<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "https://jats.nlm.nih.gov/nlm-dtd/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-13-5987-2013</article-id>
<title-group>
<article-title>Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Mailler</surname>
<given-names>S.</given-names>
<ext-link>https://orcid.org/0000-0002-4287-713X</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Khvorostyanov</surname>
<given-names>D.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Menut</surname>
<given-names>L.</given-names>
<ext-link>https://orcid.org/0000-0001-9776-0812</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Laboratoire de Météorologie Dynamique, UMR 8539 (École  Polytechnique, École Normale Supérieure, Université Paris 6,  École Nationale des Ponts et Chaussées), 91128 Palaiseau Cedex,  France</addr-line>
</aff>
<pub-date pub-type="epub">
<day>21</day>
<month>06</month>
<year>2013</year>
</pub-date>
<volume>13</volume>
<issue>12</issue>
<fpage>5987</fpage>
<lpage>5998</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2013 S. Mailler et al.</copyright-statement>
<copyright-year>2013</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 3.0 Unported License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/3.0/">https://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/articles/13/5987/2013/acp-13-5987-2013.html">This article is available from https://acp.copernicus.org/articles/13/5987/2013/acp-13-5987-2013.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/13/5987/2013/acp-13-5987-2013.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/13/5987/2013/acp-13-5987-2013.pdf</self-uri>
<abstract>
<p>Five one-year air quality simulations over a domain covering Europe have been
performed using the CHIMERE chemistry transport model and the EMEP emission
dataset for Europe. These five simulations differ only by the representation
of the effective emission heights for anthropogenic emissions: one has been
run using the EMEP standard recommendations, three others with vertical
injection profiles derived from the EMEP recommendations but multiplying the
injection height by 0.75, 0.50 and 0.25, respectively, while the last one
uses vertical profiles derived from the recent literature. It is shown that
using injection heights lower than the EMEP recommendations leads to
significantly improved simulation of background SO&lt;sub&gt;2&lt;/sub&gt;, NO&lt;sub&gt;2&lt;/sub&gt; and O&lt;sub&gt;3&lt;/sub&gt;
concentrations when compared to the Airbase station measurements.</p>
</abstract>
<counts><page-count count="12"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple">Bessagnet, B., Hodzic, A., Vautard, R., Beekmann, M., Cheinet, S., Honoré, C., Liousse, C., and Rouil, L.: Aerosol modeling with {CHIMERE}: preliminary evaluation at the continental scale, Atmos. Environ., 38, 2803–2817, 2004.</mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple">Bieser, J., Aulinger, A., Matthias, V., Quante, M., and Denier van&amp;nbsp;der Gon, H.: Vertical emission profiles for Europe based on plume rise calculations., Environ. Pollut., 159, 2935–2946, &lt;a href=&quot;http://dx.doi.org/10.1016/j.envpol.2011.04.030&quot;&gt;https://doi.org/10.1016/j.envpol.2011.04.030&lt;/a&gt;, 2011.</mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple">de Meij, A., Krol, M., Dentener, F., Vignati, E., Cuvelier, C., and Thunis, P.: The sensitivity of aerosol in Europe to two different emission inventories and temporal distribution of emissions, Atmos. Chem. Phys., 6, 4287–4309, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-6-4287-2006&quot;&gt;https://doi.org/10.5194/acp-6-4287-2006&lt;/a&gt;, 2006.</mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple">Derognat, C., Beekmann, M., Baeumle, M., Martin, D., and Schmidt, H.: Effect of biogenic volatile organic compound emissions on tropospheric chemistry during the Atmospheric Pollution Over the Paris Area({ESQUIF}) campaign in the Ile-de-France region, J. Geophys. Res., 108, 8560, 2003.</mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple">Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P. I., and Geron, C.: Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature), Atmos. Chem. Phys., 6, 3181–3210, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-6-3181-2006&quot;&gt;https://doi.org/10.5194/acp-6-3181-2006&lt;/a&gt;, 2006.</mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple">Honoré, C. and Vautard, R.: Photochemical regimes in urban atmospheres: The influence of dispersion, Geophys. Res. Lett., 27, 1895–1898, 2000.</mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple">Jöckel, P., Tost, H., Pozzer, A., Brühl, C., Buchholz, J., Ganzeveld, L., Hoor, P., Kerkweg, A., Lawrence, M. G., Sander, R., Steil, B., Stiller, G., Tanarhte, M., Taraborrelli, D., van Aardenne, J., and Lelieveld, J.: The atmospheric chemistry general circulation model ECHAM5/MESSy1: consistent simulation of ozone from the surface to the mesosphere, Atmos. Chem. Phys., 6, 5067–5104, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-6-5067-2006&quot;&gt;https://doi.org/10.5194/acp-6-5067-2006&lt;/a&gt;, 2006.</mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple">Mao, Q., Gautney, L.&amp;nbsp;L., Cook, T.&amp;nbsp;M., Jacobs, M.&amp;nbsp;E., Smith, S.&amp;nbsp;N., and Kelsoe, J.&amp;nbsp;J.: Numerical experiments on MM5-CMAQ sensitivity to various PBL schemes, Atmos. Environ., 40, 3092–3110, 2006.</mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple">Menut, L. and Bessagnet, B.: Atmospheric composition forecasting in Europe., Annals Geophys., 28, 61–74, 2010.</mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple">Menut, L., Vautard, R., Beekmann, M., and Honoré, C.: Sensitivity of Photochemical Pollution using the Adjoint of a Simplified Chemistry-Transport Model, J. Geophys. Res., 105, 15379–15402, 2000.</mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple">Menut, L., C.Schmechtig, and B.Marticorena: Sensitivity of the sandblasting fluxes calculations to the soil size distribution accuracy, J. Atmos. Ocean. Tech., 22, 1875–1884, 2005.</mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple">Menut, L., Bessagnet, B., Colette, A., and Khvorostiyanov, D.: On the impact of the vertical resolution on chemistry transport modelling, Atmos. Environ., 67, 370–384, 2012.</mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple">Menut, L., Bessagnet, B., Khvorostyanov, D., Beekman, M., Colette, A., Coll, I., Curci, G., Foret, G., Hodzic, A., Mailler, S., Meleux, F., Monge, J.-L., Pison, I., Turquety, S., Valari, M., Vautard, R., and Vivanco, M.&amp;nbsp;G.: Regional atmospheric composition modeling with CHIMERE version 2011, Geosci. Model Dev. Discuss., accepted, 2013.</mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple">Menut, L., Bessagnet, B., Khvorostyanov, D., Beekmann, M., Colette, A., Coll, I., Curci, G., Foret, G., Hodzic, A., Mailler, S., Meleux, F., Monge, J.-L., Pison, I., Turquety, S., Valari, M., Vautard, R., and Vivanco, M.&amp;nbsp;G.: Regional atmospheric composition modeling with CHIMERE, Geosci. Model Dev. Discuss., 6, 203–329, &lt;a href=&quot;http://dx.doi.org/10.5194/gmdd-6-203-2013&quot;&gt;https://doi.org/10.5194/gmdd-6-203-2013&lt;/a&gt;, 2013.</mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple">Michalakes, J., Dudhia, J., Gill, D., Henderson, T., Klemp, J., Skamarock, W., and Wang, W.: The Weather Research and Forecast Model: Software Architecture and Performance, To appear in proceeding of the Eleventh ECMWF Workshop on the Use of High Performance Computing in Meteorology, 25–29 October 2004, Reading, U.K., Ed. George Mozdzynski, 2004.</mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple">Pozzer, A., Jöckel, P., and Van Aardenne, J.: The influence of the vertical distribution of emissions on tropospheric chemistry, Atmos. Chem. Phys., 9, 9417–9432, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-9-9417-2009&quot;&gt;https://doi.org/10.5194/acp-9-9417-2009&lt;/a&gt;, 2009.</mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple">Pregger, T. and Friedrich, R.: Effective pollutant emission heights for atmospheric transport modelling based on real-world information, Environ. Pollut., 157, 552–560, 2009.</mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple">Schaap, M., Vautard, R., Bergstrom, R., van Loon, M., Bessagnet, B., Brandt, J., Christensen, H., Cuvelier, K., Foltescu, V., Graff, A., E., J.&amp;nbsp;J., Kerschbaumer, A., Krol, M., Langner, J., Roberts, P., Rouil, L., Stern, R., Tarrason, L., Thunis, P., Vignati, E., White, L., Wind, P., and Builtjes, P. H.&amp;nbsp;J.: Evaluation of long-term aerosol simulations from seven air quality models and their ensemble in the EURODELTA study, Atmos. Environ., 41, 2083–2097, 2007.</mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple">Simpson, D., Benedictow, A., Berge, H., Bergström, R., Emberson, L.&amp;nbsp;D., Fagerli, H., Flechard, C.&amp;nbsp;R., Hayman, G.&amp;nbsp;D., Gauss, M., Jonson, J.&amp;nbsp;E., Jenkin, M.&amp;nbsp;E., Nyiri, A., Richter, C., Semeena, V.&amp;nbsp;S., Tsyro, S., Tuovinen, J.-P., Valdebenito, A., and Wind, P.: The EMEP MSC-W chemical transport model - technical description, Atmos. Chem. Phys., 12, 7825–7865, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-12-7825-2012&quot;&gt;https://doi.org/10.5194/acp-12-7825-2012&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple">Skamarock, W. and Klemp, J.: A time-split nonhydrostatic atmospheric model for weather research and forecasting applications., J. Comput. Phys., 227, 3465–3485, &lt;a href=&quot;http://dx.doi.org/10.1016/j.jcp.2007.01.037&quot;&gt;https://doi.org/10.1016/j.jcp.2007.01.037&lt;/a&gt;, 2008.</mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple">Solazzo, E., Bianconi, R., Vautard, R., Appel, K.&amp;nbsp;W., Moran, M.&amp;nbsp;D., Hogrefe, C., Bessagnet, B., Brandt, J., Christensen, J.&amp;nbsp;H., Chemel, C., Coll, I., van&amp;nbsp;der Gon, H.&amp;nbsp;D., Ferreira, J., Forkel, R., Francis, X.&amp;nbsp;V., Grell, G., Grossi, P., Hansen, A.&amp;nbsp;B., Jeričević, A., Kraljević, L., Miranda, A.&amp;nbsp;I., Nopmongcol, U., Pirovano, G., Prank, M., Riccio, A., Sartelet, K.&amp;nbsp;N., Schaap, M., Silver, J.&amp;nbsp;D., Sokhi, R.&amp;nbsp;S., Vira, J., Werhahn, J., Wolke, R., Yarwood, G., Zhang, J., Rao, S., and Galmarini, S.: Model evaluation and ensemble modelling of surface-level ozone in Europe and North America in the context of AQMEII, Atmos. Environ., 53, 60–74, &lt;a href=&quot;http://dx.doi.org/10.1016/j.atmosenv.2012.01.003&quot;&gt;https://doi.org/10.1016/j.atmosenv.2012.01.003&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple">Van&amp;nbsp;Leer, B.: T}owards the ultimate conservative difference scheme. {V A second order sequel to Godunov&apos;s method, J. Computational Phys., 32, 101–136, 1979.</mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple">Van&amp;nbsp;Loon, M., Vautard, R., Schaap, M., Bergstrom, R., Bessagnet, B., Brandt, J., Builtjes, P., Christensen, J.&amp;nbsp;H., Cuvelier, K., Graf, A., Jonson, J., Krol, M., Langner, J., Roberts, P., Rouil, L., Stern, R., Tarrason, L., Thunis, P., Vignati, E., White, L., and Wind, P.: Evaluation of long-term ozone simulations from seven regional air quality models and their ensemble average, Atmos. Environ., 41, 2083–2097, 2007.</mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple">Vautard, R., Beekmann, M., Roux, J., and Gombert, D.: Validation of a hybrid forecasting system for the ozone concentrations over the Paris area, Atmos. Environ., 35, 2449–2461, 2001.</mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple">Vautard, R., Bessagnet, B., Chin, M., and Menut, L.: On the contribution of natural Aeolian sources to particulate matter concentrations in Europe: testing hypotheses with a modelling approach, Atmos. Environ., 39, 3291–3303, 2005.</mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple">Vautard, R., Builtjes, P. H.&amp;nbsp;J., Thunis, P., Cuvelier, K., Bedogni, M., Bessagnet, B., Honoré C., Moussiopoulos, N., G., P., Schaap, M., Stern, R., Tarrason, L., and Van&amp;nbsp;Loon, M.: Evaluation and intercomparison of Ozone and {PM}10 simulations by several chemistry-transport models over 4 European cities within the City-Delta project, Atmos. Environ., 41, 173–188, 2007.</mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple">Vestreng, V.: Review and revision of emission data reported to CLRTAP, Tech. rep., EMEP, Oslo, Norway, 2003.</mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple">Vestreng, V., Ntziachristos, L., Semb, A., Reis, S., Isaksen, I. S. A., and Tarrasón, L.: Evolution of NO&lt;sub&gt;x&lt;/sub&gt; emissions in Europe with focus on road transport control measures, Atmos. Chem. Phys., 9, 1503–1520, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-9-1503-2009&quot;&gt;https://doi.org/10.5194/acp-9-1503-2009&lt;/a&gt;, 2009.</mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple">Zhang, Y., Bocquet, M., Mallet, V., Seigneur, C., and Baklanov, A.: Real-time air quality forecasting, part I: History, techniques, and current status, Atmos. Environ., 60, 632–655, 2012.</mixed-citation>
</ref>
</ref-list>
</back>
</article>