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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-14-13631-2014</article-id>
<title-group>
<article-title>A global process-based study of marine CCN trends and variability</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dunne</surname>
<given-names>E. M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Mikkonen</surname>
<given-names>S.</given-names>
<ext-link>https://orcid.org/0000-0003-0595-0657</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kokkola</surname>
<given-names>H.</given-names>
<ext-link>https://orcid.org/0000-0002-1404-6670</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Korhonen</surname>
<given-names>H.</given-names>
<ext-link>https://orcid.org/0000-0001-6264-0706</ext-link>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Finnish Meteorological Institute, Atmospheric Research Centre of Eastern Finland, P.O. Box 1627, 70211 Kuopio, Finland</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>University of Eastern Finland, Department of Applied Physics, P.O. Box 1627, 70211 Kuopio, Finland</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Finnish Meteorological Institute, Climate Research, P.O. Box 503, 00101 Helsinki, Finland</addr-line>
</aff>
<pub-date pub-type="epub">
<day>19</day>
<month>12</month>
<year>2014</year>
</pub-date>
<volume>14</volume>
<issue>24</issue>
<fpage>13631</fpage>
<lpage>13642</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2014 E. M. Dunne et al.</copyright-statement>
<copyright-year>2014</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 3.0 Unported License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/3.0/">https://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/articles/14/13631/2014/acp-14-13631-2014.html">This article is available from https://acp.copernicus.org/articles/14/13631/2014/acp-14-13631-2014.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/14/13631/2014/acp-14-13631-2014.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/14/13631/2014/acp-14-13631-2014.pdf</self-uri>
<abstract>
<p>Low-level clouds have a strong climate-cooling effect in oceanic
      regions due to the much lower albedo of the underlying sea
      surface. Marine clouds typically have low droplet concentrations,
      making their radiative properties susceptible to changes in cloud
      condensation nucleus (CCN) concentrations. Here, we use the global
      aerosol model GLOMAP to investigate the processes that determine
      variations in marine CCN concentrations, and focus especially on the
      effects of previously identified wind speed trends in recent
      decades. Although earlier studies have found a link between linear
      wind speed trends and CCN concentration, we find that the effects of
      wind speed trends identified using a dynamic linear model in the
      Northern Equatorial Pacific (0.56 m s&lt;sup&gt;−1&lt;/sup&gt; per decade in the
      period 1990–2004) and the North Atlantic (−0.21 m s&lt;sup&gt;−1&lt;/sup&gt;
      per decade) are largely dampened by other processes controlling the
      CCN concentration, namely nucleation scavenging and transport of
      continental pollution. A CCN signal from wind speed change is seen
      only in the most pristine of the studied regions, i.e. over the
      Southern Ocean, where we simulate 3.4 cm&lt;sup&gt;−3&lt;/sup&gt; and
      0.17 m s&lt;sup&gt;−1&lt;/sup&gt; increases over the 15-year period in the
      statistical mean levels of CCN and wind speed, respectively. Our
      results suggest that future changes in wind-speed-driven aerosol
      emissions from the oceans can probably have a climate feedback via
      clouds only in the most pristine regions. On the other hand,
      a feedback mechanism via changing precipitation patterns and
      intensities could take place over most oceanic regions, as we have
      shown that nucleation scavenging has by far the largest absolute
      effect on CCN concentrations.</p>
</abstract>
<counts><page-count count="12"/></counts>
<funding-group>
<award-group id="gs1">
<funding-source></funding-source>
<award-id>Academy Research Fellowship 250348</award-id>
</award-group>
</funding-group>
</article-meta>
</front>
<body/>
<back>
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