<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "https://jats.nlm.nih.gov/nlm-dtd/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-13-11403-2013</article-id>
<title-group>
<article-title>An inverse modeling method to assess the source term of the Fukushima Nuclear Power Plant accident using gamma dose rate observations</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Saunier</surname>
<given-names>O.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Mathieu</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Didier</surname>
<given-names>D.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Tombette</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Quélo</surname>
<given-names>D.</given-names>
<ext-link>https://orcid.org/0000-0003-3949-6202</ext-link>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Winiarek</surname>
<given-names>V.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Bocquet</surname>
<given-names>M.</given-names>
<ext-link>https://orcid.org/0000-0003-2675-0347</ext-link>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Institut de Radioprotection et de Sûreté Nucléaire (IRSN), PRP-CRI, SESUC, BMTA, Fontenay-aux-Roses, 92262, France</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>CEREA, Joint Laboratory École des Ponts ParisTech and EDF R&amp;D, Champs-sur-Marne, France</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>INRIA, Paris-Rocquencourt research center, France</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>now at: BERTIN Technologies, Montigny-le-Bretonneux, France</addr-line>
</aff>
<pub-date pub-type="epub">
<day>25</day>
<month>11</month>
<year>2013</year>
</pub-date>
<volume>13</volume>
<issue>22</issue>
<fpage>11403</fpage>
<lpage>11421</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2013 O. Saunier et al.</copyright-statement>
<copyright-year>2013</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 3.0 Unported License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/3.0/">https://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/articles/13/11403/2013/acp-13-11403-2013.html">This article is available from https://acp.copernicus.org/articles/13/11403/2013/acp-13-11403-2013.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/13/11403/2013/acp-13-11403-2013.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/13/11403/2013/acp-13-11403-2013.pdf</self-uri>
<abstract>
<p>The Chernobyl nuclear accident, and more recently the Fukushima accident,
highlighted that the largest source of error on consequences assessment is
the source term, including the time evolution of the release rate and its
distribution between radioisotopes. Inverse modeling methods, which combine
environmental measurements and atmospheric dispersion models, have proven
efficient in assessing source term due to an accidental situation (Gudiksen,
1989; Krysta and Bocquet, 2007; Stohl et al., 2012a; Winiarek et al.,
2012). Most existing approaches are designed to use air sampling
measurements (Winiarek et al., 2012) and some of them also use deposition
measurements (Stohl et al., 2012a; Winiarek et al., 2014). Some studies
have been performed to use dose rate measurements (Duranova et al., 1999;
Astrup et al., 2004; Drews et al., 2004; Tsiouri et al., 2012) but none
of the developed methods were carried out to assess the complex source term
of a real accident situation like the Fukushima accident. However, dose rate
measurements are generated by the most widespread measurement system, and in
the event of a nuclear accident, these data constitute the main source of
measurements of the plume and radioactive fallout during releases. This
paper proposes a method to use dose rate measurements as part of an inverse
modeling approach to assess source terms.
&lt;br&gt;&lt;br&gt;
The method is proven efficient and reliable when applied to the accident at
the Fukushima Daiichi Nuclear Power Plant (FD-NPP). The emissions for the
eight main isotopes &lt;sup&gt;133&lt;/sup&gt;Xe, &lt;sup&gt;134&lt;/sup&gt;Cs, &lt;sup&gt;136&lt;/sup&gt;Cs, &lt;sup&gt;137&lt;/sup&gt;Cs,
&lt;sup&gt;137m&lt;/sup&gt;Ba, &lt;sup&gt;131&lt;/sup&gt;I, &lt;sup&gt;132&lt;/sup&gt;I and &lt;sup&gt;132&lt;/sup&gt;Te have been assessed.
Accordingly, 105.9 PBq of &lt;sup&gt;131&lt;/sup&gt;I, 35.8 PBq of &lt;sup&gt;132&lt;/sup&gt;I, 15.5 PBq of
&lt;sup&gt;137&lt;/sup&gt;Cs and 12 134 PBq of noble gases were released. The events
at FD-NPP (such as venting, explosions, etc.) known to have caused
atmospheric releases are well identified in the retrieved source term. The
estimated source term is validated by comparing simulations of atmospheric
dispersion and deposition with environmental observations. In total, it was
found that for 80% of the measurements, simulated and observed dose
rates agreed within a factor of 2. Changes in dose rates over time have been
overall properly reconstructed, especially in the most contaminated areas to
the northwest and south of the FD-NPP. A comparison with observed atmospheric
activity concentration and surface deposition shows that the emissions of
caesiums and &lt;sup&gt;131&lt;/sup&gt;I are realistic but that &lt;sup&gt;132&lt;/sup&gt;I and &lt;sup&gt;132&lt;/sup&gt;Te are
probably underestimated and noble gases are likely overestimated. Finally, an
important outcome of this study is that the method proved to be perfectly
suited to emergency management and could contribute to improve emergency
response in the event of a nuclear accident.</p>
</abstract>
<counts><page-count count="19"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple">Abida, R. and Bocquet, M.: Targeting of observations for accidental atmospheric release monitoring, Atmos. Environ., 43, 6312–6327, 2009.</mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple">Astrup, P., Turcanu, C., Puch, R., Palma, C. R., and Mikkelsen, T.: Data assimilation in the early phase: Kalman filtering RIMPUFF, Riso National Laboratory report Riso-R-1466(EN), 2004.</mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple">Baklanov, B. and Sørensen, J. H.: Parameterisation of radionuclides deposition in atmospheric long-range transport modelling, Phys. Chem. Earth, B26, 787–799, 2001.</mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple">Boutahar, J., Lacour, S., Mallet, V., Quelo, D., Roustan, Y., and Sportisse, B.: Development and validation of a fully modular platform for numerical modelling of air pollution: POLAIR, Int. J. Environ. Poll., 22, 17–28, 2004.</mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple">Chino, M., Nakayama, H., Nagai, H., Terada, H., Katata G., and Yamazawa, H.: Preliminary estimation of release amounts of &lt;sup&gt;131&lt;/sup&gt;I and &lt;sup&gt;137&lt;/sup&gt;Cs accidentally discharged from the Fukushima Daiichi Nuclear power plant into atmosphere, J. Nucl. Sci. Technol., 48, 1129–1134, 2011.</mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple">Davoine, X. and Bocquet, M.: Inverse modelling-based reconstruction of the Chernobyl source term available for long-range transport, Atmos. Chem. Phys., 7, 1549–1564, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-7-1549-2007&quot;&gt;https://doi.org/10.5194/acp-7-1549-2007&lt;/a&gt;, 2007.</mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple">Devell, L., Güntay, S., and Powers, D. A.: The Chernobyl Reactor Accident Source Term: Development of a Consensus View, CSNI Report, Organisation for Economic Co-Operation and Development (OECD), OCDE/GD(96)12, 1995.</mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple">Drews, M., Lauritzen, B., Madsen, H., and Smith, J. Q.: Kalman filtration of radiation monitoring data from atmospheric dispersion of radioactive materials, Radiation Protection Dosimetry, 111, 257–269, 2004.</mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple">Duranova, T., Bohunova, J., Bohun, L., Duran, J. and Stubna M.: Source term estimation based on gamma dose rates measured by on-line on-site monitoring network, RODOS report RODOS(WG5)-TN(98)-01, &lt;a href=&quot;http://www.rodos.fzk.de/Documents/Public/CD1/WG5_CD1_General/WG5_TN98_01.pdf&quot;&gt;http://www.rodos.fzk.de/Documents/Public/CD1/WG5_CD1_General/WG5_TN98_01.pdf&lt;/a&gt;,1999.</mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple">Enting, I. G.: Inverse Problems in Atmospheric Constituent Transport, Cambridge Univ. Press, Cambridge, UK, 392 pp., 2002.</mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple">Fukushima Prefecture: &lt;a href=&quot;http://www.pref.fukushima.jp/j/7houbu0311-0331.pdf&quot;&gt;http://www.pref.fukushima.jp/j/7houbu0311-0331.pdf&lt;/a&gt; (in Japanese, last access: 2 December 2011), 2011a.</mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple">Fukushima Prefecture: &lt;a href=&quot;http://www.pref.fukushima.jp/j/20-50km0315-0331.pdf&quot;&gt;http://www.pref.fukushima.jp/j/20-50km0315-0331.pdf&lt;/a&gt; (last access: 21 July 2011), 2011b.</mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple">Furuta, S., Sumiya, S., Watanabe, H., Nakano, M., Imaizumi, K., Takeyasu, M., Nakada, A., Fujita, H., Mizutani, T., Morisawa, M., Kokubun, Y., Kono, T., Nagaoka, M., Yokoyama, H., Hokama, T., Isozaki, T., Nemoto, M., Hiyama, Y., Onuma, T., Kato, C., and Kurachi, T.: Results of the Environmental Radiation Monitoring Following the Accident at the Fukushima Daiichi Nuclear Power Plant – Interim Report (Ambient Radiation Dose Rate, Radioactivity Concentration in the Air and Radioactivity Concentration in the Fallout), Radiation Protection Department, Nuclear Fuel Cycle Engineering Laboratories, Tokai Research and Development Center, Japan Atomic Energy Agency, JAEA-Review 2011-035, 2011.</mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple">Gudiksen, P. H., Harvey, T. F., and Lange, R.: Chernobyl Source Term, Atmospheric Dispersion, and Dose Estimation, Health Phys., 57, 697–706, 1989.</mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple">IAEA (International Atomic Energy Agency): Fukushima monitoring data base &lt;a href=&quot;https://iec.iaea.org/fmd/search_by_dataset.aspx&quot;&gt;https://iec.iaea.org/fmd/search_by_dataset.aspx&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple">IRSN (Institut de Radioprotection et de S\^ureté nucléaire): Fukushima, One Year Later: Initial Analyses of the Accident and Its Consequences, IRSN Report IRSN/DG/2012-003, &lt;a href=&quot;http://www.irsn.fr/EN/publications/technical-publications/Documents/IRSN_Fukushima-1-year-later_2012-003.pdf&quot;&gt;http://www.irsn.fr/EN/publications/technical-publications/Documents/IRSN_Fukushima-1-year-later_2012-003.pdf&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple">Isnard, O.: C3X une nouvelle plateforme d&apos;évaluation des conséquences d&apos;un rejet atmosphérique, Report, IRSN/DEI/SESUC/06-41, 2006.</mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple">Katata, G., Terada, H., Nagai, H., and Chino, M.: Numerical reconstruction of high dose rate zones due to the Fukushima Dai-ichi Nuclear Power Plant accident, J. Environ. Radioact., 111, 2–12, &lt;a href=&quot;http://dx.doi.org/10.1016/j.jenvrad.2011.09.011&quot;&gt;https://doi.org/10.1016/j.jenvrad.2011.09.011&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple">KEK (High Energy Accelerator Research Organization): &lt;a href=&quot;http://rcwww.kek.jp/norm/index-e.html&quot;&gt;http://rcwww.kek.jp/norm/index-e.html&lt;/a&gt; (last access: 2 December 2011), 2011.</mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple">Korsakissok, I., Mathieu, A., and Didier, D.: Atmospheric dispersion and ground deposition induced by the Fukushima Nuclear Power Plant accident: A local-scale simulation and sensitivity study, Atmos. Environ.,  70, 267–279, &lt;a href=&quot;http://dx.doi.org/10.1016/j.atmosenv.2013.01.002&quot;&gt;https://doi.org/10.1016/j.atmosenv.2013.01.002&lt;/a&gt;, 2013.</mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple">Krysta, M. and Bocquet, M.: Source reconstruction of an accidental radionuclide release at European scale, Q. J. Roy. Meteorol. Soc.,  133, 529–544, 2007.</mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple">Krysta, M., Bocquet, M., and Brandt, J.: Probing ETEX-II data set with inverse modelling, Atmos. Chem. Phys., 8, 3963–3971, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-8-3963-2008&quot;&gt;https://doi.org/10.5194/acp-8-3963-2008&lt;/a&gt;, 2008.</mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple">Liu, D. C. and Nocedal, J.: On the limited memory method for large scale optimization, Math. Program. B., 45, 503–528, 1989.</mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple">Louis, J. F.: A parametric model of vertical eddy fluxes in the atmosphere, Bound.-Layer Meteorol., 17, 187–202, 1979.</mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple">Mathieu, A., Korsakissok, I., Quelo, D., Groell, J., Tombette, M., Didier, D., Quentric, E., Saunier, O., Benoit, J.-P., and Isnard, O.: Atmospheric dispersion and deposition of radionuclides from the Fukushima Daiichi nuclear power plant accident, Elements, 8, 195–200, 2012.</mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple">MEXT (Ministry of Education, Culture, Sports, Science and Technology): Reading of Environmental Radioactivity Level by Prefecture, available at: &lt;a href=&quot;http://radioactivity.mext.go.jp/en/list/192/list-1.html&quot;&gt;http://radioactivity.mext.go.jp/en/list/192/list-1.html&lt;/a&gt; (last access: 4 May 2012), 2011a.</mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple">MEXT (Ministry of Education, Culture, Sports, Science and Technology): Readings of Dust Sampling, available at: &lt;a href=&quot;http://radioactivity.mext.go.jp/en/list/200/list-1.html&quot;&gt;http://radioactivity.mext.go.jp/en/list/200/list-1.html&lt;/a&gt; (last access: 4 May 2012), 2011b.</mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple">MEXT (Ministry of Education, Culture, Sports, Science and Technology): Reading of Radioactivity Level in Fallout by Prefecture, available at: &lt;a href=&quot;http://radioactivity.mext.go.jp/en/list/194/list-1.html&quot;&gt;http://radioactivity.mext.go.jp/en/list/194/list-1.html&lt;/a&gt; (last access: 4 May 2012), 2011c.</mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple">MEXT (Ministry of Education, Culture, Sports, Science and Technology) Results of the Fourth Airborne Monitoring Survey by MEXT. MEXT Report, Ministry of Education, Culture, Sport, Sciences and Technology – Japan, December 16, 2011d.</mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple">MEXT (Ministry of Education, Culture, Sports, Science and Technology) and DOE (U.S. Department of Energy): MEXT and DOE Airborne Monitoring, (accessed 04.05.12.) http://radioactivity.mext.go.jp/en/list/203/list-1.html, 2011.</mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple">Miyagi Prefecture: available at: &lt;a href=&quot;http://www.pref.miyagi.jp/gentai/Press/PressH230315-3(sokutei).html&quot;&gt;http://www.pref.miyagi.jp/gentai/Press/PressH230315-3(sokutei).html&lt;/a&gt; (in Japanese) (last access: 4 May 2012), 2011.</mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple">Nagaoka, K., Sato, S., Araki, S., Ohta, Y., and Ikeuchi Y.: Changes of radionuclides in the environment in Chiba, Japan, after the Fukushima nuclear power plant accident, Health Phys., 102, 437–442, &lt;a href=&quot;http://dx.doi.org/10.1097/HP.0b013e31823bc2d3&quot;&gt;https://doi.org/10.1097/HP.0b013e31823bc2d3&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple">Quelo, D., Krysta, M., Bocquet, M., Isnard, O., Minier, Y. and Sportisse, B.: Validation of the Polyphemus platform on the ETEX, Chernobyl and Algeciras cases, Atmos. Environ., 41, 5300–5315, 2007.</mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple">Stohl, A., Seibert, P., Wotawa, G., Arnold, D., Burkhart, J. F., Eckhardt, S., Tapia, C., Vargas, A., and Yasunari, T. J.: Xenon-133 and caesium-137 releases into the atmosphere from the Fukushima Dai-ichi nuclear power plant: determination of the source term, atmospheric dispersion, and deposition, Atmos. Chem. Phys., 12, 2313–2343, &lt;a href=&quot;http://dx.doi.org/10.5194/acp-12-2313-2012&quot;&gt;https://doi.org/10.5194/acp-12-2313-2012&lt;/a&gt;, 2012a.</mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple">Stohl, A., Seibert, P., and Wotawa G.: The total release of xenon-133 from the Fukushima Dai-ichi nuclear power plant accident, J. Environ. Radioact. 112, 155–159, &lt;a href=&quot;http://dx.doi.org/10.1016/j.jenvrad.2012.06.001&quot;&gt;https://doi.org/10.1016/j.jenvrad.2012.06.001&lt;/a&gt;, 2012b.</mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple">TEPCO (Tokyo Electric Power Company): Estimation of Radioactive Material Released to the Atmosphere during the Fukushima Daiichi NPS Accident, &lt;a href=&quot;http://www.tepco.co.jp/en/press/corp-com/release/betu12_e/images/120524e0205.pdf&quot;&gt;http://www.tepco.co.jp/en/press/corp-com/release/betu12_e/images/120524e0205.pdf&lt;/a&gt; (last access: 15 November 2013), May 2012.</mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple">Terada, H., Katata, G., Chino, M., and Nagai, H.: Atmospheric discharge and dispersion of radionuclides during the Fukushima Dai-ichi Nuclear Power plant accident. Part II: verification of the source term and analysis of regional-scale atmospheric dispersion, J. Environ. Radioact., 112, 141–154, 2012.</mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple">Tikhonov, A. N. and Glasko, V. B.: Use of the regularization method in non-linear problems, USSR Comp. Math. Math. Phys., 5/3, 93–107, 1965.</mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple">Tochigi Prefecture: &lt;a href=&quot;http://www.pref.tochigi.lg.jp/kinkyu/documents/20110312-18.pdf&quot;&gt;http://www.pref.tochigi.lg.jp/kinkyu/documents/20110312-18.pdf&lt;/a&gt; (in Japanese) (last access: 2 December 2011), 2011.</mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple">Tsuruta, H., Oura, Y., Ebihara, M., Ohara, T., and Nakajima T.: Hourly atmospheric concentrations of Cs-134 and Cs-137 at monitoring stations for suspended particulate matter in and south of Fukushima after the Fukushima Daiichi Nuclear Power Plant accident, European Geosciences Union General Assembly, Vienna, Austria, 7–12 April 2013.</mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple">Troen, I. B. and Mahrt, L.: A simple model of the atmospheric boundary layer; sensitivity to surface evaporation, Bound.-Layer Meteorol., 37, 129–148, 1986.</mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple">Tsiouri, V., Kovalets, I., Andronopoulos, S., and Bartzis, J. G.: Emission rate estimation through data assimilation of gamma dose measurements in a lagrangian atmospheric dispersion model, Rad. Protect. Dosimetr.,  148, 34–44, 2012.</mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple">US DOE/NNSA: Response to 2011 Fukushima Incident – Raw Aerial Data and Extracted Ground Exposure, &lt;a href=&quot;https://explore.data.gov/Geography-and-Environment/US-DOE-NNSA-Response-to-2011-Fukushima-Incident-Ra/prrn-6s35&quot;&gt;https://explore.data.gov/Geography-and-Environment/US-DOE-NNSA-Response-to-2011-Fukushima-Incident-Ra/prrn-6s35&lt;/a&gt;, 2011.</mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple">Winiarek, V., Vira, J., Bocquet, M., Sofiev, M., and Saunier, O.: Towards the operational estimation of a radiological plume using data assimilation after a radiological accidental atmospheric release, Atmos. Environ., 45, 2944–2955, 2011.</mixed-citation>
</ref>
<ref id="ref45">
<label>45</label><mixed-citation publication-type="other" xlink:type="simple">Winiarek, V., Bocquet, M., Saunier, O., and Mathieu, A.: Estimation of errors in the inverse modeling of accidental release of atmospheric pollutant: application to the reconstruction of the cesium-137 and iodine-131 source terms from the Fukushima Daiichi power plant, J. Geophys. Res., 117, D05122, &lt;a href=&quot;http://dx.doi.org/10.1029/2011JD016932&quot;&gt;https://doi.org/10.1029/2011JD016932&lt;/a&gt;, 2012.</mixed-citation>
</ref>
<ref id="ref46">
<label>46</label><mixed-citation publication-type="other" xlink:type="simple">Winiarek, V., Bocquet, M., Duhanyan, N., Roustan, Y., Saunier, O., and Mathieu, A.: Estimation of the caesium-137 source term from the Fukushima Daiichi nuclear power plant using a consistent joint assimilation of air concentration and deposition observations, Atmos. Environ., 82, 268–279, &lt;a href=&quot;http://dx.doi.org/10.1016/j.atmosenv.2013.10.017&quot;&gt;https://doi.org/10.1016/j.atmosenv.2013.10.017&lt;/a&gt;, 2014.</mixed-citation>
</ref>
</ref-list>
</back>
</article>