhuber et al., 2004). The implementation of the PEEX
research agenda starts with process studies in the frame of three main topics
determined for the land, atmosphere, aquatic, and social systems of the
northern Eurasian region. The research approach is designed to answer the
analytical questions on the major dynamical patters and feedback loops
relevant to Earth system science in the northern context. The PEEX program
has defined altogether 12 large-scale research questions for the 12 main
topics in the northern Eurasian domain (Kulmala et al., 2016). At the same
time, PEEX adheres to several operational ESS questions, including “what
level of complexity and resolution have to be achieved in Earth System
modelling?”, “what are the best techniques for analyzing and predicting
irregular events?”, “what might be the most effective global strategy for
generating, processing, and integrating relevant Earth system data sets?”,
and “what are the most appropriate methodologies for integrating natural
science and social science knowledge?”
(Schellnhuber et al., 2004).</p>
      <p>In terms of the level of complexity and resolution in Earth system modelling,
PEEX builds on a multi-scale modelling and observation approach originally
introduced by Kulmala et al. (2009). PEEX will construct its own multi-scale
modelling platform (Lappalainen et al., 2014). In terms of generating,
processing and integrating relevant Earth system data sets, a detailed
conceptual design of the PEEX research infrastructure (RI) will include a
concept design of a coherent in situ observation network, coordinated use of
remote sensing observations and standardized and harmonized data procedures
as well as a data system. One of the first tasks of PEEX-RI is to fill in the
observational gap in atmospheric in situ and ground base remote sensing data
in northern Eurasia, especially in Siberia. This approach is based not only
on the coordination of existing observation activities (Alekseychik et al.,
2016), but also on making plans for a new infrastructure needed. PEEX-RI
development will be largely based on the SMEAR (Station for Measuring
Ecosystem-Atmosphere Relations) concept (Kulmala et al., 2016), which has
been developed by the University of Helsinki Division of Atmospheric Sciences
together with Division of Forest Ecology starting from 1995 (Hari and
Kulmala, 2005; Hari et al., 2016). The SMEAR concept provides a
state-of-the-art foundation for establishing a PEEX observation system to be
integrated into the global GEOSS data system. Furthermore, detailed design of
greenhouse gas, aerosol, cloud, and trace gas measurements, and observation
of biological activity will find synergies with the major European
land–atmosphere observation infrastructures, such as ICOS (Integrated Carbon
Observations System; a research infrastructure to determine the greenhouse
gas balance of Europe and adjacent regions), ACTRIS (aerosols, clouds, and
trace gases research infrastructure), GAW (Global Atmospheric Watch), and
AnaEE (Infrastructure for Analysis and Experimentation on Ecosystems).</p>
      <p>PEEX is interested in developing methodologies for integrating natural
science and social science knowledge as part of the operational Earth
sustainable system questions (Schellnhuber et al., 2004). The first-priority
task in this case is to establish an integrated geographical information
background (Ribeiro et al., 2009; Shvidenko et al., 2010; Skryzhevska et al.,
2015). A common information background would be the first step serving the
development of a common language of integrated studies. For example, we need
spatially and temporally explicit descriptions of terrestrial ecosystems,
landscapes, atmosphere, and hydrosphere. A common information background
would be a unified base for the PEEX modelling platform and for the
development of integrated modelling clusters, which could combine ecological,
economic, and social dimensions. It could provide a historical background for
the future trajectories of land cover, state and resilience of ecosystems,
stability of landscapes, and dynamics of environmental indicators of
environment. The already exiting Integrated Land Information System could be
utilized here for combining all historical knowledge about the region and all
scientific results obtained by past, current, and future studies across the
region (Schepaschenko et al., 2011).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10"><caption><p>An example of the study approach to be implemented by PEEX for
integrating natural science and social science knowledge and generating
climate predictions and narratives of the northern regions.</p></caption>
        <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://acp.copernicus.org/articles/16/14421/2016/acp-16-14421-2016-f10.png"/>

      </fig>

      <p>In addition to data services, PEEX is developing procedures for integrating
and linking natural science and social science knowledge and data. As one
example, we need to analyse data on emission sources together with
population health risk factors, environment pollution, food security,
drinking water quality, changes in the spreading areas of infectious
diseases, and changes in the general epidemiological situation (Bityukova
and Kasimov, 2012; Malkhazova et al., 2013). Via novel multi-disciplinary
data interfaces and data procedures, we are able to connect satellite
observations with inverse modelling, provide fast updates to emission
inventories, estimate the emission for the climate models, and, in the end,
provide climate and air quality scenarios and the storylines of the future
development of the Arctic–boreal region (Fig. 10).</p>
      <p>In terms of strategic questions of the ESS, such as “what is the optimal mix
of adaptation and mitigation measures to respond global change?” or “what
is the structure of an effective and efficient system of global institutions
and development of institutions?”, PEEX is an active player in creating
direct contacts with the stakeholders, so that its scientific information and
services will receive an optimal impact on decision-making. Furthermore, the
PEEX approach endorses the Earth System Manifesto
(<uri>https://www.atm.helsinki.fi/peex/images/manifesti_peex_ru_hub2.pdf</uri>),
which addresses three strategic tasks: (i) construction of novel observation
systems, (ii) finding consensus addressing necessary mitigation and
adaptation actions in different parts of the world, and (iii) operational
prerequisites for technological development to moderate the global change
towards the sustainable Earth System. In this framework, PEEX will work
closely with influential organizations, such as the Intergovernmental Panel
for Climate Change (IPCC) delivering PEEX assessment of the Arctic–boreal
region, the future earth acting as an Arctic–boreal hub, and the digital
Earth via demonstrating novel methods for integrating in situ data with
satellite observations.</p>
</sec>
<sec id="Ch1.S5">
  <title>Data availability</title>
      <p>This paper is an overview of the current state of the art in selected
fields relevant to system understanding of the arctic–boreal regions. The
results and conclusions presented in this paper are based on the already
published peer reviewed papers. Their underlying research data can be
accessed via the information provided in the individual papers listed in the
references.</p>
</sec>

      
      </body>
    <back><ack><title>Acknowledgements</title><p>The preparatory work of the PEEX approach, started in 2012, has been mainly
based on the similar contribution of several European, Russian, and Chinese
research institutes. The work presented here would not have been possible
without the collaboration of the PEEX meetings participants. In 2012–2015 we
have organized five PEEX meetings in Helsinki (2012, 2015), Moscow (2013),
Hyytiälä (2013), and Saint Petersburg (2014), and the first PEEX
Science conference in Helsinki, Finland, in February 2015. PEEX has also been
active in a frame of international coordination activities and has as such
been listed as GEOSS – Gold region project, IGBP-iLEAPS Arctic and boreal
regional node, Digital Earth, Arctic Council – SAON Task, one of the main
collaborators of the International Eurasian Academy of Sciences (IEAS) and
Future Earth Arctic–boreal hub.</p><p>In addition, we would like acknowledge the support and funding from the
following bodies: Academy of Finland Centre of Excellence (grant no. 272041),
“International Working Groups, Markku Kulmala” grant by Finnish Cultural
Foundation; ICOS 271878, ICOS-Finland no. 281255, ICOS-ERIC no. 281250,
nos. 259537, 218094,
255576, 286685, 280700, and 259537 funded by Academy of Finland; Beautiful
Beijing project funded by TEKES, In GOS DEFROST, and CRAICC (no. 26060) and
Nordforsk CRAICC-PEEX (amendment to contact 26060) funded by Nordforsk.
“European-Russian Centre for cooperation in the Arctic and Sub-Arctic
environmental and climate research” (EuRuCAS, grant 295068); Erasmus<inline-formula><mml:math display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> CBHE
project ECOIMPACT 561975 funded by EU 7th Framework Program.</p><p>We thank many Russian projects, which have contributed to PEEX and have
been granted by national funding organizations: Russian Mega-Grant
no. 11.G34.31.0048 (University of Nizhny Novgorod), Russian Ministry of
Education and Science Grants (unique project identifiers RFMEFI58614X0004 and
RFMEFI58314X0003, ISR “AEROCOSMOS”, 2014–2016); Russian Science Foundation
projects no. 15-17-20009 (University of Nizhny Novgorod) and no. 15-17-30009
(Faculty of Geography, Moscow University, 2015–2018), RFBR grant
no. 14-05-91759 (ISR “AEROCOSMOS”, 2014–2016), Russian Science Foundation
projects nos. 14-47-00049 (A. M. Obukhov Institute of Atmospheric Physics
RAS, 2014–2016), 11.37.220.2016 (St.Petersburg State University) and
14-27-00083 (the Geochemical foundations of PEEX), 15-5554020 (SINP Moscow
University, 2015–2016), and 14-17-00096 (Saint-Petersburg State University,
2014–2016). We also acknowledge Presidium of the Russian Academy of Sciences
(program no. 4); the Branch of Geology, Geophysics and Mining Sciences of RAS
(program no. 5); interdisciplinary integration projects of the Siberian
Branch of the Russian Academy of Science nos. 35, 70, and 131; Russian
Foundation for Basic Research (grants nos. 14-05-00526, 14-05-00590,
14-05-93108) and Russian Science Foundation project no. 14-17-00096
(Saint-Petersburg State University, 2014–2016). AARI thanks CNTP 1.5.3.2 and
1.5.3.4 of Roshydromet. Institute of Geography thanks Russian Academy of
Sciences and Russian Science Foundation (project 14-27-00133).</p><p>University of Tartu together with University of Life Sciences, Estonia,
acknowledge the European Commission through European Regional Fund (the
“Internationalization of Science Programme” project INSMEARIN,
10.1-6/13/1028, and the “Estonian Research Infrastructures Roadmap”
project Estonian Environmental Observatory, 3.2.0304.11-0395). The
University of Tartu, Estonia, acknowledges the institutional research
funding IUT20-11 of the Estonian Ministry of Education and Research for its
support for the development of SMEAR Estonia at Järvselja. Nansen
Center, Norway, acknowledges the International Belmont Forum project
“Anthropogenic Heat Islands in the Arctic – Windows to the Future of the
Regional Climates, Ecosystems and Societies” no. 247468/E10.<?xmltex \hack{\newline}?><?xmltex \hack{\newline}?>
Edited by: I. Salma<?xmltex \hack{\newline}?>
Reviewed by: two anonymous referees</p></ack><ref-list>
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<abstract-html><p class="p">The northern Eurasian regions and Arctic Ocean will very likely
undergo substantial changes during the next decades. The Arctic–boreal
natural environments play a crucial role in the global climate via albedo
change, carbon sources and sinks as well as atmospheric aerosol production
from biogenic volatile organic compounds. Furthermore, it is expected that
global trade activities, demographic movement, and use of natural resources
will be increasing in the Arctic regions. There is a need for a novel
research approach, which not only identifies and tackles the relevant
multi-disciplinary research questions, but also is able to make a holistic
system analysis of the expected feedbacks. In this paper, we introduce the
research agenda of the Pan-Eurasian Experiment (PEEX), a multi-scale,
multi-disciplinary and international program started in 2012
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by which large-scale research topics are investigated from a system perspective
and which aims to fill the key gaps in our understanding of the feedbacks
and interactions between the land–atmosphere–aquatic–society continuum in
the northern Eurasian region. We introduce here the state of the art for the
key topics in the PEEX research agenda and present the future prospects of the
research, which we see relevant in this context.</p></abstract-html>
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