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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-14-9567-2014</article-id>
<title-group>
<article-title>Factors controlling temporal variability of near-ground atmospheric &lt;sup&gt;222&lt;/sup&gt;Rn concentration over central Europe</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Zimnoch</surname>
<given-names>M.</given-names>
<ext-link>https://orcid.org/0000-0002-0594-9376</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wach</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Chmura</surname>
<given-names>L.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Gorczyca</surname>
<given-names>Z.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rozanski</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Godlowska</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Mazur</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kozak</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Jeričević</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>AGH University of Science and Technology, Faculty of Physics and Applied Computer Science, Krakow, Poland</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Institute of Meteorology and Water Management, National Research Institute, Krakow Branch, Krakow, Poland</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>The Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences, Krakow, Poland</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Croatian Civil Aviation Agency, Zagreb, Croatia</addr-line>
</aff>
<pub-date pub-type="epub">
<day>16</day>
<month>09</month>
<year>2014</year>
</pub-date>
<volume>14</volume>
<issue>18</issue>
<fpage>9567</fpage>
<lpage>9581</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2014 M. Zimnoch et al.</copyright-statement>
<copyright-year>2014</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 3.0 Unported License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/3.0/">https://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/articles/14/9567/2014/acp-14-9567-2014.html">This article is available from https://acp.copernicus.org/articles/14/9567/2014/acp-14-9567-2014.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/14/9567/2014/acp-14-9567-2014.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/14/9567/2014/acp-14-9567-2014.pdf</self-uri>
<abstract>
<p>Concentration of radon (&lt;sup&gt;222&lt;/sup&gt;Rn) in the near-ground atmosphere has been measured
quasi-continuously from January 2005 to December 2009 at two continental
sites in Europe: Heidelberg (south-west Germany) and Krakow (southern
Poland). The atmosphere was sampled at ca. 30 and 20 m above
the local ground. Both stations were equipped with identical instruments.
Regular observations of &lt;sup&gt;222&lt;/sup&gt;Rn were supplemented by measurements of
surface fluxes of this gas in the Krakow urban area, using two different
approaches. The measured concentrations of &lt;sup&gt;222&lt;/sup&gt;Rn varied at both sites
in a wide range, from less than 2.0 Bq m&lt;sup&gt;−3&lt;/sup&gt; to approximately
40 Bq m&lt;sup&gt;−3&lt;/sup&gt; in Krakow and 35 Bq m&lt;sup&gt;−3&lt;/sup&gt; in Heidelberg. The mean &lt;sup&gt;222&lt;/sup&gt;Rn
content in Krakow, when averaged over the entire observation period, was 30%
higher than in Heidelberg (5.86 ± 0.09 and 4.50 ± 0.07 Bq m&lt;sup&gt;−3&lt;/sup&gt;, respectively). Distinct seasonality of &lt;sup&gt;222&lt;/sup&gt;Rn signal
is visible in the obtained time series of &lt;sup&gt;222&lt;/sup&gt;Rn concentration, with
higher values recorded generally during late summer and autumn. The surface
&lt;sup&gt;222&lt;/sup&gt;Rn fluxes measured in Krakow also revealed a distinct seasonality,
with broad maximum observed during summer and early autumn and minimum
during the winter. When averaged over a 5-year observation period, the
night-time surface &lt;sup&gt;222&lt;/sup&gt;Rn flux was equal to 46.8 ± 2.4 Bq m&lt;sup&gt;−2&lt;/sup&gt; h&lt;sup&gt;−1&lt;/sup&gt;. 
Although the atmospheric &lt;sup&gt;222&lt;/sup&gt;Rn levels at Heidelberg and
Krakow appeared to be controlled primarily by local factors, it was possible
to evaluate the &quot;continental effect&quot; in atmospheric &lt;sup&gt;222&lt;/sup&gt;Rn content
between both sites, related to gradual build-up of &lt;sup&gt;222&lt;/sup&gt;Rn concentration
in the air masses travelling between Heidelberg and Krakow. The mean value
of this build-up was equal to 0.78 ± 0.12 Bq m&lt;sup&gt;−3&lt;/sup&gt;. The measured minimum
&lt;sup&gt;222&lt;/sup&gt;Rn concentrations at both sites and the difference between them was
interpreted in the framework of a simple box model coupled with HYSPLIT
(Hybrid Single Particle Lagrangian Integrated Trajectory)
analysis of air mass trajectories. The best fit of experimental data was
obtained for the mean &lt;sup&gt;222&lt;/sup&gt;Rn flux over the European continent equal to
52 Bq m&lt;sup&gt;−2&lt;/sup&gt; h&lt;sup&gt;−1&lt;/sup&gt;, the mean transport velocity of the air masses within
the convective mixed layer of the planetary boundary layer (PBL) on their route from the Atlantic coast to
Heidelberg and Krakow equal to 3.5 m s&lt;sup&gt;−1&lt;/sup&gt;, the mean rate constant of
&lt;sup&gt;222&lt;/sup&gt;Rn removal across the top of the PBL equal to the &lt;sup&gt;222&lt;/sup&gt;Rn decay
constant and the mean height of the convective mixed layer equal to 1600 m.</p>
</abstract>
<counts><page-count count="15"/></counts>
</article-meta>
</front>
<body/>
<back>
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