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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
<abbrev-journal-title abbrev-type="nlm-ta">Atmos. Chem. Phys.</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus Publications</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-10-2475-2010</article-id>
<title-group>
<article-title>Linking urban aerosol fluxes in street canyons to larger scale emissions</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Tay</surname>
<given-names>B. K.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>McFiggans</surname>
<given-names>G. B.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Jones</surname>
<given-names>D. P.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Gallagher</surname>
<given-names>M. W.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Martin</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Watkins</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Harrison</surname>
<given-names>R. M.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Centre for Atmospheric Science, SEAES, The University of Manchester, Manchester, M13 9PL, UK</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>School of Mechanical, Aerospace and Civil Engineering, The University of Manchester, P.O. Box 88, Manchester M60 1QD, UK</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Division of Environmental Health &amp; Risk Management, School of Geography, Earth &amp; Environmental Sciences, University of Birmingham, Edgbaston, Birmingham B15 2TT, UK</addr-line>
</aff>
<pub-date pub-type="epub">
<day>11</day>
<month>03</month>
<year>2010</year>
</pub-date>
<volume>10</volume>
<issue>5</issue>
<fpage>2475</fpage>
<lpage>2490</lpage>
<permissions>
<copyright-statement>Copyright: &#x000a9; 2010 B. K. Tay et al.</copyright-statement>
<copyright-year>2010</copyright-year>
<license license-type="open-access">
<license-p>This work is licensed under the Creative Commons Attribution 3.0 Unported License. To view a copy of this licence, visit <ext-link ext-link-type="uri"  xlink:href="https://creativecommons.org/licenses/by/3.0/">https://creativecommons.org/licenses/by/3.0/</ext-link></license-p>
</license>
</permissions>
<self-uri xlink:href="https://acp.copernicus.org/articles/10/2475/2010/acp-10-2475-2010.html">This article is available from https://acp.copernicus.org/articles/10/2475/2010/acp-10-2475-2010.html</self-uri>
<self-uri xlink:href="https://acp.copernicus.org/articles/10/2475/2010/acp-10-2475-2010.pdf">The full text article is available as a PDF file from https://acp.copernicus.org/articles/10/2475/2010/acp-10-2475-2010.pdf</self-uri>
<abstract>
<p>In this study we investigate ultrafine particle (UFP) fluxes using a first
order eddy viscosity turbulence closure Computational Fluid Dynamics (CFD)
model and determine the different factors that influence emissions of UFP
into the urban boundary layer. Both vertical turbulent fluxes as well as the
fluxes due to mean circulatory flow are shown to contribute to the overall
ventilation characteristics of street canyons. We then derive a simple
parameterised numerical prediction model for canyon top UFP venting which is
then compared with tower based micrometeorological flux measurements
obtained during the REPARTEE &amp; CityFlux field experiments.</p>
</abstract>
<counts><page-count count="16"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple">Baik, J. J. and Kim, J. J.: A numerical study of flow and pollutant dispersion characteristics in urban street canyons, J. Appl. Meteorol., 38, 1576–1589, 1999.</mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple">Baik, J. J. and Kim, J. J.: On the escape of pollutants from urban street canyons, Atmos. Environ., 36, 527–536, 2002.</mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple">Baik, J. J. and Kim, J. J.: Effects of inflow turbulence intensity on flow and pollutant dispersion in an urban street canyon, J. Wind Eng. Ind. Aerodynam., 91, 309–329, 2003.</mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple">Barlow, J. F. and Belcher, S. E.: A wind tunnel model for quantifying fluxes in the urban boundary layer, Bound.-Lay. Meteorol., 104, 131–150, 2002.</mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple">Belcher, S. E.: Mixing and transport in urban areas, Phil. Trans. Roy. Soc., 363, 2947–2968, 2005.</mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple">Chan, T. L., Dong, G., Leung, C. W., Cheung, C. S., and Hung, W. T.: Validation of a two-dimensional pollutant dispersion model in an isolated street canyon, Atmos. Environ., 36, 861–872, 2002.</mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple">Dall&apos;Osto, M., Harrison, R. M., Thorpe, A., Williams, P. and Coe, H.: Remarkable dynamics of nanoparticle in the urban atmosphere, European Aerosol Conference 2009, Karlsruhe, Germany, Abstract T130A06, 2009.</mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple">DePaul, F. T. and Sheih, C. M.: A tracer study of dispersion in an urban street canyon, Atmos. Environ., 19, 555–559, 1985.</mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple">Dixon, N. S. and Tomlin A. S.: Evaluation of a lagrangian model for predicting concentration fluctuations in urban areas, Proceedings 11&lt;i&gt;&lt;sup&gt;th&lt;/sup&gt;&lt;/i&gt; International Conference on Harmonization within Atmospheric Dispersion Modelling for Regulatory Purposes, 2007.</mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple">Dorsey, J. R., Nemitz, E., Gallagher, M. W., Fowler, D., Williams, P. I., Bower, K. N., and Beswick, K. M.: Direct measurements and parameterisation of aerosol flux, concentration and emission velocity above a city, Atmos. Environ., 36, 791–800, 2002.</mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple">Ferziger, J. H. and Peric, M.: Computational Methods for Fluid Dynamics (3rd Edition), Springer-Verlag, Berlin, Heidelberg, Germany, 423 pp., 2001.</mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple">Flesch, T. K.: Turbulent Schmidt number from a tracer experiment, Agr. Forest Meteorol., 111, 299–307, 2002.</mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple">Foken, T.: Micrometeorology, Springer-Verlag, Berlin, Berlin, 306 pp., 2006.</mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple">Gallis, M. A., Torczynski, J. R., and Rader, D. J.: Nonzero-concentration boundary condition for advection-diffusion aerosol-transport modeling, Aerosol Sci. Technol., 42, 829–831, 2008.</mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple">Hunter, L. J., Johnson, G. T., and Watson, I. D.: An investigation of three dimensional characteristics of flow regimes within the urban canyon, Atmos. Environ., 26B, 425–432, 1992.</mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple">Jeong, S. J. and Andrew, M. J.: Application of the k-epsilon turbulence model to high reynolds number skimming flow field of an urban street canyon, Atmos. Environ., 36, 1137–1145, 2002.</mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple">Johnson, J. T. and Hunter, L. J.: Some insights into typical urban canyon airflows, Atmos. Environ., 33, 3991–3999, 1999.</mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple">Ketzel, K., Louka, P., Sahm, P., Guilloteau, E., and Sini, J.-F.: The use of computational fluid dynamics in modelling air quality in street canyons in Optimisation of Modelling Methods for Traffic Pollution in Street, Final Report for EU Trapos Project,  edited by:  Berkowicz, R., Britter, R., and Sabatino, S. D.,  Chapter 2.2, 86–93, available online at: &lt;a href=&quot;http://www2.dmu.dk/AtmosphericEnvironment/trapos/TheBook/TRAPOS_Book.pdf&quot;&gt;http://www2.dmu.dk/AtmosphericEnvironment/trapos/TheBook/TRAPOS_Book.pdf&lt;/a&gt;, 2004.</mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple">Kittelson, D. B.: Engines and nanoparticles: a review, J. Aerosol Sci., 29, 575–588, 1998.</mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple">Kovar-Panskus, A., Moulinneuf, L., Savory, E., Abdelqari, A., Sini, J.-F., Rosant, J.-M., Robins, A., and Toy, N.: A wind tunnel investigation of the influences of solar-induced wall heating on the flow regime within a simulated urban street canyon, Water Air  Soil Poll., 2, 555–571, 2002.</mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple">Kumar, P., Garmory, A., Ketzel, M., Berkowicz, R., and Britter, R.: Comparative study of measured and modelled number concentrations of nanoparticles in an urban street canyon, Atmos. Environ., 43, 949–958, 2009.</mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple">Launder, B. E. and Spalding, D. B.: The numerical computation of turbulent flows, Comput. Meth. Appl. Mech. Eng., 3, 269–289, 1974.</mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple">Launder, B. E.: Heat and Mass Transport, in: P. Bradshaw (Editor): Topics in Applied Physics, Turbulence,, Springer, Berlin, Germnay, 12, 231–287, 1978.</mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple">Longley, I. D.: Corrections to a description of turbulence in a trafficked street canyon in Manchester, Atmos. Environ., 38, 4589–4592, 2004.</mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple">Louka, P., Vachon, G., Sini, J. F., Mestayer, P. G., and Rosant, J. M.: Thermal effects on the airflow in a street canyon- Nantes&apos;99 Experimental results and model simulations, Water Air  Soil Poll. Focus, 2, 351–364, 2002.</mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple">Mårtensson, E. M., Nilsson, E. D., Buzorius, G., and Johansson, C.: Eddy covariance measurements and parameterisation of traffic related particle emissions in an urban environment, Atmos. Chem. Phys., 6, 769–785, 2006.</mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple">Martin, C., Longley, I. D., Dorsey, J. R., Thomas, R. M., Gallagher, M. W., and Nemitz, E.: Ultrafine particle fluxes above four major European cities, Atmos. Environ., 43, 4714–4721, 2009.</mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple">Mestayer, P. G., Sini, J.-F. and Jobert, M.: Simulation of the Wall Temperature Influence on Flows and Dispersion within Street Canyons, 3rd International Conference on Air Pollution, Porto Carras, Greece, Computational Mechanics Publication, 1, 109–116, 1995.</mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple">Meroney, R. N., Pavageau, M., Rafailidis, S., and Schatzmann, M.: Study of line source characteristics for 2-D physical modelling of pollutant dispersion in street canyons, J. Wind Eng. Ind. Aerodynam., 62, 37–56, 1996.</mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple">Monin, A. S. and Obukov, A. M.: Basic laws of turbulent mixing in the ground layer of the atmosphere, Acad. Nauk SSSR Tr. Geofiz., Inst., 245, 163–187, 1954.</mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple">Murakami, S.: Current Status and future trends in computational wind engineering, J. Wind Eng. Ind. Aerodynam., 67–68, 3–34, 1997.</mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple">Murena, F., Favale, G., Vardoulakis, S., and Solazzo, E.: Modelling dispersion of traffic pollution in a deep street canyon: Application of CFD and operational models, Atmos. Environ., 43, 2303–2311, 2009.</mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple">Nakamura Y. and Oke T. R.: Wind, temperature and stability conditions in an east-west oriented urban canyon, Atmos. Environ., 22, 2691–2700, 1988.</mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple">Oliveria Panão, M. J. N., Gonçlaves, H. J. P., and Ferrão, P. M. C.: Numerical analysis of the street canyon thermal conductance to improve urban design and climate, Build. Environ., 44, 177–187, 2008.</mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple">Patankar, S. V.: Numerical Heat Transfer and Fluid Flow, McGraw-Hill, NY, USA, 197 pp., 1980.</mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple">Savory, E., Rotach, M. W., Chauver, C., Guilloteau, E., Kaster-Klein, P., Kovar-Panskus, A., Louka, P., Sahm, P., and Castelli, S. T.: Street architecture and air quality in Optimisation of Modelling Methods for Traffic Pollution in Street, Final Report for EU Trapos Project, edited by: Berkowicz, R., Britter, R., and Sabatino, S. D., Chapter 1.1, 8–24, available online at: &lt;a href=&quot;http://www2.dmu.dk/AtmosphericEnvironment/trapos/TheBook/TRAPOS_Book.pdf&quot;&gt;http://www2.dmu.dk/AtmosphericEnvironment/trapos/TheBook/TRAPOS_Book.pdf&lt;/a&gt;, 2004.</mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple">Schuepp, P. H., Leclerc, M. Y., MacPherson, J. I., and Desjardins, R. L.: Footprint Prediction of Scalar Fluxes. From Analytical Solutions of the Diffusion Equation, Bound.-Lay. Meteorol., 50, 355–373, 1990.</mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple">Sini, J.-F., Anquetin, S., and Mestayer, P. G.: Pollutant dispersion and thermal effects in urban street canyon, Atmos. Environ., 30, 2659–2677, 1996.</mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple">Solazzo, E. and Britter, R. E.: Transfer processes in a simulated urban street canyon. Bound.-Lay. Meteorol., 124, 43–60, 2007.</mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple">Spalding, D. B.: Concentration fluctuations in a round turbulent free jet, J. Chem. Eng. Sci., 26, 95–107, 1971.</mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple">Tominaga, Y. and Stathopoulos, T.: Turbulent Schmidt numbers for CFD analysis with various types of flowfield, Atmos. Environ., 41, 8091–8099, 2007.</mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple">Versteeg, H. K. and Malalasekera, W: An Introduction to CFD. The Finite Volume Method, 2nd edn., Longman, London, UK, 2007.</mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple">Walton, A. and Cheng A. Y. S.: Large-eddy simulation of pollution dispersion in an urban street canyon–Part II: idealised canyon simulation, Atmos. Environ., 36, 3615–3627, 2002.</mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple">Whitby, E. R., McMurry, P. H., Shankar, U., and Binkowski, F. S.: Modal Aerosol Dynamics Modeling, Rep. 600/3-91/020, Atmospheric Research and Exposure Assessment Laboratory, US Environmental Protection Agency, Research Triangle Park, NC, available as NTIS PB911617291AS from National Technical Information Service, Springfield, VA, USA, 1991.</mixed-citation>
</ref>
</ref-list>
</back>
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